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At least 145 records · Page 8

CO2 response screen in grass Brachypodium reveals the key role of a MAP kinase in CO2-triggered stomatal closure

Abstract Plants respond to increased CO2 concentrations through stomatal closure, which can contribute to increased water use efficiency. Grasses display faster stomatal responses than eudicots due to dumbbell-shaped guard cells flanked by subsidiary cells working in opposition. However, forward genetic screening for stomatal CO2 signal transduction mutants in grasses has yet to be reported. The grass model Brachypodium distachyon is closely related to agronomically important cereal crops, sharing largely collinear genomes. To gain insights into CO2 control mechanisms of stomatal movements in grasses, we developed an unbiased forward genetic screen with an EMS-mutagenized B. distachyon M5 generation population using infrared imaging to identify plants with altered leaf temperatures at elevated CO2. Among isolated mutants, a “chill1” mutant exhibited cooler leaf temperatures than wild-type Bd21-3 parent control plants after exposure to increased CO2. chill1 plants showed strongly impaired high CO2-induced stomatal closure despite retaining a robust abscisic acid-induced stomatal closing response. Through bulked segregant whole-genome sequencing analyses followed by analyses of further backcrossed F4 generation plants and generation and characterization of sodium azide and CRISPR-cas9 mutants, chill1 was mapped to a protein kinase, Mitogen-Activated Protein Kinase 5 (BdMPK5). The chill1 mutation impaired BdMPK5 protein-mediated CO2/HCO3− sensing together with the High Temperature 1 (HT1) Raf-like kinase in vitro. Furthermore, AlphaFold2-directed structural modeling predicted that the identified BdMPK5-D90N chill1 mutant residue is located at the interface of BdMPK5 with the BdHT1 Raf-like kinase. BdMPK5 is a key signaling component that mediates CO2-induced stomatal movements and is proposed to function as a component of the primary CO2 sensor in grasses.

Lopez, Bryn N. K. (ORCID:0009000937288216)↗

Particle Acceleration in Collisionless Magnetically Arrested Disks

We present the first collisionless realization of two-dimensional axisymmetric black hole accretion consistent with a persistent magnetically arrested disk state. The accretion flow, consisting of an ion-electron disk plasma combined with magnetospheric pair creation effects, is simulated using first-principles general-relativistic particle-in-cell methods. The simulation is evolved over significant dynamical timescales during which a quasisteady accretion state is reached with several magnetic flux eruption cycles. We include a realistic treatment of inverse Compton scattering and pair production, which allows for studying the interaction between the collisionless accretion flow and pair-loaded jet. Our findings indicate that magnetic flux eruptions associated with equatorial magnetic reconnection within the black hole magnetosphere and the formation of spark gaps are locations of maximal particle acceleration. Flux eruptions, starting near the central black hole, can trigger Kelvin-Helmholtz-like vortices at the jet-disk interface that facilitate efficient mixing between disk and jet plasma in this region. Transient periods of increased pair production following magnetic flux eruptions and reconnection events are responsible for most of the highly accelerated particles.

Accretion disk & black-hole plasma↗

CHEETAH: Compact High Efficiency Electrically Tunable Amplifier (Abbreviated Final Report)

The goal of this project was to develop a new type of optically triggered, high speed and high power switch for radiofrequency applications with potential to exceed current state-of-the-art power and bandwidth. This device operates under a new operation principle, where discrete packets of charge carriers are generated with defined size. These are then swept out of the device at high enough fields to prevent diffusion and expansion of these packets. Individual pulse width are determined by the spatial extent of these packets and their drift velocity, which would enable control over both amplitude and frequency by control of the initial packet size, illumination intensity, and applied voltage. This effort demonstrated this new mode of operation, while uncovering a new regime of pulse compression using negative differential mobility (NDM) semiconductors such as GaAs, where the output electrical pulse is substantially shorter than the input optical pulse.

42 ENGINEERING↗

X-ray sources in regions of star formation. 5: The low mass stars of the Upper Scorpius association

We report followup investigations of Einstein x-ray observations of the Upper Scorpius OB association. We identify 28 low mass pre-main sequence stars as counterparts of x-ray sources in the approximately = 7 square degrees of the OB association observed. Based on kinematics and lithium abundances, these stars are low mass members of the OB association. We use optical spectra and optical and near-IR photometry to determine the stellar luminosities, effective temperatures, masses, and ages. We show that the bolometric corrections and effective temperatures of the G and K stars are consistent with those of subgiants. The low mass stars have isochronal ages of 1-2 Myr, depending on the choice of evolutionary models, with very small dispersion (sigma approximately = 1 Myr). This age is significantly younger than the 5-6 Myr found for the more massive B stars. The small dispersion in stellar ages, less than 10% the sound-crossing time of the association, suggests that star formation was triggered. We present two scenarios for star formation in this association. In the two-episode scenario, formation of the low mass stars was triggered by a supernova explosion, and the low mass stars form quickly, with high efficiency. Alternatively, high and low mass star formation was all initiated at the same time, some 5-6 Myr ago, and the apparent systematic age difference is an artifact of how the isochrones are dated. The effect of the supernova is to terminate mass accretion and yield an apparently coeval population. We show that the incompleteness in the x-ray sampling is about 65%, and is strongly dependent on stellar mass. After correction for incompleteness, we estimate there are about 2000 low mass members (stellar mass less than 2 solar mass) of this association. The mass function in this association is indistinguishable from that of the field. The ratio of naked to classical T Tauri stars is much larger than in Tau-Aur, and may be attributable to the local environment. We also present observations of eight ROX sources associated with the rho Oph cloud, and observations of non-pre-main sequence (PMS) stars in our fields.

Walter, Frederick M.↗

Inferring the spatial and energy distribution of gamma-ray burst sources. 1: Methodology

We describe Bayesian methods for analyzing the distribution of gamma-ray burst peak photon fluxes and directions. These methods fit the differential distribution, and have the following advantages over rival methods: (1) they do not destroy information by binning or averaging the data (as do, say, chi squared, the averaged value of V/V(sub max), and angular moment analyses); (2) they straightforwardly handle uncertainties in the measured quantities; (3) they analyze the strength and direction information jointly; (4) they use information available about nondetections; and (5) they automatically identify and account for biases and selection effects given a precise description of the experiment. In these methods, the most important information needed about the instrument threshold is not its value at the times of burst triggers, as is used in the average value of V/V(sub max) analyses, but rather the value of the threshold at times when no trigger occurred. We show that this information can be summarized as an average detection efficiency that is similar to the product of the exposure and efficiency reported in the First Burst and Transient Source Experiment (BATSE) Burst (1B) Catalog, but significantly different from it at low fluxes. We also quantify an important bias that results from estimating the peak flux by scanning the burst to find the peak number of counts in a window of specified duration, as was done for the 1B Catalog. When the duration of the peak of the light curve is longer than the window duration, a simple flux estimate based on the peak counts significantly overestimates the peak flux in a nonlinear fashion that distorts the shape of the log(N)-log(P) distribution. This distortion also corrupts analyses of the V/V(sub max) distribution that use ratios of counts above background to estimate V/V(sub max). The Bayesian calculation specifies how to account for this bias. Implementation of the Bayesian approach requires some changes in the way burst data are reported that we describe in detail. Subsequent papers will report analyses of the 1B Catalog data using the methods described here.

Loredo, Thomas J.↗

Fast b -tagging at the high-level trigger of the ATLAS experiment in LHC Run 3

The ATLAS experiment relies on real-time hadronic jet reconstruction and b-tagging to record fully hadronic events containing b-jets. These algorithms require track reconstruction, which is computationally expensive and could overwhelm the high-level-trigger farm, even at the reduced event rate that passes the ATLAS first stage hardware-based trigger. In LHC Run 3, ATLAS has mitigated these computational demands by introducing a fast neural-network-based b-tagger, which acts as a low-precision filter using input from hadronic jets and tracks. It runs after a hardware trigger and before the remaining high-level-trigger reconstruction. This design relies on the negligible cost of neural-network inference as compared to track reconstruction, and the cost reduction from limiting tracking to specific regions of the detector. In the case of Standard Model HH → bb̅bb̅, a key signature relying on b-jet triggers, the filter lowers the input rate to the remaining high-level trigger by a factor of five at the small cost of reducing the overall signal efficiency by roughly 2%.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Ballistic Ejection of Microdroplets from Overpacked Interfacial Assemblies

Spontaneous emulsification, resulting from the assembly and accumulation of surfactants at liquid–liquid interfaces, is an interfacial instability where microdroplets are generated and diffusively spread from the interface until complete emulsification. Here, it is shown that an external magnetic field can modulate the assembly of paramagnetic nanoparticle surfactants (NPSs) at liquid–liquid interfaces to trigger an oversaturation in the areal density of the NPSs at the interface, as evidenced by a marked reduction in the interfacial tension, γ, and corroborated with a magnetostatic continuum theory. Despite the significant reduction in γ, the presence of the magnetic field does not cause stable interfaces to become unstable. Upon rapid removal of the field, however, an explosive ejection of a plume of microdroplets from the surface occurs, a dynamical interfacial instability which is termed explosive emulsification. Further, this explosive event rapidly reduces the areal density of the NPSs to its pre-field level, stabilizing the interface. The ability to externally suppress or trigger the explosive emulsification and controlled generation of tens of thousands of microdroplets, uncovers an efficient energy storage and release process, that has potential applications for controlled and directed delivery of chemicals and remotely controlled soft microrobots, taking advantage of the ferromagnetic nature of the microdroplets.

36 MATERIALS SCIENCE↗

Probing Ultrafast Charge Transfer Dynamics in Heterostructured Nanomaterials

The increasing demand for renewable and low‐cost energy has triggered a vast amount of research aimed at developing, characterizing and optimizing materials that can efficiently convert sun light into useful chemical energy in the form of electricity or chemical fuels. So‐ called quantum dot sensitized solar cell (QDSC) materials have gained much attention in recent years based on the advantageous physicochemical properties of semiconducting quantum dots (QDs) as sensitizers, as well as their promising potential to increase the conversion efficiency beyond the Shockley‐Queisser limit of ∼33% by making use of hot‐electron transfer (HET) routes and multiple exciton generation (MEG). By finely tuning the size of the QDs, the band gap can be carefully aligned to the metal oxide (MO) conduction band such that charge transfer from the photoexcited QD is thermodynamically favorable.

14 SOLAR ENERGY↗

The Trigger System of ICARUS-T600 Detector at Fermilab

The ICARUS-T600 liquid argon (LAr) time projection chamber (TPC) detector is currently deployed as a far detector of the Short Baseline Neutrino (SBN) program at Fermilab (USA) to search for a possible LSND-like sterile neutrino signal at $\Deltam^2 \approx 1eV^2$ with the Booster (BNB) and Main Injector (NuMI) Neutrino Beams. A global physical event rate of $\approx 0.6$ Hz, including the genuine neutrino interactions in LAr, beam halos and cosmic interactions inside the proton pulse time windows, is expected, roughly corresponding to $\approx 4$ PB of data for the total 6.6 $10^{20}$ pot exposure if the full ICARUS-T600 detector is readout ($\approx 200$ MB event size). The designed trigger system described here will collect the genuine neutrino interactions with a $\approx 95$\% expected efficiency.

Copello, S. [INFN, Pavia]↗

Rapid Inference of Logic Gate Neural Networks for Anomaly Detection in High Energy Physics

The increasing data rates and complexity of detectors at the Large Hadron Collider (LHC) necessitate fast and efficient machine learning models, particularly for rapid selection of what data to store, known as triggering. Building on recent work in differentiable logic gates, we present a public implementation of a Convolutional Differentiable Logic Gate Neural Network (CLGN). We apply this to detecting anomalies at the Level-1 Trigger at CMS using public data from the CICADA project. We demonstrate that the CLGN achieves physics performance on par with or superior to conventional quantized neural networks. We also synthesize an LGN for a Field-Programmable Gate Array (FPGA) and show highly promising FPGA characteristics, notably zero Digital Signal Processor (DSP) resource usage. This work highlights the potential of logic gate networks for high-speed, on-detector inference in High Energy Physics and beyond.

FOS: Physical sciences↗

Fuel transfer system permits rapid coupling

Docking and fuel transfer system provides an efficient method for transferring fuel from a tanker to another vehicle. With this system, no triggering operation is required prior to docking, the support system can be rigidized by simply locking the rams of shock absorbers, and no separate fuel line coupling action is required.

West, A. M.↗

Effects of Shocks on Emission from Central Engines of Active Galactic Nuclei. I

In this paper we show that perturbations of the accretion flow within the central engines of some active galactic nuclei (AGNS) are likely to form shock waves in the accreting plasma. Such shocks, which may be either collisional or collisionless, can contribute to the observed high-energy temporal and spectral variability. Our rationale is the following: Observations show that the continuum emission probably originates in an optically thin, hot plasma in the AGN central engine. The flux and spectrum from this hot plasma varies significantly over light crossing timescales. Several authors have suggested that macroscopic perturbations contained within this plasma are the sources of this variability. In order to produce the observed emission the perturbations must be radiatively coupled with the optically thin hot matter and must also move with high velocities. We suggest that shocks, which can be very effective in randomizing the bulk motion of the perturbations, are responsible for this coupling. Shocks should form in the central engine, because the temperatures and magnetic fields are probably reduced below their virial values by radiative dissipation. Perturbations moving at Keplerian speeds, or strong non-linear excitations, result in supersonic and super-Alfvenic velocities leading to shock waves within the hot plasma. We show that even a perturbation smaller than the emitting region can form a shock that significantly modifies the continuum emission in an AGN, and that the spectral and temporal variability from such a shock generally resembles those of radio-quiet AGNS. As an example, the shock inducing perturbation in our model is a small main-sequence star, the capturing and eventual accretion of which are known to be a plausible process. We argue that shocks in the central engine may also provide a natural triggering mechanism for the "cold" component of Guilbert & Rees two-phase medium and an efficient mecha- nism for angular momentum transfer. Current and future missions, such as ASCA, XTE, XMM, AXAF, and ASTRO-E may determine the importance of shock-related emission from the central engines of AGNS.

Sivron, R.↗

SPLENDAQ: A Detector-Agnostic Data Acquisition System for Small-Scale Physics Experiments

Many scientific applications from rare-event searches to condensed matter system characterization to high-rate nuclear experiments require time-domain triggering on a raw stream of data, where the triggering is generally threshold-based or randomly acquired. When carrying out detector R &D, there is a need for a general data acquisition (DAQ) system to quickly and efficiently process such data. In the SPLENDOR collaboration, we are developing the Python-based SPLENDAQ package for this exact purpose—it offers two main features for offline analysis of continuous data: a threshold triggering algorithm based on the time-domain optimal filter formalism and an algorithm for randomly choosing nonoverlapping segments for noise measurements. Further, combined with the commercially available Moku platform, developed by Liquid Instruments, we have a full pipeline of event building off raw data with minimal setup. Here, we review the underlying principles of this detector-agnostic DAQ package and give concrete examples of its utility in various applications.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Trigger Detection for the sPHENIX Experiment via Bipartite Graph Networks with Set Transformer

Trigger (interesting events) detection is crucial to high-energy and nuclear physics experiments because it improves data acquisition efficiency. It also plays a vital role in facilitating the downstream offline data analysis process. The sPHENIX detector, located at the Relativistic Heavy Ion Collider in Brookhaven National Laboratory, is one of the largest nuclear physics experiments on a world scale and is optimized to detect physics processes involving charm and beauty quarks. Furthermore, these particles are produced in collisions involving two proton beams, two gold nuclei beams, or a combination of the two and give critical insights into the formation of the early universe. This paper presents a model architecture for trigger detection with geometric information from two fast silicon detectors. Transverse momentum is introduced as an intermediate feature from physics heuristics. We also prove its importance through our training experiments. Each event consists of tracks and can be viewed as a graph. A bipartite graph neural network is integrated with the attention mechanism to design a binary classification model. Compared with the state-of-the-art algorithm for trigger detection, our model is parsimonious and increases the accuracy and the AUC score by more than 15%.

97 MATHEMATICS AND COMPUTING↗

Efficient Oxidative Decomposition of Jet-Fuel exo -Tetrahydrodicyclopentadiene (JP-10) by Aluminum Nanoparticles in a Catalytic Microreactor: An Online Vacuum Ultraviolet Photoionization Study

The oxidation of gas-phase exo-tetrahydrodicyclopentadiene (JP-10, C 10 H 16 ) over aluminum nanoparticles (AlNP) has been explored between a temperature range of 300 and 1250 K with a novel chemical microreactor. The results are compared with those obtained from chemical microreactor studies of helium-seeded JP-10 and of helium–oxygen-seeded JP-10 without AlNP to gauge the effects of molecular oxygen and AlNP, respectively. Vacuum ultraviolet (VUV) photoionization mass spectrometry reveals that oxidative decomposition of JP-10 in the presence of AlNP is lowered by 350 and 200 K with and without AlNP, respectively, in comparison with pyrolysis of the fuel. Overall, 63 nascent gas-phase products are identified through photoionization efficiency (PIE) curves; these can be categorized as oxygenated molecules and their radicals as well as closed-shell hydrocarbons along with hydrocarbon radicals. Quantitative branching ratios of the products reveal diminishing yields of oxidized species and enhanced branching ratios of hydrocarbon species with the increase in temperature. While in the low-temperature regime (300–1000 K), AlNP solely acts as an efficient heat transfer medium, in the higher-temperature regime (1000–1250 K), chemical reactivity is triggered, facilitating the primary decomposition of the parent JP-10 molecule. Furthermore, this enhanced reactivity of AlNP could plausibly be linked to the exposed reactive surface of the aluminum (Al) core generated upon the rupture of the alumina shell material above the melting point of the metal (Al).

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Free-standing membrane incorporating single-atom catalysts for ultrafast electroreduction of low-concentration nitrate

The release of wastewaters containing relatively low levels of nitrate (NO 3 ⁻) results in sufficient contamination to induce harmful algal blooms and to elevate drinking water NO 3 ⁻ concentrations to potentially hazardous levels. In particular, the facile triggering of algal blooms by ultra-low concentrations of NO 3 ⁻ necessitates the development of efficient methods for NO 3 ⁻ destruction. However, promising electrochemical methods suffer from weak mass transport under low reactant concentrations, resulting in long treatment times (on the order of hours) for complete NO 3 ⁻ destruction. In this study, we present flow-through electrofiltration via an electrified membrane incorporating nonprecious metal single-atom catalysts for NO 3 ⁻ reduction activity enhancement and selectivity modification, achieving near-complete removal of ultra-low concentration NO 3 ⁻ (10 mg-N L -1 ) with a residence time of only a few seconds (10 s). By anchoring Cu single atoms supported on N-doped carbon in a carbon nanotube interwoven framework, we fabricate a free-standing carbonaceous membrane featuring high conductivity, permeability, and flexibility. The membrane achieves over 97% NO 3 ⁻ removal with high N 2 selectivity of 86% in a single-pass electrofiltration, which is a significant improvement over flow-by operation (30% NO 3 ⁻ removal with 7% N 2 selectivity). This high NO 3 ⁻ reduction performance is attributed to the greater adsorption and transport of nitric oxide under high molecular collision frequency coupled with a balanced supply of atomic hydrogen through H 2 dissociation during electrofiltration. Overall, our findings provide a paradigm of applying a flow-through electrified membrane incorporating single-atom catalysts to improve the rate and selectivity of NO 3 ⁻ reduction for efficient water purification.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Developing new analysis tools for near surface radio-based neutrino detectors

The ARIANNA experiment is an Askaryan radio detector designed to measure high-energy neutrino induced cascades within the Antarctic ice. Ultra-high-energy neutrinos above 10 16 eV have an extremely low flux, so experimental data captured at trigger level need to be classified correctly to retain as much neutrino signal as possible. We first describe two new physics-based neutrino selection methods, or "cuts", (the updown and dipole cut) that extend the previously published analysis to a specialized ARIANNA station with 8 antenna channels, which is double the number used in the prior analysis. For a standard trigger with a threshold signal to noise ratio at 4.4, the new cuts produce a neutrino efficiency of > 95% per station-year of operation, while rejecting 99.93% of the background (corresponding to 53 remaining experimental background events). When the new cuts are combined with a previously developed cut using neutrino waveform templates, all background is removed at no change of efficiency. In addition, the neutrino efficiency is extrapolated to 1,000 station-years of operation, obtaining 91%. This work then introduces a new selection method (the deep learning cut) to augment the identification of neutrino events by using deep learning methods and compares the efficiency to the physics-based analysis. The deep learning cut gives 99% signal efficiency per station-year of operation while rejecting 99.997% of the background (corresponding to 2 remaining experimental background events), which are subsequently removed by the waveform template cut at no significant change in efficiency. Here the results of the deep learning cut were verified using measured cosmic rays which shows that the simulations do not introduce artifacts with respect to experimental data. The paper demonstrates that the background rejection and signal efficiency of near surface antennas meets the requirements of a large scale future array, as considered in baseline design of the radio component of IceCube-Gen2.

97 MATHEMATICS AND COMPUTING↗

Unraveling the Luminescence Quenching Mechanism in Strong and Weak Quantum-Confined CsPbBr 3 Triggered by Triarylamine-Based Hole Transport Layers

Luminescence quenching by hole transport layers (HTLs) is one of the major issues in developing efficient perovskite light-emitting diodes (PeLEDs), particularly prominent in blue-emitting devices. While a variety of material systems have been used as interfacial layers, the origin of such quenching and the type of interactions between perovskites and HTLs are still ambiguous. Here, we present a systematic investigation of the luminescence quenching of CsPbBr 3 by a commonly employed hole transport polymer, Poly(9,9-dioctylfluorene-alt-N-(4-sec-butylphenyl)-diphenylamine) (TFB) in LEDs. Strong and weakly quantum-confined CsPbBr 3 (nanoplatelets (NPLs)/nanocrystals (NCs)) are rationally selected to study the quenching mechanism by considering the differences in their morphology, energy level alignments, and quantum confinement. The steady-state and time-resolved Stern-Volmer plots unravel the dominance of dynamic and static quenching at lower and higher concentrations of TFB, respectively, with maximum quenching efficiency of 98%. The quenching rate in NCs is faster than in NPLs owing to their longer PL lifetimes and weak quantum confinement. The ultrafast transient absorption results support these dynamics and rule out the involvement of Forster or Dexter energy transfer. Finally, the 1D 1 H and 2D NOESY NMR study confirms the exchange of native ligands at the NCs surface with TFB, leading to dark CsPbBr 3 -TFB ensemble formation accountable for luminescence quenching. This highlights the critical role of the triarylamine functional group on TFB (also the backbone of many HTLs) in the quenching process. These results shed light on the underlying reasons for the luminescence quenching in PeLEDs and will help to choose the interfacial layers rationally for developing efficient LEDs.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗