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NASA NTRS1983

10 micron polarimetry of Ceres

Linear polarimetry of Ceres at 10 micron is presented. These data represent the first published polarization measurements of an asteroid in the thermal infrared. It is found that Ceres is polarized at the 0.2-0.6 percent level. This data set is compared with theoretical models of the linear polarization of emitted radiation from a spherical plane. These models are used to derive the pole position and thermal inertia of Ceres. Ceres is best fit with a thermal inertia of 0.0010 + or 0.0003 cal (sq cm K) per square root of second and a pole orientation of beta(p) = 36 deg + or - 5 deg + or -5, lambda(p) = 270 deg + or - 3. It is concluded that 10 micron polarimetry is a potentially powerful technique for remotely sensing the pole orientation and thermal inertia of asteroids.

Johnson, P. E.↗

NASA NTRS1987

Tidal estimation in the Pacific with application to SEASAT altimetry

The techniques for computing the eigenfunctions of the velocity potential (Proudman functions) set out in Sanchez, et al. (1986) in relation to the Atlantic-Indian Oceans are here applied to the Pacific Ocean, using a 6x6 degree grid of 510 points (455 points for the associated stream functions). Normal modes are computed from the first Proudman functions and have natural periods from 43.9h downward. Tidal syntheses are derived from these modes by direct application of the (frictionless) dynamic equations and by least-squares fitting of Proudman functions to the dynamically interpolated tide-gauge data of Schwiderski (1983). The modes contributing the most energy to the principal harmonic tidal constituents are different in the two computations: their natural periods are typically in the range of 9 to 16h for semidiurnal, and 14 to 43h for diurnal tides. The rms of fit for the Proudman functions is, in all cases, better than the corresponding value for the same number of spherical harmonics.

Sanchez, Braulio V.↗

DOE OSTI2021

Re-Analysis of DARHT Axis 2 S4 Magnet Sweep Measurements

The Dual-Axis Radiographic Hydrodynamic Test (DARHT) facility provides flash radiography capabilities using two electron Linear Induction Accelerators (LIA’s). Understanding fundamental properties of the electron beams is essential to optimizing spot size and dose for radiography. This work describes distribution measurements of a single-kicked electron beam (16.5MeV, 1.7kA, 60ns) at a location downstream at imaging station C on DARHT Axis 2. The beam at station C is focused by the S4 solenoid located upstream. The beam distribution is measured by imaging optical transition radiation (OTR) from electrons striking a 51-µm thick titanium foil. This data and analysis were originally published by Ekdahl. The results here are a re-analysis of the asymmetric halo emittance contribution as compared to the emittance resulting from the FWHM of the distribution. This is accomplished using xtr2 fits to the data which include non-linear magnetic field effects in S4. Also examined are the calculated S4 spherical aberration contributions to the emittance using xtr.

43 PARTICLE ACCELERATORS↗

NASA NTRS1974

Optical polarization measurements of the Jupiter atmosphere at 103 deg phase angle

The first measurements have been made of the linear polarization of sunlight scattered by the Jupiter atmosphere at phase angles greater than 12 deg, using the imaging photopolarimeter on Pioneer 10. The data are of high accuracy, in spite of several problems in the instrument. The polarization is positive at 440 nm. There is no direct evidence for spherical particles in the Jupiter clouds. Using a simple model of Rayleigh scattering above a Lambertian cloud layer, a unique fit is found to the observed intensity and polarization at each point on the planet. The resulting Rayleigh optical depths, if they are attributed to molecular scattering alone (i.e., no aerosols above the cloud tops), can be converted into physical altitudes of the cloud tops. The first results suggest that the north tropical zone, parts of the equatorial zone, and the red spot are all elevated regions.

Coffeen, D. L.↗

NASA NTRS2005

Hybrid Systems Diagnosis

This paper reports on an on-going Project to investigate techniques to diagnose complex dynamical systems that are modeled as hybrid systems. In particular, we examine continuous systems with embedded supervisory controllers that experience abrupt, partial or full failure of component devices. We cast the diagnosis problem as a model selection problem. To reduce the space of potential models under consideration, we exploit techniques from qualitative reasoning to conjecture an initial set of qualitative candidate diagnoses, which induce a smaller set of models. We refine these diagnoses using parameter estimation and model fitting techniques. As a motivating case study, we have examined the problem of diagnosing NASA's Sprint AERCam, a small spherical robotic camera unit with 12 thrusters that enable both linear and rotational motion.

McIlraith, Sheila↗

NASA NTRS2015

Experimental, Numerical and Analytical Characterization of Slosh Dynamics Applied to In-Space Propellant Storage, Management and Transfer

Experimental and numerical results are presented from a new cryogenic fluid slosh program at the Florida Institute of Technology (FIT). Water and cryogenic liquid nitrogen are used in various ground-based tests with an approximately 30 cm diameter spherical tank to characterize damping, slosh mode frequencies, and slosh forces. The experimental results are compared to a computational fluid dynamics (CFD) model for validation. An analytical model is constructed from prior work for comparison. Good agreement is seen between experimental, numerical, and analytical results.

slosh↗

NASA NTRS2015

Experimental, Numerical and Analytical Characterization of Slosh Dynamics Applied to In-Space Propellant Storage, Management and Transfer

slosh mode frequencies↗

NASA NTRS2010

Evaluating Descent and Ascent Trajectories Near Non-Spherical Bodies

Spacecraft landing on small bodies pass through regions where conventional gravitation formulations using exterior spherical harmonics are inaccurate. An investigation shows that a formulation using interior solid spherical harmonics might be satisfactory. Interior spherical harmonic expansions are usable inside an imaginary, empty sphere. For this application, such a sphere could be positioned in empty space above the intended landing site and rotating with the body. When the spacecraft is inside this sphere, the interior harmonic expansion would be used instead of the conventional, exterior harmonic expansion. Coefficients can be determined by a least-squares fit to gravitation measurements synthesized from conventional formulations. Due to their unfamiliarity, recurrences for interior, as well as exterior, expansions are derived. Hotine's technique for partial derivatives of exterior spherical harmonics is extended to interior harmonics.

Werner, Robert A.↗

DOE OSTI2023

Calorimetric Energies and Chemical Potentials of Metal Atoms in Catalytic Nanoparticles on Oxide and Carbon Supports: Improved Size Dependencies and Adhesion Energies

The chemical potential of metal atoms, μM, in supported metal nanoparticles is an important descriptor related to both the catalytic activity and the stability of the nanoparticles. Here, we derive an expression relating μM to the radius of the particle’s contact area with the support and the adhesion energy at the metal/support interface (E adh ) that assumes the particles have the shape of spherical caps but of arbitrary contact angle with the support (θ c ) and includes an empirical correction for the increase in metal surface energy and adhesion energy with decreasing radius of curvature. We then show that, at any assumed contact angle, we can simultaneously fit previously reported measurements of both calorimetric μ M (from heats of metal vapor adsorption during nanoparticle growth by vapor deposition) versus metal coverage data and the He + low-energy ion scattering (LEIS) intensities for the metal and/or support versus metal coverage (using our recently developed spherical cap model for quantitative LEIS intensities), to determine the particle size versus coverage and E adh . Only one choice of contact angle gives a pair of values for contact angle and E adh , which is consistent with the Young–Dupré equation for the equilibrium shape of a spherical particle. At this equilibrium shape, we then applied this spherical cap model (SCM) to reanalyze microcalorimetric metal chemical potentials and LEIS signals versus coverage data for nine metal/support combinations that were previously analyzed by assuming that the particles had the shape of hemispherical caps, i.e., with a contact angle of 90°. We show that this revised approach gives close agreement with the calorimetric and LEIS data; the best-fit contact angles vary from 64 to 84°, correcting the earlier assumption of 90°. Furthermore, these results provide significant accuracy improvements in particle size versus coverage, metal chemical potential versus size and coverage, metal/support adhesion energies and contact angles for Cu, Ag and Au on CeO 2 (111), Ni on MgO(100), Ag on Fe 3 O 4 (111) and TiO 2 (100), and Ag, Ni and Pd on Ni-supported graphene. This revised approach is much more broadly applicable than the earlier hemispherical cap model (HCM).

99 GENERAL AND MISCELLANEOUS↗

DOE OSTI2022

Study of the deformed halo nucleus 31 Ne with Glauber model based on microscopic self-consistent structures

In this work, the exotic deformed nucleus 31 Ne is studied with an approach that combines self-consistent structure and reaction theories. The deformed relativistic Hartree-Bogoliubov theory in continuum (DRHBc) is utilized to demonstrate that deformation and pairing correlations give rise to a halo structure with a large-amplitude p-wave configuration in 31 Ne. Then the valence nucleon wave functions and angle-averaged density distributions of 30 Ne from this theory are used as input for the Glauber reaction model to study the observables of neutron-rich neon isotopes to search halo signatures. With NL1 effective interaction, our predictions of the reaction cross sections for these exotic neon isotopes on a carbon target can better reproduce the experimental data than those from the relativistic mean field model for a spherical shape with resonances and pairing correlation contributions, and are roughly 3.3% (~ 50 mb) larger than those with Gaussian function-fitted densities of the core nuclei. The calculated one-neutron removal cross section at 240 MeV/nucleon, and the inclusive longitudinal momentum distribution of the 30 Ne residues from the 31Ne breakup reaction are largely improved over previous theoretical predictions and agree well with data. These reaction evaluations indicate a dilute density distribution in coordinate space and are a canonical signature of a halo structure. Moreover, our predictions with the NL3 and PK1 effective interactions give slightly better descriptions of reaction observables for exotic neon isotopes.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2025

Spherical and sessile droplet dynamics by fluctuating hydrodynamics

We simulate the mesoscopic dynamics of droplets formed by phase-separated fluids at nanometer scales where thermal fluctuations are significant. Both spherical droplets fully immersed in a second fluid and sessile droplets which are also in contact with a solid surface are studied. Our model combines a Cahn–Hilliard formulation with incompressible fluctuating hydrodynamics; for sessile droplets, the fluid–solid contact angle is specified as a boundary condition. Deterministic simulations with an applied body force are used to measure the droplets' mobility from which a diffusion coefficient is obtained using the Einstein relation. Stochastic simulations are independently used to obtain a diffusion coefficient from a linear fit of the variance of a droplet's position with time. In some scenarios, these two measurements give the same value but not in the case of a spherical droplet initialized near a slip wall or in the case of sessile droplets with large contact angles (≥90°) on both slip and no-slip surfaces.

Bell, John B↗

NASA NTRS1995

Improved Bounds on Nonluminous Matter in Solar Orbit

We improve, using a larger set of observations including Voyager 2 Neptune flyby data, previous bounds on the amount of dark matter (DM) trapped in a spherically symmetric distribution about the Sun. We bound DM by noting that such a distribution would increase the effective mass of the Sun as seen by the outer planets and by finding the uncertainty in that effective mass for Uranus and Neptune in fits to the JPL developmental ephemeris residuals, including optical data and those two planets' Voyager 2 flybys. We extend our previous procedure by fitting more parameters of the developmental ephamerides. In addition, we present here the values for Pioneer 10, Pioneer 11, Voyager 1, and Voyager 2 Jupiter-ranging normal points (and incorporate these data as well). Our principal result is to limit DM in spherically symmetric distributions in orbit about the Sun interior to Neptune's orbit to less than Earth mass and interior to Uranus's orbit to about 1/6 of Earth's mass.

Anderson, John D.↗

NASA NTRS1979

Development and analysis of a twelfth degree and order gravity model for Mars

Satellite geodesy techniques previously applied to artificial earth satellites have been extended to obtain a high-resolution gravity field for Mars. Two-way Doppler data collected by 10 Deep Space Network (DSN) stations during Mariner 9 and Viking 1 and 2 missions have been processed to obtain a twelfth degree and order spherical harmonic model for the martian gravitational potential. The quality of this model was evaluated by examining the rms residuals within the fit and the ability of the model to predict the spacecraft state beyond the fit. Both indicators show that more data and higher degree and order harmonics will be required to further refine our knowledge of the martian gravity field. The model presented shows much promise, since it resolves local gravity features which correlate highly with the martian topography. An isostatic analysis based on this model, as well as an error analysis, shows rather complete compensation on a global (long wavelength) scale. Though further model refinements are necessary to be certain, local (short wavelength) features such as the shield volcanos in Tharsis appear to be uncompensated. These are interpreted to place some bounds on the internal structure of Mars.

Christensen, E. J.↗

NASA NTRS1995

The effects of redshifts and focusing on the spectrum of an accretion disk in the galactic center black hole candidate Sagittarius A(sup *)

There are firm indications that Sgr A(sup *), a compact, nonthermal radio source at the Galactic center, may be powered by the dissipation of gravitational energy as gas trapped from an ambient wind descends down the potential well, first through a quasi-spherical inflow (extending out to approximately 3 x 10(exp 16) cm) and then through a small accretion disk at less than or approximately = 5-10 Schwarzschild radii. Earlier three-dimensional Bondi-Hoyle numerical simulations have indicated that fluctuations in the accreted specific angular momentum can lead to a variability in the disk flux on a timescale of years. With greatly improved flux measurements at K and H, and the hint of a approximately 10 minute modulation in the IR luminosity, it is crucial to model the disk emission much more precisely than has been attempted thus far. In this Letter we take into account the effects of Doppler and gravitational redshifts, the light-travel time factor, and the light bending near the black hole to determine the measurable spectrum of Sgr A(sup *) in the increasingly important 10(exp 13) Hz less than or approximately = v less than or approximately = 10(exp 16) Hz frequency range. We find that the relativistic disk spectrum is much softer than its Newtonian counterpart, with a predicted UV flux roughly an order of magnitude smaller than had previously been anticipated. In addition, we find that when the physical conditions in the disk are taken to be consistent with the properties of the quasi-spherical infall (specifically, in terms of the accretion rate and disk size), only a slowly spinning or Schwarzschild black hole appears to fit the observations. Our calculations also reveal that the disk flux is much more weakly dependent on the observer's inclination angle than had been suspected on the basis of earlier Newtonian estimates.

Hollywood, J. M.↗

DOE OSTI2021

Identification of crystal plasticity model parameters by multi-objective optimization integrating microstructural evolution and mechanical data

Crystal plasticity models evolve a polycrystalline yield surface using meso-scale descriptions of deformation mechanisms. The activation of deformation mechanisms is governed by crystallography and a set of model parameters, which are typically calibrated through the fitting of mechanical data such as stress–strain curves and elastic lattice strains. Microstructural data such as phase fractions and texture evolution are used for verifying crystal plasticity parameters. In this study, we use a multi-objective genetic algorithm to identify hardening parameters from flow stress curves with an option to incorporate texture into the optimization approach. Robust, generalized objective functions are developed and used to identify sets of parameters pertaining to dislocation density-based hardening laws in visco-plastic and elasto-plastic self-consistent (VPSC and EPSC) homogenization models. First, the parameters are identified for pure Nb directly from texture using an objective function based on generalized spherical harmonics. Since texture evolution is driven by the relative contribution of active slip systems, the parameters governing the evolution of slip resistance ratios can be recovered from fitting discrete textures at a series of strains. Next, a comprehensive set of load reversal data for dual phase (DP) 780 steel is used to fit a hardening law and a back-stress law in EPSC. Finally, parameters pertaining to a complex hardening law for the evolution of slip and twinning in pure α-Ti are identified. Remarkably, using texture as an objective in combination with stress–strain objectives constrains the model of Ti to fully reproduce not only stress–strain and texture evolution but also hierarchical twinning measurements as a function of initial grain size and texture. Furthermore, given an appropriate model fit to representative experimental texture evolution, underlying twin volume fractions contributing to texture evolution can be predicted.

42 ENGINEERING↗

DOE OSTI2023

Many-Body Potential for Simulating Self-Assembly of Polymer-Grafted Nanoparticles in a Polymer Matrix

Many-body interactions between polymer-grafted nanoparticles (NPs) play a key role in promoting their assembly into low-dimensional structures within polymer melts, even when the particles are spherical and isotropically grafted. However, capturing such interactions in simulations of NP assembly is very challenging because explicit modeling of the polymer grafts and melt chains is highly computationally expensive, even using coarse-grained models. Here, we develop a many-body potential for describing the effective interactions between spherical polymer-grafted NPs in a polymer matrix through a machine-learning approach. The approach involves using permutationally invariant polynomials to fit two- and three-body interactions derived from the potential of mean force calculations. The potential developed here reduces the computational cost by several orders of magnitude, thereby, allowing us to explore assembly behavior over large length and time scales. We show that the potential not only reproduces previously known assembled phases such as 1D strings and 2D hexagonal sheets, which generally cannot be achieved using isotropic two-body potentials, but can also help discover interesting phases such as networks, clusters, and gels. We demonstrate how each of these assembly morphologies intrinsically arises from a competition between two- and three-body interactions. Our approach for deriving many-body effective potentials can be readily extended to other colloidal systems, enabling researchers to make accurate predictions of their behavior and dissect the role of individual interaction energy terms of the overall potential in the observed behavior.

36 MATERIALS SCIENCE↗

DOE OSTI2021

AT2017gfo: Bayesian inference and model selection of multicomponent kilonovae and constraints on the neutron star equation of state

The joint detection of the gravitational wave GW170817, of the short γ-ray burst GRB170817A and of the kilonova AT2017gfo, generated by the the binary neutron star (NS) merger observed on 2017 August 17, is a milestone in multimessenger astronomy and provides new constraints on the NS equation of state. We perform Bayesian inference and model selection on AT2017gfo using semi-analytical, multicomponents models that also account for non-spherical ejecta. Observational data favour anisotropic geometries to spherically symmetric profiles, with a log-Bayes’ factor of ~104, and favour multicomponent models against single-component ones. The best-fitting model is an anisotropic three-component composed of dynamical ejecta plus neutrino and viscous winds. Using the dynamical ejecta parameters inferred from the best-fitting model and numerical–relativity relations connecting the ejecta properties to the binary properties, we constrain the binary mass ratio to q < 1.54 and the reduced tidal parameter to $120\lt \tilde{\Lambda }\lt 1110$. Finally, we combine the predictions from AT2017gfo with those from GW170817, constraining the radius of a NS of 1.4 M ⊙ to 12.2 ± 0.5 km (1σ level). This prediction could be further strengthened by improving kilonova models with numerical-relativity information.

79 ASTRONOMY AND ASTROPHYSICS↗

NASA NTRS1981

Voyager 1 assessment of Jupiter's planetary magnetic field

An estimate of Jupiter's planetary magnetic field is obtained from the Voyager 1 observations of the Jovian magnetosphere. An explicit model for the magnetodisc current system is combined with a spherical harmonic model of the planetary field with both sets of parameters determined simultaneously using a nonlinear generalized inverse methodology. The resulting model fits the observations extremely well throughout the analysis interval (r 20 Jovian radii). The Jovian internal field model obtained from the Voyager 1 data is very similar to the octopole Pioneer 11 models. The best fitting magnetodisc lies in the centrifugal equator, 2/3 of the way between the rotational and magnetic equators, as appropriate for centrifugal loading of the magnetosphere by a cold plasma.

Connerney, J. E. P.↗