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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 145 records · Page 8
All sourcesNASA NTRSDOE OSTI
DOE OSTI2023

Investigating Electric Field and Light Induced Degradation in Perovskite Solar Cells through Nanometer-Scale Potential Imaging

Electric field and light induced degradations in perovskite solar cells were evaluated through nanometer-scale potential imaging across the device by using in-situ Kelvin probe force microscopy (KPFM). We derived the electric field profile from potential profiles at different bias voltages to evaluate the locations and quality of junctions across the device. We found relative changes in electric field peak intensity at the HTL/perovskite and perovskite/ETL interfaces upon stressing devices separately under voltage or light. KPFM results during 12-hour stress/rest cycling under electrical bias show both reversible and irreversible changes in the device's interfacial fields. We also observed change in the electric field profile between control and degraded devices after 100 hours of stress/rest cycling under light. Our results demonstrate how nanometer-scale potential imaging can be used to understand the impacts of external electric fields and light soaking on both irreversible degradation and reversible metastability in perovskite solar cells.

Kelvin probe force microscopy↗
NASA NTRS1981

Solar cell is housed in light-bulb enclosure

Inexpensive, conventional solar-cell module uses focusing principle of electric lamp in reverse to produce electric power from sunlight. Standard outdoor light enclosure provides low-cost housing which concentrates sunlight in solar cell. Unit is capable of producing approximately 1 watt of electric power.

Evans, J. C., Jr.↗
DOE OSTI2020

Influence of Tabula Rasa on Process- and Light-Induced Degradation of Solar Cells Fabricated From Czochralski Silicon

Monocrystalline Si solar cells are fabricated from Czochralski (Cz) Si, which contains 10 17 –10 18 cm -3 oxygen atoms. Cz Si undergoes degradation during high-temperature thermal processing steps, such as dopant diffusion to form the p - n junction. This degradation in the bulk minority carrier lifetime can be related to the formation of oxygen precipitates. We found that a high-temperature annealing process known as tabula rasa (TR) not only mitigates process-induced degradation via oxygen precipitate nuclei dissolution, but also modifies subsequent light-induced degradation. We report on the bulk carrier lifetime of n - and p -type Cz Si after TR, which homogenizes the interstitial oxygen in the bulk Si to its monoatomic form in either an N 2 or O 2 environment. A control sample, which was not subjected to a TR processing step, experienced severe process-induced degradation during a boron emitter thermal budget as oxygen precipitates were formed in the Si bulk. These precipitates could be imaged using photoluminescence. Additionally, samples that underwent a TR processing step prior to the boron emitter thermal budget show efficient gettering of metallic impurities compared to the control sample, which showed a decline in the implied open-circuit voltage after the gettering step. Furthermore, modification of the interstitial oxygen bonding by TR had a strong effect on the light-induced degradation kinetics. Instead of a typically observed monotonic decrease, minority carrier lifetime increases first, followed by a nonmonotonic decrease over a ~20 h period. Finally, we conclude that by modifying the interstitial oxygen bonding via TR pretreatment, p -type Cz Si wafers become substantially resistant to harsh solar cell processes and strongly modified light-induced degradation, which would open alternative ways to mitigate this degradation mechanism.

14 SOLAR ENERGY↗
NASA NTRS2008

Retrievals of Thick Cloud Optical Depth from the Geoscience Laser Altimeter System (GLAS) by Calibration of Solar Background Signal

Laser beams emitted from the Geoscience Laser Altimeter System (GLAS), as well as other space-borne laser instruments, can only penetrate clouds to a limit of a few optical depths. As a result, only optical depths of thinner clouds (< about 3 for GLAS) are retrieved from the reflected lidar signal. This paper presents a comprehensive study of possible retrievals of optical depth of thick clouds using solar background light and treating GLAS as a solar radiometer. To do so we first calibrate the reflected solar radiation received by the photon-counting detectors of GLAS' 532 nm channel, which is the primary channel for atmospheric products. The solar background radiation is regarded as a noise to be subtracted in the retrieval process of the lidar products. However, once calibrated, it becomes a signal that can be used in studying the properties of optically thick clouds. In this paper, three calibration methods are presented: (I) calibration with coincident airborne and GLAS observations; (2) calibration with coincident Geostationary Operational Environmental Satellite (GOES) and GLAS observations of deep convective clouds; (3) calibration from the first principles using optical depth of thin water clouds over ocean retrieved by GLAS active remote sensing. Results from the three methods agree well with each other. Cloud optical depth (COD) is retrieved from the calibrated solar background signal using a one-channel retrieval. Comparison with COD retrieved from GOES during GLAS overpasses shows that the average difference between the two retrievals is 24%. As an example, the COD values retrieved from GLAS solar background are illustrated for a marine stratocumulus cloud field that is too thick to be penetrated by the GLAS laser. Based on this study, optical depths for thick clouds will be provided as a supplementary product to the existing operational GLAS cloud products in future GLAS data releases.

Yang, Yuekui↗
NASA NTRS2023

In-Flight Validation of the Metis Visible-Light Polarimeter Coronagraph on Board Solar Orbiter

Context. The Metis coronagraph is one of the remote sensing instruments of the ESA-NASA Solar Orbiter mission. The goal for the instrument is to enable the study of the solar atmosphere and solar wind by simultaneously acquiring images of the solar corona at two different wavelengths: visible light (VL), within a band ranging from 580 nm to 640 nm, and ultraviolet light, in the HI Lyα 121.6 ± 10 nm. The visible-light channel of the coronagraph includes a polarimeter with electro-optically modulating liquid crystal variable retarders to measure the linearly polarized brightness of the K-corona and derive the electron density. Aims. In this paper, we present the first in-flight validation results of the Metis polarimetric channel together with a comparison to the on-ground calibrations. This paper seeks to validate the first use of an electro-optical device, the liquid crystal-based polarimeter, in deep space and within a hard radiation environment. Methods. We used the orientation of the K-corona’s linear polarization vector during the roll maneuvers of the Space Orbiter spacecraft for the in-flight calibration. Results. The Metis coronagraph on board the Solar Orbiter shows good agreement with the on-ground measurements. The in-flight validation confirms the expected performance of the visible-light channel polarimeter. Furthermore, a comparison between the first polarized brightness value obtained by Metis and the polarized brightness values obtained by the space-based coronagraph LASCO and the ground-based coronagraph K-Cor shows the consistency of the Metis calibrated results.

Sun: corona↗
DOE OSTI2021

3D Bacterial flagella as both synthetic biotemplates and ultrathin spacers for enhanced inter-particle coupling and solar energy harvesting

Linear light-absorbing nanomaterials are ideal for film-based solar harvesting applications as they form porous structures that can maximize the absorption and minimize the reflection of the solar light. Conventional 1D nanochains of plasmonic nanoparticle assemblies can achieve significantly broadened optical absorption through surface plasmon coupling, but their optical bands are still not broad enough to absorb through the solar spectrum and thus are not efficient solar absorbers. Here we discovered first by simulation that 3D structured nanochains of plasmonic nanoparticles presented a remarkably increased optical broadening effect and much longer redshift of the optical peaks due to the enhanced inter-particle coupling effect. Then we fabricated 3D nanochains by assembling gold nanoparticles (AuNPs) around 14 nm ultrathin bionanofibers, the bacterial flagella. Additionally, the ultrathin biotemplates enabled the 3D arrangement of 50 nm AuNPs along the nanofiber with a very small inter-particle gap, allowing the strong coupling of surface plasmons in a 3D manner. Consistent with the theoretical prediction, the 3D nanochains, when assembled into films, could effectively convert nearly the full spectrum of solar energy into heat, which was further efficiently converted into electricity through a thermoelectric generation unit. Our work represents a nanobiomaterial approach to highly efficient solar thermal power generation.

36 MATERIALS SCIENCE↗
DOE OSTI2021

Light-Induced Al Plating on Si for Fabrication of an Ag-Free All-Al Solar Cell

Light-induced electroplating of Al as the front electrode on the n-type emitter of Si solar cells is proposed as a substitute for screen-printed Ag. The advantages and disadvantages of Al over Cu as the front electrode are discussed. The power of a green laser used for patterning of the SiN x antireflection coating is optimized. Conditions for removal of laser damage and contamination on the laser-patterned surface are identified. The effect of plating temperature and post-annealing temperature on Al morphology and resistivity are investigated. Several plating additives are explored to improve the morphology and resistivity of the Al film. Nicotinic acid produces the lowest resistivity of 3.1 μ Ω-cm. However, the lowest contact resistivity between light-induced Al and Si is 69 mΩ-cm 2 due to laser-induced damage to the emitter. The Al film spikes through the thin n-type emitter when annealed at 500 °C causing cell failure. The process reproducibility is also poor due to atmospheric moisture.

14 SOLAR ENERGY↗
DOE OSTI2023

Improving estimates of sub-daily gross primary production from solar-induced chlorophyll fluorescence by accounting for light distribution within canopy

Solar-induced chlorophyll fluorescence (SIF) has long been regarded as a proxy for photosynthesis and has shown superiority in estimating gross primary production (GPP) compared to traditional vegetation indices, especially in evergreen ecosystems. However, current SIF-based GPP estimations regard the canopy as a large leaf and seldom consider the impact of interactions among light, canopy structure, and leaf physiology. In this study, we proposed GPP estimation models with different descriptions of light–structure–physiology interactions (including the layered model, the two-leaf model, and the layered two-leaf model) and compared their performances with the big-leaf model using half-hourly (or hourly) observations at evergreen needleleaf forest sites. First, we found that the big-leaf model underestimated GPP, especially at noon. All models showed higher accuracy than that of the big-leaf model. Second, we investigated the diurnal dynamics of GPP estimations in each canopy layer and found that models with a two-leaf assumption captured the diurnal variations in GPP better than that with the layered assumption. Here we also deduced that the poor performance of the big-leaf model was related to its overestimation of the overall light stress on the redox state of PSII reaction centers (qL). Finally, we noticed that the qL at the canopy scale had lower sensitivity to light change than the single-leaf qL and that the light response of canopy-scale qL was influenced by the leaf area index during seasonal cycles. Overall, this study describes methods to accurately estimate sub-daily GPP from SIF in evergreen needleleaf forests and demonstrates that the interactions among light, canopy structure, and leaf physiology regulate the SIF-GPP relationship at the canopy scale. Further, it indicates the need to consider the description of light distribution within the canopy in next-generation terrestrial biosphere models, even if they incorporate SIF to constrain their parameterization. Thus, upscaling the established leaf-scale mechanistic SIF-GPP relationship or findings to canopy-scale applications still requires much work, especially when there are significant changes in environmental conditions and their within-canopy distributions.

59 BASIC BIOLOGICAL SCIENCES↗
DOE OSTI2022

Influence of voids on the thermal and light stability of perovskite solar cells

The formation of voids in perovskite films close to the buried interface has been reported during film deposition. These voids are thought to limits the efficiency and stability of perovskite solar cells (PSCs). Here, we studied the voids formed during operation in perovskite films that were optimized during the solution deposition process to avoid voids. New voids formed during operation are found to assemble along grain boundaries at the bottom interface, caused by the loss of residual solvent and conversion of amorphous phase to crystalline phase. Unexpectedly, the formation of these voids did not negatively affect the stability of PSCs. Decreasing the amorphous region in perovskites by thermal annealing decreased the positive iodide interstitial density, and improved the light stability of PSCs. The annealed devices maintained 90% of their initial efficiency and light soaking for 1900 hours at open circuit condition under 1-sun illumination at 50°C.

14 SOLAR ENERGY↗
DOE OSTI2026

Modeling and Experimental Demonstration of Flux Spreading in Light Trapping Planar-Cavity Solar Enclosed Particle Receivers

This study experimentally validates and numerically models the flux-spreading effect in a light-trapping planar-cavity solar receiver) for particle-based concentrating solar power systems. The receiver's shallow cavity with vertical planar walls redistributes concentrated solar flux, reducing peak intensity and achieving uniform heat flux. On-sun tests at National Renewable Energy Laboratory's High-Flux Solar Furnace under flux up to 1500 kW/m2 measured cavity wall temperatures, which were compared with Monte Carlo ray-tracing (SolTrace) and computational numerical simulations. Three angular absorptance models were evaluated: constant absorptance, a Pyromark-based directional model, and a Fresnel-based Cr2O3 model. The Fresnel-derived model showed the best agreement with experiments, achieving high correlation (PC > 0.85), structural similarity (SSIM > 0.98), and signal-to-noise ratios (PSNR > 40 dB), with temperature prediction errors of 1-11%. Results confirm that flux spreading mitigates local overheating and validate the integrated modeling approach, supporting the solar receiver scalability for high-efficiency, high-temperature concentrating solar power applications.

14 SOLAR ENERGY↗
NASA NTRS2013

Low-Cost, Light Weight, Thin Film Solar Concentrator

This research addresses a cost barrier towards achieving a solar thermal collector system with an installed cost of $75/sq m and meet the Department of Energy's (DOE's) performance targets for optical errors, operations during windy conditions and lifetime. Current concentrators can cost as much as 40-50% of the total installed costs for a CSP plant. In order to reduce the costs from current $200-$250/sq m, it is important to focus on the overall system. The reflector surface is a key cost driver, and our film-based polymer reflector will help significantly in achieving DOE's cost target of $75/sq m. The ease of manufacturability, installation and replacement make this technology a compelling one to develop. This technology can be easily modified for a variety of CSP options including heliostats, parabolic dishes and parabolic troughs.

Concentrating Solar Power (CSP)↗
NASA NTRS2015

SEP Mission Design Space for Mars Orbiters

The advancement of solar-electric propulsion (SEP) technologies and larger, light-weight solar arrays offer a tremendous advantage to Mars orbiters in terms of both mass and timeline flexibility. These advantages are multiplied for round-trip orbiters (e.g. potential Mars sample return) where a large total Delta V would be required. In this paper we investigate the mission design characteristics of mission concepts utilizing various combinations and types of SEP thrusters, solar arrays, launch vehicles, launch dates, arrival dates, etc. SEP allows for greater than 50% more mass delivered and launch windows of months to years. We also present the SEP analog to the ballistic Porkchop plot - the "Bacon" plot.

Woolley, Ryan C.↗
DOE OSTI2023

Multi–Resonant Mie Resonator Arrays for Broadband Light Trapping in Ultrathin c–Si Solar Cells

Effective photon management is critical to realize high power conversion efficiencies for thin crystalline silicon (c–Si) solar cells. Standard few–100–µm–thick bulk cells achieve light trapping with macroscopic surface textures covered by thin, continuous antireflection coatings. Such sizeable textures are challenging to implement on ultrathin cells. Here, it is illustrated how nanoscale Mie–resonator–arrays with a bimodal size distribution support multiple resonances that can work in concert to achieve simultaneous antireflection and light–trapping across the broad solar spectrum. The effectiveness of these light–trapping antireflection coatings is experimentally demonstrated on a 2.8 µm–thick c–Si solar cell. The measured short–circuit current and corresponding power conversion efficiency are notably improved, achieving efficiencies as high as 11.2%. Measurements of the saturation current density on completed cells indicate that thermal oxides can effectively limit surface recombination. Finally, the presented design principles are applicable to a wide range of solar cells.

14 SOLAR ENERGY↗