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At least 145 records · Page 8

Discriminating cascading processes in nonlinear optics: A QED analysis based on their molecular and geometric origin

The nonlinear optical response of a system of molecules often contains contributions whereby the products of lower-order processes in two separate molecules give signals that appear on top of a genuine direct higher-order process with a single molecule. These many-body contributions are known as cascading and complicate the interpretation of multidimensional stimulated Raman and other nonlinear signals. In a quantum electrodynamic treatment, these cascading processes arise from second-order expansion in the molecular coupling to vacuum modes of the radiation field, i.e., single-photon exchange between molecules, which also gives rise to other collective effects. Furthermore, we predict the relative phase of the direct and cascading nonlinear signals and its dependence on the microscopic dynamics as well as the sample geometry. This phase may be used to identify experimental conditions for distinguishing the direct and cascading signals by their phase. Higher-order cascading processes involving the exchange of several photons between more than two molecules are discussed.

74 ATOMIC AND MOLECULAR PHYSICS↗

Particle production in ultrastrong-coupling waveguide QED

Understanding large-scale interacting quantum matter requires dealing with the huge number of quanta that are produced by scattering even a few particles against a complex quantum object. Prominent examples are found from high energy cosmic ray showers, to the optical or electrical driving of degenerate Fermi gases. We tackle this challenge in the context of many-body quantum optics, as motivated by the recent developments of circuit quantum electrodynamics at ultrastrong coupling. The issue of particle production is addressed quantitatively with a simple yet powerful concept rooted in the quantum superposition principle of multimode coherent states. This key idea is illustrated by the study of multi-photon emission from a single two-level artificial atom coupled to a high impedance waveguide, driven by a nearly-monochromatic coherent tone. Furthermore, we find surprisingly that the off-resonant inelastic emission lineshape is dominated by broadband particle production, due to the large phase space associated with contributions that do not conserve the number of excitations. Such frequency conversion processes produce striking signatures in time correlation measurements, which can be tested experimentally in quantum waveguides. Furthermore, these ideas open new directions for the simulation of a variety of physical systems, from polaron dynamics in solids to complex superconducting quantum architectures.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Time-dependent QED approach to x-ray nonlinear Compton scattering

Motivated by a recent experiment, we theoretically investigate the process of x-ray nonlinear Compton scattering (XNLC). Our approach is based on the time-dependent Schrödinger equation for an atomic system subject to an intense x-ray pulse, and explicitly accounts for the spontaneous scattering into a quantized photonic mode. We employ our framework to study multiple nonlinear scattering scenarios. Initially, we consider soft x rays at 500eV photon energy to scatter nonlinearly off a helium target. For this, we find that XNLC is dominated by certain third-order processes rather than the naïvely expected mechanisms pertaining to the lowest order of perturbation theory. Subsequently, we apply our model to XNLC in helium at 4.0keV photon energy and beryllium at 9.7keV. Contrary to the conclusions drawn from the experimental observations, our results suggest a good agreement of the XNLC spectrum with simple, free-electron model predictions. Furthermore, our studies reveal striking qualitative similarities of linear and nonlinear Compton scattering cross sections in this regime.

74 ATOMIC AND MOLECULAR PHYSICS↗

Self-dual ν = 1 bosonic quantum Hall state in mixed-dimensional QED

Here, we consider a (2 + 1)-dimensional Wilson-Fisher boson coupled to a (3 + 1)-dimensional U(1) gauge field. This theory possesses a strong-weak duality in terms of the coupling constant e and is self-dual at a particular value of $\mathcal{e}$. We derive exact relations between transport coefficients for a $\mathcal{ν}$ = 1 quantum Hall state at the self-dual point. Using boson-fermion duality, we map the $\mathcal{ν}$ = 1 bosonic quantum Hall state to a Fermi sea of the dual fermion and observe that the exact relationships between transport coefficients at the bosonic self-dual point are reproduced by a simple random-phase approximation (RPA), coupled with a Drude formula, in the fermionic theory. We explain this success of the RPA by pointing out a cancellation of a parity-breaking term in the fermion theory which occurs only at the self-dual point, resulting in the fermion self-dual theory explored previously. In addition, we argue that the equivalence of the self-dual structure can be understood in terms of electromagnetic duality or modular invariance, and these features are not inherited by the nonrelativistic cousins of the present model.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Fluxon-based quantum simulation in circuit QED

Long-lived fluxon excitations can be trapped inside a superinductor ring, which is divided into an array of loops by a periodic sequence of Josephson junctions in the quantum regime, thereby allowing fluxons to tunnel between neighboring sites. By tuning the Josephson couplings and, implicitly, the fluxon tunneling probability amplitudes, a wide class of one-dimensional tight-binding lattice models may be implemented and populated with a stable number of fluxons. We illustrate the use of this quantum simulation platform by discussing the Su-Schrieffer-Heeger model in the one-fluxon subspace, which hosts a symmetry-protected topological phase with fractionally charged bound states at the edges. Furthermore, this pair of localized edge states could be used to implement a superconducting qubit increasingly decoupled from decoherence mechanisms.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Prospects for simulating a qudit-based model of (1+1)D scalar QED

We present a gauge invariant digitization of (1+1)d scalar quantum electrodynamics for an arbitrary spin truncation for qudit-based quantum computers. We provide a construction of the Trotter operator in terms of a universal qudit-gate set. Here, the cost savings of using a qutrit based spin-1 encoding versus a qubit encoding are illustrated. We show that a simple initial state could be simulated on current qutrit based hardware using noisy simulations for two different native gate set.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗