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At least 145 records · Page 8

Molten Salt Reactor Signatures and Modeling Study

Molten salt reactor (MSR) technologies, either liquid fueled and cooled or only liquid cooled, pose specific, unique challenges for safeguards of the special nuclear material during the operation, fueling, and maintenance of the reactor. MSRs are one type of Generation IV technologies being invested in and considered for U.S. domestic fabrication primarily for electricity and process heat production. These designs have generated growing commercial interest for several reasons, including high (≈40%) thermal efficiency, ease of fueling, improved use of uranium fuel, potential utilization of thorium fuel, and proposed inherent safety features. U.S. companies have several planned designs that differ in fuel, cooling, and neutron energy spectrum. Driven by commercial interest and the intent of licensing MSRs, the U.S. Nuclear Regulatory Commission (NRC) has developed a vision and strategy to accommodate non-light water reactors (LWR), which include MSRs (U.S. Nuclear Regulatory Commission 2019). In addition, the Department of Energy (DOE) through the Office of Nuclear Energy (NE) Office of Advanced Reactor Technologies (ART), …sponsors research, development and deployment (RD&D) activities through its Next Generation Nuclear Plant (NGNP), Advanced Reactor Concepts (ARC), and Advanced Small Modular Reactor (aSMR) programs to promote safety, technical, economical, and environmental advancements of innovative Generation IV nuclear energy technologies. Reactor types considering the use of salts, liquid metals, or gases for coolant fall under both ARC and aSMR. Therefore, Research Design & Development is being pursued by DOE-NE through national laboratories, universities, and international and industrial collaborations. Additionally, the U.S. is a member of the Gen IV International Forum (GIF). The GIF is a cooperative, multinational organization to guide and carry out research and development needed for the GEN IV reactor systems (Forum 2018). GIF evaluated numerous reactor concepts and down-selected to the six most feasible advanced reactor technologies: gas-cooled fast reactor (GFR), lead-cooled fast reactor (LFR), MSR, supercritical watercooled reactor (SCWR), sodium-cooled fast reactor (SFR), and very high temperature reactor (VHTR). In support of the growing interest domestically and internationally, the Materials Protection, Accounting, and Control Technologies (MPACT) campaign, under the DOE-NE Fuel Cycle Technologies (FCT) program, engages in R&D activities by developing advanced instrumentation and analysis for safeguards and security of modern, advanced nuclear fuel cycle (non-LWR) facilities. Because of the historic experience in the operation of the Aircraft Reactor Experiment (ARE) and the Molten Salt Reactor Experiment (MSRE) (Robertson, MSRE Design and Operations Report Part I 1965), Oak Ridge National Laboratory (ORNL) is heavily engaged in the various R&D activities through the DOE complex related to MSRs including national technical leadership of the DOE-NE MSR campaign. This report discusses and presents the outcomes of the FY19 MPACT MSR Safeguards task. The challenges presented by MSRs for nuclear material accountancy and control (NMAC) and associated safeguards will be investigated. The objective of this research is to explore and compile the safeguards requirements and identify measurement signatures through an initial high-level MSR design and develop complementary advanced simulation and modeling capabilities. A high-level ORNL-developed MSR design called the Molten Salt Demonstration Reactor (MSDR) (Bettis, Alexander and Watts 1972) was used as the target reactor design for this research. The MSDR model incorporates technology from the MSRE and the Molten Salt Breeder Reactor (Robertson, Conceptual Design of a Single-Fluid Molten-Salt Breeder Reactor 1971). But the MSDR is a 750 MWth graphite moderated liquid fueled (low-enriched uranium) MSR compared to the MSRE’s of 7.5 MWth. The focus of this report is to discuss the evaluation of novel signatures, correlations, and indicators to understand the applicability of current safeguards instrumentation to MSRs using the modeling results from the MSDR.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Recent progress in the development of liquid metal plasma facing components for magnetic fusion devices

One of the most critical challenges for future fusion reactors is to develop longevity plasma-facing components (PFCs) exposed to extremely high heat and neutron loads. As opposed to those employing solid metals, PFCs with flowing liquid metals (LM) have shown self-healing, heat removal and good impurity control capabilities, all essential to fusion devices. Recently, significant progress in LM-PFC development has been reported globally, with data from several magnetic fusion devices. These studies reveal that LM-PFCs can endure extreme heat fluxes while maintaining plasma compatibility. New design concepts have been proposed and numerically analyzed, advancing models for liquid PFCs in future reactors. Despite existing technical challenges, these developments suggest that LM-PFCs hold promise for future fusion applications.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Thermal-Hydraulic-Mechanical Modeling and Simulation of Sodium-Potassium–Cooled MARVEL Microreactor Core

The U.S. Department of Energy's Microreactor Program, with Idaho National Laboratory's development of a nuclear microreactor applications test bed named MARVEL, aims to support R&D for the deployment of small, transportable reactors across civilian, industrial, and defense sectors. The MARVEL microreactor, an 85-kWth thermal fission reactor, incorporates TRIGA nuclear fuel and a sodium-potassium eutectic as its primary coolant, designed for safety and efficiency, with natural circulation eliminating the risk of critical heat flux conditions. The reliance on natural circulation for primary cooling means the reactor avoids using fuel spacers to minimize core pressure drop, which could disrupt the primary coolant's natural flow. However, the reactor core’s tight P/D ratio of 1.05, in the absence of fuel spacers, could pose a risk of fuel rod contact and increased peak cladding temperatures. To ensure the reactor safety, this study conducted computational modeling and simulations to investigate the reactor's thermal-hydraulic-mechanical characteristics, including the reactor core heat transfer coefficients, the potential for rod-to-rod contact, and assessed its impact on peak cladding temperature and overall reactor safety. The computational analyses of the MARVEL microreactor core revealed that the thermal deformation of fuel rods under worst-case scenario may lead to the fuel rod contact, but the peak cladding temperatures will remain significantly lower than the safety criteria, ensuring the safety operation reactor without fuel spacers under normal operating conditions.

21 - SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLAN↗

Pressure drop in a prototypical 3D magnetohydrodynamic flow across contraction of a fusion blanket manifold

Predicting 3D magnetohydrodynamic (MHD) pressure losses associated with liquid metal flows in complex geometry ducts is required to design breeding blankets for fusion reactors. Of such components, manifolds exhibit major pressure losses. Recent correlations [T. Rhodeset al. Magnetohydrodynamic pressure drop and flow balancing of liquid metal flow in a prototypic fusion blanket manifold. Phys. Fluids. 2018; 30: 057101.] demonstrate promise for predicting pressure drops in electrically insulated inlet manifolds. In the present work, the extend to which these correlations can be applied to outlet manifolds, which feature sudden contractions, is investigated in both viscous-electromagnetic (VE) and inertial-electromagnetic (IE) regimes for Reynolds numbers 50 < Re < 1500, Hartmann numbers 2500 < Ha < 5475, and expansion/contraction ratio 10. Numerical computations have shown that the MHD pressure drops in the eutectic lead-lithium (PbLi) flows in contractions are almost identical to those in the flows featuring expansion with slightly higher magnitudes in the contraction cases. The small discripancy in the MHD pressure drop between contractions and expansions (<8%) suggests that the earlier obtained correlations for the 3D MHD pressure drop in a duct flow with a sudden expansion can also be applied to flows with a sudden contraction.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

A CONDUCTION-BASED HEAT PIPE MODEL FOR ANALYZING THE ENTIRE PROCESS OF LIQUID-METAL HEAT PIPE STARTUP

The Heat Pipe-cooled Microreactor (HPM) is one of the micro nuclear reactor designs under active study at the U.S. Idaho National Laboratory. Among the major concerns of HPM research is to understand the startup behavior of the heat pipe-cooled system associated with the startup of the liquid-metal heat pipes initialing from frozen state. The startup of liquid-metal heat pipes typically involves a number of nonlinear mass and heat transport processes including the phase change from solid to liquid and vapor. Hence, it is still a huge challenge to simulate the liquid-metal heat pipe startup using conventional CFD methods and software. The major difficulties of numerical CFD modeling come from the phase-change process, multiphase interaction, microporous wick flow, and compressible gas dynamics that occur during startup of the liquid-metal heat pipes. This paper proposes a simplified conduction-based method to provide practical insights into the entire startup process of the liquid-metal heat pipes while mitigating the challenges of addressing all the complex physics. We discuss the theoretical basis and modeling assumptions to analyze the liquid-metal heat pipe startup from frozen state based solely on heat-conduction equations. Then, the proposed model is implemented into the commercial CFD software to verify the model performance. The model prediction results are discussed via the comparison with the experimental data obtained from sodium heat-pipe startup experiments.

42 ENGINEERING↗

Improved correlations of the fuel/cladding liquid penetration rate with the out-of-pile transient database

Here, utilizing data from the Out-of-Pile Transient Database (OPTD), we developed advanced correlations for the cladding liquid penetration rate in metallic fuels used in sodium-cooled fast reactors (SFRs). Based on the available OPTD data, our research highlights the key role of Pu concentration in influencing the liquid penetration behavior, showing different threshold fuel-cladding interaction temperatures, with burnup playing a substantial role, particularly in fuels with a 19% Pu concentration. The penetration rate exhibits a parabolic, diffusion-limited behavior, thereby facilitating predictions of maximum liquid penetration depth over time. These correlations are significantly more accurate, under a variety of conditions, compared to existing single-parameter models, and enhance our understanding of SFR metallic fuel behavior, promoting safer and more efficient reactor operations.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Status of GTA Gear Inspection after Testing in Sodium

The Mechanisms Engineering Test Loop (METL) is an intermediate-scale liquid metal experimental facility that provides purified reactor-grade (R-grade) sodium to various experimental test vessels. In these test vessels, components that are required to operate in an advanced fast reactor can be tested in a prototypical sodium environment. Experiments conducted in METL significantly assist in the development and maturation of systems and components for advanced reactors. The METL facility consists of multiple test segments including: a purification and diagnostic loop (cold trap was designed after EBR-II), two 18” diameter test vessels with 150 L capacities capable of operating in static or dynamic flow at 538°C, two 28” diameter test vessels with 644 L capacities capable of operating in static or dynamic flow at 650°C, a 3,180 L dump tank with 21 instrumentation ports, and the infrastructure to expand capacity in the future.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

PPPL Laboratory Directed Research and Development (Project Final Reports, FY2018 - FY2020)

The U.S. Department of Energy’s (DOE) Princeton Plasma Physics Laboratory (PPPL) is a collaborative national center for fusion energy science, basic sciences, and advanced technology. The Laboratory has three major missions: (1) to develop the scientific knowledge and advanced engineering to enable fusion to power the U.S. and the world; (2) to advance the science of nanoscale fabrication for technologies of tomorrow; and (3) to further the development of the scientific understanding of the plasma universe from laboratory to astrophysical scales. PPPL’s Laboratory Directed Research and Development (LDRD) program supports and encourages creativity and innovation and contributes to its long-term viability. New scientific and technical research areas emerge and are nurtured through the program. Furthermore, new capabilities are developed to enable the Laboratory to meet its and DOE’s missions. The program is used to systematically diversify the Laboratory’s programs and mission. In the last few years, the program has started projects in nanomaterial synthesis, microelectronics, advanced x-ray spectroscopy, high-energy-density physics, superconducting magnet technology, machine learning and artificial intelligence, 3D magnetic fields to optimize fusion plasmas, integration of permanent magnets with simple high-field magnets to reduce the cost of producing complex 3D magnetic fields, advanced computational methods for predictive understanding and control of fusion plasma, development of quantum computing algorithms for plasma physics, liquid metal plasma-facing components for fusion reactors, virtual engineering, and plasma-based space propulsion. The program is also the vehicle to recruit and train talented scientists and engineers with the new skills needed to perform the Laboratory’s mission. Many of the new hires through the program go on to become world-class scientists and engineers in their fields. This report provides descriptions and accomplishments of those LDRD projects that were completed during fiscal years 2018 through 2020.

36 MATERIALS SCIENCE↗

Conceptual design of HFIR irradiation experiment for material compatibility study on liquid Sn divertor

Liquid Sn is one of the promising coolants for liquid surface divertor concept of fusion reactors. However, the compatibility between liquid Sn and structural materials is an important issue that has to be addressed, because liquid Sn is extremely corrosive to steels at high temperatures. The corrosion may be mitigated when a protective Al2O 3 layer is formed on the surface of alumina forming steels. However, the effect of neutron irradiation on the integrity of protective layer is not made clear so far. Japan and US joint research project “FRONTIER” started in 2019 to investigate the material compatibility under neutron irradiation. The purpose of the present study is to develop the conceptual design of the irradiation test capsule which enables material compatibility tests for the alumina forming steels - liquid metal systems under neutron irradiation in the High Flux Isotope Reactor at Oak Ridge National Laboratory, TN, USA. The three dimensional drawing of capsule structure was then developed. The validity of the material selections for the capsule design was investigated by means of corrosion tests of SiC, Si3N4, Ti, and Mo in liquid Sn at 773 K for 262 hr.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Construction of 3D MHD pressure drop correlation and flow characterization in the contraction region of a fusion blanket manifold

Inlet and outlet manifolds are typical components of liquid metal (LM) blanket designs of a fusion power reactor to be used to distribute the LM flow into breeding channels and collect it at the exit of the blanket. High pressure loss in the magnetohydrodynamic (MHD) flows featuring abrupt geometrical changes is one of the main feasibility issues of such designs. Recently, optimization studies were conducted to construct 3D MHD pressure drop correlations for a LM flow in an electrically insulating manifold with gradual expansion. Here, the 3D computational approach developed in that study is applied to the outlet manifold featuring gradual contraction. A systematic analysis was performed with a total number of 135 flow cases computed with COMSOL Multiphysics for Hartmann numbers 1000 < Ha < 10,000, Reynolds numbers 100 < Re < 12,000, and contraction angles 45° < θ < 75° for a fixed contraction ratio of 4. The effects of Ha, Re and θ on the flow recirculation, development length and the total pressure drop were carefully examined. A linear regression analysis was used to determine the power rule of pressure drop coefficient k related to Ha and Re, demonstrating a good match with the Ludford layer theory. Eventually, a correlation for the 3D MHD pressure drop coefficient was constructed as a function of Ha, Re and θ. Further, the results were compared against the inlet manifold. It was found that the flow in the inlet manifold exhibits larger recirculation zones. In the investigated range of Ha, Re and θ, the pressure drop coefficient k of the LM MHD flow in the gradual contraction is only slightly lower (< 8 %) than that in the gradual expansion.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Initial Neutronics Investigation of a Chlorine Salt-Based Breeder Blanket

Tritium breeding blankets within D-T-fueled fusion reactors contain lithium compounds and typically require neutron multiplier materials to achieve a tritium breeding ratio (TBR) consistent with self-sustaining operation. Liquid breeder blankets have some advantages over solid blankets, and previous blanket studies have investigated liquid metal as well as liquid salt–based blankets. Liquid salts have reduced magnetohydrodynamic effects as compared to liquid metals, but typically have a lower TBR. Recently, advanced fission reactor concepts have considered chloride-based salts in their design, and there is a significant amount of research work occurring to study these salts. Chloride salts have previously been considered for fusion reactors, but studies have typically found lower breeding ratios than for fluoride salts, such as 2(LiF)-BeF 2 (flibe) so they have not been further developed. In this work, we use a one-dimensional cylindrical radiation transport model of a conceptual tokamak fusion reactor to investigate the neutronics feasibility of using a chloride salt–based blanket that uses chlorine enriched in 37 Cl, which has both a low capture cross section and a substantial (n,2n) cross section. It is found that chloride salts (LiCl mixed with BeCl 2 and/or PbCl 2 ) can potentially achieve a ~3% to 5% higher TBR than fluoride molten salts, notably flibe, in the absence of a solid multiplier. Including a solid multiplier, however, does narrow this advantage, with TBRs estimated within ~1% of flibe with a 2-cm Be multiplier. Chloride salts can also reach lower melting points than flibe, potentially improving the scope for the use of reduced activation ferritic-martensitic steel as a structural material. There is substantial uncertainty in the calculations driven by limited thermochemical data for the Cl salts, plus cross-section uncertainties. The production of 36 Cl through 35 Cl(n,g) and 37 Cl(n,2n) has the potential to challenge the waste disposal rating of the blanket. Calculations indicate that, while this is not an immediate showstopper, this case depends upon the exact waste disposal rating criteria used for 36 Cl. Further work could reduce these uncertainties with improved thermochemical data, higher-fidelity modeling for downselected salts, and more refined waste disposal calculations and regulatory guidance. Lastly, it must be recognized that, as for all molten salts, corrosion and chemistry can present appreciable technical challenges that require further assessment in developing a practical blanket concept, and also that the enrichment of chlorine presents an additional technical and supply chain challenge.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

UO 2 -Liquid Metal Suspension Fuel Concept: Alloy Selection and Depletion Calculations

A novel nuclear fuel was recently proposed that consists of UO 2 particles suspended in a liquid metal mixture. Two liquid metal candidates were identified: BiPbSn and PbSn. Scoping simulations were performed on an over-simplified reactor core that showed a potential limit on achievable burnup. Those findings led to two questions that needed to be addressed: What is the corrosion behavior of the liquid metals toward Zircaloy-4 (Zr4)? And what level of burnup can the fuel be expected to achieve? This report documents efforts to answer both of those questions. First, corrosion experiments were performed between the liquid metal candidates and Zr4 coupons. Second, the previous scoping simulations were expanded to include depletion analyses so that maximum burnups could be estimated. At 400°C, neither PbSn nor BiPbSn caused significant corrosion to the Zr4 coupons. At 600°C, BiPbSn did not cause significant corrosion, but PbSn did. In addition, pure bismuth and pure tin were both highly corrosive, whereas pure lead was non-corrosive. The depletion simulations found that low-enriched fuel could maintain light-water reactor operating temperatures but achieve a burnup of only about one-third of existing reactors. Higher enrichments could achieve burnups equal to or higher than those of existing reactors but at the expense of higher operating temperatures.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Conference Report on the 7th International Symposium on Liquid metals Applications for fusion (ISLA-7)

Supported by the world magnetic fusion research community, a series of International Symposia on Liquid metals Applications for fusion (ISLA) have been held biannually since 2010. The 7th edition (ISLA-7) was held for the period from 12 December through 16 December 2022, at Chubu University located in Kasugai, Aichi, Japan. For the first time in the history of this series of symposia, ISLA-7 was held in a hybrid fashion, due to the COVID-19 situation. The total number of the participants was 60, 34 out of whom attended the symposium in person, and the rest participated online. As to the presentation statistics, 29 papers were presented in person, whereas 21 presentations were delivered online but real-time by the presenters in China, Spain, the UK, and the USA. Both of the presentations delivered in person and online were recorded, and the video has been shared by all participants. These participants represent 11 countries: China, Czech, Italy, Japan, Latvia, Netherlands, Russia, Thailand, the UK, and the USA. All these numbers are among the largest in this series of symposia. Covered by these presentations are; in session-2, program overviews and liquid metal research review; in session-3, liquid metal flows, and MHD issues; in session-4, liquid metal facilities; in sessions-5 and 6, liquid metal experiments and modeling; in session-7, divertor physics and heat flux mitigation; in session-8, plasma and liquid metals interactions; in session-9 liquid metal plasma-facing components, erosion, and wettability. In addition, there were an opening session whereby several opening addresses were delivered and also a closing session where all technical session summaries were presented by the respective session chairs.

divertor↗

Divertorlets concept for low-recycling fusion reactor divertor: experimental, analytical and numerical verification

The 'divertorlets' concept is a potential non-evaporative liquid metal solution for heat removal at low recycling regime. A toroidal divertorlets prototype was built and tested in LMX-U at Princeton Plasma Physics Laboratory to evaluate the performance of this configuration. Here, details of the design, experimental results, comparison with analytical theory and MHD numerical simulations of toroidal divertorlets are covered. Experiments, analytical model and simulations showed agreement and allowed the projection of operation properties at higher magnetic flux densities (reactor-like operation), proving the concept to be a compelling solution for divertor applications.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Techno-Economic Analysis of Gas-Liquid Contactors for Tritium Extraction from Lead-Lithium

To enable a sustainable fuel cycle, any deuterium-tritium fusion reactor must breed its tritium fuel onsite. Lead-lithium (PbLi), a eutectic metal, is a leading liquid breeder material for tritium generation. One challenge with PbLi blanket technology is the extraction of tritium from the molten eutectic. Three technologies are the focus of worldwide research: the vacuum permeator, the vacuum sieve tray, and the gas-liquid contactor (GLC). The present work offers a methodology for designing, sizing, optimizing, and costing a trickle-bed GLC. Here, we analyzed tritium extraction from PbLi using MELODIE experimental data by applying traditional packed bed mass transfer efficiency models along with supplementary models, like film theory. Our analysis revealed that traditional packed bed mass transfer efficiency models do not fit the MELODIE loop experimental data. Moreover, uncertainty in PbLi solubility resulted in a 325-fold increase in required gas flow rates when comparing identical packing heights. The film theory liquid mass transfer coefficient, Delt-Olujic wettability model, and Reiter tritium solubility values fit the MELODIE data best and were used both in the design and to conduct the economic analysis. Techno-economic analysis of the GLC was performed to evaluate three design sizes, all achieving a minimum extraction efficiency of 90 [%] for a total tritium extraction of 31 [kg/yr].

Fusion Fuel Cycle↗

Development Plan for Ultrasonic Pressure Sensors [Slides]

Current light water reactors (LWRs) utilize differential pressure cells, based on strain gauges, which are remotely located from the reactor vessel via impulse lines. These pressure sensors are used to measure liquid level within the vessel and to give a general indication of system health with regard to leaks and flow system fouling. The advanced reactor types currently under development generally operate at higher temperatures than light-water reactors and utilize coolants that may be highly corrosive (i.e., liquid metals). They will use pressure measurements for varied measurands, such as level and flow rate, as well as indications of accident conditions or off-normal operating conditions. More robust pressure sensors are needed to address these more challenging conditions.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Disassembly and Initial Post-Irradiation Examination of the Mini99 Experiment

The Miniature Fuel Molybdenum-99 (Mini99) experiment is a first-of-a-kind experiment in the High Flux Isotope Reactor. Mini99 is the first MiniFuel irradiation experiment to use liquid metal inside the MiniFuel subcapsule for additional temperature control. In this work, the initial post-irradiation examination is reported. As-built simulations were conducted and compared with designs, and physical post-irradiation examinations were conducted to determine actual test temperatures via SiC thermometry samples, to evaluate the extent of fission gas release from the samples, and to remove the fuel from the subcapsules. As-built simulations compared well with experiment designs and were in reasonable agreement with the measured temperatures inferred from the passive SiC thermometers. Additionally, fission gas release values were relatively small (on the order of 3%); one sample reached approximately 8%. Although some of this behavior is attributable to recoil, most of the gas release was likely caused by the physics of the fuel behavior during the test. Finally, disassembly showed that at least four of the fuel samples degraded into small components and granules at some point during the test, with the state of the other two samples unproven. Additional work is planned for further examination of these samples via various microscopy techniques.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗