Processes in Hot-Cathode Ionization Gauges (in Reference to Explorer XVII)
Processes in hot cathode ionization gauges - electron, ions, neutral particles, and photons
NEUTRAL PARTICLE↗
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Results for “Ionization processes”
Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.
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Numerical methods for TVD transport and coupled relaxing processes in gases and plasmas
The construction of second-order upwind schemes for nonequilibrium plasmas, for both one- and two-fluid formulations is demonstrated. Coupled relaxation processes, including ionization kinetics and radiative processes and their algorithms for nonequilibrium, multiple temperature conditions are described as well. The paper applies the numerical techniques on some simple test cases, points out critical problems and their solutions, and makes qualitative comparisons with known results, whenever possible.
Cambier, Jean-Luc↗
Interferometric study of the nonequilibrium shock reflection process and thermal layer in ionizing argon
Interferometric study of nonequilibrium shock reflection process and thermal conductivity in ionizing argon
Kuiper, R. A.↗
Bayesian Statistical Analysis for Mass Spectrometric Data Processing
• Thermal ionization mass spectrometry (TIMS) is a “gold standard’ technique for actinide isotope amount ratio and assay measurements. • Ubiquitously used in: • Nuclear Nonproliferation • Nuclear Safeguards • Nuclear Forensics • Basic Science • Savannah River National Laboratory (SRNL) installed a new Thermo Scientific TRITON Plus TIMS in early 2024.
McLarty, Ellis C. [Savannah River National Laborat↗
Bayesian Statistical Analysis for Mass Spectrometric Data Processing
Thermal ionization mass spectrometry (TIMS) is a “gold standard’ technique for actinide isotope amount ratio and assay measurements. • Ubiquitously used in: • Nuclear Nonproliferation • Nuclear Safeguards • Nuclear Forensics • Basic Science • Savannah River National Laboratory (SRNL) installed a new Thermo Scientific TRITON Plus TIMS in early 2024.
McLarty, Ellis C. [Savannah River National Laborat↗
Molecular Data for a Biochemical Model of DNA Radiation Damage: Electron Impact Ionization and Dissociative Ionization of DNA Bases and Sugar-Phosphate Backbone
As part of the database for building up a biochemical model of DNA radiation damage, electron impact ionization cross sections of sugar-phosphate backbone and DNA bases have been calculated using the improved binary-encounter dipole (iBED) model. It is found that the total ionization cross sections of C3'- and C5'-deoxyribose-phospate, two conformers of the sugar-phosphate backbone, are close to each other. Furthermore, the sum of the ionization cross sections of the separate deoxyribose and phosphate fragments is in close agreement with the C3'- and C5'-deoxyribose-phospate cross sections, differing by less than 10%. Of the four DNA bases, the ionization cross section of guanine is the largest, then in decreasing order, adenine, thymine, and cytosine. The order is in accordance with the known propensity of oxidation of the bases by ionizing radiation. Dissociative ionization (DI), a process that both ionizes and dissociates a molecule, is investigated for cytosine. The DI cross section for the formation of H and (cytosine-Hl)(+), with the cytosine ion losing H at the 1 position, is also reported. The threshold of this process is calculated to be 17.1 eV. Detailed analysis of ionization products such as in DI is important to trace the sequential steps in the biochemical process of DNA damage.
Dateo, Christopher E.↗
Electron and ion spectroscopy of azobenzene in the valence and core shells
Azobenzene is a prototype and a building block of a class of molecules of extreme technological interest as molecular photo-switches. We present a joint experimental and theoretical study of its response to irradiation with light across the UV to x-ray spectrum. The study of valence and inner shell photo-ionization and excitation processes combined with measurement of valence photoelectron-photoion coincidence and mass spectra across the core thresholds provides a detailed insight into the site- and state-selected photo-induced processes. Photo-ionization and excitation measurements are interpreted via the multi-configurational restricted active space self-consistent field method corrected by second order perturbation theory. Using static modeling, we demonstrate that the carbon and nitrogen K edges of azobenzene are suitable candidates for exploring its photoinduced dynamics thanks to the transient signals appearing in background-free regions of the NEXAFS and XPS.
Chemistry↗
Narrow band imaging and long slit spectroscopy of UGC 5101
UGC 5101 (z = 0.04; D is approximately equal to 240 Mpc) is one of the so called Ultraluminous IRAS sources. Two important properties of the members of this group are their L(sub IR) is greater than or equal to 10(exp 12) solar luminosity, and their space density in the universe up to z is less than 0.1 is equal or even larger than the space density of the quasars. Further noteworthy features of the Ultraluminous IRAS sources are their being morphologically peculiar and the fact that they all seem to host active nuclei in their center. We have observed UGC 5101 in an effort to study the interplay between the gas ionized by the central active nucleus and that gas ionized by other processes which may hold important clues to the understanding of the entire picture of this object. In particular these other ionizing processes could well be massive stars formed recently after the galactic encounter and shocks possibly also related to the galaxy collision. The data that we discuss were obtained between Dec. 1989 and Jan. 1992 with the WHT 4.2 m telescope using the two-arm spectrograph ISIS. Several spectral frames were obtained at three different position angles: PA 84--along the tail of the galaxy; PA 32--along the dust lane; and PA 110. The blue spectra are centered on the H beta line, while the red spectra are centered on the H alpha line. In the configuration we used for the long slit spectra, the spectral scale was 0.74 A per pixel, and the spatial scale was .37 arcsec per pixel; we also observed the H alpha region with a spectral scale of .37 A per pixel, at position angle 84. The narrow band images were obtained at the auxiliary port of ISIS, with a scale of .2 arcsec per pixel, and were centered at the H alpha wavelength, and on the adjacent continuum. The H alpha images and the spectra support the following model. UGC 5101 hosts an active nucleus; the NLR extends up to about 1.5 kpc and shows a complex velocity field, superimposed on the rotation curve of the galaxy. Besides the NLR, in the H alpha image are visible tow bright cones that extend up to 3 kpc along PA 32. The long slit spectra at PA 32 show that the velocity field of the gas in these regions is peculiar, while the ionization structure of the gas is similar to that of the NLR.
Stanga, R. M.↗
Ionization-driven competitive (recovery) process in pre-damaged KTaO 3 : A brief review
The nuclear (S n ) and electronic (S e ) energy dissipation processes have been considered to be independent and largely uncorrelated, influencing our understanding of ion–solid interaction and damage processes in the last decades. Recently, however, it has become more generally accepted that S n and S e are coupled as they interact both in time and space. To decouple these processes, separating these effects in experiments using sequential dual-beam irradiations have become accepted as the logical path to advance the understanding of complex interactions between S e and pre-existing defects that may be created from displacement events. This experimental approach has been recently applied to studies of KTaO 3 to reveal new insights into this critical research topic. Here, we offer a forward-looking and comprehensive perspective on the fundamental coupling between Se and pre-existing defects in KTaO 3 . The origins behind the competitive two-stage phase transition process leading to damage healing are revealed and discussed. Furthermore, the evidence resulting from synergistic effects is also included for comparison. Additionally, our findings are rationalized using both Se and the ion velocity as key parameters. We highlight how the inelastic thermal spike (i-TS) calculations provide insights into the nature of this coupled process and further confirm that the ion velocity effect governs annealing kinetics. This work emphasizes that through the introduction of a small amount of local disorder in materials, MeV ion irradiation (i.e., not extreme S e ) may also be one additional option in subsequent material modification and functionalization.
46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
Certain problems associated with the processes of recombination and ionization in the earths atmosphere o nekotorykh voprosakh, svyazannykh s protsessami rekombinatsii i iowizatsii v zemnoy atmosfere
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Danilov, A. D.↗
Spontaneous-Desorption Ionizer for a TOF-MS
A time-of-flight mass spectrometer (TOF-MS) like the one mentioned in the immediately preceding article has been retrofitted with an ionizer based on a surface spontaneous-desorption process. This ionizer includes an electron multiplier in the form of a microchannel plate (MCP). Relative to an ionizer based on a hot-filament electron source, this ionizer offers advantages of less power consumption and greater mechanical ruggedness. The current density and stability characteristics of the electron emission of this ionizer are similar to those of a filament-based ionizer. In tests of various versions of this ionizer in the TOF-MS, electron currents up to 100 nA were registered. Currents of microamperes or more - great enough to satisfy requirements in most TOFMS applications - could be obtained by use of MCPs different from those used in the tests, albeit at the cost of greater bulk. One drawback of this ionizer is that the gain of the MCP decreases as a function of the charge extracted thus far; the total charge that can be extracted over the operational lifetime is about 1 coulomb. An MCP in the ion-detector portion of the TOF-MS is subject to the same limitation.
Schultz, J. Albert↗
Onset of Cosmic Reionization: Evidence of an Ionized Bubble Merely 680 Myr After the Big Bang
While most of the intergalactic medium (IGM) today is permeated by ionized hydrogen, it was largely filled with neutral hydrogen for the first 700 million years after the big bang. The process that ionized the IGM (cosmic reionization) is expected to be spatially inhomogeneous, with fainter galaxies likely playing a significant role. However, we still have only a few direct constraints on the reionization process. Here we report spectroscopic confirmation of two galaxies and very likely a third galaxy in a group (hereafter EGS77) at redshift z = 7.7, merely 680 Myr after the big bang. The physical separation among the three members is <0.7 Mpc. We estimate the radius of ionized bubble of the brightest galaxy to be about 1.02 Mpc, and show that the individual ionized bubbles formed by all three galaxies likely overlap significantly, forming a large yet localized ionized region, indicative of inhomogeneity in the reionization process. It is striking that two of three galaxies in EGS77 are quite faint in the continuum, thanks to our selection using their Lyα line emission in the narrowband filter. Indeed, one is the faintest spectroscopically confirmed galaxy yet discovered at such high redshifts. Our observations provide direct constraints on the process of cosmic reionization, and allow us to investigate the properties of sources responsible for reionizing the universe.
Reionization↗
Strong-field ionization of water: Nuclear dynamics revealed by varying the pulse duration
Polyatomic molecules in strong laser fields can undergo substantial nuclear motion within tens of femtoseconds. Ion imaging methods based on dissociation or Coulomb explosion therefore have difficulty faithfully recording the geometry dependence of the field ionization that initiates the dissociation process. Here we compare the strong-field double ionization and subsequent dissociation of water (both H 2 O and D 2 O) in 10-fs and 40-fs 800-nm laser pulses. We find that 10-fs pulses turn off before substantial internuclear motion occurs, whereas rapid internuclear motion can take place during the double ionization process for 40-fs pulses. The short-pulse measurements are consistent with a simple tunnel ionization picture whose predictions help interpret the motion observed in the long-pulse measurements.
74 ATOMIC AND MOLECULAR PHYSICS↗
Pulse shaping in strong-field ionization: Theory and experiments
Intense ultrafast pulses cause dissociative ionization and shaping the pulses may allow control of both electronic and nuclear dynamics that determine ion yields. We report on a combined experimental and theoretical effort to determine how shaped laser pulses affect tunnel ionization, the process that precedes many strong-field phenomena. We carried out experiments on Ar, N 2 , H 2 O, and O 2 using a phase-step function of amplitude 3/4π that is scanned across the spectrum of the pulse. In addition, we changed the amount of chirp in the pulses. Semiclassical as well as fully quantum mechanical time-dependent Schrödinger equation calculations are found to be in excellent agreement with experimental results. We find that precise knowledge of the field parameters in the time and frequency domains is essential to afford reproducible results and quantitative theory and experiment comparisons.
74 ATOMIC AND MOLECULAR PHYSICS↗
Observed rate of ionization in shaped-charge releases of barium in the ionosphere
Data from 36 Ba shaped-charge releases carried out at an angle of less than 25 deg to the magnetic field, by the technique of Wescott et al. (1972) and Michel (1974), were examined for evidence of a sustained rate of ionization in excess of that attributable to sunlight. In four of the experiments, the time constant for the decay of the neutrals was measured using an ultrasensitive color TV camera and was found to have a value of about 30 sec, consistent with slow (solar) ionization. Although the qualitative appearance of most jets was found to be consistent with a slow process of ionization, some releases produced a thin confined jet that was suggestive of rapid ionization. Two of these jets were analyzed in detail, but no evidence of anomalous ionization was produced. The data obtained in this work agree with the geometrical predictions of the Swift model.
Hallinan, Thomas J.↗
Measurements of the time constant for steady ionization in shaped-charge barium releases
Quantitative measurements of three solar illuminated shaped-charge barium releases injected at small angles to the magnetic field were made using a calibrated color television camera. Two of the releases were from 1989. The third release, a reanalysis of an event included in Hallinan's 1988 study of three 1986 releases, was included to provide continuity between the two studies. Time constants for ionization, measured during the first 25 s of each release, were found to vary considerably. The two 1989 time constants differed substantially, and both were significantly less than any of the 1986 time constants. On the basis of this variability, we conclude that the two 1989 releases showed evidence of continuous nonsolar ionization. One release showed nonsolar ionization which could not he attributed to Alfven's critical ionization velocity process, which requires a component of velocity perpendicular to the magnetic field providing a perpendicular energy greater than the ionization potential.
Hoch, Edward L.↗
Scaling and Systems Considerations in Pulsed Inductive Thrusters
Performance scaling in pulsed inductive thrusters is discussed in the context of previous experimental studies and modeling results. Two processes, propellant ionization and acceleration, are interconnected where overall thruster performance and operation are concerned, but they are separated here to gain physical insight into each process and arrive at quantitative criteria that should be met to address or mitigate inherent inductive thruster difficulties. The effects of preionization in lowering the discharge energy requirements relative to a case where no preionization is employed, and in influencing the location of the initial current sheet, are described. The relevant performance scaling parameters for the acceleration stage are reviewed, emphasizing their physical importance and the numerical values required for efficient acceleration. The scaling parameters are then related to the design of the pulsed power train providing current to the acceleration stage. The impact of various choices in pulsed power train and circuit topology selection are reviewed, paying special attention to how these choices mitigate or exacerbate switching, lifetime, and power consumption issues.
Polzin, Kurt A.↗
Magnetic diffusion and ionization fractions in dense molecular clouds - The role of charged grains
The physics of magnetic diffusion in dense molecular clouds is examined, with particular attention given to the role of charged grains in controlling the process. The ionization fraction of dense molecular clouds in the presence of grains is determined from considerations of charge exchange, dissociative recombination, radiative recombination and collisions between grains and charged species, and it is found that the inclusion of grains tends to lower the ionization fraction for a given cosmic-ray ionization rate and metal depletion. The kinematics of grain motion is discussed and it is shown that at temperatures less than 30 K, each grain alternates rapidly in charge between -1 and 0 and thus executes periodic motion in a self-gravitating cloud containing a magnetic field. The full kinematics of magnetic diffusion including the motions of ions and electrons are then examined, taking into account the additional viscous force from charged grains, and numerical calculations of the diffusion time scales of uniform, magnetically supported clouds or cloud cores are presented.
Elmegreen, B. G.↗