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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 145 records · Page 8
All sourcesNASA NTRSDOE OSTI
DOE OSTI2024

A Measurement of the Eta Meson Radiative Decay Width via the Primakoff Effect

The ? meson is an interesting tool to study fundamental symmetries in Quantum Chromodynamics (QCD). In particular, its radiative decay width, ? p? Ñ ??q, is an important quantity that can be predicted in the framework of Chiral Perturbation Theory. A precision measurement of this quantity would provide critical inputs to understanding the mixing of the ? and ?1 mesons and extracting constants with wide-ranging applications in low-energy QCD. This decay width has been measured in the past using two different experimental techniques. The more popular technique utilized e`e´ collisions to produce ? mesons through electromagnetic interactions. Today, the Particle Data Group (PDG) averages the results of five such experiments to obtain their currently-accepted value of the decay width as: 0.515?0.018 keV. However the first measurement of this quantity was obtained from a fixed-target experiment that measured the cross section for photoproduction of ? mesons on a nuclear target via the Primakoff effect. Their result of 0.324?0.046 keV shows strong tension with the average of the collider measurements, motivating a new, high precision measurement using the Primakoff method. For this purpose, the PrimEx-eta experiment was conducted in Hall D of the Thomas Jefferson National Accelerator Facility (Jefferson Lab or JLab). The data is currently being analyzed to measure the differential cross section for the photoproduction of ? mesons on a liquid, 4He target. Preliminary results obtained from the analysis of the first phase of the PrimEx-eta experiment show reasonable agreement with the currently-accepted PDG value of the radiative decay width. However, as will be discussed, there are many challenges to this precision measurement which must be studied before any results can be finalized and compared with previous measurements. In parallel to the ? decay width measurement, the PrimEx-eta experiment measured the total cross section for the fundamental, Quantum Electrodynamics (QED) process of Compton scattering from the atomic electrons inside the target. The results obtained from this measurement are in strong agreement with the next-to-leading order QED calculations, and the total combined uncertainties are below 3% for incident photon energies between 7-10 GeV. In addition to providing the first precision measurement of the total Compton scattering cross section within this beam energy range, this measurement verifies the capability of the PrimEx-eta experimental setup to perform absolute cross section measurements at forward angles, and serves as a reference process for the calibration of systematic uncertainties.

Smith, Andrew↗
DOE OSTI2024

Measuring Neutron Polarisation in Deuteron Photo-disintegration with the CLAS Start Counter [Thesis]

Deuteron photo-disintegration (γd → γp) is a reaction that represents the simplest case in which nuclear and hadron physics models can be tested. Despite this, associated polarization analyses are limited in terms of angular coverage and energy ranges, especially in observables related to the recoil neutron. This is largely due to a lack in dedicated polarimetry equipment, and represents a roadblock in global progress to understand high-energy phenomena such as hexaquarks, and quark-gluon degrees of freedom. To address this problem, this PhD thesis pioneers a new methodology for the parasitic measurement of nucleon polarization using kinematic reconstruction of (spin-dependent) nucleon-nucleus scattering of reaction products, prior to their detection in large acceptance particle detector apparatus. Following this novel approach, which requires no dedicated polarimeter, a determination of the double polarization observable, $C^n_{x'}$, from deuteron photo-disintegration is presented, using Jefferson Lab’s CLAS detector. The analysis utilizes the (n,p) charge exchange reaction in CLAS’s "start counter" (plastic scintillator) to determine the final state neutron polarizations. The results present the first ever data for this observable above 0.7 GeV (photon beam energy) and significantly extend the angular range of the world data set. This new data is largely statistically consistent with the previous measurement of $C^n_{x'}$ by Bashkanov et al . in the overlapping energy range of 0.4-0.7 GeV. It is planned for the statistical accuracy of the presented result to be increased by the inclusion of additional data. The analysis herein serves as a key proof of concept for future applications, including a recommended similar analysis to be implemented with data from the more modern CLAS12 detector. This paves the way for a plethora of additional analyses using existing data sets that would provide crucial new constraints for hadron and nuclear physics.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2020

Kinetic Modeling and Experimental Studies of Capacitively Coupled Macro- and Microplasmas at Microwave Frequencies

The effect of driving frequency in the range of 13.56 MHz to 73 MHz on electron energy distribution and electron heating modes in a 50 mTorr capacitively coupled argon plasma discharge is studied using 1D-3V particle-in-cell simulations. Calculated electron energy probability functions exhibit three distinct temperatures for low-, mid-, and high-energy electrons at all the studied driving frequencies. When compared to published experimental data, the calculated probability functions show a reasonable agreement for the energy range resolved in the measurements (about 2 eV to 10 eV). Discrepancies due to limitations in experimental energy resolution outside this range lead to differences between computational and experimental values of the electron number density determined from the distribution functions, and the predicted effective electron temperature is within 25 % of experimental values. The impedance of the discharge is interpreted in terms of a homogeneous equivalent circuit model and the driving frequency dependence of the inferred combined sheath thickness is found to obey a known, theoretically-derived, power law. The average power transferred from the field to the electrons (electron heating) is computed, and a region of negative heating near the sheath edge, particularly at higher driving frequencies, is identified. Analysis of the electron momentum equation shows that electron inertia, which on temporal averaging would be zero in a linear regime, is responsible for negative values of power deposition near the sheath edge at high driving frequencies due to the highly nonlinear behavior of the discharge.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2024

GENESIS: Gamma Energy Neutron Energy Spectrometer for Inelastic Scattering

Improved neutron inelastic scattering cross section data are needed to inform integral benchmark studies and advance applications in a wide variety of areas including nuclear energy, stockpile stewardship, nonproliferation, and space exploration. Neutron inelastic scattering also serves as a non-selective probe of low-lying nuclear structure. To help meet these needs, the Gamma Energy Neutron Energy Spectrometer for Inelastic Scattering (GENESIS) was constructed at the 88-Inch Cyclotron at Lawrence Berkeley National Laboratory. This array couples high-resolution γ-ray detectors and fast neutron detectors to achieve single and coincident n/γ detection over a broad energy range. The current configuration of the array includes 26 organic liquid scintillators and four high-purity germanium detectors (two single-crystal and two four-crystal CLOVER detectors with two-fold segmentation). The array was constructed with minimal supporting material and designed to cover a wide range of secondary particle angles and energies with limited inter-element scattering. Data acquisition is accomplished using Mesytec MDPP-16 multi-channel high-resolution digital pulse processing modules. The array characteristics, including γ-ray and neutron energy resolution, timing resolution, and detection efficiency were measured and used to validate a Geant4 model of the array. Furthermore, the primary sources of neutron background and the uncertainties in the determination of incident and secondary neutron energy were assessed. GENESIS provides a new capability to address nuclear data needs and facilitates the advancement of a wide range of nuclear applications.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

Performance of microchannel plate based detectors for <25 keV x rays: Monte Carlo simulations and comparisons with experimental results

We present the results of Monte Carlo simulations of the microchannel plate (MCP) response to x rays in the 250 eV to 25 keV energy range as a function of both x-ray energy and impact angle and their comparisons with the experimental results from the X8A beamline at the National Synchrotron Light Source at Brookhaven National Laboratory. Incoming x rays interact with the lead glass of the microchannel plate, producing photoelectrons. Transport of the photoelectrons is neglected in this model, and it is assumed that photoelectrons deposit all their energy at the point they are created. This deposition leads to the generation of many secondary electrons, some fraction of which diffuse to the MCP pore surface where they can initiate secondary electron cascades in the pore under an external voltage bias. X-ray penetration through multiple MCP pore walls is increasingly important above 5 keV, and the effect of this penetration on MCP performance is studied. In agreement with past measurements, we find that the dependence of MCP sensitivity with angle relative to the pore bias changes from a cotangent dependence to angular independence and then proceeds to a secant dependence as the x-ray energy increases. We also find that with the increasing x-ray energy, the MCP gain sensitivity as a function of bias voltage decreases. The simulations also demonstrate that for x rays incident normal to the MCP surface, spatial resolution shows little dependence on the x-ray energy but degrades with the increasing x-ray energy as the angle of incidence relative to the surface normal increases. This agrees with experimental measurements. Simulation studies have also been completed for MCPs gated with a subnanosecond voltage pulse. In this work, we find that the optical gate profile width increases as the x-ray energy is increased above 5 keV, a consequence of increased x-ray penetration at energies >5 keV. Simulations of the pulsed dynamic range show that the dynamic range varies between ~100 and 1000 depending on x-ray energy and peak voltage.

47 OTHER INSTRUMENTATION↗
DOE OSTI2026

Multi-GeV FFA beam transport test at CEBAF

Jefferson National Lab plans an upgrade project to reach 22 GeV high polarization electron beam by using Fixed Field Alternating-gradient (FFA) magnets. The utilization of the FFA magnets for 10-22 GeV beam energy range is unexampled, therefore those magnets need an experimental validation before their full installation to form an arc in the Continuous Electron Beam Accelerator Facility (CEBAF). For this reason, JLAB is also considering the design of an FFA magnet test bench, i.e. a half or full FFA cell, that would be deployed in the current CEBAF in order to serve as the highest energy demonstration for the FFA field uniformity, permanent magnet resiliency with the beam as well as enabling beam optics measurements with the 5-11 GeV range highly polarized beams which closely resembles the full energy range of the 22 GeV upgrade. In this report, we present the status of the planned beamline for the FFA beam transport test at CEBAF.

Accelerator Physics↗
DOE OSTI2022

Study of a Proposed fissionTPC Measurement of 233 U(n,f)/ 235 U(n,f) Cross Section Ratio

A review of the available 233 U( n, f )/ 235 U( n, f ) cross section ratio data compared to the ENDF evaluation in the fast neutron energy range, 0.1–20 MeV, shows that discrepancies exist between some of the various measurements and the evaluation. The discrepancies vary and a function of incident neutron energy and range between 1–5%. In this document we review two potential options for performing new measurements of the cross section ratio to potentially resolve these discrepancies. The two options are compared and contrasted in terms of measurement accuracy and cost. The first option would utilize the fissionTPC, which was designed specifically to achieve measurement uncertainties of better than 1% to resolve a similar data–evaluation discrepancy in the 239 Pu( n, f ) cross section. While this would seem to be an ideal option in this case also, there are challenges. The fissionTPC is a complex instrument and the cost of maintenance and operations are significant. Furthermore, some of the fissionTPC equipment is nearing the end of its useful life which presents a risk to completion of a measurement campaign. The second option is to use a dual-fission chamber, which is the more traditional approach to these types of measurements. The cost is estimated to be about half that of a fissionTPC measurement, while the much simpler design of the detector reduces overall risk. The trade-off is the measurement uncertainty, which would be on order of 1–3% with a careful measurement and analysis. This uncertainty however may not be good enough to fully resolve the discrepancies. The objective of a new measurement would be the improvement in the ENDF evaluation with the end goal of improving the accuracy of models and simulations at the end of the nuclear data pipeline. An understanding of the sensitivity of these models to the data uncertainties would help guide the choice of measurement techniques.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2022

UA'(1): The search for low-mass dark matter in liquid xenon / Infrared Light for Liquid Xenon TPCs

Liquid xenon-based time projection chambers are used in a variety of applications spanning from the search for dark matter or signals from coherent neutrino-nucleus scattering, to detectors used in medicine and for nuclear non-proliferation. Extending the useful energy range of these detectors down to lower energies will prove extremely useful for such applications. However, various sources of single- and few-electron backgrounds limit the utility of experiments such as LZ and XENONnT to searches of lighter dark matter articles in the MeV mass range. These same backgrounds also limit their utility to measure signals from coherent neutrino-nucleus scattering of solar boron-8 neutrinos and Galactic supernovae. This research worked on multiple mitigation strategies to reduce these backgrounds, through improved xenon purity, infrared irradiation, and an improved theoretical understanding. Multiple dedicated liquid xenon setups were built to execute those tests, and data was successfully taken. Liquid xenon purity was shown to have an important impact, but infrared irradiation did not reduce these backgrounds.

47 OTHER INSTRUMENTATION↗
DOE OSTI2022

A high-granularity calorimeter insert based on SiPM-on-tile technology at the future Electron-Ion Collider

Herein we present a design for a high-granularity calorimeter insert for future experiments at the Electron-Ion Collider (EIC). The sampling-calorimeter design uses scintillator tiles read out with silicon photomultipliers. It maximizes coverage close to the beampipe, while solving challenges arising from the beam-crossing angle and mechanical integration. It yields a compensated response that is linear over the energy range of interest for the EIC. Its energy resolution meets the requirements set in the EIC Yellow Report even with a basic reconstruction algorithm. Moreover, this detector will provide 5D shower data (position, energy, and time), which can be exploited with machine-learning techniques. This detector concept has the potential to unleash the power of imaging calorimetry at the EIC to enable measurements at extreme kinematics in electron–proton and electron–nucleus collisions.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2023

Quantification of the 35 Cl($\textit{n, p}$) reaction channel

The evaluated 35 Cl($\textit{n, p}$) cross sections in the ENDF/B-VIII.0 nuclear data library remain uncertain because of the lack of measured data in the neutron energy range between 100-600 keV. In this energy region, the R-matrix analysis relies heavily on estimated ($\textit{n, p}$) partial widths and level density information. This resulted in significant differences of the evaluated cross sections and predicted reactivity in nuclear reactor applications with respect to previous nuclear data libraries. Here, we present a methodology to quantify the cross sections for the 35 Cl($\textit{n, p}$) reaction channel from the combination of measured total cross sections and model calculations.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗
DOE OSTI2025

Dissipation Pathways in a Photosynthetic Complex

Determining how energy flows within and between molecules is crucial for understanding chemical reactions, material properties, and even vital processes such as photosynthesis. While the general principles of energy transfer are well established, elucidating the specific molecular pathways by which energy is funneled remains challenging, as it requires tracking energy flow in complex molecular environments. Here, we demonstrate how photon excitation energy is partially dissipated in the light-harvesting Fenna–Matthews–Olson (FMO) complex, mediating the excitation energy transfer from light-harvesting chlorosomes to the photosynthetic reaction center in green sulfur bacteria. Specifically, we isolate the contribution of the protein and specific vibrational modes of the pigment molecules to the energy dynamics. For this, we introduce an efficient computational implementation of a recently proposed theory of dissipation pathways for open quantum systems, based on second-order perturbation theory in the electronic couplings. Using it and a state-of-the-art FMO model with highly structured and chromophore-specific spectral densities, we demonstrate that energy dissipation is dominated by low-frequency modes (<800 cm –1 ) as their energy range is near-resonance with the energy gaps between electronic states of the pigments. We identify the most important modes for dissipation to be in-plane breathing modes (∼200 cm –1 ) of the bacteriochlorophylls in the complex. Conversely, far-detuned intramolecular vibrations with higher frequencies (>800 cm –1 ) play no role in dissipation. Interestingly, the FMO complex first needs to borrow energy from the environment to release excess photonic energy, indicating that the energy exchange between the system and thermal environment is not strictly unidirectional in time but involves a transient thermally activated step. Beyond their fundamental value, these insights can guide the development of artificial light-harvesting devices and, more broadly, engineer environments for chemical and quantum control tasks.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2023

Nuclear structure and elastic scattering observables obtained consistently with different N N interactions

Nucleon-nucleon ($NN$) interactions based on chiral effective theories are commonly used in ab initio calculations of light nuclei. Here we present a study based on three different $NN$ interactions (up to next-to-next-to-leading order) for which structure and elastic proton scattering observables are consistently calculated for $^4$He, $^{12}$C, and $^{16}$O. The interactions are compared at the two-body level in terms of Wolfenstein amplitudes, and their predictions for ground state energies, point-proton radii, and charge form factors, as well as proton elastic scattering observables in the leading-order spectator expansion in the energy range between 65 and 160 MeV projectile energy are presented. Finally, to gain further insight into differences visible in elastic scattering observables, we investigate the behavior of the calculated effective nucleon-nucleus interactions for the $^{12}$C nucleus based on the different $NN$ interactions.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Linear dichroism infrared resonance in overdoped, underdoped, and optimally doped cuprate superconductors

By measuring the polarization changes in terahertz, infrared, and visible radiation over an extended energy range (3–2330 meV), we observe symmetry breaking in cuprate high-temperature superconductors over wide energy, doping, and temperature ranges. We measure the polarization rotation (Re[$θ_F$]) and ellipticity (Im[$θ_F$]) of transmitted radiation through thin films as the sample is rotated. We observe a twofold rotational symmetry in $θ_F$, which is associated with linear dichroism (LD) and occurs when electromagnetic radiation polarized along one direction is absorbed more strongly than radiation polarized in the perpendicular direction. Such polarization anisotropies can be generally associated with symmetry breakings. We measure the amplitude of the LD signal and study its temperature, energy, and doping dependence. The LD signal shows a resonant behavior with a peak in the few hundred meV range, which is coincident with the midinfrared optical feature that has been associated with the formation of the pseudogap state. In this work, the strongest LD signal is found in underdoped films, although it is also observed in optimally and overdoped samples. The LD signal is consistent with an electronic nematic order which is decoupled from the crystallographic axes as well as novel magnetoelectric effects.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2023

Enabling URR Self Shielding Functionality in SAMMY [Slides]

This lecture is on enabling Unresolved Resonance Energy Range (URR) self-shielding functionality in SAMMY. This presentation covers Fiscal Year 2022 milestones, and motivations driving this endeavor. This presentation includes slides depicting the current self-shielding correction workflow. Additionally, this presentation includes a look into the doppler broadening issue and the verification of capture. This lecture concludes with envisioned future work.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2024

Nuclear structure opportunities with GeV radioactive beams at FAIR

The Facility for Antiproton and Ion Research (FAIR) is in its final construction stage next to the campus of the Gesellschaft für Schwerionenforschung Helmholtzzentrum for heavy-ion research in Darmstadt, Germany. Once it starts its operation, it will be the main nuclear physics research facility in many basic sciences and their applications in Europe for the coming decades. Owing to the ability of the new fragment separator, Super-FRagment Separator, to produce high-intensity radioactive ion beams in the energy range up to about 2 GeV/nucleon, these can be used in various nuclear reactions. This opens a unique opportunity for various nuclear structure studies across a range of fields and scales: from low-energy physics via the investigation of multi-neutron systems and halos to high-density nuclear matter and the equation of state, following heavy-ion collisions, fission and study of short-range correlations in nuclei and hypernuclei. Here, the newly developed reactions with relativistic radioactive beams (R3B) set up at FAIR would be the most suitable and versatile for such studies. An overview of highlighted physics cases foreseen at R3B is given, along with possible future opportunities, at FAIR.

FAIR↗
DOE OSTI2024

Photonuclear Physics in SCALE

Radiation shielding modeling involves a wide range of applications, such as power reactors, critical experiments, portable sources, linear accelerators, and fusion systems. Particle energy ranges vary from thermal energies to fast energy spectra. MAVRIC, as the radiation shielding sequence of the SCALE code system [1] developed and maintained by Oak Ridge National Laboratory, is capable of modeling both neutron and photon interactions in matter and is widely used by the US Nuclear Regulatory Commission, Department of Energy, the National Nuclear Security Administration, and radiation shielding practitioners all around the world. Although most applications don’t involve highly energetic photons that can cause photonuclear reactions and create coupled chains of high energy, ionized electrons and bremsstrahlung radiation within a material medium, when present, these reactions can have a significant impact upon the downstream particle fluxes from incident photons above 20 MeV. For example, linear accelerators used for medical isotope production are examples of applications in which high-energetic photons are generated and used for driving or controlling other components of a complex facility. Radiation shielding analyses of such a facility would require accounting for any and all significant sources of radiation. Unfortunately, MAVRIC included no data and methods to model either photonuclear reactions or the bremsstrahlung photons until this work, which enabled accounting for both. Photonuclear reaction cross sections were imported from the Evaluated Nuclear Data File libraries, and corresponding methods were implemented in the SCALE code system; see Section 2 for how the nuclear data are imported and used. Bremsstrahlung photons were modeled by assuming thick-target approximation whereby all generated electrons and positrons due to photon interactions are assumed to be absorbed within the same material in which they were born, yielding a quick particle transport simulation method by using fast lookup tables for generating subsequent gammas; see Section 4 for details. A suite of verification models was used to test implemented methods and associated data. Tests yielded satisfactory results for the new features. Enhancements will be released as part of the next major SCALE release (v7.0), which is anticipated to be deployed in 2025, with beta releases available in the interim.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2024

Resolved Resonance Evaluation for Neutron Interactions with 103 Rh up to 8 keV

A neutron cross-section evaluation for the n + 103 Rh reaction in the resolved resonance region was carried out in the energy range 10−5 eV to 8 keV encompassing thermal energy at 0.0253 eV. The scope of this work is to generate resonance parameters and resonance parameter covariances based on the Reich-Moore reduced R-matrix formalism using the code SAMMY. Some features of the new evaluation are the inclusion of high-resolution capture data in the SAMMY evaluation process and the extension of the resolved resonance range from 4 to 8 keV. Furthermore, the evaluation employs more accurate resonance parameter representation by exploring the use of the LRF = 7 ENDF feature and also the use of the LCOMP = 2 compact format for resonance parameter covariance representation. Included in the SAMMY evaluation are transmission data, capture cross-section data, and neutron scattering length information. Thermal cross-section values listed in the literature, as well as capture resonance integrals, were also incorporated into the evaluation process.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2021

Substituted ALPO-5 Zeolites as Promising O 2 Sorption Pump Materials: A Density Functional Theory Study

Many chemical processes depend on having an environment that is low in oxygen partial pressure (P O2 < 100 Pa); sorption pumps are a promising route to establishing that environment by either oxygen pumping or oxygen separation from an inert gas. Near ambient sorption-based processes rely on either pressure or thermal swings, requiring no moving parts, no electricity, and neither very high nor very low temperatures. In this work, we use ab initio calculations to explore zeolites as a class of materials for sorption based oxygen pumping/separation. Our calculations indicate that while the neat ALPO-5 zeolite does not adsorb O 2 , O 2 does adsorb on zeolites selectively substituted with transition metals and metalloids and hence, can enable separation and pumping. ALPO-5 substituted with Si, Ge, Sn, Pd, Pt, Ti, V, Cr, Mn, Zr, Mo, Hf, W, Ce, and Pr provides adsorption energies ranging from -0.19 to -3.92 eV, (-) indicates exothermic process. Additionally, we provide a comprehensive understanding of what controls the adsorption energy: 1) the substi-tutions must be able to adopt an oxidation state that is more positive than the cation it replaces, and 2) the size of the pore into which the O 2 adsorbs to the wall. Additionally, we conduct a ther-modynamic analysis of a thermal swing cycle to approximate the optimal O 2 binding energy for 2 low energy O 2 pumping/separation. We find that the minimum energy cost likely occurs when the adsorption energy is in the range of 0.75 – 1.00 eV (72 – 97 kJ·mol -1 ), which corresponds to Ge, V, Pt, or Ce substituted ALPO-5.

36 MATERIALS SCIENCE↗