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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 145 records · Page 8
All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

Hybridization of Bogoliubov Quasiparticles between Adjacent CuO 2 Layers in the Triple-Layer Cuprate Bi 2 Sr 2 Ca 2 Cu 3 O 10 + δ Studied by Angle-Resolved Photoemission Spectroscopy

Hybridization of Bogoliubov quasiparticles (BQPs) between the CuO 2 layers in the triple-layer cuprate high-temperature superconductor Bi 2 Sr 2 Cu 2 Cu 3 O 10+δ is studied by angle-resolved photoemission spectroscopy (ARPES). In the superconducting state, an anticrossing gap opens between the outer- and inner-BQP bands, which we attribute primarily to interlayer single-particle hopping with possible contributions from interlayer Cooper pairing. We find that the d-wave superconducting gap of both BQP bands smoothly develops with momentum without an abrupt jump in contrast to a previous ARPES study. Hybridization between the BQPs also gradually increases in going from the off nodal to the antinodal region, which is explained by the momentum dependence of the interlayer single-particle hopping. As possible mechanisms for the enhancement of the superconducting transition temperature, the hybridization between the BQPs as well as the combination of phonon modes of the triple CuO 2 layers and spin fluctuations represented by a four-well model are discussed.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2022

SWAP Gate between a Majorana Qubit and a Parity-Protected Superconducting Qubit

High fidelity quantum information processing requires a combination of fast gates and long-lived quantum memories. Here, in this Letter, we propose a hybrid architecture, where a parity-protected superconducting qubit is directly coupled to a Majorana qubit, which plays the role of a quantum memory. The superconducting qubit is based upon a π-periodic Josephson junction realized with gate-tunable semiconducting wires, where the tunneling of individual Cooper pairs is suppressed. One of the wires additionally contains four Majorana zero modes that define a qubit. We demonstrate that this enables the implementation of a SWAP gate, allowing for the transduction of quantum information between the topological and conventional qubit. This architecture combines fast gates, which can be realized with the superconducting qubit, with a topologically protected Majorana memory.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2024

Dark Matter Induced Power in Quantum Devices

We point out that power measurements of single quasiparticle devices open a new avenue to detect dark matter (DM). The threshold of these devices is set by the Cooper pair binding energy, and is therefore so low that they can detect DM as light as about an MeV incoming from the Galactic halo, as well as the low-velocity thermalized DM component potentially present in the Earth. Using existing power measurements with these new devices, as well as power measurements with SuperCDMS-CPD, we set new constraints on the spin-independent DM scattering cross section for DM masses from about 10 MeV to 10 GeV. We outline future directions to improve sensitivity to both halo DM and a thermalized DM population in the Earth using power deposition in quantum devices. Published by the American Physical Society 2024

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2025

Doping Dependence of 2-Spinon Excitations in the Doped 1D Cuprate Ba 2 ⁢CuO 3+δ

Recent photoemission experiments on the quasi-one-dimensional Ba-based cuprates suggest that doped holes experience an attractive potential not captured using the simple Hubbard model. This observation has garnered significant attention due to its potential relevance to Cooper pair formation in high-T c cuprate superconductors. To scrutinize this assertion, we examined signatures of such an attractive potential in doped 1D cuprates Ba 2 ⁢CuO 3+δ by measuring the dispersion of the 2-spinon excitations using Cu L 3 -edge resonant inelastic x-ray scattering (RIXS). Upon doping, the 2-spinon excitations appear to weaken, with a shift of the minimal position corresponding to the nesting vector of the Fermi points, q F . Notably, we find that the energy scale of the 2-spinons near the Brillouin zone boundary is substantially softened compared to that predicted by the Hubbard model in one dimension. Finally, such a discrepancy implies missing ingredients, which lends support for the presence of an additional attractive potential between holes.

1-dimensional spin chains↗
DOE OSTI2025

Berry Curvature and Spin-One Color Superconductivity

Here, we explore the interplay between Berry curvature and topological properties in single-flavor color superconductors, where quarks form spin-one Cooper pairs. By deriving a new relation, we connect the topological nodal structure of the gap function in momentum space to the (non-Abelian) Berry flux associated with paired quarks. This generalizes the early work by Li and Haldane [Phys. Rev. Lett. 120, 067003 (2018)] to systems with additional internal quantum numbers, such as color. In the ultrarelativistic limit, we uncover rich topological structures driven by the interplay of spin, chirality, and color. Specifically, we identify chirality-induced topological nodes in the transverse (opposite chirality pairing) polar and 𝐴 phases. In contrast, the color-spin-locking phase lacks these nodes due to a nontrivial color Berry flux, which in turn induces gapless excitations with total Berry monopole charges of ±3/2—differing from conventional Weyl fermions. Our findings can be potentially extended to other fermionic systems carrying additional internal degrees of freedom.

Berry curvature↗
DOE OSTI2021

Role of locally polar regions in the superconductivity of SrTiO 3

Understanding the interaction between polar and superconducting order parameters may hold the key to several classes of superconductors that remain poorly understood, including SrTiO 3 and several tellurides. Here we show that doped, strained SrTiO 3 films can exhibit both global or local polar order, respectively, depending on the amount of epitaxial mismatch strain, thereby providing a platform to understand how inversion symmetry breaking affects superconductivity. We find that the superconducting critical temperature correlates with the length scale of polar order. In particular, the transition temperature is enhanced when polar nanodomains are sufficiently large or, in the extreme limit, films are globally ferroelectric. In these cases, the Cooper pairs reside in a noncentrosymmetric environment. Conversely, low transition temperatures are found when the nanodomains are small. The findings point to the length scale of polar nanodomains and spin-orbit coupling as important parameters controlling the superconductivity of SrTiO 3 . Furthermore, the ability to control the size of the polar domains opens up new opportunities to design and control the nature of superconductivity in a wide range of materials.

36 MATERIALS SCIENCE↗
DOE OSTI2022

Absence of spin susceptibility decrease in a bulk organic superconductor with triangular lattice

The study of non-s-wave unconventional superconductivities in strongly correlated electron systems has been a central issue in condensed matter physics for more than 30 years. In such unconventional superconductivities, d-wave Cooper pairing with antiparallel spins has been often observed in various quasi-two-dimensional (quasi-2D) bulk systems. Interestingly, many theories predicted that the triangular lattice causes the d-wave pairing to be unstable and may lead to more exotic pairing such as parallel spin (spin-triplet) pairing. Here we focus on a bulk organic triangular-lattice system in which superconductivity emerges near a nonmagnetic Mott insulating phase. We demonstrate, by using low-power nuclear magnetic resonance (NMR) measurements, that the spin susceptibility of the superconducting state retains the normal state value even deep in the superconducting state. This result indicates the possibility that the material exhibits spin-triplet superconductivity. Our finding will bring insights also into understanding the 2D materials with triangular moiré superlattices that are considered also to show unconventional superconductivities near Mott-like insulating states.

36 MATERIALS SCIENCE↗
DOE OSTI2025

Anisotropic field-induced changes in the superconducting order parameter of UTe 2

UTe 2 is a newly discovered unconventional superconductor, where electron Cooper pairs combine into a spin-triplet ground state. We study the specific heat C( H,T ) of a high-quality UTe 2 single crystal, with a single anomaly at a high superconducting transition temperature T c = 2.1 K and a low residual Sommerfeld coefficient γ 0 . Applying magnetic fields up to 12 T along the crystallographic axes a, b , and c , we observe highly anisotropic behavior in γ 0 ( H ). Below 4 T, γ 0 ( H ) ≈ γ 0 + λi √H (i = a, b, c) , which is expected for an unconventional superconductor with nodes on the Fermi surface away from the direction of the magnetic field. At 4 T ( a and b axes) and 5.5 T ( c axis), distinctive changes in the behavior of γ 0 (H) suggest that a stable low-field ground state begins to evolve above 4 T. The data analysis indicates that the nodes are located near the a–b plane, with possible order parameters d B2u + iεd B1u or d B2u + iεd Au . Our findings support B 2u as the primary superconducting order parameter in UTe 2 .

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2025

Robust Nodal Behavior in the Thermal Conductivity of Superconducting UTe 2

The superconducting state of the heavy-fermion metal UTe 2 has attracted considerable interest because of evidence of spin-triplet Cooper pairing and nontrivial topology. Progress on these questions requires identifying the presence or absence of nodes in the superconducting gap function and their dimension. In this article, we report a comprehensive study of the influence of disorder on the thermal transport in the superconducting state of UTe 2 . Through detailed measurements of the magnetic-field dependence of the thermal conductivity in the zero-temperature limit, we obtain clear evidence of the presence of point nodes in the superconducting gap for all samples with transition temperatures ranging from 1.6 to 2.1 K obtained by different synthesis methods, including a refined self-flux method. This robustness implies the presence of symmetry-imposed nodes throughout the range studied, further confirmed via disorder-dependent calculations of the thermal transport in a model with a single pair of nodes. In addition to capturing the temperature dependence of the thermal conductivity up to 𝑇 𝑐 , this model provides some information about the locations of the nodes, suggesting a 𝐵 1⁢𝑢 or 𝐵 2⁢𝑢 symmetry for the superconducting order parameter. Additionally, comparing the new, ultrahigh conductivity samples to older samples reveals a crossover between a low-field and a high-field regime at a single value of the magnetic field in all samples. In the high-field regime, the thermal conductivity at different disorder levels differs from each other by a simple offset, suggesting that some simple principle determines the physics of the mixed state, a fact which may illuminate trends observed in other clean nodal superconductors.

spin-triplet pairing↗
DOE OSTI2026

Tuning of altermagnetism by strain

For all collinear altermagnets, we sort out piezomagnetic free-energy invariants allowed in the nonrelativistic limit and relativistic piezomagnetic invariants bilinear in the Néel vector $\mathbf{L}$ and magnetization $\mathbf{M}$, which include strain-induced Dzyaloshinskii-Moriya interaction. The symmetry-allowed responses are fully determined by the nonrelativistic spin Laue group. In the nonrelativistic limit, two distinct mechanisms are discussed: the band-filling mechanism, which exists in metals and is illustrated using the simple two-dimensional Lieb lattice model, and the temperature-dependent exchange-driven mechanism, which is illustrated using first-principles calculations for transition-metal fluorides. The leading second-order nonrelativistic term in the strain-induced magnetization is also obtained for CrSb. Piezomagnetism due to the strain-induced Dzyaloshinskii-Moriya interaction is calculated from first principles for transition-metal fluorides, MnTe, and CrSb. Finally, we discuss triplet superconducting correlations supported by altermagnets and protected by inversion rather than time-reversal symmetry. We apply the nonrelativistic classification of Cooper pairs to describe the interplay between strain and superconductivity in the two-dimensional Lieb lattice and in bulk rutile structures. Here, we show that triplet superconductivity is, on average, unitary in an unstrained altermagnet, but becomes non-unitary under piezomagnetically active strain.

FOS: Physical sciences↗
DOE OSTI2020

Terahertz lightwave control of non-equilibrium phases and collective modes in multi-band superconductors

A gauge-invariant density matrix approach is presented to describe the non-equilibrium dynamics of multiband superconductors after photo-excitation. The derived gauge-invariant Bloch equations extend the Anderson pseudo-spin precession model by fully incorporating the center-of-mass motion of Cooper pairs. We also describe lightwave propagation effects inside a superconducting film by including the self-consistent interaction of the photo-excited superconducting system with the propagating electromagnetic field inside the superconductor using Maxwell's equations.

Mootz, Martin↗
DOE OSTI2023

Anisotropic superconductivity at KTaO 3 (111) interfaces

A two-dimensional, anisotropic superconductivity was recently found at the KTaO 3 (111) interfaces. The nature of the anisotropic superconducting transition remains a subject of debate. To investigate the origins of the observed behavior, we grew epitaxial KTaO 3 (111)-based heterostructures. We show that the superconductivity is robust against the in-plane magnetic field and violates the Pauli limit. We also show that the Cooper pairs are more resilient when the bias is along [11$\bar{2}$] (I ∥ [11$\bar{2}$]) and the magnetic field is along [1$\bar{1}$0] (B ∥ [1$\bar{1}$0]). We discuss the anisotropic nature of superconductivity in the context of electronic structure, orbital character, and spin texture at the KTaO 3 (111) interfaces. The results point to future opportunities to enhance superconducting transition temperatures and critical fields in crystalline, two-dimensional superconductors with strong spin-orbit coupling.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2025

Observation of anomalous thermal Hall effect in a Kagome superconductor

Broken time-reversal symmetry (TRS) in superconductors can induce not only spontaneous magnetization by the finite angular momentum of Cooper pairs but also the anomalous thermal Hall effects (ATHEs), whose detection has been extremely challenging. Here, we report the successful observation of an ATHE developing below the superconducting transition temperature at zero magnetic field in the kagome-lattice superconductor CsV 3 Sb 5 . This finding is verified by the absence of a signal in a conventional type-II superconductor using the same setup and by ruling out the trapped-vortex effects through micro-Hall array measurements. Both the temperature dependence and the magnitude of the observed anomalous thermal Hall conductivity are quite different from those expected for the quantized thermal edge current of an intrinsic ATHE but consistent with extrinsic impurity-induced ATHEs in chiral superconductivity. Our study of ATHE offers an alternative approach to probe TRS breaking in the superconducting states.

Yoshida, Hiroki [Univ. of Tokyo, Chiba (Japan)] (O↗
DOE OSTI2022

Isospin magnetism and spin-polarized superconductivity in Bernal bilayer graphene

In conventional superconductors, Cooper pairing occurs between electrons of opposite spin. We observe spin-polarized superconductivity in Bernal bilayer graphene when doped to a saddle-point van Hove singularity generated by a large applied perpendicular electric field. We observe a cascade of electrostatic gate-tuned transitions between electronic phases distinguished by their polarization within the isospin space defined by the combination of the spin and momentum-space valley degrees of freedom. Although all of these phases are metallic at zero magnetic field, we observe a transition to a superconducting state at finite magnetic field B ∥ ≈ 150 milliteslas applied parallel to the two-dimensional sheet. Superconductivity occurs near a symmetry-breaking transition and exists exclusively above the B ∥ limit expected of a paramagnetic superconductor with the observed transition critical temperature T C ≈ 30 millikelvins, consistent with a spin-triplet order parameter.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2024

Anomalous normal-state gap in an electron-doped cuprate

In the underdoped n-type cuprate Nd 2-x Ce x CuO 4 , long-range antiferromagnetic order reconstructs the Fermi surface, resulting in a putative antiferromagnetic metal with small Fermi pockets. Using angle-resolved photoemission spectroscopy, here we observe an anomalous energy gap, an order of magnitude smaller than the antiferromagnetic gap, in a wide portion of the underdoped regime and smoothly connecting to the superconducting gap at optimal doping. After considering all the known ordering tendencies in tandem with the phase diagram, we hypothesize that the normal-state gap in the underdoped n-type cuprates originates from Cooper pairing. In conclusion, the high temperature scale of the normal-state gap raises the prospect of engineering higher transition temperatures in the n-type cuprates comparable to those of the p-type cuprates.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2025

High-field superconducting halo in UTe 2

The heavy fermion material UTe 2 is a candidate topological superconductor that exhibits multiple magnetic field–induced superconducting phases. One such phase exists only at fields greater than 40 tesla, a considerable scale given its critical temperature of only 2 K. Here, in this work, we extend measurements of this state with fields outside of the bc crystallographic plane and reveal its core structure: The superconducting phase wraps around the b axis in a halo-like fashion and appears to be stabilized by a field component perpendicular to the magnetic easy axis. This angle dependence points to a multicomponent spin-triplet order parameter with a finite angular momentum of the Cooper pairs. The pairing mechanism remains enigmatic, and UTe 2 ’s specific magnetophilic superconducting tendencies seem incompatible with existing models for field-enhanced superconductivity.

Lewin, Sylvia K. [National Inst. of Standards and ↗
DOE OSTI2020

Self-consistent effective Hamiltonian theory for fermionic many-body systems

Using a separable many-body variational wavefunction, we formulate a self-consistent effective Hamiltonian theory for fermionic many-body system. The theory is applied to the two-dimensional (2D) Hubbard model as an example to demonstrate its capability and computational effectiveness. Most remarkably for the Hubbard model in 2D, a highly unconventional quadruple-fermion non-Cooper pair order parameter is discovered.

Physics↗
DOE OSTI2022

Superconductivity and Local Inversion-Symmetry Breaking

Inversion and time reversal are essential symmetries for the structure of Cooper pairs in superconductors. The loss of one or both leads to modifications to this structure and can change the properties of the superconducting phases in profound ways. Superconductivity in materials lacking inversion symmetry, or noncentrosymmetric materials, has become an important topic. These materials show unusual magnetic and magnetoelectric properties and can host topological superconductivity. Recently, crystal structures with local, but not global, inversion-symmetry breaking have attracted attention. Here, superconductivity can exhibit phenomena not naively expected in centrosymmetric materials. In this review, we first introduce the concept of locally noncentrosymmetric crystals and different material realizations. We then discuss consequences of such local symmetry breaking on the normal state electronic structure and the classification of superconducting order parameters. Finally, we review the expected and, in parts, already observed phenomenology of unconventional superconductivity and possible topological superconducting phases.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗