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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 145 records · Page 8
All sourcesNASA NTRSDOE OSTI
DOE OSTI2018

Photocharging Dynamics in Colloidal CdS Quantum Dots Visualized by Electron Spin Coherence

We use a time-resolved technique with three laser pulses (pump, orientation and probe) to study the photocharging dynamics with picosecond resolution on a long timescale ranging from ps to ms in CdS colloidal quantum dots. The detection is based on measuring the coherent spin dynamics of electrons, allowing us to distinguish the type of carrier in the dot core (electron or hole). We find that although initially negative photocharging happens because of fast hole trapping on surface states, eventually it evolves to positive photocharging due to electron trapping and hole detrapping. The positive photocharging lasts up to hundreds of microseconds at room temperature.

36 MATERIALS SCIENCE↗
DOE OSTI2018

Size-Dependent Optical Properties of Colloidal CdS Quantum Dots Passivated by Thioglycolic Acid

The results of studies of the optical properties of ensembles of colloidal CdS quantum dots passivated by thioglycolic acid are reported. The average dimensions of the quantum dots lie in the range from 1.7 to 5.8 nm. By X-ray diffraction studies and Raman spectroscopy, it is established that quantum dots crystallize with the formation of a cubic crystal lattice. The systematic features of the quantum-confinement effect in the optical absorption and luminescence spectra, as well as in the luminescence excitation spectra, are established. The features manifest themselves as a blue shift of the corresponding bands with decreasing quantum-dot dimensions. From analysis of the nanosecond luminescence kinetics, it is concluded that experimentally observed radiative recombination proceeds by the donor–acceptor mechanism.

36 MATERIALS SCIENCE↗
DOE OSTI2019

On the Processes of the Self-Assembly of CdS Nanocrystal Arrays Formed by the Langmuir–Blodgett Technique

The morphology of CdS nanocrystal arrays self-assembled during the evaporation of a behenic-acid organic matrix on a wetted substrate surface is studied by atomic force microscopy. The dependence of the morphology of nanocrystal arrays on the initial matrix surface is studied. The morphology of nanocrystal arrays noticeably changes from small fractal arrays to a porous submonolayer with an increase in the nanocrystal density. The nature of attractive forces between nanocrystals which prevents their reversible adhesion and ensures their comparatively high mobility in the array composition is proposed.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2017

Defect specific luminescence dead layers in CdS and CdSe

CdS and CdSe are often used in optoelectronic devices whose effectiveness is may be dictated by defects in the near surface region. Luminescence is one of the main tools for studying such defects. The energy dependence of the x-ray excited optical luminescence (XEOL) spectra of these materials enables the extraction of the depth dependence of the defect distribution. Normal and time-gated XEOL spectra were obtained from these materials in the energy range 600 to 1500 eV. Here, we find that the results can best be understood in terms of a luminescence dead layer whose width depends on the position of the defect level in the band gap.

36 MATERIALS SCIENCE↗
NASA NTRS1966

Evaporated and recrystallized CdS layers.

Evaporated and recrystallized CdS layers, discussing electron mobility, level distribution, capture cross section and techniques of measurement

ELECTRON DISTRIBUTION↗
NASA NTRS1966

Multilayer ohmic contacts on CdS.

Multilayer technique for evaporation of ohmic contacts onto CdS, noting V-I characteristics and noise spectrum of recrystallized layer

VOLT-AMPERE CHARACTERISTICS↗