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Assessment of Natural and Anthropogenic Aerosol Air Pollution In the Middle East Using MERRA-2, CAMS Data Assimilation Products, and High-Resolution WRF-Chem Model Simulations

Modern-Era Retrospective analysis for Research and Applications v.2 (MERRA-2), Copernicus Atmosphere Monitoring Service Operational Analysis (CAMS-OA), and a high-resolution regional Weather Research and Forecasting model coupled with chemistry (WRF-Chem) were used to evaluate natural and anthropogenic particulate matter (PM) air pollution in the Middle East (ME) during 2015–2016. Two Moderate Resolution Imaging Spectrometer (MODIS) retrievals – combined product Deep Blue and Deep Target (MODIS-DB&DT) and Multi-Angle Implementation of Atmospheric Correction (MAIAC) – and Aerosol Robotic Network (AERONET) aerosol optical depth (AOD) observations as well as in situ PM measurements for 2016 were used for validation of the WRF-Chem output and both assimilation products. MERRA-2 and CAMS-OA assimilate AOD observations. WRF-Chem is a free-running model, but dust emission in WRF-Chem is tuned to fit AOD and aerosol volume size distributions obtained from AERONET. MERRA-2 was used to construct WRF-Chem initial and boundary conditions both for meteorology and chemical and aerosol species. SO2 emissions in WRF-Chem are based on the novel OMI-HTAP SO2 emission dataset. The correlation with the AERONET AOD is highest for MERRA-2 (0.72–0.91), MAIAC (0.63–0.96), and CAMSOA (0.65–0.87), followed by MODIS-DB&DT (0.56–0.84) and WRF-Chem (0.43–0.85). However, CAMS-OA has a relatively high positive mean bias with respect to AERONET AOD. The spatial distributions of seasonally averaged AODs from WRF-Chem, assimilation products, and MAIAC are well correlated with MODIS-DB&DT AOD product. MAIAC has the highest correlation (R = 0.8), followed by MERRA-2 (R = 0.66), CAMS-OA (R = 0.65), and WRF-Chem (R = 0.61). WRF-Chem, MERRA-2, and MAIAC underestimate and CAMS-OA overestimates MODIS-DB&DT AOD. The simulated and observed PM concentrations might differ by a factor of 2 because it is more challenging for the model and the assimilation products to reproduce PM concentration measured within the city. Although aerosol fields in WRF-Chem and assimilation products are entirely consistent, WRF-Chem is preferable for analysis of regional air quality over the ME due to its higher spatial resolution and better SO2 emissions. The WRF-Chem’s PM background concentrations exceed the World Health Organization (WHO) guidelines over the entire ME. Mineral dust is the major contributor to PM (≈ 75%–95%) compared to other aerosol types. Near and downwind from the SO2 emission sources, non-dust aerosols (primarily sulfate) contribute up to 30% to PM(sub 2.5). The contribution of sea salt to PM in coastal regions can reach 5%. The contributions of organic matter, black carbon and organic carbon to PM over the Middle East are insignificant. In the major cities over the Arabian Peninsula, the 90th percentile of PM(sub 10) and PM(sub 2.5) (particles with diameters less than 10 and 2.5 μm, respectively) daily mean surface concentrations exceed the corresponding Kingdom of Saudi Arabia air quality limits. The contribution of the non-dust component to PM(sub 2.5) is < 25%, which limits the emission control effect on air quality. The mitigation of the dust effect on air quality requires the development of environment-based approaches like growing tree belts around the cities and enhancing in-city vegetation cover. The WRF-Chem configuration presented in this study could be a prototype of a future air quality forecast system that warns the population against air pollution hazards.

Alexander Ukhov↗

Analysis of A Severe Dust Storm and Its Impact on Air Quality Conditions Using Wrf-Chem Modeling, Satellite Imagery, and Ground Observations

This study presents a comprehensive analysis of an extreme dust event recorded in the Arabian Peninsula and the United Arab Emirates (UAE) between 31 March and 3 April 2015. Simulations of the dust event with the Weather Research and Forecasting model coupled with the Chemistry module (WRF-Chem) were analyzed and verified using MSG-SEVIRI imagery and aerosol optical depth (AOD) from the recent 1-km Multi-Angle Implementation of Atmospheric Correction (MAIAC) algorithm for MODIS Terra/Aqua. Data from the National Centers for Atmospheric Prediction/National Center for Atmospheric Research (NCEP/NCAR) and the upper-air radiosonde observations were used to understand the synoptic of the event. In addition, the impact of the event on atmospheric and air quality conditions is investigated. The Air Quality Index (AQI) was calculated prior, during, and after the event to assess the degradation of air quality conditions. Simulated temperature, relative humidity, wind speed, and surface radiation were compared to observations at six monitoring stations in the UAE giving R2 values of 0.84, 0.63, 0.60, and 0.84, respectively. From 1 to 2 April 2015, both observations and simulations showed an average drop in temperature from 33 to 26 °C and radiance reduction from about 950 to 520 Wm−2. The AOD modeled by WRF-Chem showed a good correlation with Aerosol Robotic Network (AERONET) measurements in the UAE with R2 of 0.83. The AQI over the UAE reached hazardous levels during the peak of the dust event before rapidly decreasing to moderate–good air quality levels. This work is the first attempt to demonstrate the potential of using WRF-Chem to estimate AQI over the UAE along with two satellite products (MODIS-MAIAC and MSG-SEVIRI) for dust detection and tracking.

dust storm↗

Harmonized Emissions Component (HEMCO) 3.0 as a Versatile Emissions Component for Atmospheric Models: Application in the GEOS-Chem, NASA GEOS, WRF-GC, CESM2, NOAA GEFS-Aerosol, and NOAA UFS Models

Emissions are a central component of atmospheric chemistry models. The Harmonized Emissions Component (HEMCO) is a software component for computing emissions from a user-selected ensemble of emission inventories and algorithms. It allows users to re-grid, combine, overwrite, subset, and scale emissions from different inventories through a configuration file and with no change to the model source code. The configuration file also maps emissions to model species with appropriate units. HEMCO can operate in offline stand-alone mode, but more importantly it provides an online facility for models to compute emissions at runtime. HEMCO complies with the Earth System Modeling Framework (ESMF) for portability across models. We present a new version here, HEMCO 3.0, that features an improved three-layer architecture to facilitate implementation into any atmospheric model and improved capability for calculating emissions at any model resolution including multiscale and unstructured grids. The three-layer architecture of HEMCO 3.0 includes (1) the Data Input Layer that reads the configuration file and accesses the HEMCO library of emission inventories and other environmental data, (2) the HEMCO Core that computes emissions on the user-selected HEMCO grid, and (3) the Model Interface Layer that re-grids (if needed) and serves the data to the atmospheric model and also serves model data to the HEMCO Core for computing emissions dependent on model state (such as from dust or vegetation). The HEMCO Core is common to the implementation in all models, while the Data Input Layer and the Model Interface Layer are adaptable to the model environment. Default versions of the Data Input Layer and Model Interface Layer enable straightforward implementation of HEMCO in any simple model architecture, and options are available to disable features such as re-gridding that may be done by independent couplers in more complex architectures. The HEMCO library of emission inventories and algorithms is continuously enriched through user contributions so that new inventories can be immediately shared across models. HEMCO can also serve as a general data broker for models to process input data not only for emissions but for any gridded environmental datasets. We describe existing implementations of HEMCO 3.0 in (1) the GEOS-Chem “Classic” chemical transport model with shared-memory infrastructure, (2) the high-performance GEOS-Chem (GCHP) model with distributed-memory architecture, (3) the NASA GEOS Earth System Model (GEOS ESM), (4) the Weather Research and Forecasting model with GEOS-Chem (WRF-GC), (5) the Community Earth System Model Version 2 (CESM2), and (6) the NOAA Global Ensemble Forecast System – Aerosols (GEFS-Aerosols), as well as the planned implementation in the NOAA Unified Forecast System (UFS). Implementation of HEMCO in CESM2 contributes to the Multi-Scale Infrastructure for Chemistry and Aerosols (MUSICA) by providing a common emissions infrastructure to support different simulations of atmospheric chemistry across scales.

Haipeng Lin↗

The impact of Los Angeles Basin pollution and stratospheric intrusions on the surrounding San Gabriel Mountains as seen by surface measurements, lidar, and numerical models

In this work, the impact of Los Angeles Basin pollution transport and stratospheric intrusions on the surface ozone levels observed in the San Gabriel Mountains is investigated based on a combination of surface and lidar measurements as well as WRF-Chem (Weather Research and Forecasting with Chemistry) and WACCM (Whole Atmosphere Community Climate Model) runs. The number of days with observed surface ozone levels exceeding the National Ambient Air Quality Standards exhibit a clear seasonal pattern, with a maximum during summer, when models suggest a minimum influence of stratospheric intrusions and the largest impact from Los Angeles Basin pollution transport. Additionally, measured and modeled surface ozone and PM10 were analyzed as a function of season, time of the day, and wind direction. Measurements and models are in good qualitative agreement, with maximum surface ozone observed for southwest and west winds. For the prevailing summer wind direction, slightly south of the ozone maximum and corresponding to south-southwest winds, lower ozone levels were observed. Back trajectories suggest that this is associated with transport from the central Los Angeles Basin, where titration limits the amount of surface ozone. A quantitative comparison of the lidar profiles with WRF-Chem and WACCM models revealed good agreement near the surface, with models showing an increasing positive bias as function of altitude, reaching 75 % at 15 km above sea level. Finally, three selected case studies covering the different mechanisms affecting the near-surface ozone concentration over the San Gabriel Mountains, namely stratospheric intrusions and pollution transport, are analyzed based on surface and ozone lidar measurements, as well as co-located ceilometer measurements and models.

Impact↗

Cold Season Performance of the NU-WRF Regional Climate Model in the Great Lakes Region

As Earth’s largest collection of freshwater, the Laurentian Great Lakes have enormous ecological and socio-economic value. Their basin has become a regional hotspot of climatic and limnological change, potentially threatening its vital natural resources. Consequentially, there is a need to assess the current state of climate models regarding their performance across the Great Lakes region and develop the next generation of high-resolution regional climate models to address complex limnological processes and lake-atmosphere interactions. In response to this need, the current paper focuses on the generation and analysis of a 20-member ensemble of 3-km National Aeronautics and Space Administration (NASA)-Unified Weather Research and Forecasting (NU-WRF) simulations for the 2014-2015 cold season. The study aims to identify the model’s strengths and weaknesses; optimal configuration for the region; and the impacts of different physics parameterizations, coupling to a 1D lake model, time-variant lake-surface temperatures, and spectral nudging. Several key biases are identified in the cold-season simulations for the Great Lakes region, including an atmospheric cold bias that is amplified by coupling to a 1D lake model but diminished by applying the Community Atmosphere Model radiation scheme and Morrison microphysics scheme; an excess precipitation bias; anomalously early initiation of fall lake turnover and subsequent cold lake bias; excessive and overly persistent lake ice cover; and insufficient evaporation over Lakes Superior and Huron. The research team is currently addressing these key limitations by coupling NU-WRF to a 3D lake model in support of the next generation of regional climate models for the critical Great Lakes Basin.

Michael Notaro↗

An Evaluation of NOAA-20 ATMS Instrument Pre-Launch and On-Orbit Performance Characterization

Passive microwave sounders provide the highest-impact observations ingested by major numerical weather prediction (NWP) forecast models. The Advanced Technology Microwave Sounder (ATMS), built by Northrop Grumman, Azusa, CA, USA, is the latest operational microwave sounder series being launched by the United States to provide both temperature and water vapor soundings of the atmosphere. The first ATMS was launched on the Suomi National Polarorbiting Partnership (SNPP) satellite in 2011. This article focuses on the details of the on-orbit performance characterization of the second ATMS, which launched on November 18, 2017, on the Joint Polar Satellite System-1 (JPSS-1) satellite. After successful commissioning, JPSS-1 was renamed National Oceanic and Atmospheric Administration (NOAA)-20 (N-20). We present performance characterizations from prelaunch and postlaunch tests, including the thermal vacuum (TVAC) campaign, and postlaunch activities that contribute to the radiance data products. Significant improvements were found for reflector emissivity, 1/ f noise performance, antenna beam efficiency, inter-channel noise correlation, and scan drive bearing design. New geolocation and pointing algorithms were evaluated. The N-20 ATMS has the same channel set, polarizations, scan geometry, and calibration approach as the SNPP ATMS. The N-20 ATMS meets all performance requirements with margin.

Advanced Technology Microwave Sounder (ATMS)↗

Evaluating Meteorological Dust Events and Machine-Learning Based Dust Identification in Geostationary Satellite Imagery

NASA scientists in the Short-term Prediction Research and Transition Center (SPoRT) developed a physically-based machine learning approach to identify dust in satellite imagery with a focus on night-time dust detection (Berndt et al. 201; DustTracker-AI). NASA/NOAA Geostationary Environmental Operational Satellite-16 (GOES-16) imagery was used for training and model inputs. The training, testing and validation data set consists of 28 events in the Southwest United States, capturing dust and null events in the region from 2018-2020.With 83 distinct images and millions of pixels a random forest model was trained and validated, correctly labeling 85% of dust pixels.For the first time, the model was run in near-real time production during the spring of 2022 and dust probability visualizations were made available to NOAA National Weather Service (NWS) forecasters to assess its utility for dust forecasting. Results indicated the model helped increase the confidence in the presence of dust and enabled dust tracking for a longer period of time into the night-time hours. Forecaster assessment and running the model in near real-time allowed for the team to determine the types of events missed, captured, and false alarms. To gain additional context on model performance,the SPoRT team sought to gather more detailed information on the training database(e.g., meteorological characteristics and drivers). The goal of this project was to identify the meteorological drivers for the dust events and create a database which synthesized information from observations, forecaster discussions, and analyses pertaining to the dust events to understand the types of events currently used to train the model. A more detailed meteorological synopsis was created for each dust event in the training, testing, and validation datasets. Following the completion of the database and documentation, the classification details revealed that 88% of the dust events were synoptically driven while mesoscale events were less prevalent in model datasets. Meteorological conditions found such as mixing layer depth and wind velocity had mean values of 645mb and 21kt respectively.With conditions of deep mixed layers and moderate to strong surface winds a mesoscale thunderstorm outflow event was considered and subsequently added to the model training data set to test the impact of additional mesoscale training data. The model was retrained and then qualitatively tested on a sample thunderstorm outflow case that the original model was unable to identify. Preliminary results showed potential that the addition of more mesoscale events included in the training data could help to better identify indistinct and localized dust events.

Connor Welch↗

Improving Multiday Solar Wind Speed Forecasts

We analyze the residual errors for the Wang-Sheeley-Arge (WSA) solar wind speed forecasts as a function of the photospheric magnetic field expansion factor (fp) and the minimum separation angle (d) in the photosphere between the footpoints of open field lines and the nearest coronal hole boundary. We find the map of residual speed errors are systematic when examined as a function of fp and d. We use these residual error maps to apply corrections to the model speeds. We test this correction approach using 3-day lead time speed forecasts for an entire year of observations and model results. Our methods can readily be applied to develop corrections for the remaining WSA forecast lead times which range from 1 to 7 days in 1-day increments. Since the solar wind density, temperature, and the interplanetary magnetic field strength all correlate well with the solar wind speed, the improved accuracy of solar wind speed forecasts enables the production of multiday forecasts of the solar wind density, temperature, pressure, and interplanetary field strength, and geophysical indices. These additional parameters would expand the usefulness of Air Force Data Assimilative Photospheric Flux Transport-WSA forecasts for space weather clients.

H A Elliot↗

Tracking the Impacts of Precipitation Phase Changes Through the Hydrologic Cycle in Snowy Regions: From Precipitation to Reservoir Storage

Cool season precipitation plays a critical role in regional water resource management in the western United States. Throughout the twenty-first century, regional precipitation will be impacted by rising temperatures and changing circulation patterns. Changes to precipitation magnitude remain challenging to project; however, precipitation phase is largely dependent on temperature, and temperature predictions from global climate models are generally in agreement. To understand the implications of this dependence, we investigate projected patterns in changing precipitation phase for mountain areas of the western United States over the twenty-first century and how shifts from snow to rain may impact runoff. We downscale two bias-corrected global climate models for historical and end-century decades with the Weather Research and Forecasting (WRF) regional climate model to estimate precipitation phase and spatial patterns at high spatial resolution (9 km). For future decades, we use the RCP 8.5 scenario, which may be considered a very high baseline emissions scenario to quantify snow season differences over major mountain chains in the western U.S. Under this scenario, the average annual snowfall fraction over the Sierra Nevada decreases by >45% by the end of the century. In contrast, for the colder Rocky Mountains, the snowfall fraction decreases by 29%. Streamflow peaks in basins draining the Sierra Nevada are projected to arrive nearly a month earlier by the end of the century. By coupling WRF with a water resources model, we estimate that California reservoirs will shift towards earlier maximum storage by 1–2 months, suggesting that water management strategies will need to adapt to changes in streamflow magnitude and timing.

Melissa L. Wrzesien↗

Parameter Dependencies of Early-Stage Tangential Discontinuity-Driven Foreshock Bubbles in Local Hybrid Simulations

Foreshock bubbles (FBs) are significant foreshock transients that can accelerate particles and disturb the magnetosphere-ionosphere system. In the kinetic formation model, foreshock ions interact with the discontinuity by performing partial gyrations to generate currents that change the magnetic field topology around the discontinuity. However, how different foreshock ion properties affect the growth of the field variations is not well understood. Therefore, we use 2-D local hybrid simulations to study the effects of different foreshock ion distributions and properties on the growth of tangential discontinuity (TD)-driven FBs. We discover that for a gyrophase-bunched distribution with an initial phase where the guiding center is on the other side of the TD, the foreshock ions gyrate together across the TD, causing more foreshock ions to cross the TD and leading to a faster expansion of the structure than for a Maxwellian distribution. A ring distribution also yields higher expansion speeds because of the higher projected velocity into the new perpendicular direction. For Maxwellian distributions, there are positive and linear correlations of the FB expansion speeds with the initial foreshock ion densities, thermal speeds, parallel speeds, and sine of the TD magnetic shear angles. These parameter dependencies grow in strength as the structures evolve with time. The foreshock ion distributions and properties that lead to stronger currents produce more significant magnetic field variations and higher expansion speeds. Our study helps quantify the formation and expansion of FBs to forecast their space weather effects and contribution to shock acceleration.

Andrew Vu↗

Impact of Meteorological Factors on the Mesoscale Morphology of Cloud Streets during a Cold-Air Outbreak over the Western North Atlantic

Postfrontal clouds (PFC) are ubiquitous in the marine boundary layer, and their morphology is essential to estimating the radiation budget in weather and climate models. Here we examine the roles of sea surface temperature (SST) and meteorological factors in controlling the mesoscale morphology and evolution of shallow clouds associated with a cold-air outbreak that occurred on 1 March 2020 during phase I of the Aerosol Cloud Meteorology Interactions over the Western Atlantic Experiment (ACTIVATE). Our results show that the simulated PFC structure and ambient conditions by the Weather Research and Forecasting (WRF) Model are generally consistent with observations from GOES-16 and dropsonde measurements. We also examine the thermodynamical and dynamical influences in the cloud mesoscale morphology using WRF sensitivity experiments driven by two meteorological forcing datasets with different domain-mean SST and spatial gradients, which lead to dissimilar values of hydrometeor water path and cloud core fraction. The SST from ERA5 leads to weaker stability and higher inversion height than the SST from FNL does. In addition, the use of large-scale meteorological forcings from ERA5 yields a distinctive time evolution of wind direction shear in the inner domain, which favors the formation and persistence of longer cloud rolls. Both factors contribute to a change in the time evolution of domain-mean water path and cloud core fraction of cloud streets. Our study takes advantage of the simulation driven by the differences between two large-scale forcing datasets to illustrate the importance of SST and wind direction shear in the cloud street morphology in a realistic scenario

Jingyi Chen↗

Ensemble Forecasting/Assimilation/Emissions Estimation with WRF-Chem/DART: Accomplishments, Lessons Learned, and Future Plans

Over the past ten years, we have been conducting research on regional ensemble atmospheric composition forecasting/data assimilation/emissions estimation with WRF-Chem/DART. WRF- Chem/DART integrates the Weather Research and Forecasting model (WRF) with online chemistry (WRF-Chem) into the Data Assimilation Research Testbed (DART). DART is an ensemble data assimilation system based on the ensemble adjustment Kalman filter (EAKF) with adaptive inflation, localization (physical and state space), and an optional non-Gaussian formulation of the EAKF. DART includes assimilation of meteorological and limited chemical observations. WRF-Chem/DART extends DART to include assimilation of: MOPITT CO; IASI CO and O3; MODIS AOD; OMI O3, NO2, and SO2; TROPOMI CO, O3, NO2, and SO2, TES CO, CO2 (research mode), O3, NH3, and CH4 (research mode); CrIS CO, O3, NH3, CH4 (research mode), and PAN; SCIAMACHY NO2; GOME2a NO2; MLS O3 and HNO3; and proxy TEMPO O3, and NO2 satellite retrievals as raw retrievals or as ‘compact phase space retrievals’ (CPSRs) for profile retrievals. WRF-Chem/DART also assimilates in situ atmospheric composition measurements and uses the ‘state augmentation method’ for emissions estimation. In our presentation, we will provide an overview of WRF-Chem/DART: • applications and results; • lessons learned from: (i) independent versus joint assimilation; (ii) total/partial column versus profile retrieval assimilation; (iii) joint in situ and retrieval assimilation; (iv) assimilation at grid resolutions ranging from 100 km to 4 km; (v) dynamic emissions estimation; and • future work related to wildfire emissions estimation and intercomparison of CMAQ (online)/JEDI and CMAQ (online and offline)/DART.

WRF-Chem/DART↗

Lightning Over Central Canada: Skill Assessment for Various Land-Atmosphere Model Configurations and Lightning Indices Over a Boreal Study Area

Current lightning predictions are uncertain because they rely on empirical diagnostic relationships and often use coarse-scale climate scenario simulations in which deep convection is parameterized. Previous studies demonstrated that simulations with convection permitting resolutions improve lightning predictions compared to coarser-grid simulations using convection parameterizations for different geographical locations but not over the boreal zone. In this study, lightning simulations with the NASA Unified-Weather Research and Forecasting (NU-WRF) model are evaluated over a domain including the Great Slave Lake in Canada, for six lightning seasons. The simulations are performed at convection parameterized (9 km) and convection-permitting (3 km) resolution using the Goddard 4ICE and the Thompson microphysics schemes. Four lightning indices are evaluated against observations from the Canadian Lightning Detection Network, in terms of spatiotemporal frequency distribution, spatial pattern, daily climatology, and an event-based overall skill assessment. The Thompson scheme is, regardless of the spatial resolution, superior to the Goddard 4ICE scheme in predicting daily climatology but worse in predicting the spatial patterns of lightning occurrence. Results indicate that lightning estimation benefits from modeling at convection-permitting resolution, in particular for the ice based lightning indices. In contrast, the product of convective available potential energy and precipitation rate proved to be the most robust index that was largely invariant to varying spatial resolution. Finally, this study reveals issues of the models to reproduce the observed spatial pattern of lightning well, which might be related to an insufficient representation of land surface heterogeneity, including peatlands, in the study area.

Jonas Mortelmans↗

Emissions Characterization and Smoke Transport of A Prescribed Fire

Under the background of climate change, vast regions of the world will face a hotter and probably drier future that favors ignition and spread of wildfires. This poses additional challenges to the communities who are fighting the ever-larger wildfires. Fire and smoke models are valuable tools to fire managers and decision-makers to mitigate the impact of fires. Existing fire modeling systems bear large uncertainties due to the difficulty in collecting data to characterize fire behavior and smoke transport. More observations are urgently needed for improvement of fire modeling and reduction in model uncertainty. The coordinated prescribed burn experiment, such as the Fire and Smoke Model and Measurement Evaluation Experiment (FSMMEE), will allow the concurrent collection of critical measurements of fuel, fire behavior, smoke, and meteorology to better understand and model fires. In this preliminary investigation, we employed the data from the prescribed burn experiment at Langdon Mountain, Utah, in November 2019, to reconstruct the fire emissions and characterize the smoke transport. The NASA Unified Weather Research and Forecasting Model (NU-WRF) was utilized to assist in identifying the potential pre-fire remote sensing capabilities, such as fuel load, moisture, and fire radiative power, which are helpful to model development and advancement. Along the way, two sets of NU-WRF experiments would be done by applying either a default fire emissions inventory (i.e., NASA’s Quick Fire Emissions Dataset, QFED) or reconstructed fire emissions using the data collected from the prescribed fire. The results would help answer the questions such as “How do reconstructed emissions compare to QFED emissions and their impact on plume transport”.

NU-WRF↗

High-Resolution Mapping of Nitrogen Oxide Emissions in Large US Cities From TROPOMI Retrievals of Tropospheric Nitrogen Dioxide Columns

Satellite-derived spatiotemporal patterns of nitrogen oxide (NO x ) emissions can improve accuracy of emission inventories to better support air quality and climate research and policy studies. In this study, we develop a new method by coupling the chemical transport Model-Independent SATellite-derived Emission estimation Algorithm for Mixed-sources (MISATEAM) with a divergence method to map high-resolution NO x emissions across US cities using TROPOspheric Monitoring Instrument (TROPOMI) tropospheric nitrogen dioxide (NO 2 ) retrievals. The accuracy of the coupled method is validated through application to synthetic NO 2 observations from the NASA-Unified Weather Research and Forecasting (NU-WRF) model, with a horizontal spatial resolution of 4 km × 4 km for 33 large and mid-size US cities. Validation reveals excellent agreement between inferred and NU-WRF-provided emission magnitudes (R= 0.99, normalized mean bias, NMB = −0.01) and a consistent spatial pattern when comparing emissions for individual grid cells (R=0.88 ± 0.06). We then develop a TROPOMI-based database reporting annual emissions for 39 US cities at a horizontal spatial resolution of 0.05° × 0.05° from 2018 to 2021. This database demonstrates a strong correlation (R= 0.90) with the National Emission Inventory (NEI) but reveals some bias (NMB = −0.24). There are noticeable differences in the spatial patterns of emissions in some cities. Our analysis suggests that uncertainties in TROPOMI-based emissions and potential misallocation of emissions and/or missing sources in bottom-up emission inventories both contribute to these differences.

NOx emissions↗

Enabling the Assimilation of CrIS Shortwave Infrared Observations in Global NWP at NOAA. Part I: Background and Methods

Radiance observations from Earth-observing satellites have a significant positive impact on numerical weather prediction (NWP) forecasts, but some spectral regions are not fully exploited. Observations from hyperspectral infrared (IR) sounders in the longwave region (650-1100 cm -1 ), for instance, are routinely assimilated in many NWP models, but observations in the shortwave region (2155-2550 cm -1 ) are not. Each of these regions provides information on the temperature structure of the atmosphere, but the shortwave IR (SWIR) region is considered challenging to assimilate due to noise equivalent delta temperature (NEDT) that is highly variable depending on scene brightness temperature and to phenomena that are difficult to model, like non-Local Thermodynamic Equilibrium (NLTE) and solar reflectance. With recent advances in small-satellite technology, SWIR temperature sounders may provide an agile and cost-effective complement to the current constellation of IR sounders. Therefore, a better understanding of the use and impact of SWIR observations in data assimilation for NWP is warranted. In part one of this study, as presented here, the amount of unique information (as determined by Empirical Orthogonal Decomposition (EOD)) made available to a data assimilation system by Cross-track Infrared Sounder (CrIS) SWIR observations is reviewed, recent advancements to the Community Radiative Transfer Model (CRTM) for the simulation of CrIS shortwave radiances are tested, and enhancements to NOAA’s Global Data Assimilation System (GDAS) for the assimilation of CrIS SWIR observations are implemented and evaluated. Part two of this study, which seeks to assess the value of assimilating shortwave IR observations in global NWP, is also introduced.

Erin Jones↗

Automatic Detection of Large-scale Flux Ropes and Their Geoeffectiveness with a Machine-learning Approach

Detecting large-scale flux ropes (FRs) embedded in interplanetary coronal mass ejections (ICMEs) and assessing their geoeffectiveness are essential, since they can drive severe space weather. At 1 au, these FRs have an average duration of 1 day. Their most common magnetic features are large, smoothly rotating magnetic fields. Their manual detection has become a relatively common practice over decades, although visual detection can be time-consuming and subject to observer bias. Our study proposes a pipeline that utilizes two supervised binary classification machine-learning models trained with solar wind magnetic properties to automatically detect large-scale FRs and additionally determine their geoeffectiveness. The first model is used to generate a list of autodetected FRs. Using the properties of the southward magnetic field, the second model determines the geoeffectiveness of FRs. Our method identifies 88.6% and 80% of large-scale ICMEs (duration 1day) observed at 1au by the Wind and the Solar TErrestrial RElations Observatory missions, respectively. While testing with continuous solar wind data obtained from Wind, our pipeline detected 56 of the 64 large-scale ICMEs during the 2008–2014 period (recall = 0.875), but also many false positives (precision = 0.56), as we do not take into account any additional solar wind properties other than the magnetic properties. We find an accuracy of 0.88 when estimating the geoeffectiveness of the autodetected FRs using our method. Thus, in space-weather nowcasting and forecasting at L1 or any planetary missions, our pipeline can be utilized to offer a first-order detection of large-scale FRs and their geoeffectiveness.

Sanchita Pal↗

NASA GSFC Space Weather Center - Innovative Space Weather Dissemination: Web-Interfaces, Mobile Applications, and More

The NASA GSFC Space Weather Center (http://swc.gsfc.nasa.gov) is committed to providing forecasts, alerts, research, and educational support to address NASA's space weather needs - in addition to the needs of the general space weather community. We provide a host of services including spacecraft anomaly resolution, historical impact analysis, real-time monitoring and forecasting, custom space weather alerts and products, weekly summaries and reports, and most recently - video casts. There are many challenges in providing accurate descriptions of past, present, and expected space weather events - and the Space Weather Center at NASA GSFC employs several innovative solutions to provide access to a comprehensive collection of both observational data, as well as space weather model/simulation data. We'll describe the challenges we've faced with managing hundreds of data streams, running models in real-time, data storage, and data dissemination. We'll also highlight several systems and tools that are utilized by the Space Weather Center in our daily operations, all of which are available to the general community as well. These systems and services include a web-based application called the Integrated Space Weather Analysis System (iSWA http://iswa.gsfc.nasa.gov), two mobile space weather applications for both IOS and Android devices, an external API for web-service style access to data, google earth compatible data products, and a downloadable client-based visualization tool.

Maddox, Marlo↗