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All sourcesNASA NTRSDOE OSTI
DOE OSTI2024

Improving Fission Products at CARIBU: Near Field Detection (Q1/FY24 Quarterly Progress Report)

The article on “Direct Mass Measurements to Inform the Behavior for 128mSb in Nucleosynthesis Environments” by Daniel Hoff et al., recently published in Physical Review Letters. The results of the work are a combination of an extraordinary work on precision mass measurements performed with the Canadian Penning Trap at ANL (the most precise mass measurement of the ground state and the isomeric state in 128Sb performed to date), and an extensive nucleosynthesis theory calculation that include isomers performed by the theorists at LANL.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
NASA NTRS1992

Negative-ion formation in the explosives RDX, PETN, and TNT using the Reversal Electron Attachment Detection (READ) technique

In the search for high sensitivity and direct atmospheric sampling of trace species, techniques have been developed such as atmospheric-sampling, glow-discharge ionization (ASGDI), corona discharge, atmospheric pressure ionization (API), electron-capture detection (ECD), and negative-ion chemical ionization (NICI) that are capable of detecting parts-per-billion to parts-per-trillion concentrations of trace species. These techniques are based on positive- or negative-ion formation via charge-transfer to the target, or electron capture under multiple-collision conditions in a Maxwellian distribution of electron energies at the source temperature. One drawback of the high-pressure, corona- or glow-discharge devices is that they are susceptible to interferences either through indistinguishable product masses, or through undesired ion-molecule reactions. The ASGDI technique is relatively immune from such interferences, since at target concentrations of less than 1 ppm the majority of negative ions arises via electron capture rather than through ion-molecule chemistry. A drawback of the conventional ECD, and possibly of the ASGDI, is that they exhibit vanishingly small densities of electrons with energies in the range 0-10 millielectron volts (meV), as can be seen from a typical Maxwellian electron energy distribution function at T = 300 K. Slowing the electrons to these subthermal (less than 10 meV) energies is crucial, since the cross section for attachment of several large classes of molecules is known to increase to values larger than 10(exp -12) sq cm at near-zero electron energies. In the limit of zero energy these cross sections are predicted to diverge as epsilon(exp -1/2), where epsilon is the electron energy. In order to provide a better 'match' between the electron energy distribution function and attachment cross section, a new concept of attachment in an electrostatic mirror was developed. In this scheme, electrons are brought to a momentary halt by reversing their direction with electrostatic fields. At this turning point the electrons have zero or near-zero energy. A beam of target molecules is introduced, and the resultant negative ions extracted. This basic idea has been recently improved to allow for better reversal geometry, higher electron currents, lower backgrounds, and increased negative-ion extraction efficiency. We present herein application of the so-called reversal electron attachment detector (READ) to the study of negative-ion formation in the explosives molecules RDX, PETN, and TNT under single-collision conditions.

Chutijian, Ara↗
DOE OSTI2020

Solvent Hold Tank Sample Results for MCU-19-366- 367-368 (April 2019), MCU-19-469-470-471 (May 2019), MCU-19-524-525-526 (June 2019): Quarterly Report

A trend summary of three sets of Solvent Hold Tank (SHT) monthly samples MCU-19-366-367-368 (April), MCU-19-469-470-471 (May), and MCU-19-524-525-526 (June) are reported. Most of the conclusions are based on the June SHT sample (MCU-19-524-525-526). Analyses of the June SHT sample (MCU-19-524- 525-526) indicated that the Modifier (Cs-7SB) and the Extractant (MaxCalix) concentrations were below their nominal recommended concentrations (169,000 mg/L and 46,900 mg/L respectively) by 4% and 2% respectively but consistent with previously observed levels during normal runs. The Suppressor (N,N’,N”– tris(3,7-dimethyloctyl)guanidine or TiDG) concentration has decreased since the March 2019 measurement to 793 mg/L, which is above the minimum recommended concentration (479 mg/L). The Semi-Volatile Organic Analysis (SVOA) did not detect any impurities. However, the Fourier Transform Hydrogen Nuclear Magnetic Resonance (FT-HNMR) analysis detected presence of phthalates at a few ppm. The impurity concentration was highest in the April sample and consistently detected in the May and June samples (but always registered as a few ppm or less). Another impurity observed in the samples was mercury. Based on the June SHT sample, up to 25 ± 5 micrograms of mercury per mL of solvent was detected (as the average of the Direct Mercury Analysis (DMA) and X-Ray Fluorescence (XRF) methods). The higher mercury concentration in the solvent (as determined in the last three-monthly samples) is possibly due to the higher mercury concentration in Salt Batches 9 and 10. The gamma concentration (~2.90E4 dpm/mL) measured in the June 2019 SHT samples was consistent with previous values observed when the Modular Caustic-Side Solvent Extraction Unit (MCU) was operating continuously (for example, between December 2016 and January 2017). Statistical analysis of the different analytical methods detected a bias between the FT-HNMR and the High Performance Liquid Chromatography (HPLC) methods when measuring the MaxCalix and Modifier concentrations; the FT-HNMR gave a higher concentration possibly due to peak overlapping in the measured data. A bias was detected when measuring total mercury by the DMA method versus the XRF method with the XRF method reported higher mercury concentrations. The laboratory will continue to monitor the quality of the solvent for any new impurities or degradation of the solvent components.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗
NASA NTRS2008

RACER: Effective Race Detection Using AspectJ

The limits of coding with joint constraints on detected and undetected error rates Programming errors occur frequently in large software systems, and even more so if these systems are concurrent. In the past, researchers have developed specialized programs to aid programmers detecting concurrent programming errors such as deadlocks, livelocks, starvation and data races. In this work we propose a language extension to the aspect-oriented programming language AspectJ, in the form of three new built-in pointcuts, lock(), unlock() and may be Shared(), which allow programmers to monitor program events where locks are granted or handed back, and where values are accessed that may be shared amongst multiple Java threads. We decide thread-locality using a static thread-local objects analysis developed by others. Using the three new primitive pointcuts, researchers can directly implement efficient monitoring algorithms to detect concurrent programming errors online. As an example, we expose a new algorithm which we call RACER, an adoption of the well-known ERASER algorithm to the memory model of Java. We implemented the new pointcuts as an extension to the Aspect Bench Compiler, implemented the RACER algorithm using this language extension and then applied the algorithm to the NASA K9 Rover Executive. Our experiments proved our implementation very effective. In the Rover Executive RACER finds 70 data races. Only one of these races was previously known.We further applied the algorithm to two other multi-threaded programs written by Computer Science researchers, in which we found races as well.

data analysis↗
NASA NTRS2005

First Light from Extrasolar Planets and Implications for Astrobiology

The first light from an extrasolar planet was recently detected. These results, obtained for two transiting extrasolar planets at different infrared wavelengths, open a new era in the field of extrasolar planet detection and characterization because for the first time we can now detect planets beyond the solar system directly. Using the Spitzer Space Telescope at 24 microns, we observed the modulation of combined light (star plus planet) from the HD 209458 system as the planet disappeared behind the star during secondary eclipse and later re-emerged, thereby isolating the light from the planet. We obtained a planet-to-star ratio of 0.26% at 24 microns, corresponding to a brightness temperature of 1130 + / - 150 K. We will describe this result in detail, explain what it can tell us about the atmosphere of HD 209458 b, and discuss implications for the field of astrobiology. These results represent a significant step on the path to detecting terrestrial planets around other stars and in understanding their atmospheres in terms of composition and temperature.

Richardson, L. Jeremy↗
NASA NTRS1988

The distribution of IRAS galaxies towards the Bootes void

A redshift survey was completed for 342 galaxies detected by the IRAS in the direction of the Bootes void discovered by Kirshner et al. The number density of IRAS galaxies is well determined from the shallower full-sky redshift survey of Strauss et al. Four IRAS galaxies are found within the void as defined by Kirshner et al., of which three are part of a complete sample, implying a density depression of a factor of 4. The underdense region continues to a distance of at least 4000 km/s from the nominal center of the void. Three of the IRAS galaxies studied in this paper were previously unknown. These galaxies have emission-line spectra characteristic of H II regions, and red continuum magnitudes ranging from 16 to 17.5 mag, and thus are bright enough to have been detected in a wide-angle redshift survey as deep as that of Kirshner et al. The luminosity function derived from this sample is in good agreement with that of Lawrence et al.

Strauss, Michael A.↗
DOE OSTI2024

Single-atom materials boosting wearable orthogonal uric acid detection

Abstract Uric acid (UA) is a vital biomarker for the diagnosis and management of various health conditions, including cardiovascular diseases, gout, kidney disorders, metabolic syndrome, and wound healing. Despite significant advances in wearable sensor technology, challenges persist in developing wearable sensors that are capable of maintaining high sensitivity, selectivity, and stability. In this study, we present an epidermal sensing platform enhanced with single-atom materials (SAMs) designed for flexible and orthogonal electrochemical detection of UA. We designed and synthesized an SAM with Fe-N 5 active sites to boost the electrochemical sensing signals, integrating it with laser-engraved graphene (LEG) to fabricate a wearable SAM-based UA patch sensor. This design provides superior UA detection performance compared to sensors based on conventional nanomaterials. In addition, we enhanced the detection accuracy and range by using an orthogonal approach that combines direct oxidation through differential pulse voltammetry (DPV) along with parallel biocatalytic amperometric detection. The resulting SAM-based UA orthogonal sensor patch demonstrated exceptional performance in wearable applications through tests measuring sweat UA levels in subjects before and after consuming a purine-rich diet. Graphical Abstract

Ding, Shichao↗
DOE OSTI2022

High-Fidelity Ion State Detection Using Trap-Integrated Avalanche Photodiodes

Integrated technologies greatly enhance the prospects for practical quantum information processing and sensing devices based on trapped ions. High-speed and high-fidelity ion state readout is critical for any such application. Integrated detectors offer significant advantages for system portability and can also greatly facilitate parallel operations if a separate detector can be incorporated at each ion-trapping location. Here, we demonstrate ion quantum state detection at room temperature utilizing single-photon avalanche diodes (SPADs) integrated directly into the substrate of silicon ion trapping chips. Furthermore, we detect the state of a trapped Sr + ion via fluorescence collection with the SPAD, achieving 99.92(1)% average fidelity in 450 μs, opening the door to the application of integrated state detection to quantum computing and sensing utilizing arrays of trapped ions.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
NASA NTRS2012

On Advanced Estimation Techniques for Exoplanet Detection and Characterization using Ground-based Coronagraphs

The direct imaging of planets around nearby stars is exceedingly difficult. Only about 14 exoplanets have been imaged to date that have masses less than 13 times that of Jupiter. The next generation of planet-finding coronagraphs, including VLT-SPHERE, the Gemini Planet Imager, Palomar P1640, and Subaru HiCIAO have predicted contrast performance of roughly a thousand times less than would be needed to detect Earth-like planets. In this paper we review the state of the art in exoplanet imaging, most notably the method of Locally Optimized Combination of Images (LOCI), and we investigate the potential of improving the detectability of faint exoplanets through the use of advanced statistical methods based on the concepts of the ideal observer and the Hotelling observer. We propose a formal comparison of techniques using a blind data challenge with an evaluation of performance using the Receiver Operating Characteristic (ROC) and Localization ROC (LROC) curves. We place particular emphasis on the understanding and modeling of realistic sources of measurement noise in ground-based AO-corrected coronagraphs. The work reported in this paper is the result of interactions between the co-authors during a week-long workshop on exoplanet imaging that was held in Squaw Valley, California, in March of 2012

coronagraphs↗
NASA NTRS2012

On Advanced Estimation Techniques for Exoplanet Detection and Characterization using Ground-Based Coronagraphs

The direct imaging of planets around nearby stars is exceedingly difficult. Only about 14 exoplanets have been imaged to date that have masses less than 13 times that of Jupiter. The next generation of planet-finding coronagraphs, including VLT-SPHERE, the Gemini Planet Imager, Palomar P1640, and Subaru HiCIAO have predicted contrast performance of roughly a thousand times less than would be needed to detect Earth-like planets. In this paper we review the state of the art in exoplanet imaging, most notably the method of Locally Optimized Combination of Images (LOCI), and we investigate the potential of improving the detectability of faint exoplanets through the use of advanced statistical methods based on the concepts of the ideal observer and the Hotelling observer. We provide a formal comparison of techniques through a blind data challenge and evaluate performance using the Receiver Operating Characteristic (ROC) and Localization ROC (LROC) curves. We place particular emphasis on the understanding and modeling of realistic sources of measurement noise in ground-based AO-corrected coronagraphs. The work reported in this paper is the result of interactions between the co-authors during a week-long workshop on exoplanet imaging that was held in Squaw Valley, California, in March of 2012.

instrumentation↗
NASA NTRS2012

The Origin and Evolution of Saturn's 2011-2012 Stratospheric Vortex

The planet-encircling springtime storm in Saturn's troposphere (December 2010-July 2011, Fletcher, L.N. et al. [2011]. Science 332, 1413-1414; Sánchez-Lavega, A. et al. [2011]. Nature 475, 71-74; Fischer, G. et al. [2011]. Nature 475, 75-77) produced dramatic perturbations to stratospheric temperatures, winds and composition at mbar pressures that persisted long after the tropospheric disturbance had abated. Thermal infrared (IR) spectroscopy from the Cassini Composite Infrared Spectrometer (CIRS), supported by ground-based IR imaging from the VISIR instrument on the Very Large Telescope and the MIRSI instrument on NASA's IRTF, is used to track the evolution of a large, hot stratospheric anticyclone between January 2011 and March 2012. The evolutionary sequence can be divided into three phases: (I) the formation and intensification of two distinct warm airmasses near 0.5 mbar between 25 and 35degN (B1 and B2) between January-April 2011, moving westward with different zonal velocities, B1 residing directly above the convective tropospheric storm head; (II) the merging of the warm airmasses to form the large single 'stratospheric beacon' near 40degN (B0) between April and June 2011, disassociated from the storm head and at a higher pressure (2 mbar) than the original beacons, a downward shift of 1.4 scale heights (approximately 85 km) post-merger; and (III) the mature phase characterised by slow cooling (0.11 +/- 0.01 K/day) and longitudinal shrinkage of the anticyclone since July 2011. Peak temperatures of 221.6 +/- 1.4 K at 2 mbar were measured on May 5th 2011 immediately after the merger, some 80 K warmer than the quiescent surroundings. From July 2011 to the time of writing, B0 remained as a long-lived stable stratospheric phenomenon at 2 mbar, moving west with a near-constant velocity of 2.70 +/- 0.04 deg/day (24.5 +/- 0.4 m/s at 40degN relative to System III longitudes). No perturbations to visible clouds and hazes were detected during this period. With no direct tracers of motion in the stratosphere, we use thermal windshear calculations to estimate clockwise peripheral velocities of 200-400 m/s at 2 mbar around B0. The peripheral velocities of the two original airmasses were smaller (70-140 m/s). In August 2011, the size of the vortex as defined by the peripheral collar was 65deg longitude (50,000 km in diameter) and 25deg latitude. Stratospheric acetylene (C2H2) was uniformly enhanced by a factor of three within the vortex, whereas ethane (C2H6) remained unaffected. The passage of B0 generated a new band of warm stratospheric emission at 0.5 mbar at its northern edge, and there are hints of warm stratospheric structures associated with the beacons at higher altitudes (p < 0.1 mbar) than can be reliably observed by CIRS nadir spectroscopy. Analysis of the zonal windshear suggests that Rossby wave perturbations from the convective storm could have propagated vertically into the stratosphere at this point in Saturn's seasonal cycle, one possible source of energy for the formation of these stratospheric anticyclones.

evolution↗
NASA NTRS1981

OH emission in the direction of TV Gem and BI Cyg

The NRAO-Green Bank 43-m telescope and 18-cm receiver have detected OH maser main-line emission at 1665 MHz, in the direction of the two late-type supergiants TV Gem and BI Cyg. The detection of the two new OH maser sources is noteworthy in view of the small number of late-type supergiants known to be molecular radio sources, or associated in close proximity with OH emission clouds. The IR, UV and radio properties of the two stars are discussed.

Brown, L. W.↗
DOE OSTI2023

Optical/X-ray/radio view of Abell 1213: A galaxy cluster with anomalous diffuse radio emission

Context. Abell 1213, a low-richness galaxy system, is known to host an anomalous radio halo detected in data of the Very Large Array (VLA). It is an outlier with regard to the relation between the radio halo power and the X-ray luminosity of the parent clusters. Aims. Our aim is to analyze the cluster in the optical, X-ray, and radio bands to characterize the environment of its diffuse radio emission and to shed new light on its nature. Methods. We used optical data from the Sloan Digital Sky Survey to study the internal dynamics of the cluster. We also analyzed archival XMM-Newton X-ray data to unveil the properties of its hot intracluster medium. Finally, we used recent data from the LOw Frequency ARray (LOFAR) at 144 MHz, together with VLA data at 1.4 GHz, to study the spectral behavior of the diffuse radio source. Results. Both our optical and X-ray analysis reveal that this low-mass cluster exhibits disturbed dynamics. In fact, it is composed of several galaxy groups in the peripheral regions and, in particular, in the core, where we find evidence of substructures oriented in the NE–SW direction, with hints of a merger nearly along the line of sight. The analysis of the X-ray emission adds further evidence that the cluster is in an unrelaxed dynamical state. At radio wavelengths, the LOFAR data show that the diffuse emission is ~510 kpc in size. Moreover, there are hints of low-surface-brightness emission permeating the cluster center. Conclusions. The environment of the diffuse radio emission is not what we would expect for a classical halo. The spectral index map of the radio source is compatible with a relic interpretation, possibly due to a merger in the N–S or NE–SW directions, in agreement with the substructures detected through the optical analysis. The fragmented, diffuse radio emissions at the cluster center could be attributed to the surface brightness peaks of a faint central radio halo.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2020

Massive Stars in Molecular Clouds Rich in High-energy Sources: The Bridge of G332.809–0.132 and CS 78 in NGC 6334

Detections of massive stars in the direction of the H ii region CS 78 in NGC 6334 and of G332.809−0.132 are here presented. The region covered by the G332.809−0.132 complex coincides with the RCW 103 stellar association. In its core (40′ in radius), approximately 110 OB candidate stars (K {sub s} < 10 mag and 0.4 < A{sub K{sub s}} < 1.6 mag) were identified using 2MASS, DENIS, and GLIMPSE data. This number of OB stars accounts for more than 50% of the observed number of Lyman continuum photons from this region. Medium-resolution K-band spectra were obtained for seven early types, including one WN 8 star and one Ofpe/WN 9 star; the latter is located near the RCW 103 remnant and its luminosity is consistent with a distance of ≈3 kpc. The area analyzed encloses 9 of the 34 OB stars previously known in RCW 103, as well as IRAS 16115−5044, which we reclassify as a candidate luminous blue variable. The line of sight is particularly interesting, crossing three spiral arms; a molecular cloud at −50 (with RCW 103 in the Scutum-Crux arm) and another at −90 km s{sup −1} (in the Norma arm) are detected, both rich in massive stars and supernova remnants. We also report the detection of a B supergiant as the main ionizing source of CS 78, 2MASS J17213513−3532415. Medium-resolution H- and K-band spectra display H i and He i lines, as well as Fe ii lines. By assuming a distance of 1.35 kpc, we estimate a bolometric magnitude of −6.16, which is typical of supergiants.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2026

A First Demonstration of the SQUAT Detector Architecture: Direct Measurement of Resonator-Free Charge-Sensitive Transmons

The Superconducting Quasiparticle-Amplifying Transmon (SQUAT) is a new sensor architecture for THz (meV) detection based on a weakly charge-sensitive transmon directly coupled to a transmission line. In such devices, energy depositions break Cooper pairs in the qubit capacitor islands, generating quasiparticles. Quasiparticles that tunnel across the Josephson junction change the transmon qubit parity, generating a measurable signal. In this paper, we present the design of first-generation SQUATs and demonstrate an architecture validation. We summarize initial characterization measurements made with prototype devices, comment on background sources that influence the observed parity-switching rate, and present experimental results showing simultaneous detection of charge and quasiparticle signals using aluminum-based SQUATs.

Magoon, H. [SLAC; KIPAC, Menlo Park; Stanford U., ↗
DOE OSTI2022

Photon detection probability prediction using one-dimensional generative neural network

Abstract Photon detection is important for liquid argon detectors for direct dark matter searches or neutrino property measurements. Precise simulation of photon transport is widely used to understand the probability of photon detection in liquid argon detectors. Traditional photon transport simulation, which tracks every photon using the Geant4 simulation toolkit, is a major computational challenge for kilo-tonne-scale liquid argon detectors and GeV-level energy depositions. In this work, we propose a one-dimensional generative model which efficiently generates features using an O u t e r P r o d u c t -layer. This model bypasses photon transport simulation and predicts the number of photons detected by particular photon detectors at the same level of detail as the Geant4 simulation. The application to simulating photon detection systems in kilo-tonne-scale liquid argon detectors demonstrates this novel generative model is able to reproduce Geant4 simulation with good accuracy and 20 to 50 times faster. This generative model can be used to quickly predict photon detection probability in huge liquid argon detectors like ProtoDUNE or DUNE.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2026

A new water-based scintillator for efficient Cherenkov and scintillation separation

Neutrinos offer a unique window into the world around us, allowing us to probe otherwise unreachable regions like the interior of stars and the depths of the earth, as well as potentially offering a mechanism for monitoring nuclear activity. Both pure-water and organic liquid scintillators have been used as the detection medium of large-scale neutrino detectors. Organic liquid scintillators offer higher sensitivity at lower energies, which is desirable for many applications, but detection of the Cherenkov radiation required for directional sensitivity is very difficult. A possible solution is to use water-based liquid scintillators (WbLSs), where some fraction of the water is replaced with a micellar solution of the liquid scintillator. This can enhance the detection sensitivity beyond that of pure water, without significantly affecting the ability to leverage the topological Cherenkov signature. Very specific scintillation properties are required to achieve this goal: the scintillation decay time should be significantly slower than that of the Cherenkov emission, so timing-based discrimination of Cherenkov light from scintillation can be applied. At the same time, the light yield should be high enough to enhance the overall sensitivity of the detector, but without losing too much of the Cherenkov light. In this study, we report a new water-based liquid scintillation cocktail based on a 9-methylcarbazole fluorescent dye and a linear alkylbenzene solvent. Here, the proposed composition offers 13.8 ns scintillation decay time and 368 nm emission that matches the desired properties.

Wolszczak, Weronika W. [Lawrence Berkeley National↗