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At least 1,387 records · Page 77
All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

Time–connectivity superposition and the gel/glass duality of weak colloidal gels

Colloidal gels result from the aggregation of Brownian particles suspended in a solvent. Gelation is induced by attractive interactions between individual particles that drive the formation of clusters, which in turn aggregate to form a space-spanning structure. We study this process in aluminosilicate colloidal gels through time-resolved structural and mechanical spectroscopy. Using the time–connectivity superposition principle a series of rapidly acquired linear viscoelastic spectra, measured throughout the gelation process by applying an exponential chirp protocol, are rescaled onto a universal master curve that spans over eight orders of magnitude in reduced frequency. This analysis reveals that the underlying relaxation time spectrum of the colloidal gel is symmetric in time with power-law tails characterized by a single exponent that is set at the gel point. The microstructural mechanical network has a dual character; at short length scales and fast times it appears glassy, whereas at longer times and larger scales it is gel-like. These results can be captured by a simple three-parameter constitutive model and demonstrate that the microstructure of a mature colloidal gel bears the residual skeleton of the original sample-spanning network that is created at the gel point. Our conclusions are confirmed by applying the same technique to another well-known colloidal gel system composed of attractive silica nanoparticles. The results illustrate the power of the time–connectivity superposition principle for this class of soft glassy materials and provide a compact description for the dichotomous viscoelastic nature of weak colloidal gels.

36 MATERIALS SCIENCE↗
DOE OSTI2023

Time-refraction optics with single cycle modulation

Abstract We present an experimental study of optical time-refraction caused by time-interfaces as short as a single optical cycle. Specifically, we study the propagation of a probe pulse through a sample undergoing a large refractive index change induced by an intense modulator pulse. In these systems, increasing the refractive index abruptly leads to time-refraction where the spectrum of all the waves propagating in the medium is red-shifted, and subsequently blue-shifted when the refractive index relaxes back to its original value. We observe these phenomena in the single-cycle regime. Moreover, by shortening the temporal width of the modulator to ∼5–6 fs, we observe that the rise time of the red-shift associated with time-refraction is proportionally shorter. The experiments are carried out in transparent conducting oxides acting as epsilon-near-zero materials. These observations raise multiple questions on the fundamental physics occurring within such ultrashort time frames, and open the way for experimenting with photonic time-crystals, generated by periodic ultrafast changes to the refractive index, in the near future.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
NASA NTRS2016

Time-Dependent Stress Rupture Strength Degradation of Hi-Nicalon Fiber-Reinforced Silicon Carbide Composites at Intermediate Temperatures

The stress rupture strength of silicon carbide fiber-reinforced silicon carbide composites with a boron nitride fiber coating decreases with time within the intermediate temperature range of 700 to 950 degree Celsius. Various theories have been proposed to explain the cause of the time-dependent stress rupture strength. The objective of this paper is to investigate the relative significance of the various theories for the time-dependent strength of silicon carbide fiber-reinforced silicon carbide composites. This is achieved through the development of a numerically based progressive failure analysis routine and through the application of the routine to simulate the composite stress rupture tests. The progressive failure routine is a time-marching routine with an iterative loop between a probability of fiber survival equation and a force equilibrium equation within each time step. Failure of the composite is assumed to initiate near a matrix crack and the progression of fiber failures occurs by global load sharing. The probability of survival equation is derived from consideration of the strength of ceramic fibers with randomly occurring and slow growing flaws as well as the mechanical interaction between the fibers and matrix near a matrix crack. The force equilibrium equation follows from the global load sharing presumption. The results of progressive failure analyses of the composite tests suggest that the relationship between time and stress-rupture strength is attributed almost entirely to the slow flaw growth within the fibers. Although other mechanisms may be present, they appear to have only a minor influence on the observed time-dependent behavior.

Progressive Failure Analysis↗
NASA NTRS2023

Improving the MODIS LAI Compositing Using Prior Time-Series Information

The Moderate Resolution Imaging Spectroradiometer (MODIS) long-term leaf area index (LAI) products have significantly contributed to global energy fluxes, climate change, and biogeochemistry research. However, the maximum fraction of photosynthetically active radiation absorbed by vegetation (Max-FPAR) compositing strategy of the Collection 6 (C6) products dictates that the main or backup algorithm is always triggered by observations of different quality, which indirectly causes the observed instability in the LAI time-series. Based on MODIS daily LAI retrievals, this study develops a prior knowledge time-series compositing algorithm (PKA) using a linear kernel driven (LKD) model. Our results show that the newly proposed PKA can significantly improve the LAI composites compared to the Max-FPAR strategy using ground-based observations for validation. We found that the PKA performs better than Max-FPAR in various aspects (different sites, seasons, and retrieval index (RI) ranges), with R2 increasing from 0.69 to 0.76 and root means square error (RMSE) decreasing from 1.01 to 0.84 compared to GBOV ground truth. The same improvement was shown for the ground truth LAIs measured at the Honghe and Hailun sites in northeastern China, with R2 increasing from 0.23 to 0.41 and RMSE decreasing from 1.27 to 1.25. In addition, three newly proposed temporal uncertainty metrics (time-series stability, TSS and time-series anomaly, TSA and reconstruction error metric, RE (the proximity to the main RT-based retrievals)) were applied to compare the stability of LAI time-series before and after PKA implementation. We found that the time series stability of PKA LAI was improved, the time series anomalies were reduced, and the retrieval rates of the main algorithm were also greatly enhanced compared to Max-FPAR LAI. A case intercomparison for Max-FPAR-MODIS, Max-FPAR-VIIRS (Visible Infrared Imager Radiometer Suite), and PKA-MODIS LAIs in the Amazon Forest region showed that the PKA is also effective in improving the LAI retrieval over large regions with few qualified observations due to poor atmospheric conditions (RE decreased from 2.37/2.35 (Max-FPAR-MODIS/Max-FPAR-VIIRS) to 2.25 (PKA-MODIS) and RI increased from 61.94%/59.62% to 66.88%). The same improvement was seen in the BELMANIP 2.1 sites for almost all biomes except deciduous broadleaf forest, where the RE decreased from 1.85/2.13 to 1.15 overall. We note that the PKA has the potential to be easily implemented in the operational algorithms of subsequent MODIS and MODIS-like LAI Collections.

MODIS↗
DOE OSTI2014

From h to p efficiently: optimal implementation strategies for explicit time-dependent problems using the spectral/ hp element method: FROM h TO p EFFICIENTLY

We investigate the relative performance of a second-order Adams–Bashforth scheme and second-order and fourth-order Runge–Kutta schemes when time stepping a 2D linear advection problem discretised using a spectral/hp element technique for a range of different mesh sizes and polynomial orders. Numerical experiments explore the effects of short (two wavelengths) and long (32 wavelengths) time integration for sets of uniform and non-uniform meshes. The choice of time-integration scheme and discretisation together fixes a CFL limit that imposes a restriction on the maximum time step, which can be taken to ensure numerical stability. The number of steps, together with the order of the scheme, affects not only the runtime but also the accuracy of the solution. Through numerical experiments, we systematically highlight the relative effects of spatial resolution and choice of time integration on performance and provide general guidelines on how best to achieve the minimal execution time in order to obtain a prescribed solution accuracy. The significant role played by higher polynomial orders in reducing CPU time while preserving accuracy becomes more evident, especially for uniform meshes, compared with what has been typically considered when studying this type of problem.

42 ENGINEERING↗
DOE OSTI2020

Nonoverlapping Localized Exponential Time Differencing Methods for Diffusion Problems

In this paper, we propose nonoverlapping localized exponential time differencing (ETD) methods for diffusion problems. The model time-dependent diffusion equation is first reformulated on subdomains based on the nonoverlapping domain decomposition, in which Neumann boundary conditions are imposed on the interfaces for the subdomain problems and Dirichlet type conditions are enforced to form a space-time interface problem. After spatial discretization by standard central finite differences and temporal integration with the first or second order ETD methods, the fully discrete interface problem is obtained. Such an interface problem is then solved iteratively either at each time step or over the whole time interval: the former involves the solution of stationary problems in each subdomain at each iteration while the latter involves the solution of time-dependent subdomain problems at each iteration. For both approaches, we prove that localized ETD solutions conserve mass exactly and converge in time to the exact space semidiscrete solution. Numerical experiments in two dimensions are also presented to illustrate the performance of the proposed methods.

Mass conservation↗
DOE OSTI2018

On the Coupling Time of the Heat-Bath Process for the Fortuin–Kasteleyn Random–Cluster Model

We consider the coupling from the past implementation of the random–cluster heat-bath process, and study its random running time, or coupling time. We focus on hypercubic lattices embedded on tori, in dimensions one to three, with cluster fugacity at least one. We make a number of conjectures regarding the asymptotic behaviour of the coupling time, motivated by rigorous results in one dimension and Monte Carlo simulations in dimensions two and three. Amongst our findings, we observe that, for generic parameter values, the distribution of the appropriately standardized coupling time converges to a Gumbel distribution, and that the standard deviation of the coupling time is asymptotic to an explicit universal constant multiple of the relaxation time. Perhaps surprisingly, we observe these results to hold both off criticality, where the coupling time closely mimics the coupon collector’s problem, and also at the critical point, provided the cluster fugacity is below the value at which the transition becomes discontinuous. Finally, we consider analogous questions for the single-spin Ising heat-bath process.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2014

Second quantized scalar QED in homogeneous time-dependent electromagnetic fields

We formulate the second quantization of a charged scalar field in homogeneous, time-dependent electromagnetic fields, in which the Hamiltonian is an infinite system of decoupled, time-dependent oscillators for electric fields, but it is another infinite system of coupled, time-dependent oscillators for magnetic fields. We then employ the quantum invariant method to find various quantum states for the charged field. For time-dependent electric fields, a pair of quantum invariant operators for each oscillator with the given momentum plays the role of the time-dependent annihilation and the creation operators, constructs the exact quantum states, and gives the vacuum persistence amplitude as well as the pair-production rate. We also find the quantum invariants for the coupled oscillators for the charged field in time-dependent magnetic fields and advance a perturbation method when the magnetic fields change adiabatically. Finally, the quantum state and the pair production are discussed when a time-dependent electric field is present in parallel to the magnetic field.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2017

Statistical approach to tunneling time in attosecond experiments

Tunneling, transport of particles through classically forbidden regions, is a pure quantum phenomenon. It governs numerous phenomena ranging from single-molecule electronics to donor–acceptor transition reactions. The main problem is the absence of a universal method to compute tunneling time. This problem has been attacked in various ways in the literature. Here, in the present work, we show that a statistical approach to the problem, motivated by the imaginary nature of time in the forbidden regions, lead to a novel tunneling time formula which is real and subluminal (in contrast to various known time definitions implying superluminal tunneling). In addition to this, we show explicitly that the entropic time formula is in good agreement with the tunneling time measurements in laser-driven He ionization. Moreover, it sets an accurate range for long-range electron transfer reactions. The entropic time formula is general enough to extend to the photon and phonon tunneling phenomena.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2019

Split-pane electrochromic window control based on an embedded photometric device with real-time daylighting computing

Well-designed electrochromic (EC) glazing control can improve the energy performance of buildings and visual comfort of occupants in highly glazed buildings. Here in this paper, we designed and demonstrated a compact integrated EC glazing automation system to control tint states of a split-pane EC window according to variations of sky conditions. The control is based on monitoring the luminance distribution of the sky and real-time lighting computation for a building interior, using an embedded photometric device (EPD). It optimizes tint states of EC glazing to offer sufficient daylight provision and temper discomfort glare for occupants, which potentially mitigates excessive solar heat gain. ’In-situ’ experiments were conducted in a full-scale testbed to demonstrate the daylighting performance under various sky conditions. Finally, experimental results showed 83% of the working time for work-plane illuminance (WPI) and 95% of the time for daylight glare probability (DGP) were constrained in comfort range (WPIϵ[500, 2000] lux, DGP ≤ 0.35) by the automated EC glazing (controlled by EPD) under clear skies; 68% of the time for WPI and 94% of the time for DGP in confined range under clear skies with thin clouds; 62% of the time for WPI and 85% of the time for DGP in confined range under partly cloudy skies.

32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATI↗
DOE OSTI2019

In situ observations of reacting Al/Fe 2 O 3 thermite: Relating dynamic particle size to macroscopic burn time

Time-resolved x-ray imaging is used to capture high-resolution images of the Al/Fe 2 O 3 thermite reaction as it proceeds in an extended burn tube. The observed thermite reaction products are generally large, multi-phase composite particles. Image processing algorithms are developed to extract a continuous record of composite particle size as a function of time and distance from the ignition point. Small particles are observed immediately after ignition, followed by a rapid increase in particle size and a gradual decline toward late times. Correlating the dynamic particle size with visible light emission from the reaction, we propose a two-stage mechanism where the combination of early ignition and delayed expansion causes the material closest to the ignition point to undergo substantial coalescence before it begins moving down the tube. We also identify two mechanisms that may contribute to particle size refinement at late times, both based on the collapse of large gas bubbles that are observed preferentially in particles at earlier times. A new approach to extracting burn times from luminous intensity data is explored, and we find that a more nuanced analysis of burn time and luminous intensity may help to improve reactivity assessments when data from in situ studies is unavailable.

36 MATERIALS SCIENCE↗
DOE OSTI2014

Parareal in time 3D numerical solver for the LWR Benchmark neutron diffusion transient model

In this paper we present a time-parallel algorithm for the 3D neutrons calculation of a transient model in a nuclear reactor core. The neutrons calculation consists in numerically solving the time dependent diffusion approximation equation, which is a simplified transport equation. The numerical resolution is done with finite elements method based on a tetrahedral meshing of the computational domain, representing the reactor core, and time discretization is achieved using a θ-scheme. The transient model presents moving control rods during the time of the reaction. Therefore, cross-sections (piecewise constants) are taken into account by interpolations with respect to the velocity of the control rods. The parallelism across the time is achieved by an adequate use of the parareal in time algorithm to the handled problem. This parallel method is a predictor corrector scheme that iteratively combines the use of two kinds of numerical propagators, one coarse and one fine. Our method is made efficient by means of a coarse solver defined with large time step and fixed position control rods model, while the fine propagator is assumed to be a high order numerical approximation of the full model. The parallel implementation of our method provides a good scalability of the algorithm. Numerical results show the efficiency of the parareal method on large light water reactor transient model corresponding to the Langenbuch–Maurer–Werner benchmark.

97 MATHEMATICS AND COMPUTING↗
DOE OSTI2017

A dynamical polynomial chaos approach for long-time evolution of SPDEs

We propose a Dynamical generalized Polynomial Chaos (DgPC) method to solve time-dependent stochastic partial differential equations (SPDEs) with white noise forcing. The long-time simulation of SPDE solutions by Polynomial Chaos (PC) methods is notoriously difficult as the dimension of the stochastic variables increases linearly with time. Exploiting the Markovian property of white noise, DgPC implements a restart procedure that allows us to expand solutions at future times in terms of orthogonal polynomials of the measure describing the solution at a given time and the future white noise. The dimension of the representation is kept minimal by application of a Karhunen–Loeve (KL) expansion. Using frequent restarts and low degree polynomials on sparse multi-index sets, the method allows us to perform long time simulations, including the calculation of invariant measures for systems which possess one. We apply the method to the numerical simulation of stochastic Burgers and Navier–Stokes equations with white noise forcing. Our method also allows us to incorporate time-independent random coefficients such as a random viscosity. We propose several numerical simulations and show that the algorithm compares favorably with standard Monte Carlo methods.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2020

Space–time reduced order model for large-scale linear dynamical systems with application to Boltzmann transport problems

A classical reduced order model for dynamical problems involves spatial reduction of the problem size. However, temporal reduction accompanied by the spatial reduction can further reduce the problem size without losing much accuracy, which results in a considerably more speed-up than the spatial reduction only. Recently, a novel space–time reduced order model for dynamical problems has been developed [17], where the space–time reduced order model shows an order of a hundred speed-up with a relative error of 10 –4 for small academic problems. However, in order for the method to be applicable to a large-scale problem, an efficient space–time reduced basis construction algorithm needs to be developed. Here we present the incremental space–time reduced basis construction algorithm. The incremental algorithm is fully parallel and scalable. Additionally, the block structure in the space–time reduced basis is exploited, which enables the avoidance of constructing the reduced space–time basis. These novel techniques are applied to a large-scale particle transport simulation with million and billion degrees of freedom. The numerical example shows that the algorithm is scalable and practical. Also, it achieves a tremendous speed-up, maintaining a good accuracy. Finally, error bounds for space-only and space–time reduced order models are derived.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2014

Precision timing measurements for high energy photons

Particle colliders operating at high luminosities present challenging environments for high energy physics event reconstruction and analysis. We discuss how timing information, with a precision on the order of 10 ps, can aid in the reconstruction of physics events under such conditions. We present calorimeter based timing measurements from test beam experiments in which we explore the ultimate timing precision achievable for high energy photons or electrons of 10 GeV and above. Using a prototype calorimeter consisting of a 1.7×1.7×1.7 cm 3 lutetium–yttrium oxyortho-silicate (LYSO) crystal cube, read out by micro-channel plate photomultipliers, we demonstrate a time resolution of 33.5±2.1 ps for an incoming beam energy of 32 GeV. In a second measurement, using a 2.5×2.5×20 cm 3 LYSO crystal placed perpendicularly to the electron beam, we achieve a time resolution of 59±11 ps using a beam energy of 4 GeV. We also present timing measurements made using a shashlik-style calorimeter cell made of LYSO and tungsten plates, and demonstrate that the apparatus achieves a time resolution of 54±5 ps for an incoming beam energy of 32 GeV.

43 PARTICLE ACCELERATORS↗
DOE OSTI2016

Detection of high energy muons with sub-20 ps timing resolution using L(Y)SO crystals and SiPM readout

Precise timing capability will be a key aspect of particle detectors at future high energy colliders, as the time information can help in the reconstruction of physics events at the high collision rate expected there. Other than being used in detectors for PET, fast scintillating crystals coupled to compact Silicon Photomultipliers (SiPMs) constitute a versatile system that can be exploited to realize an ad-hoc timing device to be hosted in a larger high energy physics detector. In this paper, we present the timing performance of LYSO:Ce and LSO:Ce codoped 0.4% Ca crystals coupled to SiPMs, as measured with 150 GeV muons at the CERN SPS H2 extraction line. Small crystals, with lengths ranging from 5 mm up to 30 mm and transverse size of 2×2mm 2 or 3×3mm 2 , were exposed to a 150 GeV muon beam. SiPMs from two different companies (Hamamatsu and FBK) were used to detect the light produced in the crystals. The best coincidence time resolution value of (14.5±0.5)ps , corresponding to a single-detector time resolution of about 10 ps, is demonstrated for 5 mm long LSO:Ce,Ca crystals coupled to FBK SiPMs, when time walk corrections are applied.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2022

Sub-25 ps timing measurements with 10 × 10 cm 2 PICOSEC Micromegas detectors

The PICOSEC Micromegas detector is a precise timing gaseous detector based on a Cherenkov radiator coupled to a semi-transparent photocathode and a Micromegas amplifying structure. First single-pad prototypes demonstrated a time resolution below σ = 25 ps, however, to make the concept appropriate to physics applications, several developments are required. The objective of this work was to achieve an equivalent time resolution for a 10 × 10 cm 2 area PICOSEC Micromegas detector. The prototype was designed, produced and tested in the laboratory and successfully operated with a 80 GeV/c muon beam. Preliminary results for this device equipped with a CsI photocathode demonstrated a time resolution below σ = 25 ps for all measured pads. The time resolution was reduced to be below σ = 18 ps by decreasing the drift gap to 180 μm and using dedicated RF amplifier cards as new electronics. The excellent timing performance of the single-channel proof of concept was not only transferred to the 100-channel prototype, but even improved, making the PICOSEC Micromegas detector more suitable for large-area experiments in need of detectors with high time resolutions.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2023

Characterization of LAPPD timing at CERN PS testbeam

Large Area Picosecond PhotoDetectors (LAPPDs) are photosensors based on microchannel plate technology with about 400 cm 2 sensitive area. The external readout plane of a capacitively coupled LAPPD can be segmented into pads providing a spatial resolution down to 1 mm scale. The LAPPD signals have about 0.5 ns rise time followed by a slightly longer fall time and their amplitude reaches a few dozens of mV per single photoelectron. In this article, we report on the measurement of the time resolution of an LAPPD prototype in a test beam exercise at CERN PS. Most of the previous measurements of LAPPD time resolution had been performed with laser sources. In this article we report time resolution measurements obtained through the detection of Cherenkov radiation emitted by high energy hadrons. Our approach has been demonstrated capable of measuring time resolutions as fine as 25-30 ps. The available prototype had performance limitations, which prevented us from applying the optimal high voltage setting. Finally, the measured time resolution for single photoelectrons is about 80 ps r.m.s.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗