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All sourcesNASA NTRSDOE OSTI
NASA NTRS2012

The Response of Lower Atmospheric Ozone to ENSO in Aura Measurements and a Chemistry-Climate Simulation

The El Nino-Southern Oscillation (ENSO) is the dominant mode of tropical variability on interannual time scales. ENSO appears to extend its influence into the chemical composition of the tropical troposphere. Recent work has revealed an ENSO-induced wave-1 anomaly in observed tropical tropospheric column ozone. This results in a dipole over the western and eastern tropical Pacific, whereby differencing the two regions produces an ozone anomaly with an extremely high correlation to the Nino 3.4 Index. We have successfully reproduced this feature using the Goddard Earth Observing System Version 5 (GEOS-5) general circulation model coupled to a comprehensive stratospheric and tropospheric chemical mechanism forced with observed sea surface temperatures over the past 25 years. An examination of the modeled ozone field reveals the vertical contributions of tropospheric ozone to the column over the western and eastern Pacific region. We will show composition sensitivity in observations from NASA s Aura satellite Microwave Limb Sounder (MLS) and the Tropospheric Emissions Spectrometer (TES) and a simulation to provide insight into the vertical structure of these ENSO-induced ozone changes. The ozone changes due to the Quasi-Biennial Oscillation (QBO) in the extra-polar upper troposphere and lower stratosphere in MLS measurements will also be discussed.

Oman, L. D.↗
NASA NTRS2014

The Impact of the Atlantic Cold Tongue on West African Monsoon Onset in Regional Model Simulations for 1998-2002

The Atlantic cold tongue (ACT) develops during spring and early summer near the Equator in the Eastern Atlantic Ocean and Gulf of Guinea. The hypothesis that the ACT accelerates the timing of West African monsoon (WAM) onset is tested by comparing two regional climate model (RM3) simulation ensembles. Observed sea surface temperatures (SST) that include the ACT are used to force a control ensemble. An idealized, warm SST perturbation is designed to represent lower boundary forcing without the ACT for the experiment ensemble. Summer simulations forced by observed SST and reanalysis boundary conditions for each of five consecutive years are compared to five parallel runs forced by SST with the warm perturbation. The article summarizes the sequence of events leading to the onset of the WAM in the Sahel region. The representation of WAM onset in RM3 simulations is examined and compared to Tropical Rainfall Measuring Mission (TRMM), Global Precipitation Climatology Project (GPCP) and reanalysis data. The study evaluates the sensitivity of WAM onset indicators to the presence of the ACT by analysing the differences between the two simulation ensembles. Results show that the timing of major rainfall events and therefore theWAM onset in the Sahel are not sensitive to the presence of the ACT. However, the warm SST perturbation does increase downstream rainfall rates over West Africa as a consequence of enhanced specific humidity and enhanced northward moisture flux in the lower troposphere.

Regional model simulation↗
NASA NTRS2012

Jet-Surface Interaction Test: Phased Array Noise Source Localization Results

Subsonic jets are relatively simple. The peak noise source location gradually moves upstream toward the nozzle as frequency increases. 2) Supersonic jets are more complicated. The peak noise source location moves downstream as frequency increases through a BBSN hump. 3) In both subsonic and supersonic jets the peak noise source location corresponding to a given frequency of noise moves downstream as jet Mach number increases. 4) The noise generated at a given frequency in a BBSN hump is generated by a small number of shocks, not from all the shocks at the same time. 5) Single microphone spectrum levels decrease when the noise source locations measured with the phased array are blocked by a shielding surface. This consistency validates the phased array data and the stationary monopole source model used to process it. 6) Reflecting surface data illustrate that the law of reflection must be satisfied for noise to reflect off a surface toward an observer. Depending on the relative locations of the jet, the surface and the observer only some of the jet noise sources may satisfy this requirement. 7) The low frequency noise created when a jet flow impinges on a surface comes primarily from the trailing edge regardless of the axial extent impacted by the flow.

Podboy, Gary↗
NASA NTRS1973

Analyses of the gamma-ray pulse-height spectra from the lunar surface

The method of inferring photon spectra from an analysis of the measured pulse-height spectrum is considered along with the spectrum shape and its variation energy. The case is examined where photoelastic absorption predominates, and Compton scattering and pair production are negligible. The analytic method for obtaining the elemental composition from the observed lunar surface spectrum is described, and theoretical and calculated weight fraction fluxes for average lunar composition are tabulated.

Trombka, J. I.↗
DOE OSTI2025

Stability of Mn-Doped TiO 2 Thin-Film Anodes during Water Oxidation Reactions

Incorporating manganese atoms into TiO 2 has been shown to improve its activity for water oxidation. However, its activity has been observed to steadily degrade under constant applied potential, especially at more oxidizing applied potentials. Here, the compositional profile and electrochemical stability of Mn-doped TiO 2 (Mn:TiO 2 ) thin-film electrodes precisely fabricated by atomic layer deposition (ALD) were evaluated to elucidate the mechanisms of electrode degradation. Although ALD enables the deposition of Mn dopants throughout the film thickness, only Mn within 1.5 nm of the surface was observed to be redox active. Annealing Mn:TiO 2 films in air leads to the diffusion of Mn toward the electrode surface and oxidation of the Mn and alters the redox behavior. Annealing endows greater stability to Mn redox behavior but does not fully stabilize the water oxidation current, suggesting that the two electrochemical processes are not precisely correlated. In situ inductively coupled plasma mass spectrometry reveals that Mn is lost from Mn:TiO 2 films at potentials greater than 1.8 V vs RHE. However, the initial Mn loss is equivalent to less than a single ALD layer of MnO x . Longer-term constant potential experiments suggest that Mn is lost from up to 1 nm of the electrode surface but that this loss may account for only a portion of the diminished water oxidation activity.

atomic layer deposition↗
DOE OSTI2025

Phase-field modeling of diffusion bonding in 316H stainless steel: Impact of processing conditions on grain morphology and bonding quality

A novel multi-phase, multi-component phase‐field model is presented to study the diffusion bonding of 316H stainless steel. Combined with targeted experimental investigations, this model simulates the bond-growth process and predicts the bonding quality. Unlike previous models, our approach captures the simultaneous evolution of voids and grain structures, while quantifying bonding quality using defined bonding ratio. A comprehensive analysis of bond process control is performed by changing temperature, pressure and surface roughness observing the resulting bond structure, which is consistent with experimental observations and analytical predictions. Temperature is determined to be the dominant factor, with the transition from a flat to a robust bond occurring between 1000 °C and 1050 °C. At the ideal bonding temperature of 1050 °C, a surface roughness exceeding 0.6 μm or an applied stress below 4 MPa results in poor bonding quality. Beyond this, higher pressures and smoother surfaces reduce void size, accelerate void shrinkage, and lead to improved bond integrity. This diffuse-interface model can be extended to other material systems if supplied with appropriate thermodynamic and kinetic data. In conclusion, this makes it an effective modeling platform for optimizing high-temperature diffusion bonding and developing reliable bonded components such as compact heat exchangers.

Diffusion bonding↗
DOE OSTI2021

Land Surface Temperature from GOES-East and GOES-West

Land surface temperature (LST) is an important climate parameter that controls the surface energy budget. For climate applications, information is needed at the global scale with representation of the diurnal cycle. To achieve global coverage there is a need to merge about five independent geostationary (GEO) satellites that have different observing capabilities. An issue of practical importance is the merging of independent satellite observations in areas of overlap. An optimal approach in such areas could eliminate the need for redundant computations by differently viewing satellites. We use a previously developed approach to derive information on LST from GOES-East (GOES-E), modify it for application to GOES-West (GOES-W) and implement it simultaneously across areas of overlap at 5-km spatial resolution. We evaluate the GOES-based LST against in situ observations and an independent MODIS product for the period of 2004–09. The methodology proposed minimizes differences between satellites in areas of overlap. The mean and median values of the differences in monthly mean LST retrieved from GOES-E and GOES-W at 0600 UTC for July are 0.01 and 0.11 K, respectively. Similarly, at 1800 UTC the respective mean and median value of the differences were 0.15 and 1.33 K. These findings can provide guidelines for potential users to decide whether the reported accuracy based on one satellite alone, meets their needs in area of overlap. Since the 6 yr record of LST was produced at hourly time scale, the data are well suited to address scientific issues that require the representation of LST diurnal cycle or the diurnal temperature range (DTR).

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2017

First Detection of Prominence Material Embedded within a 2 × 10{sup 6} K CME Front Streaming away at 100–1500 km s{sup −1} in the Solar Corona

Coronal mass ejections (CMEs) are the largest and most dynamic explosions detected in the million degree solar corona, with speeds reaching up to 3000 km s{sup −1} at Earth’s orbit. Triggered by the eruption of prominences, in most cases, one of the outstanding questions pertaining to the dynamic CME-prominence system is the fate of the cool 10{sup 4}--10{sup 5} K ejected filaments. We present spectroscopic observations acquired during the 2015 March 20 total solar eclipse, which captured a plethora of redshifted plasmoids from Fe xiv emission at 2×10{sup 6} K. Approximately 10% of these plasmoids enshrouded the same neutral and singly ionized plasma below 2×10{sup 5} K, observed in prominences anchored at the Sun at that time. This discovery was enabled by the novel design of a dual-channel spectrometer and the exceptionally clear sky conditions on the island of Svalbard during totality. The Doppler redshifts corresponded to speeds ranging from under 100 to over 1500 km s{sup −1}. These are the first comprehensive spectroscopic observations to unambiguously detect a 2×10{sup 6} K filamentary CME front with inclusions of cool prominence material. The CME front covered a projected area of 2.5×1.5 R{sub s}{sup 2} starting from the solar surface. These observations imply that cool prominence inclusions within a CME front maintain their ionic composition during expansion away from the Sun.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS1981

Determination of surface stress by Seasat-SASS - A case study with JASIN data

The values of sea surface stress determined with the dissipation method and those determined with a surface-layer model from observations on F.S. Meteor during the Joint Air-Sea Interaction (JASIN) Experiment are compared with the backscatter coefficients measured by the scatterometer SASS on the satellite Seasat. This study demonstrates that SASS can be used to determine surface stress directly as well as wind speed. The quality of the surface observations used in the calibration of the retrieval algorithms, however, is important. This sample of measurements disagrees with the predictions by the existing wind retrieval algorithm under non-neutral conditions and the discrepancies depend on atmospheric stability.

Liu, W. T.↗
NASA NTRS1990

Bioclimatic distribution of vegetation for general circulation model studies

Four global bioclimatic schemes which qualify climates on the basis of the distribution of vegetation, including the Holdridge (1947), Thornthwaite (1948), Koeppen (1936), and Troll and Paffen (1964) schemes, were applied to two global climate data sets to produce maps of global vegetation distribution: the Rand set described by Schutz and Gates (1971, 1973, and 1974) and the Shea (1986) data set. The results show that only 38 to 40 percent of the observed land surface, mapped as 31 vegetation types, could be replicated by applying the four schemes to these data sets. The simulations were significantly improved by further subdividing and regrouping the climates defined by the schemes and by regrouping the observed vegetation types. With these alterations, 77 percent of the predicted vegetative landscape coresponded with the observed distribution of vegetation.

Prentice, Katharine Culbertson↗
DOE OSTI2014

Gas source molecular beam epitaxy of scandium nitride on silicon carbide and gallium nitride surfaces

Scandium nitride (ScN) is a group IIIB transition metal nitride semiconductor with numerous potential applications in electronic and optoelectronic devices due to close lattice matching with gallium nitride (GaN). However, prior investigations of ScN have focused primarily on heteroepitaxial growth on substrates with a high lattice mismatch of 7%–20%. In this study, the authors have investigated ammonia (NH{sub 3}) gas source molecular beam epitaxy (NH{sub 3}-GSMBE) of ScN on more closely lattice matched silicon carbide (SiC) and GaN surfaces (<3% mismatch). Based on a thermodynamic analysis of the ScN phase stability window, NH{sub 3}-GSMBE conditions of 10{sup −5}–10{sup −4} Torr NH{sub 3} and 800–1050 °C where selected for initial investigation. In-situ x-ray photoelectron spectroscopy (XPS) and ex-situ Rutherford backscattering measurements showed all ScN films grown using these conditions were stoichiometric. For ScN growth on 3C-SiC (111)-(√3 × √3)R30° carbon rich surfaces, the observed attenuation of the XPS Si 2p and C 1s substrate core levels with increasing ScN thickness indicated growth initiated in a layer-by-layer fashion. This was consistent with scanning electron microscopy (SEM) images of 100–200 nm thick films that revealed featureless surfaces. In contrast, ScN films grown on 3C-SiC (111)-(3 × 3) and 3C-SiC (100)-(3 × 2) silicon rich surfaces were found to exhibit extremely rough surfaces in SEM. ScN films grown on both 3C-SiC (111)-(√3 × √3)R30° and 2H-GaN (0001)-(1 × 1) epilayer surfaces exhibited hexagonal (1 × 1) low energy electron diffraction patterns indicative of (111) oriented ScN. X-ray diffraction ω-2θ rocking curve scans for these same films showed a large full width half maximum of 0.29° (1047 arc sec) consistent with transmission electron microscopy images that revealed the films to be poly-crystalline with columnar grains oriented at ≈15° to the [0001] direction of the 6H-SiC (0001) substrate. In-situ reflection electron energy loss spectroscopy measurements determined the band-gap for the NH{sub 3}-GSMBE ScN films to be 1.5 ± 0.3 eV, and thermal probe measurements indicated all ScN films to be n-type. The four point probe sheet resistance of the ScN films was observed to increase with decreasing growth temperature and decreased with unintentional oxygen incorporation. Hg probe capacitance–voltage measurements indicated N{sub D}-N{sub A} decreased with decreasing growth temperature from 10{sup 19} to 10{sup 20}/cm{sup 3} for the lowest resistivity films to ≅5 × 10{sup 16}/cm{sup 3} for the highest resistivity films. In-situ ultraviolet photoelectron spectroscopy measurements additionally showed the valence band maximum moving from 1.4 to 0.8 eV below the Fermi level with decreasing growth temperature consistent with the increased resistivity and reduction in carrier concentration. These results suggest that additional reductions in ScN carrier concentrations can be achieved via continued optimization of ScN growth conditions and selection of substrate orientation and surface termination.

36 MATERIALS SCIENCE↗
NASA NTRS2021

Variabilities in Pm2.5 and Black Carbon Surface Concentrations Reproduced by Aerosol Optical Properties Estimated by In-Situ Data, Ground Based Remote Sensing and Modeling

Because of the increased temporal and spatial resolutions of the sensors onboard recently launched satellites, satellite-based surface aerosol concentration, which is usually estimated from the aerosol optical depth (AOD), is expected to become a strategic tool for air quality studies in the future. By further exploring the relationships of aerosol concentrations and their optical properties using ground observations, the accuracies of these products can be improved. Here, we analyzed collocated observations of surface mass concentrations of fine particulate matter (PM2.5) and black carbon (BC), as well as columnar aerosol optical properties from a sky radiometer and aerosol extinction profiles obtained by multi-axis differential optical absorption spectroscopy (MAX-DOAS), during the 2019–2020 period. We focused the analyses on a daily scale, emphasizing the role of the ultraviolet (UV) spectral region. Generally, the correlation between the AOD of the fine fraction (i.e., fAOD) and the PM2.5 surface concentration was moderately strong, regardless of considerations of boundary layer humidity and altitude. In contrast, the fAOD of the partial column below 1 km, which was obtained by combining sky radiometer and MAX-DOAS retrievals, better reproduced the variability of the PM2.5 and resulted in a linear relationship. In the same manner, we demonstrated that the absorption AOD of the fine fraction (fAAOD) of the partial column was related to the variability of the BC concentration. Analogous analyses based on aerosol products from the Modern-Era Retrospective analysis for Research and Applications, Version 2 (MERRA-2) confirmed these findings and highlighted the importance of the shape of the aerosol profile. Overall, our results indicated a remarkable consistency among the retrieved datasets, and between the datasets and MERRA-2 products. These results confirmed the well-known sensitivity to aerosol absorption in the UV spectral region; they also highlighted the efficacy of combined MAX-DOAS and sky radiometer observations.

Alessandro Damiani↗
DOE OSTI2020

Poly(N-isopropylacrylamide)-grafted gold nanoparticles at the vapor/water interface

Hypothesis: Grafting nanoparticles surfaces with water-soluble polymers modify interparticle interactions that are pivotal for assembling them into ordered phases. By manipulating salt concentrations of gold nanoparticles (AuNPs) that are grafted with poly(N-isopropylacrylamide) (PNIPAM-AuNPs), we hypothesize that various aggregated phases form at the suspension/vapor interface or in the bulk that depend on the molecular weight (MW) of PNIPAM and on salt concentrations. Experiments: AuNPs are grafted with thiolated PNIPAM of molecular weights of 3 or 6 kDa, and grafting is confirmed by dynamic light scattering. Liquid-surfaces X-ray reflectivity and grazing incidence small-angle X-ray scattering are used to determine the density profiles of the suspension/vapor interface and their inplane structure as salt is added to the suspensions. Findings: We observe that surface enrichment is induced by adding NaCl to the suspensions, and that at low salt concentrations, the monoparticle layer formed is dispersed, and above a threshold salt concentration, depending on MW of PNIPAM, the PNIPAM-AuNPs order in a hexagonal structure. We show that the lattice constant of the two-dimensional hexagonal structure varies with salt concentration, and more significantly with MW of PNIPAM.

36 MATERIALS SCIENCE↗
DOE OSTI2024

Parallax-corrected VISST-derived pixel-level products from satellite GOES-16

The NASA Langley group led by William Smith produced GOES-16 satellite cloud retrievals over an approximate 10 by 10 degree region over the CACTI field campaign location. These retrievals are described here: https://www.arm.gov/capabilities/vaps/visst and are available for download here . They use algorithms historically called VISST that are now referred to as SatCORPS. More information can be found in Trepte et al. (2019), Minnis et al. (2021), and Yost et al. (2021). If using this dataset, please cite these references, the CACTI VISST dataset DOI found at the download link above, and this dataset’s DOI. The CACTI VISST pixel-level retrievals are on a 2 km spatial grid and available every 15 minutes (every 10 minutes late in the campaign), producing 21,765 files for the entire field campaign between October 2018 and April 2019. They are not corrected for parallax error, which is an offset in the actual geographical location of a cloud above the surface due to the satellite viewing the cloud partly from the side off nadir. This dataset applies a correction for parallax using the location relative to the satellite and the retrieved cloud top height above the surface, which allows the dataset to be geo-located with surface-based observations. The parallax correction for each location depends on the longitude, latitude and cloud top height above ground level (AGL) for that longitude and latitude in the original VISST files. The cloud top height AGL requires first computing the surface elevation at each VISST grid point. Data from the Advanced Spaceborne Thermal Emission and Reflection (ASTER) Global Digital Elevation Map Version 3 at 30-m resolution is projected onto the VISST grid using conservative coarsening (conserving surface elevation) in the xESMF Python package. The surface elevation is then subtracted from the VISST-retrieved cloud top height above mean sea level. These cloud top heights AGL are then combined with longitude and latitude to estimate the latitude and longitude corrections. Due to variability in cloud top height, the parallax shifts produce an irregular grid of values since higher cloud tops are shifted further than lower cloud tops. A ball tree-based neighbor search with Haversine distance is performed using the Python-based scikit-learn library to find the nearest VISST grid point to each parallax correction-shifted point. The data value of the shifted point is then assigned to that VISST grid point. In this manner, the irregular geographical shifts to correct for parallax are projected back to the rectilinear VISST grid. Because relatively higher clouds should obscure lower clouds, the variable values for the highest cloud top are preferentially chosen if two or more values are assigned to a grid point. The parallax correction should be viewed as an improved but still imperfect estimation of the cloud top locations, largely because the cloud top height is an imperfect retrieval. Please see the attached README document for further information. Users are encouraged to contact the authors with any additional questions.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS1938

Flow Observations with Tufts and Lampblack of the Stalling of Four Typical Airfoil Sections in the NACA Variable-density Tunnel

A preliminary investigation of the stalling processes of four typical airfoil sections was made over the critical range of the Reynolds Number. Motion pictures were taken of the movements of small silk tufts on the airfoil surface as the angle of attack increased through a range of angles including the stall. The boundary-layer flow also at certain angles of attack was indicated by the patterns formed by a suspension of lampblack in oil brushed onto the airfoil surface. These observations were analyzed together with corresponding force-test measurements to derive a picture of the stalling processes of airfoils.

Abbott, Ira H↗
NASA NTRS1974

Goddard earth models (5 and 6)

A comprehensive earth model has been developed that consists of two complementary gravitational fields and center-of-mass locations for 134 tracking stations on the earth's surface. One gravitational field is derived solely from satellite tracking data. This data on 27 satellite orbits is the most extensive used for such a solution. A second solution uses this data with 13,400 simultaneous events from satellite camera observations and surface gravimetric anomalies. The satellite-only solution as a whole is accurate to about 4.5 milligals as judged by the surface gravity data. The majority of the station coordinates are accurate to better than 10 meters as judged by independent results from geodetic surveys and by Doppler tracking of both distant space probes and near earth orbits.

Lerch, F. J.↗
NASA NTRS1990

Triton's streaks as windblown dust

Explanations for the surface streaks observed by Voyager 2 on Triton's southern hemisphere are discussed. It is shown that, despite Triton's tenuous atmosphere, low-cohesion dust trains with diameters of about 5 micron or less may be carried into suspension by aeolian surface shear stress, given expected geostrophic wind speeds of about 10 m/s. For geyser-like erupting dust plumes, it is shown that dust-settling time scales and expected wind velocities can produce streaks with length scales in good agreement with those of the streaks. Thus, both geyserlike eruptions or direct lifting by surface winds appear to be viable mechanisms for the origin of the streaks.

Sagan, Carl↗
NASA NTRS2005

Processing ISS Images of Titan's Surface

One of the primary goals of the Cassini-Huygens mission, in orbit around Saturn since July 2004, is to understand the surface and atmosphere of Titan. Surface investigations are primarily accomplished with RADAR, the Visual and Infrared Mapping Spectrometer (VIMS), and the Imaging Science Subsystem (ISS) [1]. The latter two use methane "windows", regions in Titan's reflectance spectrum where its atmosphere is most transparent, to observe the surface. For VIMS, this produces clear views of the surface near 2 and 5 microns [2]. ISS uses a narrow continuum band filter (CB3) at 938 nanometers. While these methane windows provide our best views of the surface, the images produced are not as crisp as ISS images of satellites like Dione and Iapetus [3] due to the atmosphere. Given a reasonable estimate of contrast (approx.30%), the apparent resolution of features is approximately 5 pixels due to the effects of the atmosphere and the Modulation Transfer Function of the camera [1,4]. The atmospheric haze also reduces contrast, especially with increasing emission angles [5].

Perry, Jason↗