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All sources NASA NTRS DOE OSTI

DOE OSTI2023

Intensified Catalytic Conversion of CO2 into High Value Chemicals

The utilization of CO2 produced from power generation plants as a feedstock for creating new valuable products offers a strategy to reduce GHG emissions, offset carbon capture costs, and facilitate the rebalancing of the carbon cycle. After considering the thermodynamic requirement of potential products from CO2 utilization and their market size, formic acid is a desirable target that offers widespread utility in industrial chemical production and chemical energy storage as a liquid fuel. To effectively utilize CO2 from power generation plants, UK proposes an enhanced bimetallic oxide carbon utilization process (EBOCU) that enables electrochemical CO2 conversion to formic acid. The UK intensified electrocatalytic process combines three main components: 1) a novel bimetallic oxide electrocatalyst; 2) a stable electrochemical reactor using robust electrodes; and 3) a pressurized electrochemical reactor. The output from this project showed the economic viability of producing high-value formic acid from CO2 to both offset the cost associated with post-combustion CCS and reduce GHG emissions. This project developed and screened a series engineered catalysts to selectively reduce CO2 directly to formic acid. The best performing catalyst based on formic acid production, stability, and Faradaic efficiency, was immobilized on carbon electrodes, and tested inside a flow through reactor. After lab-scale testing was completed, the experimental data was used to perform a Life-Cycle Analysis (LCA) and conduct an Initial Technical and Economic Feasibility Study. The LCA showed a pathway to a net negative CO2 utilization process with the incorporation of renewable energy, while the TEA showed the potential to produce formic acid below the current commercial price. The UK EBOCU process was successfully demonstrated at the TRL3 level and has a clear pathway to further development and contribution to the nation’s ambitious decarbonization goals.

20 FOSSIL-FUELED POWER PLANTS↗

DOE OSTI2024

Implementation of Detailed Polyethylene Pyrolysis Kinetics into CFD Simulations using Machine Learning

Municipal solid waste (MSW) and waste plastics have received significant attention due to the issues of waste generation and storage, as well as their potential as an energy resource. High-density polyethylene (HDPE) makes up a large portion of plastic waste and has been the subject of several conversion studies. However, the mechanisms associated with converting HDPE through pyrolysis and gasification are extensive and complex making them difficult to implement into high-fidelity computational fluid dynamic (CFD) simulations. For this project, a primary pyrolysis mechanism containing 42 unique species and 737 heterogeneous reactions was used to generate kinetic data over a range of operating conditions. A machine learning (ML) model was developed to replicate the results of the detailed pyrolysis mechanism while significantly increasing the computational efficiency. A deep operator network (DeepONet) architecture was adopted to train the model using time steps relevant to CFD simulations. The ML used physics-based loss functions to ensure mass conservation. The ML model has been deployed in simple MFiX CFD simulations, single particle, and an experimental drop tube reactor, and has shown promising performance compared to the original scheme.

Houston, Ross↗

DOE OSTI2025

Baseline Cost Model for Hydropower: Documentation (2025)

Hydropower currently contributes about 80 GW of conventional and 23 GW of pumped storage capacity to the United States (US) power grid. Previous studies have estimated a considerable amount of remaining US hydropower resources, including non-powered dams (NPD) (Hadjerioua et al., 2012), new stream-reach developments (NSD) (Kao et al., 2014), pumped storage hydropower (PSH) and canal/conduit (Kao et al., 2022). The combined theoretical capacity potential of these various hydropower resources is comparable to the existing US hydropower capacity. There is a continuing interest in developing this hydropower potential, particularly to help meet the increasing demand for electricity. However, available data (Sasthav and Oladosu, 2022) show that the rate of new hydropower development has slowed considerably over time despite the interest of industry stakeholders. This is partly due to the competition from other energy resources and from the highly dispersed nature of remaining hydropower resources, which lead to high information requirements for evaluating the feasibility of potential projects. Cost information provides the most succinct summary of the feasibility of a potential hydropower project required by stakeholders, including developers, investors, policymakers, consumer groups, etc., considering investment options. The best estimates of hydropower costs can be obtained through detailed engineering design and cost assessments of individual projects. However, this approach has high data and resource (time, funds, cross-disciplinary expertise) requirements that render it inapplicable for rapid cost estimation with limited data. Although innovative approaches can overcome some of these impediments (see Oladosu and Ma, 2024 for such an application to potential NPD projects), the development of such approaches still requires significant amounts of resources and are not generally applicable to all hydropower project types. Therefore, statistical and parametric methods using simpler cost specifications remain of significant utility to hydropower stakeholders and are, at the least, complementary to more detailed approaches, particularly when evaluating many potential projects.

13 HYDRO ENERGY↗

NASA NTRS1976

On the observed annual cycle in the ocean-atmosphere heat balance over the Northern Hemisphere

Based on the best presently available satellite radiation, atmospheric and oceanic data sets, the long-term mean heat balance of the earth and its normal seasonal variation are investigated over the Northern Hemisphere. Quantitative estimates for the various flux and storage terms in the atmospheric and terrestrial branches of the heat balance are given for 10-deg-wide latitude belts and for each calendar month. The results are presented in both graphical and tabular form. As was known before, the storage of heat in the oceans is found to dominate the energy storage in the combined atmosphere-ocean-land-cryosphere system. In the tropics, large changes in oceanic heat storage are found in the 10 N-20 N belt with a maximum in spring and a minimum in late summer. The main new finding of this study is that the inferred oceanic heat transports appear to undergo very large seasonal variations especially in the tropics.

Oort, A. H.↗

NASA NTRS1985

Solar wind control of magnetospheric pressure (CDAW 6)

The CDAW 6 data base is used to compare solar wind and magnetospheric pressures. The flaring angle of the tail magnetopause is determined by assuming that the component of solar wind pressure normal to the tail boundary is equal to the total pressure within the tail. Results indicate an increase in the tail flaring angle from 18 deg to 32 deg prior to the 1055 substorm onset and a decrease to 25 deg after the onset. This behavior supports the concept of tail energy storage before the substorm and subsequent release after the onset.

Fairfield, D. H.↗

NASA NTRS2012

Identifying and Addressing Land Surface Model Deficiencies with Data Assimilation

Land surface models (LSMs) encapsulate our understanding of terrestrial water and energy cycle physics and provide estimates of land surface states and fluxes when and where measurement gaps exist. Gaps in our understanding of the physics are a different issue. Data assimilation can address that issue both directly, through updating of prognostic model variables, or indirectly, when the simulated world conflicts with observation, necessitating adjustment of the model. Here we will focus on the latter case and present several examples, including (1) depth to bedrock adjustment to accommodate assimilated GRACE terrestrial water storage data; (2) steps to prevent immediate melting of assimilated snow cover; (3) irrigation's contribution to evapotranspiration; (4) lessons learned from soil moisture data assimilation; (5) the potential impact of satellite based runoff observation

Rodell, Matthew↗

DOE OSTI2023

Energy-Efficient and Resilient Infrastructure: Simulation, Validation, and Installation

Advanced, high-performance computing at the National Renewable Energy Laboratory (NREL) has enabled access to vast data resources with cutting-edge software techniques to understand, design, plan for, and maintain energy-efficient and resilient infrastructure. We have focused on cities and airports, but the technology we have developed will easily translate to seaports, inland ports, military installations, or other complex and large-scale energy-intensive systems. We can digitally simulate and explore current and future scenarios to make datadriven decisions for optimizing advanced energy systems, transportation and building operations, infrastructure planning and expansion, and battery storage to guide short- and long-term investments, electrification strategies, and integration of new technologies.

Athena↗

DOE OSTI2023

Carbon Mitigation Potential of Heat Pump Integrated with Thermal Storage for Grid-Interactive Residential Buildings

Residential buildings’ heating and cooling loads are associated with significant carbon emissions and peak electricity demand. Phase change material (PCM) based thermal energy storage (TES) can be used for space heating and cooling by embedding into the heat pump equipment. Past work on TES integrated with heat pumps (HP) has demonstrated significant load shifting and economic benefits. However, the potential for TES to reduce carbon emissions has not been widely explored. This study evaluates carbon mitigation potential of an ice-based TES coupled to HP (HP-TES) based on a simple rule-based control strategy accounting for electric grid emissions data. A vapor compression HP model using Engineering Equation Solver (EES). The modeled HP-TES system for single-family residential building demonstrates decreased carbon emissions with reduced peak utility cost.

Sultan, Sara↗

DOE OSTI2026

Integrated Transmission-Distribution Multi-Period Switching for Wildfire Risk Mitigation: Improving Speed and Scalability with Distributed Optimization: Preprint

With increasingly severe wildfire conditions driven by climate change, utilities must manage the risk of wildfire ignitions from electric power lines. During "public safety power shutoff'" events, utilities de-energize power lines to reduce wildfire ignition risk, which may result in load shedding. Distributed energy resources provide flexibility that can help support the system to reduce load shedding when lines are de-energized. We investigate a coordinated transmission-distribution optimization problem that balances wildfire risk mitigation and load shedding. We model distribution systems that include battery energy storage systems which may support loads when transmission lines are de-energized. This multi-period integrated transmission-distribution optimal switching problem jointly optimizes line switching decisions, the generators' setpoints, load shedding, and the batteries' states of charge, resulting in significant computational challenges. To improve scalability, we decompose the problem over both space and time and apply a distributed optimization algorithm. Using a large-scale synthetic California test case with realistic distribution models and real wildfire risk data, we show that distributed optimization can solve large-scale multi-period switching problems that are otherwise intractable for centralized solvers. We also discuss challenges and future directions for improving the distributed algorithm's convergence performance as the number of time periods increases.

24 POWER TRANSMISSION AND DISTRIBUTION↗

DOE OSTI2022

Electrochemical Ammonia Compression

An electrochemical (EC) compressor is a solid-state compression device. For decades, researchers have been studying EC compressors for applications for a variety of energy systems. As the world transitions away from fossil fuel energy sources, EC compression emerges as a promising technique for energy storage, specifically energy stored in the form of pressurized ammonia. Ammonia is also a commonly used refrigerant. The present studies examine the viability of EC compression for ammonia storage and refrigeration. EC ammonia compression increases the concentration of an ammonia-hydrogen mixture via the input of electrical energy and a series of chemical reactions. A polymer electrolyte membrane separates the low-concentration side from the high-concentration side of the device. On the low-pressure (anode) side hydrogen atoms oxidize and react with ammonia molecules, forming positively charge ammonium ions. The ions traverse the membrane electrolytically. The ammonium ions are reduced and revert back to hydrogen and ammonia upon reaching the high-pressure (cathode). An external circuit provides the current needed to sustain the reactions. In this project, we studied the performance of the ammonia EC compressor under a variety of different conditions. We replicated preliminary data and using a small cell with 5 cm2 of active area. We demonstrated the operation of larger cells with 100 cm2 of active area. Further, we used a commercially available hydrogen EC compressor stack to analyze the scaled-up compressor performance. While previous experiments examined only the transient EC compressor performance, we developed test facilities that allowed the compressor to reach steady state. We analyzed the effects of pressure and current on the EC compressor performance. We measured the flow rates of gas leaving the compressors and analyzed the composition using gas chromatography. We tested methods of separating ammonia from the effluent vapor, which contained hydrogen and water vapor. We found that back diffusion adversely affected the performance, especially when we maintained high pressure lifts.

25 ENERGY STORAGE↗

DOE OSTI2019

Seminar 13 - Advanced Methods for Grid Integration of High-Performance Residential Communities

High-performance residential communities such as net-zero energy (NZE) and NZE-ready communities are emerging across the United States as many cities and states have committed to achieve ambitious energy efficiency and renewable energy goals between now and 2050. The achievement of these goals will transform the nation's communities into the holistic paradigms consisting of pervasive solar photovoltaics (PVs) and other renewable distributed energy resources, energy storage and flexible loads. However, integrating residential communities with high PV penetration may bring many challenges to the grid. For example, during many hours of the year, electric power is flowing out of PV-enabled homes and back into the grid. When this happens simultaneously in many nearby homes, distribution feeder voltage can be raised significantly. Intermittent solar power can also cause voltage flickers, leading to potential damages on both distribution feeder and home appliances. Existing solutions, such as PV curtailment, battery storage, and direct load control, are not able to address all the challenges in a cost-effective way. Better understanding is needed on how to deploy rooftop PV, how to predict building loads, and how to coordinate the homes in a community to enhance grid reliability. This seminar consists of four integral presentations that cover different aspects of a solution to these challenges. First, we will present an automated method to identify the best surfaces to deploy PV and size PV according to the PV penetration goals in a community. Second, we will present a streamlined way to create gray-box building models that are suitable for large-scale building-grid co-simulation. Next, we will present a data-driven method to estimate the end-use energy consumption to better coordinate the behind-the-meter resources to reduce utility cost, provide grid services, and improve renewable energy integration. Lastly, we will present a hierarchical control system that integrates the building models and the estimated non-dispatchable loads into the decision-making process to enhance the reliability and resilience of the residential community. Simulation results from an NZE-ready community in Fort Collins, Colorado will be presented in all four presentations and the guidelines on better grid integration of residential communities will be provided.

14 SOLAR ENERGY↗

DOE OSTI2022

Experimental Study of Eutectic Molten Salts NaCl/KCl/ZnCl2 Heat Transfer Inside a Smooth Tube for High-Temperature Application

Abstract Eutectic salts NaCl-KCl-ZnCl2 and NaCl-KCl-MgCl2 are two of the chloride salt systems that are promising for being used as high-temperature heat transfer fluid (HTF) and thermal energy storage (TES) materials in a wide range of temperatures from 230 °C to 750 °C in concentrated solar thermal power systems. To conduct measurement of the heat transfer coefficient of the molten salt at high temperatures, a circulation system and instrumentation of flow and heat transfer was constructed. Experimental measurement of the convective heat transfer coefficients of NaCl-KCl-ZnCl2 (molar fraction: 13.8–41.9–44.3%) inside tubes has been accomplished to find the most suitable heat transfer correlations. Experience of salt processing and operation of the high-temperature heat transfer test system was obtained. Two correlations, Dittus-Boelter equation and Gnielinski’s correlation for Nusselt number against Reynolds number and Prandtl number, are evaluated using the test results, and the latter correlation is recommended due to its better agreement of prediction against tested data.

Energy & Fuels↗

DOE OSTI2024

A Techno-Economic Analysis of a 50MWth Light-Trapping Cavity-Planar Solar Receiver Tower Capital Expenditures and its Cost Mitigation Strategies

To maximize thermal efficiency, the National Renewable Energy Laboratory (NREL) has proposed a light-trapping cavity-planar receiver design intended to capture energy from reradiating surfaces. This system implements a macroscale light trapping mechanism induced by panels with triangular channels, this mechanism allows for elevated temperatures on the receiver panels and in turn the temperature of the HTF; using this design coupled with the implementation of a fluidized particle flow as the HTF, it can be expected for some components to reach a peak working temperature of nearly 1000 degrees C cyclically throughout each day-night cycle. While these temperatures correlate to higher efficiency of the CSP tower they also demand intense thermomechanical properties from the materials used to make the receiver panels. In this analysis, we will list our assumptions to provide clarity on the significance of our calculation. This cost analysis will be conducted using a combination of both case study data and surveying industry to determine costs that are relevant to the current market trends. This analysis represents an early attempt to establish the Capital Expenditures required for a CSP tower of such design to determine the feasibility of implementing such a system in the industry.

concentrated solar power (CSP)↗

DOE OSTI2022

Residential Solar-Adopter Income and Demographic Trends: November 2022 Update [Slides]

The report describes income, demographic, and other socio-economic trends among U.S. residential rooftop solar adopters. The report is based on address-level data for roughly 2.8 million residential rooftop solar systems installed through 2021, representing 86% of all U.S. systems. With its unique size, geographic scope, and level of detail, this report is intended to serve as a foundational reference document for policy-makers, industry stakeholders, and researchers. Key findings include the following: -Median solar adopter income was about $\$110$k/year in 2021, compared to a U.S. median of about $\$63$k/year for all households and $\$79$k/year for all owner-occupied households -The degree of income skew varies significantly across all states, but all states exhibit some positive income skew, with median solar-adopter incomes ranging from 131-168% of the respective county-median income for all households -Notwithstanding the fact that solar adopter incomes skew high, a substantial share of adopters could be considered low-to-moderate income (LMI), with 22% of all 2021 adopters earning less than 80% of area median income, and an additional 21% between 80% and 120% of area median income. -Solar-adopter incomes are declining over time, with median incomes dropping from $\$129$k in 2010 to $\$110$k in 2021, as adoption becomes more proportionately distributed across the population and has started to broaden into low- and middle-income states since 2016. -Solar-adopter incomes are consistently higher for systems paired with battery storage, for host-owned systems, and for systems installed on single-family homes; higher income adopters also consistently install larger systems. -Solar adopters tend to live in Census Tracts not identified as “disadvantaged communities” (using the U.S. Department of Energy’s interim definitions developed March 2022), making up 11% of adopters compared to 18% of U.S. households. -Compared to the broader population, solar adopters tend to: identify as Non-Hispanic White, be primarily English-speaking, have higher education levels, be middle-aged, work in business and finance-related occupations, and live in higher-value homes In conjunction with the report, Berkeley Lab has published an updated accompanying set of online data visualizations that allow users to further explore the underlying data. Berkeley Lab is also offering related analytical support to states, local agencies, and other organizations on issues related to solar adoption among low-to-moderate income households; requests for analytical support may be submitted through this online form.

13 HYDRO ENERGY↗

DOE OSTI2024

Techno-economic analysis and network design for CO 2 conversion to jet fuels in the United States

The conversion of carbon dioxide (CO 2 ) into jet fuel holds significant potential for reducing CO 2 emissions, providing an alternative to carbon-based resources, and offering a renewable means of energy storage. The objective of this study is to conduct a techno-economic analysis and optimize the supply chain network for converting CO 2 to jet fuel in the United States, aiming to minimize total costs while assessing the environmental and economic feasibility of two CO 2 conversion pathways. This first pathway is based on Fischer-Tropsch synthesis (FTS), and the other one is based on the valorization and upgrading of light methanol (MeOH). Incorporating spatial and techno-economic data, a mixed-integer linear programming model was developed to select source plants and conversion pathways, locations of conversion refinery sites, and the amount of captured CO 2 across the United States. The optimal results indicate that the FTS pathway is adopted at all selected refineries when the hydrogen price is 1000 dollars/t and the operating cost, mainly electricity used in conversion, is reduced to 5 % of its current level. Under this scenario, the total annual profit is 8 billion dollars, and the net carbon emissions are -88,783,284 tons. The sensitivity analyses reveal that the prices of electricity and hydrogen significantly contribute to total production costs. The CO 2 recycle percentage of the FTS pathway influences the choice of applied pathways at refineries. Additionally, a higher conversion rate holds a substantial promise for reducing the total production cost and can make the MeOH pathway a viable choice.

10 SYNTHETIC FUELS↗

DOE OSTI2023

Final Report for ARPA-E LOCOMOTIVES Advanced Locomotive Technology and Rail Infrastructure Optimization System (ALTRIOS) Project

The Advanced Locomotive Technology and Rail Infrastructure Optimization System (ALTRIOS) is a unique, fully integrated, open-source software tool used to evaluate strategies for cost-effectively deploying advanced locomotive technologies and associated infrastructure. ALTRIOS simulates freight-demand-driven train scheduling, mainline meet-pass planning, locomotive dynamics, train dynamics, energy conversion efficiencies, and energy storage dynamics of line-haul train operations. Because new locomotives represent a significant long-term capital investment and new technologies must be thoroughly demonstrated before deployment, this tool provides guidance on the risk/reward trade-offs and operation integration of different technology rollout strategies. An open, integrated simulation tool is valuable for identifying future research needs and making decisions on technology development, routes, and train selection. This final report details the ALTRIOS software architecture, major modules and components, and data validation process. It demonstrates the software's utility through a 30-year rollout case study targeting high penetration of advanced powertrain technologies by 2050 for two BNSF Railway routes: loaded taconite ore trains from Hibbing, Minnesota, to Superior, Wisconsin, and mixed-freight trains from Superior to Minneapolis, Minnesota.

33 ADVANCED PROPULSION SYSTEMS↗

DOE OSTI2022

Guidelines for Publicly Archiving Terrestrial Model Data to Enhance Usability, Intercomparison, and Synthesis

Scientific communities are increasingly publishing data to evaluate, accredit, and build on published research. However, guidelines for curating data for publication are sparse for model-related research, limiting the usability of archived simulation data. In particular, there are no established guidelines for archiving data related to terrestrial models that simulate land processes and their coupled interactions with climate. Terrestrial modelers have a unique set of challenges when publishing data due to the diversity of scientific domains, research questions, and the types and scales of simulations. Researchers in the U.S. Department of Energy’s (DOE) projects use a variety of multiscale models to advance robust predictions of terrestrial and subsurface ecosystem processes. Here, we synthesize archiving needs for data associated with different DOE models, and provide guidelines for publishing terrestrial model data components following FAIR (Findable, Accessible, Interoperable, Reusable) principles. The guidelines recommend archiving model inputs and testing data used in final simulation runs along with associated codes, workflow scripts, and metadata in public repositories. Researchers should consider archiving model outputs if they are within the storage limits of the repository. We also provide considerations for how to bundle files into different data publications with citable digital object identifiers. Finally, we identify repository features and tools that would enable storage and reuse of model data. Given the diversity of DOE terrestrial models, these guidelines are transferable to other model types and will enable efficient reuse of simulation data for purposes such as model intercomparisons, initialization, benchmarking, synthesis, and comparisons with field observations.

58 GEOSCIENCES↗

NASA NTRS2004

Low Temperature Life-cycle Testing of a Lithium-ion Battery for Low-earth-orbiting Spacecraft

A flight-qualified, lithium-ion (Li-ion) battery developed for the Mars Surveyor Program 2001 lander is undergoing life-testing at low temperature under a low-Earth-orbit (LEO) profile to assess its capability to provide long term energy storage for aerospace missions. NASA has embarked upon an ambitious course to return humans to the moon by 2015-2020 in preparation for robotic and human exploration of Mars and robotic exploration of the moons of outer planets. Li-ion batteries are excellent candidates to provide power and energy storage for multiple aspects of these missions due to their low specific energy, low energy density, and excellent low temperature performance. Laboratory testing of Li-ion technology is necessary in order to assess lifetime, characterize multi-cell battery-level performance under aerospace conditions, and to gauge safety aspects of the technology. Life-cycle testing provides an opportunity to examine battery-level performance and the dynamics of individual cells in the stack over the entire life of the battery. Data generated through this testing will be critical to establish confidence in the technology for its widespread use in manned and unmanned mission. This paper discusses the performance of the 28 volt, 25 ampere-hour battery through 6000 LEO cycles, which corresponds to one year on LEO orbit. Testing is being performed at 0 C and 40% depth-of-discharge. Individual cell behaviors and their effect on the performance of the battery are described. Capacity, impedance, energy efficiency and end-of-discharge voltage at 1000 cycle intervals are reported. Results from this life-testing will help contribute to the database on battery-level performance of aerospace Li-ion batteries and low temperature cycling under LEO conditions.

Reid, Concha↗