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At least 1,387 records · Page 77
All sourcesNASA NTRSDOE OSTI
DOE OSTI2015

Beta decay rates of neutron-rich nuclei

Heavy element nucleosynthesis models involve various properties of thousands of nuclei in order to simulate the intricate details of the process. By necessity, as most of these nuclei cannot be studied in a controlled environment, these models must rely on the nuclear structure models for input. Of all the properties, the beta-decay half-lives are one of the most important ones due to their direct impact on the resulting abundance distributions. Currently, a single large-scale calculation is available based on a QRPA calculation with a schematic interaction on top of the Finite Range Droplet Model. In this study we present the results of a large-scale calculation based on the relativistic nuclear energy density functional, where both the allowed and the first-forbidden transitions are studied in more than 5000 neutron-rich nuclei.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2016

Beta decay rates of neutron-rich nuclei

Heavy element nucleosynthesis models involve various properties of thousands of nuclei in order to simulate the intricate details of the process. By necessity, as most of these nuclei cannot be studied in a controlled environment, these models must rely on the nuclear structure models for input. Of all the properties, the beta-decay half-lives are one of the most important ones due to their direct impact on the resulting abundance distributions. In this study we present the results of a large-scale calculation based on the relativistic nuclear energy density functional, where both the allowed and the first-forbidden transitions are studied in more than 5000 neutron-rich nuclei. Aside from the astrophysical applications, the results of this calculation can also be employed in the modeling of the electron and antineutrino spectra from nuclear reactors.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Imaging multiphoton ionization dynamics of CH 3 I at a high repetition rate XUV free-electron laser

XUV multiphoton ionization of molecules is commonly used in free-electron laser experiments to study charge transfer dynamics. However, molecular dissociation and electron dynamics, such as multiple photon absorption, Auger decay, and charge transfer, often happen on competing time scales, and the contributions of individual processes can be difficult to unravel. We experimentally investigate the Coulomb explosion dynamics of methyl iodide upon core–hole ionization of the shallow inner-shell of iodine (4d) and classically simulate the fragmentation by phenomenologically introducing ionization dynamics and charge transfer. Under our experimental conditions with medium fluence and relatively long XUV pulses (~75 fs), we find that fast Auger decay prior to charge transfer significantly contributes to the charging mechanism, leading to a yield enhancement of higher carbon charge states upon molecular dissociation. Furthermore, we argue for the existence of another charging mechanism for the weak fragmentation channels leading to triply charged carbon atoms. This study shows that classical simulations can be a useful tool to guide the quantum mechanical description of the femtosecond dynamics upon multiphoton absorption in molecular systems.

Optics↗
DOE OSTI2020

Search for New Bosons in Gluon-Gluon and Vector Boson Fusion Processes at the LHC and Development of Silicon Module Assembly Techniques for the CMS High Granularity Calorimeter

A search for heavy resonances decaying to a pair of vectors bosons is presented which utilizes events in which a hadronically decaying Z or W boson is identified using jet substructure techniques and large missing transverse momentum is found. Data analyzed were recorded by the Compact Muon Solenoid experiment at the CERN Large Hadron Collider in 2016, 2017, and 2018, and correspond to 137 fb$^{-1}$ . The events are categorized as having arisen from Vector Boson Fusion process or not, and are characterized by their transverse mass distribution. The standard model backgrounds are estimated based on observed yields in control regions. No excess of events above the expected SM background are observed and limits are placed on the production cross section of Radion (spin-0), Wprime (spin-1) and Bulk graviton (spin2) particles. In adiditon, the high luminosity LHC and the CMS HGCAL upgrade are also presented. The assembly techniques and various tests for the Silicon module and the cassette are discussed.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2024

Light new physics in B → K ( * ) ν ν ¯ ?

The study of the rare decays B → K ( * ) ν ν ¯ offers a window into the dynamics operating at the electroweak scale, allowing studies of the Standard Model and searches for heavy new physics. However, the analysis of these decays is also potentially sensitive to the on shell production of new light bosons X through the process B → K ( * ) X . In particular, Belle II has recently measured B + → K + ν ν ¯ , finding a 2.8 σ excess under the assumption of heavy new physics. Since this excess is rather localized in the kaon energy, a fit that includes the decay mode B + → K + X to the kinematic distributions prefers m X ≈ 2 GeV with branching fraction Br [ B → K X ] = ( 8.8 ± 2.5 ) × 10 − 6 and a significance of ≈ 3.6 σ . However, no excess was found in the measurements of B → K ( * ) ν ν ¯ , and a global analysis of the Belle II and data leads to Br [ B → K X ] = ( 5.1 ± 2.1 ) × 10 − 6 with a reduced significance of ≈ 2.4 σ . We then study various simplified dark-flavored models and present a possible UV completion based on a gauged B 3 − L 3 symmetry, highlighting the discovery potential of dedicated searches for B → K ( * ) X at Belle II. Published by the American Physical Society 2024

Astronomy & Astrophysics↗
DOE OSTI2018

Preferential Charge Generation at Aggregate Sites in Narrow Band Gap Infrared Photoresponsive Polymer Semiconductors

Infrared organic photodetector materials are investigated using transient absorption spectroscopy, demonstrating that ultrafast charge generation assisted by polymer aggregation is essential to compensate for the energy gap law, which dictates that excited state lifetimes decrease as the band gap narrows. Short sub–picosecond singlet exciton lifetimes are measured in a structurally related series of infrared–absorbing copolymers that consist of alternating cyclopentadithiophene electron–rich “push” units and strong electron–deficient “pull” units, including benzothiadiazole, benzoselenadiazole, pyridalselenadiazole, or thiadiazoloquinoxaline. While the ultrafast lifetimes of excitons localized on individual polymer chains suggest that charge carrier generation will be inefficient, high detectivity for polymer:PC 71 BM infrared photodetectors is measured in the 0.6 < λ < 1.5 µm range. The photophysical processes leading to charge generation are investigated by performing a global analysis on transient absorption data of blended polymer:PC 71 BM films. In these blends, charge carriers form primarily at polymer aggregate sites on the ultrafast time scale (within our instrument response), leaving quickly decaying single–chain excitons unquenched. Lastly, the results have important implications for the further development of organic infrared optoelectronic devices, where targeting processes such as excited state delocalization over aggregates may be necessary to mitigate losses to ultrafast exciton decay as materials with even lower band gaps are developed.

36 MATERIALS SCIENCE↗
DOE OSTI2013

Neutrino and Z gauge boson physics

We present a short review of the physics of neutrino-photon interactions and the rare decays of the Z and Z Prime gauge bosons. In particular, we emphasize on processes induced by the anomalous trilinear and quartic vertices VVV and VVVV, where V=Z,Z Prime or a photon, within the Standard Model (SM), the 331 model and some extensions of the SM. We also include the phenomenological and experimental limits reported for these couplings.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2014

New production mechanism for keV sterile neutrino Dark Matter by decays of frozen-in scalars

We propose a new production mechanism for keV sterile neutrino Dark Matter. In our setting, we assume the existence of a scalar singlet particle which never entered thermal equilibrium in the early Universe, since it only couples to the Standard Model fields by a really small Higgs portal interaction. For suitable values of this coupling, the scalar can undergo the so-called freeze-in process, and in this way be efficiently produced in the early Universe. These scalars can then decay into keV sterile neutrinos and produce the correct Dark Matter abundance. While similar settings in which the scalar does enter thermal equilibrium and then freezes out have been studied previously, the mechanism proposed here is new and represents a versatile extension of the known case. We perform a detailed numerical calculation of the DM production using a set of coupled Boltzmann equations, and we illustrate the successful regions in the parameter space. Our production mechanism notably can even work in models where active-sterile mixing is completely absent.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2014

An interpretation of flare-induced and decayless coronal-loop oscillations as interference patterns

We present an alternative model of coronal-loop oscillations, which considers that the waves are trapped in a two-dimensional waveguide formed by the entire arcade of field lines. This differs from the standard one-dimensional model which treats the waves as the resonant oscillations of just the visible bundle of field lines. Within the framework of our two-dimensional model, the two types of oscillations that have been observationally identified, flare-induced waves and 'decayless' oscillations, can both be attributed to MHD fast waves. The two components of the signal differ only because of the duration and spatial extent of the source that creates them. The flare-induced waves are generated by strong localized sources of short duration, while the decayless background can be excited by a continuous, stochastic source. Further, the oscillatory signal arising from a localized, short-duration source can be interpreted as a pattern of interference fringes produced by waves that have traveled diverse routes of various pathlengths through the waveguide. The resulting amplitude of the fringes slowly decays in time with an inverse square root dependence. The details of the interference pattern depend on the shape of the arcade and the spatial variation of the Alfvén speed. The rapid decay of this wave component, which has previously been attributed to physical damping mechanisms that remove energy from resonant oscillations, occurs as a natural consequence of the interference process without the need for local dissipation.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2023

A simplified protocol for the automated production of 2‐[ 18 F]fluoro‐3‐[2‐((S)‐3‐pyrrolinyl)methoxy]pyridine ([ 18 F]nifene) on an IBA Synthera® module

The α4β2 nicotinic acetylcholine receptor (nAChR) ligand 2‐[18F]fluoro‐3‐[2‐((S)‐3‐pyrrolinyl)methoxy]pyridine ([18F]nifene) has been synthesized in 10% decay‐corrected radiochemical yield using the IBA Synthera® platform (IBA Cyclotron Solutions, Louvain‐la‐Neuve, Belgium) with an integrated fluidic processor (IFP). Boc‐nitronifene served as the precursor, and 20% trifluoroacetic acid (TFA) was used to deprotect the Boc‐group after radiolabeling. By omitting the solvent extraction step after radiolabeling, the process was simplified to a single step with no manual intervention. [18F]Nifene was obtained in decay‐corrected radiochemical yields of 10 ± 2% (n = 20) and radiochemical purity >99%. Typical specific radioactivities of 2700–4865 mCi/μmole (100–180 GBq/μmol) were measured at the end of synthesis; total synthesis times were about 1 h 40 min.

IBA Synthera®↗
DOE OSTI2014

What perytons are not, and might be

Chirped radio pulses known as perytons are consistent with plasma propagation, but an astronomical origin has been excluded. This paper considers several physical processes as possible explanations. TE and TM waveguide modes have dispersion relations formally similar to those of plasmas, and emission at the plasma frequency of a plasma recombining by two-particle processes also produces a chirp δt∝ω{sup –2}, but these hypotheses fail quantitatively. The chirp might be approximately fitted to three-body recombination, cyclotron radiation in exponentially decaying fields, or to the resonance of a distributed LC circuit whose component conductors move. Constraints are placed on these possible processes, but no specific source has been identified.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2019

Oxygen Ion Dynamics in the Earth's Ring Current: Van Allen Probes Observations

Oxygen (O + ) enhancements in the inner magnetosphere are often observed during geomagnetically active times, such as geomagnetic storms. In this study, we quantitatively examine the difference in ring current dynamics with and without a substantial O + ion population based on almost 6 years of Van Allen Probes observations. Here, our results have not only confirmed previous finding of the role of O + ions to the ring current but also found that abundant O + ions are always present during large storms when sym-H < -60 nT without exception, while having the pressure ratio ($\mathscr{R}$) between O + and proton (H + ) larger than 0.8 and occasionally even larger than 1 when L < 3. Simultaneously, the pressure anisotropy decreases with decreasing sym-H and increasing L shell. The pressure anisotropy decrease during the storm main phase is likely related to the pitch angle isotropization processes. In addition, we find that $\mathscr{R}$ increases during the storm main phase and then decreases during the storm recovery phase, suggesting faster buildup and decay of O + pressure compared to H + ions, which are probably associated with some species dependent source and/or energization as well as loss processes in the inner magnetosphere.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2024

Anomalies in global SMEFT analyses. A case study of first-row CKM unitarity

Recent developments in the Standard Model analysis of semileptonic charged-current processes involving light quarks have revealed ~ 3σ tensions in Cabibbo universality tests involving meson, neutron, and nuclear beta decays. In this paper, we explore beyond the Standard Model explanations of this so-called Cabibbo Angle Anomaly in the framework of the Standard Model Effective Field Theory (SMEFT), including not only low-energy charged current processes (‘L’), but also electroweak precision observables (‘EW’) and Drell-Yan collider processes (‘C’) that probe the same underlying physics across a broad range of energy scales. The resulting ‘CLEW’ framework not only allows one to test explanations of the Cabibbo Angle Anomaly, but is set up to provide near model-independent analyses with minimal assumptions on the flavor structure of the SMEFT operators. Besides the global analysis, we consider a large number of simpler scenarios, each with a subset of SMEFT operators, and investigate how much they improve upon the Standard Model fit. We find that the most favored scenarios, as judged by the Akaike Information Criterion, are those that involve right-handed charged currents. Additional interactions, namely oblique operators, terms modifying the Fermi constant, and operators involving right-handed neutral currents, play a role if the CDF determination of the W mass is included in the analysis.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2018

On the Possibility of Delayed Fission of Nuclei in the Region of Superheavy Transuranium Elements

Delayed fission of atomic nuclei was discovered in 1966. It is observed primarily in odd–odd nuclei for which the energy released in beta decay (K capture) is commensurate with the fission barrier in the nucleus formed after this process. Delayed fission was found in four nuclide regions: neutrondeficient isotopes in the Pb region, neutron-deficient isotopes in the Ac and Pa regions, and neutrondeficient and neutron-rich isotopes of transuranium elements. In the wake of investigations into the properties of isotopes of superheavy transuranium elements, numerous calculations were performed in order to determine the masses of new nuclei and to predict their decay properties. Explored and predicted properties of superheavy-element nuclides, where, for some odd–odd nuclei of transuranium elements, the K-capture energy is commensurate with the fission barriers in the corresponding daughter nuclei formed after K capture, are analyzed. Estimates of the delayed-fission probability are presented for some isotopes of elements whose charge number Z ranges from 103 to 107.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2011

Tau Trigger at the ATLAS Experiment

Many theoretical models, like the Standard Model or SUSY at large tan({beta}), predict Higgs bosons or new particles which decay more abundantly to final states including tau leptons than to other leptons. At the energy scale of the LHC, the identification of tau leptons, in particular in the hadronic decay mode, will be a challenging task due to an overwhelming QCD background which gives rise to jets of particles that can be hard to distinguish from hadronic tau decays. Equipped with excellent tracking and calorimetry, the ATLAS experiment has developed tau identification tools capable of working at the trigger level. This contribution presents tau trigger algorithms which exploit the main features of hadronic tau decays and describes the current tau trigger commissioning activities. Many of the SM processes being investigated at ATLAS, as well as numerous BSM searches, contain tau leptons in their final states. Being able to trigger effectively on the tau leptons in these events will contribute to the success of the ATLAS experiment. The tau trigger algorithms and monitoring infrastructure are ready for the first data, and are being tested with the data collected with cosmic muons. The development of efficiency measurements methods using QCD and Z {yields} {tau}{tau} events is well advanced.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2020

A Comparison of RESRAD and GoldSim Models for Assessing Radiological Dose for a RCRA Landfill - 20418

US Ecology Idaho (USEI) operates a Resource Conservation and Recovery Act (RCRA) Subtitle C, Hazardous Waste Treatment, Storage, and Disposal (TSD) Facility on a 640-acre property in Owyhee County, Idaho. USEI accepts a wide variety of RCRA-exempt low activity radioactive wastes, including naturally occurring radioactive material (NORM) and technologically enhanced NORM (TENORM) (USEI 2009). The performance of the landfill with regard to radiological operating permit requirements was previously assessed using a model constructed with the residual radioactivity (RESRAD) computer program, developed by Argonne National Laboratory for the U.S. Department of Energy (DOE). RESRAD supports the evaluation of several environmental transport pathways related to a radionuclide-contaminated soil source term, but it was not conceived as a model for the evaluation of landfill radiological performance. A more comprehensive and realistic model is desired in order to better support submissions to both the State of Idaho's Department of Environmental Quality as well as the U.S. Nuclear Regulatory Commission. A Performance Assessment (PA) computer model was developed using GoldSim software for the USEI RCRA Subtitle C landfill. The RESRAD computer model was specifically developed for calculating soil cleanup criteria and radiological dose and cancer risk from residual radioactive material in soil. To evaluate site-specific conditions, users may select from among a number of available environmental transport and exposure pathways and modify 'default' parameter values. In GoldSim, a user must construct the model 'from scratch.' However, this modeling is facilitated by a number of specialized elements available in GoldSim to support a radiological mass transport model. These include elements for defining radiological decay and ingrowth, container failure and radiological release, advective and diffusive transport, and other processes. Advantages afforded by the use of RESRAD for modeling radiological dose for a RCRA Subtitle C landfill include ease of use and reasonable flexibility in specifying site-specific conditions. GoldSim allows for considerably more flexibility and site-specificity than RESRAD, including evaluation of potentially relevant environmental transport processes not supported in RESRAD. The probabilistic modeling capabilities of GoldSim also far exceed those of RESRAD. The pros and cons of RESRAD and GoldSim for this modeling problem are explored with a focus on identifying approaches and critical factors in identifying the appropriate platform. The capabilities of RESRAD and GoldSim for mathematically modeling the disposal system will be contrasted and compared. For example, the existing RESRAD radiological safety assessment evaluated potentially complete exposure pathways related to infiltration to groundwater and upwards diffusion of radon. Additional transport pathways identified in the USEI Idaho facility Conceptual Site Model include deposition of radon decay products in cover material, root uptake of radionuclides in disposed wastes by native plants, and mixing of cover material by burrowing animals. Results of the two models and how the different transport and dose pathways affect results will be discussed. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗
DOE OSTI2016

Factors influencing photoluminescence and photocarrier lifetime in CdSeTe/CdMgTe double heterostructures

CdSeTe/CdMgTe double heterostructures were produced with both n-type and unintentionally doped absorber layers. Measurements of the dependence of photoluminescence intensity on excitation intensity were carried out, as well as measurements of time-resolved photoluminescence decay after an excitation pulse. It was found that decay times under very low photon injection conditions are dominated by a non-radiative Shockley-Read-Hall process described using a recombination center with an asymmetric capture cross section, where the cross section for holes is larger than that for electrons. As a result of the asymmetry, the center effectively extends photoluminescence decay by a hole trapping phenomenon. A reduction in electron capture cross section appeared at doping densities over 10 16 cm -3 . An analysis of the excitation intensity dependence of room temperature photoluminescence revealed a strong relationship with doping concentration. Here, this allows estimates of the carrier concentration to be made through a non-destructive optical method. Iodine was found to be an effective n-type dopant for CdTe, allowing controllable carrier concentrations without an increased rate of non-radiative recombination.

14 SOLAR ENERGY↗
DOE OSTI2019

Measurement of the 65 Cu(η, γ) cross section using the Detector for Advanced Neutron Capture Experiments at LANL

Improving our understanding of the origin of the elements in the observable universe as well as the nature of the environments responsible for their production has been of paramount importance to the nuclear physics community. More than half of the isotopes of these elements are created via neutron-capture processes, and thus accurate measurements of the salient underlying nuclear physics, such as neutron-capture cross sections, masses, and β-decay half-lives are crucial. Of particular signifcance to the synthesis of isotopes in the mass range of A ≈ 60 to A ≈ 90, via the weak s process, are the neutron-capture cross sections of 63,65 Cu, where large discrepancies between measurements exist. Recent measurements have addressed these discrepancies for 63 Cu [Weigand et al., Phys. Rev. C 95, 015808 (2017)], but questions still remain for 65 Cu. Here, we report a new measurement of the 65Cu(n, γ ) cross section performed using the Detector for Advanced Neutron Capture Experiments located at the Los Alamos Neutron Science Center of Los Alamos National Laboratory. The Maxwellian-averaged cross section (MACS) for 65 Cu(η, γ) at $kT$ = 30 keV deduced from this work is (37.0 ± 0.3 stat. ± 3.3 sys. ) mb. The impact on weak s-process nucleosynthesis of new MACS values, calculated over the range of kT = 5 to 100 keV, for 65 Cu, combined with the updated MACS for 63 Cu [Weigand et al., Phys. Rev. C 95, 015808 (2017)] and 63 Ni [Weigand et al., Phys. Rev. C 92, 045810 (2015)], were investigated. Findings of this investigation show an increase of predicted nucleosynthesis yields of elements of Zn to Zr by as much as 20%.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗