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At least 1,369 records · Page 76

Improving GCM Predictability of Mixed-Phase Clouds and Aerosol Interactions at High Latitudes with ARM Observations

The overachieving goal of this project is to improve the predictability of mixed-phase clouds and aerosol interactions in the Community Atmosphere Model version 6 (CAM6) through comparison with the ARM observations. There are three main objectives of the proposed study: (1) Improve the representation of ice microphysical processes in mixed-phase clouds; (2) Test the performance of ice microphysics in CESM-CAM6 with the ARM observations in northern and southern high latitudes; and (3) Examine mixed-phase cloud microphysics-aerosol-turbulence-radiation interactions in CESM-CAM6. In this project, we have (1) Improved the representation of ice microphysical processes in mixed-phase clouds in CESM-CAM6 by implementing the marine organic aerosol (MOA) and treating the ice nucleating particles (INPs) from MOA and its impacts on mixed-phase clouds. We improved the treatment of ice depositional growth through the Wegener–Bergeron–Findeisen (WBF) process by considering the subgrid heterogeneous distributions between liquid droplets and ice crystals in mixed-phase clouds; (2) Tested the performance of ice microphysics in CESM-CAM6 with the ARM observations at high latitudes. We compared the simulated INP concentrations with the ARM observations, e.g., from M-PACE, ISDAC, INPOP, and other data (Mace Head, Zeppelin, CAPRICORN). We examined the impact of improved WBF treatment on model simulated Arctic mixed-phase clouds observed in the M-PACE field campaign. Seasonal variations of modeled mixed-phase cloud properties (LWO, IWP) are compared with the ground-based remote sensing retrievals at the ARM’s NSA $Utqia\dot{g}vik$ site; and (3) Examined mixed-phase cloud microphysics-aerosol-dynamics-radiation interactions in CESM-CAM6 that include the impacts of MOA INPs, and impacts of different model parameterizations (CLUBB versus UW turbulence & shallow convection schemes, MG2 versus MG1) on high-latitude mixed-phase cloud properties. Aerosol indirect effects of MOA through the liquid phase (droplet activation) and ice phase processes (e.g., the glaciation indirect effect) were investigated.

54 ENVIRONMENTAL SCIENCES↗

Jupiter's atmosphere - Observations and interpretation of the microwave spectrum near 1.25-cm wavelength

Measurements of Jupiter's disk-temperature spectrum in the 20- to 24-GHz (1.5 cm less than lambda less than 1.25 cm) region are reported. These data are combined with previously published data to produce a uniformly calibrated thermal spectrum of Jupiter in the wavelength interval 0.85 to 2.1 cm. Model studies are carried out to determine optimum pressure-temperature profiles for an assumed radiative-convective temperature structure. It is found that the temperature at the 1-bar total effective pressure level is between 140 and 165 K, with a most probable value of 153 K, provided that NH3 is uniformly saturated in the clouds on a global scale. We show that the temperature profile for the microwave model is approximately 20 K cooler than the profiles derived from infrared data. An explanation of this discrepancy is discussed in terms of a model which invokes different NH3 distributions in the belts and zones.

Klein, M. J.↗

Estimates of radiative flux divergence in the atmosphere from satellite data

Several options for the inference of the atmospheric radiative flux divergence (ARD) on the basis of satellite data are discussed. Attention is given to the clear-sky case and the cloudy-sky case. LW ARD profiles for different climatological regimes are presented and the effect of cloud base height on LW ARD divergence at various heights is illustrated.

Smith, G. L.↗

Natural and anthropogenic perturbations of the stratospheric ozone layer

The paper reviews potential causes for reduction in the ozone abundance. The response of stratospheric ozone to solar activity is discussed. Ozone changes are simulated in relation with the potential development of a fleet of high-speed stratospheric aircraft and the release in the atmosphere of chlorofluorocarbons. The calculations are performed by a two-dimensional chemical-radiative-dynamical model. The importance of heterogeneous chemistry in polar stratospheric clouds and in the Junge layer (sulfate aerosol) is emphasized. The recently reported ozone trend over the last decade is shown to have been largely caused by the simultaneous effects of increasing concentrations of chlorofluorocarbons and heterogeneous chemistry. The possibility for a reduction in stratospheric ozone following a large volcanic eruption such as that of Mount Pinatubo in 1991 is discussed.

Brasseur, Guy P.↗

Cloud-Scale Numerical Modeling of the Arctic Boundary Layer

The research objective of this NASA grant-funded project was to determine in detail how large-scale processes. in combination with cloud-scale radiative, microphysical, and dynamical processes, govern the formation and multi-layered structure of Arctic stratus clouds. This information will be useful for developing and improving 1D (one dimensional) boundary layer models for the Arctic. Also, to quantitatively determine the effects of leads on the large-scale budgets of sensible heat, water vapor, and condensate in a variety of Arctic winter conditions. This information will be used to identify the most important lead-flux processes that require parameterization in climate models. Our approach was to use a high-resolution numerical model, the 2D (two dimensional) University of Utah Cloud Resolving Model (UU CRM), and its 1D version, the University of Utah Turbulence Closure Model (UU TCM), a boundary layer model based on third-moment turbulence closure, as well as a large-eddy simulation (LES) model originally developed by C.H. Moeng.

Kruegen, Steven K.↗

A Cloud Greenhouse Effect on Mars: Significant Climate Change in the Recent Past

The large variations in Mars orbit parameters are known to be significant drivers of climate change on the Red planet. The recent discovery of buried CO2 ice at the South Pole adds another dimension to climate change studies. In this paper we present results from the Ames GCM that show within the past million years it is possible that clouds from a greatly intensified Martian hydrological cycle may have produced a greenhouse effect strong enough to raise global mean surface temperatures by several tens of degrees Kelvin. It is made possible by the ability of the Martian atmosphere to transport water to high altitudes where cold clouds form, reduce the outgoing longwave radiation, and drive up surface temperatures to maintain global energy balance.

Haberle, Robert M.↗

ARM Research in the Equatorial Western Pacific: A Decade and Counting

The tropical western Pacific (TWP) is an important climatic region. Strong solar heating, warm sea surface temperatures, and the annual progression of the intertropical convergence zone (ITCZ) across this region generate abundant convective systems, which through their effects on the heat and water budgets have a profound impact on global climate and precipitation. In order to accurately evaluate tropical cloud systems in models, measurements of tropical clouds, the environment in which they reside, and their impact on the radiation and water budgets are needed. Because of the remote location, ground-based datasets of cloud, atmosphere, and radiation properties from the TWP region have come primarily from short-term field experiments. While providing extremely useful information on physical processes, these short-term datasets are limited in statistical and climatological information. To provide longterm measurements of the surface radiation budget in the tropics and the atmospheric properties that affect it, the Atmospheric Radiation Measurement program established a measurement site on Manus Island, Papua New Guinea, in 1996 and on the island republic of Nauru in late 1998. These sites provide unique datasets now available for more than 10 years on Manus and Nauru. This article presents examples of the scientific use of these datasets including characterization of cloud properties, analysis of cloud radiative forcing, model studies of tropical clouds and processes, and validation of satellite algorithms. New instrumentation recently installed at the Manus site will provide expanded opportunities for tropical atmospheric science.

tropical regions↗

Understanding Seasonal Variability in Thin Cirrus Clouds from Continuous MPLNET Observations at GSFC in 2012

Optically thin cirrus cloud (optical depth < 0.3) net radiative forcing represents one of the primary uncertainties in climate feedback, as sub-visible clouds play a fundamental role in atmospheric radiation balance and climate change. A lidar is a very sensitive optical device to detect clouds with an optical depth as low as 10-4. In this paper we assess the daytime net radiative forcing of sub-visible cirrus clouds detected at Goddard Space Flight Center, a permanent observational site of the NASA Micro Pulse Lidar Network in 2012. Depending on their height, season and hour of the day, the solar albedo effect can outweigh the infrared greenhouse effect, cooling the earth atmosphere system rather than warming it exclusively. As result, based on latitude, the net forcing of sub-visible cirrus clouds can be more accurately parameterized in climate models.

Lolli, Simone↗

Direct Radiative Effect of Aerosols Based on PARASOL and OMI Satellite Observations

Accurate portrayal of the aerosol characteristics is crucial to determine aerosol contribution to the Earth's radiation budget. We employ novel satellite retrievals to make a new measurement-based estimate of the shortwave direct radiative effect of aerosols (DREA), both over land and ocean. Global satellite measurements of aerosol optical depth, single-scattering albedo (SSA), and phase function from PARASOL (Polarization and Anisotropy of Reflectances for Atmospheric Sciences coupled with Observations from a Lidar) are used in synergy with OMI (Ozone Monitoring Instrument) SSA. Aerosol information is combined with land-surface bidirectional reflectance distribution function and cloud characteristics from MODIS (Moderate Resolution Imaging Spectroradiometer) satellite products. Eventual gaps in observations are filled with the state-of-the-art global aerosol model ECHAM5-HAM2. It is found that our estimate of DREA is largely insensitive to model choice. Radiative transfer calculations show that DREA at top-of-atmosphere is −4.6 +/- 1.5 W/sq m for cloud-free and −2.1 +/- 0.7 W/sq m for all-sky conditions, during year 2006. These fluxes are consistent with, albeit generally less negative over ocean than, former assessments. Unlike previous studies, our estimate is constrained by retrievals of global coverage SSA, which may justify different DREA values. Remarkable consistency is found in comparison with DREA based on CERES (Clouds and the Earth's Radiant Energy System) and MODIS observations.

Globalsatellite measurements↗

Global tropospheric ozone investigations

Ozone (O3) is one of the most important trace gases in the troposphere, and it is responsible for influencing many critical chemical and radiative processes. Ozone contributes to the formation of the hydroxyl radical (OH), which is central to most chemical reactions in the lower atmosphere, and it absorbs UV, visible, and infrared radiation which affects the energy budget and atmospheric temperatures. In addition, O3 can be used as a tracer of atmospheric pollution and stratosphere troposphere exchange. At elevated concentrations, O3 can also produce detrimental biological and human health effects. The US National Research Council (NRC) Board on Sustainable Development reviewed the US Global Change Research Program (USGCRP) [NRC, 1995], and it identified tropospheric chemistry as one of the high priority areas for the USGCRP in the next decade. The NRC identified the following specific challenges in tropospheric chemistry. Although we understand the reason for the high levels of 03 over several regions of the world, we need to better establish the distribution of O3 in the troposphere in order to document and understand the changes in the abundance of global tropospheric O3. This information is needed to quantify the contribution of O3 to the Earth' s radiative balance and to understand potential impacts on the health of the biosphere. Having recognized the importance of particles in the chemistry of the stratosphere, we must determine how aerosols and clouds affect the chemical processes in the troposphere. This understanding is essential to predict the chemical composition of the atmosphere and to assess the resulting forcing effects in the climate system. We must determine if the self-cleansing chemistry of the atmosphere is changing as a result of human activities. This information is required to predict the rate at which pollutants are removed from the atmosphere. Over nearly two decades, airborne Differential Absorption Lidar (DIAL) systems have been used in over fifteen major field experiments conducted all over the world to address important atmospheric processes affecting the amount and distribution of 03 and aerosols across the troposphere. This paper discusses some of these wide-ranging field experiments and their results and presents a direction for future global studies of O3 and aerosols from space.

Browell, Edward V.↗

Clouds and Radiation Processes in Regional Climate Models Evaluated Using Observations Over the Ice‐free Arctic Ocean

Abstract The presence of clouds in the Arctic regulates the surface energy budget (SEB) over the sea‐ice surface and the ice‐free ocean. Following several previous field campaigns, the cloud‐radiation relationship, including cloud vertical structure and phase, has been elucidated; however, modeling of this relationship has matured slowly. In recognition of the recent decline in the Arctic sea‐ice extent, representation of the cloud system in numerical models should consider the effects of areas covered by sea ice and ice‐free areas. Using an in situ stationary meteorological observation data set obtained over the ice‐free Arctic Ocean by the Japanese Research Vessel Mirai (September 2014), coordinated evaluation of six regional climate models (RCMs) with nine model runs was performed by focusing on clouds and the SEB. The most remarkable findings were as follows: (1) reduced occurrence of unstable stratification with low‐level cloud water in all models in comparison to the observations, (2) significant differences in cloud water representations between single‐ and double‐moment cloud schemes, (3) extensive differences in partitioning of hydrometeors including solid/liquid precipitation, and (4) pronounced lower‐tropospheric air temperature biases. These issues are considered as the main sources of SEB uncertainty over ice‐free areas of the Arctic Ocean. The results from a coupled RCM imply that the SEB is constrained by both the atmosphere and the ocean (and sea ice) with considerable feedback. Coordinated improvement of both stand‐alone atmospheric and coupled RCMs would promote a more comprehensive and improved understanding of the Arctic air‐ice‐sea coupled system.

Inoue, Jun↗

Marine and continental stratocumulus cloud microphysical properties obtained from routine ARM Cimel sunphotometer observations

This study investigates marine and continental stratocumulus (Sc) cloud properties obtained from an automated implementation of a multispectral photometer retrieval. Photometer methods simultaneously retrieve cloud optical depth (τ) and cloud droplet effective radius (r e ), with estimates for liquid water path (LWP) calculated on the availability of those quantities. These applied methods evaluate retrieved cloud properties for Sc identified during a recent 6 year period over the U.S. Department of Energy Atmospheric Radiation Measurement (ARM) program sites in Oklahoma, USA (SGP) and in the Azores, Portugal (ENA). Modest agreement in key quantity retrievals is found between the routine photometer products and multisensor collocated profiling references. Cumulative breakdowns contingent on cloud thickness indicate increases in all retrieved quantities in thicker clouds, with larger discrepancies in the relative performance between the retrievals collected in the presence of drizzle. Under continental cloud conditions, the clouds of a similar thickness and r e to those sampled under marine conditions report a factor of 1.5 larger τ and LWP. An r 2 ≅0.65 is found between photometer τ retrievals and shadowband radiometer measurements, with photometer retrievals reporting a high (relative) bias. The τ intercomparisons indicate that variability between retrievals is a factor of three larger than errors reported from individual retrieval input perturbation tests. Photometer r e retrievals suggest a low r 2 (< 0.1) having a standard deviation ≅ 3 µm when compared to ARM baseline multi-sensor radar/radiometer references (accounting for offsets in the cloud droplet number concentration assumptions of the latter). However, photometer LWP calculations remain relatively unbiased in non-drizzling conditions, with errors O (50 g m −2 ) and r 2 ≅0.5 to collocated radiometer and interferometer references. Additional sensitivity tests for island influences on marine Sc properties suggest that while island-influenced winds may promote larger cloud LWP or thickness, the influence could be within retrieval method uncertainty and/or collocated instrument variability.

54 ENVIRONMENTAL SCIENCES↗

First Results of Submillimeter Polarimetry

Airborne results of submillimeter polarization at one wavelength, 270 micro m for just three points in the sky are presented. Polarizations of 1.7% at each of two points in Orion are shown. A null result at 400 micro m from ground-based observations of Mars at opposition is also presented. A null result for W3(OH) is given. The Kleinmann-Low Nebula (KL) was chosen for one of the measurements because it is bright and polarization had been observed 10 micro m. Airborne results of submillimeter polarimetry indicate that: (1) Cool, dense interstellar clouds can emit polarized submillimeter radiation; (2) The direction of the magnetic field, averaged over the 90 beams, is the same for the Kleinmann-Low Nebula and the 400 micro m peak 1.5 south of the Nebula; and (3) The effectiveness of the grain alignment mechanism, averaged over the 90 beams, is the same for the Kleinmann-Low Nebula and the 400 micro m peak.

Hildebrand, R. H.↗

Influence of cirrus clouds on weather and climate processes A global perspective

Current understanding and knowledge of the composition and structure of cirrus clouds are reviewed and documented in this paper. In addition, the radiative properties of cirrus clouds as they relate to weather and climate processes are described in detail. To place the relevance and importance of cirrus composition, structure and radiative properties into a global perspective, pertinent results derived from simulation experiments utilizing models with varying degrees of complexity are presented; these have been carried out for the investigation of the influence of cirrus clouds on the thermodynamics and dynamics of the atmosphere. In light of these reviews, suggestions are outlined for cirrus-radiation research activities aimed toward the development and improvement of weather and climate models for a physical understanding of cause and effect relationships and for prediction purposes.

Liou, K.-N.↗

Atmospheric circulation of Venus

Observational data of Venus are utilized to study rotational effects on atmospheric circulations. The high surface temperature and planetary-scale turbulent motion at cloud tops, and the relation between energy and momentum budget are examined. The limited amount of data available on the vertical and horizontal distribution of net radiative heating, the zonal wind structure, and waves affects the study of the temperature and motion on Venus. The limitations of the scaling analysis used to estimate the properties of the circulation as regards the cyclostrophic balance, the extent of the Hadley circulation, large-scale wave transport, vertical propagation of waves, convection, and turbulence are considered. Hypotheses concerned with the deep, cloud-level, and upper atmospheres of Venus are proposed. Future research in the areas of propagating planetary- scale waves, zonal flow and planetary-scale wave instability processes, and convection is suggested.

Rossow, W. B.↗

Cirrus properties deduced from CO2 lidar observations of zenith-enhanced backscatter from oriented crystals

Many lidar researchers have occasionally observed zenith-enhanced backscatter (ZEB) from middle and high clouds. The ZEB signature consists of strong backscatter when the lidar is pointed directly at zenith and a dramatic decline in backscatter as the zenith angle dips slightly off zenith. Mirror-like reflection from horizontal facets of oriented crystals (especially plates) is generally accepted as the cause. It was found during a 3-year observation program that approximately 50 percent of ice clouds had ZEB, regardless of cloud height. The orientation of crystals and the ZEB they cause are important to study and understand for several reasons. First, radiative transfer in clouds with oriented crystals is different than if the same particles were randomly oriented. Second, crystal growth depends partly on the orientation of the particles. Third, ZEB measurements may provide useful information about cirrus microphysical and radiative properties. Finally, the remarkable effect of ZEB on lidar signals should be understood in order to properly interpret lidar data.

Eberhard, Wynn L.↗

Shortwave radiative parameterization of large atmospheric aerosols - Dust and water clouds

A parameterization of the single scattering properties of an aerosol for a dust layer in the solar spectral region is presented. The parameterization scheme accounts for the microphysical changes of an aerosol layer and is applied to dust and water clouds. A scaling parameter is presented which describes, simply and effectively, the optical properties of an aerosol layer with a large effective size parameter.

Ackerman, Steven A.↗

North Atlantic Aerosol Radiative Effects Based on Satellite Measurements and Aerosol Intensive Properties from TARFOX and ACE-2

We estimate the impact of North Atlantic aerosols on the net shortwave flux at the tropopause by combining maps of satellite-derived aerosol optical depth (AOD) with model aerosol properties. We exclude African dust, primarily by restricting latitudes to 25-60 N. Aerosol properties were determined via column closure analyses in two recent experiments, TARFOX and ACE 2. The analyses use in situ measurements of aerosol composition and air- and ship-borne sunphotometer measurements of AOD spectra. The resulting aerosol model yields computed flux sensitivities (dFlux/dAOD) that agree with measurements by airborne flux radiometers in TARFOX. It has a midvisible single-scattering albedo of 0.9, which is in the range obtained from in situ measurements of aerosol scattering and absorption in both TARFOX and ACE 2. Combining seasonal maps of AVHRR-derived midvisible AOD with the aerosol model yields maps of 24-hour average net radiative flux changes at the tropopause. For cloud-free conditions, results range from -9 W/sq m near the eastern US coastline in the summer to -1 W/sq m in the mid-Atlantic during winter; the regional annual average is -3.5 W/sq m. Using a non- absorbing aerosol model increases these values by about 30%. We estimate the effect of clouds using ISCCP cloud-fraction maps. Because ISCCP midlatitude North Atlantic cloud fractions are relatively large, they greatly reduce the computed aerosol-induced flux changes. For example, the regional annual average decreases from -3.5 W/sq m to -0.8 W/sq m. We compare results to previous model calculations for a variety of aerosol types.

Bergstrom, Robert W.↗