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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 1,369 records · Page 76
All sourcesNASA NTRSDOE OSTI
DOE OSTI2020

Beneficial Effect of Li 5 FeO 4 Lithium Source for Li-Ion Batteries with a Layered NMC Cathode and Si Anode

The energy density of lithium-ion batteries can be increased by replacing the traditional graphite anode with a high capacity silicon anode. However, volume changes and interfacial instabilities cause a large irreversible capacity and a continual loss of lithium during cycling, which lead to rapid capacity loss. In this work, we add Li 5 FeO 4 (LFO) to a LiNi 0.5 Mn 0.3 Co 0.2 O 2 (NMC) cathode as a pre-lithiation additive, which increases the lithium inventory and extends the cycle life of Si-graphite/NMC full cells, and decreases the NMC particle degradation. LFO delivers a large 764 mAh g –1 LFO capacity below 4.7 V vs Li/Li + . By tuning the LFO content in Si-graphite/LFO-NMC full cells, we show higher capacity, improved retention, lower impedance, and superior rate performance compared to full cells without LFO. Post-test characterizations demonstrate that LFO inclusion in the cathode matrix leads to less NMC secondary particle segregation/cracking and a thinner surface reduced layer on the NMC particles. The beneficial effects of LFO endure after the lithium reserve has been exhausted, highlighting a lasting synergy between the lithium source and electrode active materials. This study introduces a new approach to simultaneously increase lithium inventory and reduce cathode degradation, and makes critical advances toward enabling Si anodes for lithium-ion batteries.

25 ENERGY STORAGE↗
DOE OSTI2016

Overview of Recent Studies and Design Changes for the FNAL Magnetron Ion Source

This paper will cover several studies and design changes that will eventually be implemented to the Fermi National Accelerator Laboratory (FNAL) magnetron ion source. The topics include tungsten cathode insert, solenoid gas valves, current controlled arc pulser, cesium boiler redesign, gas mixtures of hydrogen and nitrogen, and duty factor reduction. The studies were performed on the FNAL test stand described in [1], with the aim to improve source lifetime, stability, and reducing the amount of tuning needed.

43 PARTICLE ACCELERATORS↗
DOE OSTI2015

BNL 56 MHz HOM DAMPER FABRICATION AT JLAB

The Higher-Order Mode (HOM) Dampers for the Relativistic Heavy-Ion Collider’s (RHIC) 56 MHz cavity at Brookhaven National Laboratory (BNL) are currently being fabricated at JLab. The coaxial damper is primarily constructed with high RRR niobium, with a combination of niobium and sapphire rings as the filter assembly. Several design changes have been made with respect to the performance of a prototype damper – also fabricated at JLab – which was found to quench at low power. The production dampers are being tuned and tested in the JLab vertical test area (VTA) prior to delivery. Two HOM dampers will be delivered to BNL; they are to be used in the RHIC in November, 2015. This paper outlines the challenges faced in the fabrication and tuning process.

Huque, Naeem A.↗
DOE OSTI2017

Producing coherent excitations in pumped Mott antiferromagnetic insulators

Nonequilibrium dynamics in correlated materials has attracted attention due to the possibility of characterizing, tuning, and creating complex ordered states. To understand the photoinduced microscopic dynamics, especially the linkage under realistic pump conditions between transient states and remnant elementary excitations, we performed nonperturbative simulations of various time-resolved spectroscopies. We used the Mott antiferromagnetic insulator as a model platform. The transient dynamics of multi-particle excitations can be attributed to the interplay between Floquet virtual states and a modification of the density of states, in which interactions induce a spectral weight transfer. Using an autocorrelation of the time-dependent spectral function, we show that resonance of the virtual states with the upper Hubbard band in the Mott insulator provides the route towards manipulating the electronic distribution and modifying charge and spin excitations. In conclusion, our results link transient dynamics to the nature of many-body excitations and provide an opportunity to design nonequilibrium states of matter via tuned laser pulses.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2020

Integrated performance of large HDC-capsule implosions on the National Ignition Facility

In this paper, we report on eight, indirect-drive, deuterium–tritium-layered, inertial-confinement-fusion experiments at the National Ignition Facility to determine the largest capsule that can be driven symmetrically without relying on cross-beam energy transfer or advanced Hohlraum designs. Targets with inner radii of up to 1050 μm exhibited controllable P 2 symmetry, while larger capsules suffered from diminished equatorial drive. Reducing the Hohlraum gas-fill-density from 0.45 mg/cm 3 to 0.3 mg/cm 3 did not result in a favorable shift of P 2 amplitude as observed in preceding tuning experiments. Reducing the laser-entrance-hole diameter from 4 mm to 3.64 mm decreased polar radiation losses as expected, resulting in an oblate symmetry. The experiments exhibited the expected performance benefit from increased experimental scale, with yields at a fixed implosion velocity roughly following the predicted 1D dependence. With an inner radius of 1050 μm and a case-to-capsule-ratio of 3.0, experiment N181104 is the lowest implosion-velocity experiment to exceed a total neutron yield of 10 16 .

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2016

NULLING DATA REDUCTION AND ON-SKY PERFORMANCE OF THE LARGE BINOCULAR TELESCOPE INTERFEROMETER

The Large Binocular Telescope Interferometer (LBTI) is a versatile instrument designed for high angular resolution and high-contrast infrared imaging (1.5–13 μ m). In this paper, we focus on the mid-infrared (8–13 μ m) nulling mode and present its theory of operation, data reduction, and on-sky performance as of the end of the commissioning phase in 2015 March. With an interferometric baseline of 14.4 m, the LBTI nuller is specifically tuned to resolve the habitable zone of nearby main-sequence stars, where warm exozodiacal dust emission peaks. Measuring the exozodi luminosity function of nearby main-sequence stars is a key milestone to prepare for future exo-Earth direct imaging instruments. Thanks to recent progress in wavefront control and phase stabilization, as well as in data reduction techniques, the LBTI demonstrated in 2015 February a calibrated null accuracy of 0.05% over a 3 hr long observing sequence on the bright nearby A3V star β Leo. This is equivalent to an exozodiacal disk density of 15–30 zodi for a Sun-like star located at 10 pc, depending on the adopted disk model. This result sets a new record for high-contrast mid-infrared interferometric imaging and opens a new window on the study of planetary systems.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2016

High Performance Teams Enable Mission Success for SRNL - 16363

The accomplishment of the DOE EM mission of cleaning up the radioactive waste generated as a byproduct of the development and maintenance of nuclear materials over the last 60 years is a daunting task. SRNL specializes in working directly with the 'owners' of the cleanup challenges to identify the desired outcome and develop a solution that can be put into practice. 'We put science to work' is not just a 'tag line' rather it is a concise statement of our values and approach to applying science and engineering to the cleanup objectives. The management of radioactive waste poses multi-decade challenges to DOE EM and the Nation. The ability to harness the depth of knowledge, experience, expertise and passion for safely and effectively solving the technical challenges has reached a critical junction. Perhaps too late to be a natural and organic transition the industry finds itself critically devoid of resources to effectively and efficiently keep focused on the highest order task: cleanup. When project managers plan the resources necessary to perform the planned scope they typically are focused on financial, human, and industrial resources that would be beneficial to project execution. The critical shortage we will be evaluating is experienced and skilled leaders, mentors and coaches in the workforce. The production of educated scientists and engineers is a primary focus at all levels of educational institutions with Science Technology Engineering and Mathematics (STEM) focused curricula beginning in elementary school. The need for leaders who are skilled in inspiring organizational creativity, adept in harnessing and focusing individual energy while effectively communicating to the work force and the clientele equally compelling messages, has never been greater, or their absence in the workforce more ominous. Managers trained in the classical management theory (insert references here) are aging out of the workforce. In many cases these managers have not retained close connection to advancements in their primary field of study but rather have succumbed to the administrivia burdens that typify highly regulated work. The current technically trained workforce while interested in the 'perks' of management (i.e. visibility, pay increases, advancing status) are driven to keep close connection to their technical 'roots' as a fall-back plan should they need to change their career path either by choice or necessity. The challenge is how to achieve the productive hum of a finely tuned organizational model that blends executive vision and drive with technical leadership and excellence in execution. If any of these three tenets of a high performance team falters the ability to recover erodes the performance of the team and begins to weaken the cultural foundation essential to sustaining high performance work teams. At SRNL, recognition of the need to adapt the management dynamics and the business model and to harness the energy of the workforce to sustain - and in fact increase - the level of performance is a driving force in the transformation of the organization. Examples of changes in organizations structure, business systems and employee engagement are discussed as they relate to the impact on accomplishing the cleanup mission and fostering the next generation of great leaders and innovators. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗
DOE OSTI2016

ORION: A Framework for GPU Occupancy Tuning

An important feature of modern GPU architectures is variable occupancy. Occupancy measures the ratio between the number of active threads on a GPU and the maximum number of threads the GPU hardware can schedule. High occupancy allows a large number of threads to run simultaneously and hide memory latency, but may increase resource contention. Low occupancy has less resource contention, but is also less capable of latency hiding. Occupancy tuning is an important and challenge problem. A program running at different occupancy levels can have three to four times difference in running time. There has been limited exploration in GPU program occupancy tuning. We introduce Orion, the first GPU occupancy tuning framework.

Modeling and Performance Analysis↗
DOE OSTI2019

Model Predictive Control Tuning by Inverse Matching for a Wave Energy Converter

This paper investigates the application of a method to find the cost function or the weight matrices to be used in model predictive control (MPC) such that the MPC has the same performance as a predesigned linear controller in state-feedback form when constraints are not active. This is potentially useful when a successful linear controller already exists and it is necessary to incorporate the constraint-handling capabilities of MPC. This is the case for a wave energy converter (WEC), where the maximum power transfer law is well-understood. In addition to solutions based on numerical optimization, a simple analytical solution is also derived for cases with a short prediction horizon. These methods are applied for the control of an empirically-based WEC model. The results show that the MPC can be successfully tuned to follow an existing linear control law and to comply with both input and state constraints, such as actuator force and actuator stroke.

16 TIDAL AND WAVE POWER↗
DOE OSTI2025

Mesoporous Thin Film Architectures: Addressing Material Demands through Molecular Self-Assembly

Mesoporous thin films spark interest across a wide range of disciplines due to their tunable nanostructures, large internal surface areas, and strong compatibility with planar optical, electronic, and microfluidic devices. While attention in the porous materials community has shifted toward macroporous or disordered nanoporous systems, a resurgence in mesoporous thin film research is underway, driven by new molecular self-assembly methods, advanced materials chemistry, and improved characterization techniques. The integration of high-χN block copolymer design, kinetically persistent micelle templating, and postdeposition processing protocols now allows control over structural parameters such as pore size, wall thickness, porosity, and connectivity. These advances have overcome many of the thermodynamic and processing constraints that previously limited widespread adoption. Rather than serving only as high-surface-area supports, mesoporous thin films are engineered as active interfaces where responsive chemistries and nanoscale confinement act in tandem. Embedding switchable ligands, thermoresponsive polymers, redox mediators, or ion-selective groups directly within the pore walls enables real-time control over transport, optical, and electrochemical properties. These capabilities open up new directions in adaptive coatings, gated membranes, and fast-response biosensors. To further expand their functional scope, mesoporous films are integrated into hierarchical and multicomponent architectures. Techniques such as triblock terpolymer templating, crack-directed assembly, and nanoimprint lithography allow for control over spatial organization on the micron and submicron scale and pore system orientation. This enables programmable anisotropy, enhanced molecular diffusion, and wavelength-selective photonic behavior, essential for next-generation sensing, catalysis, and energy applications. Such structural and functional complexity requires equally sophisticated characterization. Multimodal and in situ techniques can track material dynamics under operational conditions. Recent progress includes extended-range ellipsometric porosimetry (EP) for hierarchical architectures, vacuum EP for interface energetics, time-resolved EP for diffusion kinetics, and correlative AFM-SAXS mapping. The introduction of advanced neutron-based spectroscopies, particularly quasielastic neutron scattering (QENS), promises to provide real-time access to ion transport dynamics and segmental motion under nanoscale confinement, offering a path toward deeper mechanistic understanding of structure-performance correlations in mesoporous systems. This Account reflects the technical advances made and the interdisciplinary collaborations that have shaped our collective vision. The particular dimensions of mesopores enable us to subtly tune interactions at the molecular, interfacial, and mesoscopic levels that permit us to harness nanoconfinement. What emerges is a versatile, modular platform capable of chemical gating, energy transduction, and sensing with a level of tunability unmatched by other porous materials. We highlight critical challenges including the need for more robust large-area processing, a deeper understanding of dynamic behavior under cycling, and better integration with device-level architectures. Our strategies support the transition of mesoporous thin films into active high-performance components in next-generation energy, environmental, and biomedical systems.

oxides↗
DOE OSTI2017

Optimizing qPlus sensor assemblies for simultaneous scanning tunneling and noncontact atomic force microscopy operation based on finite element method analysis

Quartz tuning forks that have a probe tip attached to the end of one of its prongs while the other prong is arrested to a holder (“qPlus” configuration) have gained considerable popularity in recent years for high-resolution atomic force microscopy imaging. The small size of the tuning forks and the complexity of the sensor architecture, however, often impede predictions on how variations in the execution of the individual assembly steps affect the performance of the completed sensor. Extending an earlier study that provided numerical analysis of qPlus-style setups without tips, this work quantifies the influence of tip attachment on the operational characteristics of the sensor. The results using finite element modeling show in particular that for setups that include a metallic tip that is connected via a separate wire to enable the simultaneous collection of local forces and tunneling currents, the exact realization of this wire connection has a major effect on sensor properties such as spring constant, quality factor, resonance frequency, and its deviation from an ideal vertical oscillation.

42 ENGINEERING↗
DOE OSTI2015

Status of the MeLoDIE experiment, an advanced device for the study of the irradiation creep of LWR cladding with full online capabilities

As a prototype of future instrumented material experiments in the Jules Horowitz Reactor (JHR), the MELODIE project was launched in 2009 by the CEA in collaboration with VTT. Being designed as a biaxial creep experiment with online capability, MELODIE is able to apply an online-controlled biaxial loading on a LWR clad sample up to 120 MPa and to perform an online measurement of its biaxial deformation. An important experimental challenge was to perform reliably accurate measurements under the high nuclear heat load of in-core locations while keeping within their tight space. For that purpose, specific sensors were co-designed with and built by IFE Halden. Manufacturing of the MELODIE components was completed one year ago. The complexity of its in-pile section and of the pressurization system requested a step-by-step tuning of the setup. The toughest part of this process dealt with the Diameter gauge which required a partial redesign to take into account unexpected and unwanted electromagnetic interactions with the hosting device. Final cold performance tests of the on-board instrumentation will be presented. The MELODIE device is now ready and irradiation should start in OSIRIS reactor this spring. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗
DOE OSTI2017

Hardware Acceleration of Adaptive Neural Algorithms.

As tradit ional numerical computing has faced challenges, researchers have turned towards alternative computing approaches to reduce power - per - computation metrics and improve algorithm performance. Here, we describe an approach towards non - conventional computing that strengthens the connection between machine learning and neuroscience concepts. The Hardware Acceleration of Adaptive Neural Algorithms (HAANA) project ha s develop ed neural machine learning algorithms and hardware for applications in image processing and cybersecurity. While machine learning methods are effective at extracting relevant features from many types of data, the effectiveness of these algorithms degrades when subjected to real - world conditions. Our team has generated novel neural - inspired approa ches to improve the resiliency and adaptability of machine learning algorithms. In addition, we have also designed and fabricated hardware architectures and microelectronic devices specifically tuned towards the training and inference operations of neural - inspired algorithms. Finally, our multi - scale simulation framework allows us to assess the impact of microelectronic device properties on algorithm performance.

97 MATHEMATICS AND COMPUTING↗
DOE OSTI2020

Studies of Beam Intensity Effects in Fermilab Booster Synchrotron. Part II: Beam Emittance Evolution

Detrimental beam dynamics effects limit performance of high intensity rapid cycling synchrotrons (RCS) such as the 8 GeV Fermilab Booster. Here we report the results of comprehensive studies of various beam intensity dependent effects in the Booster. In the previous publication we presented the dependencies of the Booster beam intensity losses on the total number of protons per pulse and on key operational parameters such as the machine tunes and chromaticities. Here we discuss two methods of the Booster beam emittance measurements (the multi-wires proportional chambers and the ionization profile monitors), analyze the intensity dependent emittance growth effects and discuss the ultimate performance of the machine now and after foreseen and proposed upgrades.

43 PARTICLE ACCELERATORS↗
DOE OSTI2016

Towards Achieving Performance Portability Using Directives for Accelerators

In this paper we explore the performance portability of directives provided by OpenMP 4 and OpenACC to program various types of node architectures with attached accelerators, both self-hosted multicore and offload multicore/GPU. Our goal is to examine how successful OpenACC and the newer offload features of OpenMP 4.5 are for moving codes between architectures, how much tuning might be required and what lessons we can learn from this experience. To do this, we use examples of algorithms with varying computational intensities for our evaluation, as both compute and data access efficiency are important considerations for overall application performance. We implement these kernels using various methods provided by newer OpenACC and OpenMP implementations, and we evaluate their performance on various platforms including both X86_64 with attached NVIDIA GPUs, self-hosted Intel Xeon Phi KNL, as well as an X86_64 host system with Intel Xeon Phi coprocessors. In this paper, we explain what factors affected the performance portability such as how to pick the right programming model, its programming style, its availability on different platforms, and how well compilers can optimize and target to multiple platforms.

97 MATHEMATICS AND COMPUTING↗
DOE OSTI2025

Cage Balancing Enhances Optoelectronic and Lasing Performance in Stable Quasi-2D Tin Iodide Perovskites

Two-dimensional (2D) tin halide perovskites are highly tunable and low-toxicity semiconductors, promising for next-generation optoelectronics. However, achieving air stability and excellent photophysical properties simultaneously necessitates deliberate structure tuning using organic spacer cations and A-site cations. Here, we report a series of new quasi-2D Ruddlesden–Popper tin halide perovskites using a fluorinated aromatic spacer cation, 4-fluorophenethylammonium (4FPEA), and systematically investigate the impacts of layer thickness, spacer cation, and A-site cation on the crystal structures and optical properties of (4FPEA) 2 (A) n−1 S n I 3n+1 . These 4FPEA-based 2D tin perovskites, further tuned by the A-cations, exhibit uniquely undistorted 180° out-of-plane Sn–I–Sn bond angles and low octahedral distortions compared to other quasi-2D perovskites and demonstrate prolonged air stability, excellent photophysics, and amplified spontaneous emission and lasing in exfoliated microflakes. A comprehensive survey of reported n = 2 lead and tin iodide perovskites reveals that all structures can be classified into three types (tilted, balanced, and buckled) based on the structural distortion parameters of their perovskite cages. Notably, (4FPEA) 2 (A)Sn 2 I 7 are among the handful of “balanced” n = 2 perovskites with minimal distortion and excellent optoelectronic performance. Furthermore, the structural insights and cage-balancing approach revealed herein motivate the deliberate design of quasi-2D perovskites through the synergy of the spacer and cage cations, further paving the way for high-performance optoelectronic applications of stable tin halide perovskites.

Cations↗
DOE OSTI2023

Hexagonal Boron Nitride Reinforced Multifunctional Well Cement for Extreme Conditions

The overarching objective of this project was to provide a system approach for developing the next generation of well cementing with remarkable multifunctional, high performance characteristics including mechanical, thermal, rheological and durability properties to prevent offshore spill and leakage at extreme high temperature, high pressure (HTHP) and corrosive conditions. Building on our scientifically illustrated principles, the objective of Phase I was to develop and tune our current proof-of-concept hexagonal boron-nitride (hBN)/cement composite to offer the best hybrid nanostructure, and optimum slurry formulation and rheological properties in environments with a variety of extreme conditions including high temperature, high pressure, and high acidity. This phase also focused on testing the actual barrier efficiency and performance of our new cement formulation against gas/liquid leakage at HT, and/or corrosive conditions. The objective of Phase 2 was product validation (meeting API/EPA standards), cost/risk analysis, and scale-up to facilitate integration for primary well cementing with no/minimal modification.

02 PETROLEUM↗