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DOE OSTI2020

Nonreciprocal directional dichroism of a chiral magnet in the visible range

Nonreciprocal directional dichroism is an unusual light–matter interaction that gives rise to diode-like behavior in low-symmetry materials. The chiral varieties are particularly scarce due to the requirements for strong spin–orbit coupling, broken time-reversal symmetry, and a chiral axis. Here we bring together magneto-optical spectroscopy and first-principles calculations to reveal high-energy, broadband nonreciprocal directional dichroism in Ni 3 TeO 6 with special focus on behavior in the metamagnetic phase above 52 T. In addition to demonstrating this effect in the magnetochiral configuration, we explore the transverse magnetochiral orientation in which applied field and light propagation are orthogonal to the chiral axis and, by so doing, uncover an additional configuration with a unique nonreciprocal response in the visible part of the spectrum. In a significant conceptual advance, we use first-principles methods to analyze how the Ni 2+ d-to-d on-site excitations develop magneto-electric character and present a microscopic model that unlocks the door to theory-driven discovery of chiral magnets with nonreciprocal properties.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

DOE OSTI2014

Latitude survey investigation of galactic cosmic ray solar modulation during 1994-2007

The Galactic cosmic ray spectrum exhibits subtle variations over the 22 yr solar magnetic cycle in addition to the more dramatic variations over the 11 yr sunspot cycle. Neutron monitors are large ground-based detectors that provide accurate measurements of variations in the cosmic ray flux at the top of the atmosphere above the detector. At any given location the magnetic field of the Earth excludes particles below a well-defined rigidity (momentum per unit charge) known as the cutoff rigidity, which can be accurately calculated using detailed models of the geomagnetic field. By carrying a neutron monitor to different locations, e.g., on a ship, the Earth itself serves as a magnet spectrometer. By repeating such latitude surveys with identical equipment, a sensitive measurement of changes in the spectrum can be made. In this work, we analyze data from the 1994 through 2007 series of latitude surveys conducted by the Bartol Research Institute, the University of Tasmania, and the Australian Antarctic Division. We confirm the curious 'crossover' in spectra measured near solar minima during epochs of opposite solar magnetic polarity, and show that it is directly related to a sudden change in the spectral behavior of solar modulation at the time of the polarity reversal, as revealed from contemporaneous variations in the survey data and a fixed station. We suggest that the spectral change and crossover result from the interaction of effects due to gradient/curvature drifts with a systematic change in the interplanetary diffusion coefficient caused by turbulent magnetic helicity.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2023

Diamagnetic mechanism of critical current non-reciprocity in multilayered superconductors

The suggestion that non-reciprocal critical current (NRC) may be an intrinsic property of non-centrosymmetric superconductors has generated renewed theoretical and experimental interest motivated by an analogy with the non-reciprocal resistivity due to the magnetochiral effect in uniform materials with broken spatial and time-reversal symmetry. Theoretically it has been understood that terms linear in the Cooper pair momentum do not contribute to NRC, although the role of higher-order terms remains unclear. In this work we show that critical current non-reciprocity is a generic property of multilayered superconductor structures in the presence of magnetic field-generated diamagnetic currents. In the regime of an intermediate coupling between the layers, the Josephson vortices are predicted to form at high fields and currents. Experimentally, we report the observation of NRC in nanowires fabricated from InAs/Al heterostructures. The effect is independent of the crystallographic orientation of the wire, ruling out an intrinsic origin of NRC. Non-monotonic NRC evolution with magnetic field is consistent with the generation of diamagnetic currents and formation of the Josephson vortices. This extrinsic NRC mechanism can be used to design novel devices for superconducting circuits.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2014

SiN-SiC nanofilm: A nano-functional ceramic with bipolar magnetic semiconducting character

Nowadays, functional ceramics have been largely explored for application in various fields. However, magnetic functional ceramics for spintronics remain little studied. Here, we propose a nano-functional ceramic of sphalerite SiN-SiC nanofilm with intrinsic ferromagnetic order. Based on first principles calculations, the SiN-SiC nanofilm is found to be a ferromagnetic semiconductor with an indirect band gap of 1.71 eV. By mean field theory, the Curie temperature is estimated to be 304 K, close to room temperature. Furthermore, the valence band and conduction band states of the nanofilm exhibit inverse spin-polarization around the Fermi level. Thus, the SiN-SiC nanofilm is a typical bipolar magnetic semiconductor in which completely spin-polarized currents with reversible spin polarization can be created and controlled by applying a gate voltage. Such a nano-functional ceramic provides a possible route for electrical manipulation of carrier's spin orientation.

36 MATERIALS SCIENCE↗

DOE OSTI2010

Invariant expansion for the trigonal band structure of graphene.

We present a symmetry analysis of the trigonal band structure in graphene, elucidating the transformational properties of the underlying basis functions and the crucial role of time-reversal invariance. Group theory is used to derive an invariant expansion of the Hamiltonian for electron states near the K points of the graphene Brillouin zone. Besides yielding the characteristic k-linear dispersion and higher oder corrections to it, this approach enables the systematic incorporation of all terms arising from external electric and magnetic fields, strain, and spin-orbit coupling up to any desired order. Several new contributions are found, in addition to reproducing results obtained previously within tight-binding calculations. Physical ramifications of these new terms are discussed.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2023

Microscopic Imaging Homogeneous and Single Phase Superfluid Density in $\mathrm{UTe_2}$

Odd-parity superconductor $\mathrm{UTe_2}$ shows spontaneous time-reversal symmetry breaking and multiple superconducting phases, which imply chiral superconductivity, but only in a subset of samples. Here, we microscopically observe a homogeneous superfluid density $n_s$ on the surface of $\mathrm{UTe_2}$ and an enhanced superconducting transition temperature near the edges. We also detect vortex-antivortex pairs even at zero magnetic field, indicating the existence of a hidden internal field. The temperature dependence of $n_s$, determined independent of sample geometry, does not support point nodes along the $b$ axis for a quasi-2D Fermi surface and provides no evidence for multiple phase transitions in $\mathrm{UTe_2}$.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

NASA NTRS1985

ISEE 1 and 2 observation of the spatial structure of a compressional Pc5 wave

A compressional Pc5 was observed on an ISEE 1 and 2 outbound path on September 28, 1981 at L = 5.6-7.3 near the magnetic equator at about 10 hr local time during the recovery phase of a geomagnetic storm. The wave propagated westward with a large azimuthal wave number of about 30 and exhibited in-phase oscillations of plasma density and magnetic field magnitude. During this event, component-dependent variations in phase and amplitude were observed for the magnetic field oscillations. The radial and compressional components had a constant phase and their amplitude was finite. In contrast, the azimuthal component changed its phase by 180 deg and its amplitude became zero during the middle of the wave event. The observation as indicating the spatial structure of the Pc5 wave is interpreted. The polarization reversal is likely to be caused by a crossing of a node of a standing wave located 4 deg above the geomagnetic equator.

Takahashi, K.↗

NASA NTRS1986

Magnetization modeling in the north and equatorial Atlantic Ocean using MAGSAT data

Magsat 2 x 2-deg scalar anomalous-magnetic-field data (Langel et al., 1982) for the northern and equatorial Atlantic are inverted and combined with physiographic data and laboratory results on the magnetization of oceanic rocks and the oceanic crust to construct models explaining the shorter-wavelength component of the anomalies. An annihilator is applied to the inversion results to eliminate reverse-magnetized sources and facilitate comparisons of areas inverted separately, and a latitude effect on source spacing is tentatively attributed to greater noise contamination at lower latitudes. It is found that remanent magnetization combined with considerable crustal thickening can best explain the high intensity levels observed, although viscous magnetization or contamination of the data by noncrustal sources must also be considered.

Hayling, K. L.↗

DOE OSTI2014

Millimeter wave ferromagnetic resonance in gallium-substituted ε-iron oxide

In millimeter wave frequency range, hexagonal ferrites with high uniaxial anisotropic magnetic fields are used as absorbers. These ferrites include M-type barium ferrite (BaFe{sub 12}O{sub 19}) and strontium ferrite (SrFe{sub 12}O{sub 19}), which have natural ferromagnetic resonant frequency range from 40 GHz to 60 GHz. However, the higher frequency range lacks suitable materials that support the higher frequency ferromagnetic resonance. A new series of gallium-substituted ε-iron oxides (ε-Ga{sub x}Fe{sub 2−x}O{sub 3}) are synthesized which have ferromagnetic resonant frequencies appearing over the frequency range 30 GHz–150 GHz. The ε-Ga{sub x}Fe{sub 2−x}O{sub 3} is synthesized by the combination of reverse micelle and sol-gel techniques or the sol-gel method only. The particle sizes are observed to be smaller than 100 nm. In this paper, the free space magneto-optical approach has been employed to study these newly developed ε-Ga{sub x}Fe{sub 2−x}O{sub 3} particles in millimeter waves. This technique enables to obtain precise transmission spectra to determine the dielectric and magnetic properties of both isotropic and anisotropic ferrites in the millimeter wave frequency range from a single set of direct measurements. The transmittance and absorbance spectra of ε-Ga{sub x}Fe{sub 2−x}O{sub 3} are shown in this paper. Strong ferromagnetic resonances at different frequencies determined by the x parameter are found.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2011

THE INTERNAL-COLLISION-INDUCED MAGNETIC RECONNECTION AND TURBULENCE (ICMART) MODEL OF GAMMA-RAY BURSTS

The recent Fermi observation of GRB 080916C shows that the bright photosphere emission associated with a putative fireball is missing, which suggests that the central engine likely launches a Poynting-flux-dominated (PFD) outflow. We propose a model of gamma-ray burst (GRB) prompt emission in the PFD regime, namely, the Internal-Collision-induced MAgnetic Reconnection and Turbulence (ICMART) model. It is envisaged that the GRB central engine launches an intermittent, magnetically dominated wind, and that in the GRB emission region, the ejecta is still moderately magnetized (e.g., 1 {approx}< {sigma} {approx}< 100). Similar to the internal shock (IS) model, the mini-shells interact internally at the radius R{sub IS} {approx} {Gamma}{sup 2} c{Delta}t. Most of these early collisions, however, have little energy dissipation, but serve to distort the ordered magnetic field lines entrained in the ejecta. At a certain point, the distortion of magnetic field configuration reaches the critical condition to allow fast reconnection seeds to occur, which induce relativistic MHD turbulence in the interaction regions. The turbulence further distorts field lines easing additional magnetic reconnections, resulting in a runway release of the stored magnetic field energy (an ICMART event). Particles are accelerated either directly in the reconnection zone, or stochastically in the turbulent regions, which radiate synchrotron photons that power the observed gamma rays. Each ICMART event corresponds to a broad pulse in the GRB light curve, and a GRB is composed of multiple ICMART events. This model retains the merits of IS and other models, but may overcome several difficulties/issues faced by the IS model (e.g., low efficiency, fast cooling, electron number excess, Amati/Yonetoku relation inconsistency, and missing bright photosphere). Within this model, the observed GRB variability timescales could have two components, one slow component associated with the central engine time history, and another fast component associated with relativistic magnetic turbulence in the emission region. The model predicts a decrease of gamma-ray polarization degree and E{sub p} in each ICMART event (broad pulse) during the prompt GRB phase, as well as a moderately magnetized external reverse shock. The model may be applied to the GRBs that have time-resolved, featureless Band-function spectra, such as GRB 080916C and most GRBs detected by Fermi LAT.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2015

Microstructure and magnetic properties of (001) textured L1(0) FePt films on amorphous glass substrate

L1(0) FePt thin films with an island-like morphology and magnetic perpendicular anisotropy were grown at low temperature (300 < T-dep< 375 degrees C) by magnetron sputtering on Hoya glass substrates using a 30-nm thick Cr (2 0 0) underlayer. An MgO buffer layer with a thickness of 2 nm was used to inhibit the diffusion from the Cr underlayer and promote the growth of (0 0 1) oriented L1(0) FePt films by inducing an in-plane lattice distortion. By varying the substrate temperature and the Ar sputter pressure (3.5 < P-Ar< 15 mTorr) during the deposition, the degree of chemical order, the microstructure and the magnetic properties were tuned and the best properties in term of squareness ratio (M-r/M-s similar to 0.95) and coercive field (H-c similar to 14 kOe) were observed for films deposited at T-dep = 350 degrees C and P-Ar= 5 mTorr, due to the appearance of a tensile strain, which favors the perpendicular anisotropy. The analysis of the angular dependence of remanent magnetization curves on the optimized sample suggests that the magnetization reversal is highly incoherent due to the inter-island interactions. Our results provide useful information on the low temperature growth of FePt films with perpendicular anisotropy onto glass substrates, which are relevant for a variety of technological applications, such as magnetic recording and spintronic devices. (C) 2015 Elsevier B.V. All rights reserved.

Speliotis, T↗

DOE OSTI2018

Pore-size resolved water vapor adsorption kinetics of white cement mortars as viewed from proton NMR relaxation

The dynamic pore structure of partially saturated cement-based material is rather essential to quantify its mass transport and many other properties. To clarify the influence of water removal and re-entry, the low-field nuclear magnetic resonance technique is employed to characterize the pore structure of two white cement mortars during isopropanol exchange and water vapor adsorption kinetics. It is found that, after isopropanol replacement the pore structures of mortars become remarkably coarsen due to the significant collapse of C-S-H interlayer pores, which are only partly reversible at water re-saturation. Consistently, water vapor adsorption is not a simple progressively filling process from finer to coarser pores, but accompanied by continuous expansion of C-S-H gel adsorbing water in priority. Furthermore, the irrecoverable contraction of C-S-H gel is the physical root of irreversible shrinkage. The smaller BET surface area using nitrogen than water is also attributed to the collapse of interlayer pores after drying.

36 MATERIALS SCIENCE↗

DOE OSTI2016

First-principles approach to investigate toroidal property of magnetoelectric multiferroic GaFeO{sub 3}

A first-principles approach incorporating the concept of toroidal moments as a measure of the spin vortex is proposed and applied to simulate the toroidization of magnetoelectric multiferroic GaFeO{sub 3}. The nature of space-inversion and time-reversal violations of ferrotoroidics is reproduced in the simulated magnetic structure of GaFeO{sub 3}. For undoped GaFeO{sub 3}, a toroidal moment of −22.38 μ{sub B} Å per unit cell was obtained, which is the best theoretical estimate till date. Guided by the spin vortex free-energy minimization perturbed by an externally applied field, it was discovered that the minority spin markedly biases the whole toroidization. In summary, this approach not only calculates the toroidal moment but provides a way to understand the toroidal nature of magnetoelectric multiferroics.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

DOE OSTI2022

Anomalous Shiba states in topological iron-based superconductors

We demonstrate the formation of robust zero energy modes close to magnetic impurities in the iron-based superconductor FeSe 1–x Te x . We find that the Zeeman field generated by the impurity favors a spin-triplet inter-orbital pairing as opposed to the spin-singlet intra-orbital pairing prevalent in the bulk. The preferred spin-triplet pairing preserves time-reversal symmetry and is topological, as robust, topologically-protected zero modes emerge at the boundary between regions with different pairing states. Moreover, the zero modes form Kramers doublets that are insensitive to the direction of the spin polarization or to the separation between impurities. Here, we argue that our theoretical results are consistent with recent experimental measurements on FeSe 1–x Te x .

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

NASA NTRS1983

Eddy intrusion of hot plasma into the polar cap and formation of polar-cap arcs

Plasma and electric field signatures of polar cap arcs in their formation region above 5000 km are examined. Signatures for active and for quiet magnetic conditions are presented, both indicating a virtual equivalence of plasma and electric field signatures between the polar and evening discrete arcs, although their optical configurations can be very different. It is proposed that the two types of arcs are indeed the same at active times except that the polar cap arcs occur at multiple convection reversal boundaries of plasmasheet plasmas which intrude into the normal polar cap in the form of multiple cellular eddies. A far-reaching consequence of this hypothesis is the unification of arc formation theory clarifying the distinct roles of arc formation parallel electric fields and of arc configuration and location. Optical and particle data which support this hypothesis are discussed.

Chiu, Y. T.↗

NASA NTRS1999

Dissipative Processes in the Magnetopause Boundary Layer and Flux Transfer Events Using the Interball Spacecraft

Work on two quite distinct projects was accomplished: a study of flux transfer events and a study of the magnetosheath-polar cusp interface. The study with Oleg Vaisberg of the Space Research Institute in Moscow used only Interball data. We analyzed the magnetometer data and to assist the observations of Flux Transfer Events (FTEs) to aid in the interpretation of the data. One of the issues was to distinguish between simple traversals of the magnetopause and encounters with FTES. Once that distinction became clear then we could examine the changes in the plasma associated with the FTE. The second study was undertaken to study the turbulent interaction of the magnetosheath flow past the polar cusp. In this study Polar Data was used inside the magnetosphere as Interball crossed through the cusp into the magnetosheath. Our most interesting but least turbulent example was on May 29, 1996 when the interplanetary magnetic field (IMF) was northward. During these conditions the magnetosheath interface with the cusp becomes streamlined due to reconnection above the polar cusp. This reconnection provides a smooth surface across which the velocity shear occurs, thus minimizing turbulence in the interaction. The magnetopause current lies closer to the Earth than the flow boundary. This current layer reverses the field direction from nortward to southward in the neighborhood of the distant cusp and is somewhat noisty but not as much as this region becomes when the IMF is southward.

Russell, C. T.↗

DOE OSTI2025

Discovery of an Intrinsic Antiferromagnetic Semiconductor EuSc 2 Te 4 With Magnetism‐Driven Nonlinear Transport

Magnetic topological materials have recently emerged as a promising platform for studying quantum geometry by the nonlinear transport in thin film devices. In this work, an antiferromagnetic (AFM) semiconductor EuSc₂Te₄ as the first bulk crystal that exhibits quantum geometry-driven nonlinear transport is reported. This material crystallizes into an orthorhombic lattice with AFM order below 5.2 K and a bandgap of less than 50 meV. The calculated band structure aligns with the angle-resolved photoemission spectroscopy spectrum. The AFM order preserves combined space-time inversion symmetry but breaks both spatial inversion and time-reversal symmetry, leading to the nonlinear Hall effect (NLHE). Nonlinear Hall voltage measured in bulk crystals appears at zero field, peaks near the spin-flop transition as the field increases, and then diminishes as the spin moments align into a ferromagnetic order. This field dependence, along with the scaling analysis of the nonlinear Hall conductivity, suggests that the NLHE of EuSc₂Te₄ involves contributions from quantum metric, in addition to extrinsic contributions, such as spin scattering and junction effects. Furthermore, this NLHE is found to have the functionality of broadband frequency mixing, indicating its potential applications in electronics. This work reveals a new avenue for studying magnetism-induced nonlinear transport in magnetic materials.

36 MATERIALS SCIENCE↗

NASA NTRS2012

DC and Structured Electric Fields Observed on the C/NOFS Satellite and Their Association with Longitude, Plasma Density, and Solar Activity

Observations of DC electric fields and associated E x B plasma drifts gathered by the Vector Electric Field Investigation (VEFI) on the Air Force Communication/Navigation Outage Forecasting System (C/NOFS) satellite are presented. We show statistical averages of the vector fields and resulting E x B plasma flows for the first three years of operations as a function of season, longitude, local time, and Fl 0.7 conditions. Magnetic field data from the VEFI science magnetometer are used to compute the plasma flows. Although typically displaying eastward and outward-directed fields during the day and westward and downward-directed fields at night, the data from DC electric field detector often reveal variations from this pattern that depend on longitude, solar activity, and plasma density. Clear "wave-4" tidal effects in both electric field components have been detected and will be presented. Zonal plasma drifts show a marked variation with solar activity and may be used as a proxy for neutral winds at night. Evidence for pre-reversal enhancements in the meridional drifts that depend on solar activity is present for some longitudes, and are corroborated by clear evidence in the plasma density data that the spacecraft journeyed below the F-peak during evenings when the rise in the ionosphere is most pronounced. In addition to DC electric fields, the data reveal considerable electric field structures at large scales (approx 100's of km) that are usually confined to the nightside. Although such electric field structures are typically associated with plasma density depletions and structures, what is surprising is the number of cases in which large amplitude, structured DC electric fields are observed without a significant plasma density counterpart structure, including their appearance at times when the ambient plasma density appears relatively quiescent. We investigate the mapping of structured electric fields along magnetic field lines from distant locations and consider tropospheric thunderstorm sources to explain some of the observations. The dependence of the structuring on season and solar activity will be reported and discussed.

Pfaff, Robert↗