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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 1,369 records · Page 76
All sourcesNASA NTRSDOE OSTI
DOE OSTI2023

Nanoscale reshaping of resonant dielectric microstructures by light-driven explosions

Femtosecond-laser-assisted material restructuring employs extreme optical intensities to localize the ablation regions. To overcome the minimum feature size limit set by the wave nature of photons, there is a need for new approaches to tailored material processing at the nanoscale. Here, we report the formation of deeply-subwavelength features in silicon, enabled by localized laser-induced phase explosions in prefabricated silicon resonators. Using short trains of mid-infrared laser pulses, we demonstrate the controllable formation of high aspect ratio (>10:1) nanotrenches as narrow as ~ $λ / 80$. The trench geometry is shown to be scalable with wavelength, and controlled by multiple parameters of the laser pulse train, such as the intensity and polarization of each laser pulse and their total number. Particle-in-cell simulations reveal localized heating of silicon beyond its boiling point and suggest its subsequent phase explosion on the nanoscale commensurate with the experimental data. The observed femtosecond-laser assisted nanostructuring of engineered microstructures (FLANEM) expands the nanofabrication toolbox and opens exciting opportunities for high-throughput optical methods of nanoscale structuring of solid materials.

42 ENGINEERING↗
DOE OSTI2025

Visualizing the Three-Dimensional Arrangement of Hydrogen Atoms in Organic Molecules by Coulomb Explosion Imaging

Structure-sensitive methods based on femtosecond light or electron pulses are now making it possible to measure how molecular structures change during light-induced processes. Despite significant progress, high-fidelity imaging of nuclear positions remains a challenge even for relatively small molecular systems and, notably, regarding the positions of hydrogen atoms. As demonstrated in recent work, X-ray-induced Coulomb explosion imaging (CEI) may overcome this obstacle, as its sensitivity does not depend on the mass of the imaged atoms. The photoinduced ring opening of the heterocyclic molecule 2(5 H )-thiophenone has attracted recent interest. Here, in this work, we show that CEI offers a powerful route to imaging the peripheral H atoms in this molecule and thus, more generally, to tracking detailed nuclear motions (e.g., isomerizations) in organic molecules on ultrafast time scales. Specifically, we record momentum-space Coulomb explosion images that report on the three-dimensional positioning of all nuclei within the molecule, for instance, distinguishing H atoms in C–H bonds that lie within or are directed out of the plane defined by the heavy atoms. The prospect of imaging peripheral H atoms to probe photochemical dynamics is explored by coupling ab initio molecular dynamics with classical Coulomb explosion simulations, thereby differentiating potential photoproduct isomers, including those whose structures primarily differ in the position of the hydrogens.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
NASA NTRS1994

Advanced release technologies program

The objective of the ARTS program was to develop lighter and less expensive spacecraft ordnance and release systems that answer to the requirements of a wide variety of spacecraft applications. These improvements were to be evaluated at the spacecraft system level, as it was determined that there were substantial system-level costs associated with the present ordnance and release subsystems. New, better devices were to be developed, then flight qualified, then integrated into a flight experiment in order to prove the reliability required for their subsequent use on high-reliability spacecraft. The secondary goal of the program was to quantify the system-level benefits of these new subsystems based upon the development program results. Three non-explosive release mechanisms and one laser-diode-based ordnance system were qualified under the program. The release devices being developed were required to release high preloads because it is easier to scale down a release mechanism than to scale it up. The laser initiator developed was required to be a direct replacement for NASA Standard Initiators, since these are the most common initiator in use presently. The program began in October, 1991, with completion of the flight experiment scheduled for February, 1994. This paper provides an overview of the ARTS program, discusses the benefits of using the ARTS components, introduces the new components, compares them with conventional systems and each other, and provides recommendations on how best to implement them.

Purdy, Bill↗
DOE OSTI2020

The Young and Nearby Normal Type Ia Supernova 2018gv: UV-optical Observations and the Earliest Spectropolarimetry

The nondetection of companion stars in SN Ia progenitor systems lends support to the notion of double-degenerate systems and explosions triggered by the merging of two white dwarfs. This very asymmetric process should lead to a conspicuous polarimetric signature. By contrast, observations consistently find very low continuum polarization as the signatures from the explosion process largely dominate over the pre-explosion configuration within several days. Critical information about the interaction of the ejecta with a companion and any circumstellar matter is encoded in the early polarization spectra. In this study, we obtain spectropolarimetry of SN 2018gv with the ESO Very Large Telescope at -13.6 days relative to the B-band maximum light, or ~5 days after the estimated explosion—the earliest spectropolarimetric observations to date of any SN Ia. These early observations still show a low continuum polarization (lesssim0.2%) and moderate line polarization (0.30% ± 0.04% for the prominent Si ii λ6355 feature and 0.85% ± 0.04% for the high-velocity Ca component). The high degree of spherical symmetry implied by the low-line and continuum polarization at this early epoch is consistent with explosion models of delayed detonations and is inconsistent with the merger-induced explosion scenario. Finally, the dense UV and optical photometry and optical spectroscopy within the first ~100 days after the maximum light indicate that SN 2018gv is a normal SN Ia with similar spectrophotometric behavior to SN 2011fe.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2015

iPTF14yb: The First Discovery of a Gamma-Ray Burst Afterglow Independent of a High-Energy Trigger

We report here the discovery by the Intermediate Palomar Transient Factory (iPTF) of iPTF14yb, a luminous (Msub>r ≈ ₋27.8 mag), cosmological (redshift 1.9733), rapidly fading optical transient. We demonstrate, based on probabilistic arguments and a comparison with the broader population, that iPTF14yb is the optical afterglow of the long-duration gamma-ray burst GRB140226A. This marks the rst unambiguous discovery of a GRB afterglow prior to (and thus entirely independent of) an associated high-energy trigger. We estimate the rate of iPTF14yb-like sources (i.e., cosmologically dis- tant relativistic explosions) based on iPTF observations, inferring an all-sky value of $R_{rel}$ = 610yr -1 (68% con dence interval of 110{2000 yr -1 ). Our derived rate is consistent (within the large uncer- tainty) with the all-sky rate of on-axis GRBs derived by the Swift satellite. Finally, we brie y discuss the implications of the nondetection to date of bona de \orphan" afterglows (i.e., those lacking de- tectable high-energy emission) on GRB beaming and the degree of baryon loading in these relativistic jets.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2014

High pressure-temperature polymorphism of 1,1-diamino-2,2-dinitroethylene

Here, 1,1-diamino-2,2-dinitroethylene (FOX-7) is a low sensitivity energetic material with performance comparable to commonly used secondary explosives such as RDX and HMX. At ambient pressure, FOX-7 exhibits complex polymorphism with at least three structurally distinct phases (α, β, and γ). In this study, we have investigated the high pressure-temperature stability of FOX-7 polymorphs using synchrotron mid-infrared (MIR) spectroscopy. At ambient pressure, our MIR spectra and corresponding differential scanning calorimetry (DSC) measurements confirmed the known α → β (~110 °C) and β → γ (~160 °C) structural phase transitions; as well as, indicated an additional transition γ → δ (~210 °C), with the δ phase being stable up to ~251 degree C prior to decomposition. In situ MIR spectra obtained during isobaric heating at 0.9 GPa, revealed a potential α → β transition that could occur as early as 180 degree C, while β → β+δ phase transition shifted to ~300 °C with suppression of γ phase. Decomposition was observed slightly above 325 °C at 0.9 GPa..

36 MATERIALS SCIENCE↗
DOE OSTI2015

Constraining absolute neutrino masses via detection of galactic supernova neutrinos at JUNO

A high-statistics measurement of the neutrinos from a galactic core-collapse supernova is extremely important for understanding the explosion mechanism, and studying the intrinsic properties of neutrinos themselves. In this paper, we explore the possibility to constrain the absolute scale of neutrino masses m{sub ν} via the detection of galactic supernova neutrinos at the Jiangmen Underground Neutrino Observatory (JUNO) with a 20 kiloton liquid-scintillator detector. In assumption of a nearly-degenerate neutrino mass spectrum and a normal mass ordering, the upper bound on the absolute neutrino mass is found to be m{sub ν}<(0.83±0.24) eV at the 95% confidence level for a typical galactic supernova at a distance of 10 kpc, where the mean value and standard deviation are shown to account for statistical fluctuations. For comparison, we find that the bound in the Super-Kamiokande experiment is m{sub ν}<(0.94±0.28) eV at the same confidence level. However, the upper bound will be relaxed when the model parameters characterizing the time structure of supernova neutrino fluxes are not exactly known, and when the neutrino mass ordering is inverted.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
NASA NTRS1986

Signatures of current loop coalescence in solar flares

The nonlinear coalescence instability of current carrying solar loops can explain many of the characteristics of the solar flares such as their impulsive nature, heating and high energy particle acceleration, amplitude oscillations of electromagnetic emission as well as the characteristics of 2-D microwave images obtained during a solar flare. The physical characteristics of the explosive coalescence of currents are presented in detail through computer simulation and theory. Canonical characteristics of the explosive coalescence are: (1) a large amount of impulsive increase of kinetic energies of electrons and ions; (2) simultaneous heating and acceleration of electrons and ions in high and low energy spectra; (3) ensuing quasi-periodic amplitude oscillations in fields and particle quantities; and (4) the double peak (or triple peak) structure in these profiles, participate in the coalescence process, yielding varieties of phenomena.

Sakai, J.↗
DOE OSTI2019

Fallout melt debris and aerodynamically-shaped glasses in beach sands of Hiroshima Bay, Japan

An intricate association of millimeter-sized, aerodynamically-shaped debris, including glass spherules, glass filaments, and composite-fused melt particles was recovered from beach sands on the shores of the Motoujina Peninsula in Hiroshima Bay, Japan. Based on optical microscopy, this debris comprises six morphological groups ranging from clear glasses to rubber-like constituents. Scanning electron microscopy and synchrotron X-ray microdiffraction revealed dominant aluminum, silicon and calcium (Al-Si-Ca) elemental composition with some iron, mainly in glass, associated with precipitates of mullite and anorthite microcrystals, hematite dendrites and iron-chromium globules, indicative of original temperature conditions >1800 °C. Aerodynamically-shaped fallout debris, including glass spherules described in this study, are generally produced by single high-energy catastrophic events, such as an extraterrestrial body impacting Earth or a nuclear explosion. Our work interprets the large volumes of fallout debris generated under extreme temperature conditions as products of the Hiroshima August 6th, 1945 atomic bomb aerial detonation. The chemical composition of the melt debris provides clues to their origin, particularly with regard to city building materials. This study is the first published record and description of fallout resulting from the destruction of an urban environment by atomic bombing.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗
DOE OSTI2020

Deacetylation and Mechanical Refining (DMR) and Deacetylation and Dilute Acid (DDA) Pretreatment of Corn Stover, Switchgrass, and a 50/50 Corn Stover/Switchgrass Blend

The most economical feedstock available to future lignocellulosic biorefineries may be a feedstock blend. Corn stover, switchgrass, and a 50:50 blend of corn stover and switchgrass were subjected to three different dilute alkali deacetylation conditions in a 90 L reactor prior to either mechanical refining (DMR) in a disc refiner followed by a Szego mill or dilute acid pretreatment (DDA) at five different conditions in a 4 L batch steam explosion reactor. The forty-five DDA and nine DMR slurries were subjected to high solids enzymatic hydrolysis at an enzyme loading of 15 mg protein per gram cellulose using Novozymes Cellic CTec3 (DDA) or a 4:1 mix of Novozymes Cellic CTec3:HTec 3 (DMR). The highest glucose yield was achieved using DMR processed corn stover from the high severity deacetylation condition (92 °C and 100 kg NaOH/ODMT) at 95.9% ± 0.8%, while the greatest monomeric glucose yields for switchgrass were between 75% to 80%. The glucose yields from saccharification of the 50:50 corn stover/switchgrass blend was approximately the average of the two individual feedstocks for both DDA and DMR processes. Statistical analysis showed that for a given feedstock type dilute alkali deacetylation severity had a significant impact (p < 0.05) on enzymatic hydrolysis yields, and for a given deacetylation severity the feedstock type had a significant effect on glucose conversion with the addition of switchgrass resulting in lower glucose yields. A blending strategy to maximize enzymatic hydrolysis sugar yields while reducing carbohydrate solubilization during the alkaline treatment step was proposed that allows deacetylation of feedstocks with different recalcitrance at optimal conditions for that feedstock, then blending prior to enzymatic hydrolysis.

BIOMASS FUELS,INORGANIC, ORGANIC, PHYSICAL, AND AN↗
DOE OSTI2013

ULTRA-STRIPPED TYPE Ic SUPERNOVAE FROM CLOSE BINARY EVOLUTION

Recent discoveries of weak and fast optical transients raise the question of their origin. We investigate the minimum ejecta mass associated with core-collapse supernovae (SNe) of Type Ic. We show that mass transfer from a helium star to a compact companion can produce an ultra-stripped core which undergoes iron core collapse and leads to an extremely fast and faint SN Ic. In this Letter, a detailed example is presented in which the pre-SN stellar mass is barely above the Chandrasekhar limit, resulting in the ejection of only ∼0.05-0.20 M {sub ☉} of material and the formation of a low-mass neutron star (NS). We compute synthetic light curves of this case and demonstrate that SN 2005ek could be explained by our model. We estimate that the fraction of such ultra-stripped to all SNe could be as high as 10{sup –3}-10{sup –2}. Finally, we argue that the second explosion in some double NS systems (for example, the double pulsar PSR J0737–3039B) was likely associated with an ultra-stripped SN Ic.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2021

Tensorized Feature Spaces for Feature Explosion

In this paper 1 1 This manuscript has been authored by UT-Battelle, LLC under Contract No. DE-AC05-000R22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan) This research used resources of the Oak Ridge Leadership Computing Facility, which is a DOE Office of Science User Facility supported under Contract DE-AC05-000R22725., we present a novel framework that uses tensor factorization to generate richer feature spaces for pixel classification in hyperspectral images. In particular, we assess the performance of different tensor rank decomposition methods as compared to the traditional kernel-based approaches for the hyperspectral image classification problem. We propose Orion, which takes as input a hyperspectral image tensor and a rank and outputs an enhanced feature space from the factor matrices of the decomposed tensor. Our method is a feature explosion technique that inherently maps low dimensional input space in $\mathbb{R}^{K}$ to high dimensional space in $\mathbb{R}^{R}$ , where $R\gg K$ , say in the order of 1000x, like a kernel. We show how the proposed method exploits the multi-linear structure of hyperspectral three dimensional tensor. We demonstrate the effectiveness of our method with experiments on three publicly available hyperspectral datasets with labeled pixels and compare their classification performance against traditional linear and non-linear supervised learning methods such as SVM with Linear, Polynomial, RBF kernels, and the Multi-Layer Perceptron model. Finally, we explore the relationship between the rank of the tensor decomposition and the classification accuracy using several hyperspectral datasets with ground truth.

Pasricha, Ravdeep Singh↗
DOE OSTI2013

Optical Manipulation of Vesicles for Optofluidic Applications

In this report, we review our recent results in the optical micromanipulation of vesicles. Traditionally, vesicle manipulation has been possible by employing photon momentum and optical trapping, giving rise to unique observations of vesicle shape changes and soft matter mechanics. Contrary to these attempts, we employ photon energy rather than momentum, by sensitizing vesicles with an oxidizing moiety. The later converts incident photons to reactive oxygen species, which in turn attack and compromise the stability of the vesicle membrane. Both coherent and incoherent radiation was employed. Polymersome re-organization into smaller diameter vesicles was possible by focusing the excitation beam in the vicinity of the polymersomes. Extended vesicle illumination with a collimated beam lead to their complete destabilization and micelle formation. Single particle analysis revealed that payload release takes place within seconds of illumination in an explosive burst. We will discuss the destabilization and payload release kinetics, as revealed by high resolution microscopy at the single particle level, as well as potential applications in single cell biomodulation.

Environmental Molecular Sciences Laboratory↗
DOE OSTI2017

Magnetically-Driven Convergent Instability Growth platform on Z.

Hydrodynamic instability growth is a fundamentally limiting process in many applications. In High Energy Density Physics (HEDP) systems such as inertial confinement fusion implosions and stellar explosions, hydro instabilities can dominate the evolution of the object and largely determine the final state achievable. Of particular interest is the process by which instabilities cause perturbations at a density or material interface to grow nonlinearly, introducing vorticity and eventually causing the two species to mix across the interface. Although quantifying instabilities has been the subject of many investigations in planar geometry, few have been done in converging geometry. During FY17, the team executed six convergent geometry instability experiments. Based on earlier results, the platform was redesigned and improved with respect to load centering at installation making the installation reproducible and development of a new 7.2 keV, Co He-a backlighter system to better penetrate the liner. Together, the improvements yielded significantly improved experimental results. The results in FY17 demonstrate the viability of using experiments on Z to quantify instability growth in cylindrically convergent geometry. Going forward, we will continue the partnership with staff and management at LANL to analyze the past experiments, compare to hydrodynamics growth models, and design future experiments.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
NASA NTRS1991

Large-scale gas dynamical processes affecting the origin and evolution of gaseous galactic halos

Observations of galactic halo gas are consistent with an interpretation in terms of the galactic fountain model in which supernova heated gas in the galactic disk escapes into the halo, radiatively cools and forms clouds which fall back to the disk. The results of a new study of several large-scale gas dynamical effects which are expected to occur in such a model for the origin and evolution of galactic halo gas will be summarized, including the following: (1) nonequilibrium absorption line and emission spectrum diagnostics for radiatively cooling halo gas in our own galaxy, as well the implications of such absorption line diagnostics for the origin of quasar absorption lines in galactic halo clouds of high redshift galaxies; (2) numerical MHD simulations and analytical analysis of large-scale explosions ad superbubbles in the galactic disk and halo; (3) numerical MHD simulations of halo cloud formation by thermal instability, with and without magnetic field; and (4) the effect of the galactic fountain on the galactic dynamo.

Shapiro, Paul R.↗
NASA NTRS1993

Explosions of small Spacewatch objects in the Earth's atmosphere

It is shown here that explosions due to Spacewatch objects with diameters less than 50 m typically occur too high in the atmosphere to cause substantial surface damage. Exclusive of relatively rare iron objects, no comet or asteroid with an energy below about 2 megatons threatens the Earth's surface. The high flux of small Earth-crossing objects identified by Spacewatch therefore does not imply a greater terrestrial hazard.

Chyba, Christopher F.↗
NASA NTRS1997

Fuel Line Based Acoustic Flame-Out Detection System

An acoustic flame-out detection system that renders a large high pressure combustor safe in the event of a flame-out and possible explosive reignition. A dynamic pressure transducer is placed in the fuel and detects the stabilizing fuel pressure oscillations, caused by the combustion process. An electric circuit converts the signal from the combustion vortices, and transmitted to the fuel flow to a series of pulses. A missing pulse detector counts the pulses and continuously resets itself. If three consecutive pulses are missing, the circuit closes the fuel valve. With fuel denied the combustor is shut down or restarted under controlled conditions.

Puster, Richard L.↗
NASA NTRS2001

Quantifying and Improving International Space Station Survivability Following Orbital Debris Penetration

The increase of the orbital debris environment in low-earth orbit has prompted NASA to develop analytical tools for quantifying and lowering the likelihood of crew loss following orbital debris penetration of the International Space Station (ISS). NASA uses the Manned Spacecraft and Crew Survivability (MSCSurv) computer program to simulate the events that may cause crew loss following orbital debris penetration of ISS manned modules, including: (1) critical cracking (explosive decompression) of the module; (2) critical external equipment penetration (such as hydrazine and high pressure tanks); (3) critical internal system penetration (guidance, control, and other vital components); (4) hazardous payload penetration (furnaces, pressure bottles, and toxic substances); (5) crew injury (from fragments, overpressure, light flash, and temperature rise); (6) hypoxia from loss of cabin pressure; and (7) thrust from module hole causing high angular velocity (occurring only when key Guidance, Navigation, and Control (GN&C) equipment is damaged) and, thus, preventing safe escape vehicle (EV) departure. MSCSurv is also capable of quantifying the 'end effects' of orbital debris penetration, such as the likelihood of crew escape, the probability of each module depressurizing, and late loss of station control. By quantifying these effects (and their associated uncertainties), NASA is able to improve the likelihood of crew survivability following orbital debris penetration due to improved crew operations and internal designs.

Williamsen, Joel↗