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DOE OSTI2023

TRACER-Vertical Profile of Aerosol in Convective System (TRACER-VPACS) Field Campaign Report

We investigated physicochemical properties of aerosol at different altitudes during the U.S. Department of Energy (DOE)’s Atmospheric Radiation Measurement (ARM) user facility Tracking Aerosol Convection Interactions Experiment (TRACER). We used ARM’s tethered balloon system (TBS) and multi-modal offline analysis techniques available at DOE’s Environmental Molecular Sciences Laboratory (EMSL) at Pacific Northwest National Laboratory (PNNL) and at the Advanced Light Source (ALS) at the Lawrence Berkley National Laboratory (LBNL). The main scientific aim of this project was to understand the influence of the vertical profile of aerosol composition on the properties of deep convective clouds. The effect of aerosol properties on convective activity is still poorly understood and debated. For example, previous studies suggested that higher concentration of hygroscopic aerosol may lead to lower collection efficiency and eventually delay in onset of precipitation and total amount of precipitation. However, some observations suggested that increased aerosol concentration may result in vigorous convection and a higher amount of precipitation. In addition, the radiative forcing of the ambient aerosol is strongly influenced by the vertical distribution of aerosols and their chemical composition, and not well constrained in climate models. The estimation of the indirect effect of aerosol also has a significant uncertainty due to the spatial variation of the aerosol, especially at the cloud base. Detailed size-resolved chemical composition studies of aerosol and their microphysical properties, along with in situ measurements from ARM’s mobile facilities, help to improve our understanding of the role of aerosol in deep convective cloud formation over a broad range of environmental thermodynamic and aerosol conditions.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2026

Examining the Impacts of Microphysical-Dynamical Feedbacks on Convective Clouds in Different Aerosol Environments Using Enhanced Observational and Modeling Strategies

This project investigated how microphysical–dynamical feedbacks influence deep convective clouds across a range of aerosol conditions, storm lifecycles, and meteorological regimes, and how these sensitivities depend on the modeling framework used to represent convection and microphysics. Using the Aerosol, Cloud, Precipitation, and Climate (ACPC) Working Group model intercomparison simulations of isolated deep convection in the Houston region, we found a robust warm-phase aerosol response in most cloud-resolving models. Increased aerosol loading tended to suppress warm-rain production, increase cloud water, and reduce surface rainfall and near-surface evaporation. These impacts were typically strongest early in the convective lifecycle, with the largest aerosol-driven differences occurring during the first half of storm evolution. The ice-phase response, on the other hand, varied widely across modeling frameworks, and differed in sign, timing, and vertical structure. Ice microphysical pathways and parameterizations are therefore leading sources of uncertainty in aerosol–deep convection interactions. Theoretical analyses further suggested that aerosol-driven invigoration through cold-phase processes was much weaker than previously hypothesized for cold-based storms, and in warm-based storms could even reduce updraft strength. These results imply that any invigoration signal is more likely linked to warm-phase processes and peaks early in storm development.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS2001

Did the Eruption of the Mt. Pinatubo Volcano Affect Cirrus Properties?

Some observations suggest that the volcanic aerosols produced by the Mt. Pinatubo eruption may have altered cirrus properties. We look for evidence that such modification of cirrus is extensive enough to be climatically significant by comparing three satellite-based cirrus datasets produced by the ISCCP (International Satellite Cloud Climatology Project) analysis, the 'split-window' analysis, and 3I analysis. Since the former two have not been compared in detail before, we conduct such a comparison here. When applied to AVHRR (Advanced Very High Resolution Radiometer) data, both the ISCCP and split-window analyses identify about 0.2 - 0.3 cirrus cloud amount in tropical latitudes; however, there are detailed differences of classification for about half of these clouds. The discrepancies are attributed to the simplified assumptions made by both methods. The latter two datasets are derived from infrared radiances, so they are much less sensitive to volcanic aerosols than the ISCCP analysis. After the Mt. Pinatubo eruption, the ISCCP results indicate a dramatic decrease of thin cirrus (cloud top pressure less than 440 mb and visible optical thickness less than 1.3) over ocean, accompanied by a comparable increase of altocumulus and cumulus clouds; over land, there are no significant changes. In contrast, results from the split-window and 3I analyses show little change in thin cirrus amount over either ocean or land that is associated with the volcanic eruption. The ISCCP results can, therefore, be understood as a misclassification of thin cirrus because the additional reflected sunlight by the volcanic aerosol makes the cirrus clouds appear to be optically thicker. Examination of the split-window signature and the infrared emissivities from 3I show no significant change in infrared emissivity (or optical thickness). These results indicate that the Mt. Pinatubo volcanic aerosol did not have a significant systematic effect on tropical cirrus properties, but rather produced only temporary, local effects. Hence, these results indicate that there was no significant climate feedback produced by aerosol-cirrus-radiative interactions.

Luo, Zhengzhao↗

DOE OSTI2011

Effects of ice number concentration on dynamics of a shallow mixed-phase stratiform cloud

Previous modeling studies have shown a high sensitivity of simulated properties of mixed-phase clouds to ice number concentration, Ni, with many models losing their ability to maintain the liquid phase as Ni increases. Although models differ widely at what Ni the mixed-phase cloud becomes unstable, the transition from a mixed-phase to an ice only cloud in many cases occurs over a narrow range of ice concentration. To gain better understanding of this non-linear model behavior, in this study, we analyze simulations of a mixed-phase stratiform Artic cloud observed on 26 April 2008 during recent Indirect and Semi-Direct Aerosol Campaign (ISDAC). The BASE simulation, in which Ni is constrained to match the measured value, produces a long-lived cloud in a quasi steady state similar to that observed. The simulation without the ice (NO_ICE) produces a comparable but slightly thicker cloud because more moisture is kept in the mixed layer due to lack of precipitation. When Ni is quadrupled relative to BASE (HI_ICE), the cloud starts loosing liquid water almost immediately and the liquid water path is reduced by half in less than two hours. The changes in liquid water are accompanied by corresponding reduction in the radiative cooling of the layer and a slow down in the vertical mixing, confirming the important role of interactions among microphysics, radiation and dynamics in this type of clouds. Deviations of BASE and HI_ICE from NO_ICE are used to explore the linearity of the model response to variation in Ni. It is shown that at early stages, changes in liquid and ice water as well as in radiative cooling/heating rates are proportional to the Ni change, while changes in the vertical buoyancy flux are qualitatively different in HI_ICE compared to BASE. Thus, while the positive feedback between the liquid water path and radiative cooling of the cloud layer is essential for glaciation of the cloud at higher Ni, the non-linear (with respect to Ni) reduction in positive buoyancy flux within and below the liquid cloud layer emerges as the process that influences the initial response of the mixed layer dynamics to the appearance of ice and subsequently determines the sustainability of liquid water in the cloud in this case.

58 GEOSCIENCES↗

NASA NTRS1991

The Earth Observing System

The Earth Observing System (EOS), the centerpiece of NASA's Mission to Planet Earth, is to study the interactions of the atmosphere, land, oceans, and living organisms, using the perspective of space to observe the earth as a global environmental system. To better understand the role of clouds in global change, EOS will measure incoming and emitted radiation at the top of the atmosphere. Then, to study characteristics of the atmosphere that influence radiation transfer between the top of the atmosphere and the surface, EOS wil observe clouds, water vapor and cloud water, aerosols, temperature and humidity, and directional effects. To elucidate the role of anthropogenic greenhouse gas and terrestrial and marine plants as a source or sink for carbon, EOS will observe the biological productivity of lands and oceans. EOS will also study surface properties that affect biological productivity at high resolution spatially and spectrally.

Wilson, Stan↗

NASA NTRSDate not supplied

Study the Vertical Structure and Transportation of the Extreme African Dust Storms using MERRA-2 Data

The Modern-Era Retrospective Analysis for Research and Application, Version 2 (MERRA-2) provides the first long-term global reanalysis to assimilate space-based observations of aerosols and represents their interactions with other physical processes in the climate system. In this study, we have examined the variations of atmospheric aerosols for the last 20 years since 2002 using the sub-daily MERRA-2 data and found seven extreme African dust storms that were transported westward across the Atlantic Ocean from the Sahara, crossing 70o-80oW. In particular, the well-known ‘Godzilla’ dust storm occurred in June 2020, and its dust cloud, with the highest-on-record aerosol optical depths, was transported toward the Americas. This storm greatly degraded air quality over large areas of the Caribbean Basin and the United States. The air quality index reached unhealthy levels for sensitive groups in more than ten U.S. states. In our study, the vertical structure and transport characteristics of the dust layers during this extreme dust event are investigated. The geopotential height and temperature were found anomalously low (around 600 hPa) over the Atlantic Ocean off northwest Africa before the June 2020 dust storm. This anomalous circulation pattern was persistent for more than 12 days starting from around May 30, breaking the regular easterly waves that transport dust from the Sahara Desert to the west. To verify the data quality, daily MERRA-2 PM2.5 data were calculated and compared with PM2.5 observations from the U.S. Environmental Protection Agency (EPA) at several selected ground stations in Florida. We provide this case study to illustrate how to effectively use various MERRA-2 data services at Goddard Earth Sciences Data and Information Services Center (GES DISC) where MERRA-2 data are archived, hoping to help data users in exploring their own topics of interest using data services at GES DISC.

data management, reanalysis↗

DOE OSTI2025

Sea spray aerosol production flux retrieval based on Doppler lidar measurements

Supermicron sea spray aerosols (SSA) play a crucial role in stratocumulus cloud microphysics and drizzle formation. However, our understanding of SSA's spatiotemporal distribution, production mechanisms, and fluxes in the marine boundary layer remains limited. This study introduces a novel approach to determine supermicron SSA production flux and number concentration at various heights above the ocean surface. Our method leverages Doppler lidar data, specifically attenuated backscatter and vertical velocity, collected at a 105 m range gate during the Eastern Pacific Clouds and Aerosols for Precipitation Experiment (EPCAPE) at Scripps Pier, La Jolla, California. To focus on nascent SSA, we analyzed data from periods with wind directions between 225° and 315° and wind speeds exceeding 4 m s −1 . Cloud and precipitation events were excluded using relative humidity, backscatter thresholds, and 2D Video Disdrometer observations. Results show that calculated supermicron SSA number concentrations at 105 m ranged from 0.26 to 2.93 cm −3 for surface wind speeds between 4 and 6 ms −1 . When exceeding the method's Limit of Detection, estimated production fluxes ranged from 0.20 to 1.53 cm −2 s −1 . This methodology has potential for application in various oceanic locations, likely enhancing our understanding of SSA's role in atmospheric processes and climate interactions.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS1978

Rocket exhaust ground cloud/atmospheric interactions

An attempt to identify and minimize the uncertainties and potential inaccuracies of the NASA Multilayer Diffusion Model (MDM) is performed using data from selected Titan 3 launches. The study is based on detailed parametric calculations using the MDM code and a comparative study of several other diffusion models, the NASA measurements, and the MDM. The results are discussed and evaluated. In addition, the physical/chemical processes taking place during the rocket cloud rise are analyzed. The exhaust properties and the deluge water effects are evaluated. A time-dependent model for two aerosol coagulations is developed and documented. Calculations using this model for dry deposition during cloud rise are made. A simple model for calculating physical properties such as temperature and air mass entrainment during cloud rise is also developed and incorporated with the aerosol model.

Hwang, B.↗

DOE OSTI2024

Enhanced light absorption for solid-state brown carbon from wildfires due to organic and water coatings

Abstract Wildfires emit solid-state strongly absorptive brown carbon (solid S-BrC, commonly known as tar ball), critical to Earth’s radiation budget and climate, but their highly variable light absorption properties are typically not accounted for in climate models. Here, we show that from a Pacific Northwest wildfire, over 90% of particles are solid S-BrC with a mean refractive index of 1.49 + 0.056 i at 550 nm. Model sensitivity studies show refractive index variation can cause a ~200% difference in regional absorption aerosol optical depth. We show that ~50% of solid S-BrC particles from this sample uptake water above 97% relative humidity. We hypothesize these results from a hygroscopic organic coating, potentially facilitating solid S-BrC as nuclei for cloud droplets. This water uptake doubles absorption at 550 nm and the organic coating on solid S-BrC can lead to even higher absorption enhancements than water. Incorporating solid S-BrC and water interactions should improve Earth’s radiation budget predictions.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRSDate not supplied

Surface-Enhanced Raman Spectroscopy (SERS) for Venus Atmospheric Characterization and Trace Organics Identification

The chemical composition of Venus’ clouds has attracted considerable attention since the first atmospheric probes entered the planet in the early 1980s. We know from these early studies that cloud aerosols consist of micron and submicron droplets of sulfuric acid (~85%) and water (~15%), but outstanding questions still exist regarding their trace chemical composition, especially the identity of the unknown UV absorber(s) and the possible presence of organic material (Spacek & Benner, 2021). Veritas and DaVinci will launch at the end of the decade to advance our understanding of Venus’ surface and atmosphere, however these missions are not designed to sample and analyze cloud aerosols at trace levels. Raman spectroscopy is an ideal candidate for characterizing aerosols and has a track record in studies of Earth’s atmosphere. Raman provides broad chemical screening of organic and inorganic molecules within seconds, and Raman instrumentation can be miniaturized to meet the stringent size, weight, and power (SWaP) constraints of an atmospheric probe while retaining sensitivity and specificity that allow spectral fingerprinting of compounds and functional groups. Raman alone is insufficient to characterize trace constituents however, as limits of detection are typically in the 10s to 100s of ppm at best for planetary Raman spectrometers. Surface-Enhanced Raman Spectroscopy (SERS), a method that utilizes nanoscale materials interacting with a sample to enhance weak Raman signals by orders of magnitude when probed by a laser, has the potential to drastically improve the sensitivity of a Raman instrument while adding little-to-no SWaP nor complexity to a scientific payload. We aim to de-risk SERS technology for rapid infusion in future planetary science missions by developing custom SERS substrates tailored towards Venus atmospheric exploration. We have developed SERS substrates consisting of nanotextured silver films and tested them on potential Venus-relevant organic compounds, with preliminary results indicating sub-ppm sensitivity. Additionally, we have planned tests to investigate durability, longevity, and other key characteristics that impact SERS substrate performance to prepare SERS technology for flight.

Venus↗

NASA NTRS2005

Algorithm Science to Operations for the National Polar-orbiting Operational Environmental Satellite System (NPOESS) Visible/Infrared Imager/Radiometer Suite (VIIRS)

The VIIRS sensor provides measurements for 22 Environmental Data Records (EDRs) addressing the atmosphere, ocean surface temperature, ocean color, land parameters, aerosols, imaging for clouds and ice, and more. That is, the VIIRS collects visible and infrared radiometric data of the Earth's atmosphere, ocean, and land surfaces. Data types include atmospheric, clouds, Earth radiation budget, land/water and sea surface temperature, ocean color, and low light imagery. This wide scope of measurements calls for the preparation of a multiplicity of Algorithm Theoretical Basis Documents (ATBDs), and, additionally, for intermediate products such as cloud mask, et al. Furthermore, the VIIRS interacts with three or more other sensors. This paper addresses selected and crucial elements of the process being used to convert and test an immense volume of a maturing and changing science code to the initial operational source code in preparation for launch of NPP. The integrity of the original science code is maintained and enhanced via baseline comparisons when re-hosted, in addition to multiple planned code performance reviews.

NPOESS (NATIONAL POLAR-ORBITING OPERATIONAL ENVIRO↗

NASA NTRS2014

Sensitivity of Cirrus Properties to Ice Nuclei Abundance

The relative importance of heterogeneous and homogeneous ice nucleation for cirrus formation remains an active area of debate in the cloud physics community. From a theoretical perspective, a number of modeling studies have investigated the sensitivity of ice number concentration to the nucleation mechanism and the abundance of ice nuclei. However, these studies typically only addressed ice concentration immediately after ice nucleation. Recent modeling work has shown that the high ice concentrations produced by homogeneous freezing may not persist very long, which is consistent with the low frequency of occurrence of high ice concentrations indicated by cirrus measurements. Here, I use idealized simulations to investigate the impact of ice nucleation mechanism and ice nuclei abundance on the full lifecycle of cirrus clouds. The primary modeling framework used includes different modes of ice nucleation, deposition growth/sublimation, aggregation, sedimentation, and radiation. A limited number of cloud-resolving simulations that treat radiation/dynamics interactions will also been presented. I will show that for typical synoptic situations with mesoscale waves present, the time-averaged cirrus ice crystal size distributions and bulk cloud properties are less sensitive to ice nucleation processes than might be expected from the earlier simple ice nucleation calculations. I will evaluate the magnitude of the ice nuclei impact on cirrus for a range of temperatures and mesoscale wave specifications, and I will discuss the implications for cirrus aerosol indirect effects in general.

Nuclei↗

DOE OSTI2018

Tropospheric Ozone Variability during LASIC Field Campaign Report

Part of the U.S. Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) Climate Research Facility’s Layered Atlantic Smoke Interactions with Clouds (LASIC) field campaign. The primary goal of the measurements was to improve understanding of the evolution of the wave-one ozone maximum. The key objectives were Measure the variability of ozone mixing ratios associated with the African Easterly Jet (AEJ) on sub-synoptic time scales in which meteorology may play a role. In concert with weekly measurements from the Southern Hemisphere Additional Ozonesondes (SHADOZ) network, determine the vertical distribution of ozone and aerosols at Ascension Island. Determine from lidar measurements the locations of the biomass burning (BB layer) and its relationship to ozone mixing ratios. Determine the relative abundance of ozone in the BB layer relative to ozone mixing ratios at higher altitudes that may be associated with lightning nitrogen oxides (LNOx). Determine sources of high or low ozone mixing ratios through back trajectory models at Ascension Island.

LASIC field campaign, Ascension Island, biomass bu↗

DOE OSTI2025

Using stable isotopes in water vapor to study the interdependence of clouds, atmospheric aerosols, and precipitation processes

This project deployed water vapor isotope measurements at the La Porte, Texas TRACER site during June-September 2022 to quantify mixing processes in sea breeze circulations. Using a Picarro L2130 analyzer, we collected high-frequency measurements of δD and δ¹⁸O that revealed how marine and terrestrial air masses mix during 46 identified sea breeze events. The isotopic tracers showed systematic changes during frontal passages, with composite analyses demonstrating vertical mixing between cool marine air and warmer air aloft. We developed a transilient matrix model that explicitly treats non-local mixing and isotopic fractionation to interpret the observations. The work directly supports TRACER's core objective of understanding convective initiation by constraining the vertical transport of water vapor and its interaction with Houston's aerosol-laden urban plume during sea breeze-convection coupling.

58 GEOSCIENCES↗

NASA NTRS2001

Reaction Mechanisms and Particle Interaction in Burning Two-Phase Systems

The main objective of this research is to understand the mechanisms by which particle interactions affect ignition and combustion in the two-phase systems. Combustion of metal aerosols representing the two-phase systems is carried out in the microgravity environment enabling one to avoid the buoyant flows that mask the particle motion due to the particle-particle interaction effects. In addition, relatively large, e.g., 100 micron diameter particles can be used, that remain aerosolized (i.e., do not fall down as they would at normal gravity) so that their behavior ahead, behind, and within the propagating flame can be resolved optically. An experimental apparatus exploiting this approach has been designed for the 2.2-s drop tower microgravity experiments. A typical experiment includes fluidizing metal particles under microgravity in an acoustic field, turning off the acoustic exciter, and igniting the created aerosol at a constant pressure using a hot wire igniter. The flame propagation and details of the individual particle combustion and particle interactions are studied using high-speed movie and video cameras coupled with microscope lenses to resolve individual particles. Recorded flame images are digitized and various image processing techniques including flame position tracking, color separation, and pixel by pixel image comparisons are employed to understand the processes occurring in the burning aerosols. Condensed combustion products are collected after each experiment for the phase, composition, and morphology analyses. New experiments described in this paper address combustion of Ti and Al particle clouds in air and combustion of Mg particle clouds in CO2. In addition, microgravity combustion experiments have been conducted with the particles of the newly produced Al-Mg mechanical alloys aerosolized in air.

Dreizin, Edward L.↗

NASA NTRS2014

Far-Reaching Impacts of African Dust- A Calipso Perspective

African dust can transport across the tropical Atlantic and reach the Amazon basin, exerting far-reaching impacts on climate in downwind regions. The transported dust influences the surface-atmosphere interactions and cloud and precipitation processes through perturbing the surface radiative budget and atmospheric radiative heating and acting as cloud condensation nuclei and ice nuclei. Dust also influences biogeochemical cycle and climate through providing nutrients vital to the productivity of ocean biomass and Amazon forests. Assessing these climate impacts relies on an accurate quantification of dust transport and deposition. Currently model simulations show extremely large diversity, which calls for a need of observational constraints. Kaufman et al. (2005) estimated from MODIS aerosol measurements that about 144 Tg of dust is deposited into the tropical Atlantic and 50 Tg of dust into the Amazon in 2001. This estimated dust import to Amazon is a factor of 3-4 higher than other observations and models. However, several studies have argued that the oversimplified characterization of dust vertical profile in the study would have introduced large uncertainty and very likely a high bias. In this study we quantify the trans-Atlantic dust transport and deposition by using 7 years (2007-2013) observations from CALIPSO lidar. CALIPSO acquires high-resolution aerosol extinction and depolarization profiles in both cloud-free and above-cloud conditions. The unique CALIPSO capability of profiling aerosols above clouds offers an unprecedented opportunity of examining uncertainties associated with the use of MODIS clear-sky data. Dust is separated from other types of aerosols using the depolarization measurements. We estimated that on the basis of 7-year average, 118142 Tg of dust is deposited into the tropical Atlantic and 3860 Tg of dust into the Amazon basin. Substantial interannual variations are observed during the period, with the maximum to minimum ratio of about 1.6 and 2.5 for the deposition to the tropical Atlantic and Amazon, respectively. The MODIS-based estimates appear to fall within the range of CALIPSO-based estimates; and the difference between MODIS and CALIPSO estimates can be largely attributed to the interannual variability, which is corroborated by long-term surface dust concentration observations in the tropical Atlantic. Considering that CALIPSO generally tends to underestimate the aerosol loading, our estimate is likely to represent a low bound for the dust transport and deposition estimate. The finding suggests that models have substantial biases and considerable effort is needed to improve model simulations of dust cycle.

dust↗

DOE OSTI2022

Advancing Cross-Disciplinary Understanding of Land-Atmosphere Interactions

The evolution of disciplinary silos and increasingly narrow disciplinary boundaries have together resulted in one-sided approaches to the study of land-atmosphere interactions—a field that requires a bi-directional approach to understand the complex feedbacks and interactions that occur. The integration of surface flux and atmospheric boundary layer measurements is therefore essential to advancing our understanding. The Land-Atmosphere 2021 workshop (held virtually, June 10-11, 2021) involved almost 300 participants from around the world and promoted cross-discipline collaboration by way of talks from invited speakers, moderated discussions, breakout sessions, and a virtual poster session. The workshop focused on five main theme areas: “big picture” overview, instrumentation and remote sensing, modeling, water, and aerosols and clouds. In talks and breakout groups, there were frequent calls for more AmeriFlux sites to be instrumented for boundary layer height measurements, and for the development of some “super sites” where profiling instruments would be deployed. There was further agreement on the need for the standardization of various datasets. There was also a consensus that funding agencies need to be willing to support the sorts of large projects (including associated instrumentation) which can drive interdisciplinary work. Early-career scientists, in particular, expressed enthusiasm for working across disciplinary boundaries but noted that there need to be more financial support and training opportunities so they would be better prepared for interdisciplinary work. Investment in these career development opportunities would enable today's cohort of early-career scientists to advance the frontiers of interdisciplinary work over the next couple of decades.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2014

Development of an aerosol microphysical module: Aerosol Two-dimensional bin module for foRmation and Aging Simulation (ATRAS)

Number concentrations, size distributions, and mixing states of aerosols are essential parameters for accurate estimation of aerosol direct and indirect effects. In this study, we developed an aerosol module, designated Aerosol Two-dimensional bin module for foRmation and Aging Simulation (ATRAS), that can represent these parameters explicitly by considering new particle formation (NPF), black carbon (BC) aging, and secondary organic aerosol (SOA) processes. A two-dimensional bin representation is used for particles with dry diameters from 40 nm to 10 µm to resolve both aerosol size (12 bins) and BC mixing state (10 bins) for a total of 120 bins. The particles with diameters from 1 to 40 nm are resolved using an additional 8 size bins to calculate NPF. The ATRAS module was implemented in the WRF-chem model and applied to examine the sensitivity of simulated mass, number, size distributions, and optical and radiative parameters of aerosols to NPF, BC aging and SOA processes over East Asia during the spring of 2009. BC absorption enhancement by coating materials was about 50% over East Asia during the spring, and the contribution of SOA processes to the absorption enhancement was estimated to be 10 – 20% over northern East Asia and 20 – 35% over southern East Asia. A clear north-south contrast was also found between the impacts of NPF and SOA processes on cloud condensation nuclei (CCN) concentrations: NPF increased CCN concentrations at higher supersaturations (smaller particles) over northern East Asia, whereas SOA increased CCN concentrations at lower supersaturations (larger particles) over southern East Asia. Application of ATRAS to East Asia also showed that the impact of each process on each optical and radiative parameter depended strongly on the process and the parameter in question. The module can be used in the future as a benchmark model to evaluate the accuracy of simpler aerosol models and examine interactions between NPF, BC aging, and SOA processes under different meteorological conditions and emissions.

Matsui, H.↗