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At least 1,351 records · Page 75

Learning Coagulation Processes With Combinatorial Neural Networks

Abstract Simulating the evolution of a coagulating aerosol or cloud of droplets in a key problem in atmospheric science. We present a proof of concept for modeling coagulation processes using a novel combinatorial neural network (CombNN) architecture. Using two types of data from a high‐detail particle‐resolved aerosol simulation, we show that CombNN models outperform standard neural networks and are competitive in accuracy with traditional state‐of‐the‐art sectional models. These CombNN models could have application in learning coarse‐grained coagulation models for multi‐species aerosols and for learning coagulation models from observed size‐distribution data.

54 ENVIRONMENTAL SCIENCES↗

AGR-2 TRISO Layer Thickness Imaging Archive

As a part of fuel quality control characterization, optical microscopy images of particle cross sections near midplane were acquired at Oak Ridge National Laboratory (ORNL). These particles were produced by the Advanced Gas Reactor Fuel Development and Qualification (AGR) Program’s AGR-2 irradiation campaign. These images may be of use for the development of image processing algorithms with the benchmark values measured at ORNL. This report provides those benchmark values, along with the raw images and data generated by the ORNL particle layer thickness analysis process.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Preliminary data on the optical properties of solid ammonia and scattering parameters for ammonia cloud particles.

The infrared absorption spectrum of solid ammonia is obtained from 2 to 125 microns as a composite of the published measurements. From this, the absorption coefficient and the complex refractive index are calculated as a function of frequency by integration of the Kramers-Kroenig dispersion relations. These data are used in a Mie theory analysis to obtain the basic parameters for scattering of long wavelength radiation by solid ammonia particles; this is believed to be an important process in radiative transfer within the atmospheres of the giant planets.

Taylor, F. W.↗

Methods for obtaining and reducing experimental droplet impingement data on arbitrary bodies

Experimental water droplet impingement data are used to validate particle trajectory computer codes used in the analysis and certification of aircraft de-icing/anti-icing systems. Water droplet impingement characteristics of aerodynamic surfaces are usually obtained from wind-tunnel dye tracer experiments. This paper presents a dye tracer method for measuring water droplet impingement characteristics on arbitrary geometries and a new data reduction method, based on laser reflectance measurements, for extracting impingement data. Extraction of impingement data has been a very time-consuming process in the past. The new data reduction method developed is at least an order of magnitude more efficient than the method previously used. The accuracy of the method is discussed and results obtained are presented.

Papadakis, Michael↗

Preliminary Pioneer-10 intensity gradients of galactic cosmic rays.

Selected data from the University of Chicago charged-particle telescope on the Pioneer-10 spacecraft bound for Jupiter have been examined and compared with data from the University of Chicago charged-particle telescopes on the Earth satellites IMP-5 and IMP-6 at 1 AU to derive a preliminary integral intensity gradient for relativistic galactic protons and helium nuclei. The preliminary value obtained is (4.5 plus or minus 1.0) percent per AU over the radial range 1-2.8 AU. Preliminary differential gradients also have been obtained for the energy range 29-67 MeV per nucleon.

Mckibben, R. B.↗

Contamination of spacecraft by recontact of dumped liquids

Liquids partially freeze when dumped from spacecraft producing particles which are released into free space at various velocities. Recontact of these particles with the spacecraft is possible for specific particle sizes and velocities and, therefore, can become contamination for experiments within the spacecraft or released experiments as a result of waste and potable water dumped from Space Shuttle. An examination of dump characteristics was conducted on STS-29 using both on-board video records and ground based measurements. A preliminary analysis of data from this flight indicates particle velocities are in the range of 30 to 75 ft/sec and recontact is possible for limited particle sizes.

Fowler, M. E.↗

Charged particle distributions in Jupiter's magnetosphere

In situ data from the Pioneer and Voyager spacecraft, supplemented by earth-based observations and theoretical considerations, are used as the basis for the present quantitative, compact model of the 1 eV-several MeV charged particle distribution in the Jovian magnetosphere. The thermal plasma parameters of convection speed, number density, and characteristic energy, are specified as functions of position for electrons and for the ion species H(+), O(+), O(2+), S(+), S(2+), S(3+), and Na(+). Major features of the magnetic field, thermal plasma, and trapped particle distributions, are modeled and results for each plasma region are compared with observed spectra. Comparisons show that the model represents the data to within a factor of 2 + or - 1, except where time variations are significant. Practical applications of the model to spacecraft near Jupiter are given.

Divine, N.↗

FY23 Update: Aerosol Sampling for the Canister Deposition Field Demonstration

This report describes the results of preliminary testing of aerosol monitoring equipment that will be used to continuously monitor the aerosol source term for the multi-year Canister Deposition Field Demonstration (CDFD). These data are required inputs for the development and validation of models for the deposition of dust and potentially corrosive salts on the surface of spent nuclear fuel (SNF) dry storage canisters. Surface salt loads correlate with the extent of corrosion damage on a metal surface, and potentially to the likelihood and timing of initiation of stress corrosion cracks. Aerosols will be monitored at the CDFD site using three instruments. A Dekati ® ELPI+ cascade impactor will be used for real-time monitoring of aerosol particle sizes. It will also collect dust in 14 size bins on impactor targets that can be chemically analyzed to determine the soluble salts present as a function of particle size. However, this instrument can only measure dried aerosols, with a diameter of <10 µm. The second instrument is a Topas laser particle size spectrometer, which provides real-time monitoring of aerosol particle sizes up to ~40 µm in size. It monitors both the ambient (potentially deliquesced) aerosol particle size distributions required for the dust deposition models and the distributions of the equivalent dried particles, allowing correlation with the Dekati ® data. However, it does not discriminate between inert dust particles and salt aerosols, and it does not retain samples of the different particle sizes for later analysis. The third instrument that will monitor aerosols at the CDFD site is a Clean Air Status and Trends Network (CASTNET) tower, which uses a multiple canister system to collect weekly samples for analysis to total suspended aerosol particle compositions and atmospheric gas concentrations. This status report describes work in FY23 to develop the capabilities for using these tools. In two training exercises, the cascade impactor and laser particle sizer were deployed in two different testing environments, one indoor and one outdoor. For the cascade impactor, the tests provided opportunities for the operators to familiarize themselves with impactor substrate preparation, and post-test sample removal and analysis. For the laser particle sizer, the tests were used to evaluate different instrument parameters, to determine the most appropriate settings for capturing transient events. Data and samples were collected for weeks to months for each test, and the results are presented here. In addition to the preliminary testing, contracts were developed with WSP Analytical Labs for sample preparation and analysis of the cascade impactor samples. The impactor tower from outdoor test was delivered to WSP and used to train the staff there in disassembly, sample extraction, sample analysis, and tower reassembly with new target substrates. These are tasks that WSP will be performing routinely for the CDFD project. The CASTNET system cannot be purchased or tested until an actual site has been selected for the CDFD test. Work for this FY has been restricted to preparation of contracts for purchasing the CASTNET tower, and for sample analysis, once the tower is in operation.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

A practical way to regularize unfolding of sharply varying spectra with low data statistics

Unfolding is a well-established tool in particle physics. However, a naive application of the standard regularization techniques to unfold the momentum spectrum of protons ejected in the process of negative muon nuclear capture led to a result exhibiting unphysical artifacts. A finite data sample limited the range in which unfolding can be performed, thus introducing a cutoff. A sharply falling “true” distribution led to low data statistics near the cutoff, which exacerbated the regularization bias and produced an unphysical spike in the resulting spectrum. An improved approach has been developed to address these issues and is illustrated using a toy model. The approach uses full Poisson likelihood of data, and produces a continuous, physically plausible, unfolded distribution. Here, the new technique has a broad applicability since sharply falling spectra are common.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Operation of the ATLAS trigger system in Run 2

The ATLAS experiment at the Large Hadron Collider employs a two-level trigger system to record data at an average rate of 1 kHz from physics collisions, starting from an initial bunch crossing rate of 40 MHz. During the LHC Run 2 (2015–2018), the ATLAS trigger system operated successfully with excellent performance and flexibility by adapting to the various run conditions encountered and has been vital for the ATLAS Run-2 physics programme. For proton-proton running, approximately 1500 individual event selections were included in a trigger menu which specified the physics signatures and selection algorithms used for the data-taking, and the allocated event rate and bandwidth. The trigger menu must reflect the physics goals for a given data collection period, taking into account the instantaneous luminosity of the LHC and limitations from the ATLAS detector readout, online processing farm, and offline storage. This document discusses the operation of the ATLAS trigger system during the nominal proton-proton data collection in Run 2 with examples of special data-taking runs. Aspects of software validation, evolution of the trigger selection algorithms during Run 2, monitoring of the trigger system and data quality as well as trigger configuration are presented.

43 PARTICLE ACCELERATORS↗

Shock compression of additively manufactured high solids loaded polymer composites with aligned porosity

The effects of aligned porosity on the shock-compression response of additively manufactured (AM) composite structures with collinear and log-cabin geometries are investigated. The composites contain two inorganic and two organic particle populations and a UV-curable polymer binder. X-ray phase contrast imaging (X-PCI) is used as an in-material diagnostic in plate-impact experiments performed at the Dynamic Compression Sector of the Advanced Photon Source at the Argonne National Laboratory. Macroscale shock and particle velocities and microscale pore collapse velocities are measured from X-PCI images obtained from samples impacted in various orientations relative to the AM build directions. The linear shock and particle velocity relation for the structures with collinear build geometry shows directional differences, with the build direction exhibiting the highest slope and the filament print direction having the shallowest slope. Composites with log-cabin geometry, due to their slightly lower porosity and smaller sized pores, show higher shock velocities than the collinear structures at the same particle velocity. Microscale directionality effects are also observed, with the pore collapse velocity dependent on the pore configuration. Specifically, the pore collapse velocity is highest for pores elongated along the impact direction which is the case for the colinear structures impacted in the filament print direction, which is consistent with the directionality trend observed in the data for the shock and particle velocity equation of state. The pore collapse velocity approaches ∼80 % of the shock velocity and is several times the average bulk particle velocity, suggesting a highly hydrodynamic mechanism of pore collapse. Overall, both the macroscale response as measured by the shock and particle velocity relationship, and the microscale response as measured by the pore collapse velocity, are found to be anisotropic and dependent on the AM composite structure.

Wagner, K. B. [Georgia Institute of Technology, At↗

Tracking and data system support for the Pioneer project. Pioneers 6-9, extended missions: 1 July 1972 - 1 July 1973, volume 12

The Tracking and Data System supported the deep space phases of the Pioneer 6, 7, 8, and 9 missions, with two spacecraft in an inward trajectory and two spacecraft in an outward trajectory from the earth in heliocentric orbits. During the period of this report, scientific instruments aboard each of the spacecraft continued to register information relative to interplanetary particles and fields, and radiometric data generated by the network continued to contribute to knowledge of the celestial mechanics of the solar system. In addition, to network support activity detail, network performance and special support activities are covered.

Miller, R. B.↗

Direct measurement of 59 Ni( n, p ) 59 Co and 59 Ni( n, α ) 56 Fe at fast-neutron energies from 500 keV to 10 MeV

We report nuclear reaction data for neutron induced reactions on unstable nuclei are critical for a wide range of applications spanning studies of nuclear astrophysics, nuclear reactor designs, and radiochemistry diagnostics. However, nuclear data evaluations of the reaction cross sections are largely based on calculations due to the difficulty in performing this class of measurements and the resulting lack of experimental data. For neutron induced charged particle reactions at fast neutron energies, at the MeV scale, these cross section predictions are predominately driven by statistical Hauser-Feshbach calculations. In this work, we present partial and total 59 Ni(n, p) and 59 Ni(n, α) cross sections, measured directly with a radioactive 59 Ni target, and compare the results to the present nuclear data evaluations. In addition, the results from this work are compared to a recent study of the 59 Ni(n, xp) reaction cross section that was performed via an indirect surrogate ratio method. The expected energy trend of the cross section, based on the current work, is inconsistent with that of the surrogate work. This calls into question the reliability of that application of the surrogate ratio method and highlights the need for direct measurements on unstable nuclei, when feasible.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

A Near-Global Survey of Cirrus Particle Size Using ISCCP

Cirrus is the most frequently occurring and widely distributed cloud type. The average annual frequency of occurrence for cirrus is 34% and its global coverage is about 20-30% (Warren et al. 1985). It strongly influences weather and climate processes through its effects on the radiation budget of the earth and the atmosphere (Liou 1986). Microphysics of cirrus is a critical component in understanding cloud-climate radiative interactions. For example, ice water content feedback is positive from a 1-D model study. But the feedback is substantially reduced upon the inclusion of small ice crystals (Sinha and Shine 1994). Due to the complexity caused by the non-spherical shape of ice crystals in cirrus, retrievals of cirrus properties are difficult. In recent years, advances have been made both in models and in case studies (e.g., Takano and Liou 1989, Young et al. 1994), but no global scale survey has been conducted. Similar to our previous near-global survey of droplet sizes of liquid water clouds (Han et al. 1994), a survey of cirrus ice crystal sizes is conducted over both continental and oceanic areas. We describe a method for retrieving cirrus particle size information on a near-global scale 50 deg S to 50 deg N using currently available satellite data from ISCCP. To retrieve cirrus particle size, we use a radiative transfer model that includes all major absorbing gases and cloud scattering/absorption to compute synthetic radiances as a function of satellite viewing geometry. Ice crystal shapes are assumed to be hexagonal columns and plates. The model results have been validated against clear sky observations and are consistent with the observed radiance range under cloudy conditions.

Han, Qingyuan↗

Impulsive acceleration and scatter-free transport of about 1 MeV per nucleon ions in (He-3)-rich solar particle events

Impulsive solar energetic particle (SEP) events are studied to: (1) describe a distinct class of SEP ion events observed in interplanetary space, and (2) test models of focused transport through detailed comparisons of numerical model prediction with the data. An attempt will also be made to describe the transport and scattering properties of the interplanetary medium during the times these events are observed and to derive source injection profiles in these events. ISEE 3 and Helios 1 magnetic field and plasma data are used to locate the approximate coronal connection points of the spacecraft to organize the particle anisotropy data and to constrain some free parameters in the modeling of flare events.

Mason, G. M.↗

Interplanetary propagation of less than 1-MeV protons in nonimpulsive energetic particle events

An investigation is conducted regarding the existence of measurable transverse diffusive transport for 0.3- to 0.5 MeV protons. The study focuses on 1-hour averaged proton anisotropy data measured by detectors on board the earth-orbiting IMP 7 and 8 spacecraft. The data is restricted to nonimpulsive energetic particle events which are not explicitly associated with solar flares. It is established to within the limits of the measurements using 1-hour averages, that in nonimpulsive 0.3- to 0.5-MeV proton events as measured in the Newtonian inertial frame of the solar system, the anisotropy is predominantly transverse to the magnetic field and most hourly averages of the transverse component are essentially due to the particles' E x B drift.

Zwickl, R. D.↗

Understanding particle size effect on fast-charging behavior of graphite anode using ultra-thin-layer electrodes

Extreme fast charging (≤ 15 min) of lithium-ion batteries is highly desirable to accelerate mass-market adoption of electric vehicles. However, significant capacity fading, as well as safety issues due to the lithium plating caused by the fast charging rate, limit its implementation. In this study, we investigated the fast-charging capability of graphite materials with various particle sizes. To eliminate the Li + ion concentration gradient effect across the thickness of the electrode, ultra-thin-layer graphite electrodes were developed to investigate the "real" fast-charging capability of graphite at the particle level. Electrochemical assessments as well as microscopic characterizations revealed that smaller particles exhibited superior fast-charging performance, featuring enhanced capacity reversibility, faster charging rate, and less lithium plating under the same fast-charging conditions. It is shown that small-particle graphite (mean radius of 3.3 μm) could withstand a 4C charge (to 80 % state-of-charge) without plating, with minimal plating occurring at 6C. Thicker particles exhibited plating at lower C-rates. Since the experimental data could not directly explain whether intra-particle diffusion limitations or interfacial reaction limitations dominated the plating mechanism, the pseudo-2-dimensional model was used to evaluate the most likely plating mechanism. The model suggested that particle-level diffusion is the dominant mechanism contributing to plating at high rates. Finally, this work provides comprehensive insights into the particle size effects on fast-charging capability, offering a better understanding of fast-charging behavior and valuable guidance for designing optimal electrode architecture for high-rate lithium-ion batteries.

25 ENERGY STORAGE↗

Arctic Black Carbon Aerosol Deposition Study North Slope of Alaska 2020- UHSAS Measurements

Particles are removed from the atmosphere through both wet and dry deposition. These processes are poorly understood, though they constitute important uncertainties in climate and air quality models. This project aims to use observational constraints on particle fluxes to improve model representations of dry deposition. Within this data set, we measured fluxes of size resolved particles with an ultrahigh sensitivity aerosol spectrometer (UHSAS) at the ARM facility’s North Slope Alaska site. Measurements were made at the meteorological tower between 9 Sept and 25 Oct 2021. This site is a coastal tundra location and received snow during the project.

Aerosol concentration↗