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All sources NASA NTRS DOE OSTI

DOE OSTI2026

Enhancing NO Reduction by CO Over NiO/CeO 2 Catalyst by Optimizing the Metal Oxide–Support Interaction

Noble metal catalysts are widely used in three-way catalysts (TWCs) due to their high efficiency, but their scarcity and high cost drive the need for effective, low-cost alternatives. Here, in this work, a series of NiO/CeO 2 catalysts were engineered by modulating the OH content and crystallite size of the CeO 2 support. This approach yielded Ni species ranging from isolated single atoms to small clusters and larger aggregates, with varied NiO/CeO 2 interaction strengths. Evaluation of their performance in NO reduction by CO, CO oxidation, and the water–gas shift reaction revealed that the NiO/CeO 2 -300 catalyst, featuring small CeO 2 crystallites and highly dispersed NiO clusters, delivered superior activity for NO reduction and CO oxidation. It was demonstrated that small NiO clusters, due to their efficient CO adsorption and activation, were more active than Ni single atoms. Furthermore, the presence of water was found to influence the catalyst stability, with NiO clusters less stable than single atoms likely due to the hydroxylation effect leading to the formation of Ni(OH) 2 . Oxygen storage capacity measurements revealed that performance was governed by a combination of CeO 2 crystallite size and the abundance of NiO/CeO 2 interfaces. These findings demonstrated that the catalytic performance of Ni/CeO 2 systems could be maximized by optimizing the Ni nanostructure and its interaction with CeO 2 support, positioning them as a promising, multifunctional nonprecious alternative for three-way catalysis application.

36 MATERIALS SCIENCE↗

DOE OSTI2020

Blading Phase–Pure Formamidinium–Alloyed Perovskites for High–Efficiency Solar Cells with Low Photovoltage Deficit and Improved Stability

Currently, blade-coated perovskite solar cells (PSCs) with high power conversion efficiencies (PCEs), i.e. greater than 20%, normally employ methylammonium lead tri-iodide with a sub-optimal bandgap. Alloyed perovskites with formamidinium (FA) cation have narrower bandgap and thus enhance device photocurrent. However, FA-alloyed perovskites show low phase stability and high moisture sensitivity. Here, we report that incorporating 0.83 molar percent organic halide salts (OHs) into the perovskite inks enables phase-pure, highly crystalline FA-alloyed perovskites with extraordinary optoelectronic properties. Here, the OH molecules modulate the crystal growth, enhance the phase stability, passivate ionic defects at the surface and/or grain boundaries, and enhance the moisture stability of the perovskite film. We demonstrate a high efficiency of 22.0% under 1 sun illumination for blade-coated PSCs with an open-circuit voltage of 1.18 V, corresponding to a very small voltage deficit of 0.33 V, and significantly improved operational stability with 96% of the initial efficiency retained under one sun illumination for 500 hours.

14 SOLAR ENERGY↗

DOE OSTI2023

The promise of metal-halide-perovskite solar photovoltaics: A brief review

Solar photovoltaics (PVs) based on metal-halide perovskites (MHPs) have taken the renewable-energy world by storm. The excitement stems from the promise of a high-efficiency, low-cost, and low “carbon-footprint” new PV technology. Here, a brief overview of the important topics pertaining to MHPs, perovskite solar cells (PSCs) and perovskite solar modules (PSMs) is presented. The topics include: (1) PSC architectures, (2) MHPs, (3) synthesis and processing of MHP thin films, (4) MHP thin-film microstructures, (5) PSC functional layers, (6) interfacial engineering in PSCs, (7) PSC performance, (8) PSC stability, (9) PSMs, (10) lead toxicity, and (11) mechanical behavior and reliability. The significant challenges in the path toward commercialization of this burgeoning PV technology are also highlighted. Chief among them are scalability, stability, reliability, and safety, while achieving high efficiency, low cost, and low “carbon-footprint.” Furthermore, the promise of this new PV technology and the fascinating underlying science make it a worthwhile endeavor to address these challenges.

14 SOLAR ENERGY↗

NASA NTRS2004

Motor/Generator and Inverter Characterization for Flywheel System Applications

The Advanced Electrical Systems Development Branch at NASA Glenn Research Center (GRC) has been involved in the research and development of high speed flywheels systems for satellite energy storage and attitude applications. These flywheels will serve as replacement for chemical nickel hydrogen, nickel cadmium batteries and gyroscopic wheels. The advantages of using flywheel systems for energy storage on satellites are high energy density, high power density, long life, deep depth of discharge, and broad operating temperature ranges. A flywheel system for space applications consist of a number of flywheel modules, the motor/generator and magnetic bearing, and an electronics package. The motor/generator electronics package includes a pulse-width modulated inverter that drives the flywheel permanent magnet motor/generator located at one end of the shaft. This summer, I worked under the direct supervision of my mentor, Walter Santiago, and the goal for this summer was to characterize motor generator and inverter attributes in order to increase their viability as a more efficient energy storage source for space applications. To achieve this goal, magnetic field measurements around the motor/generator permanent magnet and the impedance of the motor/generator three phase windings were characterized, and a recreation of the inverter pulse width modulated control system was constructed. The Flywheel modules for space use are designed to maximize energy density and minimize loss, and attaining these values will aid in locating and reducing losses within the flywheel system as a whole, making flywheel technology more attractive for use as energy storage in future space applications.

Tamarcus, Jeffries L.↗

DOE OSTI2026

Synergistic Evolution of Segmental Motion and Cooperative Relaxation within the Amorphous Phase of Organic Mixed Ionic-Electronic Conductors

Organic mixed ionic-electronic conductors (OMIECs) facilitate a variety of electrochemical processes and feature a heterogeneous microstructure composed of both crystalline and amorphous phases. However, structural evolution in amorphous regions during electrochemical doping remains poorly understood, limiting our understanding of mixed conduction mechanisms. Here, in this work, we develop operando chip calorimetry to probe amorphous phase evolution in poly(3,4-ethylenedioxythiophene):poly(styrenesulfonate) (PEDOT:PSS) under swelling and electrochemical (de)doping. Our results reveal that amorphous regions providing ionic transport pathways and those within electronic transport channels undergo heterogeneous, yet synergistic, evolution during electrochemical modulation. The cooperative interplay between segmental motion and relaxation maintains ionic conductivity and intergrain electronic transport upon electrowetting and doping, while facilitating efficient ion hopping and adaptable chain conformations during dedoping. Such synergies are more pronounced in loose structures featuring a fibrillar morphology, which exhibit lower glass transition temperatures (T g ) and higher fragility (m). High-throughput robotic screening further establishes a strong correlation between elevated m/T g ratios and enhanced mixed conduction. These findings elucidate the role of the amorphous phase in the synthesis of OMIECs and underscore the potential of operando chip calorimetry in uncovering structure–property relationships in electroactive polymers.

amorphous phase↗

DOE OSTI2025

Amplifying Magnetic Field Effects on Upconversion Emission via Molecular Qubit-Driven Triplet–Triplet Annihilation

Triplet-triplet annihilation (TTA) enables photon upconversion by combining two lower-energy triplet excitons to produce a higher-energy singlet exciton. This mechanism enhances light-harvesting efficiency for solar energy conversion and enables the use of lower-energy photons in bioimaging and photoredox catalysis applications. The magnetic modulation of such high-energy excitons presents an exciting opportunity to develop molecular quantum information technologies. While the spin dynamics of triplet exciton pairs are sensitive to external magnetic fields, the magnetic field effects (MFEs) associated with these pairs are generally limited by spin statistics to at most 10% at low fields (<1 Tesla), making them challenging to apply in technological advancements. In contrast, MFEs on spin-correlated radical pairs (SCRPs) can be significantly greater, surpassing those on triplet pairs. By using SCRPs-based molecular qubits as triplet sensitizers in the sensitized TTA scheme, we can magnetically modulate TTA and consequently, the delayed fluorescence of annihilators. In our current system, we have achieved more than 70% magnetic modulation of delayed fluorescence, effectively harnessing and even amplifying magnetic modulation within SCRPs to influence high-energy excitons. In conclusion, this work opens new opportunities for advancing spin-controlled chemical reactions and molecular quantum information technologies.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2025

Ponderomotive electron physics captured in a single-fluid extended magnetohydrodynamics model

The ponderomotive force, arising from the interaction between electromagnetic waves and plasma, plays a critical role in laser fusion, astrophysical plasmas, and laser diagnostics. Traditionally, modeling this force requires multi-fluid or particle-in-cell simulations due to its strong coupling to electron-scale dynamics. In this work, we demonstrate that a one-fluid, two-temperature extended magnetohydrodynamics (XMHD) model—augmented with a generalized Ohm's law (GOL) including electron inertia—can accurately reproduce key ponderomotive effects. We derive the ponderomotive force within this framework using a phasor-based approach and then validate its nonlinear manifestations through direct numerical simulations in the PERSEUS code, where steepening and density modulation phenomena typically associated with kinetic-scale models are reproduced. These results and prior work establish XMHD as a robust and efficient alternative for modeling nonlinear laser–plasma dynamics, bridging the gap between ideal MHD and fully kinetic approaches.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2023

Evaluation of planar silicon pixel sensors with the RD53A readout chip for the Phase-2 Upgrade of the CMS Inner Tracker

The Large Hadron Collider at CERN will undergo an upgrade inorder to increase its luminosity to7.5 × 10$^{34}$ cm$^{-2}$s$^{-1}$. The increased luminosityduring this High-Luminosity running phase, starting around 2029,means a higher rate of proton-proton interactions, hence a largerionizing dose and particle fluence for the detectors. The currenttracking system of the CMS experiment will be fully replaced inorder to cope with the new operating conditions. Prototype planarpixel sensors for the CMS Inner Tracker with square50 μm × 50 μm and rectangular100 μm × 25 μm pixels read out by theRD53A chip were characterized in the lab and at the DESY-II testbeamfacility in order to identify designs that meet the requirements ofCMS during the High-Luminosity running phase. A spatial resolutionof approximately 3.4 μm (2 μm) is obtained using themodules with 50 μm × 50 μm(100 μm × 25 μm) pixels at the optimalangle of incidence before irradiation. After irradiation to a 1 MeVneutron equivalent fluence ofΦ$_{eq}$ = 5.3 × 10$^{15}$ cm$^{-2}$, a resolution of9.4 μm is achieved at a bias voltage of 800 V using a modulewith 50 μm × 50 μm pixel size. All modulesretain a hit efficiency in excess of 99% after irradiation tofluences up to 2.1 × 10$^{16}$ cm$^{-2}$. Further studies ofthe electrical properties of the modules, especially crosstalk, arealso presented in this paper.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

DOE OSTI2023

Early Fault Detection in Particle Accelerator Power Electronics Using Ensemble Learning

Early fault detection and fault prognosis are crucial to ensure efficient and safe operations of complex engineering systems such as the Spallation Neutron Source (SNS) and its power electronics (high voltage converter modulators). Following an advanced experimental facility setup that mimics SNS operating conditions, the authors successfully conducted 21 early fault detection experiments, where fault precursors are introduced in the system to a degree enough to cause degradation in the waveform signals, but not enough to reach a real fault. Nine different machine learning techniques based on ensemble trees, convolutional neural networks, support vector machines, and hierarchical voting ensembles are proposed to detect the fault precursors. Although all 9 models have shown a perfect and identical performance during the training and testing phase, the performance of most models has decreased in the next test phase once they got exposed to realworld data from the 21 experiments. The hierarchical voting ensemble, which features multiple layers of diverse models, maintains a distinguished performance in early detection of the fault precursors with 95% success rate (20/21 tests), followed by adaboost and extremely randomized trees with 52% and 48% success rates, respectively. The support vector machine models were the worst with only 24% success rate (5/21 tests). The study concluded that a successful implementation of machine learning in the SNS or particle accelerator power systems would require a major upgrade in the controller and the data acquisition system to facilitate streaming and handling big data for the machine learning models. In addition, this study shows that the best performing models were diverse and based on the ensemble concept to reduce the bias and hyperparameter sensitivity of individual models.

43 PARTICLE ACCELERATORS↗

NASA NTRS1973

High efficiency ground data transmission

It is demonstrated that state-of-the-art communications technology can be implemented and reliably operated on a global basis to increase the transmission rates and efficiencies on circuits with bandwidths greater than the typical speech channel. Optimization is affected by optimum clock recovery procedures, multilevel pulse amplitude modulation, single sideband amplitude modulation, transversal filter equalizers, data scrambling, and active compensation for phase instability.

Dickinson, W. B.↗

NASA NTRS1979

Nuclear power source for electric propulsion

A low specific weight (20 to 40 Kg/Kwe), long life (6 to 10 year), 100 to 400 KWe nuclear electric propulsion (NEP) system can deliver 2,000 to 10,000 Kg payloads for intensive study of our solar system. The nuclear power source is about 80% of the NEP system mass, thus the NASA program is focused on developing the power source technology. Because of the long life requirements, direct thermal to electric energy conversion technology (thermionic and thermoelectric) is being pursued. In order to meet the low specific weight it is necessary to develop a 10 to 15% conversion module with a 875 K minimum heat rejection temperature and a 1675 K maximum input temperature. The thermoionic converter is about 9% efficient at these temperatures. The thermoelectric converter is limited to a 1300 K input temperature. So, the thermionic program is focused on improving the efficiency while the thermoelectric program is focused on increasing the temperature.

Mondt, J. F.↗

NASA NTRS1988

Nonlinear, dispersive, elliptically polarized Alfven wavaes

The derivative nonlinear Schroedinger (DNLS) equation is derived by an efficient means that employs Lagrangian variables. An expression for the stationary wave solutions of the DNLS that contains vanishing and nonvanishing and modulated and nonmodulated boundary conditions as subcases is then obtained. The solitary wave solutions for elliptically polarized quasiparallel Alfven waves in the magnetohydrodynamic limit (nonvanishing, unmodulated boundary conditions) are obtained. These converge to the Korteweg-de Vries and the modified Korteweg-de Vries solitons obtained previously for oblique propagation, but are more general. It is shown that there are no envelope solitary waves if the point at infinity is unstable to the modulational instability. The periodic solutions of the DNLS are characterized.

Kennel, C. F.↗

NASA NTRS1993

An installed nacelle design method using multiblock Euler solver

An efficient multiblock Euler design method was developed for designing a nacelle installed on geometrically complex airplane configurations. This approach employed a design module based on a direct iterative surface curvature method developed at NASA-Langley. A multiblock Euler flow solver was used for computing flow around complex geometries. The flow solver used a finite-volume formulation with explicit time-stepping to solve the Euler equations. It used a multiblock version of the multigrid method to accelerate the convergence of the calculations. The design module successively updated the surface geometry to reduce the difference between the computed and target pressure distributions. In the flow solver, the change in surface geometry was simulated by applying surface transpiration boundary conditions to avoid repeated grid generation during design iterations. Smoothness of the designed surface was ensured by alternate application of streamwise and circumferential smoothings.

Chen, H. C.↗

NASA NTRS1993

The MSAT spacecraft of Telesat Mobile Inc.

The MSAT spacecraft of the Canadian mobile satellite operator, Telesat Mobile Inc. (TMI) is described. When launched in 1994, the large geostationary MSAT spacecraft which is currently under construction by Hughes Aircraft Co. and Spar Aerospace Ltd. will enable TMI to provide mobile and transportable communications services to its customers even in the most remote parts of the North American continent. The main elements of TMI's mobile satellite system (described in a companion paper) are the space segment and the ground segment. TMI's space segment will employ one of two nearly identical satellites, one of which will be owned and operated by TMI, the other by the U.S. mobile satellite operator, American Mobile Satellite Corporation (AMSC). The two companies are participating in a joint spacecraft procurement in order to reduce the nonrecurring costs and to ensure system compatibility between the two systems; and they have also agreed to provide in-orbit backup to each other in the event of a catastrophic satellite failure. The program status, performance requirements, main parameters, and configuration of the MSAT spacecraft are reviewed. The major features of the communications subsystem are discussed in some detail, and a brief summary is presented of the spacecraft service module. Key technology items include the L-band RF power amplifier, which must operate with a high DC to RF power efficiency and generate low intermodulation when loaded with multi-carrier signals; and the large diameter deployable L-band antenna. The development status and expected performance of these spacecraft components is examined.

Bertenyi, E.↗

NASA NTRS2002

Solar Electric Propulsion Technologies Being Designed for Orbit Transfer Vehicle Applications

There is increasing interest in employing Solar Electric Propulsion (SEP) for new missions requiring transfer from low Earth orbit to the Earth-Moon Lagrange point, L1. Mission architecture plans place the Gateway Habitat at L1 in the 2011 to 2016 timeframe. The Gateway Habitat is envisioned to be used for Lunar exploration, space telescopes, and planetary mission staging. In these scenarios, an SEP stage, or "tug," is used to transport payloads to L1--such as the habitat module, lunar excursion and return vehicles, and chemical propellant for return crew trips. SEP tugs are attractive because they are able to efficiently transport large (less than 10,000 kg) payloads while minimizing propellant requirements. To meet the needs of these missions, a preliminary conceptual design for a general-purpose SEP tug was developed that incorporates several of the advanced space power and in-space propulsion technologies (such as high-power gridded ion and Hall thrusters, high-performance thin-film photovoltaics, lithium-ion batteries, and advanced high-voltage power processing) being developed at the NASA Glenn Research Center. A spreadsheet-based vehicle system model was developed for component sizing and is currently being used for mission planning. This model incorporates a low-thrust orbit transfer algorithm to make preliminary determinations of transfer times and propellant requirements. Results from this combined tug mass estimation and orbit transfer model will be used in a higher fidelity trajectory model to refine the analysis.

Sarver-Verhey, Timothy R.↗

NASA NTRS2009

Overview of Human Factors and Habitability at NASA

This slide presentation reviews the ongoing work on human factors and habitability in the development of the Constellation Program. The focus of the work is on how equipment, spacecraft design, tools, procedures and nutrition be used to improve the health, safety and efficiency of the crewmembers. There are slides showing the components of the Constellation Program, and the conceptual designs of the Orion Crew module, the lunar lander, (i.e., Altair) the microgravity EVA suit, and the lunar surface EVA suit, the lunar rover, and the lunar surface system infrastructure.

Connolly, Janis↗

NASA NTRSDate not supplied

Evaluating the performance of portable air filter walls for the James Webb Space Telescope launch campaign

The James Webb Space Telescope (JWST) launched from the Centre Spatial Guyanais (CSG) in December 2021. JWST’s requirements permitted processing in International Organization for Standardization (ISO) Class 7 or better facilities, but CSG was only equipped with ISO Class 8 facilities. To temporarily upgrade the air cleanliness in the Payload Processing Facility, Fueling Hall, and Final Assembly Building Encapsulation Hall, NASA provided two portable High Efficiency Particulate Air (HEPA) and carbon filter walls that were used in each location. The walls were comprised of stacks of two modules high and arranged in push-push configurations as shown to be most effective via Computational Fluid Dynamics simulations of expected floor layouts in each facility. After delivery to NASA’s Goddard Space Flight Center in 2020, the walls underwent initial verification measurements inside a cleanroom and validation testing in an uncontrolled area to quantify their improvement of air cleanliness and particle and molecular fallout. Validation testing showed improvements of 83-99% for airborne particle counts, 79-91% for particle fallout, and 50-90% for molecular fallout. The particle improvements were applied to the contamination budget analysis that tracked current and predicted future cleanliness against End-of-Life requirements for JWST’s critical surfaces. At CSG, the walls successfully maintained an ISO Class 7 environment or better within their envelope in each location, despite their presence in ISO Class 8 facilities with dense integration operations.

HEPA, Contamination Control, Filtration↗

NASA NTRS2022

Evaluating the Performance of Portable Air Filter Walls for the James Webb Space Telescope Launch Campaign

HEPA, Contamination Control, Filtration↗