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At least 1,333 records · Page 74
All sourcesNASA NTRSDOE OSTI
DOE OSTI2024

237 Np Fission Spectrum Cumulative Fission Product Yield Measurement Using Godiva IV Critical Assembly

Precise integral measurement of fast neutron-induced fission product yields for various actinides is of high interest for applied nuclear science. The goal of this effort is to improve uncertainties in fission product yield values of 237 Np. Fission was induced in a NpO 2 (NO 3 ) target using the Godiva IV critical assembly in burst mode. The irradiated sample was transferred to a high-resolution γ-ray detection setup within 50 minutes. γ-ray list mode data was collected from 50 minutes to 1 week after the irradiation. γ-ray spectroscopy was performed to analyze the time dependent γ-ray yields using an automated peak search algorithm to identify isotopes by their decay γ-ray energy and half-life. Finally, the initial activity for each isotope identified was used to calculate their fission product yield.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2024

239 Pu Fission Spectrum Cumulative Fission Product Yield Measurement Using Godiva IV Critical Assembly

Precise integral measurement of fast neutron-induced fission product yields for various actinides is of high interest for applied nuclear science. The goal of this effort is to improve uncertainties in fission product yield values of 239 Pu. Fission was induced in a pure 239 Pu (>99%) target using the Godiva IV critical assembly in burst mode. Further, the irradiated sample was transferred to a high-resolution γ-ray detector within 45 minutes. γ-ray list mode data was collected from 45 minutes to 1 week after the irradiation. γ-ray spectroscopy was performed to analyze the time dependent γ-ray yields using an automated peak search algorithm to identify isotopes by their decay γ-ray energy and half-life. The initial activity for each isotope identified was used to calculate their fission product yield.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

Jet-associated deuteron production in pp collisions at $\sqrt{s}$ =13 TeV

Deuteron production in high-energy collisions is sensitive to the space–time evolution of the collision system, and is typically described by a coalescence mechanism. For the first time, we present results on jet-associated deuteron production in pp collisions at $\sqrt{s}$ =13 TeV, providing an opportunity to test the established picture for deuteron production in events with a hard scattering. Using a trigger particle with high transverse-momentum (p T > GeV/c) as a proxy for the presence of a jet at midrapidity, we observe a measurable population of deuterons being produced around the jet proxy. The associated deuteron yield measured in a narrow angular range around the trigger particle differs by 2.4–4.8 standard deviations from the uncorrelated background. The data are described by PYTHIA model calculations featuring baryon coalescence.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2021

Υ production and nuclear modification at forward rapidity in Pb–Pb collisions at $\sqrt{S_{NN}}$ = 5.02 TeV

The production of Υ mesons in Pb–Pb collisions at a centre-of-mass energy per nucleon pair $\sqrt{S_{NN}}$ = 5.02 TeV is measured with the muon spectrometer of the ALICE detector at the LHC. The yields as well as the nuclear modification factors are determined in the forward rapidity region 2.5 < y < 4.0, as a function of rapidity, transverse momentum and collision centrality. The results show that the production of the Υ(1S) meson is suppressed by a factor of about three with respect to the production in proton– proton collisions. For the first time, a significant signal for the Υ(2S) meson is observed at forward rapidity, indicating a suppression stronger by about a factor 2–3 with respect to the ground state. The measurements are compared with transport, hydrodynamic, comover and statistical hadronisation model calculations.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2022

Accessing subnuclear fluctuations and saturation with multiplicity dependent J/ψ production in p+p and p+Pb collisions

We study the production of J/ψ vector mesons as a function of charged hadron multiplicity in p+p and p+Pb collisions at LHC energies. We employ the color glass condensate framework, using running coupling Balitsky-Kovchegov evolved dipole amplitudes, to compute gluon and cc¯-pair production. We use fragmentation functions to obtain charged hadrons, and explore two different hadronization schemes for the J/ψ: non-relativistic quantum chromodynamics and the improved color evaporation model. In our framework, event-by-event multiplicity fluctuations of both hadrons and J/ψ are driven by geometric and saturation scale normalization fluctuations. Studying the correlation between J/ψ and hadron multiplicity, we show that the characteristic difference between forward and backward rapidity in p+Pb collisions is a result of different degrees of saturation probed at different rapidities. We demonstrate that experimental data on heavy-flavor production as a function of event activity provide stringent constraints on the fluctuating proton structure

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2023

First measurement of $Ω^0_c$ production in pp collisions at $\sqrt{s}=$13 TeV

The inclusive production of the charm–strange baryon $Ω^0_c$ is measured for the first time via its hadronic decay into Ω – π + at midrapidity(|y| < 0.5) in proton–proton (pp) collisions at the centre-of-mass energy $\sqrt{s}=$ 13 TeV with the ALICE detector at the LHC. The transverse momentum (p T ) differential cross section multiplied by the branching ratio is presented in the interval 2 < p T < 12 GeV/c. The p T dependence of the $Ω^0_c$-baryon production relative to the prompt D 0 -meson and to the prompt $Ξ^0_c$-baryon production is compared to various models that take different hadronisation mechanisms into consideration. In the measured p T interval, the ratio of the p T -integrated cross sections of $Ω^0_c$ and prompt $Λ^+_c$ baryons multiplied by the Ω – π + branching ratio is found to be larger by a factor of about 20 with a significance of about 4σ when compared to e + e – collisions.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2023

$f$ 0 (980) production in inelastic pp collisions at s = 5.02 TeV

The measurement of the production of f 0 (980) in inelastic pp collisions at $\sqrt{s}$ = 5.02 TeV is presented. This is the first reported measurement of inclusive f 0 (980) yield at LHC energies. The production is measured at midrapidity, |y| < 0.5, in a wide transverse momentum range, 0 < p T < 16 GeV/c, by reconstructing the resonance in the f 0 (980) → π + π - hadronic decay channel using the ALICE detector. The p T -differential yields are compared to those of pions, protons and $φ$ mesons as well as to predictions from the HERWIG 7.2 QCD-inspired Monte Carlo event generator and calculations from a coalescence model that uses the AMPT model as an input. The ratio of the p T -integrated yield of f 0 (980) relative to pions is compared to measurements in e + e - and pp collisions at lower energies and predictions from statistical hadronisation models and HERWIG 7.2. A mild collision energy dependence of the f 0 (980) to pion production is observed in pp collisions from SPS to LHC energies. All considered models underpredict the p T -integrated 2f 0 (980)/(π + +π - ) ratio. The prediction from the canonical statistical hadronisation model assuming a zero total strangeness content of f 0 (980) is consistent with the data within 1.9σ and is the closest to the data. The results provide an essential reference for future measurements of the particle yield and nuclear modification in p–Pb and Pb–Pb collisions, which have been proposed to be instrumental to probe the elusive nature and quark composition of the f 0 (980) scalar meson.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2024

Observation of abnormal suppression of f 0 (980) production in p–Pb collisions at $\sqrt{s_{NN}}$= 5.02 TeV

The dependence of f 0 (980) production on the final-state charged-particle multiplicity in p–Pb collisions at $\sqrt{s_{NN}}$= 5.02 TeV is reported. The production of f 0 (980) is measured with the ALICE detector via the f 0 (980) → π + π – decay channel in a midrapidity region of –0.5 < y < 0. Particle yield ratios of f 0 (980) to π and K*(892) 0 are found to be decreasing with increasing charged-particle multiplicity. The magnitude of the suppression of the f 0 (980)/π and f 0 (980)/K*(892) 0 yield ratios is found to be dependent on the transverse momentum p T , suggesting different mechanisms responsible for the measured effects. Furthermore, the nuclear modification factor Q pPb of f 0 (980) is measured in various multiplicity ranges. The Q pPb shows a strong suppression of the f 0 (980) production in the p T region up to about 4 GeV/c. The results on the particle yield ratios and Q pPb for f 0 (980) may help to understand the late hadronic phase in p–Pb collisions and the nature of the internal structure of f 0 (980) particle.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2025

Observation of VVZ production at $\sqrt{s}$ = 13 TeV with the ATLAS detector

A search for the production of three massive vector bosons, VVZ(V = W, Z) , in proton-proton collisions at $\sqrt{s}$ = 13 TeV is performed using data with an integrated luminosity of 140 fb -1 recorded by the ATLAS detector at the Large Hadron Collider. Events produced in the leptonic final states WWZ → ℓvℓvℓℓ (ℓ = e,μ), WZZ → ℓvℓℓℓℓ, ZZZ → ℓℓℓℓℓ, and the semileptonic final states WWZ → qq ℓvℓℓ and WZZ → ℓv qq ℓℓ, are analysed. The measured cross section for the pp → VVZ process is 660$^{+93}_{-90}$(stat.)$^{+80}_{-81}$(syst.) fb, and the observed (expected) significance is 6.4 (4.7) standard deviations, representing the observation of VVZ production. In addition, the measured cross section for the pp → WWZ process is 442 ± 94(stat.)$^{+60}_{-52}$(syst.) fb, and the observed (expected) significance is 4.4 (3.6) standard deviations, representing evidence of WWZ production. The measured cross sections are consistent with the Standard Model predictions. Constraints on physics beyond the Standard Model are also derived in the effective field theory framework by setting limits on Wilson coefficients for dimension-8 operators describing anomalous quartic gauge boson couplings.

Aad, G. (ORCID:0000000266654934)↗
DOE OSTI2025

Constraining off-shell Higgs boson production and the Higgs boson total width using WW → ℓνℓν final states with the ATLAS detector

A measurement of off-shell Higgs boson production is performed in the H* → WW channel. The measurement uses a proton–proton collision dataset with an integrated luminosity of 140 fb -1 collected at a centre-of-mass energy of 13 TeV by the ATLAS detector at the Large Hadron Collider. Final states in which both W bosons decay leptonically are targeted, and events are categorised based on the flavour of the final-state leptons, the jet multiplicity, and the output of neural network-based classifiers. The data are found to be compatible with the Standard Model expectation. An observed (expected) upper bound on the 95 % symmetric confidence level interval is set on the rate of off-shell Higgs boson production at a value of 3.4 (4.4) times the Standard Model prediction. These results are combined with the results from the measurement of on-shell Higgs boson production in the same final states to obtain an observed (expected) upper bound at 95 % confidence level on the Higgs boson total width of 13.1 (17.3) MeV.

Aad, G. [Aix-Marseille Univ., Marseille (France)] ↗
DOE OSTI2026

Electromagnetic production of kaons on the nucleon

Studies of the electromagnetic production of strange quarks started in the 1950s as something of a curiosity that puzzled experimentalists and theorists alike. Eventually, a nascent understanding of these processes began to take shape through the first pioneering experiments dedicated to explore photo- and electroproduction that were carried out in the period from the 1950s to the 1980s. As the datasets increased, concomitant advances in theoretical models were realized. However, these initial studies also made clear that more precise data was essential to continue to move forward. A paradigm shift occurred in the 1990s with the development of second-generation facilities at ELSA, MAMI, SPring-8, and JLab. High-intensity, high duty-factor accelerators, coupled with novel detector systems and advances in computing and readout electronics, brought nuclear physics experiments forward by orders of magnitude in counting statistics compared to the first-generation efforts. This was an utter boon to strangeness physics investigations, and to date, more than 50 dedicated experiments in kaon photo- and electroproduction have been completed at facilities around the world, leading to a host of experimental observables that have enabled significant advances in the exploration of strongly interacting systems that decay via $s\bar{s}$ quark pair creation. These data have proven to be an essential complementary pathway to study the spectrum and structure of the excited states of the nucleon, and the search for missing and exotic baryon configurations. As well, investigations in these channels are requisite for exploring hypernuclear production as a probe of the $YN$ interaction and for studies of the electromagnetic form factors of strange mesons. This review was designed to provide the first-ever in-depth overview of both the experimental and theoretical progress in the field of the electromagnetic production of strangeness. This work looks back over 70 years of past developments, discusses ongoing work and near-term plans, and details future possibilities being considered for third-generation facilities. Extensive lists of the available datasets and theoretical models are provided, together with a comprehensive supporting bibliography of the field. Throughout this work, the primary impacts of these explorations are highlighted, along with connections to a wide range of related phenomenological applications. An important goal of this review is to provide a complete, (reasonably) self-contained guide into this field prepared at a level that is relevant for both new and seasoned scientists, whether experimentalists, phenomenologists, or theorists, to better understand what has been accomplished by so many dedicated folks-each building on what has come before-and to appreciate the exciting future potential for continued studies in this area.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2022

Metabolic flux modeling of Gluconobacter oxydans enables improved production of bioleaching organic acids

Bioleaching with organic acids is an option for recovery of rare earth elements (REE) and or other valuable metals from consumer or industrial wastes. Biohydrometallurgy can play an economically and environmentally sustainable role in REE recycling, particularly if agriculture or food wastes are used as the carbon substrates for production of the bioleaching agents. A challenge for organic acid based REE bioleaching is the incomplete conversion of the carbon substrate to an optimal organic acid mixture with high REE extraction capability. To help meet this challenge a metabolic flux model was developed for Gluconobacter oxydans to identify options for improving sugar conversion to chelating organic acids. Here, model predictions were consistent with laboratory data for the microbial consumption of glucose and production of gluconic acid and suggested that providing growth conditions with relatively high carbon to nitrogen molar ratios could result in production of lower pH biolixiviant and thus improve REE bioleaching yields.

59 BASIC BIOLOGICAL SCIENCES↗
DOE OSTI2026

Transforming E-Waste Into Strategic Resources: Techno-Economic Analysis of Gallium and By-products Recovery from LEDs via Bioleaching

The growing demand for gallium in optoelectronics and renewable energy applications raises concerns about supply security and production sustainability. This study evaluates the techno-economic feasibility of recovering gallium and by-products (copper and nickel) from waste GaN-based LEDs via bioleaching. A process flowsheet encompassing transportation, robotic disassembly, ball milling, bioleaching, solvent extraction/electrowinning, and refining was modeled. Based on mass balance analysis, more than 53 tons of LED waste are required annually to yield 1 kg of gallium alongside substantial copper and nickel co-products. Preliminary techno-economic analysis (TEA) shows an average total cost (ATC) of 6.84 USD/kg metal when costs are allocated by mass-weighted economic value (market price) fraction, corresponding to 6.75 USD/kg for copper, 15.91 USD/kg for nickel, and 470.95 USD/kg for gallium. For gallium, direct operational costs account for more than 70% of the cost. Monte Carlo simulations further quantify cost uncertainties under market price fluctuations. This work represents the first TEA of gallium recovery from GaN-based LEDs and highlights potential pathways for future cost reduction.

36 MATERIALS SCIENCE↗
DOE OSTI2022

Ecosystem service benefits to water users from perennial biomass production

We report although many agree that a transition to renewable energy sources is needed to avoid the climate consequences of continued reliance on fossil sources, price is a barrier. For renewable energy sources, including bioenergy, penetrating energy markets depends on lowering prices to compete with the price of fossil sources, but the tools used in decision making, such as supply curves, exclude non-market benefits from ecosystem services. Here, we extend the economic concept of an economic supply curve to account for ecosystem services co-produced with perennial biomass. We developed three new types of supply curves to visualize the increased supply of biomass (‘sustainable supply’) with sufficient water-quality benefits to offset biomass production costs. Using these tools, we show that the value of water-quality improvements could significantly reduce the break-even price of perennial feedstocks if it were available to farmers. In the most optimistic case, nearly half of potential biomass supply in a large tributary of the Mississippi river basin carried water purification value exceeding the cost of biomass production. Furthermore, adding the value to swimmers and waders offset production cost for over 90% of potential supply. Simulated benefits were context specific. For example, total value for water drinkers peaked at an intermediate level of fertilizer application. Geographically, benefits were highest in the eastern portion of the river basin. This research shows where the sustainable supply is needed and can generate value; the next step is to match this supply with credit buyers. Efforts to internalize the values of ecosystem services into biomass prices could help to meet Biden administration targets to meet 100% of sustainable aviation fuels.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2022

Soil pore architecture and rhizosphere legacy define N 2 O production in root detritusphere

Root detritusphere is one of the most important sources of N 2 O, however, understanding of how N 2 O emission from the detritusphere is influenced by soil properties remains elusive. Here, we evaluated the effects of pore architecture and soil moisture on N 2 O emission during the decomposition of in-situ grown roots of switchgrass, an important bioenergy crop. We combined dual isotope labeling ( 15 C and 15 N) with zymography to gain insights into the location of the microbial N 2 O production in soils with contrasting pore architectures. In the studied soil, the effect of soil pore architecture on N 2 O emissions was 6 times greater than that of soil moisture. Soil dominated by > 30 μm Ø pores (i.e., large-pore soil) had higher chitinase activity than the soil dominated by < 10 μm Ø pores (i.e., small-pore soil), especially near the decomposing roots. The chitinase activity on the decomposing roots was positively correlated with emission of root-derived N 2 O, indicating that N released from root decomposition was an important source of N 2 O. Greater N 2 O and N2 emission was induced by switchgrass roots in soils dominated by the large- compared to the small-pore soils. Here, the microenvironment developed near decomposing roots of the large-pore soil also resulted in positive N 2 O priming. Our study challenged the traditional view on soil moisture as the main factor of N 2 O production. Production and emission of N 2 O was most intensive in microbial activity hotspots (i.e., rhizosphere legacy) in the large pores, where decomposed roots release mineral N as the main N 2 O source.

13C Pulse labeling↗
DOE OSTI2022

A novel sub-pilot-scale direct-contact ultrasonic dehydration technology for sustainable production of distillers dried grains (DDG)

DDG is a major source of protein, calcium, phosphorus, and sulfur is arguably the most important byproduct of the bioethanol industry with increasing demand over the past few years. Reducing energy consumption in the DDG production process and energy recovery from DDG is vital for sustainable bioethanol productions. In this paper, a novel direct-contact multi-frequency, multimode, and modulated (MMM) ultrasonic dryer (US) was developed for the first time and has been applied in dehydration of wet distillers' grain (WDG). Ultrasonic drying (US) was combined with a convective airflow (HA) at different temperatures of 25 (room temperature), 50 and 70 °C to evaluate the impact of US, HA, and US + HA on drying kinetics, activation energy, chemical compositions, microstructure, and color of DDG. Semi-empirical kinetic models were developed and evaluating drying performances showed that the application of ultrasound significantly enhanced the drying rate and decreased the drying time (by 46%), especially at low drying temperatures. The activation energy for moisture removal in the presence of ultrasound was about 50% of that without ultrasound. The final dried distillers' grains product processed by ultrasonic drying had a brighter color, a higher available protein, a higher digestible protein (the lowest acid detergent insoluble crude protein), and a better surface profile with no compromise on minerals and fiber contents.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2023

Mn(III)-mediated bisphenol a degradation: Mechanisms and products

Bisphenol A (BPA) is a high production volume chemical with potential estrogenic effects susceptible to abiotic degradation by MnO 2 . BPA transformation products and reaction mechanisms with MnO 2 have been investigated, but detailed process understanding of Mn(III)-mediated degradation has not been attained. Rapid consumption of BPA occurred in batch reaction vessels with 1 mM Mn(III) and 63.9 ± 0.7% of 1.76 ± 0.02 μmol BPA was degraded in 1 hour at circumneutral pH. BPA was consumed at 1.86 ± 0.09-fold higher rates in vessels with synthetic MnO 2 comprising approximately 13 mol% surface-associated Mn(III) versus surface-Mn(III)-free MnO 2 , and 10–35% of BPA transformation could be attributed to Mn(III) during the initial 10-min reaction phase. High-resolution tandem mass spectrometry (HRMS/MS) analysis detected eight transformation intermediates in reactions with Mn(III), and quantum calculations proposed 14 BPA degradation products, nine of which had not been observed during MnO 2 -mediated BPA degradation, suggesting mechanistic differences between Mn(III)- versus MnO 2 -mediated BPA degradation. Finally, the findings demonstrate that both Mn(III) and Mn(IV) can effectively degrade BPA and indicate that surface-associated Mn(III) increases the reactivity of synthetic MnO 2 , offering opportunities for engineering more reactive oxidized Mn species for BPA removal.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2021

Estrogen depletion alters osteogenic differentiation and matrix production by osteoblasts in vitro

Highlights: • Estrogen depletion accelerates osteoblast differentiation in static culture. • Mechanical stimulation exacerbated the effects of estrogen depletion on osteoblast differentiation. • Estrogen depletion alters osteoblasts capacity to produce a good quality matrix. Recent studies have revealed that the effects of estrogen deficiency are not restricted to osteoclasts and bone resorption, but that bone matrix composition is altered and osteoblasts exhibit an impaired response to mechanical stimulation. In this study, we test the hypothesis that estrogen depletion alters osteogenic differentiation and matrix production by mechanically stimulated osteoblasts in vitro. MC3T3-E1 cells were pre-treated with estrogen for 14 days, after which estrogen was withdrawn or inhibited with Fulvestrant up to 14 days. Fluid shear stress (FSS) was applied using an orbital shaker. Under estrogen depletion in static culture, osteogenic marker (ALP) and gene expression (Runx2) were decreased at 2 and after 7 days of estrogen depletion, respectively. In addition, up to 7 day the inhibition of the estrogen receptor significantly decreased fibronectin expression (FN1) under static conditions. Under estrogen depletion and daily mechanical stimulation, changes in expression of Runx2 occurred earlier (4 days) and by 14 days, changes in matrix production (Col1a1) were reported. We propose that changes in osteoblast differentiation and impaired matrix production during estrogen depletion may contribute to the altered quality of the bone and act as a contributing factor to increased bone fragility in postmenopausal osteoporosis.

60 APPLIED LIFE SCIENCES↗