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At least 1,315 records · Page 73

What the Long-Term Sunspot Record Tells Us About Space Climate

Direct observations of sunspots span the nearly 400 years since the time of Galileo. Dedicated observing programs at several observatories over the last 150 years have provided detailed information not only on the number of sunspots but on their sizes and positions as well. The data acquired by those original observers, and by those who have more recently brought those observations to light, provide important clues about the nature of the solar cycle and its contribution to space climate. The period of the cycle, the equator-ward drift of the active latitudes, the asymmetry between the rise to maximum and the fill to minimum, shifting asymmetries between northern and southern hemisphere activity, the tilt of active regions, and the increasing amplitude of the cycles since the Maunder Minimum are all well established. Other, less well established characteristics such as multi-cycle and short-term periodicities, often depend upon the method of data analysis. The strong correlation between sunspot statistics and other measures of solar activity, coupled with the length of the sunspot record, make these observations extremely valuable for characterizing and understanding space climate.

Hathaway, D. H.↗

Dark matter vs. neutrinos: the effect of astrophysical uncertainties and timing information on the neutrino floor

Future multi-tonne Direct Detection experiments will be sensitive to solar neutrino induced nuclear recoils which form an irreducible background to light Dark Matter searches. Indeed for masses around 6 GeV the spectra of neutrinos and Dark Matter are so similar that experiments are said to run into a neutrino floor, for which sensitivity increases only marginally with exposure past a certain cross section. In this work we show that this floor can be overcome using the different annual modulation expected from solar neutrinos and Dark Matter. Specifically for cross sections below the neutrino floor the DM signal is observable through a phase shift and a smaller amplitude for the time-dependent event rate. This allows the exclusion power to be improved by up to an order of magnitude for large exposures. In addition we demonstrate that, using only spectral information, the neutrino floor exists over a wider mass range than has been previously shown, since the large uncertainties in the Dark Matter velocity distribution make the signal spectrum harder to distinguish from the neutrino background. However for most velocity distributions it can still be surpassed using timing information, and so the neutrino floor is not an absolute limit on the sensitivity of Direct Detection experiments.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Muon tracking in a LiquidO opaque scintillator detector

LiquidO is an innovative radiation detector concept. The core idea is to exploit stochastic light confinement in a highly scattering medium to self-segment the detector volume. In this paper, we demonstrate event-by-event muon tracking in a LiquidO opaque scintillator detector prototype. The detector consists of a 30 mm cubic scintillator volume instrumented with 64 wavelength-shifting fibres arranged in an 8 × 8 grid with a 3.2 mm pitch and read out by silicon photomultipliers. A wax-based opaque scintillator with a scattering length of approximately 0.5 mm is used. The tracking performance of this LiquidO detector is characterised with cosmic-ray muons and the position resolution is demonstrated to be 450 μm per row of fibres. These results highlight the potential of LiquidO opaque scintillator detectors to achieve fine spatial resolution, enabling precise particle tracking and imaging.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Wavelength modulation laser-induced fluorescence for plasma characterization

Laser-Induced Fluorescence (LIF) spectroscopy is an essential tool for probing ion and atom velocity distribution functions (VDFs) in complex plasmas. VDFs carry information about the kinetic properties of species that is critical for plasma characterization. Accurate interpretation of these functions is challenging due to factors such as multicomponent distributions, broadening effects, and background emissions. Our research investigates the use of Wavelength Modulation (WM) LIF to enhance the sensitivity of VDF measurements. Unlike standard Amplitude Modulation (AM) methods, WM–LIF measures the derivative of the LIF signal. This approach makes variations in VDF shape more pronounced. VDF measurements with WM–LIF were investigated with both numerical modeling and experimental measurements. The developed model enables the generation of both WM and AM signals, facilitating comparative analysis of fitting outcomes. Experiments were conducted in a weakly collisional argon plasma with magnetized electrons and non-magnetized ions. Measurements of the argon ion VDFs employed a narrow-band tunable diode laser, which scanned the 4p 4 D 7/2 –3d 4 F 9/2 transition centered at 664.553 nm in vacuum. A lock-in amplifier detected the second harmonic WM signal, which was generated by modulating the laser wavelength with an externally controlled piezo-driven mirror of the diode laser. Finally, our findings indicate that the WM–LIF signal is more sensitive to fitting parameters, allowing for better identification of VDF parameters such as the number of distribution components, their temperatures, and velocities. In addition, WM–LIF can serve as an independent method to verify AM measurements and is particularly beneficial in environments with substantial light noise or background emissions, such as those involving thermionic cathodes and reflective surfaces.

47 OTHER INSTRUMENTATION↗

Constraints on holographic cosmologies from strong lensing systems

We use strongly gravitationally lensed (SGL) systems to put additional constraints on a set of holographic dark energy models. Data available in the literature (redshift and velocity dispersion) is used to obtain the Einstein radius and compare it with model predictions. We found that the ΛCDM is the best fit to the data. Although a preliminary statistical analysis seems to indicate that two of the holographic models studied show interesting agreement with observations, a stringent test lead us to the result that neither of the holographic models are competitive with the ΛCDM. These results highlight the importance of Strong Lensing measurements to provide additional observational constraints to alternative cosmological models, which are necessary to shed some light into the dark universe.

79 ASTRONOMY AND ASTROPHYSICS↗

The mid-infrared luminosity evolution and luminosity function of quasars with WISE and SDSS

We determine the 22 μm luminosity evolution and luminosity function for quasars from a data set of over 20,000 objects obtained by combining flux-limited Sloan Digital Sky Survey optical and Wide field Infrared Survey Explorer mid-infrared data. We apply methods developed in previous works to access the intrinsic population distributions non-parametrically, taking into account the truncations and correlations inherent in the data. We find that the population of quasars exhibits positive luminosity evolution with redshift in the mid-infrared, but with considerably less mid-infrared evolution than in the optical or radio bands. With the luminosity evolutions accounted for, we determine the density evolution and local mid-infrared luminosity function. The latter displays a sharp flattening at local luminosities below ∼10{sup 31} erg s{sup −1} Hz{sup −1}, which has been reported previously at 15 μm for AGN classified as both type 1 and type 2. We calculate the integrated total emission from quasars at 22 μm and find it to be a small fraction of both the cosmic infrared background light and the integrated emission from all sources at this wavelength.

79 ASTRONOMY AND ASTROPHYSICS↗

Two-nucleon higher partial-wave scattering from lattice QCD

We present a determination of nucleon-nucleon scattering phase shifts for ℓ ≥ 0. The S, P, D and F phase shifts for both the spin-triplet and spin-singlet channels are computed with lattice Quantum ChromoDynamics. For ℓ > 0, this is the first lattice QCD calculation using the Lüscher finite-volume formalism. This required the design and implementation of novel lattice methods involving displaced sources and momentum-space cubic sinks. To demonstrate the utility of our approach, the calculations were performed in the SU(3)-flavor limit where the light quark masses have been tuned to the physical strange quark mass, corresponding to m π = m K ≈ 800MeV. In this work, we have assumed that only the lowest partial waves contribute to each channel, ignoring the unphysical partial wave mixing that arises within the finite-volume formalism. This assumption is only valid for sufficiently low energies; we present evidence that it holds for our study using two different channels. Two spatial volumes of V ≈ (3.5fm) 3 and V ≈ (4.6fm) 3 were used. The finite-volume spectrum is extracted from the exponential falloff of the correlation functions. Said spectrum is mapped onto the infinite volume phase shifts using the generalization of the Lüscher formalism for two-nucleon systems.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Effects of Local Environment on the Ultra-Fast Carrier Dynamics of Photo-Excited 2D Transition Metal Dichalcogenides

Layered transition metal dichalcogenides (TMDs) represent a diverse, emerging source of two-dimensional (2D) nanostructures with broad application in optoelectronics and energy. In particular, tungsten disulfide (WS2) is an efficient visible light absorber with relatively high carrier mobilities and catalytic activity towards hydrogen evolution. While explanation of the quantum confinement and excitonic effects governing TMD optoelectronic properties has progressed in recent years, less is known about the ultra-fast photoresponse and carrier dynamics following light excitation. This work utilizes transient absorption spectroscopy, with pump tunability and broadband visible probing, to monitor the carrier dynamics of both CVD-grown monolayer and solution exfoliated WS2. Picosecond-scale features include simultaneous bleaching of excitonic states and a red-shifted absorption spectrum attributed to bandgap renormalization, while free carriers, defect trapped carriers, and recombination signatures are apparent at increasing pico- to nanosecond lifetimes. Features associated with excitons, trions, and photo-excited carriers exhibit strong dependence on local environmental factors. Moisture, oxygen, chemical dopants, and dielectric environment strongly affect the strength and decay lifetimes of these photo-excited species. These results highlight the importance of understanding and controlling these local environmental factors to the rational design and implementation of 2D TMDs optoelectronic device platforms.

2D materials↗

Optical magnetic resonances induced by the interference of reactive components in the near radiation-field zone of atoms in a glow discharge of a mixture of even neon isotopes

Four types of anomalous optical magnetic resonances shifted with respect to the zero magnetic field and with different shapes are found in radiation of a glow discharge in a mixture of even neon isotopes placed in a swept longitudinal magnetic field. This testifies to the manifestation of collective processes of synchronous light emission by oscillators belonging to isotopically different spatially separated atoms in discharge plasma. The origin of resonances is associated with nonstationary interference of reactive fields in the near radiation-field zones of emission of atoms, averaged over the lifetime of the fields (interference), while different types of resonances are associated with different methods of synchronization of the phases of the fields.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Attitudinal Responses to Changes in Noise Exposure in Residential Communities

The purpose of this study is (1) to investigate the current body of knowledge encompassing two related topics: (a) to what extent can we reliably predict the change in people's attitudes in response to an abrupt change in noise exposure, and (b) after the change, is there a decay in the abrupt-change effect whereby people's attitudes slowly shift from their initial reaction to a steady-state value? and (2) to provide recommendations for any future work that may be needed. The literature search located 23 studies relating to one or both of the above topics. These prior studies shed considerable light on the current ability to predict initial reaction and decay effects. The literature makes one point very clear: Great care in both experimental design and data analysis is necessary to produce credible, convincing findings, both in the reanalysis of existing data and for planning future data acquisition and analysis studies. New airport studies must be designed to minimize nuisance variables and avoid past design features that may have introduced sufficient unexplained variance to mask sought after effects. Additionally, the study must be designed to tie in with previous investigations by incorporating similar survey questions and techniques.

Horonjeff, Richard D.↗

Precision Clocks in Space and alpha-Variations

Important developments of both in theoretical and observational cosmology have fueled considerable interest in searches for variations of the fine structure constant. Experimentally, Webb et. al. have found evidence for a cosmological variation of the fine structure constant through an analysis of the absorption lines in galactic halos from quasar-emitted light. Recently developed small ion atomic clocks enable Solar System tests for equivalence principle (EP) violating (alpha)-variations by way of rate-comparisons of three ultra-stable atomic clocks near-to and far-from the sun where gravitational red-shift changes are more than 10(exp 4) larger than in low Earth orbit. No space tests of the EP have been made in nearly 30 years, since the GP-A hydrogen maser reached a 10,000 km apogee confirming EP red-shift predictions ~1 part in 10(exp 4). Today's small ion clocks, nearly 100x more stable and 100x smaller then the GP-A H-maser, could probe for EP violating scalar fields near the sun for mission costs comparable to low Earth orbiters and improve the GP-A sensitivity by 5 to 6 orders of magnitude.

(alpha)-variation↗

Activation of a chloroplast type of fructose bisphosphatase from Chlamydomonas reinhardtii by light-mediated agents

A chloroplast type of fructose-1,6-bisphosphatase, a central regulatory enzyme of photosynthetic carbon metabolism, has been partially purified from Chlamydomonas reinhardtii. Unlike its counterpart from spinach chloroplasts, the algal FBPase showed a strict requirement for a dithiol reductant irrespective of Mg2+ concentration. The enzymes from the two sources resembled each other immunologically, in subunit molecular mass and response to pH. In the presence of dithiothreitol, the pH optimum for both the algal and spinach enzymes shifted from 8.5 to a more physiologic value of 8.0 as the Mg2+ concentration was increased from 1 to 16 mM. At 1 mM Mg2+, a concentration estimated to be close to physiological, the Chlamydomonas FBPase was active only in the presence of reduced thioredoxin and was most active with Chlamydomonas thioredoxin f. Under these conditions, the enzyme showed a pH optimum of 8.0. The data suggest that the Chlamydomonas enzyme resembles its spinach counterpart in most respects, but it has a stricter requirement for reduction and less strict reductant specificity. A comparison of the properties of the FBPases from Chlamydomonas and spinach will be helpful for elucidating the mechanism of the reductive activation of this enzyme.

NASA Discipline Exobiology↗

Low-Threshold Visible-to-Ultraviolet Solid-State Triplet-Fusion Upconversion

Visible-to-ultraviolet (UV) triplet-triplet annihilation (TTA) upconversion is an energy-relevant photon-management strategy that converts visible photons into UV photons capable of driving high-energy photochemical processes. Practical implementation requires solid-state thin films, which often require high excitation power. Here, we demonstrate the first solid-state visible-to-UV TTA upconversion thin-film device, using 1,4-bis((tricyclopentylsilyl)ethynyl)naphthalene (TCPS-NAP) as the annihilator and tris(2-phenylpyridine)iridium(III) (Ir(ppy) 3 ) as the sensitizer on silver. Under incoherent 455 nm excitation, the device exhibits blue-to-UV upconversion with a threshold of 4.8 mW/cm 2 . Using surface plasmons in the planar silver film, we achieve green-to-UV upconversion with a 1.11 eV anti-Stokes shift and 6.9 mW/cm 2 threshold, a 12.2 × threshold enhancement over far-field 532 nm excitation. In solution, TCPS-NAP shows excimer-dominated anti-Stokes emission rather than UV upconversion. These results establish a platform for harvesting low-intensity visible light to drive UV processes while demonstrating that solution-phase screening does not predict solid-state upconversion performance.

Luminescence↗

Photoinduced, reversible phase transitions in all-inorganic perovskite nanocrystals

Significant interest exists in lead trihalides that present the perovskite structure owing to their demonstrated potential in photovoltaic, lasing, and display applications. These materials are also notable for their unusual phase behavior often displaying easily accessible phase transitions. In this work, time-resolved X-ray diffraction, performed on perovskite cesium lead bromide nanocrystals, maps the lattice response to controlled excitation fluence. These nanocrystals undergo a reversible, photoinduced orthorhombic-to-cubic phase transition which is discernible at fluences greater than 0.34 mJ cm -2 through the loss of orthorhombic features and shifting of high-symmetry peaks. This transition recovers on the timescale of 510 ± 100 ps. A reversible crystalline-to-amorphous transition, observable through loss of Bragg diffraction intensity, occurs at higher fluences (greater than 2.5 mJ cm -2 ). These results demonstrate that light-driven phase transitions occur in perovskite materials, which will impact optoelectronic applications and enable the manipulation of non-equilibrium phase characteristics of the broad perovskite material class.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Light polarization sensitive photodetectors with m- and r-plane homoepitaxial ZnO/ZnMgO quantum wells

Homoepitaxial ZnO/(Zn,Mg)O multiple quantum wells (MQWs) grown with m- and r-plane orientations are used to demonstrate Schottky photodiodes sensitive to the polarization state of light. In both orientations, the spectral photoresponse of the MQW photodiodes shows a sharp excitonic absorption edge at 3.48 eV with a very low Urbach tail, allowing the observation of the absorption from the A, B and C excitonic transitions. The absorption edge energy is shifted by ∼30 and ∼15 meV for the m- and r-plane MQW photodiodes, respectively, in full agreement with the calculated polarization of the A, B, and C excitonic transitions. The best figures of merit are obtained for the m-plane photodiodes, which present a quantum efficiency of ∼11%, and a specific detectivity D* of ∼6.4 × 10{sup 10} cm Hz{sup 1/2}/W. In these photodiodes, the absorption polarization sensitivity contrast between the two orthogonal in-plane axes yields a maximum value of (R{sub ⊥}/R{sub ||}){sub max} ∼ 9.9 with a narrow bandwidth of ∼33 meV.

77 NANOSCIENCE AND NANOTECHNOLOGY↗

Calibration of photoelastic modulator based dichrometers: maintaining constant phase across the spectrum

Photoelastic modulators can alter the polarization state of a beam of ultraviolet, visible or infrared photons by means of periodic stress-induced differences in the refractive index of a transparent material that forms the optical element of the device and is isotropic in the absence of stress. Furthermore, they have found widespread application in instruments that characterize or alter the polarization state of a beam in fields as diverse as astronomy, structural biology, materials science and ultraviolet lithography for the manufacture of nano-scale integrated circuits. Measurement of circular dichroism, the differential absorption of left- and right circularly polarized light, and of strain-induced birefringence of optical components are major applications. Instruments using synchrotron radiation and photoelastic modulators with CaF 2 optical elements have extended circular dichroism measurements down to wavelengths of about 130 nm in the vacuum ultraviolet. Maintaining a constant phase shift between two orthogonal polarization states across a spectrum requires that the amplitude of the modulated stress be changed as a function of wavelength. For commercially available photoelastic modulators, the voltage that controls the amplitude of modulation required to produce a specified phase shift, which is a surrogate for the stress modulation amplitude, has been shown to be an approximately linear function of wavelength in the spectral region where the optical element is transparent. But, extrapolations of such straight lines cross zero voltage at a non-zero wavelength, not at zero-wavelength. For modulators with calcium fluoride and fused silica optical elements, the zero-crossing wavelength is always in the spectral region where the optical element of the modulator strongly absorbs the incident radiation, and at a wavelength less than the longest-wavelength apparent resonance deduced from experimental values of the refractive index fit to the Sellmeier equation. Using a model that relates the refractive indices of a stressed optical element to the refractive index of its unstressed state, an expression for the modulator control voltage was derived that closely fits the experimental data. Our result provides a theoretical rational for the apparently linear constant-phase programming voltage, and thus provides theoretical backing for the calibration procedure frequently used for these modulators. Lastly there are other factors that can influence the calibration of a photoelastic modulator, including temperature and atmospheric pressure, are discussed briefly.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Low duty cycle pulsed UV technique for spectroscopy of aluminum monochloride

We present what we believe to be a novel technique to minimize UV-induced damage in experiments that employ second-harmonic generation cavities. The principle of our approach is to reduce the duty cycle of the UV light as much as possible to prolong the lifetime of the used optics. The low duty cycle is achieved by ramping the cavity into resonance for a short time during the experimental cycle when the light is used and tuning it to an off-resonant state otherwise. The necessary fast ramp and length-stabilization control of the cavity is implemented with the FPGA-based STEMlab platform. We demonstrate the utility of this method by measuring the isotope shift of the electronic transition (X 1 Σ ← A 1 Π) in AlCl at 261.5 nm in a pulsed molecular beam experiment.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗