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At least 1,315 records · Page 73

Validating ENDF/B-VIII.1beta2 with LLNL Pulsed-Sphere Neutron-Leakage Spectra [Slides]

This presentation covers noteworthy changes from VIII.1beta0/1 to VIII.1beta2. 6 Li has been fixed (also seen in 7 Li sphere). For 9 Be: we would recommend studying what nuclear data led to an increase in C/E right after peak. For Pb isotopes: we are concerned about new structures introduced after peak. Finally discussed for 239 Pu: Is it worth improving right now?

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Characterization of a mixed high-energy spallation neutron–proton field using monoisotopic activation detectors

In this paper, we used monoisotopic Co, Au, and Bi threshold activation detectors to characterize the high-energy ( > 5 MeV) portion of a mixed spallation neutron–proton (n/p) field. The field was produced by irradiating the natural uranium target–blanket subcritical assembly Quinta with 660-MeV protons from Phasotron accelerator at the Joint Institute for Nuclear Research (JINR) in Dubna. Experimental yields of the (n,x) and (p,x) reactions were compared to the calculated reaction rates, which represent the convolution of particle flux and reaction cross section. The flux was simulated using the radiation transport code MCNPX 2.7.0, and the cross sections were extracted from the following three sources: the intranuclear cascade model INCL4.2, the phenomenological spherical optical model from TALYS-1.8, and the evaluated nuclear data file TENDL-2015. We show that, in most cases, the evaluated data provide a closer agreement with the experimental data in comparison with INCL4.2 model, which is an integral part of MCNPX. Finally, our results bring a contribution to those fields of physics research that utilize computer prediction of neutron generation in the energy range of tens to hundreds MeV, such as the medical radioisotope production, radiation shielding of spallation neutron sources, and nuclear transmutation in accelerator-driven systems.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

MCNP6.1 k -Eigenvalue Sensitivity Capability: A User’s Guide

MCNP6.1 is the first production version of MCNP to include the ability to compute sensitivity coefficients of the effective multiplication k for nuclear data. These types of calculations are useful for code validation and the development of benchmark suites applicable to specific set of applications, for the design of critical (integral) experiments, and uncertainty quantification.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Neutron Absorber Plate Characterization Plan for Criticality Experiments Design [Slides]

The goal of this presentation is to show the feasibility of performing a critical experiment with a B 4 C/Aluminum alloy neutron absorber plate. The motivation of this experiment is to provide integral data on modern neutron absorber product “Boralcan” by Rio Tinto. In 2020, used in about 20% of spent fuel pools in the US, and in casks for storage and transportation in the US and in Europe. The added value of this experiment: Neutron absorber plate modeling method verification: homogeneous or not, a lot of potential savings by relaxing boron loading credit limits. No available critical benchmark involving Boralcan, other boron-related experiments are relatively old. Nuclear data validation for B, C, and Al in the form of B 4 C in Al matrix.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Summary: Verification of the ENDF/B-VII.1 and VIII.0 AMPX 1597-group Libraries for Advanced Reactor Analysis

The SCALE/AMPX multigroup (MG) cross section processing procedure has been updated to minimize reactivity differences for various advanced thermal and fast reactor designs, as observed for the current MG libraries, resulting in excellent agreement between the calculations with the new MG libraries and the continuous-energy reference calculations. The SCALE MG calculations are widely applied to thermal spectrum light-water reactor systems, as well as fast spectrum metallic systems. Due to growing interest from industry and regulators in applying SCALE for the design of fast spectrum reactors—both sodium and molten salt—it was desirable to review and improve the SCALE/AMPX procedure for unresolved resonance self-shielded data and high-energy neutron spectra. The data were improved by generating MG unresolved resonance data based on the analytic probability table method with the narrow resonance approximation and by using very fine and intermediate group structures that are typical for fast system analysis. This study focused on verifying the improved SCALE/AMPX MG cross section processing procedure and the new AMPX 1597-group library with the ENDF/B-VII.1 and VIII.0 evaluated nuclear data. The verification was made by performing reaction rate analysis and benchmark calculations for various thermal and fast reactor systems. Results indicate that the improved SCALE/AMPX MG cross section processing and libraries provide excellent results for advanced reactor analysis.

Kim, Kang Seog↗

Verification of the ENDF/B-VII.1 and VIII.0 AMPX 1597-Group Libraries for Advanced Reactor Analysis

The SCALE/AMPX multigroup (MG) cross section processing procedure has been updated to minimize reactivity differences for various advanced thermal and fast reactor designs, as observed for the current MG libraries, resulting in excellent agreement between the calculations with the new MG libraries and the continuous-energy reference calculations. The SCALE MG calculations are widely applied to thermal spectrum light-water reactor systems, as well as fast spectrum metallic systems. Due to growing interest from industry and regulators in applying SCALE for the design of fast spectrum reactors—both sodium and molten salt—it was desirable to review and improve the SCALE/AMPX procedure for unresolved resonance self-shielded data and high-energy neutron spectra. The data were improved by generating MG unresolved resonance data based on the analytic probability table method with the narrow resonance approximation and by using very fine and intermediate group structures that are typical for fast system analysis. This study focused on verifying the improved SCALE/AMPX MG cross section processing procedure and the new AMPX 1597-group library with the ENDF/B-VII.1 and VIII.0 evaluated nuclear data. The verification was made by performing reaction rate analysis and benchmark calculations for various thermal and fast reactor systems. Results indicate that the improved SCALE/AMPX MG cross section processing and libraries provide excellent results for advanced reactor analysis.

Kim, Kang Seog↗

SCALE capabilities for high temperature gas-cooled reactor analysis

The SCALE code system’s ability to address stochastic distributions of fuel particles within a graphite matrix has been revisited in both multigroup (MG) features and continuous-energy (CE) Monte Carlo methods. Furthermore, this paper describes current and emergent SCALE capabilities within the CSAS sequence to address double-heterogeneous systems and presents verification and validation studies of these methods and data. Good agreement was obtained for a high temperature gas-cooled reactor (HTGR) fuel pebble model between CSAS MG eigenvalue calculations and corresponding CE reference solutions. Code-to-code comparisons for this HTGR pebble model showed good agreement of CSAS-KENO and CSAS-Shift CE calculations and the Serpent and MCNP codes in terms of eigenvalues and reaction rate ratios. Validation studies based on two HTGR experiments resulted in good agreement between MG and CE results, as well as between experiment and calculation, although the level of agreement was significantly influenced by the applied ENDF/B nuclear data library.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

FLUKA simulation validation to measure the beam energy of a cyclotron

FLUKA is a fully integrated particle physics MonteCarlo simulation package which has many applications in high energy experimental physics and engineering. When using a cyclotron for medical radionuclide production, it is important to know that the beam energy is suitable to cause the intended nuclear reaction and minimize unwanted impurities. Here, this work focuses on the comparison of FLUKA as a tool to measure the beam energy of a cyclotron with experimental results using the method of stacked copper foils interspaced by an aluminum degrader. We compared two methods to determine the activity ratio: determining the activity in each foil using the experimentally measured cross-sections from the National Nuclear Data Center (NNDC) cross-section data and calculating the activity in the two Cu foils using the FLUKA program. These results were compared to those reported by Gagnon et al., 2011. The FLUKA results gave energy measurements that were different than the true energy by a percentage in the range of 2.4% to 13%, suggesting that FLUKA is not recommended for pre-calculating the cyclotron beam energy using these low Z materials without experimental confirmation. It also confirms that the experimental cross-section data from the NNDC database is superior for this application giving energy values that ranged from 0.1% to 1.6% from the true energy.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Serpent and MCNP Calculations of the Energy Deposition in the Transformational Challenge Reactor

This paper focuses on the calculation of the energy deposition in the Transformational Challenge Reactor by two major Monte Carlo codes: Serpent and MCNP. The first software computation relies on Kinetic Energy Released per unit Mass (KERMA) factors while the second one relies on Q-values. The results from these two independent computation methodologies are in very good agreement; however, Serpent runs much faster than MCNP (for the same computational model) and allows for a detailed energy deposition distribution from a 1-mm-side square mesh with a relative statistical error between 0.5% and 1%. This detailed energy deposition is suitable for multiphysics analyses aimed at design optimizations. In order to calculate the energy deposition, Serpent needs enhanced ACE files (distributed by the software developers). Unlike other Monte Carlo software that uses inputs based on Python or Java languages, the Serpent input syntax is very similar to that of MCNP; a Python script can convert a MCNP input to a Serpent input in seconds. For simulations not requiring the calculation of the energy deposition, Serpent can also read nuclear data from MCNP ACE files, which eventually improves the comparison of the results of the two codes.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Stereolithographic geometry model of the IBR-2M experimental facility

The IBR-2M is a fast research reactor that operates in supercritical condition for ∼ 800 μs every 200 ms. Two reflector parts in nickel rotate in opposite directions generating 1.8 GWth peak power when they align with the fuel zone changing the reactor status from deep subcritical to supercritical. The reactor core uses high-enriched plutonium fuel and is cooled by sodium. This reactor has been modeled by MCNP and SERPENT computer programs. The MCNP model uses combinatorial geometry, whereas the SERPENT model employs the Stereolithographic (STL) geometry representation that can be used by 3D printers. The STL geometry was constructed using the CUBIT computer program. The CUBIT program was also used for a three-dimensional visualization of the Monte Carlo models. SERPENT and MCNP models use the same geometry, material specifications, and nuclear data. The latter are based on the ENDF/B-7.0 library. SERPENT and MCNP using same geometry and same material specifications produce similar k{sub eff} values within 120 pcm.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Benchmark Progress towards TREAT M8CAL Core Loading to Support Validation of TREAT Operations

Benchmark experiment data is necessary to validate modeling and simulation activities to support Transient Reactor Experiment Test (TREAT) Facility restart and operations. Key measurements of interest include criticality, control rod worth, excess reactivity, and shutdown margin for varying core loading sizes. Benchmark evaluations are being developed according the guidelines provided in the International Handbook of Evaluated Reactor Physics Benchmark Experiments (IRPhEP Handbook) that can also support advanced modeling and simulation activities, new experiment design for advanced reactors and accident tolerant fuel, and potential low-enriched uranium conversion of the TREAT reactor. This summary discusses development activities supporting a benchmark evaluation of the TREAT M8CAL core loading, which will be submitted for peer-review and publication in the IRPhEP Handbook with the identifier TREAT-FUND-RESR-002. Detailed models of TREAT were developed and evaluated to prepare benchmark models of the minimum critical mass configuration. Calculations were performed using MCNP6.1 with ENDF/B-VII.1 nuclear data libraries. Discussion of results.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Benchmark Development for TREAT Minimum Critical Mass Core Loading to Support Validation of TREAT Operations

Benchmark experiment data is necessary to validate modeling and simulation activities to support Transient Reactor Experiment Test (TREAT) Facility restart and operations. Key measurements of interest include criticality, control rod worth, excess reactivity, and shutdown margin for varying core loading sizes. Benchmark evaluations are being developed according the guidelines provided in the International Handbook of Evaluated Reactor Physics Benchmark Experiments (IRPhEP Handbook) that can also support advanced modeling and simulation activities, new experiment design for advanced reactors and accident tolerant fuel, and potential low-enriched uranium conversion of the TREAT reactor. This summary discusses development activities supporting a benchmark evaluation of the TREAT minimum critical mass core loading, which will be submitted for peer-review and publication in the IRPhEP Handbook with the identifier TREAT-FUND-RESR-001. Detailed models of TREAT were developed and evaluated to prepare benchmark models of the minimum critical mass configuration. Calculations were performed using MCNP6.1 with ENDF/B-VII.1 nuclear data libraries. Discussion of results.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Neutron Activation Self-Shielding Factors for Common Dosimetry Foils in an ACRR Equivalent Environment

The results of a computational analysis of self-shielding factors are presented. The analysis highlights the total self-shielding, which is a combination of energy and spatial self-shielding, associated with different neutron detection materials. The Monte Carlo N-Particle (MCNP) transport code was used in conjunction with the Evaluated Nuclear Data File (ENDF) and the International Reactor Dosimetry and Fusion Files (IRDFF). This analysis was done with neutron activation analysis in mind, and therefore is modeled and presented in a similar fashion.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Fission In R-Process Elements

The goal of the FIRE topical collaboration in nuclear theory is to determine the astrophysical conditions of the rapid neutron capture process (r-process), which is responsible for the formation of heavy elements. This will be achieved by including in r-process simulations the most advanced models of fission (spontaneous, neutron-induced, β-delayed) that have been developed at LLNL and LANL. The collaboration is composed of LLNL (lead) and LANL for fission work, BNL for nuclear data management, and the university of Notre Dame and North Carolina State University for r -process simulations. Under DOE/NNSA agreement, both universities receive funds from DOE Office of Science, while national laboratories receive funds directly from NA221.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Calculating infinite-medium α-eigenvalue spectra with Monte Carlo using a transition rate matrix method

The time-dependent behavior of the energy spectrum in neutron transport was investigated with a formulation, based on continuous-time Markov processes, for computing α eigenvalues and eigenvectors in an infinite medium. In this study, a research Monte Carlo code called “TORTE” (To Obtain Real Time Eigenvalues) was created and used to estimate elements of a transition rate matrix. TORTE is capable of using both multigroup and continuous-energy nuclear data, and verification was performed. Eigenvalue spectra for infinite homogeneous mixtures were obtained, and an eigenfunction expansion was used to investigate transient behavior of the neutron energy spectrum.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

UO{sub 2} and PuO{sub 2} utilization in high temperature engineering test reactor with helium coolant

High temperature engineering test reactor (HTTR) is one of high temperature gas cooled reactor (HTGR) types which has been developed by Japanese Atomic Energy Research Institute (JAERI). The HTTR is a graphite moderator, helium gas coolant, 30 MW thermal output and 950 °C outlet coolant temperature for high temperature test operation. Original HTTR uses UO{sub 2} fuel. In this study, we have evaluated the use of UO{sub 2} and PuO{sub 2} in form of mixed oxide (MOX) fuel in HTTR. The reactor cell calculation was performed by using SRAC 2002 code, with nuclear data library was derived from JENDL3.2. The result shows that HTTR can obtain its criticality condition if the enrichment of {sup 235}U in loaded fuel is 18.0% or above.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Fission In R-process Elements (FY20 Q2 Quarterly Report)

The goal of the FIRE topical collaboration in nuclear theory is to determine the astrophysical conditions of the rapid neutron capture process (r-process), which is responsible for the formation of heavy elements. This will be achieved by including in r-process simulations the most advanced models of fission (spontaneous, neutron-induced, β-delayed) that have been developed at LLNL and LANL. The collaboration is composed of LLNL (lead) and LANL for fission work, BNL for nuclear data management, and the university of Notre Dame and North Carolina State University for r-process simulations. Under DOE/NNSA agreement, both universities receive funds from DOE Office of Science, while national laboratories receive funds directly from NA221.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Fission In R-process Elements (Q4 FY2020 Quarterly Report)

The goal of the FIRE topical collaboration in nuclear theory is to determine the astrophysical conditions of the rapid neutron capture process (r-process), which is responsible for the formation of heavy elements. This will be achieved by including in r-process simulations the most advanced models of fission (spontaneous, neutron-induced, β-delayed) that have been developed at LLNL and LANL. The collaboration is composed of LLNL (lead) and LANL for fission work, BNL for nuclear data management, and the university of Notre Dame and North Carolina State University for r-process simulations. Under DOE/NNSA agreement, both universities receive funds from DOE Office of Science, while national laboratories receive funds directly from NA221.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗