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Remote Sensing of Aerosol and Non-Aerosol Absorption

Remote sensing of aerosol from the new satellite instruments (e.g. MODIS from Terra) and ground based radiometers (e.g. the AERONET) provides the opportunity to measure the absorption characteristics of the ambient undisturbed aerosol in the entire atmospheric column. For example Landsat and AERONET data are used to measure spectral absorption of sunlight by dust from West Africa. Both Application of the Landsat and AERONET data demonstrate that Saharan dust absorption of solar radiation is several times smaller than the current international standards. This is due to difficulties of measuring dust absorption in situ, and due to the often contamination of dust properties by the presence of air pollution or smoke. We use the remotely sensed aerosol absorption properties described by the spectral sin le scattering albedo, together with statistics of the monthly optical thickness for the fine and coarse aerosol derived from the MODIS data. The result is an estimate of the flux of solar radiation absorbed by the aerosol layer in different regions around the globe where aerosol is prevalent. If this aerosol forcing through absorption is not included in global circulation models, it may be interpreted as anomalous absorption in these regions. In a preliminary exercise we also use the absorption measurements by AERONET, to derive the non-aerosol absorption of the atmosphere in cloud free conditions. The results are obtained for the atmospheric windows: 0.44 microns, 0.66 microns, 0.86 microns and 1.05 microns. In all the locations over the land and ocean that were tested no anomalous absorption in these wavelengths, was found within absorption optical thickness of +/- 0.005.

Kaufman, Y. J.↗

Airborne Sunphotometer Studies of Aerosol Properties and Effects, Including Closure Among Satellite, Suborbital Remote, and In situ Measurements

Airborne sunphotometry has been used to measure aerosols from North America, Europe, and Africa in coordination with satellite and in situ measurements in TARFOX (1996), ACE-2 (1997), PRIDE (2000), and SAFARI 2000. Similar coordinated measurements of Asian aerosols are being conducted this spring in ACE-Asia and are planned for North American aerosols this summer in CLAMS. This paper summarizes the approaches used, key results, and implications for aerosol properties and effects, such as single scattering albedo and regional radiative forcing. The approaches exploit the three-dimensional mobility of airborne sunphotometry to access satellite scenes over diverse surfaces (including open ocean with and without sunglint) and to match exactly the atmospheric layers sampled by airborne in situ measurements and other radiometers. These measurements permit tests of the consistency, or closure, among such diverse measurements as aerosol size-resolved chemical composition; number or mass concentration; light extinction, absorption, and scattering (total, hemispheric back and 180 deg.); and radiative fluxes. In this way the airborne sunphotometer measurements provide a key link between satellite and in situ measurements that helps to understand any discrepancies that are found. These comparisons have led to several characteristic results. Typically these include: (1) Better agreement among different types of remote measurements than between remote and in situ measurements. (2) More extinction derived from transmission measurements than from in situ measurements. (3) Larger aerosol absorption inferred from flux radiometry than from in situ measurements. Aerosol intensive properties derived from these closure studies have been combined with satellite-retrieved fields of optical depth to produce fields of regional radiative forcing. We show results for the North Atlantic derived from AVHRR optical depths and aerosol intensive properties from TARFOX and ACE-2. Companion papers show analogous, preliminary results for Asian-Pacific aerosols and results of SAFARI-2000 closure studies on African aerosols.

Russlee, Philip B.↗

The 1998-2000 SHADOZ (Southern Hemisphere ADditional Ozonesondes) Tropical Ozone Climatology: Comparison with TOMS and Ground-Based Measurements

A network of 10 southern hemisphere tropical and Subtropical stations, designated the Southern Hemisphere ADditional OZonesondes, (SHADOZ) project and established from operational sites, provided over 1000 ozone profiles during the period 1998-2000. Balloon-borne electrochemical concentration cell (ECC) ozonesondes, combined with standard radiosondes for pressure, temperature and relative humidity measurements, collected profiles in the troposphere and lower- to mid-stratosphere at: Ascension Island; Nairobi, Kenya; Irene, South Africa: Reunion Island, Watukosek Java; Fiji; Tahiti; American Samoa; San Cristobal, Galapagos; Natal, Brazil.

Thompson, Anne M.↗

Importance of the Annual Cycles of SST and Solar Irradiance for Circulation and Rainfall: A Climate Model Simulation Study

Annual cycle of climate and precipitation is related to annual cycle of sunshine and sea-surface temperatures. Understanding its behavior is important for the welfare of humans worldwide. For example, failure of Asian monsoons can cause widespread famine and grave economic disaster in the subtropical regions. For centuries meteorologists have struggled to understand the importance of the summer sunshine and associated heating and the annual cycle of sea-surface temperatures (SSTs) on rainfall in the subtropics. Because the solar income is pretty steady from year to year, while SSTs depict large interannual variability as consequence of the variability of ocean dynamics, the influence of SSTs on the monsoons are better understood through observational and modeling studies whereas the relationship of annual rainfall to sunshine remains elusive. However, using NASA's state of the art climate model(s) that can generate realistic climate in a computer simulation, one can answer such questions. We asked the question: if there was no annual cycle of the sunshine (and its associated land-heating) or the SST and its associated influence on global circulation, what will happen to the annual cycle of monsoon rains? By comparing the simulation of a 4-year integration of a baseline Control case with two parallel anomaly experiments: 1) with annual mean solar and 2) with annual mean sea-surface temperatures, we were able to draw the following conclusions: (1) Tropical convergence zone and rainfall which moves with the Sun into the northern and southern hemispheres, specifically over the Indian, African, South American and Australian regions, is strongly modulated by the annual cycles of SSTs as well as solar forcings. The influence of the annual cycle of solar heating over land, however, is much stronger than the corresponding SST influence for almost all regions, particularly the subtropics; (2) The seasonal circulation patterns over the vast land-masses of the Northern Hemisphere at mid and high latitudes also get strongly influenced by the annual cycles of solar heating. The SST influence is largely limited to the oceanic regions of these latitudes; (3) The annual mode of precipitation over Amazonia has an equatorial regime revealing a maxima in the month of March associated with SST, and another maxima in the month of January associated with the solar annual cycles, respectively. The baseline simulation, which has both annual cycles, depicts both annual modes and its rainfall is virtually equal to the sum of those two modes; (4) Rainfall over Sahelian-Africa is significantly reduced (increased) in simulations lacking (invoking) solar irradiation with (without) the annual cycle. In fact, the dominant influence of solar irradiation emerges in almost all monsoonal-land regions: India, Southeast Asia, as well as Australia. The only exception is the Continental United States, where solar annual cycle shows only a relatively minor influence on the annual mode of rainfall.

Sud, Yogesh C.↗

Enhancement of Tropical Land Cover Mapping with Wavelet-Based Fusion and Unsupervised Clustering of SAR and Landsat Image Data

The characterization and the mapping of land cover/land use of forest areas, such as the Central African rainforest, is a very complex task. This complexity is mainly due to the extent of such areas and, as a consequence, to the lack of full and continuous cloud-free coverage of those large regions by one single remote sensing instrument, In order to provide improved vegetation maps of Central Africa and to develop forest monitoring techniques for applications at the local and regional scales, we propose to utilize multi-sensor remote sensing observations coupled with in-situ data. Fusion and clustering of multi-sensor data are the first steps towards the development of such a forest monitoring system. In this paper, we will describe some preliminary experiments involving the fusion of SAR and Landsat image data of the Lope Reserve in Gabon. Similarly to previous fusion studies, our fusion method is wavelet-based. The fusion provides a new image data set which contains more detailed texture features and preserves the large homogeneous regions that are observed by the Thematic Mapper sensor. The fusion step is followed by unsupervised clustering and provides a vegetation map of the area.

LeMoigne, Jacqueline↗

TOMS Tropical Tropospheric Ozone Data Sets at the University of Maryland Website

Since 1997, shortly after the launch of the Earth-Probe TOMS (Total Ozone Mapping Spectrometer) satellite instrument, we have been processing data in near-real time to post maps of tropical tropospheric ozone at a website: metosrv2.umd.edu/-tropo. Daily, 3-day and 9-day averages of tropical tropospheric ozone column depth (TTO) are viewable from 10N to 10S. Data can be downloaded (running 9-day means) from 20N-30S. Pollution events are trackable along with dynamically-induced variations in tropospheric ozone column. TOMS smoke aerosol (toms.gsfc.nasa.gov) can be used to interpret biomass burning ozone, as for example, during the extreme ozone and smoke pollution period during the ENSO-related fires of August November 1997. During that time plumes of ozone and smoke were frequently decoupled and ozone from Indonesian fires and from Africa merged in one large feature by late October 1997. In addition to the Earth-Probe TOMS record, data as half-month averages and as daily 9-day means from the Nimbus 7 TOMS instrument are at the metosrv2.umd.edu/-tropo website. A guide to the website and examples of ozone time-series and maps will be shown.

Kochhar, A. K.↗

Highlights from the 1998-2000 SHADOZ (Southern Hemisphere Additional Ozonesondes) Satellite Validation Project

There are three years of data (more than 1000 individual ozone profiles) available from a network of 10 southern hemisphere tropical and subtropical stations, designated the Southern Hemisphere ADditional OZonesondes (SHADOZ) project. Since late 1999, a tropical station in the northern hemisphere (Paramaribo, Surinam; lat/long) joined SHADOZ, providing coordinated weekly ozone and radiosonde data from the surface to approx. 7 hPa for satellite validation, process studies, and model evaluation. Profiles are also collected at: Ascension Island; Nairobi, Kenya; Irene, South Africa; R (union Island; Watukosek, Java; Fiji; Tahiti; American Samoa; San Cristobal, Galapagos; Natal, Brazil. The archive, station characteristics and photos are available at http://code9l6.gsfc.nasa.gov/Data_ services/shadoz>. SHADOZ ozone time-series and profiles in 1998-2000 display highly variable tropospheric ozone, a zonal wave-one pattern in total (and tropospheric) column ozone, and signatures of the Quasi-Biennial Oscillation (QBO) in stratospheric ozone. Total, stratospheric and tropospheric column ozone amounts peak between August and November and are lowest between March and May. Integrated total ozone column amounts from the sondes are lower than independent measurements from a ground-based network and from the TOMS (Total Ozone Mapping Spectrometer) satellite (version 7 data).

Witte, J. C.↗

Latent Heating Retrievals Using the TRMM Precipitation Radar: A Multi-Seasonal Study

Rainfall is a key link in the hydrologic cycle and is a primary heat source for the atmosphere. The vertical distribution of latent heat release, which is accompanied by rainfall, modulates the large-scale circulations of the tropics and in turn can impact midlatitude weather. This latent heat release is a consequence of phase changes between vapor, liquid, and solid water. Present largescale weather and climate models can simulate latent heat release only crudely, thus reducing their confidence in predictions on both global and regional scales. This paper represents the first attempt to use NASA Tropical Rainfall Measuring Mission (TRMM) rainfall information to estimate the four-dimensional structure of global monthly latent heating profiles over the global tropics from December 1997 to October 2000. The Goddard Convective-Stratiform. Heating (CSH) algorithm and TRMM precipitation radar data are used for this study. We will examine and compare the latent heating structures between 1997-1998 (winter) ENSO and 1998-2000 (non-ENSO). We will also examine over the tropics. The seasonal variation of heating over various geographic locations (i.e., oceanic vs continental; Indian oceans vs west Pacific; Africa vs S. America) will be also examined and compared. In addition, we will examine the relationship between latent heating (max heating level) and SST. The period of interest also coincides with several TRMM field campaigns that recently occurred over the South China Sea in 1998 (SCSMEX), Brazil in 1999 (TRMM-LBA), and in the central Pacific in 1999 (KWAJEX). Sounding diagnosed Q1 budgets from these experiments could provide a means of validating the retrieved profiles of latent heating from the CSH algorithm.

Tao, Wei-Kuo↗

Precipitation Processes Derived from TRMM Satellite Data, Cloud Resolving Model and Field Campaigns

Rainfall is a key link in the hydrologic cycle and is a primary heat source for the atmosphere. The vertical distribution of latent-heat release, which is accompanied by rainfall, modulates the large-scale circulations of the tropics and in turn can impact midlatitude weather. This latent heat release is a consequence of phase changes between vapor, liquid. and solid water. Present large-scale weather and climate models can simulate cloud latent heat release only crudely thus reducing their confidence in predictions on both global and regional scales. In this paper, NASA Tropical Rainfall Measuring (TRMM) precipitation radar (PR) derived rainfall information and the Goddard Convective and Stratiform Heating (CSH) algorithm used to estimate the four-dimensional structure of global monthly latent heating and rainfall profiles over the global tropics from December 1997 to October 2000. Rainfall latent heating and radar reflectively structure between ENSO (1997-1998 winter) and non-ENSO (1998-1999 winter) periods are examined and compared. The seasonal variation of heating over various geographic locations (i.e. Indian ocean vs west Pacific; Africa vs S. America) are also analyzed. In addition, the relationship between rainfall latent heating maximum heating level), radar reflectively and SST are examined.

Tao, W.-K.↗

Combining New Satellite Tools and Models to Examine Role of Mesoscale Interactions in Formation and Intensification of Tropical Cyclones

The objective of this research is to start filling the mesoscale gap to improve understanding and probability forecasts of formation and intensity variations of tropical cyclones. Sampling by aircraft equipped to measure mesoscale processes is expensive, thus confined in place and time. Hence we turn to satellite products. This paper reports preliminary results of a tropical cyclone genesis and early intensification study. We explore the role of mesoscale processes using a combination of products from TRMM, QuikSCAT, AMSU, also SSM/I, geosynchronous and model output. Major emphasis is on the role of merging mesoscale vortices. These initially form in midlevel stratiform cloud. When they form in regions of lowered Rossby radius of deformation (strong background vorticity) the mesoscale vortices can last long enough to interact and merge, with the weaker vortex losing vorticity to the stronger, which can then extend down to the surface. In an earlier cyclongenesis case (Oliver 1993) off Australia, intense deep convection occurred when the stronger vortex reached the surface; this vortex became the storm center while the weaker vortex was sheared out as the major rainband. In our study of Atlantic tropical cyclones originating from African waves, we use QuikSCAT to examine surface winds in the African monsoon trough and in the vortices which move westward off the coast, which may or may not undergo genesis (defined by NHC as reaching TD, or tropical depression, with a west wind to the south of the surface low). We use AMSU mainly to examine development of warm cores. TRMM passive microwave TMI is used with SSM/I to look at the rain structure, which often indicates eye formation, and to look at the ice scattering signatures of deep convection. The TRMM precipitation radar, PR, when available, gives precipitation cross sections. So far we have detailed studies of two African-origin cyclones, one which became severe hurricane Floyd 1999, and the other reached TD2 in June 2000 and then died out. The atmosphere off West African is dry and stable. It becomes less so between June and September, as the SST and convection heat up. QuikSCAT shows the African monsoon trough and shear zone extend westward over the ocean to nearly 30 degrees West. The evidence is strong that the two cyclones had in common multiple midlevel mergers, which extended to the surface keeping the surface vortex strong. These continued until both systems were designated TD's by NHC. In the June 2000 case, the main reason for failure was the lower SST and dry, stable atmosphere. This is shown by the comparison of the equivalent potential temperature maps and profiles with those from pre-Floyd. In the vortex which became Floyd, QuikSCAT shows continuous importation of high theta e (warm, moist) air from the south. From September 2-8, this air flowed around the vortex center, building up a high theta-e pool to the north. Then late on September 9, a 100-km wide jet of high theta-e air penetrated the vortex core, a major convective burst' was observed, and an intensifying, more elevated warm core was seen on AMSU. Rapid pressure fall and wind intensification were underway by 0000 UTC on September 10. Floyd became a Hurricane at 1200 UTC on Sept 10, 1999, with successive convective bursts running the hurricane thermodynamic engine by intensifying the warm core. TD2 was a strong African vortex, sustained by moderate convection (up to about 12.5 km) offshore of Africa. It peaked on June 23, showing an apparent "eye" on passive microwave composites. However, it could not assemble the ingredients for a convective burst. Thus it failed to get the thermodynamic hurricane engine going before it moved too far west of the region of lowered Rossby radius. By June 26, cloud systems were dying out. On June 25, a surface vortex was no longer seen on QuikSCAT, although one continued above the surface on model profiles until June 27. One of our main findings so far is showing the role of the mesoscale vortex interactions in sustaining some African vortices far out in to the mid Atlantic, where under adequate thermal/moisture conditions the hurricane heat engine can sometimes be started. We are working on similar studies of Cindy and Irene 1999. Cindy illustrates a case of wind shear working against an early-stage hurricane heat engine, while Irene formed from a Caribbean wave. An enormous value of combinations of satellite tools is that tropical cyclones can be studied in all parts of the global oceans where they occur. Detailed studies like ours are labor intensive but many statistical studies can be based on physical postulates developed. There are other new tools such as MODIS on TERRA of the Earth Observing System (EOS) which can be used to study the microphysics of tropical cyclones world wide, in particular to investigate the presence of mixed phase and the impact of atmospheric aerosols on the hydrometeor structure and rainfall from tropical cyclones.

Simpson, Joanne↗

STS-109 Flight Day 11 Highlights

On the 11th day of the STS-109 mission, Commander Scott Altman, Pilot Duane Carey, Payload Commander John Grunsfeld, and Mission Specialists Nancy Currie, James Newman, Richard Linnehan, and Michael Massimino are seen answering questions from students in an on-orbit interview. Various shots of the Earth are shown as Columbia orbits over the north of the Australian coast, the west coast of Mexico, Madagascar and the southern Indian Ocean, and the Atlantic coast of Africa.

Source record↗

Fires and Smoke Observed from the Earth Observing System MODIS Instrument: Products, Validation, and Operational Use

The MODIS sensor, launched on NASA's Terra satellite at the end of 1999, was designed with 36 spectral channels for a wide array of land, ocean, and atmospheric investigations. MODIS has a unique ability to observe fires, smoke, and burn scars globally. Its main fire detection channels saturate at high brightness temperatures: 500 K at 4 microns and 400 K at 11 microns, which can only be attained in rare circumstances at the I kin fire detection spatial resolution. Thus, unlike other polar orbiting satellite sensors with similar thermal and spatial resolutions, but much lower saturation temperatures (e.g. AVHRR and ATSR), MODIS can distinguish between low intensity ground surface fires and high intensity crown forest fires. Smoke column concentration over land is for the first time being derived from the MOMS solar channels, extending from 0.41 microns to 2.1 microns. The smoke product has been provisionally validated both globally and regionally over southern Africa and central and south America. Burn scars are observed from MODIS even in the presence of smoke, using the 1.2 to 2.1 micron channels. MODIS burned area information is used to estimate pyrogenic emissions. A wide range of these fire and related products and validation are demonstrated for the wild fires that occurred in northwestern United States in the summer of 2000. The MODIS rapid response system and direct broadcast capability is being developed to enable users to obtain and generate data in near real time. It is expected that health and land management organizations will use these systems for monitoring the occurrence of fires and the dispersion of smoke within two to six hours after data acquisition.

Kaufman, Y. J.↗

Large-Scale Air Mass Characteristics Observed Over the Remote Tropical Pacific Ocean During March-April 1999: Results from PEM-Tropics B Field Experiment

Eighteen long-range flights over the Pacific Ocean between 38 S to 20 N and 166 E to 90 W were made by the NASA DC-8 aircraft during the NASA Pacific Exploratory Mission (PEM) Tropics B conducted from March 6 to April 18, 1999. Two lidar systems were flown on the DC-8 to remotely measure vertical profiles of ozone (O3), water vapor (H2O), aerosols, and clouds from near the surface to the upper troposphere along their flight track. In situ measurements of a wide range of gases and aerosols were made on the DC-8 for comprehensive characterization of the air and for correlation with the lidar remote measurements. The transition from northeasterly flow of Northern Hemispheric (NH) air on the northern side of the Intertropical Convergence Zone (ITCZ) to generally easterly flow of Southern Hemispheric (SH) air south of the ITCZ was accompanied by a significant decrease in O3, carbon monoxide, hydrocarbons, and aerosols and an increase in H2O. Trajectory analyses indicate that air north of the ITCZ came from Asia and/or the United States, while the air south of the ITCZ had a long residence time over the Pacific, perhaps originating over South America several weeks earlier. Air south of the South Pacific Convergence Zone (SPCZ) came rapidly from the west originating over Australia or Africa. This air had enhanced O3 and aerosols and an associated decrease in H2O. Average latitudinal and longitudinal distributions of O3 and H2O were constructed from the remote and in situ O3 and H2O data, and these distributions are compared with results from PEM-Tropics A conducted in August-October 1996. During PEM-Tropics B, low O3 air was found in the SH across the entire Pacific Basin at low latitudes. This was in strong contrast to the photochemically enhanced O3 levels found across the central and eastern Pacific low latitudes during PEM-Tropics A. Nine air mass types were identified for PEM-Tropics B based on their O3, aerosols, clouds, and potential vorticity characteristics. The data from each flight were binned by altitude according to air mass type, and these results showed the relative observational frequency of the different air masses as a function of altitude in seven regions over the Pacific. The average chemical composition of the major air mass types was determined from in situ measurements in the NH and SH, and these results provided insight into the origin, lifetime, and chemistry of the air in these regions.

Browell, Edward V.↗

Vertical Transport Processes for Inert and Scavenged Species: TRACE-A Measurements

The TRACE-A mission of the NASA DC-8 aircraft made a large-scale survey of the tropical and subtropical atmosphere in September and October of 1992. Both In-situ measurements of CO (G. Sachsen NASA Langley) and aerosol size (J. Browell group, NASA Langley) provide excellent data sets with which to constrain vertical transport by planetary boundary layer mixing and deep-cloud cumulus convection. Lidar profiles of aerosol-induced scattering and ozone (also by Bremen) are somewhat require more subtle interpretation as tracers, but the vertical information on layering largely compensates for these complexities. The reason this DC-8 dataset is so useful is that very large areas of biomass burning over Africa and South America provide surface sources of appropriate sizes with which to characterize vertical and horizontal motions; the major limitation of our source description is that biomass burning patterns move considerably every few days, and daily burning inventories are a matter of concurrent, intensive research. We use the Penn State / NCAR MM5 model in an assimilation mode on the synoptic and intercontinental scale, and assess the success it shows in vertical transport descriptions. We find that the general level of emissions suggested by the climatological approach (Will. Has, U. of Montana) appears to be approximately correct, possibly a bit low, for this October, 1992, time period. Vertical transport in planetary boundary layer mixing to 5.5 kin was observed and reproduced in our simulations. Furthermore we find evidence that Blackader "transilient" or matrix-transport scheme is needed, but may require some adaptation in our tracer model: CO seems to exhibit very high values at the top of the planetary boundary layer, a process that stretches the eddy-diffusion parameterization. We will report on progress in improving the deep convective transport of carbon monoxide: the Grail scheme as we used it at 100 kin resolution did not transport enough material to the upper troposphere. We expect to be able to attribute this to either parameterization reasons (inadequacy of this parameterization at the large 100km scale) or other reasons. Nevertheless, the qualitative nature of deep transport by clouds shows up well in the simulations. As for scavengable species, the simulations predict tens of micrograms per standard cubic meter of smoke aerosol in the boundary layer. In a straightforward illustration of our simple bulk-mass scavenging parameterization, to one or two micrograms per standard cubic meter of smoke aerosol in the free troposphere just above the source regions: very high concentrations for the free troposphere. We expect to report on comparisons of these predictions to a variety of observations.

Chatfield, Robert B.↗

Making Intercontinental Burning Influences Quantitative: Lessons on Transport and Geochemistry From the 3-D Simulation of CO in PEM-T A and TRACE-A

We report on two aspects of the simulation of global transport of plumes originating from subtropical biomass fires. We use of meteorological assimilation (MM5) at 2-degree resolution with a Grail cloud parameterization and a Blackadar-based planetary boundary layer parameterization. Ames's GRACES model provides emissions, transport, and an appropriate level of simulated chemical transformation. We have worked with passive-tracer CO or linear chemistry. This is appropriate since we find major work to be done in evaluating CO source strengths and transport mechanisms before chemical integrations could be meaningful. First, we present mechanisms by which CO and other pollutants are introduced into the free troposphere, and are then transported with hate dilution from approx. 0 to approx. 180 degrees longitude. One principal conduit for these plumes is the vernal subtropical jet; however the plumes appear at various altitudes and latitudes as they influenced by frontal motions and (most likely) radiative processes. A common, repeated pattern of transport has pollutant plumes arriving in the distant Pacific Ocean from Africa and South America at 25 degrees south and 14 km altitude. Following this, there is then a general appearance of pollution at extending down to 5 kin at more equatorial (10 S) and polar latitudes (to 45 S). Second, we evaluate the quantitative success of our simulation. (Such success requires efforts considerably beyond trajectory analyses, and is necessary for our community to claim an understanding of the effects of biomass burning on global atmospheric chemistry and the planet's trend in oxidizing capacity.) We find that we simulate most pollution episodes sampled by Glenn Sachse's CO instrument and the Blake hydrocarbon analyses during PENT A. We will present our current ideas on why our general levels appear satisfactory when the observations are within 20 ppb of background levels, but substantially miss the variability associated with the most intense biomass burning plumes. As time allows, we will speculate on the origins of a class of plumes that appear in the mid-troposphere, but are missing from our simulations.

Chatfield, Robert↗

Ground-Based Lidar Measurements of Aerosols During ACE-2: Instrument Description, Results, and Comparisons with Other Ground-Based and Airborne Measurements

A micro-pulse lidar system (MPL) was used to measure the vertical and horizontal distribution of aerosols during the Aerosol Characterization Experiment 2 (ACE-2) in June and July of 1997. The MPL measurements were made at the Izana observatory (IZO), a weather station located on a mountain ridge (28 deg 18 min N, 16 deg 30 min W, 2367 m asl) near the center of the island of Tenerife, Canary Islands. The MPL was used to acquire aerosol backscatter, extinction, and optical depth profiles for normal background periods and periods influenced by Saharan dust from North Africa. System tests and calibration procedures are discussed, and an analysis of aerosol optical profiles acquired during ACE-2 is presented. MPL data taken during normal IZO conditions (no dust) showed that upslope aerosols appeared during the day and dissipated at night and that the layers were mostly confined to altitudes a few hundred meters above IZO. MPL data taken during a Saharan dust episode on 17 July showed that peak aerosol extinction values were an order of magnitude greater than molecular scattering over IZO, and that the dust layers extended to 5 km asl. The value of the dust backscatter-extinction ratio was determined to be 0.027 +/- 0.007 sr(exp -1). Comparisons of the MPL data with data from other collocated instruments showed good agreement during the dust episode.

Welton, Ellsworth J.↗

Impact of Mineral Aerosol on TOVS Temperature and Moisture Retrievals

Mineral aerosols can absorb significant radiation in the infrared spectrum. Consequently, there may be errors in TIROS Operational Vertical Sounder (TOVS) retrieved temperature and moisture profiles in regions of heavy dust loading. We first investigate the potential error in the temperature retrievals and secondly attempt to account for radiative effects of the dust in retrievals. Information on the dust concentrations and size distribution is from the Goddard Chemistry Aerosol Transport model (GOCART). Aerosol optical parameters are calculated from mie scattering theory assuming a composition of pure illite. We used the cloud-clearing DAO TOVS retrieval system of Joiner and Rokke (2000). It is incorporated into the Data Assimilation Office (DAO) Finite Volume Data Assimilation System (NDAS). The advantage of this approach is that the first guess temperature profile used in the TOVS retrieval are forecasted temperatures from the previous assimilated time period. The operational DAO fvDAS was run for 10 days during June 2001 during a period of dust outbreaks off the coast of Africa over the Atlantic. The observed minus the forecast (O-F) brightness temperature at each TOVS channel is a measure of the accuracy of the retrieval. Since there was no account of dust during this operational run, a dependence of O-F on the estimated atmospheric dust concentrations from GOCART indicates that the dust is contaminating the TOVS retrievals. Channels that measure the surface temperature, lower tropospheric temperature and moisture show this dependence. There are errors in the retrieved brightness temperature of a half a degree or more during heavy dust loading conditions. The forecasted brightness temperature is always greater than the observed value. The radiative transfer module used in the DAO TOVS retrieval system was modified to account for dust. We calculate the sensitivity of the brightness temperature of the TOVS channels to the dust concentrations in GOCART assuming pure illite. For most channels the observed relationship between O-F and dust concentrations in GOCART is consistent with these calculated sensitivities. The fvDAS run was repeated using the modified DAO TOVS retrieval system that accounts for dust. Preliminary results from this run show that there are significant effects on the retrieved surface temperature and tropospheric moisture.

Weaver, Clark↗

MODIS Observations of Smoke and Fires

The MODIS (Moderate Resolution Imaging Spectroradiometer) instruments collect daily measurements of our planet since early 2000 from the Terra spaceborne polar platform. It has unique channels to observe smoke over land and ocean and to observe fires. Using unsaturated channels at 3.9 micron MODIS detects the fires and estimates the fire radiative energy. Using solar channels in the visible (0.47 and 0.66 micron) and in the mid IR (2.1 micron) MODIS measures the smoke optical thickness distribution and evolution over the land. Seven Channels in the solar spectrum are used to detect the smoke properties and distribution over the oceans. Data from the Aerosol Robotic Network, are used to validate the MODIS observations. The MODIS aerosol data presented in a movie form is used to observe the generation of smoke plumes and their dispersion around the globe. For example a key conclusion is that smoke in particular from Southern Africa can pollute significantly the 'pristine' Southern Hemisphere zonal range of 45'S-60'S, and the Northern Pacific.

Kaufman, Yoram↗