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At least 1,297 records · Page 72
All sourcesNASA NTRSDOE OSTI
DOE OSTI2023

In-Situ Spatial Mapping of Hydrogen in Yttrium Hydrides at LANSCE (FY23 Version, Rev. 1)

This report summarizes the development of neutron imaging capabilities and experimental activities performed at the Los Alamos Neutron Science Center (LANSCE) with the main goal of measuring temperature-driven hydrogen diffusion within bulk-yttrium hydride (YH x ) materials. Yttrium hydride is the leading candidate to serve as a solid neutron moderator in microreactor cores, owing to its high density of hydrogen atoms as well as its superior thermal stability compared to all other metal hydrides. The experimental results and technique developments reported herein support the U.S. Department of Energy Office of Nuclear Energy’s (DOE-NE) Microreactor Program under Technology Maturation. In particular, it addresses the critical need to experimentally validate and verify hydrogen-diffusion models of metal hydrides used in high-temperature microreactor designs by means of high-spatial-resolution neutron imaging. These capabilities were designed to apply large temperature gradients across centimeter-sized YH x pellets to simulate conditions faced in the microreactor environment. In principle, neutron imaging, combined with in-situ sample heating, enables near real-time tracking of hydrogen diffusion in YH x on the sub-millimeter scale. In this report, an overview of neutron imaging methodology and technologies are given in the context of recent spatial measures of hydrogen concentrations in similar metal hydrides. Additionally, the commissioning and operation of a custom-built compact dual-zone furnace is given along with details on three in-situ heating measurements of YH x performed over the 2020 to 2022 LANSCE operation cycles. The aims of these experiments ranged from furnace commissioning, determining sample quality, i.e., hydrogen uniformity via neutron computed tomography, and studying the effects of applied temperature-gradients on YH x pellets. Analyses and results from these neutron imaging measurements are given along with outlooks and guidelines for optimal future hydrogen diffusion measurements. Our conclusions are as follows. Image analyses indicate that centimeter-sized yttrium hydride cylindrical pellets exhibit uniform, whole-body hydrogen desorption and absorption without clear temperature dependence as reflected in the image attenuation at the opposing ends of each sample. This suggests that despite the large magnitude in temperature gradients applied by the furnace heating elements, the sample equilibrates to an unknown intermediate temperature. The origin of this result is likely the combination of short sample length (∼1cm) and use of a TZM can for containment where the latter created a thermal short across the sample. Nevertheless, the results from the most recent measurements indicate that neither significant concentration gradients of hydrogen were formed in centimeter-sized samples through the entire temperature range (25 °C to 950 °C) nor any formed due to temperature gradients on the order of 50 °C/cm up to 700 °C/cm. Furthermore, images from the FY2021 and FY2022 measurements indicate that samples of YH x , fabricated from either the direct hydride or powder metallurgy methods, are highly uniform in their hydrogen concentration to within the measurements’ spatial resolutions. The following questions arise from these latest results: 1) What is the intermediate temperature of the pellets in the TZM cans? 2) How quickly does the temperature equilibrate within the sample? and, 3) Do the observed changes in image attenuation follow known pressure-composition-temperature relations of yttrium hydride?

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2024

FY2024 Mid-Year Report: Verification of Spent Fuel Inside Dry Storage Casks by Cask Top Fast Neutron Mapping

This project is developing a prototype scanner array verification system for detection of missing fuel assemblies in spent-fuel storage casks. The prototype consists of six fast-neutron scintillator detectors mounted to a linear actuator frame that is placed on the top of a spent fuel cask to scan across all fuel assembly positions. The scanner array was assembled and tested at LLNL in prior years. A field test schedule has been requested at the Idaho National Laboratory (INL) Cask Farm site for FY2024. Following the Field Test, we will present results and discuss the technology with the IAEA. The IAEA may have special requirements for portability, shipping, lifting, and installation. We will incorporate additional improvements to the system based on lessons learned from the Field Test and feedback from the IAEA. If successful, the technology can be transferred to the IAEA or other stakeholders for assessment.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2024

Axially Symmetric E-Lens Based on McMillan Map

In this work, we investigate the transverse dynamics of a single particle in a model integrable accelerator lattice, based on a McMillan axially symmetric electron lens. Although the McMillan e-lens has been considered as a device potentially capable of mitigating collective space charge forces, some of its fundamental properties have not been described yet. The main goal of our work is to close this gap and understand the limitations and potential of this device. We classify possible regimes with stable trajectories and provide set of canonical action-angle variables, along with an evaluation of the dynamical aperture, Poincar\'e rotation numbers as functions of amplitudes, and spread in nonlinear tunes.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2024

Monte Carlo Simulation with CAD Interface for Calculation of 3D Maps of Residual Dose (CRADA)

Objective: To develop an easy-to-use software application to predict and mitigate radiation effects in research environment, space instruments, nuclear plants and medical facilities and help nonproliferation and national security efforts. Tech-X will develop standalone software libraries and command-line tools for ( 1) translating CAD into tessellated surfaces and tetrahedral meshes in GDML (for Geant4 and MARS 15), ROOT (for MARS 15) and HDF5 (for compact representation and for the visualization) formats, (2) healing CAD geometries to make them suitable for Monte Carlo simulations; (3) creating uniform and variable Cartesian and cylindrical meshes for detailed scoring; and ( 4) efficient Monte Carlo navigation in CAD geometries. JLAB will finish automation of simulations of residual dose in CAD geometries and integrate Tech-X software into Geant4 and MARS15. Finally, Tech-X will develop a Graphical User Interface to set up and heal CAD geometries, create input files, run and visualize simulations for residual dose. This application will run on local desktops, local and remote clusters and supercomputers and will be made available through public clouds, such as Amazon Web Services.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2024

Mapping Dark Matter on Small Scales with the Cosmic Microwave Background (Final Report)

Sehgal was funded by DOE Grant DE-SC0020441 over the period from 11/1/2019 - 04/30/2024 (no remaining funds are anticipated). Most recently, Sehgal and her group completed a publication forecasting cosmological parameter constraints for a CMB-HD survey, in addition to SO and CMB-S4 (1). One focus of this work was determining the improvement in parameter constraints when removing the gravitational lensing effect from the primordial CMB (a process called delensing). This work also explored the bias to parameters from neglecting baryonic effects, and ways to mitigate that. In addition, this work highlighted that a CMB-HD N eff measurement could tightly constrain the QCD axion in a modelindependent way (see left panel of Figure 1). Sehgal also developed a novel way to probe inflation via CMB experiments by measuring inflationary magnetic fields (IMFs) (2). IMFs are thought to seed the large magnetic fields we observe in galaxies today, and can be measured by looking for anisotropic rotation of the CMB polarization vectors across the sky (an effect called cosmic birefringence). The cosmic birefringence from IMFs has a unique frequency dependence, allowing it to be separated from other sources of cosmic birefringence. In (2), Sehgal and her postdoc also presented a novel way to remove foreground contamination from Galactic magnetic fields using measurements of the polarization of nearby radio sources. The removal of this Galactic contamination is necessary when measuring IMFs at the level of 0.1 nG; IMFs with a strength of at least 0.1 nG are needed to seed the magnetic fields in galaxies we observe today. Since only inflation can generate such a strong magnetic field, measuring such a signal would be a “smoking gun” signature that inflation occurred. Sehgal showed in (2) that CMB-HD could detect such IMFs with at least 3σ significance (see right panel of Figure 1).

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2024

A Road Map to Determine Chemical Phenomenology Required for Molten Salt Reactor Accident Modeling

The differences between molten salt reactors (MSRs) and light water reactors (LWRs) has required modification of previous approaches to model reactor accident progression. Part of this is related to the different chemical phenomenology of these reactors as their fuel is not as contained and can react with their surroundings. MELCOR is a reactor simulation tool that has implemented methods and models to model MSRs. However, additional development of MELCOR for modeling MSRs is required. Although understanding the chemistry surrounding MSRs is important to general MSR licensing and operation, only a subset of reactions and phenomenology are required to model beyond design basis incidents and therefore to be captured by MELCOR. This report is intended to guide the chemical phenomenology to improve MELCOR MSR accident modeling and discusses phenomenology models that are in development.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗