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At least 1,297 records · Page 72

Toward Aerosol/Cloud Condensation Nuclei (CCN) Closure during CRYSTAL-FACE

During July 2002, measurements of cloud condensation nuclei were made in the vicinity of southwest Florida as part of the Cirrus Regional Study of Tropical Anvils and Cirrus Layers-Florida Area Cirrus Experiment (CRYSTAL-FACE) field campaign. These observations, at supersaturations of 0.2 and 0.85%, are presented here. The performance of each of the two CCN counters was validated through laboratory calibration and an in situ intercomparison. The measurements indicate that the aerosol sampled during the campaign was predominantly marine in character: the median concentrations were 233 cm-3 (at S = 0.2%) and 371 cm(sup -3) (at S = 0.85%). Three flights during the experiment differed from this general trend; the aerosol sampled during the two flights on 18 July was more continental in character, and the observations on 28 July indicate high spatial variability and periods of very high aerosol concentrations. This study also includes a simplified aerosol/CCN closure analysis. Aerosol size distributions were measured simultaneously with the CCN observations, and these data are used to predict a CCN concentration using Kohler theory. For the purpose of this analysis, an idealized composition of pure ammonium sulfate was assumed. The analysis indicates that in this case, there was good general agreement between the predicted and observed CCN concentrations: at S = 0.2%, N(sub predicted)/N(sub observed)= 1.047 (R(sup 2)= 0.911)); at S = 0.85%, N(sub predicted)/N(sub observed)=1.201 (R(sup 2)= 0.835)). The impacts of the compositional assumption and of including in-cloud data in the analysis are addressed. The effect of removing the data from the 28 July flight is also examined; doing so improves the result of the closure analysis at S = 0.85%. When omitting that atypical flight, N(sub predicted)/N(sub observed) = 1.085 (R(sup 2) = 0.770) at S = 0.85%.

VanReken, Timothy M.↗

SMART-COMMIT Observations and Deep-Blue Retrievals of Saharan Dust Properties during NAMMA

Monsoon rainfalls sustain the livelihood of more than half of the world's population. The interaction between natural/anthropogenic aerosols, clouds, and precipitation is a critical mechanism that drives the water cycle and fresh water distribution. Analyses of the longterm trend of July-August precipitation anomaly for the last 50 years in the 20" century depict that the largest regional precipitation deficit occurs over the Sahel, where the monsoon water cycle plays an important role. Thus, it is of paramount importance to study how dust aerosols, as well as air pollution and smoke, influence monsoon variability. The NASA African Monsoon Multidisciplinary Activities (NAMMA) was conducted during the international AMMA Special Observation Period (SOP-3) of September 2006 to better comprehend the key attributes of the Saharan Air Layer (SAL) and how they evolve from the source regions to the Atlantic Ocean. The SAL occurs during the late spring through early fall and originates as a result of low-level convergence induced by heat lows over the Sahara that lifts hot, dry, dust laden air aloft into a well mixed layer that extends up to 500mb. This is crucial for understanding the impact of SAL on the key atmospheric processes that determine precipitation over West Africa and tropical cyclogenesis. Results obtained from the synergy of satellite (Deep- Blue) and surface (SMART-COMMIT) observations will be presented and discussed how the physical, optical and radiative properties of the dust in the SAL evolve from the continental to the marine environment.

Tsay, Si-Chee↗

Variability and Quasi-Decadal Changes in the Methane Budget over the Period 2000-2012

Following the recent Global Carbon Project (GCP) synthesis of the decadal methane (CH4) budget over 2000- 2012, we analyse here the same dataset with a focus on quasi-decadal and inter-annual variability in CH4 emissions. The GCP dataset integrates results from top-down studies (exploiting atmospheric observations within an atmospheric inverse-modelling framework) and bottom-up models (including process-based models for estimating land surface emissions and atmospheric chemistry), inventories of anthropogenic emissions, and data-driven approaches. The annual global methane emissions from top-down studies, which by construction match the observed methane growth rate within their uncertainties, all show an increase in total methane emissions over the period 2000-2012, but this increase is not linear over the 13 years. Despite differences between individual studies, the mean emission anomaly of the top-down ensemble shows no significant trend in total methane emissions over the period 2000-2006, during the plateau of atmospheric methane mole fractions, and also over the period 2008-2012, during the renewed atmospheric methane increase. However, the top-down ensemble mean produces an emission shift between 2006 and 2008, leading to 22 [16-32] Tg CH4 yr(exp -1) higher methane emissions over the period 2008-2012 compared to 2002-2006. This emission increase mostly originated from the tropics, with a smaller contribution from mid-latitudes and no significant change from boreal regions. The regional contributions remain uncertain in top-down studies. Tropical South America and South and East Asia seem to contribute the most to the emission increase in the tropics. However, these two regions have only limited atmospheric measurements and remain therefore poorly constrained. The sectorial partitioning of this emission increase between the periods 2002-2006 and 2008-2012 differs from one atmospheric inversion study to another. However, all top-down studies suggest smaller changes in fossil fuel emissions (from oil, gas, and coal industries) compared to the mean of the bottom-up inventories included in this study. This difference is partly driven by a smaller emission change in China from the top-down studies compared to the estimate in the Emission Database for Global Atmospheric Research (EDGARv4.2) inventory, which should be revised to smaller values in a near future. We apply isotopic signatures to the emission changes estimated for individual studies based on five emission sectors and find that for six individual top-down studies (out of eight) the average isotopic signature of the emission changes is not consistent with the observed change in atmospheric 13CH4. However, the partitioning in emission change derived from the ensemble mean is consistent with this isotopic constraint. At the global scale, the top-down ensemble mean suggests that the dominant contribution to the resumed atmospheric CH4 growth after 2006 comes from microbial sources (more from agriculture and waste sectors than from natural wetlands), with an uncertain but smaller contribution from fossil CH4 emissions. In addition, a decrease in biomass burning emissions (in agreement with the biomass burning emission databases) makes the balance of sources consistent with atmospheric 13CH4 observations. In most of the top-down studies included here, OH concentrations are considered constant over the years (seasonal variations but without any inter-annual variability). As a result, the methane loss (in particular through OH oxidation) varies mainly through the change in methane concentrations and not its oxidants. For these reasons, changes in the methane loss could not be properly investigated in this study, although it may play a significant role in the recent atmospheric methane changes as briefly discussed at the end of the paper.

Saunois, Marielle↗

Tropical Oceanic Influences on Observed Global Tropical Cyclone Frequency

Abstract The global tropical cyclone (TC) number has historically been relatively constant from year‐to‐year, however, the reason remains unknown. Furthermore, climate projections are inconclusive regarding future global TC frequency changes. Here, we investigated years in which observed global TC activity deviated from the mean and potential links to ocean drivers from 1980 to 2021. We found that the annual global number of named storm days and accumulated cyclone energy (ACE) were significantly linked with El Niño–Southern Oscillation (ENSO) and the Atlantic Meridional Mode (AMM). La Niña and positive AMM are associated with the bottom percentiles of both TC metrics, and vice versa for El Niño and negative AMM. The ENSO Longitude Index explains variability in annual global named storm days and ACE as well as the Niño 3.4 index. This research reveals that reliable future projections of ENSO are necessary, but not sufficient, to understand future changes in global TC frequency.

54 ENVIRONMENTAL SCIENCES↗

Interannual and Decadal Variability of Summer Rainfall over South America

Using the CPC (Climate Prediction Center) Merged Analysis of Precipitation product along with the Goddard Earth Observing System reanalysis and the Climate Analysis Center sea surface temperature (SST) data, we conduct a diagnostic study of the interannual and decadal scale variability of summer rainfall over South America. Results show three leading modes of rainfall variation identified with interannual, decadal, and long-term trend variability. Together, these modes explain more than half the total variance. The first mode is highly correlated with El Nino/southern oscillation (ENSO), showing severe drought over Northeast Brazil and copious rainfall over the Ecuador coast and the area of Uruguay-Southern Brazil in El Nino years. This pattern is attributed to the large scale zonal shift of the Walker circulation and local Hadley cell anomaly induced by positive (negative) SST anomaly over the eastern (western) equatorial Pacific. In El Nino years, two convective belts indicated by upper tropospheric velocity potential trough and mid-tropospheric rising motion, which are somewhat symmetric about the equator, extend toward the northeast and the southeast into the tropical North and South Atlantic respectively. Sandwiched between the ascent is a region of descending motion over Northeast Brazil. The southern branch of the anomalous Hadley cell is dynamically linked to the increase of rainfall over Uruguay-Southern Brazil. The regional response of anomalous circulation shows a stronger South American summer monsoon and an enhanced (weakened) subtropical high over the South Atlantic (South Pacific) Ocean. The decadal variation displays a meridional shift of the Intertropical Convergence Zone (ITCZ), which is tie to the anomalous cross-equatorial SST gradient over the Atlantic and the eastern Pacific. In conjunction with this mode is a large scale mass swing between the polar regions and midlatitudes in both hemispheres. Over the South Atlantic and the South Pacific, the changes of the strength of the subtropical high and the associated surface wind are dynamically consistent with the distribution of local SST anomalies, suggesting the importance of the atmospheric forcing in the decadal time scale. The decadal mode also presents a weak summer monsoon in its positive phase, which reduces the moisture supply from the equatorial Atlantic and the Amazon Basin and results in negative rainfall anomalies over the central Andes and Gran Chaco. The long-term trend shows decrease of rainfall from the northwest coast to the southeast subtropical region and a southward shift of Atlantic ITCZ that leads to increased rainfall over northern and eastern Brazil. Our result shows a close link of this mode to the observed SST warming trend over the subtropical South Atlantic and a remote connection to the interdecadal SST variation over the extratropical North Atlantic found in previous studies.

Zhou, Jiayu↗

Circles and triangles, the NLSM and Tr(Φ 3 )

A surprising connection has recently been made between the amplitudes for Tr(Φ 3 ) theory and the non-linear sigma model (NLSM). A simple shift of kinematic variables naturally suggested by the associahedron/stringy representation of Tr(Φ 3 ) theory yields pion amplitudes at all loops. In this note we provide an elementary motivation and proof for this link going in the opposite direction, starting from the non-linear sigma model and discovering its formulation as a sum over triangulations of surfaces with simple numerator factors. This uses an ancient connection between “circles” and “triangles”, interpreting the equation y = $\sqrt{1 – x^2}$ both as parametrizing points a circle as well as generating the number of triangulations of polygons. A further simplification of the numerator factors exposes them as arising from the kinematically shifted Tr(Φ3) theory, and gives rise to novel tropical representations of NLSM amplitudes. The connection to Tr(Φ 3 ) theory defines a natural notion of “surface-soft limit” intrinsic to curves on surfaces. Remarkably, with this definition, the soft limit of pion amplitudes vanishes directly at the level of the integrand, via obvious pairwise cancellations. We also give simple, explicit expressions for the multi-soft factors for tree and loop-level integrands in the limit as any number of pions are taken “surface-soft”.

Scattering Amplitudes↗

Cloud and boundary layer structure over San Nicolas Island during FIRE

The temporal evolution of the structure of the marine boundary layer and of the associated low-level clouds observed in the vicinity of the San Nicolas Island (SNI) is defined from data collected during the First ISCCP Regional Experiment (FIRE) Marine Stratocumulus Intense Field Observations (IFO) (July 1 to 19). Surface, radiosonde, and remote-sensing measurements are used for this analysis. Sounding from the Island and from the ship Point Sur, which was located approximately 100 km northwest of SNI, are used to define variations in the thermodynamic structure of the lower-troposphere on time scales of 12 hours and longer. Time-height sections of potential temperature and equivalent potential temperature clearly define large-scale variations in the height and the strength of the inversion and periods where the conditions for cloud-top entrainment instability (CTEI) are met. Well defined variations in the height and the strength of the inversion were associated with a Cataline Eddy that was present at various times during the experiment and with the passage of the remnants of a tropical cyclone on July 18. The large-scale variations in the mean thermodynamic structure at SNI correlate well with those observed from the Point Sur. Cloud characteristics are defined for 19 days of the experiment using data from a microwave radiometer, a cloud ceilometer, a sodar, and longwave and shortwave radiometers. The depth of the cloud layer is estimated by defining inversion heights from the sodar reflectivity and cloud-base heights from a laser ceilometer. The integrated liquid water obtained from NOAA's microwave radiometer is compared with the adiabatic liquid water content that is calculated by lifting a parcel adiabatically from cloud base. In addition, the cloud structure is characterized by the variability in cloud-base height and in the integrated liquid water.

Albrecht, Bruce A.↗

An Equation for Moist Entropy in a Precipitating and Icy Atmosphere

Moist entropy is nearly conserved in adiabatic motion. It is redistributed rather than created by moist convection. Thus moist entropy and its equation, as a healthy direction, can be used to construct analytical and numerical models for the interaction between tropical convective clouds and large-scale circulations. Hence, an accurate equation of moist entropy is needed for the analysis and modeling of atmospheric convective clouds. On the basis of the consistency between the energy and the entropy equations, a complete equation of moist entropy is derived from the energy equation. The equation expresses explicitly the internal and external sources of moist entropy, including those in relation to the microphysics of clouds and precipitation. In addition, an accurate formula for the surface flux of moist entropy from the underlying surface into the air above is derived. Because moist entropy deals "easily" with the transition among three water phases, it will be used as a prognostic variable in the next generation of cloud-resolving models (e. g. a global cloud-resolving model) for low computational noise. Its equation that is derived in this paper is accurate and complete, providing a theoretical basis for using moist entropy as a prognostic variable in the long-term modeling of clouds and large-scale circulations.

Tao, Wei-Kuo↗

Measurement report: Closure Analysis of Aerosol–cloud Composition in Tropical Maritime Warm Convection

Cloud droplet chemical composition is a key observable property that can aid understanding of how aerosols and clouds interact. As part of the Clouds, Aerosols and Monsoon Processes – Philippines Experiment (CAMP2Ex), three case studies were analyzed involving collocated airborne sampling of relevant clear and cloudy air masses associated with maritime warm convection. Two of the cases represented a polluted marine background, with signatures of transported East Asian regional pollution, aged over water for several days, while the third case comprised a major smoke transport event from Kalimantan fires. Sea salt was a dominant component of cloud droplet composition, in spite of fine particulate enhancement from regional anthropogenic sources. Furthermore, the proportion of sea salt was enhanced relative to sulfate in rainwater and may indicate both a propensity for sea salt to aid warm rain production and an increased collection efficiency of large sea salt particles by rain in subsaturated environments. Amongst cases, as precipitation became more significant, so too did the variability in the sea salt to (non-sea salt) sulfate ratio. Across cases, nitrate and ammonium were fractionally greater in cloud water than fine-mode aerosol particles; however, a strong covariability in cloud water nitrate and sea salt was suggestive of prior uptake of nitrate on large salt particles. A mass-based closure analysis of non-sea salt sulfate compared the cloud water air-equivalent mass concentration to the concentration of aerosol particles serving as cloud condensation nuclei for droplet activation. While sulfate found in cloud was generally constrained by the sub-cloud aerosol concentration, there was significant intra-cloud variability that was attributed to entrainment – causing evaporation of sulfate-containing droplets –and losses due to precipitation. In addition, precipitation tended to promote mesoscale variability in the sub-cloud aerosol through a combination of removal, convective downdrafts, and dynamically driven convergence. Physical mechanisms exerted such strong control over the cloud water compositional budget that it was not possible to isolate any signature of chemical production/loss using in-cloud observations. The cloud-free environment surrounding the non-precipitating smoke case indicated sulfate enhancement compared to convective mixing quantified by a stable gas tracer; however, this was not observed in the cloud water (either through use of ratios or the mass closure), perhaps implying that the warm convective cloud timescale was too short for chemical production to be a leading-order budgetary term and because precursors had already been predominantly exhausted. Closure of other species was truncated by incomplete characterization of coarse aerosol (e.g., it was found that only 10 %–50% of sea salt mass found in cloud was captured during clear-air sampling) and unmeasured gasphase abundances affecting closure of semi-volatile aerosol species (e.g., ammonium, nitrate and organic) and soluble volatile organic compound contributions to total organic carbon in cloud water.

Ewan Crosbie↗

Decoding the dynamics of poleward shifting climate zones using aqua-planet model simulations

Growing evidence indicates that the atmospheric and oceanic circulation experiences a systematic poleward shift in a warming climate. However, the complexity of the climate system, including the coupling between the ocean and the atmosphere, natural climate variability and land-sea distribution, tends to obfuscate the causal mechanism underlying the circulation shift. Here, using an idealised coupled aqua-planet model, we explore the mechanism of the shifting circulation, by isolating the contributing factors from the direct CO 2 forcing, the indirect ocean surface warming, and the wind-stress feedback from the ocean dynamics. We find that, in contrast to the direct CO 2 forcing, ocean surface warming, in particular an enhanced subtropical ocean warming, plays an important role in driving the circulation shift. This enhanced subtropical ocean warming emerges from the background Ekman convergence of surface anomalous heat in the absence of the ocean dynamical change. Additionally, it expands the tropical warm water zone, causes a poleward shift of the mid-latitude temperature gradient, hence forces a corresponding shift in the atmospheric circulation and the associated wind pattern. The shift in wind, in turn drives a shift in the ocean circulation. Our simulations, despite being idealised, capture the main features of the observed climate changes, for example, the enhanced subtropical ocean warming, poleward shift of the patterns of near-surface wind, sea level pressure, storm tracks, precipitation and large-scale ocean circulation, implying that increase in greenhouse gas concentrations not only raises the temperature, but can also systematically shift the climate zones poleward.

54 ENVIRONMENTAL SCIENCES↗

A Comparison of the Diurnal Variation of Rainfall in the LBA Area Derived from Satellite Infrared Observations and Raingages

In this paper we will present results from the application of a satellite infrared (IR) technique for estimating rainfall over northern South America. Our main objectives are to examine the diurnal variability of rainfall and to investigate the relative contributions from the convective and stratiform components. Estimates for Jan-Apr. 1999 will be presented for a large(30 by 50 degree) area that includes the Amazon Basin and the Large-Scale Biosphere-Atmosphere (LBA) study area. An analysis of the LBA raingage has begun, and results from the analysis of the gage-derived diurnal cycle will be compared to the satellite estimates. See the attached figure for preliminary results. Also, we hope to perform a comparison of results with LBA case studies of mesoscale convective systems using TOGA and S-bands radars. Future calibration of the IR technique using rain estimates from Tropical Rainfall Measuring Mission (TRMM) is anticipated.

Negri, Andrew J.↗

Multi-Model Assessment of the Factors Driving the Ozone Evolution Over the 21st Century

The evolution of ozone from 1960 to 2100 is examined in simulations from fourteen chemistry-climate models. There is general agreement among the models at the broadest levels, with all showing column ozone decreasing at all latitudes from 1960 to around 2000, then increasing at all latitudes over the first half of the 21 st century (21 C), and latitudinal variations in the rate of increase and date of return to historical values. In the second half of the century, ozone is projected to carry on increasing, level off or even decrease depending on the latitude, resulting in variable dates of return to historical values at latitudes where column ozone has declined below those levels. Separation into partial column above and below 20 hPa reveals that these latitudinal differences are almost completely due to differences in the lower stratosphere. At all latitudes, upper stratospheric ozone increases throughout the 21 C and returns to 1960 levels before the end of the century, although there is a spread among the models in dates that ozone returns to historical values. Using multiple linear regression the upper stratospheric ozone increase comes from almost equal contributions due to decrease in halogens and cooling from increased greenhouse gas concentrations. The evolution of lower stratospheric ozone differs with latitude. In the tropical lower stratosphere an increase in tropical upwelling causes a steady decrease in ozone through the 21C, and total column ozone does not return to 1960 levels in all models. In contrast, lower stratospheric and total column ozone in middle and high latitudes increases during the 21 C and returns to 1960 levels. For all models there is an earlier return for ozone to historical levels in the northern hemisphere. This is thought to be due to interhemispheric differences in transport.

Oman, L.↗

Temperature Responses to Spectral Solar Variability on Decadal Time Scales

Two scenarios of spectral solar forcing, namely Spectral Irradiance Monitor (SIM)-based out-of-phase variations and conventional in-phase variations, are input to a time-dependent radiative-convective model (RCM), and to the GISS modelE. Both scenarios and models give maximum temperature responses in the upper stratosphere, decreasing to the surface. Upper stratospheric peak-to-peak responses to out-of-phase forcing are approx.0.6 K and approx.0.9 K in RCM and modelE, approx.5 times larger than responses to in-phase forcing. Stratospheric responses are in-phase with TSI and UV variations, and resemble HALOE observed 11-year temperature variations. For in-phase forcing, ocean mixed layer response lags surface air response by approx.2 years, and is approx.0.06 K compared to approx.0.14 K for atmosphere. For out-of-phase forcing, lags are similar, but surface responses are significantly smaller. For both scenarios, modelE surface responses are less than 0.1 K in the tropics, and display similar patterns over oceanic regions, but complex responses over land.

Cahalan, Robert F.↗

Increased seminal root number associated with domestication improves nitrogen and phosphorus acquisition in maize seedlings

Abstract Background and Aims Domesticated maize (Zea mays ssp. mays) generally forms between two and six seminal roots, while its wild ancestor, Mexican annual teosinte (Zea mays ssp. parviglumis), typically lacks seminal roots. Maize also produces larger seeds than teosinte, and it generally has higher growth rates as a seedling. Maize was originally domesticated in the tropical soils of southern Mexico, but it was later brought to the Mexican highlands before spreading to other parts of the continent, where it experienced different soil resource constraints. The aims of this study were to understand the impacts of increased seminal root number on seedling nitrogen and phosphorus acquisition and to model how differences in maize and teosinte phenotypes might have contributed to increased seminal root number in domesticated maize. Methods Seedling root system architectural models of a teosinte accession and a maize landrace were constructed by parameterizing the functional–structural plant model OpenSimRoot using plants grown in mesocosms. Seedling growth was simulated in a low-phosphorus environment, multiple low-nitrogen environments, and at variable planting densities. Models were also constructed to combine individual components of the maize and teosinte phenotypes. Key Results Seminal roots contributed ~35 % of the nitrogen and phosphorus acquired by maize landrace seedlings in the first 25 d after planting. Increased seminal root number improved plant nitrogen acquisition under low-nitrogen environments with varying precipitation patterns, fertilization rates, soil textures and planting densities. Models suggested that the optimal number of seminal roots for nutrient acquisition in teosinte is constrained by its limited seed carbohydrate reserves. Conclusions Seminal roots can improve the acquisition of both nitrogen and phosphorus in maize seedlings, and the increase in seed size associated with maize domestication may have facilitated increased seminal root number.

59 BASIC BIOLOGICAL SCIENCES↗

Toward a Unified Parameterization of the Boundary Layer and Moist Convection: A New Type of Mass-Flux Model - Part 1

Higher-order closure (HOC) models have been proposed for parameterization of the turbulent planetary boundary layer (PBL). HOC models must include closures for higher-order moments (e.g., fourth moments in third-order closure models), for pressure terms, and for dissipation terms. Mass-flux closure (MFC) models have been proposed for parameterization of cumulus convection and, more recently, the convective PBL. MFC models include closures for lateral mass exchanges and for pressure terms (which are usually ignored). The authors developed a new kind of model that combines HOC and MFC, which they hope will be useful for the parameterization of both the PBL and cumulus convection, in a unified framework. Such a model is particularly well suited to regimes in which the PBL turbulence and the cumulus convection are not well separated, for example, the broken stratocumulus and shallow cumulus regimes. The model makes use of an assumed joint probability distribution for the variables of interest, and the equations typically used in HOC models can be derived by integrating over the distribution. Accordingly, the model is called Assumed-Distribution Higher-Order Closure (ADHOC). The prognostic variables of ADHOC are the mean state, the second and third moments of the vertical velocity, and the vertical fluxes of other quantities of interest. All of the parameters of the distribution can be determined from the predicted moments, thereafter the joint distribution is effectively known, and so any and all moments can be constructed as needed. In this way, the usual closure problem of "higher moments" is avoided. The pressure-term parameterizations previously developed for HOC models are used to predict the convective fluxes and the moments of the vertical velocity. In companion papers, parameterizations of lateral mass exchanges and subplume-scale fluxes are presented, and then ADHOC is applied to several observationally based tropical, subtropical, and dry convective boundary layers.

Lappen, Cara-Lyn↗

Genomes to ecosystem function: Targeting critical knowledge gaps in methanogenesis and translation to updated global biogeochemical models

Natural freshwater temperate wetland systems currently represent the largest natural source of atmospheric methane, but are relatively understudied using systems biology tools (e.g. meta-omics) compared to other high producing methane systems (e.g. peat, tropical, or reconstructed wetlands). Using field investigations at the NOAA operated sentinel site on Lake Erie, methane producing activities and responses to geochemical conditions will be determined along seasonal and spatial gradients (Objective 1). Here, a combination of high-throughput activity and gas measurements, combined with high-resolution systems biology and analytical methods, will provide in depth knowledge of the microbiological, chemical, and physical constraints on methane production in wetlands. Using laboratory microcosms, the formation of anoxic microsites and their capacity to facilitate methane production in wetland soils will be simulated (Objective 2). This objective will validate the findings from the field investigations, offering a more controlled environment for teasing out the role of different yet interrelated variables. Lastly, these field and laboratory data will be used for multi-scale, process-level evaluation of an ecosystem biogeochemical model that accommodates these newly identified processes and parameterizes representation of these processes along relevant environmental gradients (Objective 3).This research will identify multiple interacting geochemical, ecological, and metabolic constraints that are poorly understood, oversimplified, or missing in global biogeochemical methane models. This proposal targets the role of oxygen limitation on methane processes in soil domains, to improve reactive transport models of microbial carbon cycling across terrestrial-aquatic soils and generate data on nutrient cycling activities in Great Lake wetlands. This information could provide new insights into the microbial controllers of Lake Erie eutrophication.

59 BASIC BIOLOGICAL SCIENCES↗

VisMetHack2022: Visualizing winds and surface variables from the ECMWF IFS 1-km nature run

This data collection was contributed to the Visualisation Hackathon 2022 (#VisMetHack2022), in conjunction with the Using ECMWF's Forecasts (UEF2022) workshop. The European Center for Medium-Range Weather Forecasts (ECMWF) and the Oak Ridge National Laboratory (ORNL) are pleased to announce access to the data collection from global 1-km nature run (NR) simulations using the Integrated Forecast System (IFS) with explicit convection. We invite you to join us in exploring this precursor to a digital twin of the earth! The NR simulations reveal unprecedented detail of the earth’s atmosphere, and the then outgoing Editor-in-Chief of AGU JAMES commended the project as one of “stunning ambitions,” enabled by computational capacity at scale. The project also won the 2020 HPCwire Readers Choice Award for Best Use of HPC in Physical Sciences. A set of two NR seasonal simulations have been completed, one corresponding to the northern hemispheric winter months (NDJF) and the other for the North Atlantic tropical cyclone season (ASO). The project used the Summit supercomputer at the Oak Ridge Leadership Computing Facility (OLCF). The simulations were facilitated with an INCITE award from the US Department of Energy Office of Science. For the first seasonal run of four months (NDJF), the hydrostatic IFS model was initialized at 00Z on 1 November 2018. The NR for the TC season (AS) was initialized at 00Z on 1 August 2019. The NR simulations were constrained only by sea surface temperatures (SST) at the lower boundary. The IFS output was saved every 3 hours. After feedback and interest from the scientific community, the simulations were rerun for four specific extreme events, with output every 15 minutes. The special cases include a tropical cycle and three severe storm events over the continental USA.

54 ENVIRONMENTAL SCIENCES↗

A Global Assessment of Long-Term Greening and Browning Trends in Pasture Lands Using the GIMMS LAI3g Dataset

Pasture ecosystems may be particularly vulnerable to land degradation due to the high risk of human disturbance (e.g., overgrazing, burning, etc.), especially when compared with natural ecosystems (non-pasture, non-cultivated) where direct human impacts are minimal. Using maximum annual leaf area index (LAImax) as a proxy for standing biomass and peak annual aboveground productivity, we analyze greening and browning trends in pasture areas from 1982-2008. Inter-annual variability in pasture productivity is strongly controlled by precipitation (positive correlation) and, to a lesser extent, temperature (negative correlation). Linear temporal trends are significant in 23% of pasture cells, with the vast majority of these areas showing positive LAImax trends. Spatially extensive productivity declines are only found in a few regions, most notably central Asia, southwest North America, and southeast Australia. Statistically removing the influence of precipitation reduces LAImax trends by only 13%, suggesting that precipitation trends are only a minor contributor to long-term greening and browning of pasture lands. No significant global relationship was found between LAImax and pasture intensity, although the magnitude of trends did vary between cells classified as natural versus pasture. In the tropics and Southern Hemisphere, the median rate of greening in pasture cells is significantly higher than for cells dominated by natural vegetation. In the Northern Hemisphere extra-tropics, conversely, greening of natural areas is 2-4 times the magnitude of greening in pasture areas. This analysis presents one of the first global assessments of greening and browning trends in global pasture lands, including a comparison with vegetation trends in regions dominated by natural ecosystems. Our results suggest that degradation of pasture lands is not a globally widespread phenomenon and, consistent with much of the terrestrial biosphere, there have been widespread increases in pasture productivity over the last 30 years.

ecosystems↗