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At least 1,261 records · Page 70

Specimen Size Artifacts Associated with a Glovebox Deployable Laser Flash Diffusivity Measurement System

To accelerate nuclear fuel qualification and deployment efforts, Oak Ridge National Laboratory has led the world in developing vehicles for accelerating burnup accumulation in nuclear fuel by testing miniature samples in the High Flux Isotope Reactor. However, a challenge remains to establish parity between post irradiation characterization methods for miniature fuel specimens in comparison to conventional fuel elements. This work aims to identify artifacts associated with the thermal analysis of miniature disk specimens in comparison to samples of standardized dimensions through a combination of experimental and computational tools. Using a newly procured Netzsch 427 laser flash diffusivity system, preliminary data on mild steel specimens were collected, and finite element techniques were used to model heat transfer using 1D conditions to assess issues associated with pulse width and data collection frequency effects. These preliminary investigations found that significant variability in measured thermal diffusivity exist within datasets. These variations are not necessarily attributed to limitations with respect to data collection rate; nor are they associated with limitations on pulse width. Instead, these artifacts may be a result of limitations in detector intensity. Future work aims to design a focusing lens to better measure the smaller surface area of miniature specimens analyzed using the laser flash analysis system.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Thermo-economic analysis of a solid oxide fuel cell-gas turbine hybrid with commercial off-the-shelf gas turbine

The thermodynamic and economic performance of a natural gas-fueled solid oxide fuel cell (SOFC)-gas turbine (GT) hybrid system with a commercial off-the-shelf GT is investigated. Until today, commercial GTs are primarily engineered for the direct use of energy dense fuels, such as natural gas, and the integration of commercial GTs into a SOFC-GT hybrid remains challenging. In this work technically feasible and economically viable GT operating modes are identified to gauge the technology’s competitiveness on the free market. Steady state, full load operating conditions were established for various GT operating modes: I) constant spool speed operation, II) variable spool speed operation and III) partially closed compressor inlet guide vanes. For each GT operating mode, the performance was investigated over a range of SOFC fuel utilization factors, while considering physical constraints inside the SOFC, such as local temperature gradients in flow direction as well as overall cell temperature differences. The results of the thermodynamic evaluation served as inputs for the economic analysis of the SOFC-GT hybrid power plant. The results show that the integration of an off-the-shelf GT not only results in a significant derating of the GT, but also substantially impacts the SOFC operation, the main power producer in this SOFC-GT hybrid. To maximize the SOFC power output it is desirable operate the GT in a region of high air mass flow rates and low pressure ratios, which increases the number of stacks that can be accommodated and reduces the SOFC cooling requirement. The lowest costs of electricity are obtained at constant spool speed operation, while the highest efficiencies are reached at variable spool speed operation. Critical for the integration of off-the-shelf GTs, which historically have been designed for natural gas, is the surge margin. The largest surge margins are obtained by closing the compressor inlet guide vanes. Furthermore, higher SOFC fuel utilization factors are shown to increase the surge margin as the turbine firing temperature is decreased.

25 ENERGY STORAGE↗

Numerical Methods to Evaluate Hyperelastic Transducers: Hexagonal Distributed Embedded Energy Converters

Hexagonal distributed embedded energy converters, also known as hexDEECs, are centimeter-scale energy transducers that leverage variable capacitance to generate electricity when their hyperelastic structure is dynamically deformed. To better understand, characterize, and optimize hexDEEC designs, a series of numerical methods and techniques were developed to model the hyperelastic mechanics of hexDEECs, electrostatic properties, and electricity generation characteristics. The numerical methods developed for the hyperelastic structural analysis were corroborated by empirical results from another study, and the models and equations for capacitance, electrostatic forces, and electrical potential energy were derived from fundamental electrostatic equations. These methods and techniques were implemented within the STAR-CCM+ multiphysics software Version 2020.3 (15.06.008) environment. Results from this analysis revealed methodologies and techniques necessary to model the energy converters, which will enable future exploration and optimization of more specific designs and corresponding applications.

24 POWER TRANSMISSION AND DISTRIBUTION↗

Cloud Atlas: Unraveling the Vertical Cloud Structure with the Time-series Spectrophotometry of an Unusually Red Brown Dwarf

Rotational modulations of emission spectra in brown dwarf and exoplanet atmospheres show that clouds are often distributed non-uniformly in these ultracool atmospheres. The spatial heterogeneity in cloud distribution demonstrates the impact of atmospheric dynamics on cloud formation and evolution. In this study, we update the Hubble Space Telescope (HST) time-series data analysis of the previously reported rotational modulations of WISEP J004701+680352—an unusually red late-L brown dwarf with a spectrum similar to that of the directly imaged planet HR 8799e. We construct a self-consistent spatially heterogeneous cloud model to explain the HST and the Spitzer time-series observations, as well as the time-averaged spectra of WISE 0047. Additionally, in the heterogeneous cloud model, a cloud thickness variation of around one pressure scale height explains the wavelength dependence in the HST near-IR spectral variability. By including disequilibrium CO/CH 4 chemistry, our models also reproduce the redder $J-{K}_{{\rm{s}}}$ color of WISE 0047 compared to that of field brown dwarfs. We discuss the impact of vertical cloud structure on atmospheric profile and estimate the minimum eddy diffusivity coefficient for other objects with redder colors. Our data analysis and forward modeling results demonstrate that time-series spectrophotometry with a broad wavelength coverage is a powerful tool for constraining heterogeneous atmospheric structure.

79 ASTRONOMY AND ASTROPHYSICS↗

Dynamic Building Load Control to Facilitate High Penetration of Solar Photovoltaic Generation (Final Technical Report)

Solar photovoltaic (PV) resources are the most common form of distributed generation in residential and commercial customer premises within electric distribution networks. A higher penetration of PV generation in distribution circuits will impose challenges on maintaining service voltages within the range of industry standards, power quality, and power flow. Buildings consume 74% of the electricity produced in the United States, and a significant portion of the building load is dispatchable, making them responsive to electrical grid needs. Oak Ridge National Laboratory—in collaboration with Southern Company; the University of Tennessee, Knoxville; and the Georgia Institute of Technology—is examining the PV integration issues in distribution-level electrical grids and developing integrated demand-side control and communication systems to enable responsive loads. The proposed responsive loads mechanism performs renewable generation following to increase the penetration of solar PV within each feeder. The specific objectives of this project are to (1) examine distribution-level PV integration scenarios to understand requirements, (2) undertake an end-to-end simulation-based design of a distributed control strategy of loads geographically near the PV generation asset to minimize the effect on the distribution feeder, (3) deploy and demonstrate the control technology developed in partnership with utilities, and (4) perform a scalability analysis at the utility scale. This 3-year integrated project aims to develop, demonstrate, and validate demand-side control technology to enable increased the penetration of renewables while mitigating challenges that arise due to their intermittency. Activities in Budget Period (BP) 1 focused on a literature review and the formal design of a control system for integrating local distribution with generation and loads. The team used modeling and simulation to evaluate the impact of varying buildings loads, variable PV generation, and power flow dynamics on the distribution circuit. The dynamic models developed in BP 1 were used in BP 2 to develop a model-based control design and a test bed. The test bed has enabled the simulation-based testing and comparison of different control designs and formulations applied to different configurations of the distribution grid, PVs, and building loads. The control approaches developed in BP 2 were implemented in BP 3 in the form of hardware deployed at the Central Baptist Church (CBC) in Knoxville, Tennessee, for testing and evaluation. The outcome of this project was the development and demonstration of open-source, low-cost, low-touch sensing and control retrofits to distributed PV generation and building loads that, in a coordinated fashion, provide the load-shaping response needed to integrate high levels of renewable penetration. This research addresses the target metrics by dynamically controlling a load with solar generation variability to minimize the extent of two-way power flow, enhance reliability, facilitate high PV penetration (>100% of peak load in a line segment), and generate scalable software and hardware solutions adaptable to any penetration levels. The research and development activities are focused and designed to be impactful within the relevant 2020 targets time frame.An accurate open-source integration simulation framework for end-to-end control design was developed and deployed at the CBC facility for testing and evaluation. This final report provides a detailed review of the technical results achieved during this 3-year integrated project. A novel spectral analysis of PV data is demonstrated to derive the requirements of the control design. A detailed simulation-based analysis of PV integration at increasing penetration levels is presented using 1 year of PV data to demonstrate the impact on the distribution circuits. Two different control strategies were developed and demonstrated via simulation to track variable PV generation with adaptive load dispatch. The report concludes with a summary of accomplishments and recommendations for a path forward.

14 SOLAR ENERGY↗

Improving air leakage prediction of buildings using the fan pressurization method with the Weighted Line of Organic Correlation

In many countries, the fan pressurization method is the most frequently chosen approach for measuring the air leakage of houses. The measurements are usually performed at pressures that far exceed pressures to which buildings are exposed to under normal conditions. A fit of these tests to the power-law formulation allows an extrapolation to data points outside the measured pressure range. With the Ordinary Least Square (OLS) fitting method, the pressure exponent and flow coefficient can be determined. However, the measurement results are highly sensitive to uncertainties induced by external factors like changing wind conditions during the tests, which is neglected by OLS. This may lead to errors in the prediction of flows at lower pressures. The Weighted Line of Organic Correlation (WLOC) is an alternative approach and takes measurement uncertainty into account. In this paper, a statistical analysis of an extensive data set of pressurization measurements has been performed. Both regression techniques have been compared for almost 7500 fan pressurization measurements of six houses in 109 different house leak configurations. The variability in predicting pressure exponent and flow coefficient for both WLOC and OLS regression was analyzed using probability density functions. It was found that the Weighted Line of Organic Correlation significantly decreases the uncertainty in predicting pressure exponent, flow coefficient, and other low-pressure air leakage metrics compared to the Ordinary Least Square fitting. Here, the authors highly recommend the implementation of WLOC in current measurement standards and test equipment.

32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATI↗

Modeling assessment of storm surge in the Salish Sea

Here we present a modeling assessment of storm surge in the Salish Sea—a large and complex estuarine system in the Pacific Northwest that is exposed to extratropical cyclones. A method was developed to systematically identify storm surge events in the Salish Sea based on water level records at four representative tidal gauges in the Salish Sea. The maximum storm surge distribution in the Salish Sea was calculated based on model simulations of 34 major historical storm events from 1980 to 2016. The model simulations were validated by field observations of water level and velocity using a suite of model performance metrics. Model results suggest that the maximum storm surge in the Salish Sea is generally in the range of 0.8 m–1.03 m and is heterogeneous in space. The model results also show a strong north-south gradient with larger surge magnitudes occurring in the north that is primarily caused by the southerly wind in winter months. The sensitivity analysis of wind forcing suggested that storm surge in the Salish Sea is dominated by the remote surge from the Pacific Ocean, and the local wind contributes up to approximately 20% of the surge variability. This paper systematically elucidates storm surge characteristics and potential risk in the Salish Sea.

54 ENVIRONMENTAL SCIENCES↗

A Satellite-Based Estimate of Convective Vertical Velocity and Convective Mass Flux: Global Survey and Comparison with Radar Wind Profiler Observations

Convective vertical velocity (w c ) and convective mass flux (M c ) lie at the heart of GCM cumulus parameterizations, but few observations of these critical parameters are available. In this paper, we develop and evaluate a novel, satellite-based method for estimating profiles of w c and M c . Here, comparisons with collocated ground-based radar wind profiler (RWP) observations show that satellite estimated median w c is slightly greater than the RWP estimates, but they show solid agreement when compared at the 95th percentiles (intense updrafts). RWP-derived and satellite estimated M c are broadly comparable in the lower and middle troposphere, with some differences in the upper troposphere due to differences in convective core sampling. A k-means cluster analysis of multiple years of w c data shows that convective characteristics are distinctly different among extratropical convection, tropical land convection, and tropical oceanic convection. Tropical land convection is significantly more intense and more variable than the oceanic counterpart.

54 ENVIRONMENTAL SCIENCES↗

Regional and Temporal Variability of Atmospheric River Seasonality: Influences of Detection Algorithms and Moisture Transport Dynamics

Abstract Understanding the regional and temporal variability of atmospheric river (AR) seasonality is crucial for preparedness and mitigation of extreme events. While ARs were thought to peak in winter, recent research shows they exhibit region‐specific seasonality and are heavily influenced by the chosen detection algorithm. This study examines the link between the year‐to‐year consistency of peak‐AR activity to the presence of a dominant seasonal pattern, considering both location and algorithm choice. Regions are categorized by their temporal characteristics: consistent patterns (e.g., East Asia), patterns with occasional outliers (e.g., British Columbia coast), and regions lacking a clear dominant peak season (e.g., South Atlantic, parts of Australia). Hence, not all regions display a consistent seasonal cycle of AR activity. This study quantifies the extent to which a region experiences a dominant peak season of AR activity (or lacks one) and offers insights to enhance decision‐making in water management, natural hazard preparedness, and forecasting. Furthermore, given our finding that detection algorithms influence the peak season of AR activity, we also examine two diagnostic variables representative of moisture transport to corroborate our results. Integrated vapor transport, which captures meridional and zonal moisture transport, and Moist Wave Activity, representing moisture intrusions from lower to higher latitudes, are examined. Our analysis indicates that inconsistencies in the seasonal cycle of AR activity are not solely due to discrepancies in detection algorithms but also arise from changes in moisture transport. Plain Language Summary Atmospheric rivers (ARs) are critical weather phenomena that can cause extreme events like heavy rainfall and flooding. Understanding when and where ARs are most likely to occur throughout the year is essential for preparing and responding to these events. Traditionally, ARs were thought to peak in winter, but recent studies show this varies by region. Our study helps address the challenge decision‐makers face in anticipating and preparing for AR events by providing insights into the consistency of peak seasonal patterns across different areas. Some regions, like East Asia, and the British Columbia coast, show a consistent peak season, while others, like the South Atlantic and parts of Australia, have significant year‐to‐year variations, making it hard to identify a dominant season. To better understand these changes over time, the study also examines how moisture moves in the atmosphere, using Integrated Vapor Transport (which looks at moisture movement in various directions) and Moist Wave Activity (which tracks moisture shifts from lower to higher latitudes). The findings suggest that inconsistencies in AR patterns are due not only to detection methods but also due to changes in moisture transport. Key Points The peak season of atmospheric river activity can change depending on the year in some areas Interannual variations in the peak season can make identifying a dominant season challenging for some regions Frequent shifts in peak season across years reflect inconsistencies tied to detection algorithms and to underlying dynamics

Kamnani, Diya↗

Renormalized site density functional theory

Site density functional theory (SDFT) provides a rigorous framework for statistical mechanics analysis of inhomogeneous molecular liquids. The key defining feature of these systems is the presence of two very distinct interactions scales (intra- and inter-molecular), and as such proper description of both effects is critical to the accuracy of the calculations. Current SDFT applications utilize the same approximation scheme for both interaction motifs, which negatively impacts the results. Dual space methodology, used in this work, alleviates this issue by providing the flexibility of evaluating part of the interactions in traditional field representation. For molecular liquid this translates into retaining density representation for inter-molecular interactions but describing stiff intra-molecular remainder by more appropriate conventional field based methods. This opens the way to decouple analysis of the two interactions scales - the idea which is developed further in this work for the case of homogeneous reference approximation of inter-molecular interactions. We demonstrate that by defining new collective variables, the behavior of the original molecular liquid system at the inter-molecular level can be transformed to resemble that of an effective simple fluid mixture. The latter is linked to intra-molecular scale through renormalized interaction parameters. We illustrate this renormalization procedure for several types of diatomic liquids, showing that this approach cures many of the shortcomings of existing SDFT methods.

Chuev, Gennady N.↗

Detailed study of quark-hadron duality in spin structure functions of the proton and neutron

Background: The response of hadrons, the bound states of the strong force (QCD), to external probes can be described in two different, complementary frameworks: as direct interactions with their fundamental constituents, quarks and gluons, or alternatively as elastic or inelastic coherent scattering that leaves the hadrons in their ground state or in one of their excited (resonance) states. The former picture emerges most clearly in hard processes with high momentum transfer, where the hadron response can be described by the perturbative expansion of QCD, while at lower energy and momentum transfers, the resonant excitations of the hadrons dominate the cross section. The overlap region between these two pictures, where both yield similar predictions, is referred to as quark-hadron duality and has been extensively studied in reactions involving unpolarized hadrons. Some limited information on this phenomenon also exists for polarized protons, deuterons, and 3 He nuclei, but not yet for neutrons. Purpose: In this paper, we present comprehensive and detailed results on the correspondence between the extrapolated deep inelastic structure function g 1 of both the proton and the neutron with the same quantity measured in the nucleon resonance region. Thanks to the fine binning and high precision of our data, and using a well-controlled perturbative QCD (pQCD) fit for the partonic prediction, we can make quantitative statements about the kinematic range of applicability of both local duality and global duality. Method: We use the most updated QCD global analysis results at high x from the Jefferson Lab Angular Momentum Collaboration to extrapolate the spin structure function g 1 into the nucleon resonance region and then integrate over various intervals in the scaling variable x. We compare the results with the large data set collected in the quark-hadron transition region by the CLAS Collaboration, including, for the first time, deconvoluted neutron data, integrated over the same intervals. We present this comparison as a function of the momentum transfer Q 2 . Results: We find that, depending on the integration interval and the minimum momentum transfer chosen, a clear transition to quark-hadron duality can be observed in both nucleon species. Furthermore, we show, for the first time, the approach to scaling behavior for g 1 measured in the resonance region at sufficiently high momentum transfer. Conclusions: Here, our results can be used to quantify the deviations from the applicability of pQCD for data taken at moderate energies and can help with extraction of quark distribution functions from such data.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Empirical radius formulas for canonical neutron stars from bidirectionally selecting features of equations of state in extended Bayesian analyses of observational data

Significant advancement in Bayesian inference of nuclear equation of state (EOS) from gravitational wave and x-ray observations of neutron stars (NSs) has been made by the nuclear astrophysics community especially since GW170817. By extending the traditional Bayesian analysis which normally ends at presenting the marginalized posterior probability distribution functions (PDFs) of individual EOS parameters and their correlations (or sometimes only the Pearson correlation coefficients which are only reliably useful when the variables are linearly correlated while they are actually often not), we search for a data-driven and robust empirical formula for the radius 𝑅 1.4 of canonical NSs in terms of the characteristic EOS parameters (features). We also identify the single most important but currently poorly known EOS parameter for determining the 𝑅 1.4 . Using three regression-model-building methodologies: bidirectional stepwise feature selection, least absolute shrinkage selection operator (LASSO) regression, and neural network regression on a large set of posterior EOSs and the corresponding 𝑅 1.4 values inferred from earlier comprehensive Bayesian analyses of NS observational data, we systematically and rigorously develop the most probable 𝑅 1.4 formulas with varying statistical accuracy and technical complexity. Here, the most important EOS parameters for determining 𝑅 1.4 are found consistently in each of the feature selection processes to be (in order of decreasing importance): curvature 𝐾 sym , slope 𝐿, skewness 𝐽 sym of nuclear symmetry energy, skewness 𝐽 0 , incompressibility 𝐾 0 of symmetric nuclear matter, and the magnitude 𝐸 sym ⁡(𝜌 0 ) of symmetry energy at the saturation density 𝜌 0 of nuclear matter.

Bayesian methods↗

Enhancing Short-Range Weather Forecasts through Temporal Variation Encoding: A Multiperiod Embedding Approach

Machine learning (ML) techniques have emerged as promising approaches to improve regional weather forecast accuracy and reliability through data-driven methods. We propose a novel ML-based weather forecasting model, the Multiperiod Embed Net (MPENet). A key distinguishing feature of MPENet is its explicit utilization of the inherent cyclic nature in weather dynamics, unlike the autoregressive strategies commonly used in other ML weather forecasting approaches. Critical cyclic structures are identified via Fourier analyses of dynamic time series. Cyclicity in the convolutional representation is achieved by transforming one-dimensional time series of meteorological variables into two-dimensional tensors based on identified periods. This approach enables the model to leverage intrinsic weather patterns, enhancing regional forecast performance. To demonstrate the effectiveness of MPENet, we conduct a comparative analysis with Nvidia’s FourCastNet. Both models are trained on High-Resolution Rapid Refresh (HRRR) data from 2015 to 2022, over a 192 km × 192 km region in Tennessee. The comparisons are performed locally at two specific locations known to have different weather dynamics due to orographic effects: Crossville, on the relatively flat Cumberland Plateau with fewer topographic airflow disruptions, and Oak Ridge, in the ridge-and-valley region, where airflow is heavily influenced by surrounding valleys and mountains. Our results indicate that FourCastNet achieves strong accuracy at very short lead times, while MPENet maintains competitive skill and shows advantages in capturing temporal evolution over longer periods. Cross-correlation analyses of MPENet and FourCastNet predictions with the HRRR data suggest that encoding critical cyclicity into the network architecture leads to improvements in the forecasting skill.

Artificial intelligence↗

Time dependent supervisory control update with FARM using rolling window

This report describes improvements to the Feasible Actuator Range Modifier (FARM) component of the RAVEN-based HYBRID framework for analysis of Integrated Energy Systems (IES). FARM supports the HERON plug-in that solves the power dispatch problem. The solution to the dispatch problem involves economically optimal dispatches that satisfy limits on production variables and their rates of variation (explicit constraints) as well as process variables tied to the service life of equipment (implicit constraints). FARM serves to validate or confirm that a HERON solution for explicit constraints also satisfies the implicit constraints. FARM-alpha was released by Argonne National Laboratory in January 2021 followed by FARM-Beta in January 2022 with the latter providing increased flexibility for the user. In this report, FARM-Gamma, the latest version of the code, is described. The major improvement is the implementation of a system identification algorithm based on the Dynamic Mode Decomposition with Control (DMDc) coupled with a “Rolling Window” scheme that allows obtaining linear time-varying state-space models. This feature equips FARM with the most accurate approximation of system dynamics, and it relieves the user from the burden of performing an exhaustive off-line characterization of the dynamics. FARM-Gamma capabilities are assessed by solving the power dispatch problem for a representative IES unit. The simulation times corresponding to the different releases are estimated and compared. These values capture the increasing computational burden of the successively higher fidelity state-space models adopted by FARM-Alpha, FARM-Beta and FARM-Gamma. The code implementation provides significant flexibility, i.e., the user can always select the most suitable version of FARM according to the problem to be solved and the available computational resources. It is anticipated that FARM will play a role in addressing several future IES applications. We outline how it can support the coordinated management and safe operation of a nuclear plant coupled to industrial processes to produce hydrogen and synfuels.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Proteomic Tissue-Based Classifier for Early Prediction of Prostate Cancer Progression

Although ~40% of screen-detected prostate cancers (PCa) are indolent, advanced-stage PCa is a lethal disease with 5-year survival rates around 29%. Identification of biomarkers for early detection of aggressive disease is a key challenge. Starting with 52 candidate biomarkers, selected from existing PCa genomics datasets and known PCa driver genes, we used targeted mass spectrometry to quantify proteins that significantly differed in primary tumors from PCa patients treated with radical prostatectomy (RP) across three study outcomes: (i) metastasis ≥1-year post-RP, (ii) biochemical recurrence ≥1-year post-RP, and (iii) no progression after ≥10 years post-RP. Sixteen proteins that differed significantly in an initial set of 105 samples were evaluated in the entire cohort (n = 338). A five-protein classifier which combined FOLH1, KLK3, TGFB1, SPARC, and CAMKK2 with existing clinical and pathological standard of care variables demonstrated significant improvement in predicting distant metastasis, achieving an area under the receiver-operating characteristic curve of 0.92 (0.86, 0.99, p = 0.001) and a negative predictive value of 92% in the training/testing analysis. This classifier has the potential to stratify patients based on risk of aggressive, metastatic PCa that will require early intervention compared to low risk patients who could be managed through active surveillance.

60 APPLIED LIFE SCIENCES↗

Modulation of springtime surface sensible heating over the Tibetan Plateau on the interannual variability of East Asian dust cycle

Previous observational evidence and numerical simulations have revealed that the surface sensible heating in spring (March–April–May, MAM) over the Tibetan Plateau (TPSH) can affect the Asian regional hydrological cycle, surface energy balance, and climate through altering atmospheric heat source of the Tibetan Plateau (TP). This study aims to investigate the impacts of MAM TPSH on the interannual variability of East Asian dust cycle by using CAM4-BAM (version 4 of the Community Atmosphere Model coupled to a bulk aerosol model), MERRA-2 (version 2 of the Modern-Era Retrospective analysis for Research and Applications) surface dust concentration, and TPSH measurements. Our simulations show that the surface dust concentrations over the East Asian (EA) dust source region and over the northwestern Pacific (NP) in MAM are significantly positively correlated with TPSH, with regionally averaged correlation coefficients of 0.49 for EA and 0.44 for NP. Similar positive correlations are also shown between the MAM TPSH measurements averaged over the 73 observation sites and the surface dust concentration from MERRA-2. Simulation-based comparisons between strongest and weakest TPSH years reveal that, the MAM surface dust concentration in the strongest TPSH years increases with relative differences of 13.1 % over EA and 36.9 % over NP. These corresponding differences are found in MERRA-2 with 22.9 % and 13.3 % over EA and NP, respectively. Further simulated results show that the processes of whole dust cycles (e.g., dust loading, emission, and transport, as well as dust deposition) are also significantly enhanced during the strongest TPSH years over EA and NP. Through enhancing the TP heat source, stronger TPSH in MAM generates an anticyclonic anomaly in middle and upper troposphere over the TP and over the downstream Pacific region, respectively. These atmospheric circulation anomalies induced by the increased TPSH result in increasing the westerly winds over both EA and NP, which in turn increases dust emissions over the dust source, and dust transport over these two regions, as well as the regional dust cycles. These results suggest that addressing the East Asian dust changes in the future climates requires considering not only increasing greenhouse gas emissions but also the variations of the TP's heat source under global warming.

54 ENVIRONMENTAL SCIENCES↗

Observations of high-time-resolution and size-resolved aerosol chemical composition and microphysics in the central Arctic: implications for climate-relevant particle properties

Abstract. Aerosols play a critical role in the Arctic's radiative balance, influencing solar radiation and cloud formation. Limited observations in the central Arctic leave gaps in understanding aerosol dynamics year-round, affecting model predictions of climate-relevant aerosol properties. Here, we present the first annual high-time-resolution observations of submicron aerosol chemical composition in the central Arctic during the Arctic Ocean 2018 (AO2018) and the 2019–2020 Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expeditions. Seasonal variations in the aerosol mass concentrations and chemical composition in the central Arctic were found to be driven by typical Arctic seasonal regimes and resemble those of pan-Arctic land-based stations. Organic aerosols dominated the pristine summer, while anthropogenic sulfate prevailed in autumn and spring under haze conditions. Ammonium, which impacts aerosol acidity, was consistently less abundant, relative to sulfate, in the central Arctic compared to lower latitudes of the Arctic. Cyclonic (storm) activity was found to have a significant influence on aerosol variability by enhancing emissions from local sources and the transport of remote aerosol. Local wind-generated particles contributed up to 80 % (20 %) of the cloud condensation nuclei population in autumn (spring). While the analysis presented herein provides the current central Arctic aerosol baseline, which will serve to improve climate model predictions in the region, it also underscores the importance of integrating short-timescale processes, such as seasonal wind-driven aerosol sources from blowing snow and open leads/ocean in model simulations. This is particularly important, given the decline in mid-latitude anthropogenic emissions and the increase in local ones.

Heutte, Benjamin (ORCID:0000000173727460)↗

Near-Surface Hydrology and Soil Properties Drive Heterogeneity in Permafrost Distribution, Vegetation Dynamics, and Carbon Cycling in a Sub-Arctic Watershed: Modeling Archive

This Modeling Archive is in support of a NGEE-Arctic publication: Shirley et al. (2022) “Near-Surface Hydrology and Soil Properties Drive Heterogeneity in Permafrost Distribution, Vegetation Dynamics, and Carbon Cycling in a Sub-Arctic Watershed". [DOI].The dataset contains outputs from the global sensitivity analysis (GSA) of the “ecosys” model as reported in Shirley et al. (2022). The study showed that discontinuous permafrost environments are characterized by complex feedback loops and strong spatial heterogeneity which is created by variability in near-surface hydrology and soil properties. Additionally, the study demonstrated that missing representation of sub-grid heterogeneity in terrestrial ecosystem models can lead to biased estimates of the high-latitude carbon budget. Included in this dataset are the factor values for each run in the GSA and the model outputs used in this study. Included are two *.csv data files and one *.pdf.The Next-Generation Ecosystem Experiments: Arctic (NGEE Arctic), was a research effort to reduce uncertainty in Earth System Models by developing a predictive understanding of carbon-rich Arctic ecosystems and feedbacks to climate. NGEE Arctic was supported by the Department of Energy's Office of Biological and Environmental Research.The NGEE Arctic project had two field research sites: 1) located within the Arctic polygonal tundra coastal region on the Barrow Environmental Observatory (BEO) and the North Slope near Utqiagvik (Barrow), Alaska and 2) multiple areas on the discontinuous permafrost region of the Seward Peninsula north of Nome, Alaska.Through observations, experiments, and synthesis with existing datasets, NGEE Arctic provided an enhanced knowledge base for multi-scale modeling and contributed to improved process representation at global pan-Arctic scales within the Department of Energy's Earth system Model (the Energy Exascale Earth System Model, or E3SM), and specifically within the E3SM Land Model component (ELM).

54 ENVIRONMENTAL SCIENCES↗