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At least 1,261 records · Page 70

Tight Bound on the Neutron Star Radius with Quasiperiodic Oscillations in Short Gamma-Ray Bursts

Abstract Quasiperiodic oscillations (QPOs) have been recently discovered in the short gamma-ray bursts (GRBs) 910711 and 931101B. Their frequencies are consistent with those of the quasiradial and quadrupolar oscillations of binary neutron star (BNS) merger remnants, as obtained in numerical relativity simulations. These simulations reveal quasi-universal relations between the remnant oscillation frequencies and the tidal coupling constant of the binaries. Under the assumption that the observed QPOs are due to these postmerger oscillations, we use the frequency–tide relations in a Bayesian framework to infer the source redshift, as well as the chirp mass and the binary tidal deformability of the BNS progenitors for GRBs 910711 and 931101B. We further use this inference to estimate bounds on the mass–radius relation for neutron stars. By combining the estimates from the two GRBs, we find a 68% credible range R 1.4 = 12.4 8 − 0.40 + 0.41 km for the radius of a neutron star with mass M = 1.4 M ⊙ , which is one of the tightest bounds to date.

Guedes, Victor↗

In situ observation of irradiation-induced enhancement to the desorption pressure of zirconium hydride in a nuclear reactor

We quantify the effect of a nuclear-reactor environment on the hydrogen isotope equilibrium vapor pressure over pure zirconium and zirconium hydride. A vacuum-sealed capsule containing a zirconium foil with 6 atom% deuterium was irradiated at a neutron flux of ~10 14 cm -2 s -1 at the University of Missouri Research Reactor (MURR). The internal stainless-steel (SS) sample holder acted as the heat source via gamma absorption. To measure low desorption pressures in a high-flux environment, we developed a method to transduce pressure from the measured sample temperature during irradiation, calibrating with known deuterium pressures in unirradiated capsules at various heating powers using an internal filament-heated system designed to mimic irradiation-induced heating. Our temperature-pressure transduction method operates similarly to a Pirani or thermocouple pressure gauge. The in-reactor measurements revealed a roughly 4-fold enhancement in desorption pressure after only 6 h of irradiation (~2 × 10 18 cm -2 neutron fluence) compared to thermal desorption in control experiments, indicating a nonthermal contribution from neutron irradiation. The slower temperature/pressure stabilization rate in the reactor suggests that desorption pressure enhancement increases with neutron fluence. Further, this enhancement signifies increased solubility of hydrogen isotopes in zirconium during irradiation. We propose that high-energy neutron collisions with hydrogen isotopes in hydrides lead to their decomposition at lower temperatures, supersaturating the surrounding αZr lattice and resulting in higher desorption pressure, which continues to rise as more hydrides dissolve with increasing neutron fluence.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Review of recent activities with MOOSE, an open-source finite element & finite volume multi-fidelity simulation framework

Modeling and simulation are an increasing part of engineering. This is undoubtedly driven by the high costs of constructing experimental facilities, but also enabled by the exponential increase in computing powers over the last decades, which allows computational models to be closer than ever to reality. One of the main drivers for the development of MOOSE is supporting advanced nuclear reactor simulations. A challenging aspect of modeling advanced nuclear reactors is the plurality of physics involved, including neutronics, thermal hydraulics and fuel performance. These physics are all coupled to some extent and are generally solved in a sequential but iterative fashion. The United States (U.S.) national laboratories have been developing MOOSE, an open source multiphysics framework since its inception at the Idaho National Laboratory (INL) in 2008. This framework enables seamless coupling of multiphysics simulations and facilitates the implementation of new physics and material governing laws. It is continuously expanded with novel numerical methods and new pre-implemented physics module. Numerous applications, developed within the Department of Energy (DOE) laboratories, academia, and industry, including outside of nuclear engineering, have been developed to study specialized physics problems. International collaborations are welcome on this open-source modeling and simulation project.

22 - GENERAL STUDIES OF NUCLEAR REACTORS↗

Multigroup Neutron Transport Using a Collision-Based Hybrid Method

A collision-based hybrid algorithm for the discrete ordinates approximation of the neutron transport equation is extended to the isotropic multigroup setting. The algorithm uses discrete energy and angle grids at two different resolutions and approximates the fission and scattering sources on the coarser grids. The coupling of a collided transport equation, discretized on the coarse grid, with an uncollided transport equation, discretized on the fine grid, yields an algorithm that, in most cases, is more efficient than the traditional multigroup approach. In conclusion, the improvement over existing techniques is demonstrated for time-dependent problems with different materials, geometries, and energy groups.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Interfacial alloying contributions to the magnetic proximity effect in Pt/dysprosium iron garnet

The magnetic proximity effect (MPE), a magnetic response from a heavy metal layer induced by an adjacent magnetic layer, plays an important role in the behavior of heavy-metal/ferro- or ferrimagnet thin film heterostructures. However, in the case of heavy-metal/rare earth iron garnet bilayers the presence and magnitude of the MPE has been debated. We previously reported an MPE in a Pt/dysprosium iron garnet (DyIG) heterostructure where the two layers were grown without breaking vacuum, finding that the magnetic moment present in the Pt layer scales with the magnitude of the DyIG moment and varies nonmonotonically through the DyIG compensation temperature. However, the origin of the magnetic signal from the Pt layer was not identified. In contrast, Pt/DyIG grown with a vacuum break did not exhibit an MPE. Here we investigate the origin of the magnetic moment in the Pt layer using x-ray absorption spectroscopy, x-ray circular dichroism, composition mapping and simulations of ion bombardment. In conclusion, the results are consistent with the presence of an intermixed Fe-Dy-Pt interfacial alloy layer formed during the growth of the Pt on the DyIG and resulting in a measurable MPE.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

3D xRAGE simulation of inertial confinement fusion implosion with imposed mode 2 laser drive asymmetry

Low-mode asymmetries represent an important obstacle to achieving high-gain inertial confinement fusion implosions. As a step in learning how to control such effects, an OMEGA experiment with imposed mode 2 laser drive asymmetries was done to study the expected signatures of this type of asymmetry [M. Gatu Johnson et al., PRE 2018]. In the present work, a 3D xRAGE simulation including the stalk mount has been brought to bear on the data from that experiment. Furthermore, comprehensive comparisons between simulated and measured observables are made. Good agreement between simulated and measured x-ray image-inferred shell trajectories, bang times and neutron emission widths are seen, showing that the hydrodynamics are well captured in the simulation. Asymmetries seen in simulated and measured time-resolved and time-integrated x-ray images and areal densities also compare well, showing impact of both stalk and mode 2. On the other hand, important differences in measured and simulated neutron emission histories, yield, and ion temperature (T ion ) asymmetries are seen, suggesting that the simulation is overestimating shock yield. Overall, the results clearly demonstrate the importance of considering all asymmetry sources when interpreting measured signatures of asymmetry.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Robustness of neutron star merger simulations to changes in neutrino transport and neutrino-matter interactions

Binary neutron star mergers play an important role in nuclear astrophysics: Their gravitational wave and electromagnetic signals carry information about the equation of state of cold matter above nuclear saturation density, and they may be one of the main sources of r-process elements in the Universe. Neutrino-matter interactions during and after merger impact the properties of these electromagnetic signals and the relative abundances of the produced r-process elements. Existing merger simulations are, however, limited in their ability to realistically model neutrino transport and neutrino-matter interactions. Here, we perform a comparison of the impact of the use of state-of-the art two-moment or Monte Carlo transport schemes on the outcome of merger simulations, for a single binary neutron star system with a short-lived neutron star remnant [(5–10) ms]. We also investigate the use of different reaction rates in the simulations. While the best transport schemes generally agree well on the qualitative impact of neutrinos on the system, differences in the behavior of the high-density regions can significantly impact the collapse time and the properties of the hot tidal arms in this metastable merger remnant. The chosen interaction rates and transport algorithm as well as recent improvements by Radice et al. to the two-moment algorithms can all contribute to changes at the (10–30)% level in the global properties of the merger remnant and outflows. Furthermore, the limitations of previous moment schemes fixed by Radice et al. also appear sufficient to explain the large difference that we observed in the production of heavy-lepton neutrinos in a previous comparison of Monte Carlo and moment schemes in the context of a low-mass binary neutron star system.

79 ASTRONOMY AND ASTROPHYSICS↗

Testing claims of the GW170817 binary neutron star inspiral affecting β-decay rates

On August 17, 2017, the first gravitational wave signal from a binary neutron star inspiral (GW170817) was detected by Advanced LIGO and Advanced VIRGO. Here we present radioactive β-decay rates of three independent sources 44 Ti, 60 Co and 137 Cs, monitored during the same period by a precision experiment designed to investigate the decay of long-lived radioactive sources. We do not find any significant correlations between decay rates in a 5 h time interval following the GW170817 observation. This contradicts a previous claim published in this journal of an observed 2.5σ Pearson Correlation between fluctuations in the number of observed decays from two β-decaying isotopes ( 32 Si and 36 Cl) in the same time interval. By correcting for the choice of an arbitrary time interval, we find no evidence of a correlation above 1.5σ confidence. In addition, we argue that such analyses on correlations in arbitrary time intervals should always correct for the so-called Look-Elsewhere effect by quoting the global significance.

79 ASTRONOMY AND ASTROPHYSICS↗

Review of uncertainties in the cosmic supernova relic neutrino background

We review the computation of and associated uncertainties in the current understanding of the relic neutrino background due to core-collapse supernovae, black hole formation and neutron star merger events. We consider the current status of uncertainties due to the nuclear equation of state (EoS), the progenitor masses, the source supernova neutrino spectrum, the cosmological star formation rate, the stellar initial mass function, neutrino oscillations, and neutrino self-interactions. We summarize the current viability of future neutrino detectors to distinguish the nuclear EoS and the temperature of supernova neutrinos via the detected relic supernova neutrino spectrum.

Astronomy & Astrophysics↗

Imaging electric field with electrically neutral particles

It used to think that is impossible to determine/measure electric field inside a physically isolated volume, especially inside an electrically shielded space, because a conventional electric-field sensor can only measure electric field at the location of the sensor, and when an electric-field source is screened by conductive materials, no leakage electric field can be detected. For first time, we experimentally demonstrated that electrically neutral particles, neutrons, can be used to measure/image electric field behind a physical barrier. This work enables a new measurement capability that can visualize electric-relevant properties inside a studied sample or detection target for scientific research and engineering applications.

42 ENGINEERING↗

Subcriticality Measurements for a Changing Concentration Uranyl Nitrate Solution Tank by Californium Source-Driven Noise Analysis

Subcritical californium source-driven noise analysis (CSDNA) measurements were performed at the Oak Ridge Critical Experiments Facility in 1983 using a stainless-steel tank with an inside diameter of 76.2 cm and a height of 91.4 cm but only filled with a uranyl (93.16 wt.% 235 U) nitrate solution to a height of 76.2 cm for all measurements. The free acid content of the uranyl nitrate solution was less than 0.01 N to minimize hazards in handling. The total available highly enriched uranium for these measurements was 5,296 g. The concentration of the solution was varied from the highest density of 14.71 grams of uranium per liter (g U/L) initially in 16 steps, lowering the concentration to 0.3492 g U/L, and finally using a tank filled with only water. The tank had a Plexiglas lid to minimize evaporation. The Cf source was contained in a re-entrant Lexan tube which could be in the solution parallel to the axis of the cylindrical tank. The detectors were 3 He proportional counters in the solution in shrink-fit tubing to isolate the counters from the fissile solution and adjacent to the outside of the tank. In some cases, the detectors were scintillators adjacent to the outside of the tank. In other cases, the source was external to the tank. Some data presented in this report are from notes and are not in the logbook. The prompt neutron decay constant was obtained from fitting the date from the CSDNA measurements. The purpose of this report is to document the experimental information for the measurements performed so that later, researchers could perform the required uncertainty and calculational analyses and documentation to use these data for an International Nuclear Criticality Safety Benchmark Program (ICSBEP) or a Nuclear Energy Agency benchmark. The prompt neutron decay measurements could be the basis of as International Reactor Physic Benchmark Program. The data from these measurements are available from the Records Management Services Department of Oak Ridge National Laboratory, and the logbook is also available from the ICSBEP at Idaho National Laboratory. Preparation of the present report is part of a larger cooperative effort between Idaho National Laboratory (INL) and Oak Ridge National Laboratory (ORNL) to document more than 15 undocumented critical and subcritical experiments enumerated in ORNL/TM-2019/18 and performed by ORNL at ORCEF and other USDOE critical experiments facilities using more than 500 operational days of critical facility time.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗

The Challenges Ahead for Multimessenger Analyses of Gravitational Waves and Kilonova: A Case Study on GW190425

In recent years, there have been significant advances in multimessenger astronomy due to the discovery of the first, and so far only confirmed, gravitational wave event with a simultaneous electromagnetic (EM) counterpart, as well as improvements in numerical simulations, gravitational wave (GW) detectors, and transient astronomy. This has led to the exciting possibility of performing joint analyses of the GW and EM data, providing additional constraints on fundamental properties of the binary progenitor and merger remnant. Here, in this work, we present a new Bayesian framework that allows inference of these properties, while taking into account the systematic modeling uncertainties that arise when mapping from GW binary progenitor properties to photometric light curves. We extend the relative binning method presented in Zackay et al. to include extrinsic GW parameters for fast analysis of the GW signal. The focus of our EM framework is on light curves arising from r-process nucleosynthesis in the ejected material during and after merger, the so-called kilonova, and particularly on black hole–neutron star systems. As a case study, we examine the recent detection of GW190425, where the primary object is consistent with being either a black hole or a neutron star. We show quantitatively how improved mapping between binary progenitor and outflow properties, and/or an increase in EM data quantity and quality are required in order to break degeneracies in the fundamental source parameters.

79 ASTRONOMY AND ASTROPHYSICS↗

Generalized method for the optimization of pulse shape discrimination parameters

Organic scintillators exhibit fast timing, high detection efficiency for fast neutrons and pulse shape discrimination (PSD) capability. PSD is essential in mixed radiation fields, where different types of radiation need to be detected and discriminated. In neutron measurements for nuclear security and non proliferation effective PSD is crucial, because a weak neutron signature needs to be detected in the presence of a strong gamma-ray background. Here, the most commonly used deterministic PSD technique is charge integration (CI). This method requires the optimization of specific parameters to obtain the best gamma-neutron separation. These parameters depend on the scintillating material and light readout device and typically require a lengthy optimization process and a calibration reference measurement with a mixed source. In this paper, we propose a new method based on the scintillation fluorescence physics that enables to find the optimum PSD integration gates using only a gamma-ray emitter. We demonstrate our method using three organic scintillation detectors: deuterated trans-stilbene, small-molecule organic glass, and EJ-309. In all the investigated cases, our method allowed finding the optimum PSD CI parameters without the need of iterative optimization.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Nuclear Data for Spallation Neutron Radioisotope Production (Final Technical Report)

Over 50 million nuclear medicine procedures are performed annually, leading to a multi-billion dollar market for radioisotope production. The demand for new medical and research isotopes is growing, and radioisotope supply is insufficient. Most radioisotope production today utilizes charged particle or low-energy neutron irradiation of a target. Isotope production with tens to hundred MeV incident energies is a relatively unexplored option. There is a tremendous opportunity associated with a growing number of suitable domestic and international facilities buttressed by hundred million dollar global investments (e.g., the Los Alamos and Brookhaven Isotope Production Facilities, the European Spallation Source in Lund, and the Korean Multi-purpose Accelerator Complex in Gyeongbuk). In part due to a lack of supporting nuclear data that would make modeling radioisotope yields and purities possible, these facilities do not utilize their high-energy neutron fluxes for isotope production. This project attempted to measure neutron reaction excitation functions relevant to the large-scale production of critical radioisotopes, enabling development of cost-efficient isotope production methods, contributing to the improvement of theoretical models, and enhancing the value of national isotope production facilities. Reactions which form 67 Cu, 32 Si, and alpha-emitting isotopes like 225 Ac were chosen for their consistent prioritization by expert panels, representation of diverse reaction mechanisms, and relative lack of supporting nuclear data. Accurate measurement of these data is presently made only using quasi-monoenergetic neutron beams, which are produced by bombarding thin lithium targets with protons at only a few laboratories in the world. Ultimately, the projects efforts were incompletely accomplished due to a combination of multi-year technical issues at the only laboratory in the world which can make the proposed measurements, iThemba Labs in South Africa, and the onset of a global pandemic, which precluded the significant effort and time required to develop an independent measurement capability in the United States.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

Solid, structured composite neutron detectors with high dynamic range capability

Neutron detectors are essential across disciplines such as fundamental science, nuclear security, safeguards, and civilian applications. While 3 He-filled gas proportional counters have long been revered for their efficacy in detecting thermal neutrons and praised for their efficiency, neutron/gamma discrimination, and stability, the scarcity of 3He has spurred a search for alternatives. Here, we explore a solid structured scintillating particle composite (SPC) consisting of 6 Li-containing scintillating glass particles within an acrylic matrix as a neutron detector for high dynamic range applications. We show for the first time that an SPC neutron detector can boast an intrinsic detection efficiency of 0.261% for pure 252 Cf fission neutrons and an overall neutron detection efficiency of (0.546 ± 0.003)% at the Neutron Free-in-Air facility while being able to function in an intense gamma-ray environment. We also show that the SPC neutron detector supports fast neutron capture times and enables a dual-readout scheme that extends the detector dynamic range to high incident neutron fluxes. A scalable fabrication process allows for tailoring the SPC detector properties to the requirements of specific applications. Good agreement is found between the experimental results taken with a National Institute of Standards and Technology traceable 252 Cf source and the coupled MCNP6 and optical-ray-tracing simulations.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Neutron resonance transmission analysis prototype system for thorium fuel cycle safeguards

Emerging thorium-based reactor designs and fuel cycles present challenges to traditional non-destructive assay techniques used in international safeguards. Specifically, assaying the masses of 233 U and 235 U when they are present together in samples with high gamma ray backgrounds is difficult because of similar passive neutron signatures and relatively weak gamma-ray emissions of 233 U. The Pacific Northwest National Laboratory (PNNL) and the Massachusetts Institute of Technology (MIT) are developing a compact neutron resonance transmission analysis (NRTA) system as one potential solution to these challenges. The NRTA technique provides isotopic information for a sample via neutron time-of-flight (TOF) measurements that exploit a sample’s epithermal neutron resonance cross-sections. A recently developed portable NRTA system uses a commercially available, pulsed deuterium-tritium neutron generator with a ~2 m flight path and a GS20 lithium glass scintillator detector. Finally, this paper describes the prototype NRTA system design, a refined radiation transport model of the system, preliminary measurements with thorium and uranium sources, and demonstration of a quantitative isotopic estimation algorithm.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Improved MPACT energy deposition and explicit heat generation coupling with CTF

The CASL neutronics code MPACT assumes local energy deposition with equilibrium delayed energy for steady-state and transient calculations. These approximations limit the accurate representation of the heat generation in space and its variations over time, both of which are essential for power distribution and thermal–hydraulic coupling analyses. This paper presents an explicit energy deposition model considering the neutron and gamma heating of all regions and the time-dependent delayed energy. The MPACT/CTF interfaces are updated to transfer the explicit heat sources. The new model agrees well with MCNP for problems without thermal–hydraulic feedback. The MPACT/CTF coupled calculation for a hot-full-power quarter-core case using the new model exhibits a reduction of peak pin power by 2.3% and fuel centerline temperature by 17 K. The new model also shows a keff difference up to -100 pcm in depletion and a 30 K peak fuel temperature reduction in a reactivity-initiated-accident problem.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗