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At least 1,261 records · Page 70

The Acceleration of Energetic Particles at Coronal Shocks and Emergence of a Double Power-law Feature in Particle Energy Spectra

We present numerical modeling of particle acceleration at coronal shocks propagating through a streamer-like magnetic field by solving the Parker transport equation with spatial diffusion both along and across the magnetic field. We show that the location on the shock where the high-energy particle intensity is the largest, depends on the energy of the particles and on time. The acceleration of particles to more than 100 MeV mainly occurs in the shock-streamer interaction region, due to perpendicular shock geometry and the trapping effect of closed magnetic fields. A comparison of the particle spectra to that in a radial magnetic field shows that the intensity at 100 MeV (200 MeV) is enhanced by more than one order (two orders) of magnitude. This indicates that the streamer-like magnetic field can be an important factor in producing large solar energetic particle events. We also show that the energy spectrum integrated over the simulation domain consists of two different power laws. Further analysis suggests that it may be a mixture of two distinct populations accelerated in the streamer and open field regions, where the acceleration rate differs substantially. Our calculations also show that the particle spectra are affected considerably by a number of parameters, such as the streamer tilt angle, particle spatial diffusion coefficient, and shock compression ratio. While the low-energy spectra agree well with standard diffusive shock acceleration theory, the break energy ranges from ~1 MeV to ~90 MeV and the high-energy spectra can extend to ~1 GeV with a slope of ~2–3.

97 MATHEMATICS AND COMPUTING↗

Thermodynamic properties and enhancement of diamagnetism in nitrogen doped lutetium hydride synthesized at high pressure

Nitrogen doped lutetium hydride has drawn global attention in the pursuit of room-temperature superconductivity near ambient pressure and temperature. However, variable synthesis techniques and uncertainty surrounding nitrogen concentration have contributed to extensive debate within the scientific community about this material and its properties. We used a solid-state approach to synthesize nitrogen doped lutetium hydride at high pressure and temperature (HPT) and analyzed the residual starting materials to determine its nitrogen content. High temperature oxide melt solution calorimetry determined the formation enthalpy of LuH 1.96 N 0.02 (LHN) from LuH 2 and LuN to be −28.4 ± 11.4 kJ/mol. Magnetic measurements indicated diamagnetism which increased with nitrogen content. Ambient pressure conductivity measurements observed metallic behavior from 5 to 350 K, and the constant and parabolic magnetoresistance changed with increasing temperature. High pressure conductivity measurements revealed that LHN does not exhibit superconductivity up to 26.6 GPa. We compressed LHN in a diamond anvil cell to 13.7 GPa and measured the Raman signal at each step, with no evidence of any phase transition. Despite the absence of superconductivity, a color change from blue to purple to red was observed with increasing pressure. Thus, our findings confirm the thermodynamic stability of LHN, do not support superconductivity, and provide insights into the origins of its diamagnetism.

Science & Technology - Other Topics↗

Evolution of Magnetohydrodynamic Turbulence in the Expanding Solar Wind: Residual Energy and Intermittency

We conduct 3D magnetohydrodynamic simulations of decaying turbulence in the context of the solar wind. To account for the spherical expansion of the solar wind, we implement the expanding box model. The initial turbulence comprises uncorrelated counterpropagating Alfvén waves and exhibits an isotropic power spectrum. Our findings reveal the consistent generation of negative residual energy whenever nonlinear interactions are present, independent of the normalized cross helicity σc and compressibility. The spherical expansion facilitates this process. The resulting residual energy is primarily distributed in the perpendicular direction, with S 2 (b) − S 2 (u) ∝ l ⊥ or equivalently –E r ∝ k$^{–2}_{⟂}$. Here S 2 (b) and S 2 (u) are second-order structure functions of magnetic field and velocity respectively. In most runs, S 2 (b) develops a scaling relation S 2 (b) ∝ $l$$^{1/2}_{⊥}$ (E b ∝ k$^{–3/2}_{⟂}$). In contrast, S 2 (u) is consistently shallower than S 2 (b), which aligns with in situ observations of the solar wind. We observe that the higher-order statistics of the turbulence, which act as a proxy for intermittency, depend on the initial σc and are strongly affected by the expansion effect. Generally, the intermittency is more pronounced when the expansion effect is present. Finally, we find that in our simulations, although the negative residual energy and intermittency grow simultaneously as the turbulence evolves, the causal relation between them seems to be weak, possibly because they are generated on different scales.

Interplanetary turbulence↗

Collapse and fragmentation of molecular cloud cores. 2: Collapse induced by stellar shock waves

The standard scenario for low-mass star formation involves 'inside-out' collapse of a dense molecular cloud core following loss of magnetic field support through ambipolar diffusion. However, isotopic anomalies in presolar grains and meteoritical inclusions imply that the collapse of the presolar cloud may have been triggered by a stellar shock wave. This paper explores 'outside-in' collapse, that is, protostellar collapse initiated directly by the compression of quiescent dense cloud cores impacted by relatively slow stellar shock waves. A second-order accurate, gravitational hydrodynamics code has been used to study both the spherically symmetrical and three-dimensional evolution of initially centrally condensed, isothermal, self-gravitating, solar-mass cloud cores that are struck by stellar shock waves with velocities up to 25 km/s and postshock temperatures of 10 to 10,000 K. The models show that such mild shock waves do not completely shred and destroy the cloud, and that the dynamical ram pressure can compress the cloud to the verge of self-gravitational collapse. However, compression caused by a high postshock temperature is a considerably more effective means of inducing collapse. Shock-induced collapse produces high initial mass accretion rates (greater than 10(exp -4) solar mass/yr in a solar-mass cloud) that decline rapidly to much lower values, depending on the presence (approximately 10(exp -6) solar mass/yr) or absence (approximately 10(exp -8) to 10(exp -7) solar mass/yr) of an infinite reservoir of mass. Stellar mass accretion rates approximately 10(exp -7) solar mass/yr have been previously inferred from the luminosities of T Tauri stars; balanced mass accretion (stellar rate = envelope rate) at approximately 10(exp -7) solar mass/yr could then be possible if accretion occurs from a finite mass reservoir. Fluid tracers are used to determine what fraction of the stellar shock material is incorporated into the resulting protostellar object and disk; roughly half the impinging material is injected into the collapsing cloud core when there is a high postshock temperature. The models are consistent with a scenario where an AGB star wind triggered the collapse of the presolar cloud while injecting about 0.01 solar mass of matter derived from the AGB star envelope, as has been separately inferred on the basis of nucleosynthesis calculations.

Boss, Alan P.↗

Magnetoresistance Hysteresis Evolution in the Granular Y–Ba–Cu–O High-Temperature Superconductor in a Wide Temperature Range

The temperature evolution of the magnetoresistance hysteresis in the granular YBa{sub 2}Cu{sub 3}O{sub 7-δ} high-temperature (T{sub C} ≈ 92 K) superconductor has been investigated. The measurements have been performed in the high-temperature region (78–90 K) and at the liquid helium temperature (4.2 K). The results obtained have been analyzed using the developed model of the behavior of transport properties of a granular high-temperature superconductor in an external magnetic field. Within the discussed model, the dissipation of the grain boundary subsystem is determined by the intergrain spacing-averaged effective field B{sub eff}, which is a superposition of external field H and the field induced by the magnetic moments of superconducting grains. Such a consideration yields the expression B{sub eff}(H) = H − 4πM(H) α for the effective field in the intergrain medium, where M(H) is the experimental hysteretic dependence of magnetization and α is the parameter of magnetic flux crowding in the intergrain medium. Here, the magnetoresistance is assumed to be proportional to the absolute value of the effective field: R(H) ~ |B{sub eff}(H)|. Analysis of the experimental R(H) and M(H) dependences obtained under the same conditions for the investigated high-temperature superconductor sample showed that in the high-temperature region this parameter is α ≈ 25. At the low temperature (4.2 K), we may state that the degree of flux crowding increases and the estimated α value is ~ 50. The estimates made are indicative of the strong effect of flux compression in the intergrain medium on the magnetotransport properties of the investigated granular high-temperature superconductor system. Possible reasons for a discrepancy between the developed model concepts and experimentally observed low-temperature R(H) hysteresis are analyzed.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Regimes of magnetic reconnection in colliding laser-produced magnetized plasma bubbles

Here, we conduct a multiparametric study of driven magnetic reconnection relevant to recent experiments on colliding magnetized laser-produced plasmas using particle-in-cell simulations. Varying the background plasma density, plasma resistivity, and plasma bubble geometry, the 2D simulations demonstrate a rich variety of reconnection behaviors and show the coupling between magnetic reconnection and the global hydrodynamical evolution of the system. We consider both the collision between two radially expanding bubbles where reconnection is seeded by the pre-existing X-point and the collision between two flows in a quasi-1D geometry with initially anti-parallel fields where reconnection must be initiated by the tearing instability. At a baseline case of low-collisionality and low background density, the current sheet is strongly compressed to below scale of the ion-skin-depth scale, and rapid, multi-plasmoid reconnection results. Increasing the plasma resistivity, we observe a collisional slow-down of reconnection and stabilization of plasmoid instability for Lundquist numbers less than approximately S ~10 3 . Second, increasing the background plasma density modifies the compressibility of the plasma and can also slow down or even prevent reconnection, even in completely collisionless regimes, by preventing the current sheet from thinning down to the scale of the ion-skin depth. These results have implications for understanding recent and future experiments, and signatures for these processes for proton-radiography diagnostics of these experiments are discussed.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Discrete decoding based ultrafast multidimensional nuclear magnetic resonance spectroscopy

The three-dimensional (3D) nuclear magnetic resonance (NMR) spectroscopy constitutes an important and powerful tool in analyzing chemical and biological systems. However, the abundant 3D information arrives at the expense of long acquisition times lasting hours or even days. Therefore, there has been a continuous interest in developing techniques to accelerate recordings of 3D NMR spectra, among which the ultrafast spatiotemporal encoding technique supplies impressive acquisition speed by compressing a multidimensional spectrum in a single scan. However, it tends to suffer from tradeoffs among spectral widths in different dimensions, which deteriorates in cases of NMR spectroscopy with more dimensions. In this study, the discrete decoding is proposed to liberate the ultrafast technique from tradeoffs among spectral widths in different dimensions by focusing decoding on signal-bearing sites. For verifying its feasibility and effectiveness, we utilized the method to generate two different types of 3D spectra. The proposed method is also applicable to cases with more than three dimensions, which, based on the experimental results, may widen applications of the ultrafast technique.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

H-Mat Hydrogen Compatibility of Polymers and Elastomers

The H2@Scale program of the U.S. Department of Energy (DOE) Fuel Cell Technologies Office is supporting work on the hydrogen compatibility of polymers to improve the durability and reliability of materials for hydrogen infrastructure. The hydrogen compatibility program (H-Mat) seeks “to address the challenges of hydrogen degradation by elucidating the mechanisms of hydrogen-materials interactions with the goal of providing science-based strategies to design materials, (micro)structures, and morphology with improved resistance to hydrogen degradation.” This research has observed interactions of hydrogen and pressure with model rubber-material compounds resulting in volume change and compression-set differences in the materials. The materials were investigated using helium-ion microscopy (HeIM), which revealed significant morphological changes in the plasticizer-incorporating compounds after exposure, as evidenced by time-of-flight secondary ion mass spectrometry. Additional studies using transmission electron microscopy and nuclear magnetic resonance were performed to correlate morphological change to potential chemical change in the materials.

08 HYDROGEN↗

Stirling cycle cryogenic cooler

A long lifetime Stirling cycle cryogenic cooler particularly adapted for space applications is described. It consists of a compressor section centrally aligned end to end with an expansion section, and respectively includes a reciprocating compressor piston and displacer radially suspended in interconnecting cylindrical housings by active magnetic bearings and has adjacent reduced clearance regions so as to be in noncontacting relationship therewith and wherein one or more of these regions operate as clearance seals. The piston and displacer are reciprocated in their housings by linear drive motors to vary the volume of respectively adjacent compression and expansion spaces which contain a gaseous working fluid and a thermal regenerator to effect Stirling cycle cryogenic cooling.

Gasser, M. G.↗

Noiseless coding for the magnetometer

Future unmanned space missions will continue to seek a full understanding of magnetic fields throughout the solar system. Severely constrained data rates during certain portions of these missions could limit the possible science return. This publication investigates the application of universal noiseless coding techniques to more efficiently represent magnetometer data without any loss in data integrity. Performance results indicated that compression factors of 2:1 to 6:1 can be expected. Feasibility for general deep space application was demonstrated by implementing a microprocessor breadboard coder/decoder using the Intel 8086 processor. The Comet Rendezvous Asteroid Flyby mission will incorporate these techniques in a buffer feedback, rate-controlled configuration. The characteristics of this system are discussed.

Rice, Robert F.↗

Effects of uniaxial stress on magnetoacoustic emission and magnetoacoustic responses in steel

Results of magnetoacoustic emission (MAE) and magnetoacoustic (MAC) measurements performed with an unembrittled HY-80 steel specimen are presented. The MAE measurements were obtained by applying an ac magnetic field of 20 Hz parallel to the uniaxial stress axis. The effects of tensile stress were shown to monotonically decrease the peak amplitude of the MAE burst, and they were consistent with the predicted trend based on the tensile stress-induced domain alignment. The effects of compressive stress were found to increase the peak amplitude of the MAE burst initially and to eventually decrease as the magnitude of compressive stress increased.

Namkung, M.↗

Mechanically Strong, Polymer Cross-linked Aerogels (X-Aerogels)

Aerogels comprise a class of low-density, high porous solid objects consisting of dimensionally quasi-stable self-supported three-dimensional assemblies of nanoparticles. Aerogels are pursued because of properties above and beyond those of the individual nanoparticles, including low thermal conductivity, low dielectric constant and high acoustic impedance. Possible applications include thermal and vibration insulation, dielectrics for fast electronics, and hosting of functional guests for a wide variety of optical, chemical and electronic applications. Aerogels, however, are extremely fragile materials, hence they have found only limited application in some very specialized environments, for example as Cerenkov radiation detectors in certain types of nuclear reactors, aboard spacecraft as collectors of hypervelocity particles (refer to NASA's Stardust program) and as thermal insulators on planetary vehicles on Mars (refer to Sojourner Rover in 1997 and Spirit and Opportunity in 2004). Along these lines, the X-Aerogel is a new NASA-developed strong lightweight material that has resolved the fragility problem of traditional (native) aerogels. X-Aerogels are made by applying a conformal polymer coating on the surfaces of the skeletal nanoparticles of native aerogels (see Scanning Electron Micrographs). Since the relative amounts of the polymeric crosslinker and the backbone are comparable, X-Aerogels can be viewed either as aerogels modified by the templated accumulation of polymer on the skeletal nanoparticles, or as nanoporous polymers made by remplated casting of polymer on a nanostructured framework. The most striking feature of X-Aerogels is that for a nominal 3-fold increase in density (still a ultralighweight material), the mechanical strength can be up to 300 times higher than the strength of the underlying native aerogel. Thus, X-Aerogels combine a multiple of the specific compressive strength of steel, with the the thermal conductivity of styrofoam. X-Aerogels have been demonstrated with several polymers such as polyurethanes/polyureas, epoxies and polyolefins, while crosslinking of approximately 35 different oxide aerogels yields a range of dimensionally stable, porous lightweight materials with unique combinations of structural, magnetic and optical properties. The main theme in materials development for space exploration is multifunction. For example, use of one material for thermal insulation/structural component will free weight for useful payload. In that regard, X-aerogels are evaluated at NASA for cryogenic fuel storage tanks and for spacesuits. Along the same lines, major impact fro X-Aerogels is also expected in commercial applications for thermal/acoustic insulation, in catalytic reformers and converters, in filtration membranes and membranes for fuel cells, as platforms for optical, electrical and magnetic sensors, and as lightweight structural component for aircraft and satellites.

Leventis, Nicholas↗

Unveiling the Emergent Traits of Chiral Spin Textures in Magnetic Multilayers

Abstract Magnetic skyrmions are topologically wound nanoscale textures of spins whose ambient stability and electrical manipulation in multilayer films have led to an explosion of research activities. While past efforts focused predominantly on isolated skyrmions, recently ensembles of chiral spin textures, consisting of skyrmions and magnetic stripes, are shown to possess rich interactions with potential for device applications. However, several fundamental aspects of chiral spin texture phenomenology remain to be elucidated, including their domain wall (DW) structure, thermodynamic stability, and morphological transitions. Here the evolution of these textural characteristics are unveiled on a tunable multilayer platform—wherein chiral interactions governing spin texture energetics can be widely varied—using a combination of full‐field electron and soft X‐ray microscopies with numerical simulations. With increasing chiral interactions, the emergence of Néel helicity, followed by a marked reduction in domain compressibility, and finally a transformation in the skyrmion formation mechanism are demonstrated. Together with an analytical model, these experiments establish a comprehensive microscopic framework for investigating and tailoring chiral spin texture character in multilayer films.

36 MATERIALS SCIENCE↗

Diamond precipitation dynamics from hydrocarbons at icy planet interior conditions

The pressure and temperature conditions at which precipitation of diamond occurs from hydrocarbon mixtures is important for modelling the interior dynamics of icy planets. However, there is substantial disagreement from laboratory experiments, with those using dynamic compression techniques finding much more extreme conditions are required than in static compression. Here we report the time-resolved observation of diamond formation from statically compressed polystyrene, (C 8 H 8 ) n , heated using the 4.5 MHz X-ray pulse trains at the European X-ray Free Electron Laser facility. Diamond formation is observed above 2,500 K from 19 GPa to 27 GPa, conditions representative of Uranus’s and Neptune’s shallow interiors, on 30 μs to 40 μs timescales. This is much slower than may be observed during the ~10 ns duration of typical dynamic compression experiments, revealing reaction kinetics to be the reason for the discrepancy. In conclusion, reduced pressure and temperature conditions for diamond formation has implications for icy planetary interiors, where diamond subduction leads to heating and could drive convection in the conductive ice layer that has a role in their magnetic fields.

79 ASTRONOMY AND ASTROPHYSICS↗

Simulating dirty bosons on a quantum computer

Abstract Quantum computers hold the potential to unlock new discoveries in complex quantum systems by enabling the simulation of physical systems that have heretofore been impossible to implement on classical computers due to intractability. A system of particular interest is that of dirty bosons, whose physics highlights the intriguing interplay of disorder and interactions in quantum systems, playing a central role in describing, for instance, ultracold gases in a random potential, doped quantum magnets, and amorphous superconductors. Here, we demonstrate how quantum computers can be used to elucidate the physics of dirty bosons in one and two dimensions. Specifically, we explore the disorder-induced delocalized-to-localized transition using adiabatic state preparation. In one dimension, the quantum circuits can be compressed to small enough depths for execution on currently available quantum computers. In two dimensions, the compression scheme is no longer applicable, thereby requiring the use of large-scale classical state vector simulations to emulate quantum computer performance. In addition, simulating interacting bosons via emulation of a noisy quantum computer allowed us to study the effect of quantum hardware noise on the physical properties of the simulated system. Our results suggest that scaling laws control how noise modifies observables versus its strength, the circuit depth, and the number of qubits. Moreover, we observe that noise impacts the delocalized and localized phases differently. A better understanding of how noise alters the observed properties of the simulated system is essential for leveraging near-term quantum devices for simulation of dirty bosons, and indeed for condensed matter systems in general.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Doping- and Strain-Dependent Electrolyte-Gate-Induced Perovskite to Brownmillerite Transformation in Epitaxial La 1– x Sr x CoO 3–δ Films

Much recent attention has focused on the voltage-driven reversible topotactic transformation between the ferromagnetic metallic perovskite (P) SrCoO 3-δ and oxygen-vacancy-ordered antiferromagnetic insulating brownmillerite (BM) SrCoO 2.5 . This is emerging as a paradigmatic example of the power of electrochemical gating (using, e.g., ionic liquids/gels), the wide modulation of electronic, magnetic, and optical properties generating clear application potential. SrCoO 3 films are challenging with respect to stability, however, and there has been little exploration of alternate compositions. Here, we present the first study of ion-gel-gating-induced P. BM transformations across almost the entire La 1-x SrxCoO 3 phase diagram (0 ≤ x ≤ 0.70), under both tensile and compressive epitaxial strain. Electronic transport, magnetometry, and operando synchrotron X-ray diffraction establish that voltage-induced P → BM transformations are possible at essentially all x, including x ≤ 0.50, where both P and BM phases are highly stable. Under small compressive strain, the transformation threshold voltage decreases from approximately +2.7 V at x = 0 to negligible at x = 0.70. Both larger compressive strain and tensile strain induce further threshold voltage lowering, particularly at low x. The P → BM threshold voltage is thus tunable, via both composition and strain. At x = 0.50, voltage-controlled ferromagnetism, transport, and optical transmittance are then demonstrated, achieving Curie temperature and resistivity modulations of similar to 220 K and at least 5 orders of magnitude, respectively, and enabling estimation of the voltage-dependent Co valence. The results are analyzed in the context of doping- and strain-dependent oxygen vacancy formation energies and diffusion coefficients, establishing that it is thermodynamic factors, not kinetics, that underpin the decrease in the threshold voltage with x, that is, with increasing formal Co valence. These findings substantially advance the practical and mechanistic understanding of this voltage-driven transformation, with fundamental and technological implications.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Coronal Magnetic Field Measurement from EUV Images Made by the Solar Dynamics Observatory

By measuring the geometrical properties of the coronal mass ejection (CME) flux rope and the leading shock observed on 2010 June 13 by the Solar Dynamics Observatory (SDO) mission's Atmospheric Imaging Assembly we determine the Alfven speed and the magnetic field strength in the inner corona at a heliocentric distance of approx. 1.4 Rs The basic measurements are the shock standoff distance (Delta R) ahead of the CME flux rope, the radius of curvature of the flux rope (R(sub c)), and the shock speed. We first derive the Alfvenic Mach number (M) using the relationship, Delta R/R(sub c) = 0.81[(gamma−1) M(exp 2) + 2] / [(gamma +1)(M2 − 1)], where gamma is the only parameter that needed to be assumed. For gamma = 4/3, the Mach number declined from 3.7 to 1.5 indicating shock weakening within the field of view of the imager. The shock formation coincided with the appearance of a type II radio burst at a frequency of approx. 300 MHz (harmonic component), providing an independent confirmation of the shock. The shock compression ratio derived from the radio dynamic spectrum was found to be consistent with that derived from the theory of fast-mode MHD shocks. From the measured shock speed and the derived Mach number, we found the Alfven speed to increase from approx 140 km/s to 460 km/s over the distance range 1.2-1.5 Rs. By deriving the upstream plasma density from the emission frequency of the associated type II radio burst, we determined the coronal magnetic field to be in the range 1.3-1.5 G. The derived magnetic field values are consistent with other estimates in a similar distance range. This work demonstrates that the EUV imagers, in the presence of radio dynamic spectra, can be used as coronal magnetometers

magnetic fields↗