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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 127 records · Page 7

Radiological Safety Analysis Computer (RSAC) Program Version 7.4 Users’ Manual

The Radiological Safety Analysis Computer (RSAC) Program Version 7.4 (RSAC-7) is the newest version of the RSAC legacy code. RSAC-7 calculates the consequences of a release of radionuclides to the atmosphere. Users generates a fission product inventory from either reactor operating history or a nuclear criticality event. RSAC-7 models the effects of high-efficiency particulate air filters or other cleanup systems and calculates the decay and ingrowth during transport through processes, facilities, and the environment. Doses are calculated for inhalation, air immersion, ground surface, ingestion, and cloud gamma pathways. RSAC-7 is used as a tool to evaluate accident conditions in emergency response scenarios, radiological sabotage events, and safety basis accident consequences. This users’ manual contains the mathematical models and operating instructions for RSAC-7. Instructions, screens, and examples are provided to guide the user through the functions provided by RSAC-7. This program is designed for users who are familiar with radiological dose assessment methods.

73 - NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Radiological Dose Consequence Modeling Parameters for Reactor and Nonreactor Nuclear Facilities

To assure consistency between DOE and NRC safety basis requirements this ECAR documents the DOE basis requirements for dose consequence assessments in accordance with Standard DOE-STD-3009-2014. The methodology in this ECAR outlines parameters for evaluating airborne radiological releases and provides a consistent basis for assessing current and future DOE NE facilities.

73 - NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Measurements of the 239 Pu(n,f)/ 235 U(n,f) and 238 U(n,f)/ 235 U(n,f) Cross-Section Ratios Using Quasi-Monoenergetic Neutron Beams

Neutron-induced fission cross-section ratio measurements were carried out at Triangle Universities Nuclear Laboratory (TUNL) over multiple experiment campaigns from 2021-2023. The total beam time for these measurements across all the experimental campaigns was approximately three weeks. This work was intended to serve as an independent validation of the fissionTPC cross-section ratio measurements. In contrast to the white spectrum neutron source and time-projection chamber utilized in the fissionTPC, these measurements utilized pulsed, quasi-monoenergetic neutron beams and fission ionization chambers. Therefore, this work has different sources of systematic error and can be used as a complementary measurement. In this report we describe our fission cross-section ratio measurements, analysis, results and provide a detailed uncertainty budget.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Getting Started with Evaluations with Means and Uncertainties (EMU 3.0)

One of the most fundamental quantities in nuclear physics is the reaction cross section. A cross section represents the probability that a nuclear reaction will resolve through a given channel given a target nucleus and a projectile with a certain energy. A nuclear evaluation is a set of discrete data and interpolation rules to convert those discrete nuclear reaction data—such as the cross section—into a continuous function at arbitrary energies. Evaluated nuclear data files that can appear in Evaluated Nuclear Data File (ENDF) and Generalized Nuclear Data Structure (GNDS) formats, storing a “most-complete” discretized representation of nuclear data, based on both experimental measurements and theory models.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Advanced Test Reactor Neutron Dosimetry Report - Cycle 175C: Results of Neutron Dosimetry Measurements for the Advanced Test Reactor Cycle 175C

Results of neutron dosimetry measurements in ATR for cycle 175C are presented. A single set of cobalt and nickel wires were installed in numerous irradiation locations for the duration of the cycle. The specific activity of these wire segments can be used in conjunction with the presented cycle history information to determine the thermal- and fast-neutron fluence rates for each irradiation position during the cycle using the referenced standard test methods.

73 - NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Building surrogate models of nuclear density functional theory with Gaussian processes and autoencoders

From the lightest Hydrogen isotopes up to the recently synthesized Oganesson (Z = 118), it is estimated that as many as about 8,000 atomic nuclei could exist in nature. Most of these nuclei are too short-lived to be occurring on Earth, but they play an essential role in astrophysical events such as supernova explosions or neutron star mergers that are presumed to be at the origin of most heavy elements in the Universe. Understanding the structure, reactions, and decays of nuclei across the entire chart of nuclides is an enormous challenge because of the experimental difficulties in measuring properties of interest in such fleeting objects and the theoretical and computational issues of simulating strongly-interacting quantum many-body systems. Nuclear density functional theory (DFT) is a fully microscopic theoretical framework which has the potential of providing such a quantitatively accurate description of nuclear properties for every nucleus in the chart of nuclides. Thanks to high-performance computing facilities, it has already been successfully applied to predict nuclear masses, global patterns of radioactive decay like β or γ decay, and several aspects of the nuclear fission process such as, e.g., spontaneous fission half-lives. Yet, predictive simulations of nuclear spectroscopy—the low-lying excited states and transitions between them—or of nuclear fission, or the quantification of theoretical uncertainties and their propagation to basic or applied nuclear science applications, would require several orders of magnitude more calculations than currently possible. However, most of this computational effort would be spent into generating a suitable basis of DFT wavefunctions. Such a task could potentially be considerably accelerated by borrowing tools from the field of machine learning and artificial intelligence. In this paper, we review different approaches to applying supervised and unsupervised learning techniques to nuclear DFT.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Learning from knockout reactions using a dispersive optical model

We present the empirical dispersive optical model (DOM) as applied to direct nuclear reactions. The DOM links both scattering and bound-state experimental data through a dispersion relation, which allows for fully consistent, data-informed predictions for nuclei where such data exist. In particular, we review investigations of the electron-induced proton knockout reaction from both 40 Ca and 48 Ca in a distorted-wave impulse approximation (DWIA) utilizing the DOM for a fully consistent description. Viewing these reactions through the lens of the DOM allows us to connect the documented quenching of spectroscopic factors with the increased high-momentum proton content in neutron-rich nuclei. A similar DOM-DWIA description of the proton-induced knockout from 40 Ca, however, does not currently fit in the consistent story of its electron-induced counterpart. With the main difference in the proton-induced case being the use of an effective proton–proton interaction, we suggest that a more sophisticated in-medium interaction would produce consistent results.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Generation of the TSL for Zirconium Hydrides from Ab Initio Methods

Zirconium hydride (ZrHx) is a moderator material used in TRIGA and other reactors that may exist in multiple phases with varying stoichiometry, which include the δ phase and the ϵ phase. Current ENDF/B-VIII.0 ZrHx thermal scattering law (TSL) evaluations do not distinguish between phases. These sub-libraries were generated with the LEAPR module of NJOY using historic phonon spectra derived from a central force model and assume incoherent elastic scattering for both bound hydrogen and zirconium, which neglects the effects of crystal structures important for scattering from zirconium bound in ZrHx. In this work, the TSLs for hydrogen and zirconium bound in δ-ZrHx and ϵ-ZrH2 were generated from phonon spectra derived from modern ab initio lattice dynamics methods and ab initio molecular dynamics. Subsequently, TSLs for hydrogen and zirconium in ZrHx and ZrH2 were generated using the Full Law Analysis Scattering System Hub (FLASSH) code. The built-in generalized coherent elastic routine was used to generate the previously neglected elastic contribution from zirconium for this material. The present TSLs provide both a re-evaluation of the current ZrH sub-libraries and expansion of the set of TSLs available for the examination of neutrons in systems with zirconium hydride, permitting explicit treatment of δ and ϵ phases.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Detailed study of the eikonal reaction theory for the breakup of one-neutron halo nuclei

Background: One-neutron removal reactions are used to study the single-particle structure of unstable nuclei, and in particular the exotic halo nuclei. The eikonal reaction theory (ERT) has been developed by Yahiro, Ogata, and Minomo [Prog. Theor. Phys. 126, 167 (2011)] to include dynamical effects, which are missing in the usual eikonal description of these reactions. Encouraging results have been obtained for total breakup cross sections in comparison to more elaborate reaction models. Purpose: Here, we extend these comparisons to more differential breakup cross sections expressed as functions of the relative energy or parallel momentum between the core and halo neutron. Method: ERT predictions of these cross sections are compared to state-of-the-art calculations. Results: The hypotheses upon which the ERT is based are confirmed and their range of validity is made clearer. The actual ordering of the evolution operators affects ERT differential cross sections and a specific choice leads to excellent agreement with the reference calculation. Dynamical effects in the treatment of the neutron-target interaction can be significant in the parallel-momentum observable. Conclusions: The role of the different interactions in the dynamics of breakup reactions of one-neutron halo nuclei are better understood and improvements to the ERT are suggested.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Experimental Study of Acceptor Removal in UFSD

The performance of the Ultra-Fast Silicon Detectors (UFSD) after irradiation with neutrons and protons is compromised by the removal of acceptors in the thin layer below the junction responsible for the gain. In this study, the effect is tested both with capacitance–voltage, C–V, measurements of the doping concentration and with measurements of charge collection, CC, using charged particles. We find a perfect linear correlation between the bias voltage to deplete the gain layer determined with C–V and the bias voltage to collect a defined charge, measured with charge collection. An example for the usefulness of this correlation is presented.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Preparation of excited states for nuclear dynamics on a quantum computer

We study two different methods to prepare excited states on a quantum computer, a key initial step to study dynamics within linear response theory. The first method uses unitary evolution for a short time T = O(√1 - F) to approximate the action of an excitation operator Ô with fidelity F and success probability P ≈ 1 – F. The second method probabilistically applies the excitation operator using the Linear Combination of Unitaries (LCU) algorithm. We benchmark these techniques on emulated and real quantum devices, using a toy model for thermal neutron-proton capture. Despite its larger memory footprint, the LCU-based method is efficient even on current generation noisy devices and can be implemented at a lower gate cost than a naive analysis would suggest. Here, these findings show that quantum techniques designed to achieve good asymptotic scaling on fault tolerant quantum devices might also provide practical benefits on devices with limited connectivity and gate fidelity.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Indirect determination of the astrophysical S factor for the Li 6 ( p , γ ) Be 7 reaction using the asymptotic normalization coefficient method

The 6 Li(p,γ) 7 Be cross section influences a variety of astrophysical scenarios, including big-bang and stellar nucleosynthesis. In recent years, conflicting results of direct measurements have been published, reporting contradictory low-energy trends. To shed light on the contradiction between the existing data sets, the reaction was studied using the asymptotic normalization coefficient (ANC) technique which was up-to-now never used for this reaction. To derive the ANC, the 6 Li( 3 He,d) 7 Be transfer reaction, studied at the Department of Physics and Astronomy of the University of Catania and at the John. D. Fox Superconducting Accelerator Laboratory at Florida State University, was re-analyzed, focusing on the proton transfer mechanism [the α transfer process is discussed by Kiss et al. [Phys. Lett. B 807, 135606 (2020)]. Here, the energy of the 3 He beam impinging on a 6 Li target was E lab = 3 MeV and E lab = 5 MeV. The yield of the emitted deuterons was measured with high precision by using silicon ΔE – E telescopes.

6 ≤ A ≤ 19↗

Phase I Final Report

Explore the source record for details and available documents.

36 MATERIALS SCIENCE↗

Gamma Spectroscopy

Gamma Spectroscopy, or the identification of radio-isotopes based on energy, is extraordinarily useful in the Nuclear field. High Purity German (HPGe) gamma detectors along with Sodium Iodine (NaI) gamma detectors are commonly used to identify possible contamination and determine enrichments, among many other applications.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗