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At least 127 records · Page 7

MOSAIC - A space-multiplexing technique for optical processing of large images

A technique for Fourier processing of images larger than the space-bandwidth products of conventional or smart spatial light modulators and two-dimensional detector arrays is described. The technique involves a spatial combination of subimages displayed on individual spatial light modulators to form a phase-coherent image, which is subsequently processed with Fourier optical techniques. Because of the technique's similarity with the mosaic technique used in art, the processor used is termed an optical MOSAIC processor. The phase accuracy requirements of this system were studied by computer simulation. It was found that phase errors of less than lambda/8 did not degrade the performance of the system and that the system was relatively insensitive to amplitude nonuniformities. Several schemes for implementing the subimage combination are described. Initial experimental results demonstrating the validity of the mosaic concept are also presented.

Athale, Ravindra A.↗

Coherent-Precipitation-Stabilized Phase Formation in Over-Stoichiometric Rocksalt-Type Li Superionic Conductors

Rationalizing synthetic pathways is crucial for material design and property optimization, especially for polymorphic and metastable phases. Over-stoichiometric rocksalt (ORX) compounds, characterized by their face-sharing configurations, are a promising group of materials with unique properties; however, their development is significantly hindered by challenges in synthesizability. Here, taking the recently identified Li superionic conductor, over-stoichiometric rocksalt Li–In–Sn–O (o-LISO) material as a prototypical ORX compound, the mechanisms of phase formation are systematically investigated. It is revealed that the spinel-like phase with unconventional stoichiometry forms as coherent precipitate from the high-temperature-stabilized cation-disordered rocksalt phase upon fast cooling. This process prevents direct phase decomposition and kinetically locks the system in a metastable state with the desired face-sharing Li configurations. This insight enables us to enhance the ionic conductivity of o-LISO to be >1 mS cm -1 at room temperature through low-temperature post-annealing. This work offers insights into the synthesis of ORX materials and highlights important opportunities in this new class of materials.

36 MATERIALS SCIENCE↗

Magnetic field dependence of the spin fluctuations in CeCu 5.8 ⁢Ag 0.2

Quantum phase transitions are among the most intriguing phenomena that can occur when the electronic ground state of correlated metals are tuned by external parameters such as pressure, magnetic field, or chemical substitution. Such transitions between distinct states of matter are driven by quantum fluctuations, and can give rise to macroscopically coherent phases that are at the forefront of condensed matter research. However, the nature of the critical fluctuations, and thus the fundamental physics controlling many quantum phase transitions, remain poorly understood in numerous strongly correlated metals. Here we study the model material CeCu 5.8⁢ Ag 0.2 to gain insight into the implications of critical fluctuations originating from different regions in reciprocal space. By employing an external magnetic field along the crystallographic 𝑎 and 𝑐 axis as auxiliary tuning parameter, we observe a pronounced anisotropy in the suppression of the quantum critical fluctuations, reflecting the spin anisotropy of the long-range ordered ground state at larger silver concentration. Coupled with the temperature dependence of the quantum fluctuations, these results suggest that the quantum phase transition in CeCu 5.8⁢ Ag 0.2 is driven by three-dimensional spin-density wave fluctuations.

Boraley, Xavier [Paul Scherrer Inst. (PSI), Villig↗

Precision X-ray Timing of RX J0806.3+1527 with CHANDRA: Evidence for Gravitational Radiation from an Ultracompact Binary

RX J0806.3+1527 is a candidate double degenerate binary with possibly the shortest known orbital period. The source shows an approximately equal to 100% X-ray intensity modulation at the putative orbital frequency of 3.11 mHz (321.5 s). If the system is a detached, ultracompact binary gravitational radiation should drive spin-up with a magnitude of nu(sup dot) approximately 10(exp -16) Hz per second. Efforts to constrain the X-ray frequency evolution to date have met with mixed success, principally due to the sparseness of earlier observations. Here we describe the results of the first phase coherent X-ray monitoring campaign on RX J0806.3+1527 with Chandra. We obtained a total of 70 ksec of exposure in 6 epochs logarithmically spaced over 320 days. With these data we conclusively show that the X-ray frequency is increasing at a rate of 3.77 plus or minus 0.8 x 10(exp -16) Hz per second. Using the ephemeris derived from the new data we are able to phase up all the earlier Chandra and ROSAT data and show they are consistent with a constant nu(sup dot) = 3.63 plus or minus 0.06 x 10(exp -16) Hz per second over the past decade. This value appears consistent with that recently derived by Israel et al. largely from monitoring of the optical modulation, and is in rough agreement with the solutions reported initially by Hakala et al., based on ground-based optical observations. The large and stable nu(sup dot) over a decade is consistent with gravitational radiation losses driving the evolution. An intermediate polar (IP) scenario where the observed X-ray period is the spin period of an accreting white dwarf appears less tenable because the observed nu(sup dot) requires an m(sup dot) approximately equal to 4 x 10 (exp -8) solar mass yr(sup -l), that is much larger than that inferred from the observed X-ray luminosity (although this depends on the uncertain distance and bolometric corrections), and it is difficult to drive such a high m(sup dot) in a binary system with parameters consistent with all the multiwavelength data. If the ultracompact scenario is correct, then the X-ray flux cannot be powered by stable accretion which would drive the components apart, suggesting a new type of energy source (perhaps electromagnetic) may power the X-ray flux.

Strohymayer, Tod E.↗

Precision X-ray Timing of RX J0806.3+1527 with CHANDRA: Evidence for Gravitational Radiation from an Ultracompact Binary

RX J0806.3+1527 is a candidate double degenerate binary with possibly the shortest known orbital period. The source shows an $\approx 100 \%$ X-ray intensity modulation at the putative orbital frequency of 3.11 mHz (321.5 s). If the system is a detached, ultracompact binary gravitational radiation should drive spin-up with a magnitude of $\dot\nu \sim 10(exp -16)$ Hi s$(exp -l}$. Efforts to constrain the X-ray frequency evolution to date have met with mixed success, principally due to the sparseness of earlier observations. Here we describe the results of the first phase coherent X-ray monitoring campaign on RX J0806.3+1527 with {\it Chandra) . We obtained a total of 70 ksec of exposure in 6 epochs logarithmically spaced over 320 days. With these data we conclusively show that the X-ray frequency is increasing at a rate of $3.77 \pm\ 0.8 \times l0(exp -16)$ Hz s$(exp -l)$. Using the ephemeris derived from the new data we are able to phase up all the earlier {\it Chandra) and ROSAT data and show they are consistent with a constant $\dot\nu = 3.63 \pm 0.06 \times 10(exp -16)$ Hz s$(exp -1)s over the past decade. This value appears consistent with that recently derived by Israel et al. largely from monitoring of the optical modulation, and is in rough agreement with the solutions reported initially by Hakala et al., based on ground-based optical observations. The large and stable $\dot\nu$ over a decade is consistent with gravitational radiation losses driving the evolution. An intermediate polar (IP) scenario where the observed X-ray period is the spin period of an accreting white dwarf appears less tenable because the observed $\dot\nu$ requires an $\dot m \approx 2 \times 10(exp -8)$ $M-{\odot)$ yr$(exp -l)$, that is much larger than that inferred from the observed X-ray luminosity (although this depends on the uncertain distance and bolometric corrections), and it is difficult to drive such a high $\dot m$ in a binary system with parameters consistent with all the multiwavelength data. If the ultracompact scenario is

Strohmayer, Tod↗

Coupling of fingertip somatosensory information to head and body sway

Light touch contact of a fingertip with a stationary surface can provide orientation information that enhances control of upright stance. Slight changes in contact force at the fingertip provide sensory cues about the direction of body sway, allowing attenuation of sway. In the present study, we asked to which extent somatosensory cues are part of the postural control system, that is, which sensory signal supports this coupling? We investigated postural control not only when the contact surface was stationary, but also when it was moving rhythmically (from 0.1 to 0.5 Hz). In doing so, we brought somatosensory cues from the hand into conflict with other parts of the postural control system. Our focus was the temporal relationship between body sway and the contact surface. Postural sway was highly coherent with contact surface motion. Head and body sway assumed the frequency of the moving contact surface at all test frequencies. To account for these results, a simple model was formulated by approximating the postural control system as a second-order linear dynamical system. The influence of the touch stimulus was captured as the difference between the velocity of the contact surface and the velocity of body sway, multiplied by a coupling constant. Comparison of empirical results (relative phase, coherence, and gain) with model predictions supports the hypothesis of coupling between body sway and touch cues through the velocity of the somatosensory stimulus at the fingertip. One subject, who perceived movement of the touch surface, demonstrated weaker coupling than other subjects, suggesting that cognitive mechanisms introduce flexibility into the postural control scheme.

NASA Discipline Neuroscience↗

Phase Averaged Measurements of the Coherent Structure of a Mach Number 0.6 Jet

The existence of a large scale structure in a Mach number 0.6, axisymmetric jet of cold air was proven. In order to further characterize the coherent structure, phase averaged measurements of the axial mass velocity, radial velocity, and the product of the two were made. These measurements yield information about the percent of the total fluctuations contained in the coherent structure. These measured values were compared to the total fluctuation levels for each quantity and the result expressed as a percent of the total fluctuation level contained in the organized structure at a given frequency. These measurements were performed for five frequencies (St=0.16, 0.32, 0.474, 0.95, and 1.26). All of the phase averaged measurements required that the jet be artificially excited.

Emami, S.↗

Evidence for a Binary Companion to the Enigmatic Compact Central Object 1E 1207.4-5209

Located in the supernova remnant G296.5+10.0, 1E 1207.4-5209 is a 0.424 s period X-ray pulsar that exhibits strong absorption lines in its energy spectrum. The physical origin of the spectral features in 1E 1207.4-5209 and more generally, the absence of similar features in other radio-quiet neutron stars remains a mystery. Another, possibly related, anomalous property of 1E 1207.4-5209 is its non-monotonic spin frequency evolution. Zavlin, Pavlov & Sanwal(2004) proposed that the irregular spin-down was caused by either (i) frequent, recurrent glitches, (ii) the presence of a fall-back disk or (iii) a binary companion. Here, we report on a sequence of seven XMM-Newton observations of 1E 1207.4-5209 performed during a 40 day window between 2005 June 22 and July 3 1. Due to unanticipated phase noise, we identified three statistically-acceptable phase-coherent timing solutions with frequency time derivatives of +0.9, -2.6, and +1.6 x 10-12 Hz/s (listed in descending order of significance). We concluded that the local frequency derivative during our XMM-Newton observing campaign differs from the long-term spin-down rate by more than an order of magnitude. This measurement strongly supports the binary interpretation for the observed spin irregularities in 1E 1207.4-5209. We identified a family of orbital solutions that are consistent with our phase-connected solution as well as all archival data. We will discuss possible orbital solutions, prospects for constraining binary parameters with future observations, and consequences for the nature of 1E 1207.4-5209.

Woods, P. M.↗

Wide-range tracking oscillator generates phase and frequency coherent output

Tracking oscillator consists of modified phase-lock loop which controls voltage-controlled oscillator capable of automatic lock-on and track of periodic input waveform over frequency ratio 500-1. It is used in telemetry and communications systems where large signal fluctuations are encountered.

Howard, J. R.↗

Coherence between QPOs in X-Ray Pulsars

Rossi X-ray Timing Explorer (RXTE) observations of Cen X-3 and 4U 1626 have shown that when a low frequency (upsilon(sub qpo) approx. 50 mHz) Quazi-Periodic Oscillation (QPO) is presented in the power spectrum of these sources, smaller QPOs also appear in the upper and lower sidebands of the spin frequency upsilon(sub s), and in the sidebands of the spin frequency harmonics. This is expected if the QPO is a modulation in the accretion rate.However, the QPO in the lower sideband of the spin frequency (upsilon = upsilon(sub s) - upsilon(sub qpo)) is stronger than the QPO in the upper sideband (upsilon = upsilon(sub s) + upsilon(sub qpo)), which is not consistent with pure acretion rate modulation. I will present a method for measuring the phase coherent between the main QPO and any of the sideband QPOs, and apply this to RXTE observations. Preliminary results for Cen X-3 show that the QPO in the lower sideband of the spin frequency is highly coherent with the main QPO, while the QPO in the upper sideband is not. Implications for possible QPO mechanisms will be discussed.

Finger, Mark H.↗

Timing of the Accreting Millisecond Pulsar IGR J17591-2342: Evidence of Spin-down during Accretion

We report on the phase-coherent timing analysis of the accreting millisecond X-ray pulsar IGR J17591–2342, using Neutron Star Interior Composition Explorer (NICER) data taken during the outburst of the source between 2018 August 15 and 2018 October 17. We obtain an updated orbital solution of the binary system. We investigate the evolution of the neutron star spin frequency during the outburst, reporting a refined estimate of the spin frequency and the first estimate of the spin frequency derivative ( ˙ν ∼ −7 × 10−14 Hz s−1), confirmed independently from the modelling of the fundamental frequency and its first harmonic. We further investigate the evolution of the X-ray pulse phases adopting a physical model that accounts for the accretion material torque as well as the magnetic threading of the accretion disc in regions where the Keplerian velocity is slower than the magnetosphere velocity. From this analysis we estimate the neutron star magnetic field Beq = 2.8(3) × 108 G. Finally, we investigate the pulse profile dependence on energy finding that the observed behaviour of the pulse fractional amplitude and lags as a function of energy is compatible with the down-scattering of hard X-ray photons in the disc or the neutron star surface.

A Sanna↗

Ligand Control of Ultrafast Hot-Carrier Cooling in CdSe Quantum Dots by a Coherent Nonadiabatic Mechanism

Using the results from global modeling of the broadband two-dimensional electronic spectrum and an analysis of the concurrent damping of excited-state vibronic coherences, we show herein that a coherent nonadiabatic mechanism converts the electronic excitation energy of the X3 (1P 3/2 –1P e ) exciton state to ligand vibrations on the <50 fs time scale in oleate- and hexadecylamine-capped CdSe quantum dots. A comparison of the rates for the two ligands suggests that this process is promoted by mid-frequency vibrations of the ligands due to modulation of their electron-donating tendency. An intramolecular vibrational redistribution process then follows on the ∼200 fs time scale with both ligands, which accompanies thermalization in the band-edge X1 (1S 3/2 –1S e ) state and dephasing of the spectator ligand vibrations. These findings suggest that charge-separated intermediates associated with photoinduced charge transfer or triplet–triplet excitation energy transfer will be produced with retention of phase coherence in the vibrations that modulate the charge-transfer character of surface-bound organic acceptors.

14 SOLAR ENERGY↗

Influence of Disorder on the Electronic Properties and Magnetotransport of Ti 3 C 2 T x Single-Flake Devices

The exploration of MXenes for electronic applications is a rapidly growing field in materials science. However, most research has focused on MXene films, with only a limited number of studies addressing the characterization of single-flake devices. In this work, we investigate the electronic and magnetotransport properties of Ti 3 C 2 T x single-flake devices, exploring the influence of structural defectivity on their transport mechanisms. We show that negative magnetoresistance present at low temperatures in single flake samples arises from weak localization, which we analyze to extract the phase coherence length of single-layer and multi-layer flakes. The study of magnetoresistance for this metallic MXene shows that the material exhibits quantum transport phenomena when intrinsic electronic behavior dominates. Moreover, by increasing the defect density via thermal annealing in ultrahigh vacuum, we uncover and characterize the metal-to-disordered metal transition in Ti 3 C 2 T x , shedding light on new properties and enriching fundamental knowledge about MXenes.

MXenes↗

Slow Electron Spin Relaxation at Ambient Temperatures with Copper Coordinated by a Rigid Macrocyclic Ligand

Paramagnetic transition metal complexes can serve as quantum bits, storing phase information through unpaired electrons. Despite their promise, these systems often require low temperatures and tend to rapidly decohere. Recent efforts have sought to improve longitudinal relaxation (T 1 ), which provides an upper limit for phase coherence (T m ), by investigating existing literature compounds with reduced vibrational coupling and orbital angular momentum. However, synthetic strategies for improving T 1 through novel ligand design have remained scant. Here, we disclose the synthesis of a new modular macrocyclic ligand framework with four nitrogen donors (N 4 ) derived from phenanthroline that supports room-temperature coherent Cu(II) spin centers. The optimized complex more than doubles the T 1 over the next best Cu(II)-N 4 compound and exhibits a room temperature coherence time (T m ) of 0.28 μs, close to previously reported values. This performance enhancement arises from a tight binding site with short Cu–N distances, resulting in a stronger ligand field and reduced thermal accessibility of symmetric vibrational modes. This work demonstrates a practical approach to enabling spin coherence at room temperature, a factor critical to accessing relevant quantum bits and biological sensors, through a designer macrocyclic ligand platform.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Super-resolution stimulated X-ray Raman spectroscopy

Propagation of intense X-ray pulses through dense media has led to the observation of phenomena such as atomic X-ray lasing, self-induced transparency and stimulated X-ray Raman scattering (SXRS)4. SXRS has been long predicted as a means to launch and probe valence-electron wavepackets and as a building block for nonlinear X-ray spectroscopies. However, experimental observations of SXRS to date have not provided spectroscopic information, and theoretical modelling has largely implemented hard-to-realize phase-coherent attosecond pulses. Here we demonstrate SXRS with spectroscopic precision, that is, detection of valence-excited states in neon with a near Fourier-limited joint energy–time resolution of 0.1 eV–40 fs. We used a new covariance analysis between statistically spiky broadband incident X-ray and scattered X-ray Raman pulses. Using 18,000 single shots, we beat not only the incident (about 8 eV) bandwidth but also the approximately 0.2 eV instrumental energy resolution, thus creating super-resolution conditions, in analogy to super-resolved fluorescence microscopy. Our experimental results, supported by ab initio propagation simulations, reveal the competition between lasing in the ion and stimulated Raman scattering in the neutral. We demonstrate enhanced signal collection efficiency and a broad excitation window, surpassing spontaneous Raman efficiencies by orders of magnitude. This stochastic SXRS approach represents a first step towards tracking elementary events that determine chemical outcomes.

nonlinear x-ray spectroscopy↗

Electrostatic gate-controlled quantum interference in a high-mobility two-dimensional electron gas at the (La 0.3 ⁢Sr 0.7 )(Al 0.65 ⁢Ta 0.35 )O 3 /SrTiO 3 interface

Here, we report quantum oscillations in magnetoresistance that are periodic in magnetic field (𝐵), observed at the interface between (La 0.3 ⁢Sr 0.7 )(Al 0.65 ⁢Ta 0.35 )O 3 and SrTiO 3 . Unlike Shubnikov–de Haas oscillations, which appear at magnetic fields > 7 T and diminish quickly as the temperature rises, these 𝐵-periodic oscillations emerge at low fields and persist up to 10 K. Their amplitude decays exponentially with both temperature and field, specifying dephasing of quantum interference. Increasing the carrier density through electrostatic gating results in a systematic reduction in both the amplitude and frequency of the oscillations, with complete suppression beyond a certain gate voltage. We attribute these oscillations to the Altshuler-Aronov-Spivak effect, likely arising from naturally formed closed-loop paths due to the interconnected quasi-one-dimensional conduction channels along SrTiO 3 domain walls. The relatively long phase coherence length (≃ 1.8 µ⁢m at 0.1 K), estimated from the oscillation amplitude, highlights the potential of complex oxide interfaces as a promising platform for exploring quantum interference effects and advancing device concepts in quantum technologies, such as mesoscopic interferometers and quantum sensors.

36 MATERIALS SCIENCE↗

Photodynamic melting of phase-reversed charge stripes and enhanced condensation

The interplay between charge stripes and pairing has long been a subject of scrutiny in a broad class of unconventional superconductors, as in some cases it is unclear whether this interplay benefits the ensuing superfluidity. Experiments that explore the out-of-equilibrium dynamics of these systems aim to tip the balance toward one phase or the other by selectively coupling to relevant modes. Leveraging the fact that competition between stripes and pairing is not exclusive to fermionic systems, we explore the photoirradiation dynamics of interacting hardcore bosons in which density-wave phase-reversal melting leads to enhanced phase-coherent transport response, as quantified by the dynamic amplification of both the zero-momentum occupancy and the condensate fraction, as well as finite out-of-equilibrium charge stiffness and superfluid weight, for a given system size. Finally, our results, obtained using unbiased methods for an interacting system on a ladder geometry, demonstrate how one can engineer time-dependent perturbations to release suppressed orders, potentially providing insight into the underlying mechanism in related experiments.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Weak localization and universal conductance fluctuations in large-area twisted bilayer graphene

We study diffusive magnetotransport in highly 𝑝-doped large-area twisted bilayer graphene in 1∘, 7∘, 9∘, and 20∘ samples. All samples exhibit weak localization, from which we extract the phase coherence length and intervalley scattering lengths, and from that determine that dephasing is caused by electron-electron scattering and intervalley scattering is caused by point defects. We observe signatures of universal conductance fluctuations in the 9∘ sample, which has high mobility and is near the van Hove singularity. Further improvements in sample quality and applications to large-area moiré materials will open new avenues to observe quantum interference effects.

Talkington, Spenser [University of Pennsylvania]↗