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DOE OSTI2021

Oscillations of the thermal conductivity in the spin-liquid state of α-RuCl 3

In the class of materials called spin liquids a magnetically ordered state cannot be attained even at millikelvin temperatures because of conflicting constraints on each spin; for example, from geometric or exchange frustration. The resulting quantum spin-liquid state is currently of intense interest because it exhibits unusual excitations as well as wave-function entanglement. The layered insulator α-RuCl 3 orders as a zigzag antiferromagnet at low temperature in zero magnetic field. The zigzag order is destroyed when a magnetic field is applied parallel to the zigzag axis. At moderate magnetic field strength, there is growing evidence that a quantum spin-liquid state exists. Here we report the observation of oscillations in its thermal conductivity in that field range. The oscillations, whose amplitude is very large within this field range and strongly suppressed on either side, are periodic. This is analogous to quantum oscillations in metals, even though α-RuCl 3 is an excellent insulator with a large gap. As the temperature is raised above 0.5 K, the oscillation amplitude decreases exponentially, anticorrelating with the emergence of an anomalous planar thermal Hall conductivity above approximately 2 K.

36 MATERIALS SCIENCE↗

DOE OSTI2023

Online real-time learning of dynamical systems from noisy streaming data

Abstract Recent advancements in sensing and communication facilitate obtaining high-frequency real-time data from various physical systems like power networks, climate systems, biological networks, etc. However, since the data are recorded by physical sensors, it is natural that the obtained data is corrupted by measurement noise. In this paper, we present a novel algorithm for online real-time learning of dynamical systems from noisy time-series data, which employs the Robust Koopman operator framework to mitigate the effect of measurement noise. The proposed algorithm has three main advantages: (a) it allows for online real-time monitoring of a dynamical system; (b) it obtains a linear representation of the underlying dynamical system, thus enabling the user to use linear systems theory for analysis and control of the system; (c) it is computationally fast and less intensive than the popular extended dynamic mode decomposition (EDMD) algorithm. We illustrate the efficiency of the proposed algorithm by applying it to identify the Van der Pol oscillator, the chaotic attractor of the Henon map, the IEEE 68 bus system, and a ring network of Van der Pol oscillators.

97 MATHEMATICS AND COMPUTING↗

DOE OSTI2021

Electron Activity (Secondary Electron & Field Emission ) Suppression by Magnetic Field Placed on the Surface of Metals And Dielectric [Slides]

Secondary electron emission happens when the surface is exposed to an oscillating electromagnetic field. It has extremely dangerous effect when resonance condition of this oscillating field and higher SEY conditions are met. The dependence of the secondary electron on primary electron energy is shown in the figure. This multiplication effect on the number of electrons in oscillating electromagnetic field is called multipacting. The problem with multipacting exist in many scientific fields like LHC, ISS, ITER involving particle accelerator, space science and fusion research. In high intensity proton rings this multiplies electron get trapped inside the potential created by proton beam called electron cloud. In High power microwave sources, rf couplers and rf window to couple the power also hugely affected by multipacting.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2025

Microcarbonation of Naphthalene: An Experimental and Computational Study of Photoionization in Naphthalene-Carbon Dioxide Clusters

The photoionization of naphthalene (N)-carbon dioxide (CO 2 ) clusters was studied using tunable vacuum ultraviolet (VUV) radiation from a synchrotron in the photon range of 8.0 to 13.7 eV, in combination with time-of-flight mass spectrometry. Clusters of monomer, dimer, and trimer naphthalene with CO 2 (N(CO 2 ) 0–6 , N 2 (CO 2 ) 0–3 , N3) were observed. The lowest-energy conformers were obtained via a conformer search, followed by geometry optimizations at the ωB97X-V2/aug-cc-pVTZ (monomer) and ωB97X-V2/aug-cc-pVDZ (dimer) levels of theory. Carbon dioxide was found to preferentially cluster on top of the naphthalene molecule (in an out-of-plane configuration). From the mass spectra, photoionization intensity curves (PICs) were constructed, and appearance energies (AEs) were determined. No substantial trend in AE was observed with increasing size of the naphthalene-carbon dioxide clusters; rather, AE oscillations around the value for pure naphthalene were observed. These AE oscillations are also observed in a recently studied naphthalene-water cluster system, though in this system a slight downward trend in AE for pure naphthalene clusters (N1/2/3/4) was observed. The differences between the two systems are attributed to differing interaction strengths. In conclusion, understanding these differences may aid in determining how photoprocessing can proceed differently depending on the dominant matrix component in interstellar ices.

Wannenmacher, Anna [Lawrence Berkeley National Lab↗

DOE OSTI2023

Lightning Rings and Gravity Waves: Insights Into the Giant Eruption Plume From Tonga's Hunga Volcano on 15 January 2022

Abstract On 15 January 2022, Hunga Volcano in Tonga produced the most violent eruption in the modern satellite era, sending a water‐rich plume at least 58 km high. Using a combination of satellite‐ and ground‐based sensors, we investigate the astonishing rate of volcanic lightning (>2,600 flashes min −1 ) and what it reveals about the dynamics of the submarine eruption. In map view, lightning locations form radially expanding rings. We show that the initial lightning ring is co‐located with an internal gravity wave traveling >80 m s −1 in the stratospheric umbrella cloud. Buoyant oscillations of the plume's overshooting top generated the gravity waves, which enhanced turbulent particle interactions and triggered high‐current electrical discharges at unusually high altitudes. Our analysis attributes the intense lightning activity to an exceptional mass eruption rate (>5 × 10 9 kg s −1 ), rapidly expanding umbrella cloud, and entrainment of abundant seawater vaporized from magma‐water interaction at the submarine vent.

58 GEOSCIENCES↗

DOE OSTI2024

Electron energy gain due to a laser frequency modulation experienced by electron during betatron motion

Direct laser acceleration of electrons is an important energy deposition mechanism for laser-irradiated plasmas that is particularly effective at relativistic laser intensities in the presence of quasi-static laser-driven plasma electric and magnetic fields. These radial electric and azimuthal magnetic fields provide transverse electron confinement by inducing betatron oscillations of forward-moving electrons undergoing laser acceleration. Electrons are said to experience a betatron resonance when the frequency of betatron oscillations matches the average frequency of the laser field oscillations at the electron position. In this paper, we show that the modulation of the laser frequency as seen by an electron performing betatron oscillations can be another important mechanism for net energy gain that is qualitatively different from the betatron resonance. Specifically, we show that the frequency modulation experienced by the electron can lead to net energy gain in the regime where the laser field performs three oscillations per betatron oscillation. There is no net energy gain in this regime without the modulation because the energy gain is fully compensated by the energy loss. The modulation slows down the laser oscillation near transverse stopping points, increasing the time interval during which the electron gains energy and making it possible to achieve net energy gain.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2022

Observation of light-driven band structure via multiband high-harmonic spectroscopy

Intense light–matter interactions have revolutionized our ability to probe and manipulate quantum systems at sub-femtosecond timescales, opening routes to the all-optical control of electronic currents in solids at petahertz rates. Such control typically requires electric-field amplitudes in the range of almost volts per angstrom, when the voltage drop across a lattice site becomes comparable to the characteristic bandgap energies. In this regime, intense light–matter interaction induces notable modifications to the electronic and optical properties, dramatically modifying the crystal band structure. Yet, identifying and characterizing such modifications remain an outstanding problem. As the oscillating electric field changes within the driving field’s cycle, does the band structure follow and how can it be defined? Here we address this fundamental question, proposing all-optical spectroscopy to probe the laser-induced closing of the bandgap between adjacent conduction bands. Our work reveals the link between nonlinear light–matter interactions in strongly driven crystals and the sub-cycle modifications in their effective band structure.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

DOE OSTI2026

Charged Pion Production Explorations Using the NOvA Near Detector

Measurements of neutrino-nucleus interactions in the few-GeV region provide crucial inputs to the neutrino oscillation program being carried out by currently running experiments (NOvA, SBN, T2K), and next-generation experiments (DUNE, 2HK). This poster presents the status of a measurement using the high-intensity NuMI beam and the NOvA Near Detector of the flux-integrated differential cross-section in pion kinetic energy for $\nu_\mu + N \rightarrow \mu^- + \pi^\pm + X$, where X does not include any charged pions. This signal is sensitive to inelastic processes with Delta resonance production, which dominate at neutrino energies relevant for NOvA and DUNE. To overcome the difficulty of reconstructing the energy of charged pions in a lower-spatial-resolution detector, a novel analysis technique is used that incorporates a multi-template fit to extract the number of events for two signal categories that differ from one another by their purity and resolution. The two signal categories are combined leveraging their complementary errors into a more informative cross section result.

Ewart, Erin [Indiana U.]↗

DOE OSTI2025

The Nature of Standing Plasma Waves Following Fast Breakdown in Thunderstorms

Narrow bipolar events (NBEs) are produced by large-scale systems of streamer corona discharges that occur inside thunderstorms and radiate intensely at very-high frequencies. Here we examine 14 high-power NBEs recorded in Florida which are followed by a lasting oscillatory signal. We isolate the dominant frequencies of the oscillations using empirical mode decomposition methods, and cross-reference this information with the radiator size inferred from broadband interferometry. We conclude that the oscillations are evidence of a standing electromagnetic wave in the plasma cavity created by the preceding streamer system, that is, the cavity's fundamental mode with wavelength equal to twice the radiator length. Contrasting the dispersive and attenuation properties of these waves across several different events allows us to conclude that the cavity is filled with ions resulting in an average conductivity of 0.01–0.1 mS/m, which are left behind after the streamers decay via electron attachment to oxygen molecules.

58 GEOSCIENCES↗

DOE OSTI2025

Enhanced energy gain through higher-order resonances during direct laser acceleration with superluminal phase velocity

Ultra-high intensity laser–plasma interactions can produce ultra-relativistic electrons via direct laser acceleration, assisted by quasi-static plasma magnetic and electric fields. These fields transversely confine electron motion and induce betatron oscillations. The net energy gain is strongly influenced by the interplay between two frequencies: the betatron frequency and the frequency of laser field oscillations experienced by the electron. Prior work has shown that energy gain is enabled by a resonance between the betatron oscillations and the oscillations of the laser field. In particular, higher-order resonances occur when the laser field completes multiple cycles during one betatron oscillation, allowing additional regimes of energy transfer beyond the fundamental (betatron) resonance. In this work, we demonstrate that such resonances become particularly effective when the laser's phase velocity is superluminal. Although the two frequencies generally evolve differently with increasing electron energy—leading to detuning—a superluminal phase velocity introduces a non-monotonic frequency ratio with a global minimum. This minimum allows sustained frequency matching over a broad energy range, thereby enabling enhanced energy gain. As the phase velocity increases, the betatron resonance becomes ineffective due to premature frequency detuning. At the same time, higher-order resonances become increasingly effective, emerging as the dominant mechanisms for enhanced energy gain in this regime of direct laser acceleration.

Laser plasma interactions↗

DOE OSTI2026

Phase-controlled direct laser acceleration enabled by longitudinal variation of the laser-driven quasi-static plasma magnetic field

Direct laser acceleration (DLA) enables energy transfer from an ultra-high-intensity laser to plasma electrons and underpins many laser-driven particle and radiation-source concepts. A laser-driven azimuthal plasma magnetic field is a key player in this process: it confines energetic electrons, induces betatron oscillations, and makes possible a resonant interaction between the betatron motion and the laser field. While this betatron resonance can enhance electron energy gain, the gain itself generally drives frequency detuning and promotes largely reversible energy exchange that limits net acceleration. Here we show, using a test-electron model with prescribed fields, that a slow longitudinal increase of the quasi-static plasma magnetic field qualitatively changes DLA by introducing hysteresis in the ratio of the betatron frequency to the laser frequency experienced by the electron, so that this ratio depends on the prior evolution of the electron even at the same energy. This hysteresis enables phase control of the electron-laser energy exchange and suppresses the usual reversibility of DLA, allowing electrons to retain the acquired energy and sustain energy gain without intermittent losses.

direct laser acceleration↗

DOE OSTI2023

Probing C–I bond fission in the UV photochemistry of 2-iodothiophene with core-to-valence transient absorption spectroscopy

The UV photochemistry of small heteroaromatic molecules serves as a testbed for understanding fundamental photo-induced chemical transformations in moderately complex compounds, including isomerization, ring-opening, and molecular dissociation. Here, a combined experimental-theoretical study of 268 nm UV light-induced dynamics in 2-iodothiophene (C 4 H 3 IS) is performed. The dynamics are experimentally monitored with a femtosecond extreme ultraviolet (XUV) probe that measures iodine N-edge 4d core-to-valence transitions. Experiments are complemented by density functional theory calculations of both the pump-pulse induced valence excitations and the XUV probe-induced core-to-valence transitions. Possible intramolecular relaxation dynamics are investigated by ab initio molecular dynamics simulations. Furthermore, gradual absorption changes up to ~0.5 to 1 ps after excitation are observed for both the parent molecular species and emerging iodine fragments, with the latter appearing with a characteristic rise time of 160 ± 30 fs. Comparison of spectral intensities and energies with the calculations identifies an iodine dissociation pathway initiated by a predominant π → π* excitation. In contrast, initial excitation to a nearby n ⟂ → σ* state appears unlikely based on a significantly smaller oscillator strength and the absence of any corresponding XUV absorption signatures. Excitation to the π → π* state is followed by contraction of the C–I bond, enabling a nonadiabatic transition to a dissociative π→σ C-I * state. For the subsequent fragmentation, a relatively narrow bond-length region along the C–I stretch coordinate between 230 and 280 pm is identified, where the transition between the parent molecule and the thienyl radical + iodine atom products becomes prominent in the XUV spectrum due to rapid localization of two singly occupied molecular orbitals on the two fragments.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2021

The JSNS 2 detector

The JSNS 2 (J-PARC Sterile Neutrino Search at J-PARC Spallation Neutron Source) experiment aims to search for oscillations involving a sterile neutrino in the eV 2 mass-splitting range. The experiment will search for the appearance of electron antineutrinos oscillated from muon antineutrinos. The electron antineutrinos are detected via the inverse beta decay process using a liquid scintillator detector. A 1 MW beam of 3 GeV protons incident on a spallation neutron target produces an intense and pulsed neutrino source from pion, muon, and kaon decay at rest. The JSNS detector is located 24 m away from the neutrino source and began operation from June 2020. The detector contains 17 tonnes of gadolinium (Gd) loaded liquid scintillator (LS) in an acrylic vessel, as a neutrino target. It is surrounded by 31 tonnes of unloaded LS in a stainless steel tank. Optical photons produced in LS are viewed by 120 R7081 Hamamatsu 10-inch Photomultiplier Tubes (PMTs). In this study, we describe the JSNS detector design, construction, and operation.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2026

Efficiency-optimized relativistic plasma harmonics for extreme fields

Bright harmonic radiation from relativistically oscillating laser plasmas offers a direct route for generating extreme electromagnetic fields. Theory predicts that under optimized conditions, the plasma medium can support strong spatiotemporal compression of laser energy in a coherent harmonic focus (CHF), delivering intensity boosts many orders of magnitude greater than the incident driving laser pulse. Although diffraction-limited performance (spatial compression) and attosecond phase locking (temporal compression) have been demonstrated experimentally, efficient coupling of relativistically intense laser pulse energy into the emitted harmonic cone has not been realized so far. Here we demonstrate that this highly nonlinear interaction can be tailored to deliver the maximum conversion efficiencies predicted from simulations. By fine-tuning the temporal profile of the driving laser on sub-picosecond (<10 −12 s) timescales, energies >9 mJ between the 12th and 47th harmonics are observed. These results are in agreement with the theoretically expected efficiency dependence on harmonic order, verifying that optimal conditions have been achieved in the generation process. This is the important final element required to achieve the expected intensity boosts from a CHF in experiments. Although obtaining spatiotemporal compression and optimal efficiency simultaneously remains challenging, the path to realizing extreme optical field strengths approaching the critical field of quantum electrodynamics (the Schwinger limit at >10 16 V cm −1 or >10 29 W cm −2 ) is now open, permitting all-optical studies of the quantum vacuum and new frontiers for intense attosecond science.

High-harmonic generation↗

DOE OSTI2020

Regional MJO Modulation of Northwest Pacific Tropical Cyclones Driven by Multiple Transient Controls

The Madden–Julian Oscillation (MJO) is widely acknowledged for its ability to modulate Northwest Pacific tropical cyclones (TCs), but a complete understanding of the underlying mechanisms remains uncertain. Beyond established effects of the MJO's relative humidity envelope, other dynamical factors have recently been invoked via new genesis potential indices and high-resolution modeling studies. Here we revisit the ability of the MJO to modulate West Pacific TCs through a quasi-explicit cyclone downscaling strategy driven by composited observations, paired later with a genesis index to investigate regional drivers of modulation. In this work, we reveal two distinct spatial modes of TC modulation in which the MJO's dynamic and thermodynamic effects act in tandem to increase TCs. In the South China Sea, for instance, shear reductions associated with the MJO's circulation lead to increasing potential intensity ahead of the arrival of a positive humidity anomaly, all of which combine for an extended period of cyclogenesis favorability.

58 GEOSCIENCES↗

DOE OSTI2021

Detector Instrumentation, Energy Reconstruction and Data Analysis in the DUNE and NOvA Neutrino Experiments

Neutrino oscillations are so far the only experimental observation beyond the standard model since its development four decades ago. The remaining fundamental questions that can be answered by long-baseline neutrino oscillations are (1) the CP violation (whether neutrinos and antineutrinos behave the same way in oscillation), and (2) the mass hierarchy ($m_3>m_{1,2}$ or $m_{1,2}>m_3$), and (3) the octant of $\theta_{23}$ ($\theta_{23}>45^\circ, =45^\circ$ or $<45^\circ$). The PI's group at UCI focuses on long-baseline neutrino experiments DUNE and NOvA, key components of DOE's Intensity Frontier program. NOvA is the current major U.S.-based long-baseline neutrino experiment aiming to solve the mass hierarchy and $\theta_{23}$ octant. It is taking $\nu$ and $\bar{\nu}$ data from the NuMI beam at Fermilab. DUNE is the next-generation flagship neutrino experiment in the U.S. which is designed to decisively determine neutrino CP violation, mass hierarchy and $\theta_{23}$ octant. DUNE is Fermilab's first priority, and has been established as an international collaboration. During the period covered by the report, the PI's group has been exceptionally productive, with leading contributions to DUNE argon-purity monitoring detectors, NOvA/DUNE deep-learning reconstruction, and NOvA oscillation and near detector (ND) analyses. The group also is actively involved in DUNE/NOvA detector operation, data production, calibration, software upgrade and maintenance, and ProtoDUNE cold electronic QA/QC. Specifically, we have made accomplishments in the following four research projects: 1) Purity monitor R\&D and data analysis for DUNE, 2) Deep-learning-based energy reconstruction at NOvA and DUNE, 3) Oscillation analysis at NOvA, and 4) $\nu$-e elastic scattering analysis at NOvA.

47 OTHER INSTRUMENTATION↗

DOE OSTI2025

Investigation of the genesis and intensification of simultaneous cyclones in the Arabian sea and Bay of Bengal in November 2020

The North Indian Ocean (NIO), which includes the Bay of Bengal (BoB) and the Arabian Sea (AS), is frequently impacted by tropical cyclones (TCs). Notably, in November 2020, the simultaneous occurrence of Cyclones Gati in the AS and Nivar in the BoB presented a rare and compelling phenomenon worthy of investigation. This study delves into the underlying mechanisms driving the genesis and intensification of these two Very Severe Cyclonic Storms (VSCS). Key contributing factors include elevated sea surface temperatures (SST) and Tropical Cyclone Heat Potential (TCHP), both crucial for the development and intensification of TCs. Notably, the BoB exhibits higher TCHP values compared to the AS, which facilitated greater intensity for Nivar over Gati. Despite their concurrent formation, the genesis processes of Gati and Nivar were distinct. The early November development of Gati in the AS was modulated by the Rossby wave and the Madden–Julian Oscillation (MJO). Subsequently, the eastward propagation of the MJO triggered the formation of Cyclone Nivar in the BoB, enhancing convective activity from the AS and coinciding with the arrival of a downward-propagating Rossby wave. This study provides a comprehensive analysis of the simultaneous formation of Gati and Nivar, contributing novel insights into the complex interactions between oceanic and atmospheric phenomena. In conclusion, such insights are vital for enhancing the predictive capabilities for destructive weather events in the NIO.

Climate Change↗

DOE OSTI2024

Contribution of El Niño Southern Oscillation (ENSO) Diversity to Low‐Frequency Changes in ENSO Variance

Abstract El Niño Southern Oscillation (ENSO) diversity is characterized based on the longitudinal location of maximum sea surface temperature anomalies (SSTA) and amplitude in the tropical Pacific, as Central Pacific events are typically weaker than Eastern Pacific events. SSTA pattern and intensity undergo low‐frequency modulations, affecting ENSO prediction skill and remote impacts, and resulting in low‐frequency changes in ENSO variance. Yet, how different ENSO types contribute to these decadal variance changes remains unclear. Here, we decompose the low‐frequency changes of ENSO variance into contributions from ENSO diversity categories. We propose a fuzzy clustering of monthly SSTA to allow for non‐binary event category memberships, where each event can belong to different clusters. Our approach identifies two La Niña and three El Niño categories and shows that the major shift of ENSO variance in the mid‐1970s was associated with an increasing likelihood of strong La Niña and extreme El Niño events.

Geology↗