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At least 127 records · Page 7
All sourcesNASA NTRSDOE OSTI
DOE OSTI2023

Design of Instrumentation for Noble Gas Transport in LSTL Needed for Model Development

Development of molten salt reactors (MSRs) requires consideration of several physical phenomena that are different from the light water reactor (LWR) experience. While small-scale tests have been performed to understand the behavior of molten salts, the scale-up to larger experiments is an important step in the development of MSR designs. These small-scale experiments have given information on the thermodynamic state of the heat transport fluid and its constituents, thermophysical properties, convective flow, and corrosion. As detailed models have been developed, using these models to simulate larger scale experiments must incorporate physics that becomes important during scale-up, temperature inhomogeneities, complex flow behavior, and two-phase flow. The purpose of the work package has been to link experimental and modeling efforts in the support of licensing development to design and evaluate technologies to mitigate radionuclide release from MSRs. There were two main activities in this work package—one investigating fission product transport into the cover gas and the other on fission gas transport in the molten salt.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
NASA NTRS1973

Noble gas concentrations and cosmic ray exposure ages of eight recently fallen chondrites

Abundances and isotopic compositions of He, Ne, Ar, and Xe have been measured in eight recently fallen chondrites. Ratios of concentrations of cosmic ray-produced He-3, Ne-21, Ne-22, and Ar-38 indicate that all eight samples experienced less than average cosmic ray shielding. He-3 and Ne-21 exposure ages were calculated using shielding corrected chondritic production rates and the measured Ne-22/Ne-21. Exposure ages calculated from Na-22/Ne-22 and Al-26/Ne-21 ratios and constant relative production rates show a bias between the two ages due to variations in Na-22/Al-26. Arguments are presented that this bias is due to irradiation hardness differences, and therefore the use of constant values for both the Na-22/Ne-22 and Al-26/Ne-21 production ratios is not permitted.

Bogard, D. D.↗
NASA NTRS1976

Production of Mg and Al Auger electrons by noble gas ion bombardment of Mg and Al surfaces

Relative production efficiencies of Mg and Al Auger electrons by He, Ne, Ar, Kr, and Xe ion bombardment are reported as a function of ion energy for energies not exceeding 3 keV. The experimental apparatus employed consisted of a LEED-Auger system equipped with an ion gun and a four-grid retarding-potential analyzer. It is found that: (1) the shape of the ion-excited Auger signal was independent of the rare gas and quite symmetric; (2) the Al signal was about an order of magnitude smaller than the Mg signal for a given bombarding species and ion-gun voltage; (3) no signal was observed for He(+) bombardment under any of the experimental conditions; (4) signal strengths were independent of temperature and ion dose; (5) the Auger production efficiencies differed by no more than a factor of two among the different gases - except for He(+) - on a given metal; (6) all the signal strengths increased with increasing ion-gun voltage, with no maximum exhibited; and (7) the apparent threshold energy for the Al signal was higher than that for the Mg signal. The differences between the results for the two metals are attributed to the fact that the Al 2p orbital lies deeper in energy and closer to the nucleus than the corresponding Mg orbital.

Ferrante, J.↗
NASA NTRS1980

High sensitivity pulse-counting mass spectrometer system for noble gas analysis

A pulse-counting mass spectrometer is described which is comprised of a new ion source of cylindrical geometry, with exceptional optical properties (the Baur source), a dual focal plane externally adjustable collector slits, and a 17-stage Allen-type electron multiplier, all housed in a metal 21 cm radius, 90 deg magnetic sector flight tube. Mass discrimination of the instrument is less than 1 per mil per mass unit; the optical transmission is more than 90%; the source sensitivity (Faraday collection) is 4 ma/torr at 250 micron emission; and the abundance sensitivity is 30,000.

Hohenberg, C. M.↗
NASA NTRS1980

Computational study of alkali-metal-noble gas collisions in the presence of nonresonant lasers - Na + Xe + h/2/pi/omega sub 1 + h/2/pi/omega sub 2 system

The collision of Na with Xe in the presence of both the rhodamine-110 dye laser and the Nd-glass laser is investigated within a quantum-mechanical close-coupled formalism, utilizing ab initio potential curves and transition dipole matrix elements. Both one- and two-photon processes are investigated; the Na + Xe system is not asymptotically resonant with the radiation fields, so that these processes can only occur in the molecular collision region. The one-photon processes are found to have measurable cross sections at relatively low intensities; even the two-photon process has a significant section for field intensities as low as 10 MW/sq cm.

Devries, P. L.↗
NASA NTRS1981

Collisional radiative recombination in high-pressure noble gas mixtures

Rate coefficients are calculated for neutral-assisted collisional radiative recombination in dense, weakly ionized rare-gas mixtures using the quasiequilibrium model developed by Bates. It is shown that the recombination rate can be significantly altered by the presence of a buffer gas. In particular, the presence of helium can enhance the collisional radiative recombination rate coefficient of heavy rare gases by a factor of 5.

Whitten, B. L.↗
NASA NTRS1985

Noble gas component organization in Apollo 14 breccia 14318 I-129 and Pu-244 regolith chronology

Drozd et al. (1972) have first detected the presence of Xe-129 in lunar material. Bernatowicz et al. (1979, 1980) established that this xenon component resides exclusively on grain surfaces and confirmed previous observations that it is less tightly bound than other surface components. The present investigation extends many of the observations made on the basis of a study of the 14301 to 14318, which is the only other lunar regolith breccia for which the isotopic structure of 'parentless xenon' has been accurately resolved. Actually this isotope has two parents, including Pu-244 and I-129, which are both now extinct. Attention is given to the analyzed samples, the employed analytical methods, the petrology and chemistry of the grain size separates, and stepwise heating experiments. On the basis of the obtained results, it is concluded that the I-Pu-Xe system can be used as a chronometer.

Swindle, T. D.↗
NASA NTRS1987

Nucleogenic noble gas components in the Cape York iron meteorite

The paper reports data on neutron capture products of the secondary cosmic ray component, the inferred proton and neutron fluences, and the identification of double beta decay of Se-82 in heavily shielded samples of the Cape York iron meteorite. One purpose of this study is to develop a new chronometer for cosmic ray exposure, based on the nuclides I-129 (16 My half-life) and Xe-129 from low energy cosmic ray reactions on Te. The abundance ratio of these two nuclides permits the determination of an (effective) exposure age of 93 + or - 16 My, which represents the first exposure age datum of Cape York. The very small concentrations of spallogenic Ar-38 = 6.5 x 10 to the -10th cu cm STP/g in the metal and troilite (per g Fe) document the heavily shielded locations of the sample. An excess of Xe-129 in the troilite is shown to be entirely due to the decay of cosmic-ray-produced I-129. On the other hand, an inclusion in the troilite reveals the presence of Xe-129 from extinct I-129 and documents its about 4.5 Gy formation age. Mono-isotopic excess of Kr-82 is identified as due to beta-beta-decay of Se-82 with an inferred half-life of 1.0 x 10 to the 20th y. This represents the first beta-beta-decay product observed in a meteorite.

Murty, S. V. S.↗