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At least 127 records · Page 7

Development of Large-Volume-Diamond Anvil Cell for Neutron Diffraction: The Neutron Diamond Anvil Cell Project at ORNL

10 years ago, Dave Mao, director of EFree (energy frontier research in extreme environments), a DOE energy frontier recognized the importance of neutron science for energy research. The subsequent establishment of a neutron group within EFree lead to the establishment of an “Instrument Development Team” for SNAP, the High-Pressure beamline at the Spallation Neutron Source at Oak Ridge National Laboratory in Tennessee. The idea was to develop novel high pressure techniques to expand the pressure range for neutron diffraction. A goal was set to reach half megabar levels (50 GPa), which at the time was considered as extremely challenging. Here we will give a brief overview of the developments during the last decade in this novel area of research. Fortunately, during this period multi carat diamond anvils have become available mainly by the chemical vapor deposition process (CVD), making research in this pressure range and beyond rather routine. This paper shows the latest developments in large anvil designs, compact multiple ton diamond cells and some examples of high-quality neutron diffraction patterns of sample sizes far below conventional levels.

Boehler, Reinhard↗

Microstructure and water absorption of ancient concrete from Pompeii: An integrated synchrotron microtomography and neutron radiography characterization

There is renewed interest in using advanced techniques to characterize ancient Roman concrete due to its exceptional durability and low-carbon footprint. In the present work, samples were drilled from the “Hospitium” in Pompeii and were analyzed by synchrotron microtomography (μCT) and neutron radiography to study how the microstructure, including the presence of induced cracks, affects their water adsorption. The water distribution and absorptivity were quantified by neutron radiography. The 3D crack propagation, pore size distribution and orientation, tortuosity, and connectivity were analyzed from μCT results using advanced imaging methods. Porosity was also measured by mercury intrusion porosimetry (MIP) as a reference. Ductile fracture patterns were observed once cracks were introduced. Compared to Portland cement mortar/concrete, the Pompeii samples had relatively high porosity, low connectivity, and a similar coefficient of capillary penetration. In addition, permeability was predicted from models based on percolation theory and pore structure data to evaluate the fluid transport properties. Understanding the microstructure of ancient Pompeii concrete is important because it could inspire the development of modern concrete with high durability.

36 MATERIALS SCIENCE↗

Design of Premoderated Pulsed-Neutron Die-Away Experiments for Validating Beryllium Thermal Neutron Scattering Laws

Accurate thermal scattering laws (TSLs) are essential for reliable neutron transport simulations, particularly for systems with low-energy neutrons. Pulsed-neutron die-away (PNDA) experiments provide a highly sensitive platform for TSL validation but face challenges from fast neutron leakage and material constraints in nonhydrogenous targets such as beryllium. This work investigates the use of high-density polyethylene (HDPE) as a premoderator to reduce leakage, improve thermalization, and shorten experimental run times while preserving sensitivity to the Be TSL. Here, three premoderated configurations, encapsulation, slab, and interstitial, were evaluated using MCNP6.3® simulations with ENDF/B-VIII.0 nuclear data. The effects of the Be TSL was quantified by comparing decay constants from simulations with and without 𝑆⁡(𝛼,𝛽) treatments for both beryllium and HDPE. The results show that premoderation enables the use of as little as 5.20% of the beryllium volume required for an unreflected geometry, achieving uncertainties below 0.5% and reducing run time by up to 72.2% in the studied configurations. The interstitial configuration achieved the best balance between low statistical uncertainty and high TSL sensitivity, outperforming the slab and encapsulation designs. These findings demonstrate that carefully optimized premoderation can significantly enhance the efficiency, feasibility, and precision of PNDA experiments for Be TSL validation.

Integral Experiments↗

Pulsed-Neutron Die-Away Response of H 2 O Targets to a D-T Neutron Generator Pulse

Pulsed-neutron die-away (PNDA) experiments were completed at Lawrence Livermore National Laboratory (LLNL). The goal of these experiments was to provide a benchmark to validate thermal neutron scattering laws of H 2 O. The experiment was conducted with a deuterium-tritium (D-T) neutron generator producing pulses of 14.1 MeV neutrons that impinged on a moderating target.

3He Detectors↗

EXPANSE: A time-of-flight EXPanded Angle Neutron Spin Echo spectrometer at the Second Target Station of the Spallation Neutron Source

EXPANSE, an EXPanded Angle Neutron Spin Echo instrument, has been proposed and selected as one of the first suite of instruments to be built at the Second Target Station of the Spallation Neutron Source at the Oak Ridge National Laboratory. This instrument is designed to address scientific problems that involve high-energy resolution (neV– μeV) of dynamic processes in a wide range of materials. The wide-angle detector banks of EXPANSE provide coverage of nearly two orders of magnitude in scattering wavenumbers, and the wide wavelength band affords approximately four orders of magnitude in Fourier times. This instrument will offer unique capabilities that are not available in the currently existing neutron scattering instruments in the United States. Specifically, EXPANSE will enable direct measurements of slow dynamics in the time domain over wide Q-ranges simultaneously and will also enable time-resolved spectroscopic studies. The instrument is expected to contribute to a diverse range of science areas, including soft matter, polymers, biological materials, liquids and glasses, energy materials, unconventional magnets, and quantum materials.

47 OTHER INSTRUMENTATION↗

Quasi-differential neutron induced neutron emissions from 235 U, and 239 Pu

Uncertainty in nuclear reaction cross sections, angular distributions, and other nuclear data directly impact how well simulations of nuclear systems represent physical observations. Here, to determine how well the nuclear data in ENDF/B-VIII.0, JEFF-3.3, and JENDL-4.0 evaluations describe the physical behaviour of 235 U, and 239 Pu when subjected to a neutron flux, the neutron emission spectrum was measured for carbon, 93.0% 235 U, and 93.9% 239 Pu samples, and compared against detailed MCNP6 simulations. The measurements were performed at the Los Alamos Neutron Science Center using a quasi-differential method previously developed at Rensselaer Polytechnic Institute. The measurement spanned 0.82–20 MeV and 30–150 degrees. The measurements show there are a significant number of discrepancies between library predictions of the neutron yield and physical observation. A few of the main discrepancies found are described in this paper. Based on these results a new evaluation utilizing these results for carbon, 235 U, and 239 Pu is recommended.

235U↗

Neutron capture measurements at UMass lowell research reactor

A new facility was designed around the thermal column beam port of the 1 MW Research Reactor at the University of Massachusetts Lowell. Thermal neutrons are collimated to a 1-inch diameter beam and incident on samples to induce the radiative neutron capture. New measurements of capture gamma rays are planned for Mn, Cu, Ni, Cr, and Gd samples in the next few years. The experiments will be carried out in close collaboration with the ENSDF (Evaluated Nuclear Structure Data File) evaluation group at Brookhaven National Laboratory. The gamma rays are measured using an array of high-resolution HPGe detectors. Some of the HPGe detectors use active Compton shields that were designed from scintillation detectors and improve significantly the signal-to-background in the measured gamma-ray spectra with HPGe. The experimental spectra will be validated by the GEANT4 simulations of the array and theoretical models of the emission of gamma rays from the compound nucleus. In conclusion, the new experimental results on the capture gamma ray intensities will be incorporated in future ENSDF evaluations.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Synthesizing pseudo-Kossel lines from neutron transmission data. II. Validation with neutron diffraction data

A new method to recover the orientation matrix of a single crystal with a known unit cell by analyzing synthesized pseudo-Kossel lines from time-of-flight neutron transmission data has been outlined in a companion article [Dessieux et al. (2023). J. Appl. Cryst. 56, https://dx.doi.org/10.1107/S1600576723001346; referred to here as Article I]. In this work, validation of this new technique is presented by employing experimental neutron transmission and diffraction measurements performed on two copper single-crystal specimens. Time-of-flight spectra were recorded during rotation (ω) of the single crystals about a vertical axis perpendicular to the incident neutron beam. The λ–ω maps recorded in transmission are utilized to determine the crystal orientation with respect to the neutron beam, following the procedure presented in Article I. Further, to validate the indexing procedure, the crystal orientations are compared with those obtained via conventional methods using the diffraction data. The resulting pseudo-Kossel lines across the 2D detectors are also observed for the first time.

36 MATERIALS SCIENCE↗

Annihilation signatures of neutron dark decay models in neutron oscillation and proton decay searches

We point out that two models that reconcile the neutron lifetime anomaly via dark decays of the neutron, also predict dark matter-neutron ($\bar{χ} - n$) annihilation that may be observable in neutron-antineutron oscillation and proton decay searches at Super-Kamiokande, Hyper-Kamiokande and DUNE. We study signatures of $\bar{χ}n$ →γπ0 (or multi-π0) and $\bar{χ}n$ →φγπ0 (or φ+multi-π0), where φ is an almost massless boson in one of the two models.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

High-resolution neutron spectroscopy using backscattering and neutron spin-echo spectrometers in soft and hard condensed matter

The instruments best suited to performing high-energy-resolution neutron spectroscopy are spin-echo spectrometers and backscattering spectrometers. The development of these experimental techniques dates back almost half a century, and most major neutron scattering facilities operate mature spectrometers of one or both classes. Recent advances in instrumentation and neutron sources are enhancing their performance and expanding their capabilities, with the objective of enabling researchers to tackle new and more complex problems. Finally, in this Technical Review, we assess the current state of the art in high-energy-resolution neutron spectrometers, showcasing their role in the study of nanoscale dynamics in soft and biological materials, as well as disordered magnets.

47 OTHER INSTRUMENTATION↗

The neutron electric dipole moment experiment at the Spallation Neutron Source

Novel experimental techniques are required to make the next big leap in neutron electric dipole moment experimental sensitivity, both in terms of statistics and systematic error control. The nEDM experiment at the Spallation Neutron Source (nEDM@SNS) will implement the scheme of Golub & Lamoreaux [Phys. Rep., 237, 1 (1994)]. The unique properties of combining polarized ultracold neutrons, polarized 3 He, and superfluid 4He will be exploited to provide a sensitivity to ~ 10-28 e · cm. Our cryogenic apparatus will deploy two small (3 L) measurement cells with a high density of ultracold neutrons produced and spin analyzed in situ. The electric field strength, precession time, magnetic shielding, and detected UCN number will all be enhanced compared to previous room temperature Ramsey measurements. Our 3 He co-magnetometer offers unique control of systematic effects, in particular the Bloch-Siegert induced false EDM. Furthermore, there will be two distinct measurement modes: free precession and dressed spin. This will provide an important self-check of our results. Following five years of “critical component demonstration,” our collaboration transitioned to a “large scale integration” phase in 2018. An overview of our measurement techniques, experimental design, and brief updates are described in these proceedings.

Leung, Kent↗

Validation of neutron emission and neutron energy spectrum calculations on a Mega Ampere Spherical Tokamak with directional relativistic spectrum simulator

The recently developed directional relativistic spectrum simulator (DRESS) code has been validated for the first time against numerical calculations and experimental measurements performed on the Mega Ampere Spherical Tokamak . In this validation, the neutron emissivities and rates computed by DRESS are benchmarked against TRANSP/NUBEAM predictions while the neutron energy spectra provided by DRESS taking as input TRANSP/NUBEAM and ASCOT/BBNBI in Gyro-Orbit mode fast ion distributions are validated against proton pulse height spectra measured by the neutron flux monitor. Finally, excellent agreement was found between DRESS and TRANSP/NUBEAM predictions of local and total neutron emission.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Influence of 73 Rb on the ashes of accreting neutron stars

We find that the proton separation energy, S(p), of 73 Rb is –640(40) keV, deduced from the observation of β-delayed ground-state protons following the decay of 73 Sr. This lower-limit determination of the proton separation energy of 73 Rb coupled with previous upper limits from nonobservation, provides a full constraint on the mass excess with ΔM ( 73 Rb) = –46.01 ± 0.04 MeV. With this new mass excess and the excitation energy of the J π = 5/2 – isobaric-analog state (T = 3/2) in 73 Rb, an improved constraint can be put on the mass excess of 73Sr using the isobaric-multiplet mass equation (IMME), and we find ΔM( 73 Sr) = –31.98 ± 0.37 MeV. Furthermore, these new data were then used to study the composition of ashes on accreting neutron stars following Type I x-ray bursts. Counterintuitively, we find that there should be an enhanced fraction of A > 102 nuclei with more negative proton separation energies at the 72 Kr rp-process waiting point. Larger impurities of heavier nuclei in the ashes of accreting neutron stars will impact the cooling models for such astrophysical scenarios.

79 ASTRONOMY AND ASTROPHYSICS↗

Measurement of γ -ray production via the neutron- O 16 reaction using a 77 MeV quasimonoenergetic neutron beam

Understanding of γ-ray production via neutron interactions on oxygen is essential for the study of neutrino neutral-current quasielastic interactions in water Cherenkov detectors. A measurement of γ-ray production from such reactions was performed using a 77 MeV quasi-monoenergetic neutron beam. Several γ-ray peaks, which are expected to come from neutron- 16 O reactions, are observed and production cross sections are measured for nine γ-ray components of energies between 2 and 8~MeV. Finally, these are the first measurements at this neutron energy using a nearly monoenergetic beam.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

First Measurement of Deeply Virtual Compton Scattering on the Neutron with Detection of the Active Neutron

Measuring deeply virtual Compton scattering (DVCS) on the neutron is one of the necessary steps to understand the structure of the nucleon in terms of generalized parton distributions (GPDs). Neutron targets play a complementary role to transversely polarized proton targets in the determination of the GPD E . This poorly known and poorly constrained GPD is essential to obtain the contribution of the quarks’ angular momentum to the spin of the nucleon. DVCS on the neutron was measured for the first time selecting the exclusive final state by detecting the neutron, using the Jefferson Lab longitudinally polarized electron beam, with energies up to 10.6 GeV, and the CLAS12 detector. The extracted beam-spin asymmetries, combined with DVCS observables measured on the proton, allow a clean quark-flavor separation of the imaginary parts of the Compton form factors H and E . Published by the American Physical Society 2024

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Performance Evaluation of the Starfire nGen-350 DD Neutron Generator for use with the Fast Neutron Coincidence Collar

The Starfire Industries nGen-350 DD neutron generator has been developed for use with the Fast Neutron Coincidence Collar (FNCL). The generator was adapted from the nGen-310 model generator by Starfire to accommodate an International Atomic Energy Agency (IAEA) request to incorporate a neutron yield stabilization mechanism. An nGen-350 generator was obtained by Oak Ridge National Laboratory (ORNL) for evaluation as a potential neutron interrogation source replacement for Am(Li) in the FNCL. This report provides a summary of the performance of the nGen-350.

43 PARTICLE ACCELERATORS↗

Survey of Neutron Flux Sensors for Monitoring Advanced Reactor Concepts Operating with Low Neutron Fluence Rate and Extended Uninterrupted Lifespans

The purpose of this report is to provide a survey of neutron sensors applicable to the low power levels (low neutron fluence rate) for reactor monitoring and controls. A survey of detectors for reactor power monitoring and controls from various commercial vendors—Reuter Stokes, Framatome, Exosens, and Mirion—is presented in the following sections based on application of reactor power ranges. Detector specifications are provided where available per each of the vendor’s catalogues and specification sheets found on their websites. While this is not an all encompassing list, it provides an example of detector options. Fission chambers and self powered neutron detectors (SPNDs) for in-core application with changes to the neutron-sensitive materials—fissile depots for fission chambers and emitters for SPNDs—for regenerative capabilities will be discussed in the latter sections.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗