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At least 127 records · Page 7

Results of Neutron Dosimetry Measurements for the Advanced Test Reactor Cycle 173-C

Results of neutron dosimetry measurements in ATR for cycle 173-C are presented. Cobalt and nickel wires were installed in numerous irradiation locations for the duration of the cycle. The specific activity of these wire segments can be used in conjunction with the presented cycle history information to determine the thermal- and fast-neutron fluence rates for each irradiation position during the cycle using the referenced standard test methods.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Advanced Test Reactor Neutron Dosimetry Report – 174 A & B

Results of neutron dosimetry measurements in ATR for cycle 174 A B are presented. Cobalt and nickel wires were installed in numerous irradiation locations for the duration of the cycle. The specific activity of these wire segments can be used in conjunction with the presented cycle history information to determine the thermal- and fast-neutron fluence rates for each irradiation position during the cycle using the referenced standard test methods.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

HYDRODYNAMIC TESTING OF ZIRCALOY TO STEEL HUB COUPLINGS FOR USE IN ADVANCED TEST REACTOR I-LOOP TUBE

The ATR I-positions' isolation from the flux trap region provides an opportunity for a test facility that could create conditions representative of commercial light water reactors. Such a facility requires piping couplings and joints that withstand extreme thermal and pressure cycling. Also, transitioning from steel to zircaloy piping inside the reactor vessel allows the neutronic properties of zircaloy to be leveraged while using cost-effective stainless steel outside of the core. Grayloc-style hub couplings will act as transition points between stainless steel piping and zircaloy piping inside the reactor vessel. These couplings have not been sufficiently tested for leakage where there is a transition between materials. This transition is a concern because the thermal expansion coefficients of the materials differ. Seal integrity between the two components may be greatly affected by thermal expansion at the connection. Thus, the effect of thermal cycling must be assessed. Thermal and pressure cycling and hydrodynamic testing will be conducted to verify seal integrity of the steel to zircaloy hub coupling when subjected to ATR conditions.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

A Fast Reactor Irradiation Experiment Design in the ATR

Modern modeling techniques were used to investigate a proposed method for fast neutron irradiations in an existing thermal-spectrum reactor, the Advanced Test Reactor (ATR). This method builds upon pre-existing ideas, where fast flux is increased by surrounding the specimens with fissionable “booster fuel” but diverges from historical approaches by using an already developed fuel element design used in the Belgian Reactor 2 (BR2) as the booster fuel while leveraging modern 3-D modeling and simulation techniques. Design evaluations and neutronics simulations were performed to evaluate the performance of a BR2 fuel element irradiated in an ATR flux trap with test pins in the central channel of the BR2 fuel element. These efforts have yielded promising results. Adding a BR2 fuel element in the northeast (NE) flux trap of ATR was predicted to result in a 150% increase to the incident fast neutron flux with a fast (>0.1 MeV) to thermal (<0.625 eV) neutron flux ratio ranging from approximately 50 to 150, dependent on the material used for thermal neutron filtering and volume of moderator within the central channel of the BR2 element. The predicted annual fast neutron fluence (>0.1 MeV) ranges from 7.9 × 1021 to 9.1 × 1021 n/cm2. Given the relatively large fast to thermal neutron flux ratio, the calculated radial power profiles within 4.3 mm outer diameter U10Zr fueled specimens irradiated within the BR2 booster fuel element are adequate representations of those within fast neutron reactors. The predicted radial power profiles are not flat, but they are more prototypic than those seen in advanced fuels tests which began in ATR in 2003. Another distinct advantage of this experiment design is that full-scale test pins can be irradiated to augment the ongoing series of reduced scale advanced fuels tests. The proposed experiment design irradiated within a BR2 fuel element in a flux trap of ATR offers an improved alternative to the current testing of advanced reactor fuels in ATR. Selected results from this design evaluation are presented.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Irradiation performance of nonfertile (Pu-MA-Zr) fast reactor metal fuels

This work was part of a program begun in 2001 to develop advanced nuclear fuels, originally as carriers for plutonium and minor actinides (neptunium, curium, and americium) taken from spent commercial light-water reactors (LWR) so that the plutonium and minor actinides could be ‘burned’ or transmuted in an accelerator or a fast nuclear reactor. A central part of these experiment programs has been the development of advanced fast reactor fuels, because a fast reactor was considered the most efficient vehicle to transmute the actinide waste products, and metallic fuels is a central focus of these tests. An experiment design was developed in which a thermal test reactor, the Advanced Test Reactor (ATR), was used to test small fuel pin prototypes, by creating areas in the core shielded by cadmium filters to produce a largely epithermal and fast neutron spectrum environment in which the pins could be irradiated. The results of non-fertile metallic fuel (no uranium) tests are presented here. Pu-Am-Np-Zr fuels were irradiated to fission densities up to 33 × 10 20 fission/cm 3 and Pu-239 depletions of up to 39%. The depletions were created by roughly 2/3 by fission and 1/3 by transmutation neutron capture. Up to five fuel ‘rodlets’ were irradiated in three sealed capsules stacked axially in the core, and the peak cladding temperatures ranged from 300°C to 500°C, depending on axial location as those near the core centerline are operating hotter and to higher fission densities. Several post-irradiation examinations (precision gamma scanning and fission gas release) were similar to other historical metal fuel experiments in fast reactors. However, optical metallography indicated that two of the rodlets had breached. The exact reasons are unclear. Due to the design of this irradiation experiment a rodlet breach could have increased the temperature in others in the same capsule by contaminating the thermal gap helium with heavier and less conductive fission product gases. Finally, some of those rodlets showed high amounts of fuel/cladding chemical interaction (FCCI).

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Accident Progression and Source Term Demonstration Calculations for the Advanced Burner Test Reactor (ABTR)

As advanced reactor designers approach broad deployment of new reactor technologies and the associated applications, a critical milestone on this path includes licensing or authorization of these designs in the current regulatory environment. Commercial licensing and DOE authorization both consist of numerous aspects to not only certify the designed plant will operate as intended, but also related to confirmation of the safe operation of these facilities that comply with specific standards and requirements. To that end, domestic industry and regulators require toolsets and methods which can be used to confirm that advanced reactor designs not only align with expected performance during normal operation, but also a series of transient scenarios. These codes require a satisfactory validation basis, and in the absence of such a basis, code-to-code comparisons are often utilized as a surrogate to confirm model adequacy. To support this need for fast reactor technologies, a series of analyses using SAS4A/SASSYS- 1 and the Simplified Radionuclide Transport (SRT) code have been conducted for the Advanced Burner Test Reactor (ABTR). These analyses are expected to not only provide a baseline for transient and source term analyses of ABTR, but to also provide context for the key physics that determine evolution of specific transient scenarios in a sodium-cooled fast reactor (SFR). These codes are utilized for this work given their adoption in the SFR industry and by key SFR stakeholders.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Candidacy Renewal Report for ICERR Designation

The International Atomic Energy Agency (IAEA) has established a designation for an International Centre based on Research Reactors (ICERR). The intention of this designation is to provide a vehicle for IAEA member states to access international research-reactor and ancillary nuclear research and development infrastructure. The U.S. Department of Energy (DOE) has made a commitment to world leadership in the development of advanced nuclear energy, science, and technology. To this end, DOE has established programs and initiatives to enhance this leadership role. ICERR designation constitutes an important step in achieving the DOE vision. DOE, represented by Idaho National Laboratory (INL) and Oak Ridge National Laboratory (ORNL), is submitting this application for re-designation as an IAEA ICERR. Both INL and ORNL have a decades-long and storied history that supports nuclear research, development, and deployment both nationally and internationally. Both have a history of safe and efficient nuclear operations and have demonstrated a track record of international collaboration and cooperation. INL and ORNL are home to two primary and two secondary research reactors. The primary reactors are Advanced Test Reactor at INL, and High-Flux Isotope Reactor at ORNL. Secondary reactors include: Neutron Radiography Reactor at INL, Transient Reactor Test (TREAT) Facility at INL, and INL Advanced Test Reactor: Critical Facility (ATRC). ICERR designation will also include numerous ancillary facilities at both laboratories, including the following: Multiple post-irradiation examination facilities at both INL and ORNL, Radiochemistry hot-cell facilities at ORNL, INL nuclear-fuel-fabrication and materials-science facilities, and INL and ORNL radiological and nuclear analytical capabilities.

99 GENERAL AND MISCELLANEOUS↗

Accelerated Fuel Qualification of Fast Modular Reactor Fuel in a Thermal Reactor: Modeling and Simulation Paired with Irradiation Testing

The accelerated fuel qualification (AFQ) methodology is applied by simulating accelerated fuel tests of the General Atomics Electromagnetic Systems’ fuel system for its 44-MW(electric) gas-cooled, fast-spectrum fast modular reactor (FMR). This fuel is comprised of UO 2 pellets in SiGA® cladding, a silicon carbide ceramic matrix composite. Fast reactors, like the FMR, offer many benefits, including high fuel utilization and flexibility, but may require a lengthy material design process if tests are performed using fast neutron irradiation alone. A thermal neutron irradiation can instead be used to rapidly test how well key components of the current material models extend to high burnup. Thermal neutrons produce a different radial power distribution within the pin than fast neutrons. However, the temperature and burnup values for the two neutron types are comparable, and the differences between the simulated fuel responses are relatively small, demonstrating the weak sensitivity of the physics-based fuel model calculations on the neutron type and the irradiation rate. Furthermore, the deformation of the SiGA cladding saturates after about 1 displacement per atom for both neutron spectra. In an accelerated fuel test, the irradiation time required to reach the target fuel burnup can be reduced by a factor of 3 by using a small rodlet with a 45% smaller pellet diameter while maintaining the same linear power. Therefore, the time for data collection up to high burnup can be significantly reduced while maintaining the same temperature profile, which largely determines the material response. Tests of fuel rodlets of standard and compact size will be carried out in the Idaho National Laboratory’s Advanced Test Reactor (ATR), including full size and compact rodlets with varying gap sizes. By applying physics-based mechanistic modeling and simulation in accordance with the AFQ methodology, this type of compact rodlet testing in a thermal test reactor captures the necessary phenomena to test fuel material models up to high burnup and to simulate the expected impact of fast neutron radiation on the fuel in FMR operations. Finally, this approach to testing fast reactor fuels in existing thermal test reactors, paired with advanced physics-based mechanistic modeling and simulation, is expected to be applicable to a range of advanced fuels and will decrease the overall fuel qualification timeframe from decades to years.

Advanced test reactor (ATR)↗

Operational Experience and Development of a Reliability Model for the ATR Demineralizer System (Slides)

The Advanced Test Reactor (ATR) is a light water reactor with aluminum clad driver fuel. Strict limits are implemented on pH, conductivity, and filterable solids to assure the performance of the driver fuel limit corrosion of the primary coolant system (PCS) pressure boundary components. A bypass demineralizer system is used to maintain PCS coolant within allowable bands for each of the aforementioned variables. Unlike many other reactors, the ATR does not have a filtration system. As such, failure of ion exchange resin in the bypass demineralizer can defeat the purpose of the system and result in high filterable solids in the PCS. Power operations with high filterable solids is prohibited by a technical safety requirement. This paper discusses recent failures of the ATR bypass demineralizer system. The testing and analysis done to deduce the cause of the failures is covered, as well as short term mitigative steps that were taken. To prevent the likelihood of future issues, historical data from the ATR and industry is used to develop a reliability model of the ATR bypass demineralizer system. Evidence of radiolytic decomposition of ion exchange resin was found in the cause investigation. As such, special attention is given to ion exchange resin failure due to high radiation environments. The reliability model is used to develop the ATR testing and maintenance program. Specifically, limits on resin service life are discussed.

21 - SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLAN↗

Machine learning predictions of irradiation embrittlement in reactor pressure vessel steels

Abstract Irradiation increases the yield stress and embrittles light water reactor (LWR) pressure vessel steels. In this study, we demonstrate some of the potential benefits and risks of using machine learning models to predict irradiation hardening extrapolated to low flux, high fluence, extended life conditions. The machine learning training data included the Irradiation Variable for lower flux irradiations up to an intermediate fluence, plus the Belgian Reactor 2 and Advanced Test Reactor 1 for very high flux irradiations, up to very high fluence. Notably, the machine learning model predictions for the high fluence, intermediate flux Advanced Test Reactor 2 irradiations are superior to extrapolations of existing hardening models. The successful extrapolations showed that machine learning models are capable of capturing key intermediate flux effects at high fluence. Similar approaches, applied to expanded databases, could be used to predict hardening in LWRs under life-extension conditions.

36 MATERIALS SCIENCE↗

Analysis of Radiological Release From Fueled Irradiation Experiments During Manual Handling (Slides)

Irradiation experiments are manually handled at the Advanced Test Reactor (ATR) by qualified operators using long handled tools. Standard handling evolutions include insertion and removal from the reactor vessel, transfer to/from a storage location or cask in the ATR canal, and handling/reconfigurations at a canal working tray. Such routine handling has the potential to result in mechanical damage to the experiment boundary which is credited to retain fission products. Since damage can occur due to operator error, this is an anticipated occurrence. This work determines the radiological consequences to receptors inside the ATR facility, as well as public receptors. Given the wide variety of fuel types tested at the ATR, a generic approach to the analysis is taken. The radiological inventory is determined to bound a variety of fuel types (e.g., ceramic and molten fuel matrices) and fission powers on the U-235 enrichment spectrum. The source term analysis considers different release fractions to bound different fuel types and burnups. The postulated handling events occur underwater; thus, retention of the released isotopic content is considered within the canal water column. Retention of radionuclides in the water column is determined using a modified approach of United States (US) Nuclear Regulatory Commission (NRC) Regulatory Guide (RG) 1.183. Radiological dose to the facility receptor is determined using a compartment release model. Dose to the public receptor is determined using atmospheric dispersion models using site specific atmospheric conditions with the use of the Radiological Safety Analysis Computer (RSAC) program version 7.2.

21 - SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLAN↗

Neutronics analysis of Full Size Plate–1 Experiment using MC21

Qualification and testing of Low Enriched Uranium fuel is desired so that it can be used in research reactors instead of High Enriched Uranium. The Full Size Plate - 1 (FSP-1) experiment involves irradiating a low enriched metallic fuel in the Advanced Test Reactor to assist in this general qualification. Prior to irradiation, an in-depth neutronics analysis is needed to ensure the safety requirements of the Advanced Test Reactor are met. To accomplish this, the MC21 software was used to analyze the FSP-1 experiment, which will allow a test run to be performed with this new fuel in the Advanced Test Reactor Critical facility. By verifying and validating the results of the MC21 software with comparisons to other codes and the preliminary irradiation in the Advanced Test Reactor Critical facility, the FSP-1 experiment will be ready to irradiate using the Advanced Test Reactor. This work is concerned with the neutronics analysis of the FSP-1 experiment using the MC21 software.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Comparison of fluence-rate determination techniques for the Advanced Test Reactor-Critical Facility

A technique using small, enriched uranium-aluminum alloy monitors to measure fission rates in fuel plate assembly reactors was developed at the Idaho National Laboratory Radiation Measurements Laboratory in support of Advanced Test Reactor Critical (ATR-C) Facility irradiations. Previous measurements were performed to determine the correlation between the beta-particle activity and the fission rate in the U-Al monitors following irradiation. The American Society for Testing and Materials (ASTM) has established a standard practice E704 for determining neutron fluence rate by radioactivation of depleted uranium by measuring the concentration of fission-products in irradiated uranium monitors. Rather than measuring the beta-particle decay from fission-products, the decay rate of fission-products is determined by gamma-ray spectroscopy. The feasibility of using a method adapted from the ASTM standard practice E704 was investigated for ATR-C irradiations and compared to the present method by analyzing a subset of 21 monitor wires using both methods. The resulting calculated fission rates agreed with an average standard deviation of 7.45%, within the average combined measurement error of 9.05%. Practical considerations such as expected fluence-rates, sample activity, and counting-time were compared between the two methods and the sources of error for each method were investigated. Quality assurance measurements utilizing the modified ASTM standard method are recommended for future test irradiation, but gross-beta-particle counting remains the most practical solution for ATR-C fluence-rate determination.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗