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At least 127 records · Page 7

Accelerometer Drift Study

Accelerometers are energy transducers that convert mechanical energy into an electrical signal. That electrical signal is proportional to the amount of mechanical stress the accelerometer was subjected to. Knowing this proportionality allows the electrical signal to be interpreted as an acceleration. There are three types of sensing technologies utilized in capacitors: piezoelectric, piezoresistive and capacitive. In this study, all of the accelerometers utilized are of the piezoelectric type and purchased from one particular vendor, MEGGITT. The piezoelectric effect is the phenomena by which a material generates an electrical charge when subjected to a mechanical stress. A piezoelectric accelerometer will not generate an electrical charge when placed in a static acceleration field because no stress will be placed on the piezoelectric element. However if the acceleration field is dynamic, the piezoelectric element will generate an electrical charge. So the types of accelerations these accelerometers are measuring are dynamic in nature, such as vibrations. Knowledge of dynamic acceleration is useful in characterizing the structural response of some object. The sensitivity of an accelerometer is the ratio of its electrical output to mechanical input. The more sensitive an accelerometer is, the greater the value of the electrical output to a given mechanical input. An accelerometer’s sensitivity is known to drift over time. The objective of this study is to quantify this drift. Questions to answer are: Does the accelerometer become more or less sensitive over time and by how much. This is important to understand because this will establish a time frame of when readings from the accelerometer can be utilized. The larger this time frame is the better because that would preclude the need to purchase accelerometers frequently, which saves on costs. This would further bolster the relationship between MEGGITT and LANL if it is found that MEGGITT produces accelerometers that can be used for a relatively long period of time. This would create less uncertainty in picking a vendor for accelerometers.

42 ENGINEERING↗

The Dark Energy Spectrographic Instrument (DESI) Corrector Assembly

The specific research of the DESI project is to study in detail the expansion history of the Universe over the past 10 billion years. In order to do this, the project designed, fabricated, tested and commissioned the DESI instrument which has been deployed at the Mayall Telescope at the Kitt Peak National Observatory near Tucson, Arizona. The DESI project was conducted by approximately 30 US and foreign national laboratories. Our CRADA with University College London (UCL) involved both research planning for eventual observing on the DESI telescope; and in the build of the optical corrector, a major part of the instrument. The key major goals of this CRADA were achieved. For survey planning, Drs. Lahav, Abdalla, Peiris, Pontzen and Dr. Farihi were all important contributors to the working groups to which they were assigned. Their modelling efforts, cosmological simulations, target selection and analyses of imaging surveys have been vital in the early planning for targets during commissioning. The major role UCL played in the development of the instrument was performed by Drs. Doel and Brooks. The optical corrector components were developed by scientists and engineers at Lawrence Berkeley National Laboratory and at Fermi National Accelerator Laboratory. UCL was assigned the arduous responsibility for creating the instrumentation necessary to take all the separate components (lenses, cells, rings) and incorporate them, while precisely aligning the optics. Following that, they installed the corrector inside the barrel and shipped everything to the Mayall. It was a great success that the optical barrel arrived safely in good condition. Drs. Doel and Brooks were involved in every step of the fabrication and kept in constant contact with the LBNL DESI Project Manager and Project Director. They were extremely successful in their alignment, which was proved by early observations. First light on the telescope was achieved on October 22, 2020. The first spectrum was taken of a random star at zenith. Shortly thereafter, the telescope slewed to M33 and several spectra were taken there and later in the Persus nebula. It was a major accomplishment for the project.

79 ASTRONOMY AND ASTROPHYSICS↗

Recent developments in catalyst-related PEM fuel cell durability

Cost and durability remain the two major barriers to the widespread commercialization of polymer electrolyte membrane fuel cell (PEMFC)-based power systems, especially for the most impactful but challenging fuel cell electric vehicle (FCEV) application. Commercial FCEVs are now on the road; however, their PEMFC systems do not meet the cost targets established by the U.S. Department of Energy, primarily due to the high platinum loading needed on the cathode to achieve the requisite performance and lifetime. Furthermore, while the activities of a number of commercial Pt-based alloy cathode catalysts exceed the beginning-of-life (BOL) targets, these activities, and the overall cathode performance, degrade via a variety of mechanisms described herein. Degradation is mitigated in current FCEVs by utilizing a cathode catalyst with a lower BOL activity (e.g., much lower transition metal alloy content and larger BOL nanoparticle size), necessitating higher catalyst loadings, and through the utilization of system controls that avoid conditions known to exacerbate degradation processes, such as limiting the fuel cell stack voltage range. The design and development of active and robust materials and eliminating the need for vehicle mitigation strategies would greatly simplify the operating system, allowing for greater transient operation, avoiding large hybridization, and curtailing of fuel cell power. Although system mitigation strategies have provided the near-term pathway for FCEV commercialization, material-specific solutions are required to further reduce costs and improve operability and efficiency. Future material developments should focus on stabilization of the electrode structure and minimization of the catalyst particle susceptibility to dissolution caused by oxide formation and reduction over PEMFC cathode-relevant operating potentials plus minimization of support corrosion. Ex situ accelerated stress tests have provided insight into the processes responsible for material and performance degradation and will continue to provide useful information on the relative stability of materials and benchmarks for robust and stable materials-based solutions not requiring system mitigation strategies to achieve adequate lifetime.

25 ENERGY STORAGE↗

Likely accelerated weakening of Atlantic overturning circulation emerges in optimal salinity fingerprint

The long-term response of the Atlantic meridional overturning circulation (AMOC) to anthropogenic forcing has been difficult to detect from the short direct measurements available due to strong interdecadal variability. Here, we present observational and modeling evidence for a likely accelerated weakening of the AMOC since the 1980s under the combined forcing of anthropogenic greenhouse gases and aerosols. This likely accelerated AMOC weakening signal can be detected in the AMOC fingerprint of salinity pileup remotely in the South Atlantic, but not in the classic warming hole fingerprint locally in the North Atlantic, because the latter is contaminated by the “noise” of interdecadal variability. Our optimal salinity fingerprint retains much of the signal of the long-term AMOC trend response to anthropogenic forcing, while dynamically filtering out shorter climate variability. Given the ongoing anthropogenic forcing, our study indicates a potential further acceleration of AMOC weakening with associated climate impacts in the coming decades.

54 ENVIRONMENTAL SCIENCES↗

Seeded Stage III glass dissolution behavior of a statistically designed glass matrix

The glass dissolution rate of some glasses accelerates after prolonged time spent at a slow, residual glass dissolution rate. This phenomenon is referred to as Stage III behavior. Here, the acceleration in glass dissolution rate linked to Stage III behavior is significant and may be the most impactful to long-term performance of glass in a repository. This work is aimed at understanding the effect of glass composition on Stage III behavior to add a level of technical defensibility to glass disposal. To this end, a set of twenty-four glass compositions were statistically designed, where eight glass components (SiO 2 , B 2 O 3 , Al 2 O 3 , CaO, Na 2 O, SnO 2 , ZrO 2 , and Others) have been independently varied in order to study the individual effects of each. These glasses have been subjected to static dissolution tests at 90 °C in deionized water and then seeded with zeolite Na-P2 28 days into the testing to induce Stage III behavior. The response of the glasses to the zeolite seeds fell into four primary types: 1) no response to seeds; 2) an immediate linear sustained acceleration in the rate; 3) an immediate linear acceleration in the rate followed by a decrease; and, 4) a progressive acceleration in the rate that is concurrent with the addition of the seeds. The main glass components observed to influence these behaviors were CaO, Al 2 O 3 , B 2 O 3 , and ZrO 2 , where: 1) CaO influenced which glasses showed a Stage III response to seeds (high CaO: Types 2, 3, and 4) or did not respond to seeds (low CaO: Type 1), 2) Al 2 O 3 and B 2 O 3 influenced which glasses showed a sustainable Stage III response (high Al 2 O 3 : Types 2 and 4) versus transitory response (low Al 2 O 3 and high B 2 O 3 : Type 3), and 3) ZrO 2 concentration influenced whether glasses showed a linear (high ZrO 2 : Type 2) versus progressive (low ZrO 2 : Type 4) response to seeds.

36 MATERIALS SCIENCE↗

Assessment of Aging Degradation Mechanisms of Alloy 709 for Sodium Fast Reactors

This project was initiated in October 2015 to investigate the creep and creep-fatigue behavior of Alloy 709 for structural components in Gen IV sodium cooled fast spectrum reactors. The goal of this project is to develop an understanding of the mechanisms responsible for the behavior of austenitic stainless steel alloy 709 under accelerated testing conditions to confidently predict long term creep and creep-fatigue behavior at the times (500,000 hours) and temperatures (550°C) of interest for fast reactor structural applications. Alloy 709 has exhibited significantly better creep resistance than Alloy 316H, which is currently specified in design of fast reactor structural components. However, the alloy has not been code qualified for elevated temperature nuclear design. The elevated temperature microstructure stability and creep and creep-fatigue behavior need to be better understood so service life can be accurately predicted. Alloy 709 was developed for fossil boiler applications, which operate at a higher temperature than the nuclear components. Thus, there is a strong need to characterize its creep and creep-fatigue behavior at these lower temperatures and corresponding longer service lifetimes. The overall objective of this project is to develop sufficient understanding of the mechanisms responsible for behavior of Alloy 709 under accelerated testing conditions to confidently predict long term creep and creep-fatigue behavior at the times (500,000 hours) and temperatures (550°C) of interest for fast reactor structural applications. The following report summarizes the findings of the creep-fatigue and creep behavior with respect to the research questions identified during the course of the project. Additionally, the training and professional development that occurred through the project and the products resulting from the project are summarized.

36 MATERIALS SCIENCE↗

Relativistic non-thermal particle acceleration in two-dimensional collisionless magnetic reconnection

Magnetic reconnection, especially in the relativistic regime, provides an efficient mechanism for accelerating relativistic particles and thus offers an attractive physical explanation for non-thermal high-energy emission from various astrophysical sources. I present a simple analytical model that elucidates key physical processes responsible for reconnection-driven relativistic non-thermal particle acceleration in the large-system, plasmoid-dominated regime in two dimensions. The model aims to explain the numerically observed dependencies of the power-law index $p$ and high-energy cutoff $\gamma _c$ of the resulting non-thermal particle energy spectrum $f(\gamma )$ on the ambient plasma magnetization $\sigma$ , and (for $\gamma _c$ ) on the system size $L$ . In this self-similar model, energetic particles are continuously accelerated by the out-of-plane reconnection electric field $E_{\rm rec}$ until they become magnetized by the reconnected magnetic field and eventually trapped in plasmoids large enough to confine them. The model also includes diffusive Fermi acceleration by particle bouncing off rapidly moving plasmoids. I argue that the balance between electric acceleration and magnetization controls the power-law index, while trapping in plasmoids governs the cutoff, thus tying the particle energy spectrum to the plasmoid distribution.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Comparison of Simulated and Experimentally Measured Detector Impulse Responses to Pulsed X-rays

The Gamma Array Simulation Toolkit (GAST) is a multi-physics software stack comprised of Geant4, MATLAB, and experimentally measured photomultiplier tube (PMT) impulse response waveforms that is used to model and inform the end-to-end performance of radiation detector systems. In order to validate the ability of GAST to predict the impulse response of a modeled detector configuration operated in current mode, experimental measurements using the Nevada National Security Site Transformational Diagnostics and Imaging 2 MeV endpoint energy electron linear accelerator (linac) with a tungsten target were performed. Seven different detector configurations consisting of unique combinations of scintillator material, size, reflectivity conditions, presence or absence of light guide, and PMT were evaluated. The resultant impulse response of each detector configuration was recorded and compared to a GAST simulation that emulated the respective linac experiment conditions. The comparison of the experimental and simulated detector impulse responses indicated that GAST can reliably predict detector impulse responses.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Assessment of the Pan-Arctic Accelerated Rate of Sea Ice Decline in CMIP6 Historical Simulations

Abstract Arctic sea ice loss in response to a warming climate is assessed in 42 models participating in phase 6 of the Coupled Model Intercomparison Project (CMIP6). Sea ice observations show a significant acceleration in the rate of decline commencing near the turn of the twenty-first century. It is our assertion that state-of-the-art climate models should qualitatively reflect this accelerated trend within the limitations of internal variability and observational uncertainty. Our analysis shows that individual CMIP6 simulations of sea ice depict a wide range of model spread on biases and anomaly trends both across models and among their ensemble members. While the CMIP6 multimodel mean captures the observed sea ice area (SIA) decline relatively well, an individual model’s ability to represent the acceleration in sea ice decline remains a challenge. Seventeen (40%) out of 42 CMIP6 models and 37 (13%) out of the total 286 ensemble members reasonably capture the observed trends and acceleration in SIA decline. In addition, a larger ensemble size appears to increase the odds for a model to include at least one ensemble member skillfully representing the accelerated SIA trends. Simulations of sea ice volume (SIV) show much larger spread and uncertainty than SIA; however, due to limited availability of sea ice thickness data, these are not as well constrained by observations. Finally, we find that models with more ocean heat transport simulate larger sea ice declines, which suggests an emergent constraint in CMIP6 ensembles. This relationship points to the need for better understanding and modeling of ice–ocean interactions, especially with respect to frazil ice growth.

54 ENVIRONMENTAL SCIENCES↗

Electron energization dynamics in interaction of self-generated magnetic vortices in upstream of collisionless electron/ion shocks

Abstract Relativistic collisionless shocks are considered responsible for particle energization mechanisms leading to particle acceleration. While electron energization in shock front region of electron/ion collisionless shocks are the most studied, the mechanism of electron energization in interaction with self-generated magnetic vortices (MVs) in the upstream region is still unclear. We investigate electron energization mechanism in the upstream region of electron/ion relativistic collisionless shocks, using two dimensional particle-in-cell (PIC) simulations. We discuss mechanism of electron energization which takes place in the upstream region of the shock, where the counter stream particles interact with incoming flow. The energy gain of electrons happens during their interaction with evolving fields of self-generated magnetic vortices in this region. Three Fermi-like electron energization scenarios are discussed. Stochastic acceleration of electrons in interaction with fields of MV leads to anisotropic heating of fast electrons due to diffusion in the momentum space of electrons and, finally, synergetic effect of evolving fields of MVs leads to the formation of a power-law tail of supra-thermal particles.

Naseri, N.↗

Thermal evolution of ferroelectric behavior in epitaxial Hf 0.5 Zr 0.5 O 2

In this paper, we report a cryogenic-temperature study on the evolution of the ferroelectric properties of epitaxial Hf 0.5 Zr 0.5 O 2 thin films on silicon. Wake-up, endurance, and fatigue of these films are found to be intricately correlated, strongly hysteretic, and dependent on available thermal energy. Field-dependent measurements reveal a decrease in polarization with temperature, which has been determined not to be an intrinsic change of the material property, rather a demonstration of the increase in the coercive bias of the material. Our findings suggest that a deficiency in thermal energy suppresses the mobility of defects presumed to be oxygen vacancies during wake-up and trapped injected charge during fatigue, which is responsible for polarization evolution during cycling. This permits accelerated wake-up and fatigue effects at high temperatures where thermal energy is abundant but delays these effects at cryogenic temperatures.

36 MATERIALS SCIENCE↗

Landscape fragmentation overturns classical metapopulation thinking

Habitat loss and isolation caused by landscape fragmentation represent a growing threat to global biodiversity. Existing theory suggests that the process will lead to a decline in metapopulation viability. However, since most metapopulation models are restricted to simple networks of discrete habitat patches, the effects of real landscape fragmentation, particularly in stochastic environments, are not well understood. To close this major gap in ecological theory, we developed a spatially explicit, individual-based model applicable to realistic landscape structures, bridging metapopulation ecology and landscape ecology. This model reproduced classical metapopulation dynamics under conventional model assumptions, but on fragmented landscapes, it uncovered general dynamics that are in stark contradiction to the prevailing views in the ecological and conservation literature. Notably, fragmentation can give rise to a series of dualities: a) positive and negative responses to environmental noise, b) relative slowdown and acceleration in density decline, and c) synchronization and desynchronization of local population dynamics. Furthermore, counter to common intuition, species that interact locally (“residents”) were often more resilient to fragmentation than long-ranging “migrants.” This set of findings signals a need to fundamentally reconsider our approach to ecosystem management in a noisy and fragmented world.

54 ENVIRONMENTAL SCIENCES↗

Intraspecific Reaction Norm Variation Controls the Eco-Evolutionary Consequences of Environmental Change

As environmental change accelerates globally, understanding concurrent organismal, species, and community responses is increasingly vital. Here, we examine these collective responses by incorporating genotype-specific thermal reaction norms into an eco-evolutionary predator-prey model, allowing us to track simultaneous phenotypic, ecological, and evolutionary responses to environmental change within ecological communities. We show that the reaction norms expressed by genotypes within a population determine how a community switches between different eco-evolutionary outcomes with changes in temperature. We identify how different components of phenotypic variation in thermal reaction norms—environmental (E), additive environmental and genetic (E + G), and gene-by-environment interactions (G × E)—influence eco-evolutionary dynamics and outcomes as temperature changes. Furthermore, our findings underscore how complex eco-evolutionary responses to environmental change ultimately emerge from variation in reaction norms among genotypes, offering new mechanistic insights into environmental impacts on adaptation, the maintenance of phenotypic and genetic variation, and ecological stability, which is crucial for understanding and predicting eco-evolutionary effects of rapid environmental change in the future.

Eco-evolutionary↗

Machine Learning Benchmarks for the Classification of Equivalent Circuit Models from Electrochemical Impedance Spectra

Analysis of Electrochemical Impedance Spectroscopy (EIS) data for electrochemical systems often consists of defining an Equivalent Circuit Model (ECM) using expert knowledge and then optimizing the model parameters to deconvolute various resistance, capacitive, inductive, or diffusion responses. For small data sets, this procedure can be conducted manually; however, it is not feasible to manually define a proper ECM for extensive data sets with a wide range of EIS responses. Automatic identification of an ECM would substantially accelerate the analysis of large sets of EIS data. We showcase machine learning methods to classify the ECMs of 9,300 impedance spectra provided by QuantumScape for the BatteryDEV hackathon. The best-performing approach is a gradient-boosted tree model utilizing a library to automatically generate features, followed by a random forest model using the raw spectral data. A convolutional neural network using boolean images of Nyquist representations is presented as an alternative, although it achieves a lower accuracy. We publish the data and open source the associated code. The approaches described in this article can serve as benchmarks for further studies. A key remaining challenge is the identifiability of the labels, underlined by the model performances and the comparison of misclassified spectra.

25 ENERGY STORAGE↗

Redesign of the Timeline Generator at Fermilab using a web-based Flutter application, GraphQL API and an IOC

The control system at Fermilab is undergoing an evolution with a shift towards web-based applications with connections to the EPICS infrastructure. The Timeline Generator (TLG) is an application that serves to coordinate events across the lab using different timing links. These links include the Tevatron clock (TCLK), a 10 MHz serial link with events encoded at 20Hz and Machine Data (MDAT), a communication link with states encoded at 720Hz. This paper covers the redesign of the major components of the TLG. This includes a web-based Flutter application for building timelines. A placement service is in use that has a GraphQL interface and uses a timeline input to compute a schedule of events and states. The Flutter application sends this computed schedule to the TLG IOC via a GraphQL interface to the Data Pool Manager (DPM). The TLG IOC runs on an Arria FPGA, the Accelerator Clock Generator (ACLK-GEN), which is responsible for writing the events and states on to the different timing links.

Carmichael, Linden [Fermilab]↗

Redesign of the Timeline Generator at Fermilab using a web-based Flutter Application, GraphQL API and an IOC

Redesign of the Timeline Generator at Fermilab using a web-based Flutter application, GraphQL API and an IOC ABSTRACT = The control system at Fermilab is undergoing an evolution with a shift towards web-based applications with connections to the EPICS infrastructure. The Timeline Generator (TLG) is an application that serves to coordinate events across the lab using different timing links. These links include the Tevatron clock (TCLK), a 10 MHz serial link with events encoded at 20Hz and Ma-chine Data (MDAT), a communication link with states encoded at 720Hz. This paper covers the redesign of the major components of the TLG. This includes a web-based Flutter application for building timelines. A placement service is in use that has a GraphQL interface and uses a timeline input to compute a schedule of events and states. The Flutter application sends this computed schedule to the TLG IOC via a GraphQL interface to the Data Pool Manager (DPM). The TLG IOC runs on an Arria FPGA, the Accelerator Clock Generator (ACLK-GEN), which is responsible for writing the events and states on to the different timing links.

Carmichael, Linden [Fermilab]↗

Electrification Futures Study: Power Systems Operation with Newly Electrified and Flexible Loads

The Electrification Futures Study (EFS) is a multi-year study designed to analyze the impacts of widespread electrification in the U.S. energy system. In this webinar we present the detailed power systems operational analysis from the final report in the EFS series. For this analysis, we simulate multiple 2050 power systems for the conterminous United States to assess how variations in the magnitude and shape of electricity demand driven by electrification, and the extent of load participation to more-actively provide grid services, might impact the hourly operation, operational costs, and emissions of various power systems in 2050. The impacts of electrification and demand flexibility are overlayed across systems with significantly greater penetrations of variable renewable energy than today. Overall, we find that the high electrification scenarios envisioned in the EFS with significant VRE penetration (66% of annual national generation) can be operated to meet future increased levels of electrified demand. We also find that demand-side flexibility can enhance operational efficiency and reduce overall annual production costs by $5-$10 billion. The complementary relationship between flexible electric vehicle charging loads and solar generation is particularly pronounced, but in the absence of demand-side flexibility electrification can lead to increased wind and solar curtailment. By helping to reduce renewable curtailment, flexibility can also reduce power sector CO2 emissions. The analysis highlights the value of increased integration and coordination of demand- and supply-side resources in future electric system planning and operations—particularly under high electrification futures.

43 PARTICLE ACCELERATORS↗

‪A Novel Methodology for Longitudinal Studies of Home Thermal Comfort Perception and Behavior

Human-building interactions significantly influence building energy consumption and affect peak energy demand. For example, heating and cooling contribute 46% of daily peak residential energy demand. Grid-interactive efficient buildings (GEBs) can potentially increase energy-demand flexibility and accelerate the adoption of renewables. However, traditional demand response (DR) programs focused on shedding peak loads disregard the human-building interactions leading to occupant thermal frustration. Specifically, they do not model occupants’ ability to override thermostat controls, nor how indoor environmental conditions and sociocultural factors affect the timing and magnitude of overrides. Studies have found 20% of occupants override thermostat setpoints during DR events longer than 6 hours yet lack detail about the motivation that might guide more successful efforts. Balancing energy-demand flexibility with occupant thermal comfort requires understanding dynamic occupant behavior, the underlying psychophysiological drivers, in the context of homes. This paper presents methods for scalable longitudinal studies of residential occupant behavior dynamics to inform the development of psychophysiological occupant-centric building models. Smart sensors were installed to measure local environmental conditions in 20 homes in two regions of the United States. Just-in-time ecological momentary assessments (EMAs) provided qualitative data on occupant thermal comfort and local environmental conditions not captured in Internet-of-Things (IoT) based studies or existing datasets. Participant interviews provided insight into environmental attitudes, mental models, and the role of economics in comfort and behavior, which in turn may affect thermostat interactions. Based on these data, interventions in the next phase of the study will collect data and monitor occupant behavior during simulated DR events.

Kane, Michael↗