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At least 127 records · Page 7

Design of a Thermal Precipitator for the Characterization of Smoke Particles from Common Spacecraft Materials

A thermal precipitator (TP) was designed to collect smoke aerosol particles for microscopic analysis in fire characterization research. Information on particle morphology, size and agglomerate structure obtained from these tests supplements additional aerosol data collected. Modeling of the thermal precipitator throughout the design process was performed with the COMSOL Multiphysics finite element software package, including the Eulerian flow field and thermal gradients in the fluid. The COMSOL Particle Tracing Module was subsequently used to determine particle deposition. Modeling provided optimized design parameters such as geometry, flow rate and temperatures. The thermal precipitator was built and testing verified the performance of the first iteration of the device. The thermal precipitator was successfully operated and provided quality particle samples for microscopic analysis, which furthered the body of knowledge on smoke particulates. This information is a key element of smoke characterization and will be useful for future spacecraft fire detection research.

Smoke↗

Aircraft-Measured Indirect Cloud Effects from Biomass Burning Smoke in the Arctic and Subarctic

The incidence of wildfires in the Arctic and subarctic is increasing; in boreal North America, for example, the burned area is expected to increase by 200-300% over the next 50-100 years, which previous studies suggest could have a large effect on cloud microphysics, lifetime, albedo, and precipitation. However, the interactions between smoke particles and clouds remain poorly quantified due to confounding meteorological influences and remote sensing limitations. Here, we use data from several aircraft campaigns in the Arctic and subarctic to explore cloud microphysics in liquid-phase clouds influenced by biomass burning. Median cloud droplet radii in smoky clouds were approx. 40- 60% smaller than in background clouds. Based on the relationship between cloud droplet number (N(liq)/ and various biomass burning tracers (BBt/ across the multi-campaign data set, we calculated the magnitude of subarctic and Arctic smoke aerosol-cloud interactions (ACIs, where ACI = (1/3) x dln(N(liq))/dln(BBt)) to be approx. 0.16 out of a maximum possible value of 0.33 that would be obtained if all aerosols were to nucleate cloud droplets. Interestingly, in a separate subarctic case study with low liquid water content (0.02 gm/cu m and very high aerosol concentrations (2000- 3000/ cu cm in the most polluted clouds, the estimated ACI value was only 0.05. In this case, competition for water vapor by the high concentration of cloud condensation nuclei (CCN) strongly limited the formation of droplets and reduced the cloud albedo effect, which highlights the importance of cloud feedbacks across scales. Using our calculated ACI values, we estimate that the smoke-driven cloud albedo effect may decrease local summertime short-wave radiative flux by between 2 and 4 W/sq m or more under some low and homogeneous cloud cover conditions in the subarctic, although the changes should be smaller in high surface albedo regions of the Arctic.We lastly explore evidence suggesting that numerous northern-latitude background Aitken particles can interact with combustion particles, perhaps impacting their properties as cloud condensation and ice nuclei.

cloud microphysics↗

The Relationship Between MAIAC Smoke Plume Heights and Surface PM

Biomass burning is a source of fine particulate matter (PM2.5) air pollution, which adversely impacts human health. However, quantifying the health effects from biomass burning PM2.5 is difficult. Monitoring networks generally lack the spatial density needed to capture the heterogeneity of biomass burning smoke. Satellite aerosol optical depth (AOD) can be used to fill spatial gaps but does not distinguish surface‐level aerosols. Plume height (PH) observations may provide constraints on the vertical distribution of smoke and its impact on surface concentrations. We assessed PH characteristics from Multi‐Angle Implementation of Atmospheric Correction (MAIAC) and evaluated its correlation with colocated PM2.5 and AOD measurements. PH is generally highest over the western United States. The ratio PM2.5:AOD generally decreases with increasing PH:PBLH (planetary boundary layer height), showing that PH has the potential to refine surface PM2.5 estimates for collections of smoke events.

satellite retrieved smoke plume heights↗

Constraints on Wildfire Smoke Source Strength, Injection Height, and Particle Evolution

Aerosol sources are represented in climate and air quality models with an injection height and a source strength. We have applied a combination of Multi-angle Imaging SpectroRadiometer (MISR) and MODerate resolution Imaging Spectroradiometer (MODIS) observations to help constrain these two key model variables for wildfire smoke plumes. Injection height is obtained from MISR stereo imagery, which makes it possible to map plume elevation and estimate the associated motion vectors at plume altitude near-source, where contrast features in the plume can be identified in the multi-angle views. A current limitation of injection-height mapping is the relatively narrow MISR swath width (~380 km) and 10:30 AM equator crossing time on the day side of Earth. However, upcoming missions, as well as advanced imagers on geostationary platforms, promise to greatly expand the spatial and temporal range over which this technique can be applied. We estimate source strength by matching forward-simulated plume aerosol optical depth (AOD) from models with AOD snapshots retrieved from MODIS observations. This technique works best for large, isolated plumes common in boreal forest, and tends to fail where plume AOD is low and/or background AOD, distinct from the specific source of interest, is high. These two approaches for constraining aerosol modeling with satellite observations have been the subject of ongoing AeroCom/AeroSat studies by our group. A third effort applies the combination of MISR plume heights, wind vectors, and particle microphysical property constraints to infer smoke-plume particle evolution processes and timescales, including the emission and subsequent evolution of black and brown smoke. In this presentation, we will provide an update on the status of these efforts.

wildfire↗

Quantifying SAGE II (1984-2005) and SAGE III/ISS (2017-2022) Observations of Smoke in the Stratosphere

The Stratospheric Aerosol and Gas Experiment (SAGE II) operated for over 20 years (1984-2005) and collected near global observations of aerosol extinction coefficient from the upper troposphere to about 40 km. SAGE III has flown aboard the International Space Station (ISS) since 2017 and has collected comparable aerosol measurements during this period. The SAGE II record is dominated by recovery from El Chichón (1982) and the Pinatubo eruption of 1991 with a few smaller volcanic events that are detectable in the data set. In addition, a number of pyrocumulus events injected smoke into the lower stratosphere with magnitudes that are comparable to the smaller volcanic events. The shorter SAGE III/ISS record is qualitatively different than SAGE II’s with a number of small to moderate volcanic eruptions in both low and high latitudes (e.g., Ambae in 2018 and Raikoke in 2020) as well several smoke events including the two largest events seen by SAGE-like instruments: the BC pyrocumulus event in 2017 and the Australian brush fires of 2020/2021. In this paper, I will review the detection and quantification of the magnitude of these smoke events with a particular focus on the differences between the two data periods.

Smoke↗

Quantifying SAGE II (1984-2005) and SAGE III/ISS (2017-2022) Observations of Smoke in the Stratosphere

The Stratospheric Aerosol and Gas Experiment (SAGE II) operated for over 20 years (1984-2005) and collected near global observations of aerosol extinction coefficient from the upper troposphere to about 40 km. SAGE III has flown aboard the International Space Station (ISS) since 2017 and has collected comparable aerosol measurements during this period. The SAGE II record is dominated by recovery from El Chichón (1982) and the Pinatubo eruption of 1991 with a few smaller volcanic events that are detectable in the data set. In addition, a number of pyrocumulus events injected smoke into the lower stratosphere with magnitudes that are comparable to the smaller volcanic events. The shorter SAGE III/ISS record is qualitatively different than SAGE II’s with a number of small to moderate volcanic eruptions in both low and high latitudes (e.g., Ambae in 2018 and Raikoke in 2020) as well several smoke events including the two largest events seen by SAGE-like instruments: the BC pyrocumulus event in 2017 and the Australian brush fires of 2020/2021. In this talk, I will review the detection and quantification of the magnitude of these smoke events with a particular focus on the differences between the two data periods.

Smoke Stratosphere SAGE↗

StratoFIRE: Modeling Wildfire Smoke in the Stratosphere

The most extreme manifestation of a fire–weather interaction is the formation of pyrocumulonimbus (pyroCb) thunderstorms, triggered by super-heated updrafts, which can eject smoke at altitudes exceeding 20 Km. In this study, we investigated climate-related impacts from the most intensive pyroCb-triggered injection of smoke in the stratosphere: the Australian New Year wildfires in 2019/2020. We first provide a general overview of the vision and objectives of the StratoFIRE project. With the aid of the global chemistry-climate model EMAC, we then simulate radiative and chemical perturbations in the stratosphere in relation to 0.9 Tg smoke in the stratosphere assuming different injection heights, from 13 to 16 Km. The simulation of stratospheric optical depth perturbations were found to be sensitive to the assumed injection height, with a maximum height at 16 Km showing the best agreement with the GLOSSAC and SAGE-ISS aerosol extinction observations.

PyroCb↗

Quantifying SAGE II (1984-2005) and SAGE III/ISS (2017-2022) Observations of Smoke in the Stratosphere

The Stratospheric Aerosol and Gas Experiment (SAGE II) operated for over 20 years (1984-2005) and collected near global observations of aerosol extinction coefficient from the upper troposphere to about 40 km. SAGE III has flown aboard the International Space Station (ISS) since 2017 and has collected comparable aerosol measurements during this period. The SAGE II record is dominated by recovery from El Chichón (1982) and the Pinatubo eruption of 1991 with a few smaller volcanic events that are detectable in the data set. In addition, a number of pyrocumulus events injected smoke into the lower stratosphere with magnitudes that are comparable to the smaller volcanic events. The shorter SAGE III/ISS record is qualitatively different than SAGE II’s with a number of small to moderate volcanic eruptions in both low and high latitudes (e.g., Ambae in 2018 and Raikoke in 2020) as well several smoke events including the two largest events seen by SAGE-like instruments: the BC pyrocumulus event in 2017 and the Australian brush fires of 2020/2021. In this talk, I will review the detection and quantification of the magnitude of these smoke events with a particular focus on the differences between the two data periods.

SAGE↗

Photogrammetric and photometric investigation of a smoke plume viewed from space.

Use of detailed analyses of an Apollo 6 stereographic photograph of a smoke plume which originated in southern Arizona and crossed over into Mexico to illustrate how high-resolution photography can aid meteorologists in evaluating specific air pollution events. Photogrammetric analysis of the visible smoke plume revealed that the plume was 8.06 miles long and attained a maximum width of 4000 ft, 3.0 miles from the 570-ft chimney emitting the effluent. Stereometric analysis showed that the visible top of the plume rose nearly 2400 ft above stack top, attaining 90% of this total rise 1.75 miles downwind from the source. Photometric analysis of the plume revealed a field of plume optical density that portrayed leptokurtic and bimodal distributions rather than a true Gaussian distribution. A horizontal eddy diffusivity of about 650,000 sq cm/sec and a vertical eddy diffusivity of 230,000 sq cm/sec were determined from the plume dimensions. Neutron activation analysis of plume samples revealed the elemental composition of the smoke to be copper, arsenic, selenium, indium and antimony, with trace amounts of vanadium and scandium.

Randerson, D.↗

Smoke Plume Analysis Using Fan-beam and Single-beam Radiometers

Smoke plume data were taken using the stacks of the Mills Road Steam Plant on Redstone Arsenal, Huntsville, Alabama. The fan-beam unit was placed approximately 235 meters east of the Mills Road Steam Plant, and the single-beam unit was placed approximately 80 meters north of the fan-beam unit. Results of the smoke plume measurements indicate that the smoke plume is a periodic process near the mouth of the smokestack. The usefulness of the system is limited because of inaccurate and cumbersome positioning methods and base line constraints due to cable length. It is recommended that the radiometers be mounted on pedestals which have both azimuth and elevation positions determined by digitally controlled stepper drive motors. It is also recommended that a time multiplex system be used to transmit data from the radiometers to the electronics van.

Dodd, J. L.↗

Smoke density studies with the Arapahoe and NBS chambers

Smoke density studies on twelve cellulosic and five synthetic materials using the Arapahoe and NBS smoke chambers show an empirical relationship between smoke weight as per cent of initial weight in the Arapahoe test and maximum specific optical density under piloted conditions in the NBS test. The NBS optical density data under piloted conditions exhibited sensitivity to test artifacts such as type of pilot burner.

Hilado, C. J.↗

Visualization of the laminar-turbulent transition in the flow over an airfoil using the smoke-wire technique

A flow visualization technique, referred to as the smoke-wire, was used for visualization of the transition of the free shear layer associated with the laminar separation bubble of a NACA 66 sub 3-018 airfoil section at low Reynolds number (50,000-130,000). The smoke-wire technique allows the introduction of fine smoke streaklines into the flow field through the electrical resistive heating of a very fine wire which has been coated with oil and which is located upstream from the leading edge of the airfoil section. Streakline data were collected using both high speed still and motion picture photography.

Batill, S. M.↗

Analytical electron microscopy of Mg-SiO smokes - A comparison with infrared and XRD studies

Analytical electron microscopy conducted for Mg-SiO smokes (experimentally obtained from samples previously characterized by IR spectroscopy) indicates that the microcrystallinity content of unannealed smokes increases with increased annealing for up to 30 hr. The growth of forsterite microcrystallites in the initially nonstoichiometric smokes may give rise to the contemporaneous growth of the SiO polymorph tridymite and MgO; after 4 hr of annealing, these react to form enstatite. It is suggested that XRD analysis and IR spectroscopy should be conducted in conjunction with detailed analytical electron microscopy for the detection of emerging crystallinity in vapor-phase condensates.

Rietmeijer, F. J. M.↗

Smoke optical depths - Magnitude, variability, and wavelength dependence

An airborne autotracking sun-photometer has been used to measure magnitudes, temporal/spatial variabilities, and the wavelength dependence of optical depths in the near-ultraviolet to near-infrared spectrum of smoke from two forest fires and one jet fuel fire and of background air. Jet fuel smoke optical depths were found to be generally less wavelength dependent than background aerosol optical depths. Forest fire smoke optical depths, however, showed a wide range of wavelength depedences, such as incidents of wavelength-independent extinction.

Pueschel, R. F.↗

Trapping Ne, Ar, Kr, and Xe in Si2O3 smokes

Simple Si2O3 smokes have been condensed at both low (less than 750 K) and high (greater than 1000 K) temperature at 35 torr H2 pressure in the presence of 0, 10, 100, and 1000 microns of a noble gas mixture containing Ne, Ar, Kr, and Xe. In general, both Ne and Ar are quite loosely bound in the smokes (6.0 x 10 to the -8th and 2.6 x 10 to the -4th ccSTP/g, respectively), and are degassed at temperatures below 1200 K. Both Kr and Xe are somewhat more strongly bound at concentrations of 1.0 x 10 to the -7th and 8.2 x 10 to the -8th ccSTP/g, respectively, and in addition show a double release with a second component at a temperature of about 1875 K. With the exception that Si2O3 smokes appear to show a particular affinity for argon, possibly due to an anomalous absorption of atmospheric argon, none of the other noble gases are found in sufficient concentration to explain the gases observed in meteorites as primary circumstellar condensates. However, this data in conjunction with observations of Honda et al. (1979) do seem to show a degree of dependence between noble gas retention and chemical composition.

Nuth, Joseph A., III↗

Smoke Generator For Studies Of Vortices In Flight

Smoke-generating system used to identify vortex-core and vortex-core-breakdown locations in flights. Housed in forebody of airplane, includes multiple pyrotechnic smoke cartridges fired simultaneously or in sequence. Firing of cartridges controlled from cockpit, and smoke produced ducted to desired locations on or near surface of aircraft. Useful for other aerodynamic flight research in which necessary to visualize local flows. Nonaerospace applications include research in reduction of aerodynamic drag on vehicles and reduction of turbulence related to structures or other obstacles.

Richwine, David M.↗

Kuwait oil fires - Compositions of source smoke

While the Kuwait oil-fire smoke plumes manifested a pronounced impact on solar radiation in the Gulf region (such as visibility and surface temperatures), smoke plume concentrations of combustion-generated pollutants suggest that the overall chemical impact on the atmosphere of the smoke from these fires was probably much less than anticipated. Combustion in the Kuwaiti oil fires was surprisingly efficient, releasing on average more than 93 percent of the combusted hydrocarbon fuels as CO2. Correspondingly, combustion-produced quantities of carbon monoxide (CO) and carbonaceous particles were low, each about 2 percent by weight. The fraction of CH4 produced by the fires was also relatively low (about 0.2 percent), but source emissions of nonmethane hydrocarbons were high (about 2 percent). Processes other than combustion (e.g., volatilization) probably contributed significantly to the measured in-plume hydrocarbon concentrations. Sulfur emissions (particulate and gaseous) measured at the source fires were lower (about 0.5 percent) than predicted based on average sulfur contents in the crude. N2O emissions from the Kuwaiti oil fires were very low and often could not be distinguished from background concentrations.

Cofer, Wesley R., III↗

Directional and spectral reflectance of the Kuwait oil-fire smoke

The angular reflectance pattern of the Kuwait oil-fire smoke was measured from an aircraft at 13 discrete wavelengths between 0.5 and 2.3 microns. Measurements at 0.75 and 1.64 micron showed that the reflectance of the smoke layer was about 12 percent in the nadir direction, with considerable limb brightening toward the horizon. Furthermore, these observations revealed a backscattering maximum in the antisolar direction and an enhanced scattering near the rainbow direction. These characteristics suggest that the smoke layer 90 km downwind of the Kuwait oil fires was composed of a significant number of oil drizzle droplets that scatter solar radiation as a layer composed of spherical particles.

King, Michael D.↗