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Advanced Diagnostics For Megahertz Imaging Of Mixing, Fuel Spray, And Combustion Processes For Rotating Detonation Combustors

Recent advancements in megahertz rate, high-power, burst-mode laser technology are leveraged to perform and explore imaging measurements that spatially and temporally resolve the mixing, combustion, and detonation flow field in two laboratory-scale rotating detonation combustors (RDCs). In a non-premixed annular RDC, multiple imaging diagnostics are explored to investigate gaseous and liquid injector behavior, the detonation wave structure, and the propellant refill. In one instance, OH planar laser-induced fluorescence (OH-PLIF) imaging is performed up to a 2 MHz repetition rate to track the combustion products and reaction zone locations. In the same annular RDC, a single liquid fuel jet is injected, and laser-based 355-nm imaging of the fuel spray is performed up to a 1 MHz repetition rate. For this configuration, the annular RDC is used as a detonation driver to impose periodic detonation waves to interact with the fuel spray. Moreover, in this annular RDC, a range of tracer-based laser imaging measurements are explored to time-resolve the unsteady oxidizer air recovery and refill process. In a non-premixed linear RDC, planar imaging measurements of the fuel mixing are performed up to a 200 kHz repetition rate using PLIF of a tracer in the fuel supply. The fuel mixing imaging helps explain the origin of the observed pre and post wave burning, detonation structure, and enables quantifying injector recovery timescales. This paper will provide a high-level broad survey of diagnostics applied in these RDCs, lessons learned, and interesting observations.

Combustion↗
DOE OSTI2021

Scaling of oxygen-methane reacting coaxial jets using x-ray fluorescence to measure mixture fraction

Stoichiometric mixing length L s of reacting coaxial jet flames is a critical scaling parameter for liquid rocket engine combustors. Previous studies have shown that L s for shear coaxial flames can be scaled like their non-reacting counterparts using a non-dimensional momentum flux ratio J. In addition, stoichiometric mixing lengths of reacting and nonreacting coaxial jets collapse upon a single line by altering J using an effective outer flow gas density. This effective density is calculated from a modified version of the equivalence principle, originally developed by Tacina and Dahm [1, 2] and accounts for the effects of heat release on mixing. However, previous studies also required a second nonphysical scaling constant S c for the reacting jets, which is not predicted by the equivalence principle [3]. It was originally hypothesized that S c is attributed to the limitation of hydroxyl (OH) planar laser-induced fluorescence, which only infers L s . Direct quantitative measurement of conserved scalar fields using conventional optical diagnostics is difficult due to the lack of a tracer that easily fluoresces, survives high temperature oxygen flames, and is not dominated by quenching effects. To measure a conserved scalar field, this work implements x-ray fluorescence of Kr and Ar tracers to obtain quantitative mixture fraction fields. From these mixture fraction fields, stoichiometric mixing lengths for two CH 4 /O 2 flames are calculated and scaled against nonreacting coaxial mixing lengths using the equivalence principle. By directly measuring the stoichiometric mixing length, it is established that the additional constant is a byproduct of the OH measurement technique and the equivalence principle fully captures the scaling. Finally, comparison with high-fidelity simulation of the flame further supports this conclusion. In addition to further strengthening this scaling method, this work represents the first use of x-ray fluorescence to make quantitative conserved scalar measurements in turbulent flames.

33 ADVANCED PROPULSION SYSTEMS↗
DOE OSTI2025

Characterization of Flashback and Flame-Holding in a Jet-in-Crossflow Mixing Configuration with Methane-Hydrogen Fuel Blends

An approach that combines experimental and numerical analyses has been implemented to characterize the fundamentals of flashback events and flame-holding phenomena during high-hydrogen combustion in a jet-in-crossflow (JICF) configuration. Such flame dynamics are visualized experimentally using nanosecond (ns)-based hydroxyl planar laser-induced fluorescence (OH-PLIF) and chemiluminescence diagnostics techniques. The JICF burner has an optically accessible pre-mixing tube allowing the optical diagnostics. The testing was conducted for varied pre-mixer velocities (V) and equivalence ratio (ϕ) for 90%-100% (H2, by mole) H2/CH4 reactant mixtures at atmospheric temperature and pressure conditions. Two distinct flashback events were identified – conventional rich flashback and lean flashback, recorded while increasing ϕ and decreasing ϕ, respectively. The cause of lean flashback was attributed to the lower momentum flux ratio which bends the jet sharply, closer toward the injection plane. The mean OH-PLIF images characterized the flame-holding behavior where the flame was found to be stabilized on the leeward side only or on both windward and leeward sides as a lifted flame near the fuel port. A Large Eddy Simulation (LES) with detailed chemistry combustion modeling approach was implemented along an OH* sub-mechanism, and it showed qualitative agreement with the integrated line-of-sight chemiluminescence results as well as the planar OH-PLIF measurements.

flame holding↗
DOE OSTI2021

Beyond Taylor’s hypothesis: a novel volumetric reconstruction of velocity and density fields for variable‑density and shear flows

Abstract This work presents a novel numerical procedure for reconstructing volumetric density and velocity fields from planar laser-induced fluorescence (PLIF) and stereoscopic particle image velocimetry (SPIV) data. This new method is theoretically and practically demonstrated to provide more accurate 3D vortical structures and density fields in high shear flows than reconstruction methods based on the mean convective velocity. While Taylor’s hypothesis of frozen turbulence is commonly applied by using the local mean streamwise velocity, the proposed algorithm uses the measured local instantaneous velocity for data convection. It consists of a step-by-step reconstruction based on a mixed Lagrangian–Eulerian solver that includes the 3D interpolation of scattered flow data and that relaxes the Taylor’s hypothesis by iterative enforcement of the incompressibility constraint on the velocity field. This methodology provides 3D fields with temporal resolution, spatial resolution, and accuracy comparable to that of real 3D snapshots, thus providing a practical alternative to tomographic measurements. The procedure is validated using numerical data of the constant-density channel flow available on the Johns Hopkins University Turbulence Database (JHTDB), showing the accurate reconstruction of the 3D velocity field. The algorithm is applied to an experimental dataset of PLIF and SPIV measurements of a variable-density jet flow, demonstrating its capability to provide 3D velocity and density fields that are more consistent with the Navier–Stokes equations compared to the mean flow convective method. Graphic abstract

42 ENGINEERING↗
DOE OSTI2021

Fog Formation Related to Gravity Currents Interacting with Coastal Topography

An interesting mixing-fog event was identified during IOP7 of the C-FOG project, where a cold front arriving from the north-east collided with the Downs peninsula in Ferryland, Newfoundland, to produce foggy conditions. A comprehensive set of field observations suggests that this collision caused turbulent mixing of nearly saturated ambient air with an almost saturated cold front, creating conditions for mixing fog. Additionally, laboratory experiments were performed to study the interaction of lock-exchange induced gravity currents with a (rectangular) obstacle to delve into physical processes underlying this phenomenon. Instantaneous velocity and density fields were obtained using particle image velocimetry and planar laser-induced fluorescence. The observations suggest that the obstacle starts affecting the approaching gravity-current propagation at an upstream distance of 2 H and, upon collision, the mixing is taking place over a spatial scale of 0.83 H , where H is the depth of the ambient fluid layer. The time for largerscale turbulent stirring to permeate to the smallest scales of turbulence and activate the condensation nuclei was estimated as 3t * , where t* = √H/g' is the intrinsic time scale of the gravity current and g' the reduced gravity. Extrapolation of results to IOP7 showed a good agreement with observations.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2022

On the effects of reactant stratification and wall curvature in non-premixed rotating detonation combustors

The optimization of non-premixed rotating detonation combustors (RDCs) requires improved understanding of the coupled effects of reactant stratification, fluid property gradients, and complex shock-wave interactions on the detonation wave structure within annular geometries. In the current work, simultaneous orthogonal views of chemiluminescence and hydroxyl planar laser-induced fluorescence (PLIF) are utilized to establish the existence of a dual-wave system characterized by leading and trailing detonation waves that are closely coupled by the local flow physics. These features are persistent over a wide range of mass flow rates and are consistent with prior observations of non-premixed rotating detonations in annular geometries. The detailed instantaneous time sequences are compared with a 3D reactive unsteady Reynolds averaged Navier-Stokes (URANS) simulation to more clearly elucidate the in-situ combustion dynamics and the sensitivity to reactant inlet conditions. It is found that the dual-wave system results from unburned reactants that survive the leading detonation wave in the injector near field and are consumed within a trailing azimuthal reflected-shock combustion (ARSC) zone. By contrast, the injector far field is characterized by rapid mixing due to a sudden drop to subsonic conditions, and the bifurcated detonation wave structure collapses into a stronger, single-wave detonation front with higher overall pressure ratio as compared with the dual-wave system. While each RDC will have different inflow, mixing, and combustion characteristics, the underlying interactions between the stratified reactants and azimuthal wave dynamics identified through the combination of advanced MHz-rate diagnostics and 3D numerical simulations have important implications for the study of detonation wave stability, mode transition, and combustion efficiency in non-premixed annular RDCs.

3D URANS↗
DOE OSTI2023

Verification and validation of the open-source plasma fluid code: Zapdos

Zapdos is an open-source finite element plasma fluid solver based on the MOOSE multiphysics framework. This paper outlines Zapdos verification, benchmarking, and validation efforts for 1D and 2D RF capacitively coupled plasma discharge models for mid-range pressures (0.1 - 1 Torr). The verification process involved using the method of manufactured solutions to assess Zapdos spatial and temporal error convergence. L2 errors ranged from 10 -2 to 10 -4 , while the convergence’s slope were in agreement with the predicted slopes for the tested variable and time integration orders. The benchmarking process involved comparisons to previously results from the validated finite element code, LSODI. These works included 1D and 2D simulations for a range of plasma parameters (densities, temperatures, voltage, etc.). For the 1D cases, Zapdos and LSODI results were in very good agreement. In the 2D cases, variable behaviors matched, with slight discrepancies in peak values. The validation process involved comparisons to experimental works including electron density measurements by microwave interferometry and metastable density measurements by planar laser-induced fluorescence imaging. Results shown reasonable agreement at higher pressure, with results starting to diverge at low pressures. Furthermore, probable causes for this diverges are the limitation of the fluid assumption for plasmas at low pressure, or the need for more robust boundary conditions. Overall, Zapdos shown reasonable results for the verification, benchmarking, and validation efforts, and Zapdos can be downloaded at https://github.com/shannon-lab/zapdos.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2020

Liquid-phase turbulence measurements in air-water two-phase flows using particle image velocimetry

Liquid-phase turbulence plays a vital role in determining various gas-liquid two-phase flow parameters, such as void fraction distribution, bubble morphology, bubble-bubble interactions, and interfacial area concentration. In this study, a two-phase flow database including both the gas- and liquid-phases measurements was developed focusing on three bubbly flow conditions in an air-water two-phase flow loop with a vertical one-inch diameter circular pipe test section. A particle image velocimetry (PIV) system integrating an optical phase separation method, i.e., the planar laser-induced fluorescence (PLIF) technique using fluorescent particles and optical filtration, was applied to measure the liquid-phase turbulence information, including the time-averaged velocity, Reynolds stress, and turbulent kinetic energy for the liquid phase. The PIV measurements were taken at three ports along the test section at 14.5, 51.5, and 88.5 pipe inner diameters downstream of a bubble injector. In addition, a double-sensor conductivity probe was used to measure radial distributions of the local time-averaged void fraction and gas velocity. The measured liquid-phase turbulence was used to benchmark Sato's turbulence model considering the bubble-induced shear stress for the three tested bubbly flows. The benchmark results showed good agreement between the PIV measurements and model predictions. Lastly, in the two bubbly flows tested that have low void fractions being less than 3%, the effect of the bubble-induced turbulence was found not significant. However, the bubble-induced shear stress becomes important with the increase of the void fraction.

42 ENGINEERING↗
DOE OSTI2022

The role of cool-flame fluctuations in high-pressure spray flames, studied using high-speed optical diagnostics and Large-Eddy Simulations

Here this work investigates the low- and high-temperature ignition and combustion processes, applied to the Engine Combustion Network Spray A flame, combining advanced optical diagnostics and large-eddy simulations (LES). Simultaneous high-speed (50 kHz) formaldehyde (CH 2 0) planar laser-induced fluorescence (PLIF) and line-of-sight OH* chemiluminescence imaging were used to measure the low- and high-temperature flame, during ignition as well as during quasi-steady combustion. While tracking the cool flame at the laser sheet plane, the present experimental setup allows detection of distinct ignition spots and dynamic fluctuations of the lift-off length over time, which overcomes limitations for flame tracking when using schlieren imaging. After significant development to improve LES prediction of the low-and high-temperature flame position, both during the ignition processes and quasi-steady combustion, the simulations were analyzed to gain understanding of the mixture variance and how this variance affects formation/consumption of CH 2 0. Analysis of the high-temperature ignition period shows that a key improvement in the LES is the ability to predict heterogeneous ignition sites, not only in the head of the jet, but in shear layers at the jet edge close to the position where flame lift-off eventually stabilizes. The LES analysis also shows concentrated pockets of CH 2 0, in the center of jet and at 20 mm downstream of the injector (in regions where the equivalence ratio is greater than 6), that are of similar length scale and frequency as the experiment (approximately 5–6 kHz). The periodic oscillation of CH 2 0 match the frequency of pressure waves generated during auto-ignition and reflected within the constant-volume vessel throughout injection. The ability of LES to capture the periodic appearance and destruction of CH 2 0 is particularly important because these structures travel downstream and become rich premixed flames that affect soot production.

42 ENGINEERING↗
DOE OSTI2023

Simultaneous measurements of kinetic and scalar energy spectrum time evolution in the Richtmyer–Meshkov instability upon reshock

The Richtmyer–Meshkov instability (Richtmyer, Commun. Pure Appl. Maths , vol. 13, issue 2, 1960, pp. 297–319; Meshkov, Fluid Dyn. , vol. 4, issue 5, 1972, pp. 101–104) of a twice-shocked gas interface is studied using both high spatial resolution single-shot (SS) and lower spatial resolution, time-resolved, high-speed (HS) simultaneous planar laser-induced fluorescence and particle image velocimetry in the Wisconsin Shock Tube Laboratory's vertical shock tube. The initial condition (IC) is a shear layer with broadband diffuse perturbations at the interface between a helium–acetone mixture and argon. This IC is accelerated by a shock of nominal strength Mach number $M = 1.75$ , and then accelerated again by the transmitted shock that reflects off the end wall of the tube. An ensemble of experiments is analysed after reshock while the interface mixing width grows linearly with time. The kinetic and scalar energy spectra and the terms of their evolution equation are calculated and compared between SS and HS experiments. The inertial range scaling of the scalar power spectrum is found to follow Gibson's relation (Gibson, Phys. Fluids , vol. 11, issue 11, 1968, pp. 2316–2327) as a function of Schmidt number when the effective turbulent Schmidt number is used in place of the material Schmidt number that controls equilibrium scaling. Further, the spatially integrated scalar flux follows similar behaviour observed for the kinetic energy in large eddy simulation studies by Zeng et al. ( Phys. Fluids , vol. 30, issue 6, 2018, 064106) while the spatially varying scalar flux exhibits back scatter along the centre of the mixing layer and forward energy transfer in the spike and bubble regions.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2021

Implosion dynamics of triple-nozzle gas-puff z pinches on COBRA

Experiments on the 1-MA, 220-ns COBRA generator at Cornell University were conducted to provide detailed measurements of structured cylindrical gas-puff z pinches. In the experiments, a 7 cm diameter triple-nozzle gas valve assembly with concentric outer and inner annular nozzles and a central gas jet initialize the z-pinch load with various working gases, radial density profiles, and externally applied axial magnetic fields. Planar laser-induced fluorescence provides a measure of the initial neutral gas density of the load, while three-frame laser shearing interferometry and multi-frame extreme ultraviolet (XUV) cameras reveal the formation and propagation of a magneto-Rayleigh–Taylor (MRT) unstable shock layer. Implosion trajectories are compared to simple, experimentally informed models and found to be in good agreement. Differences in the structure of the accelerating plasma sheath and evolution of the MRT instability are observed for different gas species and axial magnetic field strengths, correlating with differences in pinch uniformity and x-ray emission. Here, the average instability growth is compared to linear MRT theory predictions using the instantaneous acceleration of the best-fit implosion models and characteristic instability wavelength, with the effective Atwood number and seed perturbation size as fit parameters. For high density argon center jets, ionization prior to the arrival of the imploding plasma sheath suggests a heating mechanism consistent with photoionization by XUV self-emission.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2025

Multimode turbulent flow measurements using magnetic resonance imaging- and laser-based techniques and computational fluid dynamics simulations

We studied the flow field characteristics of a turbulent flow over a regularized cube array with a perpendicular injection flow through the floor between the second and third cubical elements, representing the complex flow interactions of a 3D jet and the wake flows behind cubical obstacles. Four different experimental measurements were performed: two magnetic resonance imaging-based measurements for three-dimensional three-component velocity (MRV) and concentration (MRC) and two laser-based techniques, particle image velocimetry (PIV) and planar laser-induced fluorescence (PLIF), for two-dimensional two-component velocity and concentration measurement, respectively. The mainstream Reynolds number is Re = 15 000⁠, based on the primary inlet velocity U m and channel height D H ⁠, whereas the injector Reynolds number is Re j = 3400⁠, based on the injector velocity U j and the injector's exit width D j ⁠. Numerical simulations were performed for the studied flow configuration of turbulent flow over a regularized cube array using Reynolds-averaged Navier–Stokes (RANS) and large-eddy simulation (LES) approaches. Results obtained from experimental measurements—including MRV, MRC, PIV, and PLIF—as well as RANS and LES simulations are discussed and compared along several horizontal and vertical planes of the studied configuration. In addition, 3D turbulent flow structures, such as leading-edge vortex, horseshoe vortex, and jet shear-layer vortex, and the isosurfaces of scalar concentration successfully revealed by MRV and MRC techniques were found to be in very good agreement with those 3D features extracted from RANS and LES simulations. In conclusion, the high-resolution experimental and numerical database obtained from this study could be useful for validation and verification of numerical codes.

Computational fluid dynamics↗
DOE OSTI2020

Scalar Power Spectra and Scalar Structure Function Evolution in the Richtmyer–Meshkov Instability Upon Reshock

The Richtmyer–Meshkov instability of a twice-shocked gas interface is studied using high-speed planar laser-induced fluorescence in the Wisconsin Shock Tube Laboratory's vertical shock tube. The initial condition is a shear layer with broadband diffuse perturbations at the interface between a helium–acetone mixture and argon. Furthermore, this initial condition is accelerated by a shock of nominal strength M = 1.9, and then accelerated again by the transmitted shock that reflects off the end wall of the tube. Three individual experiments are analyzed, the energy spectrum and the structure functions of the light gas mole fraction field are calculated and compared.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2020

Development of a Comprehensive Two-Phase Flow Database for the Validation of NEK-2P

Three-dimensional (3-D) two-phase Computational Fluid Dynamics (CFD) codes are emerging as a powerful and potentially practical tool for applications in which detailed local flow information is needed. However, two-phase flow models and associated closure relations are not well established for CFD applications, which is partly due to the lack of high-quality validation data. The main objective of this work is to develop a comprehensive database of two-phase flows that can be used to validate two-phase CFD codes such as NEK-2P. In this project, four advanced local measurement systems, including Particle Image Velocimetry and Planar Laser-Induced Fluorescence (PIV-PLIF), high-speed imaging, x-ray densitometry, and multi-sensor conductivity probe are employed to measure the local two-phase flow parameters of both gas and liquid phases. By combining these techniques, the local void fraction, bubble velocity, interfacial area concentration, bubble frequency, liquid velocity, turbulence intensity, etc., in various two-phase flow regimes can be obtained. These local measurement techniques are first used in a 25.4 mm circular pipe test section. Seven air-water two-phase flow conditions spanning the bubbly, slug, churn-turbulent, and annular flow regimes are measured in this facility. The obtained database contains the radial profiles of both gas- and liquid-phase parameters at three axial locations along the test section. The second facility used in this work contains a 30 mm × 10 mm rectangular test section, in which three two-phase flow and two single-phase flow conditions are measured. Two-dimensional distributions of local two-phase flow parameters in the cross-sectional plane are measured in this facility at three axial locations as well. A facility featuring a 3×3 electrically heated rod bundle is also designed and being constructed in this project. This facility is specially designed for optical measurements and is expected to provide high-quality boiling data in the future. Preliminary analyses have been performed for the data taken in the 25.4 mm circular pipe. Both center-peaked and wall-peaked void fraction profiles have been observed in the data depending on the two-phase flow conditions and/or developing lengths. The 1-D drift-flux model was evaluated with the newly obtained datasets, in which both gas- and liquid-phases data were directly measured. The distribution parameter model has been optimized based on a new void-profile classification method proposed in this study. The optimized drift-flux model shows a significant improvement in predicting both gas velocity and void fraction. The measured liquid-phase turbulence was used to benchmark Sato’s turbulence model considering the bubble-induced shear stress for the three tested bubbly flows. The benchmark results showed good agreement between the PIV measurements and model predictions. In the bubbly flows tested that have low void fractions less than 3%, the effect of the bubble-induced turbulence was found not significant. However, the bubble-induced shear stress becomes important with the increase of the void fraction. The Conjugate Heat Transfer (CHT) model was developed and implemented in NEK-2P. This model allows the coupled simulation of the solid domain and two-phase fluid domain, allowing the specification of realistic boundary conditions. The CHT implementation was verified first with non-boiling simulations. The predicted temperatures in the fluid domain were shown to be identical in simulations with or without the CHT model. The CHT model was then validated through simulations of three Becker benchmark CHF tests performed under both Dryout (DO) and Departure from Nucleate Boiling (DNB) conditions. Reasonably good agreement was obtained between calculated wall temperatures and corresponding experimental data.

42 ENGINEERING↗
DOE OSTI2022

High-Speed Diagnostic and Simulation Capabilities for Reacting Hypersonic Reentry Flows (LDRD Final Report)

High-enthalpy hypersonic flight represents an application space of significant concern within the current national-security landscape. The hypersonic environment is characterized by high-speed compressible fluid mechanics and complex reacting flow physics, which may present both thermal and chemical nonequilibrium effects. We report on the results of a three-year LDRD effort, funded by the Engineering Sciences Research Foundation (ESRF) investment area, which has been focused on the development and deployment of new high-speed thermochemical diagnostics capabilities for measurements in the high-enthalpy hypersonic environment posed by Sandia's free-piston shock tunnel. The project has additionally sponsored model development efforts, which have added thermal nonequilibrium modeling capabilities to Sandia codes for subsequent design of many of our shock-tunnel experiments. We have cultivated high-speed, chemically specific, laser-diagnostic approaches that are uniquely co-located with Sandia's high-enthalpy hypersonic test facilities. These tools include picosecond and nanosecond coherent anti-Stokes Raman scattering at 100-kHz rates for time-resolved thermometry, including thermal nonequilibrium conditions, and 100-kHz planar laser-induced fluorescence of nitric oxide for chemically specific imaging and velocimetry. Key results from this LDRD project have been documented in a number of journal submissions and conference proceedings, which are cited here. The body of this report is, therefore, concise and summarizes the key results of the project. The reader is directed toward these reference materials and appendices for more detailed discussions of the project results and findings.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2024

Flashback Measurements in Hydrogen Enriched Low Swirl Flames Using High Speed OH-PLIF

The fundamentals of stabilized flame dynamics and flashback events in a premixed low swirl burner (LSB) configuration are visualized experimentally using nanosecond (ns)-based high-speed hydroxyl radical planar laser-induced fluorescence (OH-PLIF). Swirlers with two different turning angles, 〖26〗^o and 〖33〗^o and three different center-body hole diameters, 1.08, 1.12 and 1.16 mm with measured swirl numbers varying from 0.43 to 0.49 are tested in this study at atmospheric temperature and pressure inlet conditions. An increase in flashback propensity is observed with increasing ϕ, X_(H_2 ) and decreasing V via detailed investigation of flame lift-off length (L) above the burner rim. Flashback ϕ (ϕ_FB) investigations show an expected linearly increasing trend with decreasing X_(H_2 ) and increasing V for each swirler studied and the results agree well with detailed L investigations in a stable flame configuration. ϕ_FB studies for different swirlers show an increase in flashback resistance with the increase in center-body hole diameter and swirl angle. Spatiotemporally resolved kHz-rate OH-PLIF is a promising technique to observe rapidly occurring flashback events and it can be applied for turbulence-chemistry interaction model validation.

Parajuli, Pradeep↗
DOE OSTI2021

Hybrid Large Eddy Simulation/Reynolds-Averaged Navier–Stokes Analysis of a Premixed Ethylene-Fueled Dual-Mode Scramjet Combustor

Hydrocarbon fuels offer optimal high energy per volume for scramjet applications for sustained hypersonic flight but require additional residence time due to slower ignition delays (compared with hydrogen fuel). The injection of ethylene at the start of the isolator of a dual-mode scramjet combustor, operating in ramjet mode, allows sufficient mixing to achieve efficient premixed turbulent combustion. A cavity flameholder anchors the flame, supplying sufficient radicals to sustain a stable flame in the high-speed environment. This work investigates flame structure and stabilization limits of a new configuration with a scaled-down cavity embedded in the flow path of the combustor with a strut and insert. The cavity is reduced in size by one-third to enable eventual direct numerical simulations of the flame stabilization process. This work, however, focuses on modeling the full isolator/combustor geometry using a hybrid large eddy simulation/Reynolds-averaged Navier–Stokes simulation strategy. Additionally, particle image velocimetry, planar laser-induced fluorescence, coherent anti-Stokes Raman spectroscopy, and pressure measurements are compared with numerical predictions to analyze and characterize the conditions within the combustor, including flame structure, flow velocities, species composition, and wall pressure. An adjustable air throttle in the extender is able to control the placement of the shock train in the isolator and maintain a stable flame at various equivalence ratios. The simulations show reasonably good agreement with the experimental scalar and velocity data and predict a flame angle consistent with premixed turbulent flame-speed correlations.

42 ENGINEERING↗
DOE OSTI2025

100 kHz OH PLIF of High-Pressure H2/NH3 and H2/CH4 Flames

The reaction zones in a multi-element, multi-stage, micromix injector are investigated using planar laser-induced fluorescence (PLIF) imaging of the hydroxyl (OH) radical at a 100 kHz repetition rate. The combustor is operated at a pressure of ∼10 bar. Multiple fuel blends of hydrogen, methane, and ammonia are considered to study the effect of changing fuel composition on the flame structure. Compact regions of high OH signal are observed in each flame for fuel mixtures with high hydrogen content, indicating rapid reactant consumption in the shear layers. Instantaneous images exhibit wrinkled flame fronts and the formation of unreacted pockets due to highly turbulent burning. The addition of methane is observed to reduce the reactivity and flame speed, resulting in more diffuse regions of OH between each flame. The shape of the reactant core is altered, and the length scale of the flame surface wrinkling is increased. Ammonia addition has a more severe effect on the distribution of OH and the local flame structure than methane addition. A time series of images shows the presence of OH vortical structures and significant turbulent fluctuations in the flames near the wall, suggesting the presence of a recirculation zone that could drive the observed disparity in flame lengths.

Hodge, Alexander J. [Purdue University]↗