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At least 127 records · Page 7
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NASA NTRS1995

Pinatubo Aerosol Global-to-Micro-Scale Evolution: A Unified Picture From Space, Air, and Ground Measurements

We combine a variety of measurements to develop a composite picture of the post-Pinatubo aerosol and assess the consistency and uncertainties of the measurement and retrieval techniques Satellite infrared spectroscopy, particle morphology, and evaporation temperature measurements are in accord with theoretical calculations In showing a dominant particle composition of H2SO4-H2O mature with H2SO4 weight traction of 65-80% for most stratospheric temperatures and humidities. Important exceptions are: (1) the presence of volcanic ash at all attitudes initially and in a layer just above the tropopause until at least March 1992, and (2) much smaller H2SO4 weight fractions at the low temperatures attained In high latitude winters and at the tropical tropopause. Laboratory spectroscopy and theoretical calculations yield wavelength- and temperature-dependent refractive indices for the dominant H2SO4-H2O droplets. These in turn permit derivation of particle size spectra from measured optical depth spectra for comparison to direct measurements by impactors and optical counters, All three techniques paint a generally consistent picture of the evolution of R(sub eff) the effective, or area-weighted, particle radius. In the first month after the eruption, although particle numbers increased by orders of magnitude, R(sub eff) was similar to the pre-eruption value of 0.1 to 0.2 microns because both small (r less than 0.2 microns) and large (r greater than 0.6 microns) particles increased in number. Over the next 3-6 months, R(sub eff) increased to about 0.5 microns, reflecting particle growth through condensation and coagulation. In general, R(sub eff) continued to increase for about a year after the eruption. Extinction spectra computed from in situ size distribution measurements are consistent with optical depth measurements, which show spectra with maxima initially at wavelengths of 0.42 microns or less, and thereafter progressively increasing to between 0.78 and 1 micron. Not until 1993 does optical depth spectra begin to show a clear return to the preeruption signature of maximizing at the shortest visible wavelengths or in the near UV. This coupled evolution in particle size distribution and optical depth spectra helps explain the relationship between the global maps of 0.5- and 1.0-kilometer optical depth derived from the AVHRR and SAGE satellite measurements. It also sets a context for evaluating remaining uncertainties in each of these satellite data products. We also show how the effects of wavelength-dependent refractive index on backscatter spectra can influence particle sizes retrieved from multiwavelength lidar measurements.

Russell, Philip B.↗
NASA NTRS1995

A Unified Picture of Pinatubo Aerosol Global-to Micro-Scale Evolution, From Space, Air, and Ground Measurements

We combine a variety of measurements to develop a composite picture of the post-Pinatubo aerosol and assess the consistency and uncertainties of the measurement and retrieval techniques. Satellite infrared spectroscopy, particle morphology, and evaporation temperature measurements are in accord with theoretical calculations in showing a dominant particle composition of H2SO4-H2O mixture, with H2SO4 weight fraction of 65-80% for most stratospheric temperatures and humidities. Important exceptions are: (1) the presence of volcanic ash at all altitudes initially and in a layer just above the tropopause until at least March 1992, and (2) much smaller H2SO4 weight fractions at the low temperatures attained in high latitude winters and at the tropical tropopause, Laboratory spectroscopy and theoretical calculations yield wavelength- and temperature-dependent refractive indices for the dominant H2SO4-H2O droplets. These in turn permit derivation of particle size spectra from measured optical depth spectra, for comparison to direct measurements by impactors and optical counters. All three techniques paint a generally consistent picture of the evolution of R(sub eff), the effective, or area-weighted, particle radius. In the first month after the eruption, although particle numbers increased by orders of magnitude, R(sub eff) was similar to the preemption value of 0.1 to 0.2 microns, because both small (r less than 0.2 microns) and large (r greater than 0.6 micron particles increased in number. Over the next 3-6 months, R(sub eff) increased to about 0.5 microns reflecting particle growth through condensation and coagulation. In general, R(sub eff) continued to increase for about a year after the eruption. Extinction spectra computed from in situ size distribution measurements are consistent with optical depth measurements, which show spectra with maxima initially at wavelengths of 0.42 microns or less, and thereafter progressively increasing to between 0.78 and 1 micron. Not until 1993 do optical depth spectra begin to show a clear return to the preemption signature of maximizing at the shortest visible wavelengths or in the near UV. This coupled evolution in particle size distribution and optical depth spectra helps explain the relationship between the global maps of 0.5- 1.0- micron optical depth derived from the AVHRR and SAGE satellite measurements.

Russell, Philip B.↗
NASA NTRS2012

Dispersion of the Volcanic Sulfate Cloud from the Mount Pinatubo Eruption

We simulate the transport of the volcanic cloud from the 1991 eruption of Mount Pinatubo with the GEOS-5 general circulation model. Our simulations are in good agreement with observational data. We tested the importance of initial condition corresponding to the specific meteorological situation at the time of the eruption by employing reanalysis from MERRA. We found no significant difference in the transport of the cloud. We show how the inclusion of the interaction between volcanic sulfate aerosol and radiation is essential for a reliable simulation of the transport of the volcanic cloud. The absorption of long wave radiation by the volcanic sulfate induces a rising of the volcanic cloud up to the middle stratosphere, combined with divergent motion from the latitude of the eruption to the tropics. Our simulations indicate that the cloud diffuses to the northern hemisphere through a lower stratospheric pathway, and to mid- and high latitudes of the southern hemisphere through a middle stratospheric pathway, centered at about 30 hPa. The direction of the middle stratospheric pathway depends on the season. We did not detect any significant change of the mixing between tropics and mid- and high latitudes in the southern hemisphere.

Aquila, Valentina↗
NASA NTRS2012

The Chemical and Dynamical Responses of Ozone and Nitrogen Dioxide to the Eruption of Mt. Pinatubo

Observations have shown that the concentration of nitrogen dioxide decreased in both hemispheres in the years following the eruption of Mt. Pinatubo. In contrast, the observed ozone response was largely asymmetrical with respect to the equator, with a decrease in the northern hemisphere and little or no change in the southern hemisphere. Simulations including enhanced heterogeneous chemistry due to the presence of the volcanic aerosol reproduce a decrease of ozone in the northern hemisphere, but also produce a comparable ozone decrease in the southern hemisphere contrary to observations. Our simulations show that the heating due to the volcanic aerosol enhanced both the tropical upwelling and the extratropical downwelling. The enhanced extratropical downwelling, combined with the time of the eruption relative to the seasonal phase of the Brewer-Dobson circulation, increased the ozone in the southern hemisphere and counteracted the ozone depletion due to heterogeneous chemistry on volcanic aerosol.

Aquila, V.↗
NASA NTRS2012

The Response of Ozone and Nitrogen Dioxide to the Eruption of Mount Pinatubo

Observations have shown that the global mass of nitrogen dioxide decreased in both hemispheres in the year following the eruption of Mt. Pinatubo, indicating an enhanced heterogeneous chemistry. In contrast, the observed ozone response was largely asymmetrical with respect to the equator, with a decrease in the northern hemisphere and little change in the southern hemisphere. Simulations including enhanced heterogeneous chemistry due to the presence of the volcanic aerosol reproduce a decrease of ozone in the northern hemisphere, but also produce a comparable ozone decrease in the southern hemisphere, contrary to observations. Our simulations show that the heating due to the volcanic aerosol enhanced both the tropical upwelling and the extratropical downwelling. The enhanced extratropical downwelling, combined with the time of the eruption relative to the phase of the Brewer-Dobson circulation, increased the ozone in the southern hemisphere and counteracted the ozone depletion due to heterogeneous chemistry on volcanic aerosol.

Aquila. Valentina↗
NASA NTRS2012

The Response of Ozone and Nitrogen Dioxide to the Eruption of Mt. Pinatubo

Observations have shown that the global mass of nitrogen dioxide decreased in both hemispheres in the year following the eruption of Mt. Pinatubo. In contrast, the observed ozone response was largely asymmetrical with respect to the equator, with a decrease in the northern hemisphere and little change and even a small increase in the southern hemisphere. Simulations including enhanced heterogeneous chemistry due to the presence of the volcanic aerosol reproduce a decrease of ozone in the northern hemisphere, but also produce a comparable ozone decrease in the southern hemisphere, contrary to observations. Our simulations show that the heating due to the volcanic aerosol enhanced both the tropical upwelling and the extratropical downwelling. The enhanced extratropical downwelling, combined with the time of the eruption relative to the phase of the Brewer-Dobson circulation, increased the ozone in the southern hemisphere and counteracted the ozone depletion due to heterogeneous chemistry on volcanic aerosol.

Aquila, Valentina↗
NASA NTRSDate not supplied

Calculating the Height of Volcanic Cloud SO2 With a Lagrangian Trajectory Tool: Raikoke (2019) and Pinatubo (1991) Cases

We have developed a new data analysis tool to reconstruct the altitude of SO2 clouds ejected by avolcanic eruption. Starting with 2D fields of satellite observed SO2 column density, known volcanolocation, and reanalysis wind fields, the Goddard Lagrangian trajectory tool allows us to estimatethe altitude and local concentration of SO2 at the time of observation. We demonstrate this tool forthe June 21, 2019 Mt. Raikoke eruption (8h, 30h and 78 hours after eruption). We use SO2 data fromthe Ozone Mapping and Profiler Suite/Nadir Mapper (OMPS/NM) onboard the NASA-NOAASuomi National Polar Partnership satellite and the Tropospheric Monitoring Instrument(TROPOMI) onboard the European Copernicus Sentinel 5 precursor satellite and wind fields fromthe NASA Goddard Earth Observing System (GEOS) model. We obtained a wide distribution ofSO2 altitudes between 1 and 19 kilometers in different parts of the Raikoke SO2 clouds, with thehighest SO2 concentration between 11 and 16 km, in good agreement with data from independentSO2 layer height retrievals from TROPOMI and Infrared Atmospheric Sounding Interferometer(IASI). We then applied this method to the June 15, 1991 Mt. Pinatubo eruption using SO2 columnmeasurements from the NASA Total Ozone Mapping Spectrometer (TOMS) on June 16, 17, 18 andusing wind fields from the National Centers for Environmental Prediction Reanalysis version 2. Weobtained a wide distribution of SO2 heights from 6 km up to 30 km in the northern part of the cloud.We use our new trajectory tool to reconstruct volcanic SO2/aerosol emission sources as functions oftime and altitude, providing inputs to the GEOS model aerosol and chemistry schemes in order tosimulate the dispersion of volcanic SO2 and aerosol clouds from these events.

SO2↗
NASA NTRS2023

The Impact of ENSO and NAO Initial Conditions and Anomalies on the Modeled Response to Pinatubo-Sized Volcanic Forcing

Strong, strato-volcanic eruptions are a substantial, intermittent source of natural climate variability. Initial atmospheric and oceanic conditions, such as El Niño Southern Oscillation (ENSO) and the North Atlantic Oscillation (NAO), also naturally impact climate on interannual timescales. We examine how initial conditions of ENSO and NAO contribute to the evolution of climate in the period following a Pinatubo-type eruption using a large (81-member) ensemble of model simulations in GISS model E2.1-G. Simulations are initialized from sampled conditions of ENSO and NAO using the protocol of the coordinated CMIP6 Volcanic Model Intercomparison Project (VolMIP) – where aerosols are forced with respect to time, latitude, and height. We analyze paired anomalous variations (perturbed – control) to understand changes in global and regional climate responses under positive, negative, and neutral ENSO and NAO conditions. In particular, we find that for paired anomalies there is a high probability of strong (∼1.5 °C) warming of northern Eurasia surface air temperature in the first winter after the volcanic eruption for negative NAO ensembles coincident with decreased lower stratospheric temperature at the poles, decreased geopotential height, and strengthening of the stratospheric polar vortex. Climate anomalies (relative to average conditions across the control period), however, show no mean warming and suggest that the strength of this response is impacted by conditions present in the selected period of the control run. Again using paired anomalies, we also observe that under both +ENSO and −ENSO ensembles sea surface temperature decreases in the first post-eruptive boreal winter coinciding with surface cooling from volcanic aerosols. Neutral ENSO ensembles, on the other hand, show variability in their response with no clear trend in post-eruptive warming or cooling. In general, paired anomalies from unperturbed simulations give insight into the evolution of the climate response to volcanic forcing; however, when compared with anomalies from climatological conditions, it is clear that paired anomalies are significantly affected by sampled initial conditions occurring at the time of the volcanic eruption.

volcanic eruptions↗
NASA NTRS1992

Stratospheric Backscatter, Extinction, and Lidar Ratio Profiling After the Mt. Pinatubo Eruptions

Since August 1991 the stratospheric aerosol layer is continuously monitored with a combination Raman elastic-backscatter lidar, groundbased systems. XeCl excimer laser is used as the radiation source. Signals elastically backscattered from air molecules and particles and inelastically Raman backscattered from nitrogen molecules are detected. The measurements of these two signal profiles up to 35 km height allows the separate and independent determination of aerosol extinction and backscatter properties in the perturbed lower stratosphere. The extinction coefficient is derived from the nitrogen Raman signal profile, while the backscatter coefficient is obtained from the elastic-to-inelastic backscatter signal ratio. In this way, also the extinction-to-backscatter, or lidar, ratio profile is determined. For the first time, lidar ratios are determined in the perturbed stratospheric layer by the use of remote sensing only. The lidar ratio contains information about the size range of the stratospheric particles which are assumed to be sulfuric acid droplets, and it is needed in the calculation of aerosol optical properties from data taken with a typical backscatter lidar.

Ansmann, Albert↗
NASA NTRS1992

Initial assessment of the stratospheric and climatic impact of the 1991 Mount Pinatubo eruption - Prologue

An overview is given of the techniques employed to evaluate the early effects of the volcanic eruption on the stratosphere and climate, and data are given on the initial eruption yield. Global satellite measurements were taken by TOMS, SAGE II, AVHRR, and other devices, and the initial results indicate an eruption yield of 20 megatons of SO2 and 20-30 megatons of H2SO4/H2O aerosol mass. The predicted effects of the eruption - accelerated global ozone depletion and surface cooling - can be compared to meteorological data to test the validity of present climate models based on these data.

Mccormick, M. P.↗