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At least 127 records · Page 7

Aerosol Impacts on California Winter Clouds and Precipitation during CalWater 2011: Local Pollution versus Long-Range Transported Dust

Mineral dust aerosols often observed over California in winter and spring, associated with long-range transport from Asia and Sahara, have been linked to enhanced precipitation based on observations. Local anthropogenic pollution, on the other hand, was shown in previous observational and modeling studies to reduce precipitation. Here we incorporate recent developments in ice nucleation parameterizations to link aerosols with ice crystal formation in a spectral-bin cloud microphysical model coupled with the Weather Research and Forecasting (WRF) model, to examine the relative and combined impacts of dust and local pollution particles on cloud properties and precipitation type and intensity. Simulations are carried out for two cloud cases with contrasting meteorology and cloud dynamics that occurred on February 16 (FEB16) and March 02 (MAR02) from the CalWater 2011 field campaign. In both cases, observations show the presence of dust and biological particles in a relative pristine environment. The simulated cloud microphysical properties and precipitation show reasonable agreement with aircraft and surface measurements. Model sensitivity experiments indicate that in the pristine environment, the dust and biological aerosol layers increase the accumulated precipitation by 10-20% from the Central Valley to the Sierra Nevada Mountains for both FEB16 and MAR02 due to a ~40% increase in snow formation, validating the observational hypothesis. Model results show that local pollution increases precipitation over the windward slope of the mountains by few percent due to increased snow formation when dust is present but reduces precipitation by 5-8% if dust is removed on FEB16. The effects of local pollution on cloud microphysics and precipitation strongly depend on meteorology including the strength of the Sierra Barrier Jet, and cloud dynamics. This study further underscores the importance of the interactions between local pollution, dust, and environmental conditions for assessing aerosol effects on cold season precipitation in California.

aerosol impacts↗

Antarctic-Wide Array of High-Resolution Ice Core Records Reveals Pervasive Lead Pollution Began in 1889 and Persists Today

Interior Antarctica is among the most remote places on Earth and was thought to be beyond the reach of human impacts when Amundsen and Scott raced to the South Pole in 1911. Here we show detailed measurements from an extensive array of 16 ice cores quantifying substantial toxic heavy metal lead pollution at South Pole and throughout Antarctica by 1889 - beating polar explorers by more than 22 years. Unlike the Arctic where lead pollution peaked in the 1970s, lead pollution in Antarctica was as high in the early 20th century as at any time since industrialization. The similar timing and magnitude of changes in lead deposition across Antarctica, as well as the characteristic isotopic signature of Broken Hill lead found throughout the continent, suggest that this single emission source in southern Australia was responsible for the introduction of lead pollution into Antarctica at the end of the 19th century and remains a significant source today. An estimated 660 t of industrial lead have been deposited over Antarctica during the past 130 years as a result of mid-latitude industrial emissions, with regional-to-global scale circulation likely modulating aerosol concentrations. Despite abatement efforts, significant lead pollution in Antarctica persists into the 21st century.

pollution↗

The Net Decay Time of Anomalies in Concentrations of Atmospheric Pollutants

This paper introduces a new parameter to characterize the random component in temporal variability of atmospheric pollutants and proposes a simple statistical technique for its evaluation. That parameter is the net decay time (or the time scale) of the local anomalies in concentrations of atmospheric pollutants, rather than the traditionally used chemical lifetimes of total amounts of the species. Using widely available data of hourly multi-year surface trace gas pollutant concentrations we demonstrate a simplified way to estimate the net decay time with an exponential approximation of lag-correlation functions. We assessed the decay times of fluctuations in observations of eight atmospheric pollutants (SO2, NO, NO2, NOy, O3, CO, NH3, and HNO3) at two urban sites and one cleaner rural site in the Eastern US. The time scales of temporal fluctuations (net decay times) vary from about one hour to slightly more than one day. These scales are generally much shorter in urban environments than in remote regions. We also compared day- and night-time observations in warm and cold seasons. At night in the cold season, time scales of fluctuations in atmospheric pollutants are usually the longest. Such estimates should be useful to air quality prediction, public health, and satellite remote sensing research communities.

air quality prediction↗

Influence of Cloud, Fog, and High Relative Humidity during Pollution Transport Events in South Korea: Aerosol Properties and PM2.5 Variability

This investigation examines aerosol dynamics during major fine mode aerosol transboundary pollution events in South Korea primarily during the KORUS-AQ campaign from May 1 – June 10, 2016, particularly when cloud fraction was high and/or fog was present to quantify the change in aerosol characteristics due to near-cloud or fog interaction. We analyze the new AERONET Version 3 data that have significant changes to cloud screening algorithms, allowing many more fine-mode observations in the near vicinity of clouds or fog. Case studies for detailed investigation include May 25–26, 2016 when cloud fraction was high over much of the peninsula, associated with a weak frontal passage and advection of pollution from China. These cloud-influenced Chinese transport dates also had the highest aerosol optical depth (AOD), surface PM2.5 concentrations and fine mode particle sizes of the entire campaign. Another likewise cloud/high relative humidity (RH) case is June 9 and 10, 2016 when fog was present over the Yellow Sea that appears to have affected aerosol properties well downwind over the Korean peninsula. In comparison we also investigated aerosol properties on air stagnation days with very low cloud cover and relatively low RH (May 17 & 18, 2016), when local Korean emissions dominated. Aerosol volume size distributions show marked differences between the transport days (with high RH and cloud influences) and the local pollution stagnation days, with total column-integrated particle fine mode volume being an order of magnitude greater on the pollution transport dates. The PM2.5 over central Seoul were significantly greater than for coastal sites on the transboundary transport days yet not on stagnation days, suggesting addi-tional particle formation from gaseous urban emissions in cloud/fog droplets and/or in the high RH humidified aerosol environment. Many days had KORUS-AQ research aircraft flights that provided observations of aerosol absorption, particle chemistry and vertical profiles of extinction. AERONET retrievals and aircraft in situ mea-surements both showed high single scattering albedo (weak absorption) on the cloudy or cloud influenced days, plus aircraft profile in situ measurements showed large AOD enhancements (versus dried aerosol) at ambient relative humidity (RH) on the pollution transport days, consistent with the significantly larger fine mode particle radii and weak absorption.

Aerosol↗

Spatiotemporal interpolation of air pollutants in the Greater Cairo and the Delta, Egypt

Highlights: • Data from network of monitoring stations in Egypt are used for studying SO{sub 2}, NO{sub 2}, and PM{sub 10.} • Trans-Gaussian Spatiotemporal kriging is used as a spatiotemporal interpolation method. • The whole area under study is suffering from high values of PM{sub 10} throughout 2015. • For NO{sub 2} and SO{sub 2}, the highest value is noticed in February. • Concerns must be given to the monitoring network to improve the prediction precision. This paper analyses the spatiotemporal variability of air pollutants in Egypt using monthly averages from the air quality monitoring network from 2011 to 2015. Particulate Matters (PM{sub 10}) Nitrogen Dioxide (NO{sub 2}) and Sulfur Dioxide (SO{sub 2}), measured by the monitoring stations network are studied. A log transformation is applied for the three pollutants to achieve normality. The sum-metric function is utilized for modelling the spatiotemporal variogram as it gave the smallest Mean Squared Error (MSE) compared to other forms namely separable, metric, and product sum models. Therefore, employing the gstat package in R together with the trans-Gaussian spatiotemporal kriging, the maps are generated for the interpolated surfaces for the monthly averages of 2015 and the corresponding standard error values. These maps will help the decision maker to understand and visualize the spatial and temporal variability of the measured pollutants and hence undertake the necessary policies and decisions. The results show that the down town area has the highest pollutants levels. As concerns the temporal dimension, the highest values are depicted during the month of February as compared to the rest of the year. Furthermore, Egypt is suffering from a serious PM{sub 10} problem for the area and period under study that extremely exceed the WHO and Egyptian guidelines.

54 ENVIRONMENTAL SCIENCES↗

Effect of oxidation on the release of multiple metals from industrially polluted sediments and synchrotron-based evidence of Cu–S dynamic association

Disposal operations for industrially polluted sediments are usually accompanied by disturbance and resuspension, which can induce metal remobilization and secondary pollution. Evaluating the risk of metal release under various redox conditions is fundamental for predicting contaminant mobilization and guiding remediation measures. An abandoned oxidation pond, Yanjia Lake, China, was selected as a typical industrially polluted site. Re-suspension experiments were carried out by mixing polluted sediments with lake water under oxic or anoxic conditions, then investigating the effect of oxidation conditions on the release of multiple metals. Metal concentrations and aqueous chemistry in the overlying water were monitored. Synchrotron-based methods, including X-ray absorption near-edge structure (XANES) and extended X-ray absorption fine structure (EXAFS), were used to characterize oxidation states and coordination conditions of metals in sediments. The release of metals, including Cr, Co, Ni, Cu, Zn, Se, Mo, Sn, Cd, and Pb, was enhanced under oxic vs. anoxic conditions. The XANES analysis revealed that elevated Cr and Zn concentrations under oxic conditions likely resulted from the oxidation of Cr(III) and oxidizing dissolution of ZnS, respectively. K-edge Cu XANES, S XANES, and Cu EXAFS analyses reconstructed the Cu–S association, indicating that S-related oxidation promoted Cu release and Cu–O partly replaced Cu–S in the sediment after a 7-day oxic treatment. The release of most metals was promoted under oxic conditions, resulting from the oxidation of sulfides and metals as indicated by aqueous and synchrotron-based evidence. The risk of secondary pollution is greatly enhanced under oxic conditions, which suggests that measures should be taken to minimize the redox disturbance during sediment remediation. This information can guide the management of sediments in Yanjia Lake and other contaminated sites with similar properties.

54 ENVIRONMENTAL SCIENCES↗

Persistent high PM 2.5 pollution driven by unfavorable meteorological conditions during the COVID-19 lockdown period in the Beijing-Tianjin-Hebei region, China

Lockdown measures to curtail the COVID-19 pandemic in China halted most nonessential activities on January 23, 2020. Despite significant reductions in anthropogenic emissions, the Beijing-Tianjin-Hebei (BTH) region still experienced high air pollution concentrations. In this work, employing two emissions reduction scenarios, the Community Multiscale Air Quality (CMAQ) model was used to investigate the PM 2.5 concentrations change in this region. The model using the scenario (C3) with greater traffic reductions performed better compared to the observed PM 2.5 . Compared with the no reductions base-case (scenario C1), PM 2.5 reductions with scenario C3 were 2.70, 2.53, 2.90, 2.98, 3.30, 2.81, 2.82, 2.98, 2.68, and 2.83 µg/m 3 in Beijing, Tianjin, Shijiazhuang, Baoding, Cangzhou, Chengde, Handan, Hengshui, Tangshan, and Xingtai, respectively. During high-pollution days in scenario C3, the percentage reductions in PM 2.5 concentrations in Beijing, Tianjin, Shijiazhuang, Baoding, Cangzhou, Chengde, Handan, Hengshui, Tangshan, and Xingtai were 3.76, 3.54, 3.28, 3.22, 3.57, 3.56, 3.47, 6.10, 3.61, and 3.67%, respectively. However, significant increases caused by unfavorable meteorological conditions counteracted the emissions reduction effects resulting in high air pollution in BTH region during the lockdown period. This study shows that effective air pollution control strategies incorporating these results are urgently required in BTH to avoid severe pollution.

54 ENVIRONMENTAL SCIENCES↗

Fine-scale damage estimates of particulate matter air pollution reveal opportunities for location-specific mitigation of emissions

Fine particulate matter (PM 2.5 ) air pollution has been recognized as a major source of mortality in the United States for at least 25 years, yet much remains unknown about which sources are the most harmful, let alone how best to target policies to mitigate them. Such efforts can be improved by employing high-resolution geographically explicit methods for quantifying human health impacts of emissions of PM 2.5 and its precursors. Here, we provide a detailed examination of the health and economic impacts of PM 2.5 pollution in the United States by linking emission sources with resulting pollution concentrations. We estimate that anthropogenic PM 2.5 was responsible for 107,000 premature deaths in 2011, at a cost to society of $886 billion. Of these deaths, 57% were associated with pollution caused by energy consumption [e.g., transportation (28%) and electricity generation (14%)]; another 15% with pollution caused by agricultural activities. A small fraction of emissions, concentrated in or near densely populated areas, plays an outsized role in damaging human health with the most damaging 10% of total emissions accounting for 40% of total damages. We find that 33% of damages occur within 8 km of emission sources, but 25% occur more than 256 km away, emphasizing the importance of tracking both local and long-range impacts. Our paper highlights the importance of a fine-scale approach as marginal damages can vary by over an order of magnitude within a single county. Information presented here can assist mitigation efforts by identifying those sources with the greatest health effects.

54 ENVIRONMENTAL SCIENCES↗

The evolution of carbon-polluted white dwarfs at low effective temperatures

Taking advantage of the Gaia Data Release 2, recent studies have revisited the evolution of carbon-polluted white dwarfs (DQs) across a large range of effective temperatures. These analyses have clearly confirmed the existence of two distinct DQ evolutionary sequences: one with normal-mass white dwarfs and one with heavily polluted and generally more massive objects. The first sequence is thought to result from the dredge-up of carbon from the core, while the second could at least partially be made of descendants of hot DQs. However, the evolution of carbon-polluted white dwarfs below 6500 K remains unexplored, mainly due to the theoretical difficulties associated with modelling their dense atmospheres. In this work, we present a detailed star-by-star analysis of cool carbon-polluted white dwarfs. Our recently improved atmosphere models allow us to obtain good fits to most objects, including very cool DQpec white dwarfs with strongly shifted C2 molecular bands. We show herein that cool carbon-polluted white dwarfs keep following the two distinct evolutionary tracks previously identified at higher temperatures. We also find that most DQ white dwarfs transform into DQpec when their photospheric densities exceed ${\approx}0.15\, {\textrm{g\,cm}}^{-3}$. However, we identify stars for which the DQ→DQpec transition occurs at lower photospheric densities, possibly due to the presence of a strong magnetic field.

79 ASTRONOMY AND ASTROPHYSICS↗

Linking atmospheric pollution to cryospheric change in the Third Pole region: current progress and future prospects

ABSTRACT The Tibetan Plateau and its surroundings are known as the Third Pole (TP). This region is noted for its high rates of glacier melt and the associated hydrological shifts that affect water supplies in Asia. Atmospheric pollutants contribute to climatic and cryospheric changes through their effects on solar radiation and the albedos of snow and ice surfaces; moreover, the behavior and fates within the cryosphere and environmental impacts of environmental pollutants are topics of increasing concern. In this review, we introduce a coordinated monitoring and research framework and network to link atmospheric pollution and cryospheric changes (APCC) within the TP region. We then provide an up-to-date summary of progress and achievements related to the APCC research framework, including aspects of atmospheric pollution's composition and concentration, spatial and temporal variations, trans-boundary transport pathways and mechanisms, and effects on the warming of atmosphere and changing in Indian monsoon, as well as melting of glacier and snow cover. We highlight that exogenous air pollutants can enter into the TP’s environments and cause great impacts on regional climatic and environmental changes. At last, we propose future research priorities and map out an extended program at the global scale. The ongoing monitoring activities and research facilitate comprehensive studies of atmosphere–cryosphere interactions, represent one of China's key research expeditions to the TP and the polar regions and contribute to the global perspective of earth system science.

54 ENVIRONMENTAL SCIENCES↗

Storm Water Pollution Prevention Plan Middle DP Road Recovery Effort, June 26, 2020

The United States Environmental Protection Agency (EPA) has issued a final 2017 Construction General Permit (CGP) that covers discharges of stormwater from construction sites. The 2017 National Pollutant Discharge Elimination System (NPDES) General Permit for Storm Water Discharges from Construction Activity (Appendix D) includes the following requirements:(1) conduct a critical habitat and threatened/endangered species study; (2) develop and implement a Storm Water Pollution Prevention Plan (SWPPP) in accordance with good engineering practices; (3) submit a Notice of Intent (NOI); (4) install and maintain erosion and stormwater controls; (5) perform and document storm water inspections during construction and site stabilization; (6) amend the SWPPP as necessary; and (7) submit a Notice of Termination (NOT) following project completion and final stabilization of disturbed areas. Authorization to discharge storm water is required under this Permit for both large and small construction projects disturbing more than one (1) acre or part of a larger common plan of development that collectively disturbs more than one (1) acre. All parties that meet the definition of Operator must be permitted. Each permittee is not required to develop and implement a separate SWPP Plan. It is required that there be at least one SWPP Plan for a site that incorporates the required elements for all Operators. The 2017 CGP number for New Mexico (Region 6) is NMR100000. This Plan, which has been developed for Triad National Security, LLC (Triad), describes the nature and sequencing of construction activities, potential sources of pollution, and identifies the Best Management Practices (BMPs) to minimize the potential for erosion and storm water pollution. The Plan was developed in accordance with the provisions of the Clean Water Act (33 U.S.C. § §1251 et seq., as amended by the Water Quality Act of 1987, P.L. 100-4), and the regulations established by the U.S. Environmental Protection Agency (EPA) for National Pollutant Discharge Elimination System (NPDES) General Permits for Storm Water Discharges From Construction Activities.

54 ENVIRONMENTAL SCIENCES↗

Storm Water Pollution Prevention Plan Middle DP Road Recovery Effort, June 26, 2020 (Copy for Informational Puproses Only)

The United States Environmental Protection Agency (EPA) has issued a final 2017 Construction General Permit (CGP) that covers discharges of stormwater from construction sites. The 2017 National Pollutant Discharge Elimination System (NPDES) General Permit for Storm Water Discharges from Construction Activity (Appendix D) includes the following requirements: (1) conduct a critical habitat and threatened/endangered species study; (2) develop and implement a Storm Water Pollution Prevention Plan (SWPPP) in accordance with good engineering practices; (3) submit a Notice of Intent (NOI); (4) install and maintain erosion and stormwater controls; (5) perform and document storm water inspections during construction and site stabilization; (6) amend the SWPPP as necessary; and (7) submit a Notice of Termination (NOT) following project completion and final stabilization of disturbed areas. Authorization to discharge storm water is required under this Permit for both large and small construction projects disturbing more than one (1) acre or part of a larger common plan of development that collectively disturbs more than one (1) acre. All parties that meet the definition of Operator must be permitted. Each permittee is not required to develop and implement a separate SWPP Plan. It is required that there be at least one SWPP Plan for a site that incorporates the required elements for all Operators. The 2017 CGP number for New Mexico (Region 6) is NMR100000. This Plan, which has been developed for Triad National Security, LLC (Triad), describes the nature and sequencing of construction activities, potential sources of pollution, and identifies the Best Management Practices (BMPs) to minimize the potential for erosion and storm water pollution. The Plan was developed in accordance with the provisions of the Clean Water Act (33 U.S.C. § §1251 et seq., as amended by the Water Quality Act of 1987, P.L. 100-4), and the regulations established by the U.S. Environmental Protection Agency (EPA) for National Pollutant Discharge Elimination System (NPDES) General Permits for Storm Water Discharges From Construction Activities.

54 ENVIRONMENTAL SCIENCES↗

Impacts of air pollutants from fire and non-fire emissions on the regional air quality in Southeast Asia

Abstract. Severe haze events in Southeast Asia caused by particulate pollution have become more intense and frequent in recent years. Widespread biomass burning occurrences and particulate pollutants from human activities other than biomass burning play important roles in degrading air quality in Southeast Asia. In this study, numerical simulations have been conducted using the Weather Research and Forecasting (WRF) model coupled with a chemistry component (WRF-Chem) to quantitatively examine the contributions of aerosols emitted from fire (i.e., biomass burning) versus non-fire (including fossil fuel combustion, and road dust, etc.) sources to the degradation of air quality and visibility over Southeast Asia. These simulations cover a time period from 2002 to 2008 and are driven by emissions from (a) fossil fuel burning only, (b) biomass burning only, and (c) both fossil fuel and biomass burning. The model results reveal that 39 % of observed low-visibility days (LVDs) can be explained by either fossil fuel burning or biomass burning emissions alone, a further 20 % by fossil fuel burning alone, a further 8 % by biomass burning alone, and a further 5 % by a combination of fossil fuel burning and biomass burning. Analysis of an 24 h PM 2.5 air quality index (AQI) indicates that the case with coexisting fire and non-fire PM 2.5 can substantially increase the chance of AQI being in the moderate or unhealthy pollution level from 23 to 34 %. The premature mortality in major Southeast Asian cities due to degradation of air quality by particulate pollutants is estimated to increase from ∼ 4110 per year in 2002 to ∼ 6540 per year in 2008. In addition, we demonstrate the importance of certain missing non-fire anthropogenic aerosol sources including anthropogenic fugitive and industrial dusts in causing urban air quality degradation. An experiment of using machine learning algorithms to forecast the occurrence of haze events in Singapore is also explored in this study. All of these results suggest that besides minimizing biomass burning activities, an effective air pollution mitigation policy for Southeast Asia needs to consider controlling emissions from non-fire anthropogenic sources.

54 ENVIRONMENTAL SCIENCES↗

Impacts of air pollutants from fire and non-fire emissions on the regional air quality in Southeast Asia

Severe haze events in Southeast Asia caused by particulate pollution have become more intense and frequent in recent years, degrading air quality, threatening human health, and interrupting economic and societal activities. Widespread biomass burning activities are a major source of severe haze events in Southeast Asia. On the other hand, particulate pollutants from human activities other than biomass burning also play an important role in degrading air quality in Southeast Asia. In this study, numerical simulations have been conducted using the Weather Research and Forecasting (WRF) model coupled with a chemistry component (WRF-Chem) to quantitatively examine the contributions of aerosols emitted from fire (i.e., biomass burning) versus non-fire (including fossil fuel combustion, road and industrial dust, land use, and land change, etc.) sources to the degradation of air quality and visibility over Southeast Asia. These simulations cover a time period from 2002 to 2008 and were respectively driven by emissions from: (a) fossil fuel burning only, (b) biomass burning only, and (c) both fossil fuel and biomass burning. Across ASEAN 50 cities, these model results reveal that 39 % of observed low visibility days can be explained by either fossil fuel burning or biomass burning emissions alone, a further 20 % by fossil fuel burning alone, a further 8 % by biomass burning alone, and a further 5 % by a combination of fossil fuel burning and biomass burning. The remaining 28 % of observed low visibility days remain unexplained, likely due to emissions sources that have not been accounted for. Further analysis of 24-hr PM 2.5 Air Quality Index (AQI) indicates that comparing to the simulated result of the case with stand-alone non-fire emissions, the case with coexisting fire and non-fire PM 2.5 can substantially increase the chance of AQI being in the moderate or unhealthy pollution level from 23 % to 34 %. The premature mortality among major Southeast Asian cities due to degradation of air quality by particulate pollutants is estimated to increase from ~ 4110 per year in 2002 to ~ 6540 per year in 2008. In addition, we demonstrate the importance of certain missing non-fire anthropogenic aerosol sources including anthropogenic fugitive and industrial dusts in causing urban air quality degradation. An exploratory experiment of using machine learning algorithms to forecasting the occurrence of haze events in Singapore is also demonstrated in this study. All these results suggest that besides minimizing biomass burning activities, an effective air pollution mitigation policy for Southeast Asia needs to consider controlling emissions from non-fire anthropogenic sources.

Lee, Hsiang-He (ORCID:0000000251407324)↗

North China Plain as a hot spot of ozone pollution exacerbated by extreme high temperatures

Abstract. A large population in China has been exposed to both severe ozone (O3) pollution and extreme heat under global warming. Here, the spatiotemporal characteristics of coupled extremes in surface O3 and heat (OPCs) over China are investigated using surface observations, a process-based chemical transport model (GEOS-Chem), and multi-model simulations from Phase 6 of the Coupled Model Intercomparison Project (CMIP6). North China Plain (NCP; 37–41∘ N; 114–120∘ E) is identified as a hot spot of OPCs, where more than half of the O3 pollution days are accompanied by high temperature extremes. OPCs over NCP exceeded 40 d during 2014–2019, exhibiting an increasing trend. Both O3 concentrations and temperatures are elevated during OPCs compared with O3 pollution days occurring individually (OPIs). Therefore, OPCs impose more severe health impacts to humans than OPIs, but the stronger health effects are mainly driven by the higher temperatures. GEOS-Chem simulations further reveal that enhanced chemical production resulting from hot and stable atmospheric conditions under anomalous weather patterns primarily contributes to the exacerbated O3 levels during OPCs. In the future, CMIP6 projections suggest increased occurrences of OPCs over NCP in the middle of this century, but by the end of this century, OPCs may decrease or increase depending on the pollutant emission scenarios. However, for all future scenarios, extreme high temperatures will play an increasingly important role in modulating O3 pollution in a warming climate.

Wang, Pinya (ORCID:0000000170347868)↗

The CHRONOS mission: capability for sub-hourly synoptic observations of carbon monoxide and methane to quantify emissions and transport of air pollution

The CHRONOS space mission concept provides time-resolved abundance for emissions and transport studies of the highly variable and highly uncertain air pollutants carbon monoxide and methane, with sub-hourly revisit rate at fine (-4 km) horizontal spatial resolution across a North American domain. CHRONOS can provide complete synoptic air pollution maps ("snapshots") of the continental domain with less than 10 min of observations. This rapid mapping enables visualization of air pollution transport simultaneously across the entire continent and enables a sentinel-like capability for monitoring evolving, or unanticipated, air pollution sources in multiple locations at the same time with high temporal resolution. CHRONOS uses a compact imaging gas filter correlation radiometer for these observations, with heritage from more than 17 years of scientific data and algorithm advances by the science teams for the Measurements of Pollution in the Troposphere (MOPITT) instrument on NASA's Terra spacecraft in low Earth orbit. To achieve continental-scale sub-hourly sampling, the CHRONOS mission would be conducted from geostationary orbit, with the instrument hosted on a communications or meteorological platform. CHRONOS observations would contribute to an integrated observing system for atmospheric composition using surface, suborbital and satellite data with atmospheric chemistry models, as defined by the Committee on Earth Observing Satellites. Addressing the U.S. National Academy's 2007 decadal survey direction to characterize diurnal changes in tropospheric composition, CHRONOS observations would find direct societal applications for air quality management and forecasting to protect public health.

54 ENVIRONMENTAL SCIENCES↗

Remote measurement of pollution

A summary of the major conclusions and recommendations developed by the panels on gaseous air pollution, water pollution, and particulate air pollution is presented. It becomes evident that many of the trace gases are amenable to remote sensing; that certain water pollutants can be measured by remote techniques, but their number is limited; and that a similar approach to the remote measurement of specific particulate pollutants will follow only after understanding of their physical, chemical, and radiative properties is improved. It is also clear that remote sensing can provide essential information in all three categories that can not be obtained by any other means.

Source record↗

Aircraft engine pollution reduction.

The effect of engine operation on the types and levels of the major aircraft engine pollutants is described and the major factors governing the formation of these pollutants during the burning of hydrocarbon fuel are discussed. Methods which are being explored to reduce these pollutants are discussed and their application to several experimental research programs are pointed out. Results showing significant reductions in the levels of carbon monoxide, unburned hydrocarbons, and oxides of nitrogen obtained from experimental combustion research programs are presented and discussed to point out potential application to aircraft engines. An experimental program designed to develop and demonstrate these and other advanced, low pollution combustor design methods is described. Results that have been obtained to date indicate considerable promise for reducing advanced engine exhaust pollutants to levels significantly below current engines.

Rudey, R. A.↗