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At least 127 records · Page 7
All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

Microstructure Scale Lithium-Ion Battery Modeling: Part III. When and Where Lithium Plating Occurs and its Correlation with the Electrode Microstructure

Li-ion battery performance and degradation are closely related to the cell’s underlying electrode microstructure. Electrode microstructures are typically characterized with volume-averaged properties that neglect the impact of local heterogeneities. However, local heterogeneities create hot spots that can trigger degradation onset. Herein, a microstructure scale electrochemical model is used to investigate the impact of microstructure heterogeneity on lithium plating. The model predicts lithium plating is not uniform, even when considering a relatively small portion of the electrode (a cross-sectional area of 154×144 µm 2 ), preferring to plate on larger particles as compared to smaller particles. While local heterogeneities control where plating occurs, the model predicts that volume-averaged properties control when plating occurs. Additionally, the model predicts that the active material specific surface area has a linear relationship with the plating onset. However, the linear relationship between increased active material surface area and delayed plating response appears to be sensitive to the microstructure feature used to increase the active interface area. Here, a comparative case-study is explored where the specific surface area is increased by either reducing the active material particle diameter, adding open-porosity cracks, or increasing the active material surface roughness. The model predicts that increasing the specific surface area by reducing the active material particle diameter is the most effective strategy for delaying lithium plating. At 6C, reducing particle size is shown to be 3 and 20 times more effective than, respectively, adding open-porosity cracks and increasing surface roughness. A dual-layer electrode architecture combining gradations both for average properties and uniformities is eventually proposed to improve homogeneous material utilization and reduce degradation at high charge rates.

25 ENERGY STORAGE↗
DOE OSTI2024

Interplay of intercalation dynamics and lithium plating in monolithic and architectured graphite anodes during fast charging

Fast charging of high-capacity anodes is challenging due to lithium plating reactions, which lead to poor cycling performance and safety concerns. Thus, accurate predictions of plating onset and an understanding of this electrochemical process are crucial for robust battery design. However, the most commonly used models, based on porous electrode theory (e.g., the pseudo-2D model), are notoriously difficult to calibrate due to their complexity, limiting their predictive power. This work studies the process of lithium plating during fast charging of (small-particle) graphite half-cells by measuring local reaction progression and plating behavior using optical operando techniques. These experiments employ a realistic 1D graphite electrode geometry with commercially-relevant mass loading charged at fast charge rates. It is demonstrated that the local reaction progression and plating onset can not only be predicted accurately with a p2D numerical model, but that these processes follow a simple scaling law. Remarkably, the entire reaction histories of different electrodes charged at different rates (e.g., 160 μm thickness at 0.5C, 111 μm at 1C or 66 μm at 4C) were observed to have self-similar intercalation profiles. It is demonstrated that plating onset is in turn governed by the reaction profile which explains why both processes exhibit the same scaling behavior. Finally, operando measurements of local reaction dynamics are conducted for the first time in electrodes with channeled architectures, quantitatively determining how channels affect reaction uniformity and plating onset. Together, these results reveal underlying simplicity in the complex electrochemical environment of fast charging and lithium plating, improving understanding of this process. These fundamental insights are broadly applicable for design processes, modeling and experimental evaluation of lithium ion batteries.

25 ENERGY STORAGE↗
NASA NTRS1971

Theoretical buckling loads of boron/aluminum and graphite/resin fiber composite anisotropic plates

Theoretical results are presented for the buckling of anisotropic plates. The plates are subjected to simple and combined in-plane loading. The plates are made from fiber composite material of boron/aluminum or high-modulus graphite/resin. The results are presented in nondimensional form as buckling load against fiber orientation angle for various plate aspect ratios. The results indicate that buckling loads of boron/aluminum plates are independent of fiber direction if the plate aspect ratios are greater than about 1, and moderately dependent when this ratio is less than about 1. In addition, the results indicate that the buckling loads are independent of aspect ratio for plates with aspect ratios greater than about 2. Boron/ aluminum composite plates can resist buckling loads more efficiently than graphite/resin composites on a specific buckling stress basis. The numerical algorithm and a listing of the computer code used to obtain the results are included.

Chamis, C. C.↗
NASA NTRS1985

Noise Transmission Loss of a Rectangular Plate in an Infinite Baffle

An improved analytical procedure was developed that allows for the efficient calculation of the noise transmission characteristics of a finite rectangular plate. Both isotropic and symmetrically laminated composite plates are considered. The plate is modeled with classic thin-plate theory and is assumed to be simply supported on all four sides. The incident acoustic pressure is assumed to be a plane wave impinging on the plate at an arbitrary angle. The reradiated pressure is assumed to be negligible compared with the blocked pressure, and the plate vibrations are calculated by a normal-mode approach. A Green's function integral equation is used to link the plate vibrations to be transmitted far-field sound waves, and transmission loss is calculated from the ratio of incident to transmitted acoustic powers. The result is a versatile research and engineering analysis tool that predicts noise transmission loss and enables the determination of the modal behavior of the plate.

Roussos, Louis A.↗
NASA NTRS1986

Buckling behavior of compression-loaded symmetrically-laminated angle-ply plates with holes

An approximate analysis for buckling of a rectangular specially-orthotropic plate with a central circular hole is applied to symmetrically-laminated angle-ply plates. Results obtained from finite element analyses and experiments indicate that the approximate analysis predicts accurately the buckling loads of (+/-theta sub m)s plates with integer values of m not below 6 and with hole diameters up to 50 percent of the plate width. Moreover, the results indicate that the approximate analysis can be used to predict the buckling trends of plates with hole diameters up to 70 percent of the plate width. Results of a parametric study indicate the influence of hole size, plate aspect ratio, loading conditions, boundary conditions, and orthotropy on the buckling load. Results are also presented that indicate the relationship of the bending stiffness and the prebuckling load distribution to the buckling load of a plate with a hole.

Nemeth, M. P.↗
NASA NTRS1988

Dual passband dichroic plate for X-band

A need arose in the Deep Space Network for a dichroic plate that would simultaneously pass two desired frequency bands in the X-band region. In addition, the plate must be totally reflective for S-band frequencies. A dielectrically loaded dichroic plate is described that was developed to meet this need. The unique microwave properties that the new dichroic plate had to possess were: (1) insertion losses of less than 0.04 dB for X-band uplink frequencies centered at 7167 MHz and for X-band downlink frequencies centered at about 8425 MHz; (2) insertion losses that met the low loss requirements at 30 deg incidence angle simultaneously for both parallel and perpendicular polarizations; (3) total reflectivity at S-band frequencies; and (4) ability to maintain these electrical characteristics while passing 100 kW of CW power at X-band or while reflecting 100 kW of CW power at S-band. The dual passband dichroic plate is a thick metallic plate having an array of periodic round holes filled with Teflon plugs. Test results on an experimental prototype plate indicate that it is technically possible to design a dielectrically filled dichroic plate that meets all of the technical requirements.

Otoshi, T. Y.↗
NASA NTRS1990

Power flow analysis of two coupled plates with arbitrary characteristics

In the last progress report (Feb. 1988) some results were presented for a parametric analysis on the vibrational power flow between two coupled plate structures using the mobility power flow approach. The results reported then were for changes in the structural parameters of the two plates, but with the two plates identical in their structural characteristics. Herein, limitation is removed. The vibrational power input and output are evaluated for different values of the structural damping loss factor for the source and receiver plates. In performing this parametric analysis, the source plate characteristics are kept constant. The purpose of this parametric analysis is to determine the most critical parameters that influence the flow of vibrational power from the source plate to the receiver plate. In the case of the structural damping parametric analysis, the influence of changes in the source plate damping is also investigated. The results obtained from the mobility power flow approach are compared to results obtained using a statistical energy analysis (SEA) approach. The significance of the power flow results are discussed together with a discussion and a comparison between the SEA results and the mobility power flow results. Furthermore, the benefits derived from using the mobility power flow approach are examined.

Cuschieri, J. M.↗
NASA NTRS1990

On the tones of round choked jets impinging on normal flat plates

An experimental investigation of the sound produced by an axisymmetric supersonic jet impinging on plates with variable size and nozzle-to-plate spacings was performed. Spectral analysis and schlieren photography were used to determine the sound characteristics and flow disturbances associated with the production of discrete tones. Two classes of tones, associated with small and large plates, existed for pressure ratios above 2.70. For lower pressure ratios, however, only large plate tones occurred for all plate sizes with choked jet screech appearing at the largest spacings. Reflector tests indicated that both classes of tones were part of a feedback loop to the nozzle. Schlieren photography revealed both symmetric and asymmetric disturbances in the large plate jet flows which corresponded to symmetrical and helical modes of oscillation in the cross-spectrum studies. In addition to this, both symmetric and asymmetric oscillations of the shock waves occurred in the large plate case while symmetric oscillations of the shock wave occurred in the small plate case.

Powell, Alan↗
NASA NTRS1990

Present-day kinematics of the Rivera plate and implications for tectonics in southwestern Mexico

A model for the present-day motion of the Rivera plate relative to the North America, Cocos, and Pacific plates is derived using new data from the Pacific-Rivera rise and Rivera transform fault, together with new estimates of Pacific-Rivera motions. The results are combined with the closure-consistent NUVEL-1 global plate motion model of DeMets et al. (1990) to examine present-day deformation in southwestern Mexico. The analysis addresses several questions raised in previous studies of the Rivera plate. Namely, do plate motion data from the northern East Pacific rise require a distinct Rivera plate? Do plate kinematic data require the subduction of the Rivera plate along the seismically quiescent Acapulco trench? If so, what does the predicted subduction rate imply about the earthquake recurrence interval in the Jalisco region of southwestern Mexico?

Demets, Charles↗
NASA NTRS1992

Photometric calibration of NGS/POSS and ESO/SRC plates using the NOAO PDS measuring engine. I - Stellar photometry

The PDS/Monet measuring engine at the National Optical Astronomy Observatory was used to obtain photometry of nearly 10,000 stars on the NGS/POSS and 2000 stars on the ESO/SRC Survey glass plates. These measurements have been used to show that global transformation functions exist that allow calibration of stellar photometry from any blue or red plate to equivalent Johnson B and Cousins R photoelectric magnitudes. The four transformation functions appropriate for the POSS O and E and ESO/SRC J and R plates were characterized, and it was found that, within the measurement uncertainties, they vary from plate to plate only by photometric zero-point offsets. A method is described to correct for the zero-point shifts and to obtain calibrated B and R photometry of stellar sources to an average accuracy of 0.3-0.4 mag within the range R between values of 8 and 19.5 for red plates in both surveys, B between values of 9 and 20.5 on POSS blue plates, and B between values of 10 and 20.5 on ESO/SRC blue plates. This calibration procedure makes it possible to obtain rapid photometry of very large numbers of stellar sources.

Cutri, Roc M.↗
NASA NTRS1989

Comparison of full 3-D, thin-film 3-D, and thin-film plate analyses of a postbuckled embedded delamination

Strain-energy release rates are often used to predict when delamination growth will occur in laminates under compression. Because of the inherently high computational cost of performing such analyses, less rigorous analyses such as thin-film plate analysis were used. The assumptions imposed by plate theory restrict the analysis to the calculation of total strain energy, G(sub t). The objective is to determine the accuracy of thin-film plate analysis by comparing the distribution of G(sub t) calculated using fully three dimensional (3D), thin-film 3D, and thin-film plate analyses. Thin-film 3D analysis is the same as thin-film plate analysis, except 3D analysis is used to model the sublaminate. The 3D stress analyses were performed using the finite element program NONLIN3D. The plate analysis results were obtained from published data, which used STAGS. Strain-energy release rates were calculated using variations of the virtual crack closure technique. The results demonstrate that thin-film plate analysis can predict the distribution of G(sub t) quite well, at least for the configurations considered. Also, these results verify the accuracy of the strain-energy release rate procedure for plate analysis.

Whitcomb, John D.↗
NASA NTRS1993

Kinematics of the New Zealand plate boundary: Relative motion by GPS across networks of 1000 km and 50 km spacing

The NASA/DOSE 'Kinematics of the New Zealand Plate Boundary' experiment is a four-year cooperative Global Positioning System (GPS) experiment involving 6 universities and institutions in New Zealand and the United States. The investigation covers two scales, the first on the scale of plates (approximately 1000 km) and the second is on the scale of the plate boundary zone (approximately 50 km). In the first portion of the experiment, phase A, the objective is to make direct measurements of tectonic plate motion between the Australian and Pacific plates using GPS in order to determine the Euler vector of this plate pair. The phase A portion of this experiment was initiated in December 1992 with the first-epoch baseline measurements on the large scale network. The network will be resurveyed two years later to obtain velocities. The stations which were observed for phase A are shown and listed. Additional regional stations which will be used for this study are listed and are part of either CIGNET or other global tracking networks. The phase A portion of the experiment is primarily the responsibility of the UNAVCO investigators. Therefore, this report concentrates on phase A. The first year of NASA funding for phase A included only support for the field work. Processing and analysis will take place with the second year of funding. The second part of the experiemnt measured relative motion between the Australian and Pacific plates across the pate boundary zone between Hokitika and Christchurch on the South Island of New Zealand. The extent and rate of deformation will be determined by comparisons with historical, conventional surveys and by repeated GPS measurements to be made in two years. This activity was the emphasis of the LDGO portion of the study. An ancillary experiment, phase C, concentrated on plate boundary deformation in the vicinity of Wellington and was done as part of training during the early portion of the field campaign. Details of the objectives of the field investigations are given in the appendix. An overview of the 1992 GPS field program is also given in the appendix.

Meertens, Charles M.↗
NASA NTRS1993

On the effect of acoustic coupling on random and harmonic plate vibrations

The effect of acoustic coupling on random and harmonic plate vibrations is studied using two numerical models. In the coupled model, the plate response is obtained by integration of the nonlinear plate equation coupled with the nonlinear Euler equations for the surrounding acoustic fluid. In the uncoupled model, the nonlinear plate equation with an equivalent linear viscous damping term is integrated to obtain the response of the plate subject to the same excitation field. For a low-level, narrow-band excitation, the two models predict the same plate response spectra. As the excitation level is increased, the response power spectrum predicted by the uncoupled model becomes broader and more shifted towards the high frequencies than that obtained by the coupled model. In addition, the difference in response between the coupled and uncoupled models at high frequencies becomes larger. When a high intensity harmonic excitation is used, causing a nonlinear plate response, both models predict the same frequency content of the response. However, the level of the harmonics and subharmonics are higher for the uncoupled model. Comparisons to earlier experimental and numerical results show that acoustic coupling has a significant effect on the plate response at high excitation levels. Its absence in previous models may explain the discrepancy between predicted and measured responses.

Frendi, A.↗
NASA NTRS1991

Control of boundary layer transition location and plate vibration in the presence of an external acoustic field

The experiment is aimed at controlling the boundary layer transition location and the plate vibration when excited by a flow and an upstream sound source. Sound has been found to affect the flow at the leading edge and the response of a flexible plate in a boundary layer. Because the sound induces early transition, the panel vibration is acoustically coupled to the turbulent boundary layer by the upstream radiation. Localized surface heating at the leading edge delays the transition location downstream of the flexible plate. The response of the plate excited by a turbulent boundary layer (without sound) shows that the plate is forced to vibrate at different frequencies and with different amplitudes as the flow velocity changes indicating that the plate is driven by the convective waves of the boundary layer. The acoustic disturbances induced by the upstream sound dominate the response of the plate when the boundary layer is either turbulent or laminar. Active vibration control was used to reduce the sound induced displacement amplitude of the plate.

Maestrello, L.↗
NASA NTRS1993

Effect of acoustic coupling on random and harmonic plate vibrations

The effect of acoustic coupling on random and harmonic plate vibrations is studied using two numerical models. In the coupled model, the plate response is obtained by integration of the nonlinear plate equation coupled with the nonlinear Euler equations for the surrounding acoustic fluid. In the uncoupled model, the nonlinear plate equation with an equivalent linear viscous damping term is integrated to obtain the response of the plate subject to the same excitation field. For a low-level, narrow-band excitation, the two models predict the same plate response spectra. As the excitation level is increased, the response power spectrum predicted by the uncoupled model becomes broader and more shifted towards the high frequencies than that obtained by the coupled model. In addition, the difference in response between the coupled and uncoupled models at high frequencies becomes larger. When a high intensity harmonic excitation is used, causing a nonlinear plate response, both models predict the same frequency content of the response. However, the level of the harmonics and subharmonics are higher for the uncoupled model. Comparisons to earlier experimental and numerical results show that acoustic coupling has a significant effect on the plate response at high excitation levels. Its absence in previous models may explain the discrepancy between predicted and measured responses.

Frendi, Abdelkader↗
NASA NTRS1931

Strength of Rectangular Flat Plates Under Edge Compression

Flat rectangular plates of duralumin, stainless iron, monel metal, and nickel were tested under loads applied at two opposite edges and acting in the plane of the plate. The edges parallel to the direction of loading were supported in V grooves. The plates were all 24 inches long and varied in width from 4 to 24 inches by steps of 4 inches, and in thickness from 0.015 to 0.095 inch by steps of approximately 0.015 inch. There were also a few 1, 2, 3, and 6 inch wide specimens. The loads were applied in the testing machine at the center of a bar which rested along the top of the plate. Load was applied until the plate failed to take any more load. The tests show that the loads carried by the plates generally reached a maximum for the 8 or 12 inch width and that there was relatively small drop in load for the greater widths. Deflection and set measurement perpendicular to the plane of the plate were taken and the form of the buckle determined. The number of buckles were found to correspond in general to that predicted by the theory of buckling of a plate uniformly loaded at two opposite edges and simply supported at the edges.

Schuman, Louis↗
NASA NTRS1993

Acoustic radiation damping of flat rectangular plates subjected to subsonic flows

The acoustic radiation damping for various isotropic and laminated composite plates and semi-infinite strips subjected to a uniform, subsonic and steady flow has been predicted. The predictions are based on the linear vibration of a flat plate. The fluid loading is characterized as the perturbation pressure derived from the linearized Bernoulli and continuity equations. Parameters varied in the analysis include Mach number, mode number and plate size, aspect ratio and mass. The predictions are compared with existing theoretical results and experimental data. The analytical results show that the fluid loading can significantly affect realistic plate responses. Generally, graphite/epoxy and carbon/carbon plates have higher acoustic radiation damping values than similar aluminum plates, except near plate divergence conditions resulting from aeroelastic instability. Universal curves are presented where the acoustic radiation damping normalized by the mass ratio is a linear function of the reduced frequency. A separate curve is required for each Mach number and plate aspect ratio. In addition, acoustic radiation damping values can be greater than or equal to the structural component of the modal critical damping ratio (assumed as 0.01) for the higher subsonic Mach numbers. New experimental data were acquired for comparison with the analytical results.

Lyle, Karen Heitman↗
NASA NTRS1994

Experimental and theoretical studies of rewetting of unheated/heated grooved plates

Theoretical experimental investigations of the rewetting characteristics of thin liquid films over unheated and heated grooved plates were performed. Studied factors which affected the rewetting characteristics of the plate were mass flow rate of the rewetting liquid on the plate, the orientation of the plate (face up, face down or inclined) and smooth/groove surface conditions. The initial plate temperature was also varied, with experiments being performed between room temperature and 150 C. It was found that the rewetting velocity increased with the initial plate temperature. But when the temperature was increased further above the Leidenfrost temperature (liquid front temperature), the rewetting velocity decreases with the initial plate temperature. Hydrodynamically controlled and conductively controlled rewetting models were presented to explain and to predict the rewetting characteristics in these two distinct regions. Also found was a higher rewetting velocity when the grooved plate was placed in the face up orientation than in the face down orientation.

Chan, Shih H.↗