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NASA NTRSDate not supplied

Assessing the Radiative Impact of the 2019 – 2020 Australian Bushfires using Trajectory-Mapped CALIPSO Observations.

During the 2019/2020 fire season, Australian bushfires burned 46 million acres, killed 39 people and billions of animals, and became the costlier fire season in Australian history. Between the end of December and early January, a series of pyrocumulonimbus injected thick smoke layers in the upper troposphere and lower stratosphere which were observed over the Tasmanian Sea and New Zealand by the Ozone Mapping and Profiler Suite (OMPS) and the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO). The smoke plume crossed the tropopause and was further dispersed across the Eastern Pacific Ocean rising up to 30 km height after two weeks. . In this study, we use CALIPSO and the NASA Langley Trajectory Model (LaTM), driven by Modern-Era Retrospective analysis for Research and Application, Version 2 (MERRA-2) meteorological data, to track the dispersion of Australian fire smoke plumes in both the troposphere and the stratosphere. Trajectory mapping is used to re-construct the 3-dimension structure of the smoke plumes. Results are compared with independent observations from the Stratospheric Aerosol and Gas Experiment (SAGE) III on the International Space Station (ISS) to understand the complex transport of the plume into the stratosphere and its lifetime. Using trajectory maps, the impact of the Australian bushfires on the Earth’s radiative energy budget is assessed with the Clouds and the Earth’s Radiant Energy System (CERES).

Australian Bushfires↗

NASA NTRSDate not supplied

Assessing the Radiative Impact of the 2019 – 2020 Australian Bushfires using Trajectory-Mapped CALIPSO and SAGE III/ISS Observations.

Australian bushfire↗

NASA NTRS1993

Hypertext-Based Design of a User Interface for Scheduling

Operations Mission Planner (OMP) is an ongoing research project at JPL that utilizes Artificial Intelligence techniques to create an intelligent, automated planning and scheduling system. The challenge with a user interface is to 1) present as much information as possible at a given moment and 2) allow the user to quickly navigate through the various types of displays. This paper describes a design which applies the hypertext model to solve user interface problems. The general paradigm is to provide maps and search queries to allow the user to quickly find an interesting conflict or problem. Then allow the user to navigate through the displays in a hypertext fashion.

hypertext↗

NASA NTRS2021

Depletion & Recovery of the O3 Layer Observed from Space Over the Past 50 Years of the Anthropocene

This year we are celebrating the 50th anniversary of the launch of the backscatter UV (BUV) instrument on NASA’s Nimbus-4 satellite. Since then 10 more advanced instruments, but based on the same basic measurement principle, have been launched on polar orbiting NASA and NOAA satellites. The datasets produced by these instruments are unique for they have captured the period before the onset of the decline of the ozone layer due to manmade chemicals, the declining period, and the present slow recovery period. This period includes the rapid development of the iconic anthropocene era feature called the “Ozone Hole” . However, stitching together data from 11 separate satellite instruments to create a homogeneous record has presented many challenges. The first two NASA instruments suffered considerable degradation after launch that required the development of novel techniques to characterize their calibration. The next 7 instruments were launched on NOAA’s polar orbiting weather satellites that were not designed for long-term monitoring of climate variables. In particular, they didn’t have the station keeping capabilities needed to maintain a stable equator crossing time. Drifting orbits not only stress the retrieval algorithm and the calibration system of UV instruments but also make the interpretation of data difficult because the upper stratospheric ozone has systematic and complex diurnal variabilities that are comparable to the anthropogenic signal one wants to extract. We will highlight our recent efforts in untangling this knot. Finally, we will discuss the results from the OMPS limb scattering instrument, a recent addition to this constellation, that has been operating on the Suomi NPP satellite since October 2011. It is helping us capture how the ozone layer in the lower stratosphere and troposphere is evolving in response to the climate change and rising chemical pollutants in some parts of the world, while the upper stratosphere slowly recovers due to phaseout of the chemicals that initiated the decline of the ozone layer in the late 70s.

P Bhartia↗

NASA NTRSDate not supplied

Polar Vortex Outbreak Air Transport: Observation using Satellite IR Sounder Derived Ozone Product and Comparison with Model

The Single Field of View (SFOV) Sounder Atmospheric Products (SiFSAP) derived from Cross-track Infrared Sounder (CrIS) on SNPP and JPSS have a spatial resolution ( ~14.5 km) better than most global weather and climate models. Most recent significant improvement in the quality of these products enables us to use these high-resolution observation-based sounding data for weather studies and model evaluation. The aim of this study is to explore the value to use these SFOV products for studying the dynamic transport associated with polar vortex outbreak. In a few cases studies, we used SiFSAP products, especially ozone, as well as the data of wind, geopotential height (GPH) and potential velocity (PV) from the fifth-generation ECMWF reanalysis (ERA5) data, to analyze the variation of total ozone, relative humidity and ozone in different layers, as well as their correlation with GPH and PV. Some comparison of the retrieved temperature and water vapor with ERA5 data, and ozone with the Ozone Mapping and Profiler Suite (OMPS) measurements have also been made. It is found (1) the transport of O3-riched polar air accompanying the polar vortex breakup to lower latitude and lower atmosphere, and (2) the transport path of O3 agreeing well with the path of polar cold air (illustrated using the retrieved RH, wind fields and GPH). These results demonstrate the 3-D structure of O3 distribution as derived from CrIS measurements provides some insights of the cold air transport, and can be used to track the dynamic transport of polar cold air following the outbreak of polar vortex. The observed enhancement of O3 following the polar vortex outbreak also suggests some possible linkage between the tropospheric cold air advected with stratospheric air source.

Xiaozhen Xiong↗

NASA NTRS2022

Optimized Umkehr Profile Algorithm for Ozone Trend Analyses

The long-term record of Umkehr measurements from four NOAA Dobson spectrophotometers was reprocessed after updates to the instrument calibration procedures. In addition, a new data quality-control tool was developed for the Dobson automation software (WinDobson). This paper presents a comparison of Dobson Umkehr ozone profiles from NOAA ozone network stations (Boulder, OHP, MLO, Lauder) against several satellite records, including Aura Microwave Limb Sounder (MLS; ver. 4.2), and combined SBUV and OMPS records (NASA AGG and NOAA COH). A subset of satellite data is selected to match Dobson Umkehr observations at each station spatially (distance less than 200 km) and temporally (within 24 hours). Umkehr Averaging Kernels (AKs) are applied to vertically smooth all overpass satellite profiles prior to comparisons. The station Umkehr record consists of several instrumental records, which have different optical characterizations, and thus instrument-specific stray light contributes to the data processing errors and creates step changes in the record. This work evaluates the overall quality of Umkehr long-term measurements at NOAA ground-based stations and assesses the impact of the instrumental changes on the stability of the Umkehr ozone profile record. This paper describes a method designed to correct biases and discontinuities in the retrieved Umkehr profile that originate from the Dobson calibration process, repair, or optical realignment of the instrument. The M2GMI and GMI CTM ozone profile model output matched to station location and date of observation is used to evaluate instrumental step changes in the Umkehr record. Homogenization of the Umkehr record and discussion of the apparent stray light error in retrieved ozone profiles are the focus of this paper. Homogenization of ground-based records is of great importance for studies of long-term ozone trends and climate change.

Umkehr↗

NASA NTRSDate not supplied

Validation of CrIS Ozone and Carbon Oxide Products from CrIS Single-Field-of-View Retrievals

Single Field-of-view Sounder Atmospheric Products (SiFSAP) from Cross-track Infrared Sounder (CrIS) on S-NPP have been developed at NASA Langley Research center, and recently a significant improvement in its trace gases products has been made. These products are derived based on the Principal Component (PC)-based Radiative Transfer Model (PCRTM) and an optimal estimation retrieval method (PCRTM-RA). Use of the PCRTM in this method allows for fast and accurate calculations for thousands of spectral channels under clear and cloudy sky conditions. The use of principal component to compress information from all spectral channels into the PC domain enables to reduce the observational noise and use the information from all hyperspectral infrared channels. The retrieval is made on PC-domain, and temperature, water vapor, trace gases, cloud and surface parameters are retrieved simultaneously. This presentation will present some validation to the SiFSAP ozone (O3) and carbon monoxide (CO) products. Since the SiFSAP has a spatial resolution of about 14 km at nadir, which is better than most global weather and climate models and enables to make process-oriented analysis of the transport of these gases, this study will focus on validation of CO and O3 products under some extreme weather and/or climate events, such as CO emission and transport from large biomass burning, and O3 variation impacted by fire emission, stratospheric intrusion, and tropical cyclones. Data used in our validation include CO and O3 from NASA aircraft campaigns, plus other satellite products such as CO and O3 from AIRS, IASI and TROPOMI, MOPPIT CO and OMPS O3. Some comparison of SiFSAP O3 with the O3 from the fifth-generation ECMWF reanalysis (ERA5) data the NASA Modern-Era Retrospective Analysis for Research and Applications, Version 2 (MERRA-2) will also present. Such a validation not only helps to quantify the performance of the retrievals in these extreme conditions, but also displays the capability of satellite observation to capture the fine-scale spatial pattern of CO and O3 variation.

Xiaozhen Xiong↗

NASA NTRSDate not supplied

A Comparison of Stratospheric Smoke Events Seen by SAGE II (1984-2005) and SAGE III (2017-2021)

The ongoing Stratospheric Aerosol and Gas Experiment aboard the International Space Station (SAGE III/ISS) has mostly occurred during a period of relatively low aerosol loading. At the same time, it has almost observed a number of small to moderate injections of volcanic material in the stratosphere from the Aoba/Ambae eruption of 2018 to that of Karymsky in 2022. In addition, two of the largest known smoke intrusions into the stratosphere have occurred during the SAGE III/ISS mission (the British Columbia fire of August 2017 and the Australian Wildfire Event of 2019/2020). At least two other much smaller smoke events have also been observed in the SAGE III data (California Creek in September 2020 and McKay Creek in June 2021). Particularly with the two large events, it is tempting to speculate that these events are increasing in intensity and frequency possibly due to ongoing climate change. Realistically, change is difficult to assess since instrument data sets that can be used for quantifying historical events can be quite different in what and where they provide measurements. This complicates comparing one event to another potentially separated by many years. An exception to this issues are the measurements by SAGE III/ISS and those of its predecessor SAGE II (1984-2005). Both use the same measurement strategy, measure aerosol extinction coefficient at 1020 nm, and have similar spatial/temporal coverage. Both instruments are known to observe smoke events in the stratosphere. However, both have the same low observation density characteristic of solar occultation such that near-global coverage takes almost a month and characterizing effectively instant events like smoke and volcanic events take a matter of weeks depending on the vagaries of where the observations are being made at a critical juncture unlike instruments with high temporal/spatial resolution like limb-scatter instruments such as OMPS and OSIRIS. The goal of this work will be to use the same analysis approach to both the SAGE II and SAGE III data and compare both the frequency and intensity of smoke events observed by these instruments. While we do not expect to be able to make conclusions about change between the periods, the analysis is a first step in interpreting changes in the contribution of smoke to the stratospheric aerosol budget between the time frames encompassed by these instruments.

L. W. Thomason↗

NASA NTRSDate not supplied

Revisiting GloSSAC Using Space Based Measurements

We revisit Global Space-based stratospheric aerosol climatology (GloSSAC) and extend the dataset through 2021 in the latest version (version 2.2). Several space-based measurements have been used to construct GloSSAC. For version 2.2, important changes include implementation of a revised aerosol/cloud categorization for The Stratospheric Aerosol and Gas Experiment (SAGE III/ISS). SAGE III/ISS began its mission in June 2017. While SAGEIII/ISS makes reliable and robust solar occultation measurements in stratosphere—similar to its predecessors, interpreting aerosol extinction measurements in the vicinity of tropopause and in the troposphere have been a challenge for all SAGE measurements. Here, we study the challenges associated with the discrimination of aerosols and clouds from the extinction measurements. Here, we describe the methods implemented to categorize Clouds and aerosols using available SAGEIII/ISS aerosol measurements. We use version 5.2 of SAGE III/ISS extinction coefficients for the analysis. The current algorithm now classifies standard (background) and non-standard (enhanced) aerosols in the stratosphere and identify enhanced aerosols and aerosol/cloud mixture in the tropopause region. Extinction coefficient measurements from SAGE series of observations make an important contribution in the GloSSAC data base and therefore, the impact of cloud-filtered aerosol extinction coefficient measurements on the latest version of GloSSAC (version 2.2) is also discussed. Additionally, we discuss minor version changes occurred in other space-based measurements that include Optical Spectrograph and InfraRed Imaging System(OSIRIS) and Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation(CALIPSO). We also plan on evaluating and using aerosol extinction profiles from other satellite data sets such as Ozone Mapping Profiler Suite (OMPS) in a future version.

stratospheric aerosol↗

NASA NTRS2022

SAGE III/ISS Ozone and NO2 Validation Using Diurnal Scaling Factors

We developed a set of solar zenith angle, latitude- and altitude-dependent scaling factors to account for the diurnal variability in ozone (O3) and nitrogen dioxide (NO2) when comparing Stratospheric Aerosol and Gas Experiment (SAGE) III/ISS observations to observations from other times of day. The scaling factors are calculated as a function of solar zenith angle from the four-dimensional output of a global atmospheric chemistry model simulation of 2017–2020 that shows good agreement with observed vertical profiles. Using a global atmospheric chemistry model allows us to account for both chemically and dynamically driven variability. Both year-specific scale factors and a multi-year monthly climatology are available to decrease the uncertainty in inter-instrument comparisons and allow consistent comparisons between observations from different times of day. We describe the variability in the diurnal scale factors as a function of space and time. The quasi-biennial oscillation (QBO) appears to be a contributing factor to interannual variability in the NO2 scaling factors, leading to differences between years that switch sign with altitude. We show that application of these scaling factors improves the comparison between SAGE III/ISS and OSIRIS NO2 and between SAGE III/ISS and OMPS LP, OSIRIS, and ACE-FTS O3 observations. The comparisons between SAGE III/ISS O3 for sunrise or sunset vs. Microwave Limb Sounder (MLS) daytime or nighttime observations are also more consistent when we apply the diurnal scaling factors. There is good agreement between SAGE III/ISS V5.2 ozone and correlative measurements, with differences within 5 % between 20 and 50 km when corrected for diurnal variability. Similarly, the SAGE III/ISS V5.2 NO2 agreement with correlative measurement is mostly within 10 %. While the scale factors were designed for use with SAGE III/ISS observations, they can easily be applied to other observation intercomparisons as well.

Sarah A. Strode↗

NASA NTRS2022

Global Total Ozone Recovery Trends Attributed to Ozone-Depleting Substance (ODS) Changes Derived From Five Merged Ozone Datasets

We report on updated trends using different merged zonal mean total ozone datasets from satellite and ground-based observations for the period from 1979 to 2020. This work is an update of the trends reported in Weber et al. (2018) using the same datasets up to 2016. Merged datasets used in this study include NASA MOD v8.7 and NOAA Cohesive Data (COH) v8.6, both based on data from the series of Solar Backscatter Ultraviolet (SBUV), SBUV-2, and Ozone Mapping and Profiler Suite (OMPS) satellite instruments (1978–present), as well as the Global Ozone Monitoring Experiment (GOME)-type Total Ozone – Essential Climate Variable (GTO-ECV) and GOME-SCIAMACHY-GOME-2 (GSG) merged datasets (both 1995–present), mainly comprising satellite data from GOME, SCIAMACHY, OMI, GOME-2A, GOME-2B, and TROPOMI. The fifth dataset consists of the annual mean zonal mean data from ground-based measurements collected at the World Ozone and Ultraviolet Radiation Data Centre (WOUDC). Trends were determined by applying a multiple linear regression (MLR) to annual mean zonal mean data. The addition of 4 more years consolidated the fact that total ozone is indeed slowly recovering in both hemispheres as a result of phasing out ozone-depleting substances (ODSs) as mandated by the Montreal Protocol. The near-global (60° S–60° N) ODS-related ozone trend of the median of all datasets after 1995 was 0.4 ± 0.2 (2σ) %/decade, which is roughly a third of the decreasing rate of 1.5 ± 0.6 %/decade from 1978 until 1995. The ratio of decline and increase is nearly identical to that of the EESC (equivalent effective stratospheric chlorine or stratospheric halogen) change rates before and after 1995, confirming the success of the Montreal Protocol. The observed total ozone time series are also in very good agreement with the median of 17 chemistry climate models from CCMI-1 (Chemistry-Climate Model Initiative Phase 1) with current ODS and GHG (greenhouse gas) scenarios (REF-C2 scenario). The positive ODS-related trends in the Northern Hemisphere (NH) after 1995 are only obtained with a sufficient number of terms in the MLR accounting properly for dynamical ozone changes (Brewer–Dobson circulation, Arctic Oscillation (AO), and Antarctic Oscillation (AAO)). A standard MLR (limited to solar, Quasi-Biennial Oscillation (QBO), volcanic, and El Niño–Southern Oscillation (ENSO)) leads to zero trends, showing that the small positive ODS-related trends have been balanced by negative trend contributions from atmospheric dynamics, resulting in nearly constant total ozone levels since 2000.

Total Column Ozone Trends↗

NASA NTRSDate not supplied

Multi-Decadal Nitrogen Dioxide and Derived Products from Satellites (MINDS) Datasets Released by NASA GES DISC and Their Applications for Air Quality

Nitrogen dioxide (NO2), a pervasive air pollutant, comes from vehicles, power plants, industrial emissions, and off-road sources such as construction or lawn and gardening equipment. The NASA Goddard Earth Sciences Data and Information Services Center (GES DISC) curates many remote sensing datasets with NO2 retrievals, which have been utilized for air quality research and applications. The remotely-sensed datasets include those generated by the Ozone Monitoring Instrument (OMI) on the Aura satellite, the TROPOspheric Monitoring Instrument (TROPOMI) onboard the Copernicus Sentinel-5 Precursor (S5P), and the Ozone Mapping and Profiling Suite (OMPS) Nadir-Mapper (NM) instrument on the Suomi National Polar-orbiting Partnership (S- NPP). In collaboration with the NASA Making Earth System Data Records for Use in Research Environments (MEaSUREs) Multi-Decadal Nitrogen Dioxide and Derived Products from Satellites (MINDS) project, the GES DISC recently released MINDS datasets. The NASA MEaSUREs MINDS project aims to develop long-term NO2 global data records by adapting a consistent retrieval algorithm to multiple instrument measurements. Long-term data records will be achieved by applying consistent retrieval approaches to multiple satellite instruments, including OMI (2004 - ); the Global Ozone Monitoring Experiment (GOME, 1995-2011) onboard the second European Remote Sensing satellite (ERS-2); the Scanning Imaging Spectrometer for Atmospheric Cartography (SCIAMACHY, 2002-2012) onboard the ENVIronmental SATellite (ENVISAT); GOME-2 on the Meteorological Operational satellites (MetOp-A and MetOp-B, 2006 - ); and TROPOMI onboard the Copernicus S5P (2017 - ). The long-term record (1995 to present) of MINDS datasets makes them very useful for air quality trend studies. Some MINDS datasets with high spatial resolution of only a few kilometers can be used for air quality research and applications at regional scales. In this presentation, we will introduce all of the MINDS products and services, and demonstrate use cases of MINDS data for studying air quality. We will also present a few other NO2 datasets acquired from NASA’s Health and Air Quality Applied Sciences Team (HAQAST), to be archived and distributed by the GES DISC, and highlight some of their applications for air quality and health.

Feng Ding↗

NASA NTRS2022

Tropospheric Ozone Retrieval By A Combination of TROPOMI/S5P Measurements With BASCOE Assimilated Data

We present a new tropospheric ozone dataset based on TROPOspheric Monitoring Instrument (TROPOMI)/Sentinel-5 Precursor (S5P) total ozone measurements combined with stratospheric ozone data from the Belgian Assimilation System for Chemical ObsErvations (BASCOE) constrained by assimilating ozone observations from the Microwave Limb Sounder (MLS). The BASCOE stratospheric data are interpolated to the S5P observations and subtracted from the TROPOMI total ozone data. The difference is equal to the tropospheric ozone residual column from the surface up to the tropopause. The tropospheric ozone columns are retrieved at the full spatial resolution of the TROPOMI sensor (5.5×3.5 km 2 ) with daily global coverage. Compared to the Ozone Mapping and Profiler Suite Modern-Era Retrospective analysis for Research and Applications 2 (OMPS-MERRA-2) data, a global mean positive bias of 3.3 DU is found for the analysed period April 2018 to June 2020. A small negative bias of about −0.91 DU is observed in the tropics relative to the operational TROPOMI tropical tropospheric data based on the convective cloud differential (CCD) algorithm throughout the same period. The new tropospheric ozone data (S5P-BASCOE) are compared to a set of globally distributed ozonesonde data integrated up to the tropopause level. We found 2254 comparisons with cloud-free TROPOMI observations within 25 km of the stations. In the global mean, S5P-BASCOE deviates by 2.6 DU from the integrated ozonesondes. Depending on the latitude the S5P-BASCOE deviate from the sondes and between −4.8 and 7.9 DU, indicating a good agreement. However, some exceptional larger positive deviations up to 12 DU are found, especially in the northern polar regions (north of 70∘). The monthly mean tropospheric column and time series for selected areas showed the expected spatial and temporal pattern, such as the wave one structure in the tropics or the seasonal cycle, including a summer maximum, in the mid-latitudes.

Satellite Retrieval↗

NASA NTRS2022

Out of the blue: volcanic SO e2 emissions during the 2021–2022 eruptions of Hunga Tonga – Hunga Ha'apai (Tonga)

Most volcanism on Earth is submarine, but volcanic gas emissions by submarine eruptions are rarely observed and hence largely unquantified. On January 15, 2022 a submarine eruption of Hunga Tonga-Hunga Ha'apai (HTHH) volcano (Tonga) generated an explosion of historic magnitude, and was preceded by ≈1 month of Surtseyan eruptive activity and two precursory explosive eruptions. We present an analysis of ultraviolet (UV) satellite measurements of volcanic sulfur dioxide (SO 2 ) between December 2021 and the climactic January 15, 2022 eruption, comprising an unprecedented record of Surtseyan eruptive emissions. UV measurements from the Ozone Monitoring Instrument (OMI) on NASA’s Aura satellite, the Ozone Mapping and Profiler Suite (OMPS) on Suomi-NPP, the Tropospheric Monitoring Instrument (TROPOMI) on ESA’s Sentinel-5P, and the Earth Polychromatic Imaging Camera (EPIC) aboard the Deep Space Climate Observatory (DSCOVR) are combined to yield a consistent multi-sensor record of eruptive degassing. We estimate SO 2 emissions during the eruption’s key phases: the initial December 19, 2021 eruption (≈0.01 Tg SO 2 ); continuous SO 2 emissions from December 20, 2021 – early January 2022 (≈0.12 Tg SO 2 ); the January 13, 2022 stratospheric eruption (0.06 Tg SO 2 ); and the paroxysmal January 15, 2022 eruption (≈0.4-0.5 Tg SO 2 ); yielding a total SO 2 emission of ≈0.60.7 Tg SO 2 for the eruptive episode. We interpret the vigorous SO 2 emissions observed prior to the January 2022 eruptions, which were significantly higher than measured in the 2009 and 2014 HTHH eruptions, as strong evidence for a rejuvenated magmatic system. High cadence DSCOVR/EPIC SO 2 imagery permits the first UV-based analysis of umbrella cloud spreading and volume flux in the January 13, 2022 eruption, and also tracks early dispersion of the stratospheric SO 2 cloud injected on January 15. The ≈0.4-0.5 Tg SO 2 discharged by the paroxysmal January 15, 2022 HTHH eruption is low relative to other eruptions of similar magnitude, and a review of other submarine eruptions in the satellite era indicates that modest SO 2 yields may be characteristic of submarine volcanism, with the emissions and atmospheric impacts likely dominated by water vapor. The origin of the low SO 2 loading awaits further investigation but scrubbing of SO 2 in the water-rich eruption plumes and rapid conversion to sulfate aerosol are plausible, given the exceptional water emission by the January 15, 2022 HTHH eruption.

Volcanoes↗

NASA NTRSDate not supplied

PyroCbs from Australia Fires and its Impact Using Satellite Observations from CrIS and TROPOMI and Reanalysis Data

Pyrocumulonimbus (pyroCb) clouds are thunder clouds created by intense heat from the Earth’s surface. They are formed similarly to cumulonimbus clouds, but the intense heat that results in the vigorous updraft comes from fire, either large wildfires or volcanic eruptions. Australia’s unprecedented fire disasters at the end of 2019 to early 2020 emitted huge amounts of carbon monoxide (CO) and fire aerosol particles to the atmosphere, particularly during the pyroCb outbreak that occurred in southeast Australia between 29 December 2019 and 4 January 2020. It was estimated that at least 18 pyroCbs were generated during this episode, and some of them injected ice, smoke, and biomass burning gases above the local tropopause. An unprecedented abundance of H2O and CO in the stratosphere, and the displacement of background ozone (O3) and N2O from rapid ascent of air from the troposphere and lower stratosphere were found from satellite observations. Some other studies also found that the fire emissions and their long-range transport resulted in stratospheric aerosol, temperature, and O3 anomalies after the 2020 Australian bushfires and altered the Antarctic ozone and vortex, posing great impact to local air quality and climate change. Further study on the atmospheric thermodynamic status of atmosphere associated with these pyroCbs, and the change of the cloud properties and trace gases during this unprecedented Australia fires will be made using a new single Field of View (SFOV) Sounder Atmospheric Products (SiFSAP). SiFSAP was developed by NASA using the Cross-track Infrared Sounder (CrIS) and Advanced Technology Microwave Sounder (ATMS) onboard SNPP and JPSS-1, and will soon be available to the public at NASA DAAC. Since this product has a spatial resolution of 15 km at nadir, which is better than most global weather and climate models and other current operational sounding products, a process-oriented analysis of the dynamic transport of CO and fire plumes during this unprecedented fire disasters will be made in this study. Based on a Principal Component Radiative Transfer Model (PCRTM) and an optimized estimation retrieval algorithm, a simultaneously retrieval is made using the whole spectral information measured by CrIS, and the derived SiFSAP include temperature, water vapor, trace gases (such as O3, CO2, CO, CH4 and N2O), cloud properties and surface properties. Use of ATMS together with CrIS allows SiFSAP to get accurate retrieval products under thick pyroCb conditions, and an algorithm to detect pyroCb based on the hyperspectral infrared sounder spectrum from CrIS will be developed and verified. In addition to SiFSAP sounding products, other products like CO, O3, NO2 from TROPOMI, O3 from OMPS will be used for retrospective analysis. The wind fields from the NASA’s Modern-Era Retrospective Analysis for Research and Applications Version-2 (MERRA-2) and ERA5 will be used to characterize the transport, and the SiFSAP temperature and water vapor profiles within and around pyroCbs will be compared with MERRA-2 and ERA5 products.

Xiaozhen (Shawn) Xiong↗

NASA NTRSDate not supplied

Simulating Sulfate Aerosol Size in the Hunga Tonga Plume: Comparisons with Observations

Using the NASA GEOS Chemistry Climate Model (CCM) coupled to a detailed sectional aerosol microphysical model, we have simulated the January 2022 Hunga Tonga-Hunga Ha’apai (HTHH) plume. We have developed a version of the Global Modeling Initiative (GMI) chemistry mechanism to include the requisite sulfur chemistry and coupled it to the Community Aerosol and Radiation Model for Atmospheres (CARMA) sectional aerosol microphysics within the GEOS CCM. Our simulations focus on the lifecycle of stratospheric sulfur injected by the eruption–from the oxidation of the injected sulfur dioxide to the nucleation, growth, coagulation, hydration, and eventual settling of the volcanic sulfate aerosol particles. In order to constrain the simulated microphysics, we focus on comparing our model to observations with aerosol size information, namely in-situ particle counter observations and multi-wavelength satellite observations from OMPS-LP and SAGE-III. This eruption provides an interesting test case for our model; both the modeled gas-phase chemistry as well as the modeled aerosol microphysics are perturbed by the massive injection of water that accompanied the primary sulfur emissions from the eruption.

aerosols↗

NASA NTRS2024

Investigating Zonal Asymmetries in Stratospheric Ozone Trends From Satellite Limb Observations and a Chemical Transport Model

This study investigates the origin of a zonal asymmetry in stratospheric ozone trends at northern high latitudes, identified in satellite limb observations over the past two decades. We use a merged data set consisting of ozone profiles retrieved at the University of Bremen from SCIAMACHY and OMPS-LP measurements to derive ozone trends. We also use TOMCAT chemical transport model (CTM) simulations, forced by ERA5 reanalyses, to investigate the factors that drive the asymmetry observed in the long-term changes. By studying seasonally and longitudinally resolved observation-based ozone trends, we find, especially during spring, a well-pronounced asymmetry at polar latitudes with values up to +6 % per decade over Greenland and −5 % per decade over western Russia. The control CTM simulation agrees well with these observed trends, whereas sensitivity simulations indicate that chemical mechanisms involved in the production and removal of ozone, or their changes, are unlikely to explain the observed behavior. The decomposition of TOMCAT ozone time series and ERA5 geopotential height into the first two wavenumber components shows a clear correlation between the two variables in the middle stratosphere and demonstrates a weakening and a shift in the wavenumber-1 planetary wave activity over the past two decades. Finally, the analysis of the polar vortex position and strength points to a decadal oscillation with a reversal pattern at the beginning of the century. The same is found in the ozone trend asymmetry. This further stresses the link between changes in the polar vortex position and the identified ozone trend pattern.

Instrumentation↗

NASA NTRSDate not supplied

Tracking the Hunga Tonga-Hunga Ha’apai Eruption Stratospheric Aerosol and Trace Gas Plumes Using Machine Learning

On January 15, 2022, the Hunga Tonga-Hunga Ha’apai (hereafter, Hunga Tonga) submarine volcano had an explosive eruption that thrusted ash, gases, and water vapor through the troposphere into the stratosphere and mesosphere. Previous studies manually tracked the aerosol and trace gas plumes over time across different positions in the southern hemisphere. Using data retrieved from low earth orbiting satellite instruments (e.g., OMPS, OMI, and CALIPSO), this research demonstrates how open-source machine learning (ML) models, like Meta’s Segment Anything Model (SAM), with prompt engineering can perform automatic plume tracking following the Hunga Tonga eruption. This extensible methodology, and modular data processing and modeling pipeline using NASA Earthdata and Openscapes, establishes a framework for systematically and rapidly studying extreme events, including volcanic eruptions and large-scale wildfires. By combining advanced machine learning techniques, such as SAM’s zero-shot learning, with large volumes of remote sensing data, this work demonstrates how AI and open science can accelerate research and generate actionable results. The tools and technologies presented here can help translate earth science to action from NASA’s current and future Earth observing satellite missions (e.g., the Atmosphere Observing System (AOS)), and assist researchers and stakeholders in understanding, mapping, and responding to natural disasters and extreme events in a changing world.

David M. Giles↗