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Advances in Autoradiography Systems for Nuclear Forensic Analysis

Nuclear forensic analysis techniques work to determine the contents of radiological samples with nondestructive and destructive analysis methods. Autoradiography is a nondestructive analysis method that creates an image of the distribution of radioactivity within the sample. These images allow the location of the radiological content within a sample to be ascertained, which can be used for further analysis. Autoradiography has been used since the discovery of radiation and has been continuously developed to better suit the needs of the medical, nuclear security, nuclear safeguards, and nuclear forensic communities. Recent developments in autoradiography have led to a higher spatial resolution down to a level of tens of microns, real-time capabilities that minimize the risk of overexposure, and the ability to discriminate particles. All of these developments in autoradiography would assist the nuclear forensics community in understanding the placement of radiological content within a sample and in understanding the locations of beta-particle interactions versus those for alpha-particle interactions. This article aims to discuss the history of autoradiography as well as multiple different autoradiographic technologies while focusing on imaging plates, the BeaQuant system, and the ionizing-radiation Quantum Imaging Detector system. This article reviews three autoradiographic techniques and detectors, discusses how they relate to nuclear forensics, and addresses the drawbacks and benefits of each detector.

Autoradiography↗

Synergistic effects of Al, Ga, and In doping on ZnO nanorod arrays grown via citrate-assisted hydrothermal technique for highly efficient and fast scintillator screens

To be used as efficient alpha particle scintillator in the fields of nuclear security, nuclear nonproliferation and high-energy physics, scintillator screens must have high light output and fast decay properties. While there has been a great deal of progress in scintillation efficiency, achieving fast decay time properties are still a challenge. In this work, the near band edge (NBE) UV luminescence and alpha particle induced scintillation properties of vertically aligned densely packed ZnO nanorods (NRs) doped with Al, Ga, and In have been thoroughly investigated. The high crystalline hexagonal wurtzite structure with a strong orientation through the c -axis plane (002) and aspect ratios in the range 13–22 have been observed for all ZnO NRs. Electron paramagnetic resonance (EPR) analysis exhibited paramagnetic signals at g ≈ 1.96 for all ZnO NRs. A cost effective green hydrothermal synthesis technique was employed to grow well-aligned NRs. Using citrate as an additive acting as a strong reducing agent in the solution during the crystal growth, defects on the surface are significantly suppressed, thereby enhancing the NBE UV emission. Significantly higher NBE UV emission was observed from the top surface of ZnO NRs in cathodoluminescence (CL) microscopy. Results show that citrate assisted donor doping of ZnO NRs not only reduces the defect emission and NBE self-absorption, but also induces fast decay time (~ 600–700 ps), which makes ZnO NRs a good candidate for fast alpha particle scintillator screens used in associated particle imaging for time and direction tagging of individual neutrons generated in D–T and D–D neutron generators.

36 MATERIALS SCIENCE↗

American Chemical Society's summer school in nuclear and radiochemistry. Final report

The ACS Summer Schools in Nuclear and Radiochemistry (herein called “Summer Schools”) were held each year at San Jose State University (SJSU) and Brookhaven National Laboratory (BNL). The Summer Schools are an intensive, six-week program that includes both a lecture component covering fundamental principles of nuclear chemistry and radiochemistry and a laboratory component providing hands-on experience for the students to observe and test many of the basic principles that they learn about in lecture and in the special seminars. Each site hosts 12 undergraduate students annually. Participants are selected from a nation-wide pool of applicants who are currently enrolled as undergraduates seeking bachelors’ degrees, preferably in disciplines of physical sciences or engineering. To broaden the students’ perspectives on nuclear science, prominent research scientists active in nuclear and/or radiochemical research participate in a Guest Lecture Series. Symposia emphasizing nuclear security, nuclear medicine, and career opportunities are conducted as a part of the program.

07 ISOTOPE AND RADIATION SOURCES↗

Nuclear Weapon Security DOD Perspective

Presentation Overview: Nuclear Weapon Security DOD Perspective; DOD and DOE Nuclear Security Policy Standards; Weapon Secure Storage Methods; Modes of Transportation: DOD and DOE; Security Breeches; Basic Security Classification Practices

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗

INS Nuclear Material Accounting and Control Instructional Video Materials- FY 25 Guides

This training video provides an essential guide to understanding and utilizing Tamper Indicating Devices (TIDs), with a specific focus on a common Mylar (Adhesive) variety during the application process. TIDs are a critical part of nuclear security, used to detect unauthorized access to sensitive materials or facilities. The Mylar (adhesive) TID employes a tamper-evident film integrated into the TID that visually indicates any tampering attempts. This video will explain how an example Mylar (adhesive) TID works, demonstrate proper installation techniques, and highlight how to interpret its indicators to ensure the security of nuclear materials.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗

INSEN 2023 Yearly Updates

The International Nuclear Security Education Network (INSEN) is the primary international network for nuclear security educational initiatives. INSEN plays a central role in fostering collaboration and knowledge-sharing among nuclear security education experts worldwide. In the wake of the global pandemic, INSEN remained committed to strengthening nuclear security education and resumed in-person activities. The International Atomic Energy Agency (IAEA) confirmed its continued dedication and support to the network’s mission and presented new activities aimed at elevating global nuclear security efforts. Throughout the year and during the annual and leadership meetings, working groups showcased their vibrant work and presented innovative ideas, invigorating the attendees’ dedication to their crucial work. Comprehensive presentations by the IAEA during the INSEN annual and leadership meetings highlighted the importance of the network and its continued commitment to promoting nuclear security on a global scale. One notable and encouraging trend was the increase in network membership, signifying a growing commitment to nuclear security worldwide and the continued interest in nuclear security from member states and international organizations. The value of initiatives such as the Women in Nuclear Security Initiative was emphasized at the annual meeting, accenting the need for diverse perspectives and expertise to ensure a secure nuclear landscape.

96 KNOWLEDGE MANAGEMENT AND PRESERVATION↗

The research challenges in security and safeguards for nuclear fission batteries

This paper discusses the nuclear security and safeguards research challenges presented by the development and deployment of nuclear fission batteries. These are defined as easily transportable and deployable nuclear systems which are designed to operate either unattended or autonomously. We start by defining the current landscape of domestic and international safeguards and security and discuss how it can be affected by the introduction these new nuclear systems. We then specifically discuss the technology gaps and technologies to be developed to facilitate their practical deployment. We find that, as expected, we can leverage conclusions from existing security and safeguards studies for small modular rectors and develop bespoke target set analyses to inform security postures based on probabilistic risk assessment. We find also that specific fission battery security economic analysis tools are needed and security by design must be applied early. However, the most important finding is that these new systems will require a new comprehensive set of cyber tools covering transportation, installation, operation, maintenance security of the fission battery systems. Altogether, we find that the development of the necessary security and safeguards requirements at the design phase of such a technology will be of great benefit in the smooth deployment of this modern nuclear energy system.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

First Report of the Nuclear Data Subcommittee of the Nuclear Science Advisory Committee

Accurate, reliable nuclear data is essential for the success of Federal missions such as nonproliferation, nuclear forensics, homeland security, national defense, space exploration, clean energy generation, and scientific research. Data access is also key to innovative commercial developments such as new medicines, automated industrial controls, energy exploration, energy security, nuclear reactor design, and isotope production. The United States Nuclear Data Program (USNDP) is the domestic custodian of nuclear data. In its April 2022 meeting, the DOE/NSF Nuclear Science Advisory Committee was charged with preparing two reports on nuclear data. In this first report, we review recent accomplishments of the USNDP and discuss complementary and collaborative international efforts. Detailed descriptions of nuclear data needs for basic science, nonproliferation, national security, nuclear energy together with medical and space applications are also presented. Lastly, a set of specific cross-cutting nuclear data needs with relevance for multiple applications areas are also identified for further discussion in a follow-on report planned for release at the end of January 2023.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Data Driven Analysis for Modernization Program Management

NNSA is responsible for managing national nuclear security missions: ensuring a safe, secure, and reliable nuclear deterrent; supplying nuclear fuel to the Navy; and supporting the nation’s nuclear nonproliferation efforts. However, over half of NNSA’s facilities are more than 40 years old, and roughly one-third date back to the Manhattan Project. To execute its critical nuclear security missions, NNSA is making large investments to modernize its nuclear production capabilities. This ramp up represents NNSA’s largest modernization effort since the Cold War. Given the scale of these efforts, NNSA’s Office of Secondary Stage Production Modernization has implemented data driven techniques to prioritize investments and inform strategic decision making. NNSA, with support from its site managing contractors, has developed and implemented an integrated schedule and risk management system to address the issues and limitations with the traditional approach. The multi-year integrated schedules are key to identifying program linkages and managing large portfolios comprised of many different projects and efforts. In conjunction with the integrated schedule, a new program risk management system has also been developed and implemented, which manages program risks and opportunities, along with specific mitigation strategies to reduce or eliminate the risks per timelines that are tracked in the integrated schedule. This paper is supplemented with a follow-on presentation on effective management of program material and throughput modeling.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

2024 Annual Site Environmental Report for Sandia National Laboratories, Livermore, California

Sandia National Laboratories is a multimission laboratory managed and operated by National Technology & Engineering Solutions of Sandia, LLC, a wholly-owned subsidiary of Honeywell International Inc., for the U.S. Department of Energy’s National Nuclear Security Administration. The National Nuclear Security Administration’s Sandia Field Office administers the Prime Contract and oversees contractor operations at Sandia National Laboratories, California. Activities at this multi-program engineering and science laboratory support the nuclear weapons stockpile program, energy and environmental research, homeland security, micro- and nanotechnologies, and basic science and engineering research. The U.S. Department of Energy’s National Nuclear Security Administration and its management and operating contractor are committed to fulfilling regulatory obligations, safeguarding the environment, assessing sustainability practices, and ensuring the validity and accuracy of the monitoring data presented in this annual site environmental report (ASER). This report provides a summary of environmental monitoring and compliance activities that occurred at Sandia National Laboratories, California, during calendar year 2024, unless noted otherwise. General site and environmental program information is also included. This report was prepared in accordance with DOE Order 231.1B, Admin Change 1, Environment, Safety and Health Reporting.

54 ENVIRONMENTAL SCIENCES↗