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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 127 records · Page 7
All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

Ferroelectric Self-Polarization Controlled Magnetic Stratification and Magnetic Coupling in Ultrathin La 0.67 Sr 0.33 MnO 3 Films

Multiferroic oxide heterostructures consisting of ferromagnetic and ferroelectric components hold the promise for nonvolatile magnetic control via ferroelectric polarization, advantageous for the low-dissipation spintronics. Modern understanding of the magnetoelectric coupling in these systems involves structural, orbital, and magnetic reconstructions at interfaces. Previous works have long proposed polarization-dependent interfacial magnetic structures; however, direct evidence is still missing, which requires advanced characterization tools with near-atomic-scale spatial resolutions. Here, extensive polarized neutron reflectometry (PNR) studies have determined the magnetic depth profiles of PbZr 0.2 Ti 0.8 O 3 /La 0.67 Sr 0.33 MnO 3 (PZT/LSMO) bilayers with opposite self-polarizations. When the LSMO is 2–3 nm thick, the bilayers show two magnetic transitions on cooling. However, temperature-dependent magnetization is different below the lower-temperature transition for opposite polarizations. PNR finds that the LSMO splits into two magnetic sublayers, but the inter-sublayer magnetic couplings are of opposite signs for the two polarizations. Near-edge X-ray absorption spectroscopy further shows contrasts in both the Mn valences and the Mn–O bond anisotropy between the two polarizations. Finally, this work completes the puzzle for the magnetoelectric coupling model at the PZT/LSMO interface, showing a synergic interplay among multiple degrees of freedom toward emergent functionalities at complex oxide interfaces.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2021

Updated magnetized transport coefficients: impact on laser-plasmas with self-generated or applied magnetic fields

Errors in the Epperlein and Haines (1986 Phys. Fluids ) transport coefficients were recently found at low electron magnetizations, with new magnetic transport coefficients proposed simultaneously by two teams (Sadler et al 2021 Phys. Rev. Lett. and Davies et al 2021 Phys. Plasmas ); these two separate sets of updated coefficients are shown in this paper to be in agreement. Here, the importance of these new coefficients in laser-plasmas with either self-generated or applied magnetic fields is demonstrated. When an external magnetic field is applied, the cross-gradient-Nernst term twists the field structure; this twisting is reduced by the new coefficients in the low magnetization regime. For plasmas where only self-generated magnetic fields are present, the new coefficients are found to result in the magnetic field moving with the Righi–Leduc heat-flow, enhancing the impact of MHD. Simulations of Biermann battery magnetic fields around ICF hot-spot perturbations are presented, with cross-gradient-Nernst transport increasing spike penetration.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2020

Magnetic field dependence of low-energy magnons, anisotropic heat conduction, and spontaneous relaxation of magnetic domains in the cubic helimagnet ZnCr 2 Se 4

Here, anisotropic low-temperature properties of the cubic spinel helimagnet ZnCr 2 Se 4 in the single-domain spin-spiral state are investigated by a combination of neutron scattering, thermal conductivity, ultrasound velocity, and dilatometry measurements. In an applied magnetic field, neutron spectroscopy shows a complex and nonmonotonic evolution of the spin-wave spectrum across the quantum-critical point that separates the spin-spiral phase from the field-polarized ferromagnetic phase at high fields. A tiny spin gap of the pseudo-Goldstone magnon mode, observed at wave vectors that are structurally equivalent but orthogonal to the propagation vector of the spin helix, vanishes at this quantum critical point, restoring the cubic symmetry in the magnetic subsystem. The anisotropy imposed by the spin helix has only a minor influence on the lattice structure and sound velocity but has a much stronger effect on the heat conductivities measured parallel and perpendicular to the magnetic propagation vector. The thermal transport is anisotropic at T≲ 2K, highly sensitive to an external magnetic field, and likely results directly from magnonic heat conduction. We also report long-time thermal relaxation phenomena, revealed by capacitive dilatometry, which are due to magnetic domain motion related to the destruction of the single-domain magnetic state, initially stabilized in the sample by the application and removal of magnetic field. Our results can be generalized to a broad class of helimagnetic materials in which a discrete lattice symmetry is spontaneously broken by the magnetic order.

36 MATERIALS SCIENCE↗
DOE OSTI2022

Origins of magnetic memory and strong exchange bias bordering magnetic compensation in mixed-lanthanide systems

Here, the unexpected physical phenomena resulting from the seemingly inconsequential substitutions of chemically similar lanthanide elements in the Pr 1-x Gd x ScGe system are exploited to further the understanding of rare-earth magnetism and inform materials design. By directly probing magnetic moments of crystallographically indistinguishable Pr and Gd we solve the puzzles of how an unusual magnetic memory and strong exchange bias emerge at specific, easily predictable chemistries. Both effects are rooted in a robust antiparallel arrangement of large 4f magnetic moments of light and heavy lanthanides. This enables precise control of nearly zero net magnetization either opposed to, or aligned with, the external magnetic field that persists over a wide range of temperatures and fields. Further, spontaneous perturbations in the random distribution of lanthanide ions makes strong exchange bias possible in bulk single-phase compounds bordering magnetic compensation, consequently expanding the materials base beyond artificial magnetic multilayers and broadening the range of potential applications of the phenomenon.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2025

Switching of Magnetic Order via Non‐Magnetic Al Addition in FeCoNiMnAl x Films

Magnetic high entropy alloys (HEAs) consisting of 3 d transition metals offer an exciting platform to explore novel magnetic phases as they often house competing exchange interactions in combination with random site disorders. In this work, a sensitive and tunable magnetic order is demonstrated in sputtered single-layer FeCoNiMnAl x films, as a function of non-magnetic Al addition, along with an unexpected exchange bias effect. Thin films of 50 nm FeCoNiMn exhibit a face-centered-cubic ( fcc ) phase, reentrant spin glass (SG) transition near 100 K, and a large exchange bias of over 500 Oe after field-cooling to 5 K. The exchange bias is increased to 930 Oe through a small addition of 5 at.% Al. Further Al addition to 12 at.% results in a body-centered-cubic ( bcc ) phase, coinciding with a large increase in the saturation magnetization, decrease of exchange bias to 50 Oe, and suppression of SG behavior. The change in magnetic order across the Al-induced structural transformation is mediated by the switching of Mn ground state from AF to FM, which is supported by first-principles calculations and experimentally confirmed via X-ray magnetic circular dichroism. These results open up new HEA strategies for explorations of novel magnetic phases.

competing exchange interactions↗
DOE OSTI2025

Spin excitations and dynamics in 2D magnets: An overview of magnons and magnetic skyrmions

van der Waals magnetic materials open up exciting possibilities to investigate fundamental spin properties in low-dimensional systems and to build compact functional spintronic structures. This review focuses on the recent progress in two-dimensional (2D) magnets that explore beyond the homogenous magnetically ordered state, including magnons (spin waves), magnetic skyrmions, and complex magnetic domains. Properties of these spin and topology excitations in 2D magnets provide insights into spin-orbit interactions and other forms of coupling between electrons, phonons, and spin-dependent excitations. Such spin-based quasiparticles can also serve as information carriers for next-generation high-speed computing elements. Furthermore, we will first lay out the general theoretical basis of dynamical responses in magnetic systems, followed by detailed descriptions of experimental progress in magnons and spin textures (including magnetic domains and skyrmions). Discussion on the experimental techniques and future perspectives are also included.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2025

Self-Assembled Magnetic Nanoparticle Layers: Structural Control for Reconfigurable Magnetism and Functional Applications

We advance soft X-ray vector ptychographic tomography to map the 3D magnetization field in self-assembled superparamagnetic nanoparticles at a liquid–liquid interface, revealing how layered structures influence magnetic ordering. We observe that monolayers with low coordination numbers exhibit weak magnetic order, with magnetic vortices disrupting spin alignment. In contrast, bilayers and trilayers with higher coordination numbers display long-range magnetic order with strong spin correlations across larger distances and a suppression of magnetic vortices. We further quantify the average distance for vortex–antivortex pairs as 26.0 ± 2.0 nm, while vortex–vortex and antivortex–antivortex pairs exhibit larger separations, averaging 44.9 ± 5.2 and 54.1 ± 7.4 nm, respectively. These experimental results are supported by micromagnetic Monte Carlo simulations. Our findings illustrate how layered structures enhance magnetic order and spin correlation in superparamagnetic nanoparticle assemblies, providing a promising approach for tuning magnetic properties in applications such as data storage, microrobotics, and biomedicine.

Lu, Xingyuan↗
DOE OSTI2026

Discovery of van Hove singularities: electronic fingerprints of 3Q magnetic order in a van der Waals quantum magnet

Magnetically intercalated transition metal dichalcogenides are emerging as a rich platform for exploring exotic quantum states in van der Waals magnets. Among them, Co x TaS 2 has attracted intense interest following the recent discovery of a distinctive 3Q magnetic ground state and a pronounced topological Hall effect below a critical doping of x ≈ 1/3, both intimately tied to cobalt concentration. To date, direct signatures of this enigmatic 3Q magnetic order in the electronic structure remain elusive. Here we report a comprehensive doping dependent angle resolved photoemission spectroscopy study that unveils these long-sought fingerprints. Our data reveal an unexpected inverse-Mexican-hat dispersion along the K-M-K' direction, accompanied by two van Hove singularities. These features are consistent with theoretical predictions for a 3Q magnetic order near three-quarters band filling on a cobalt triangular lattice. These results provide evidence of 3Q magnetic order in the electronic structure, establishing TMD van der Waals magnets as tunable materials to explore the interplay between magnetism and topology.

Luo, Hai-Lan [University of California, Berkeley, ↗
DOE OSTI2021

Influence of magnetic angle on the E × B drift in a magnetic presheath

In this work, we provide experimental measurements of the E X B flow above a non-magnetic, absorbing boundary in a magnetized plasma. Measurements are taken as a function of the angle between the background magnetic field and the boundary normal. The measurements are compared to computational predictions for oblique magnetic fields based on Chodura's model. Ion flow measurements were obtained with laser induced fluorescence and the presheath potential structure was measured with an emissive probe. The ions were found to accelerate to nearly 30% of the sound speed parallel to the boundary at oblique angles of the magnetic field (~80°) and the ion speed at the electrostatic sheath edge was found to decrease with angle. The edge of the magnetic presheath has been experimentally determined based on the appearance of the E X B drift and is found to be independent of the angle of the magnetic field. We also demonstrate that laser induced fluorescence is suitable as a non-perturbative diagnostic to measure the electric field in a magnetized sheath.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2024

Magnetic vortex control with current-induced axial magnetization in centrosymmetric Weyl materials

We consider magnetic Weyl metals as a platform to achieve current control of magnetization textures with transport currents utilizing their underlying band geometry. We show that the transport current in a Weyl semimetal produces an axial magnetization due to orbital magnetic moments of the Weyl electrons. The associated axial magnetization can generate a torque acting on the localized magnetic moments. For the case of a magnetic vortex in a nanodisk of Weyl materials, this current-induced torque can be used to reverse its circulation and polarity. We discuss the axial magnetization torques in Weyl metals on general symmetry grounds and compare their strength to current-induced torques in more conventional materials.

Physics↗
DOE OSTI2025

Tuning magnetism in Ising-type van der Waals magnet FePS 3 by lithium intercalation

Recently, layered transition metal thiophosphate MPX 3 (M = transition metals, X = S or Se) have gained significant attention because of their rich magnetic, optical, and electronic properties. Specifically, the diverse magnetic structures and the robustness of magnetism in the two-dimensional (2D) limit have made them prominent candidates to study 2D magnetism. Numerous efforts such as substitutions and interlayer intercalations have been adopted to tune the magnetic properties of these materials, which has greatly deepened the understanding of the underlying mechanisms that govern the properties. In this work, we focus on modifying the magnetism of Ising-type antiferromagnet FePS 3 using electrochemical lithium intercalation. Furthermore, our work demonstrate the effectiveness of electrochemical intercalation as a controllable tool to modulating magnetism, including tuning magnetic ordering temperature and inducing low temperature spin-glass state, offering an approach for implementing this material into applications.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2023

Interplay between magnetism and band topology in the kagome magnets R Mn 6 Sn 6

Kagome-lattice magnets R Mn 6 Sn 6 recently emerged as a new platform to exploit the interplay between magnetism and topological electronic states. Some of the most exciting features of this family are the dramatic dependence of the easy magnetization direction on the rare-earth specie, despite other magnetic and electronic properties being essentially unchanged, and the kagome geometry of the Mn planes that in principle can generate flat bands and Dirac points; gapping of the Dirac points by spin-orbit coupling has been suggested recently to be responsible for the observed anomalous Hall response in the member TbMn 6 Sn 6 . In this paper, we address both issues with ab initio calculations. We have discovered the significant role played by higher-order crystal-field parameters and rare-earth magnetic anisotropy constants in these systems. Further, we demonstrate that the microscopic origin of rare-earth magnetic anisotropy can also be quantified and understood at various levels: ab initio, phenomenological, and analytical. In particular, using a simple and physically transparent analytical model based on perturbation theory, we are able to explain, with full quantitative agreement, the evolution of rare-earth magnetic anisotropy across the series. We analyze in detail the topological properties of Mn-dominated bands and demonstrate how they emerge from the multiorbital planar kagome model. We further show that, despite this fact, most of the topological features at the Brillouin zone corner K are strongly 3D and therefore cannot explain the observed quasi-2D anomalous Hall effect, while the most pronounced quasi-2D dispersion are too far removed from the Fermi level. By employing self-consistent calculations with ab initio many-body approaches, we demonstrate that the exchange-correlation effects beyond the density functional theory for itinerant Mn- d electrons do not significantly alter the obtained electronic and magnetic structure. Therefore, we conclude that, contrary to previous claims, the most pronounced 2D kagome-derived topological band features bear little relevance to transport in RMn 6 Sn 6 , albeit they may possibly be brought to focus by electron or hole doping.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2024

Magnetic properties of Lutetium and Yttrium doped Ce 2 Fe 14 B magnets

The increasing demand for Nd-Dy and Sm-Co based permanent magnets is exacerbating the current critical materials shortage, therefore improving and optimizing current candidate critical element free permanent magnets is necessary to develop future clean energy technologies. In this work, we aim to increase the thermal stability and magnetic performance of Ce 2 Fe 14 B based permanent magnets through the substitution of Ce ions with noncritical rare earth elements Lu and Y. The substitution of Lu (x=0; 0.05; 0.1; 0.15) for Ce ions in (LuxCe 2-x )Fe 14 B was unsuccessful, likely due to disparities in ionic size and valencies, and failed to exhibit improved thermal stability or magnetic performance. In contrast, Y substitution for Ce ions in (Y x Ce 2-x )Fe14B (x= 0.1; 0.2; 0.3; 0.4; 0.5) alloys was successful. Notably, these alloys demonstrated enhanced thermal stability, as evidenced by an increase in the Curie temperature, reaching a peak of 443 K at x= 0.5. Y substitution also helped to suppress the CeFe2 Laves phase. Without loss of the anisotropy field Y substitution increased the saturation magnetization, MS, peaking at MS = 125 emu/g for a Y concentration of x= 0:4, demonstrating (Y 0.4 Ce 1.6 )Fe 14 B as a potential critical element free permanent magnet with an energy product as high as 29 MGOe. This work is advantageous in developing low cost high performance permanent magnets with reduced or little to no critical rare earth elements.

Rai, Binod K.↗
NASA NTRS1974

Magnetization and magnetic entropy of Dy2Ti2O7

Isothermal measurements of the magnetic entropy, magnetization, and differential susceptibility of Dy2Ti2O7 have been made. Absolute values of magnetic entropy have been determined as a function of applied magnetic field for several temperatures in the range 2-20 K, and several isofield lines in the magnetic entropy-temperature plane have been determined. Magnetization measurements, which extended into the saturation region, yield a powder-average magnetic moment of about 4.7 Bohr magnetons per ion. A van Vleck contribution to M was also observed. The results are consistent with the assumption of a nearly pure Jz equals + or - 15/2 ground-state Kramers doublet for the Dy(+++) ion. Comments on the suitability of Dy2Ti2O7 for use in a magnetic refrigerator cycling between 4.2 and 20 K are included.

Flood, D. J.↗
NASA NTRS1990

Nonlogarithmic magnetization relaxation at the initial time intervals and magnetic field dependence of the flux creep rate in Bi2Sr2Ca(sub I)Cu2Ox single crystals

At the initial time intervals, preceding the thermally activated flux creep regime, fast nonlogarithmic relaxation is found. The fully magnetic moment Pm(t) relaxation curve is shown. The magnetic measurements were made using SQUID-magnetometer. Two different relaxation regimes exist. The nonlogarithmic relaxation for the initial time intervals may be related to the viscous Abrikosov vortices flow with j is greater than j(sub c) for high enough temperature T and magnetic field induction B. This assumption correlates with Pm(t) measurements. The characteristic time t(sub O) separating two different relaxation regimes decreases as temperature and magnetic field are lowered. The logarithmic magnetization relaxation curves Pm(t) for fixed temperature and different external magnetic field inductions B are given. The relaxation rate dependence on magnetic field, R(B) = dPm(B, T sub O)/d(1nt) has a sharp maximum which is similar to that found for R(T) temperature dependences. The maximum shifts to lower fields as temperature goes up. The observed sharp maximum is related to a topological transition in shielding critical current distribution and, consequently, in Abrikosov vortices density. The nonlogarithmic magnetization relaxation for the initial time intervals is found. This fast relaxation has almost an exponentional character. The sharp relaxation rate R(B) maximum is observed. This maximum corresponds to a topological transition in Abrikosov vortices distribution.

Moshchalcov, V. V.↗
NASA NTRS1991

Makeup and uses of a basic magnet laboratory for characterizing high-temperature permanent magnets

A set of instrumentation for making basic magnetic measurements was assembled in order to characterize high intrinsic coercivity, rare earth permanent magnets with respect to short term demagnetization resistance and long term aging at temperatures up to 300 C. The major specialized components of this set consist of a 13 T peak field, capacitor discharge pulse magnetizer; a 10 in. pole size, variable gap electromagnet; a temperature controlled oven equipped with iron cobalt pole piece extensions and a removable paddle that carries the magnetization and field sensing coils; associated electronic integrators; and sensor standards for field intensity H and magnetic moment M calibration. A 1 cm cubic magnet sample, carried by the paddle, fits snugly between the pole piece extensions within the electrically heated aluminum oven, where fields up to 3.2 T can be applied by the electromagnet at temperatures up to 300 C. A sample set of demagnetization data for the high energy Sm2Co17 type of magnet is given for temperatures up to 300 C. These data are reduced to the temperature dependence of the M-H knee field and of the field for a given magnetic induction swing, and they are interpreted to show the limits of safe operation.

Niedra, Janis M.↗
NASA NTRS1992

Venus internal magnetic field and its interaction with the interplanetary magnetic field

In a previous study, Knudsen et al. suggested that Venus has a weak internal magnetic dipole field of the order of 7 x 10 + 20 G cm(exp -3) that is manifested in the form of magnetic flux tubes threading the ionospheric holes in the Venus nightside ionosphere. They pointed out that any internal field of Venus, dipole or multipole, would be weakened in the subsolar region and concentrated in the antisolar region of the planet by the supersonic transterminator convection of the dayside ionosphere into the nightside hemisphere. The inferred magnitude of the dipole field does not violate the upper limit for an internal magnetic field established by the Pioneer Venus magnetometer experiment. The most compelling objection to the model suggested by Knudsen et al. has been the fact that it does not explain the observed interplanetary magnetic field (IMF) control of the polarity of the ionospheric hole flux tubes. In this presentation I suggest that a magnetic reconnection process analogous to that occurring at earth is occurring at Venus between the IMF and a weak internal dipole field. At Venus in the subsolar region, the reconnection occurs within the ionosphere. At Earth it occurs at the magnetopause. Reconnection will occur only when the IMF has an appropriate orientation relative to that of the weak internal field. Thus, reconnection provides a process for the IMF to control the flux tube polarity. The reconnection in the subsolar region takes place in the ionosphere as the barrier magnetic field is transported downward into the lower ionosphere by downward convection of ionospheric plasma and approaches the oppositely directed internal magnetic field that is diffusing upward. The reconnected flux tubes are then transported anti-Sunward by the anti-Sunward convecting ionospheric plasma as well as by the anti-Sunward-flowing solar wind. Reconnection will also occur in the Venus magnetic tail region, somewhat analogously to the reconnection that occurs in the magnetotail of the Earth. The possibility that reconnection is occurring between the IMF and an internal dipole field may be tested by measuring the orientation of the IMF projected into a plane perpendicular to the solar wind velocity during time intervals for which ionospheric holes are observed. The orientations of the IMV components should fall within a 180 deg angle.

Knudsen, W. C.↗