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DOE OSTI2021

Search for the rare decay of the W boson into a pion and a photon in proton-proton collisions at $ \sqrt{s}$=13TeV

A search is performed for the rare decay W ± → π ± γ in proton-proton collisions at s = 13 TeV . Data corresponding to an integrated luminosity of 137 fb - 1 were collected during 2016 to 2018 with the CMS detector. This analysis exploits a novel search strategy based on W boson production in top quark pair events. An inclusive search for the W ± → π ± γ decay is not optimal at the LHC because of the high trigger thresholds. Instead, a trigger selection is exploited in which the W boson originating from one of the top quarks is used to tag the event in a leptonic decay. The W boson emerging from the other top quark is used to search for the W ± → π ± γ signature. Such decays are characterized by an isolated track pointing to a large energy deposit, and by an isolated photon of large transverse momentum. The presence of b quark jets reduces the background from the hadronization of light-flavor quarks and gluons. The W ± → π ± γ decay is not observed. An upper exclusion limit is set to this branching fraction, corresponding to 1.50 × 10 - 5 at 95% confidence level, whereas the expected upper exclusion limit is 0.85 - 0.29 + 0.52 × 10 - 5 .

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2024

Search for Rare Decays of D s + to Final States π + e + e − , ρ + e + e − , π + π 0 e + e − , K + π 0 e + e − , and K S 0 π + e + e −

Using 7.33 fb − 1 of e + e − collision data collected by the BESIII detector at center-of-mass energies in the range of s = 4.128 – 4.226 GeV , we search for the rare decays D s + → h + ( h 0 ) e + e − , where h represents a kaon or pion. By requiring the e + e − invariant mass to be consistent with a ϕ ( 1020 ) , 0.98 < M ( e + e − ) < 1.04 GeV / c 2 , the decay D s + → π + ϕ , ϕ → e + e − is observed with a statistical significance of 7.8 σ , and evidence for the decay D s + → ρ + ϕ , ϕ → e + e − is found for the first time with a statistical significance of 4.4 σ . The decay branching fractions are measured to be B ( D s + → π + ϕ , ϕ → e + e − ) = ( 1.1 7 − 0.21 + 0.23 ± 0.03 ) × 10 − 5 , and B ( D s + → ρ + ϕ , ϕ → e + e − ) = ( 2.4 4 − 0.62 + 0.67 ± 0.16 ) × 10 − 5 , where the first uncertainties are statistical and the second systematic. No significant signals for the three four-body decays of D s + → π + π 0 e + e − , D s + → K + π 0 e + e − , and D s + → K S 0 π + e + e − are observed. For D s + → π + π 0 e + e − , the ϕ mass region is vetoed to minimize the long-distance effects. The 90% confidence level upper limits set on the branching fractions of these decays are in the range of ( 7.0 – 8.1 ) × 10 − 5 . Published by the American Physical Society 2024

Physics↗

DOE OSTI2022

Search for invisible Higgs-boson decays in events with vector-boson fusion signatures using 139 fb -1 of proton-proton data recorded by the ATLAS experiment

A direct search for Higgs bosons produced via vector-boson fusion and subsequently decaying into invisible particles is reported. The analysis uses 139 fb -1 of pp collision data at a centre-of-mass energy of $\sqrt{s}$ = 13 TeV recorded by the ATLAS detector at the LHC. The observed numbers of events are found to be in agreement with the background expectation from Standard Model processes. For a scalar Higgs boson with a mass of 125 GeV and a Standard Model production cross section, an observed upper limit of 0.145 is placed on the branching fraction of its decay into invisible particles at 95% confidence level, with an expected limit of 0.103. These results are interpreted in the context of models where the Higgs boson acts as a portal to dark matter, and limits are set on the scattering cross section of weakly interacting massive particles and nucleons. Invisible decays of additional scalar bosons with masses from 50 GeV to 2 TeV are also studied, and the derived upper limits on the cross section times branching fraction decrease with increasing mass from 1.0 pb for a scalar boson mass of 50 GeV to 0.1 pb at a mass of 2 TeV.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2024

Search for ∆S = 2 nonleptonic hyperon decays Ω− → Σ0π− and Ω− → nK−

Abstract Using (27.12 ± 0.14) × 10 8 ψ(3686) events collected by the BESIII detector at the center-of-mass energy of$$ \sqrt{s} $$ s = 3.686 GeV, we search for the first time for two nonleptonic hyperon decays that change strangeness by two units, Ω − → Σ 0 π − and Ω − →nK − . No significant signal is observed. The upper limits on their decay branching fractions are determined to be$$ \mathcal{B} $$ B (Ω − → Σ 0 π − )<5.4 × 10 −4 and$$ \mathcal{B} $$ B (Ω − →nK − )<2.4 × 10 −4 at the 90% confidence level.

Physics↗

DOE OSTI2023

Search for the semi-leptonic decays Λ c + → Λ π + π - e + ν e and Λ c + → p K S 0 π - e + ν e

We search for the semi-leptonic decays $Λ^+_c$ → Λπ + π - e + ν e and $Λ^+_c$ → p$K^0_S$π - e + ν e in a sample of 4.5 fb -1 of e + e - annihilation data collected in the center-of-mass energy region between 4.600 GeV and 4.699 GeV by the BESIII detector at the BEPCII. No significant signals are observed, and the upper limits on the decay branching fractions are set to be B($Λ^+_c$ → Λπ + π - e + ν e ) < 3.9 × 10 -4 and B($Λ^+_c$ → p$K^0_S$π - e + ν e ) < 3.3 × 10 -4 at the 90% confidence level, respectively

$Λ^+_c$↗

DOE OSTI2024

Searches for exclusive Higgs boson decays into D *$\gamma$ and Z boson decays into D 0 $\gamma$ and K $^{0}_{s}$$\gamma$ in pp collisions at $\sqrt{s}$ = 13 TeV with the ATLAS detector

Searches for exclusive decays of the Higgs boson into D*$\gamma$ and of the Z boson into D 0 $\gamma$ and K$_{s}^{0}$$\gamma$ can probe flavour-violating Higgs boson and Z boson couplings to light quarks. Searches for these decays are performed with a pp collision data sample corresponding to an integrated luminosity of 136.3 fb -1 collected at $\sqrt{s}$ = 13TeV between 2016–2018 with the ATLAS detector at the CERN Large Hadron Collider. In the D*$\gamma$ and D 0 $\gamma$ channels, the observed (expected) 95% confidence-level upper limits on the respective branching fractions are B(H→D*$\gamma$) < 1.0(1.2)×10 -3 , B(Z→D 0 $\gamma$) < 4.0(3.4)×10 -6 , while the corresponding results in the K$_{s}^{0}$$\gamma$ channel are B(Z→K$_{s}^{0}$$\gamma$) < 3.1(3.0)×10 -6 .

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2026

Confinement-Controlled Rearrangements in Dioxolane Upgrading on H-ZSM-5 Revealed by Periodic DFT

Zeolitic Brønsted acid sites catalyze carbocation rearrangements central to upgrading biomass-derived oxygenates. Here we elucidate the mechanism of dioxolane conversion to methyl ethyl ketone and isobutanal on H-ZSM-5 using periodic density functional theory on the MFI model, complemented by ab initio molecular dynamics to probe confinement effects. Dioxolane adsorption at the Brønsted site is followed by protonation-assisted ring opening to form an oxocarbenium intermediate stabilized by the deprotonated framework. From this common intermediate, selectivity is governed by two competing rearrangements, namely, the 1,2-hydride shift with a free-energy barrier of 18.05 kcal mol –1 at 498 K leading toward MEK, and the 1,2-methyl shift with a higher barrier of 25.40 kcal mol –1 leading toward isobutanal. The hydride-shift channel is kinetically preferred over the methyl-shift channel, lowering the isobutanal/MEK ratio below the 3:1 limit expected for equal branching. Adsorption thermodynamics further indicate stronger stabilization of MEK than isobutanal within ZSM-5 channels, suggesting that confinement-controlled binding can bias product distributions in addition to intrinsic rearrangement barriers. These results highlight how Brønsted acidity and pore confinement jointly shape the rearrangement landscape in MFI zeolites.

adsorption↗

DOE OSTI2020

Wave function analysis with a maximum flow algorithm

An efficient algorithm for computing the maximum-flow path in a network is applied to the identification of the dominant configuration state functions (CSFs) in a graphically contracted function (GCF), configuration interaction, wave function. The flow network is a space of spin-adapted CSFs represented by a Shavitt graph, wherein the nodes correspond to orbital occupations and spin quantum numbers. The graph nodes are connected by arcs, and an arc density is defined as sums of the associated squared CSF coefficients. A max-min approach determines an upper bound to the maximum possible incoming flow for each graph node. A backtracking step generates a candidate walk and is followed by a limited search of alternative branching paths for the dominant CSF. The arc density contributions are removed from the graph, and the algorithm is reapplied to the updated graph. This list of generated walks can be partitioned in order to guarantee that the dominant CSFs have been identified. All of the steps in this algorithm are computationally efficient and do not depend on the potentially large dimension of the underlying linear CSF expansion space. An analysis of low-lying valence states of C-2 illustrates the method.

74 ATOMIC AND MOLECULAR PHYSICS↗

DOE OSTI2024

Search for η c ( 2 S ) → π + π − η c and η c ( 2 S ) → π + π − K S 0 K ± π ∓ decays

Based on ( 27.12 ± 0.14 ) × 10 8 ψ ( 2 S ) events collected by the BESIII detector, we search for the decay η c ( 2 S ) → π + π − η c via ψ ( 2 S ) → γ η c ( 2 S ) . No significant signal is observed, and the upper limit on the product branching fraction B ( ψ ( 2 S ) → γ η c ( 2 S ) ) × B ( η c ( 2 S ) → π + π − η c ) is determined to be 2.21 × 10 − 5 at the 90% confidence level. In addition, the η c ( 2 S ) → π + π − K S 0 K ± π ∓ decay is studied via ψ ( 2 S ) → γ η c ( 2 S ) and is observed with a statistical significance of 10 σ for the first time. The branching fraction of η c ( 2 S ) → π + π − K S 0 K ± π ∓ is determined to be ( 1.33 ± 0.11 ± 0.40 ± 0.95 ) × 10 − 2 , where the first uncertainty is statistical, the second is systematic, and the third uncertainty is due to the quoted B ( ψ ( 2 S ) → γ η c ( 2 S ) ) . Published by the American Physical Society 2024

Astronomy & Astrophysics↗

DOE OSTI2025

Search for η c ( 2 S ) → ω ω and ω ϕ and measurements of χ c J → ω ω and ω ϕ in ψ ( 2 S ) radiative processes

Using ( 2712 ± 14 ) × 10 6 ψ ( 2 S ) events collected with the BESIII detector at the BEPCII collider, we search for the decays η c ( 2 S ) → ω ω and η c ( 2 S ) → ω ϕ via the process ψ ( 2 S ) → γ η c ( 2 S ) . No statistically significant signals are observed. The upper limits of their product branching fractions at the 90% confidence level are determined to be B ( ψ ( 2 S ) → γ η c ( 2 S ) , η c ( 2 S ) → ω ω ) < 1.04 × 10 − 6 and B ( ψ ( 2 S ) → γ η c ( 2 S ) , η c ( 2 S ) → ω ϕ ) < 1.85 × 10 − 7 , respectively. We also update the branching fractions of χ c J → ω ω and χ c J → ω ϕ via the ψ ( 2 S ) → γ χ c J transition. Their branching fractions are determined to be B ( χ c 0 → ω ω ) = ( 10.66 ± 0.11 ± 0.57 ) × 10 − 4 , B ( χ c 1 → ω ω ) = ( 6.43 ± 0.07 ± 0.31 ) × 10 − 4 , B ( χ c 2 → ω ω ) = ( 8.75 ± 0.08 ± 0.42 ) × 10 − 4 , B ( χ c 0 → ω ϕ ) = ( 1.18 ± 0.03 ± 0.07 ) × 10 − 4 , B ( χ c 1 → ω ϕ ) = ( 2.04 ± 0.15 ± 0.11 ) × 10 − 5 , and B ( χ c 2 → ω ϕ ) = ( 9.58 ± 1.07 ± 0.76 ) × 10 − 6 , where the first uncertainties are statistical and the second are systematic. Published by the American Physical Society 2025

Ablikim, M.↗

DOE OSTI2023

Search for Lepton-Flavor-Violating τ Decays to a Lepton and an Invisible Boson at Belle II

We search for lepton-flavor-violating $τ^– \rightarrow e^–α$ $τ^– \rightarrow μ^–α$ decays, where α is an invisible spin-0 boson. The search uses electron-positron collisions at 10.58 GeV center-of-mass energy with an integrated luminosity of 62.8 fb –1 , produced by the SuperKEKB collider and collected with the Belle II detector. We search for an excess in the lepton-energy spectrum of the known $τ^–\rightarrow e^–\bar{v}_{e}v_τ$ decays. We report 95% confidence-level upper limits on the branching-fraction ratio $\mathscr{B}(τ^–\rightarrow e^–α) \ / \mathscr{B}(τ^–\rightarrow e^– \bar{v}_{e}v_τ)$ in the range (1.1-9.7) × 10 –3 and on $\mathscr{B}(τ^–\rightarrow μ^–α) \ / \mathscr{B}(τ^–\rightarrow μ^– \bar{v}_{μ}v_τ)$ in the range (0.7-12.2)×10 –3 for α masses between 0 and 1.6 GeV/c 2 . These results provide the most stringent bounds on invisible boson production from τ decays.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

NASA NTRS1972

Process for synthesizing and formulating condensed ring polymers

Chemical process for forming low molecular weight, fully cyclized heteroaromatic prepolymers under conditions which limit chain extension or branching is described. Exact procedures used in conducting chemical reaction are defined. Advantages of process over conventional methods are presented.

Hughes, C. T.↗

NASA NTRS1995

Stellar photometry in the inner bulge of M31 using the Hubble Space Telescope wide field camera

We present photometry of two fields in the M31 bulge imaged with the Hubble Space Telescope (HST) Wide-Field Camara (WFC). The nuclear field (r less than 40 arcsecs = 150 pc) giant branch extends to I = 19.5, M(sub I) = -5 (Cousins system), a full 0.9 mag brighter than the giant-branch tips of metal-poor Galactic globular clusters and M31 halo fields. This is also approximately = 1.5 mag brighter than the giant branches of metal-rich Galactic globular clusters, but is no brighter than Mould's (1986) M31 bulge field 1 kpc from the nucleus. The data also suggest that the brighter stars may be preferentially concentrated to the center. The 648 luminous stars detected in 2 x 10(exp 9) solar luminosity is approximately = 25% that expected from a hypothetical population of evolved asymptotic giant branch (AGB) stars with lifetimes approximately = 10(exp 5) yr, with the cautionary note that we are near the detection limit. The number of bright stars is also consistent with the progeny of blue stragglers, if one uses a lifetime for the thermal-pulsing AGB of 2 x 10(exp 6) yr. We strongly caution that incompleteness becomes severe below I = 19.9 mag and that future surveys are likely to find numbers of bright stars too large to accomodate the blue straggler progeny hypothesis. We have imaged an additional field 2 arcmin = 500 pc south of the nucleus. The brightest stars in this field are also I = 19.5, but bright stars appear less numerous than in the nuclear field. If the population resembles that of the Galactic bulge, then M(sub bol) = -4.5 is a lower limit to the giant-branch tip luminosity; infrared studies should reveal stars 0.5 mag or more brighter. Either high-metallicity or (more likely) age approximately = 10 Gyr may be responsible for the presence of these luminous AGB stars. These observations confirm that previous ground-based infrared studies (e.g., Rich & Mould 1991) very likely detect an extended giant branch and not spurious luminous stars caused by crowding or disk contamination. However, published integrated colors for the M31 bulge/nucleus are extremely red, making it difficult to accomodate a young or intermediate-age population.

Rich, R. M.↗

NASA NTRS2000

(BOREAS) BOREAS TE-8 Aspen Bark Chemistry Data

The BOREAS TE-8 team collected pigment density data from aspen bark and leaves from four sites within the BOREAS SSA from 24-May-1994 to 16-Jun-1994 (IFC-1), 19-Jul-1994 to 08-Aug- 1994 (IFC-2), and 30-Aug-1994 to 19-Sep-1994 (IFC-3). One to nine trees from each site were sampled during the three IFCs. Each tree was sampled in five different locations for bark pigment properties: basal stem section, which was any bark sample taken below one-half the tree height; upper stem section, which was any bark sample taken from the main stem above one-half the tree height; bark taken from branches up to 3 years old; a 2-year-old branch segment, and a 1-year-old branch segment. Additionally, a limited number of leaves were collected. Bark samples were removed from the stem of the tree, placed in ziplock bags, and transported to UNH, where they were processed and analyzed by a spectrophotometer. In each data file, samples are identified by Site, Date, Tree#, and Sample Location (see I st paragraph above. Pigment density values are normalized to mg/m2. Density values for the following pigments are provided: Chi a, Chi b, Total Chi (Chi a+b), Carotenoids, Chi a to b ratio, and the Total Chi to carotenoids ratio. The data are stored in ASCII files. The data files are available on a CD-ROM (see document number 20010000884), or from the Oak Ridge National Laboratory (ORNL) Distrobuted Activity Archive Center (DAAC).

Hall, Forrest G.↗

NASA NTRS2014

Cloud Retrieval Intercomparisons Between SEVIRI, MODIS and VIIRS with CHIMAERA PGE06 Data Collection 6 Products

The Cross-platform HIgh resolution Multi-instrument AtmosphEric Retrieval Algorithms (CHIMAERA) system allows us to perform MODIS-like cloud top, optical and microphysical properties retrievals on any sensor that possesses a minimum set of common spectral channels. The CHIMAERA system uses a shared-core architecture that takes retrieval method out of the equation when intercomparisons are made. Here we show an example of such retrieval and a comparison of simultaneous retrievals done using SEVIRI, MODIS and VIIRS sensors. All sensor retrievals are performed using CLAVR-x (or CLAVR-x based) cloud top properties algorithm. SEVIRI uses the SAF_NWC cloud mask. MODIS and VIIRS use the IFF-based cloud mask that is a shared algorithm between MODIS and VIIRS. The MODIS and VIIRS retrievals are performed using a VIIRS branch of CHIMAERA that limits available MODIS channel set. Even though in that mode certain MODIS products such as multilayer cloud map are not available, the cloud retrieval remains fully equivalent to operational Data Collection 6.

cloud retrieval↗

DOE OSTI2022

DOE new players Carbon cycle (2016-2021)

The overarching scientific goals of our multidisciplinary grant was to further expand understanding about the key microorganisms (players), metabolic strategies (processes), and interspecies relationships (interactions) involved in the formation and oxidation of methane in the environment. This research applied novel environmental metagenomics, transcriptomics, and proteomic techniques, state-of-the-art analytical imaging, stable isotope geochemistry, and reaction-transport modeling to address these goals and develop an ‘ecosystems level’ understanding of the factors which regulate microbial methane cycling in anoxic sedimentary ecosystems. For decades, it was believed that the obligate step in methanogenesis catalyzed by methyl coenzyme M reductase (Mcr) was limited to a specific branch of the archaeal Domain, formerly known as the Euryarchaeota. Less than a decade ago co-I Tyson’s team published a surprising metagenomic-based discovery of divergent Mcr genes in a novel uncultured phylum (Bathyarchaeota), catalyzing a major shift in thinking about the diversity of microorganisms that encode the potential for methane (or higher alkane) metabolism in anoxic environments (Evans et al., 2015). In our work here, we further expand on the groups of archaea harboring the genomic potential for methane or hydrocarbon metabolism using environmental metagenomics and new gene targeted bioinformatics techniques. We additionally advanced understanding about the terminal electron acceptors and metabolic potential supporting the anaerobic oxidation of methane (AOM) in terrestrial ecosystems, specifically focused on new lineages of ANME archaea capable of respiring manganese oxides with methane presumably using large extracellular multi-heme cytochrome complexes. New details about specific syntrophic mechanisms underlying the exchange of electrons during sulfate-coupled methane oxidation between ANME-2 archaea and their sulfate-reducing bacterial partners were also elucidated as part of this funded project. Through a series of experimental ‘omics and single cell stable isotope probing studies with incubated environmental sediment samples and a cultured model electrogenic microorganism combined with model-based predictions. Combined, this work provides strong support for the hypothesis of direct interspecies electron transfer (DIET) is the dominant syntrophic mechanism controlling the anaerobic oxidation of methane with sulfate over other proposed mechanisms and additionally illustrates important spatial constraints and the underlying physico-chemical factors influencing AOM syntrophic consortia structure for DIET and extracellular metal respiration. This collaborative multi-institutional project successfully advanced several of our milestone goals including the identification of new microbial players containing methyl coenzyme M reductases hypothesized to be central to methane or hydrocarbon cycling in anoxic environments and enhancing fundamental knowledge about the role extracellular electron transfer plays in the ecophysiology of methanotrophic archaea respiring metal oxides and in the physical and metabolic structuring of syntrophic interactions in methane-rich sedimentary ecosystems.

03 NATURAL GAS↗

DOE OSTI2023

Search for pair-produced vector-like top and bottom partners in events with large missing transverse momentum in $pp$ collisions with the ATLAS detector

A search for pair-produced vector-like quarks using events with exactly one lepton ($e$ or $μ$), at least four jets including at least one $b$-tagged jet, and large missing transverse momentum is presented. Data from proton–proton collisions at a centre-of-mass energy of $\sqrt{s}$ = 13 TeV, recorded by the ATLAS detector at the LHC from 2015 to 2018 and corresponding to an integrated luminosity of 139 fb –1 , are analysed. Vector-like partners $T$ and $B$ of the top and bottom quarks are considered, as is a vector-like $X$ with charge +5/3, assuming their decay into a $W$, $Z$, or Higgs boson and a third-generation quark. No significant deviations from the Standard Model expectation are observed. Upper limits on the production cross-section of $T$ and $B$ quark pairs as a function of their mass are derived for various decay branching ratio scenarios. The strongest lower limits on the masses are 1.59 assuming mass-degenerate vector-like quarks and branching ratios corresponding to the weak-isospin doublet model, and 1.47 TeV (1.46 TeV) for exclusive $T$→$Zt$ ($B/X$→$Wt$) decays. In addition, lower limits on the $T$ and $B$ quark masses are derived for all possible branching ratios.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2024

Search for a scalar or pseudoscalar dilepton resonance produced in association with a massive vector boson or top quark-antiquark pair in multilepton events at s = 13 TeV

A search for beyond the standard model spin-0 bosons, ϕ , that decay into pairs of electrons, muons, or tau leptons is presented. The search targets the associated production of such bosons with a W or Z gauge boson, or a top quark-antiquark pair, and uses events with three or four charged leptons, including hadronically decaying tau leptons. The proton-proton collision data set used in the analysis was collected at the LHC from 2016 to 2018 at a center-of-mass energy of 13 TeV, and corresponds to an integrated luminosity of 138 fb - 1 . The observations are consistent with the predictions from standard model processes. Upper limits are placed on the product of cross sections and branching fractions of such new particles over the mass range of 15 to 350 GeV with scalar, pseudoscalar, or Higgs-boson-like couplings, as well as on the product of coupling parameters and branching fractions. Several model-dependent exclusion limits are also presented. For a Higgs-boson-like ϕ model, limits are set on the mixing angle of the Higgs boson with the ϕ boson. For the associated production of a ϕ boson with a top quark-antiquark pair, limits are set on the coupling to top quarks. Finally, limits are set for the first time on a fermiophilic dilaton-like model with scalar couplings and a fermiophilic axion-like model with pseudoscalar couplings.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗