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At least 127 records · Page 7

Probing electron-hole coherence in strongly driven 2D materials using high-harmonic generation

Under strong electromagnetic excitation, electron–hole (e-h) pairs may be generated in solids, which are subsequently driven to high energy and high momentum, producing high harmonics (HH) of the driving field. The HH efficiency depends on the degree of coherence between the driven electron and hole created by the laser field. Here, we disrupt this e-h coherence in an atomically thin semiconductor by photodoping via incoherent e-h pairs. We observe a strong, systematic harmonic order-dependent intensity reduction. This trend is explained by an exponential decay of the inter-band polarization, proportional to the sub-cycle excursion time of the e-h pair. Our study provides a platform to probe the importance of many-body effects, such as excitation density-dependent decoherence time for strongly driven electrons without the need of ultrashort laser pulses.

74 ATOMIC AND MOLECULAR PHYSICS↗

Stress waves in an isotropic elastic plate excited by a circular transducer

Steady state harmonic stress waves in an isotropic elastic plate excited on one face by a circular transducer are analyzed theoretically. The transmitting transducer transforms an electrical voltage into a uniform normal stress at the top of the plate. To solve the boundary value problem, the radiation into a half-space is considered. The receiving transducer produces an electrical voltage proportional to the average spatially integrated normal stress over its face due to an incident wave. A numerical procedure is given to evaluate the frequency response at a receiving point due to a multiply reflected wave in the near field. Its stability and convergence are discussed. Parameterization plots which determine the particular wave whose frequency response has maximum magnitude compared with other multiple reflected waves are given for a range of values of dimensionless parameters. The effects of changes in the values of the parameters are discussed.

Karagulle, H.↗

Effects of low-frequency voltage on nonlinear standing wave excitation, plasma uniformity, and ion dynamics in dual-frequency asymmetric capacitive discharges

Abstract It is known that in very-high-frequency (VHF) capacitively coupled plasmas, the higher harmonics generated by nonlinear sheath motion can enhance the standing wave effect (SWE), which can lead to center-peaked plasma density profiles. In this work, an improved nonlinear electromagnetic model incorporating a transmission line model, an electron momentum balance model, a bulk plasma model, a collisionless nonlinear numerical sheath model, and an ion Monte-Carlo collision (MCC) model is developed to study the effects of low-frequency (LF) voltage V L on the nonlinear standing wave excitation, plasma uniformity, and ion energy and angular distribution functions (IEDFs and IADFs) in dual-frequency (DF) asymmetric capacitive argon discharges at relatively low pressure of 3 Pa. The plasma diffusion in the radial direction and ion dynamics within the LF oscillating sheath are self-consistently considered. The LF voltage V L at 2 MHz varies from 0 to 700 V while the HF voltage V H at 60 MHz is fixed at 100 V. Simulation results indicate that without the addition of an LF source (i.e. V L = 0 V), there are a considerable number of high-order harmonics with short wavelengths, leading to significant SWE and central peak in the radial plasma density profile. Nevertheless, the high-order harmonic excitations tend to be weakened and merely occur around the phase of the full LF sheath collapse due to a shorter characteristic damping time of the surface waves as V L increases. This, combined with increased surface wavelengths of both the driving frequency and the higher harmonics at a higher V L , leads to suppressed standing waves and improved plasma uniformity. Meanwhile, the simulations show that both the low and the high energy peaks of IEDF move towards higher energies, and the energy peak separation width ΔEbecomes wider with the increase of V L . The IEDF at the radial center of the powered electrode exhibits a broader ΔEthan that at the edge. For the IADF, an increased V L results in more ions incident on the electrode with a smaller deflection angle. Because of a thinner sheath and a higher sheath voltage at the electrode center, the peak value of IADF at the electrode center is greater than that at the edge.

Physics↗

A theoretical study of the excited states of Ag3

Calculations of the excited states of the Ag3 molecule are reported. The excitation energies, geometries, derived harmonic frequencies, and transition moments are given and discussed. The results of other calculations of the excited states are reviewed and assessed.

Walch, Stephen P.↗

Brushless Excitation for Wound-field Synchronous Machines using Multi-harmonic Windings

Wound-field synchronous machines (WFSM) are promising alternatives to electric machines with permanent magnets (PM). The ability to control the rotor field in these machines makes them well-suited to safety critical applications, while the absence of rare-earth permanent magnets makes these machines sustainable. The WFSM rotor excitation schemes have traditionally used carbon brushes, which significantly reduces the reliability of these machines, limiting their widespread adoption. To overcome this limitation and improve the reliability of WFSMs, several brushless rotor excitation schemes have been developed. However, most of these systems require additional windings or dedicated power electronics, making them expensive and limiting achievable power-density. In this paper a new brushless excitation scheme is proposed. In this scheme, a multiphase, multi-harmonic stator winding is designed. This winding can independently control two spatial harmonics in the airgap of the machine; the first to create torque and the second to wirelessly transfer power to the rotor to excite it.

Gadiyar, Nishanth [ORNL] (ORCID:0000000348267524)↗

On the effect of acoustic coupling on random and harmonic plate vibrations

The effect of acoustic coupling on random and harmonic plate vibrations is studied using two numerical models. In the coupled model, the plate response is obtained by integration of the nonlinear plate equation coupled with the nonlinear Euler equations for the surrounding acoustic fluid. In the uncoupled model, the nonlinear plate equation with an equivalent linear viscous damping term is integrated to obtain the response of the plate subject to the same excitation field. For a low-level, narrow-band excitation, the two models predict the same plate response spectra. As the excitation level is increased, the response power spectrum predicted by the uncoupled model becomes broader and more shifted towards the high frequencies than that obtained by the coupled model. In addition, the difference in response between the coupled and uncoupled models at high frequencies becomes larger. When a high intensity harmonic excitation is used, causing a nonlinear plate response, both models predict the same frequency content of the response. However, the level of the harmonics and subharmonics are higher for the uncoupled model. Comparisons to earlier experimental and numerical results show that acoustic coupling has a significant effect on the plate response at high excitation levels. Its absence in previous models may explain the discrepancy between predicted and measured responses.

Frendi, A.↗

Effect of acoustic coupling on random and harmonic plate vibrations

The effect of acoustic coupling on random and harmonic plate vibrations is studied using two numerical models. In the coupled model, the plate response is obtained by integration of the nonlinear plate equation coupled with the nonlinear Euler equations for the surrounding acoustic fluid. In the uncoupled model, the nonlinear plate equation with an equivalent linear viscous damping term is integrated to obtain the response of the plate subject to the same excitation field. For a low-level, narrow-band excitation, the two models predict the same plate response spectra. As the excitation level is increased, the response power spectrum predicted by the uncoupled model becomes broader and more shifted towards the high frequencies than that obtained by the coupled model. In addition, the difference in response between the coupled and uncoupled models at high frequencies becomes larger. When a high intensity harmonic excitation is used, causing a nonlinear plate response, both models predict the same frequency content of the response. However, the level of the harmonics and subharmonics are higher for the uncoupled model. Comparisons to earlier experimental and numerical results show that acoustic coupling has a significant effect on the plate response at high excitation levels. Its absence in previous models may explain the discrepancy between predicted and measured responses.

Frendi, Abdelkader↗

High-order harmonic generation in solid C 60

High-order harmonic generation (HHG) has unleashed the power of strong laser physics in solids. Here we investigate HHG from a large system, solid C 60 , with 240 valence electrons engaging harmonic generation at each crystal momentum. We employ the density functional theory and the time-dependent Liouville equation of the density matrix to compute HHG signals. We find that under a moderately strong laser pulse, HHG signals reach 15th order, consistent with the experimental results from C 60 plasma. The helicity dependence in solid C 60 is weak, due to the high symmetry. In contrast to the general belief, HHG is unsuitable for band structure mapping in C 60 . However, we find a window of opportunity using a long wavelength, where harmonics are generated through multiple-photon excitation. In particular, the fifth-order harmonic energies closely follow the transition energy dispersion between the valence and conduction bands. Finally, this finding is expected to motivate future experimental investigations.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

A mechanism for plasma waves at the harmonics of the plasma frequency foreshock boundary

A bump-on-tail unstable reduced velocity distribution, constructed from data obtained at the upstream boundary of the electron foreshock by the GSFC electron spectrometer experiment on the ISEE-1 satellite, is used as the initial plasma state for a numerical integration of the 1D-Vlasov-Maxwell system of equations. The integration is carried through the growth of the instability, beyond its saturation, and well into the stabilized plasma regime. A power spectrum computed for the electric field of the stabilized plasma is dominated by a narrow peak at the Bohm-Gross frequency of the unstable field mode but also contains significant power at the harmonics of the Bohm-Gross frequency. The harmonic power is in sharp peaks which are split into closely spaced doublets. The fundamental peak at the Bohm-Gross frequency is split into a closely spaced triplet. The mechanism for excitation of the second harmonic is shown to be second order wave-wave coupling.

Klimas, A. J.↗

A mechanism for plasma waves at the harmonics of the plasma frequency in the electron foreshock boundary

A bump-on-tail unstable reduced velocity distribution, constructed from data obtained at the upstream boundary of the electron foreshock by the GSFC electron spectrometer experiment on the ISEE-1 satellite, is used as the initial plasma state for a numerical integration of the 1D-Vlasov-Maxwell system of equations. The integration is carried through the growth of the instability, beyond its saturation, and well into the stabilized plasma regime. A power spectrum computed for the electric field of the stabilized plasma is dominated by a narrow peak at the Bohm-Gross frequency of the unstable field mode but also contains significant power at the harmonics of the Bohm-Gross frequency. The harmonic power is in sharp peaks which are split into closely spaced doublets. The fundamental peak at the Bohm-Gross frequency is split into a closely spaced triplet. The mechanism for excitation of the second harmonic is shown to be second order wave-wave coupling. Previously announced in STAR as N83-17315

Klimas, A. J.↗

A theoretical study of the excited states of Ag3

Recently there was considerable interest in the properties and reactivities of small metal clusters. However, for the transition metal trimers, gas phase spectroscopy exists only for Cu3. Calculations are reported for the excited states of the Ag3 molecule. The excitation energies, geometries, derived harmonic frequencies, and transition moments are presented. The electronic structure of these states is very similar to the analogous states of Cu3. From the VCI wave functions transition moments were calculated between each of the Rydberg excited states and the ground state for an equilateral triangle geometry with R sub Ag-Ag = 5.3 a sub 0. One state was computed for the configuration 4d29 5sa sup prime 2 sub 1 5se sup prime 1 sub x 5se sup prime 1 sub y. This configuration was considered since the corresponding configuration for Cu3 is low-lying. Calculations were carried out for a quartet wavefunction in which the 4d hole was localized on the central Ag atom. The spectrum for Ag3 is expected to be simpler than for Cu3 since the 5s2 4d9 states are shifted to higher energy.

Walch, Stephen P.↗

Time evolution from linear to nonlinear stages in magnetohydrodynamic parametric instabilities

The nonlinear evolution of the magnetohydrodynamic (MHD) parametric instability of wave fluctuations propagating along an unperturbed magnetic field is investigated. Both a magnetohydrodynamic perturbation-theoretical approach and a nonlinear MHD simulation are used. It is shown that high harmonic waves are rapidly excited by wave-wave coupling, and that the wave spectrum evolves from a state containing a small number of degrees of freedom in k space to one which contains a large number of degrees of freedom. It is found that the spectral evolution prior to nonlinear saturation is well described by the prturbation theory. During this stage, the ratio of the growth rate of the nth harmonic wave to the linear growth rate of the fundamental wave is n. The nonlinear saturation stage is characterized by a frequency shift of the fundamental wave that destroys the wave-wave resonance condition which, in turn, causes the wave amplitude to cease its growth.

Hoshino, M.↗

Low-frequency electromagnetic waves driven by gyrotropic gyrating ion beams

The origin of left- and right-hand-polarized low-frequency waves in space plasmas is analyzed. It has been shown that a gyrotropic gyrating ion beam, a ring in velocity space, can excite electromagnetic modes in the plasma near the beam gyrofrequency. It excites left-hand-polarized shear Alfven waves and their harmonics via the coupling of Alfven modes with the beam modes. It can also excite right-hand-polarized fast-mode magnetosonic waves and their harmonics as well. The excitation is possible for beam ions heavier than the plasma ions. The growth rate varies as one-third power of the beam density and decreases with the angle of wave propagation with respect to the ambient magnetic field. The nonlocality has a stabilizing effect on the instability. The predicted values of the wave frequencies compare reasonably well with those observed in satellite data.

Sharma, O. P.↗

Impact of toroidal magnetic field direction on integrated ELM-stable operation and divertor power exhaust via boron powder injection in EAST

We report the first in-depth comparison of the impact of toroidal magnetic field direction on solid boron injection used for Edge-Localized Mode (ELM) control, power exhaust, and core high-Z impurity control in the Experimental Advanced Superconducting Tokamak. With favorable ion ∇B drift towards the upper X-point in an upper-single-null configuration, boron injection effectively suppresses ELMs, produces a detachment of the inner divertor target, and leads to improved energy confinement. ELM suppression in this configuration is accompanied by the excitation of an Edge Harmonic Mode. In contrast, with unfavorable ion ∇B drift away from the upper X-point, boron injection also suppresses ELMs but leads to a more symmetric detachment state of both the inner and outer divertor targets, while plasma energy confinement is slightly degraded despite similar boron injection levels; a different low-frequency coherent mode without multiple harmonics is observed. Measurements from toroidally separated views show that the divertor response to boron injection is essentially toroidally symmetric, supporting the use of two-dimensional SOLPS-ITER modeling with a toroidally uniform impurity source. These experimental observations are qualitatively consistent with SOLPS-ITER simulations, which highlight the critical role of E × B drift effects in setting the Bt-dependent in–out asymmetry of detachment and in asymmetrically transporting particles and injected impurities within the scrape-off layer and private-flux region. These findings underscore the importance of drift physics and real-time wall conditioning in controlling low-Z impurity transport and optimizing edge solutions for integrated, ELM-stable, high-performance tokamak operation.

E × B drift↗

Comprehensive anisotropic linear optical properties of the Weyl semimetals TaAs and NbAs

We report that TaAs and NbAs are two of the earliest identified Weyl semimetals that possess many intriguing optical properties, such as chirality-dependent optical excitations and giant second harmonic generation (SHG). Linear and nonlinear optics have been employed as tools to probe the Weyl physics in these crystals. Here, we extend these studies to address two important aspects: determining the complete anisotropic dielectric response and exploring if and how they can reveal essential Weyl physics. We determine the complete anisotropic dielectric functions of TaAs and NbAs by combining spectroscopic ellipsometry and density functional theory (DFT). Parameterized Lorentz oscillators are reported from 1.2 - 6 eV (experiment) and 0 - 6 eV (DFT), and good agreement is shown between them. Both linear and nonlinear optical properties have been previously reported to reveal Weyl physics. We suggest that strong optical resonances from trivial bands are the likely origin of the large optical SHG previously reported at these energies. Furthermore, by comparing the contribution of a small k -space centered around the Weyl cones with the total linear dielectric function, we find that these contributions are highly anisotropic and are < 25% of the total dielectric function below 0.5 eV; abov1 eV, these contributions are negligible. Thus, the study of Weyl physics using optical techniques requires very low energies, and even there, a careful assessment is required in distinguishing the much smaller contributions of the Weyl bands from the dominant contributions of the trivial bands and Drude response to the total dielectric function.

36 MATERIALS SCIENCE↗

Hypersonic wake velocity measurements using acetone molecular tagging velocimetry

Molecular tagging velocimetry, a minimally intrusive laser diagnostic, was used to find quantitative off-body velocity measurements in the wake of both strut-mounted and free-flight spheres in hypersonic flow. Acetone gas seeded in the flow was excited using the fourth harmonic of a pulse-burst Nd:YAG laser. The experimental tests were validated and compared to simulations using a continuous Galerkin flow solver and an adaptive mesh refinement process. Near the centerline in the wake of the sphere, velocities between −105 and 65 m/s were observed due to reverse flow in the viscous shear layer. Similarly, the simulated data showed negative velocity values in the shear layer region. Outside of the shear layer, average velocities of 730 m/s were observed in both the experimental and simulated results. The overall average uncertainty for the strut-mounted and free-flight cases was estimated to have an accuracy of ±4% (±35.5m/s or 4.9%). In conclusion, this non-intrusive technique provides a velocity map of the wake behind a sphere under hypersonic conditions.

42 ENGINEERING↗

Center for Tokamak Transients Simulations

The major goals for the Center for Tokamak Transients Simulations (CTTS) were to develop detailed numerical simulations of disruptive transients in tokamak experiments and to use them in theoretical studies of the thermal-quench (TQ) and current-quench (CQ) phases of disruption. The University of Wisconsin-Madison component of CTTS contributed relevant development for the NIMROD code (https://nimrodteam.org) and applied it to disruptions that involve global vertical displacement. Code-development contributions include boundary conditions that represent sheath effects which occur when tokamak plasma is in contact with the surrounding vessel wall during vertical displacement events (VDEs). We also implemented a reduced model of energetic runaway electrons (REs) to simulate the effect of these energetic electrons on the CQ phase of tokamak disruptions. Our computations of VDEs include 2D and 3D verification through benchmarks with two other widely used macroscale plasma simulation codes, M3D-C1 and JOREK. Over nonlinear evolution to the final termination of plasma current, the 2D simulation results on magnetic axis location, toroidal current, and halo current track each other well. With the 3D benchmark computation, all three codes found the same qualitative behavior of the asymmetric instabilities having increasing growth rate after contact with the wall, followed by nonlinear excitation of other toroidal harmonics. Our NIMROD computations for an idealized configuration show agreement with an analytical assessment by V. D. Pustovitov [Nucl. Fusion 55, 113032 (2015)] that the plasma and non-ideal wall remain in force-balance such that net forces only result from magnetic stresses over the outer surface of the wall. Our study of the influence of boundary conditions on VDEs shows that extended-MHD simulations of VDEs are sensitive to electron energy transport to the wall and that boundary conditions on flow are only significant to the extent that they influence the electron energy transport. Resistive-MHD NIMROD simulations of the tokamak discharges in the Madison Symmetric Torus show that magnetic perturbations of poloidal wavenumber m=3 lead to chaotic magnetic topology over the edge region, which helps deconfine energetic electrons. A second area of RE study shows that the coupled resistive MHD/reduced RE model reproduces the resistive-hose particle-beam instability. With respect to educational opportunities, this effort involved and supported four graduate students at the University of Wisconsin-Madison and one postdoctoral associate. The results of this study have been disseminated through journal publications, conference presentations, technical reports, and PhD dissertations.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Hypersonic Wake Velocity Measurements Using Acetone Molecular Tagging Velocimetry

A non-intrusive laser diagnostic known as molecular tagging velocimetry was used to find quantitative off-body velocity measurements in the wake of a sphere in the Mach 7 Ludwieg Tube Wind Tunnel located at The University of Texas at San Antonio. Acetone gas seeded in the flow was excited using the 4th harmonic of a pulse-burst Nd:YAG laser. The experimental results were used to validate and compare to simulations using a continuous Galerkin flow solver. Both the experimental and simulated results agreed on negative velocities in the viscous shear layer. Near the centerline of the sphere, average velocities of -200 m/s were observed due to reverse flow in the recirculation region. Outside of the shear layer, velocities of 800 m/s were observed in both the experimental and simulated results. The overall average uncertainty for the strut-mounted and free-flight case was estimated to be ±27 m/s. The flow features of the wake were visualized using schlieren imaging, and the experimental results agreed well with the simulated results.

Shoemake, Lawton↗