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At least 127 records · Page 7

Rate and Gain Limitations of MSGC's and MGC's Combined with GEM and other Preamplification Structures

We have studied the rate and gain limits of diamond-coated Microstrip Gas Counters (MSGC's) and Micro-Gap Counters (MGC's) when combined with various preamplification structures: Gas Electron Multiplier (GEM), Parallel-Plate Avalanche Chamber (PPAC) or a MICROMEGAS-type structure. Measurements were done both with X rays and alpha particles with various detector geometries and in different gas mixtures at pressures from 0.05 to 10 atm. The results obtained varied significantly with detector design, gas mixture and pressure, but some general features can be identified. We found that in all cases, bare MSGC'S, MGC'S, PPAC's and MICROMEGAS, the maximum achievable gain drops with rate. The addition of preamplification structures significantly increases the gain of MSGC's and MGC'S, but this gain is still rate dependent. There would seem to be a general rate-dependent effect governing the usable gain of all these detectors. We speculate on possible mechanisms for this effect, and identify a safe, spark-free, operation zone for each system (detector + preamplification structure) in the rate-gain coordinate plane.

Fonte, P.↗

Path integral molecular dynamics: A high-fidelity approach to quantum dynamics of electrons

We investigate electron transport in the uniform electron gas using ring-polymer molecular dynamics (RPMD). Working in the weakly coupled, non-degenerate regime, we use RPMD to probe how the onset of quantum diffraction effects at high temperature reshapes electron–electron collisions and leads to a classical-to-quantum crossover in macroscopic transport properties. Static thermodynamics obtained with RPMD are consistent with the weak-coupling equation of state, confirming correct quantum Boltzmann sampling. Real-time transport extracted from mean square displacements exhibits the expected ballistic-to-diffusive transition and a systematic reduction of the electronic self-diffusivity as quantum effects strengthen, due to quantum diffraction modifying electron–electron collisions. Direct ring-polymer scattering simulations reveal diffractive “softening” of binary deflections, providing a micro-to-macro link between collision physics and diffusion. The present study establishes RPMD as a quantitative, trajectory-based tool for electron transport across the classical–quantum crossover and furnishes benchmarks for improving Coulomb-log interpolation models. We outline extensions to multi-component plasmas and a path to incorporate Fermi–Dirac statistics within path-integral dynamics.

Electronic transport↗

Many-Body Effects in Quantum-Well Intersubband Transitions

Intersubband polarization couples to collective excitations of the interacting electron gas confined in a semiconductor quantum well (Qw) structure. Such excitations include correlated pair excitations (repellons) and intersubband plasmons (ISPs). The oscillator strength of intersubband transitions (ISBTs) strongly varies with QW parameters and electron density because of this coupling. We have developed a set of kinetic equations, termed the intersubband semiconductor Bloch equations (ISBEs), from density matrix theory with the Hartree-Fock approximation, that enables a consistent description of these many-body effects. Using the ISBEs for a two-conduction-subband model, various many-body effects in intersubband transitions are studied in this work. We find interesting spectral changes of intersubband absorption coefficient due to interplay of the Fermi-edge singularity, subband renormalization, intersubband plasmon oscillation, and nonparabolicity of bandstructure. Our results uncover a new perspective for ISBTs and indicate the necessity of proper many-body theoretical treatment in order for modeling and prediction of ISBT line shape.

Li, Jian-Zhong↗

Electron Paramagnetic Resonance Imaging of the Spatial Distribution of Free Radicals in PMR-15 Polyimide Resins

Prior studies have shown that free radicals generated by heating polyimides above 300 C are stable at room temperature and are involved in thermo-oxidative degradation in the presence of oxygen gas. Electron Paramagnetic Resonance Imaging (EPRI) is a technique to determine the spatial distribution of free radicals. X-band (9.5 GHz) EPR images of PMR-15 polyimide were obtained with a spatial resolution of about 0.18 mm along a 2 mm dimension of the sample. In a polyimide sample that was not thermocycled, the radical distribution was uniform along the 2 mm dimension of the sample. For a polyimide sample that was exposed to thermocycling in air for 300 one-hour cycles at 335 C, one-dimensional EPRI showed a higher concentration of free radicals in the surface layers than in the bulk sample. A spectral-spatial two-dimensional image showed that the EPR lineshape of the surface layer remained the same as that of the bulk. These EPRI results suggest that the thermo-oxidative degradation of PMR-15 resin involves free radicals present in the oxygen-rich surface layer.

Ahn, Myong K.↗

Electron Paramagnetic Resonance Imaging of the Spatial Distribution of Free Radicals in PMR-15 Polyimide Resins

Prior studies have shown that free radicals generated by heating polyimides above 300 C are stable at room temperature and are involved in thermo-oxidative degradation in the presence of oxygen gas. Electron paramagnetic resonance imaging (EPRI) is a technique to determine the spatial distribution of free radicals. X-band (9.5 GHz) EPR images of PMR-15 polyimide were obtained with a spatial resolution of approximately 0.18 mm along a 2-mm dimension of the sample. In a polyimide sample that was not thermocycled, the radical distribution was uniform along the 2-mm dimension of the sample. For a polyimide sample that was exposed to thermocycling in air for 300 1-h cycles at 335 C, one-dimensional EPRI showed a higher concentration of free radicals in the surface layers than in the bulk sample. A spectral-spatial two-dimensional image showed that the EPR lineshape of the surface layer remained the same as that of the bulk. These EPRI results suggest that the thermo-oxidative degradation of PMR-15 resin involves free radicals present in the oxygen-rich surface layer.

Ahn, Myong K.↗

Electrons in the ionosphere of Titan

A theoretical model of the spatial and energy distribution of electrons in the ionosphere of Titan has been constructed using the two-stream electron transport method and the electron energy equation. The calculated electron spectra show abrupt decreases that can contribute to the 'bite-out' signature observed by the Voyager 1 plasma science instrument. Energy deposition rates in the exosphere of Titan by photoelectrons and magnetospheric electrons are calculated. Calculated N2 EUV airglow emission rates lead to the conclusion that airglow emission due to photoelectron impact is much more important than airglow emission due to magnetospheric electron interactions. Thermal electron temperatures at Titan are calculated for the first time. The electron gas remains well thermalized with the neutral atmosphere for radial distances from the center of Titan less than 3500 km. For radial distances beyond about 4000 km, energy transport dominates the energetics, and the electrons are almost isothermal along magnetic field lines.

Gan, L.↗

The equation of state for stellar envelopes. II - Algorithm and selected results

A free-energy-minimization method for computing the dissociation and ionization equilibrium of a multicomponent gas is discussed. The adopted free energy includes terms representing the translational free energy of atoms, ions, and molecules; the internal free energy of particles with excited states; the free energy of a partially degenerate electron gas; and the configurational free energy from shielded Coulomb interactions among charged particles. Internal partition functions are truncated using an occupation probability formalism that accounts for perturbations of bound states by both neutral and charged perturbers. The entire theory is analytical and differentiable to all orders, so it is possible to write explicit analytical formulas for all derivatives required in a Newton-Raphson iteration; these are presented to facilitate future work. Some representative results for both Saha and free-energy-minimization equilibria are presented for a hydrogen-helium plasma with N(He)/N(H) = 0.10. These illustrate nicely the phenomena of pressure dissociation and ionization, and also demonstrate vividly the importance of choosing a reliable cutoff procedure for internal partition functions.

Mihalas, Dimitri↗

N2O analysis in the atmosphere via electron capture-gas chromatography

The potential of commercially available pulse-modulated electron capture detector (ECD)-equipped gas chromatographs for direct measurement of ambient levels of N2O is assessed. Since the sensitivity of ECD to N2O is directly proportional to the detector operating temperature and detector standing current, it is necessary to use a 'hot' ECD (250-350 C). The method is shown to be very precise with a standard error not exceeding 1% for automated analysis of ambient air samples. The technology is available to permit highly accurate routine direct analysis of N2O in the troposphere and stratosphere. Both captured air samples or direct real-time measurement from research vessels or airborne platforms are possible.

Rasmussen, R. A.↗

Energy branching in the Io plasma torus - The failure of neutral cloud theory

Model calculations are used to explore the energy source characteristics of the energy branching of the hot Io plasma torus. It is assumed that the energy is derived from the kinetic energy acquired by ions created in the rotating planetary magnetic field, and that Coulomb collisions with the electron gas control the flow of energy to the ionizing and radiative processes. The results show that neutral cloud theory is qualitatively inadequate. It is shown that neutral cloud theory can only support a dominantly singly ionized system (at the measured electron densities in the plasma torus) and that it fails to predict observed plasma properties relative to variations in number density.

Shemansky, D. E.↗

A possible energy source to power stable auroral red arcs - Precipitating electrons

Results of coincident measurements by ground-based photometers and the low-altitude plasma instrument on board the Dynamics Explorer 2 satellite are presented that demonstrate the association of precipitating low-energy electrons with stable auroral red (SAR) arcs. A search of available data has yielded 23 instances of DE 2 overflights during the presence of SAR arcs being monitored by the photometers. For each case, downward fluxes of electrons are found to be enhanced along field lines penetrating the arcs in relation to regions both north and south of the features. Modeling of the atmospheric response to these influxes indicates that these electrons can represent a major source of the energy required to establish temperature profiles within the ionospheric electron gas that are sufficient to produce the recorded 6300-A emission rates. The sensitivity of these results to uncertainties of the assumed spacecraft potential and thermospheric composition has been investigated and found to be important, but does not alter the conclusion that precipitating electrons are a fundamental link in the production of SAR arcs.

Slater, D. W.↗

The atmosphere of a dirty-clathrate cometary nucleus - A two-phase, multifluid model

The dynamical and thermal structure of a dirty-clathrate cometary nucleus' gas atmosphere is presently given a self-consistent, transonic multifluid solution in which, although the heavy neutron and ion species are treated as a single fluid in the collision-dominated region, the photoproduced H is treated separately. The thermal profile of the atmosphere thus obtained is entirely different from those predicted by the earlier, single-fluid models as well as the multifluid models which assumed equipartition of energy between electrons and ions. While the electron gas, like the neutrals and the ions, cools due to expansion, its main mode of energy loss in the inner coma is by way of inelastic collisions with the predominant H2O molecule. The high electron temperature in the outer coma also decreases the efficiency of electron removal by dissociative recombination, thereby increasing electron density throughout the coma.

Marconi, M. L.↗

Relativistic plasmas

Recent work on the kinetic theory of a highly relativistic electron gas and the associated photon opacity is discussed. The relaxation time for thermalization by Moller scattering is compared with the characteristic times associated with various loss processes acting to perturb the distribution away from equilibrium. For an optically thin plasma, bremsstrahlung is found to dominate Moller scattering when the dimensionless electron temperature is greater than about 3.5. Results are presented for the opacity from Compton scattering, pair production in the fields of electrons and ions, inverse bremsstrahlung, and synchrotron self-absorption.

Gould, R. J.↗

Low-Noise Wide Bandwith, Hot Electron Bolometer Mixers for Submillimeter Wavelengths

Recently a novel superconductive hot-electron micro-bolometer has been proposed which is both fast and sensitive (D. E. Prober, Appl. Phys. Lett. 62, 2119, 1993). This device has several important properties which make it useful as a heterodyne sensor for radioastronomy applications at frequencies above 1 THz. The thermal response time of the device is fast enough, several 10's of picoseconds, to allow for IF's of several GHz. This bolometer mixer should operate well up to at least 10 THz. There is no energy gap limitation as in an SIS mixer, since the mixing process relies on heating of the electron gas. In fact, rf power is absorbed more uniformly above the gap frequency. The mixer noise should be near quantum-limited, and the local oscillator (LO) power requirement is very low: / 10 nW for a Nb device. One of the unique features of this device is that it employs rapid electron diffusion into a normal metal, rather than phonon emission, as the thermal conductance that cools the heated electrons. In order for diffusion to dominate over phonon emission, the device must be short, less than 0.5.

Bolometer Mixers↗

Evaluation and universal curves of the photon loss probability

In the transfer of radiation in a plasma, an important parameter (which measures the coupling between the radiation field and the electron gas) is the photon loss probability per scattering epsilon, defined as the ratio of collisional de-excitation to total de-excitation. The evaluation of epsilon requires normally knowledge of specific collisional excitation rates and radiative transition rate coefficients. In the considered investigation a general formula for epsilon is obtained which depends only on electron density, temperature, and line wavelength. Use is made of a simple Bethe-Coulomb expression recently derived by Kastner (1980) for the collisional excitation rate coefficient. Epsilon is obtained as a function of the three variables, and universal curves of it can be constructed with one of the variables as parameter. As an example of the application of the considered procedure, the variation of epsilon with height h in the solar atmosphere is shown in a graph for several solar lines.

Kastner, S. O.↗

Calculation of the electron wave function in a graded-channel double-heterojunction modulation-doped field-effect transistor

Three double-heterojunction modulation-doped field-effect transistor structures with different channel composition are investigated theoretically. All of these transistors have an In(x)Ga(1-x)As channel sandwiched between two doped Al(0.3)Ga(0.7)As barriers with undoped spacer layers. In one of the structures, x varies from 0 from either heterojunction to 0.15 at the center of the channel quadratically; in the other two, constant values of x of 0 and 0.15 are used. The Poisson and Schroedinger equations are solved self-consistently for the electron wave function in all three cases. The results showed that the two-dimensional electron gas (2DEG) concentration in the channel of the quadratically graded structure is higher than the x = 0 one and slightly lower than the x = 0.15 one, and the mean distance of the 2DEG is closer to the center of the channel for this transistor than the other two. These two effects have important implications on the electron mobility in the channel.

Mui, D. S. L.↗

Nonlinear transient neutralization theory of ion beams with dissipation

An analytical theory of nonlinear neutralization waves generated by injection of electrons from a grid in the direction of a homogeneous ion beam of uniform velocity and infinite extension is presented. The electrons are assumed to interact with the ions through the self-consistent space charge field and by strong collective interactions. The associated nonlinear boundary-value problem is solved in closed form by means of a von Mises transformation. It is shown that the electron gas moves into the ion space in the form of a discontinuous neutralization wave. This periodic wave structure is damped out by intercomponent momentum transfer, i.e., after a few relaxation lengths a quasi-neutral beam results. The relaxation scale in space agrees with neutralization experiments of rarefied ion beams, if the collective momentum transfer between the electron and ion streams is assumed to be of the Buneman type.

Wilhelm, H. E.↗

Nanoscale control of LaAlO 3 /SrTiO 3 conductance beyond the polar catastrophe

Conductive atomic force microscope (c-AFM) lithography can be utilized to create a wide range of LaAlO 3 /SrTiO 3 (LAO/STO)-based nanoelectronic devices in a reconfigurable manner. Experiments were generally performed with intrinsically insulating LAO/STO heterostructures, with LAO thickness less than the critical value at which a polar catastrophe takes place [<4 unit cell (u.c.)]. Here, we use inductively coupled plasma reactive ion etching (ICPRIE) to fabricate c-AFM “canvases” on intrinsically conducting LAO/STO samples with ≥4 u.c. LAO. We observe that its interfacial two-dimensional electron gas (2DEG) can be pinched off and then switched back on by c-AFM lithography. Nanowires created with initially conductive LAO/STO interfaces have an order-of-magnitude longer lifetime in ambient conditions, when compared to an identically created 3.4 u.c. LAO/STO nanowire. We also demonstrate key nanoscale properties such as ballistic transport in a quasi-one-dimensional electron waveguide at a 5 u.c. LAO/STO interface. This approach frees c-AFM-written nanodevice designs from time constraints in air associated with <4 u.c. LAO/STO heterostructures.

36 MATERIALS SCIENCE↗

Structural expansions for the ground state energy of a simple metal

A structural expansion for the static ground state energy of a simple metal is derived. An approach based on single particle band structure which treats the electron gas as a non-linear dielectric is presented, along with a more general many particle analysis using finite temperature perturbation theory. The two methods are compared, and it is shown in detail how band-structure effects, Fermi surface distortions, and chemical potential shifts affect the total energy. These are of special interest in corrections to the total energy beyond third order in the electron ion interaction, and hence to systems where differences in energies for various crystal structures are exceptionally small. Preliminary calculations using these methods for the zero temperature thermodynamic functions of atomic hydrogen are reported.

Hammerberg, J.↗