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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 127 records · Page 7
All sourcesNASA NTRSDOE OSTI
DOE OSTI2015

Decoupling Superconducting Qubits from the Quantum Bus/Readout Resonator to Enable Scaling

Superconducting qubits have made great strides in coherence time, gating, and algorithms. However, to achieve real scalability, more is required. We propose to study the problem of coupling and decoupling a transmon, a popular type of superconducting qubit, from its host resonator, which serves the dual role of a bus connecting qubits together and a readout channel. The transmon couples to its host resonator via its electric-dipole moment. We plan to use a trick of quantum mechanics to null the dipole moment and decouple the transmon. In doing so, we hope to study a variety of physics associated with multi-qubit operation, control, and readout.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2019

Early Career Award: Decoupling the Electronic and Geometric Parameters of Metal Nanocatalysts

Central in many industrial processes (e.g., petroleum refining) and the realization of new energy platforms (e.g., fuel cells and biomass conversion) is heterogeneous catalysis. The performance of a catalyst is governed by interplay between electronic and geometric factors, but controlling these parameters to achieve efficient catalysis remains a grand challenge. The overall goal of this project was to decouple the electronic and geometric parameters of nanoscale metal catalysts for independent manipulation through the design and use of new architecturally controlled bimetallic nanocrystals. Specifically, shape-controlled core@shell nanocrystals were studied as catalysts. The binary composition of these structures provided a means of electronic control while the shape of the nanocrystals provided geometric control. Through a series of experiments with nanocrystals of different shapes and bimetallic compositions, the electronic and geometric parameters of such metal nanocatalysts were effectively decoupled for independent manipulation of catalyst performance. These concepts were applied toward new nanocatalysts for semihydrogenation, formic acid electrooxidation and for the oxygen reduction reaction. Ultimately, with the development of new synthetic strategies toward bimetallic nanocrystals, this research has advanced the design and synthesis of bimetallic nanocrystals as catalysts for diverse chemical transformations.

36 MATERIALS SCIENCE↗
DOE OSTI2023

Flexible Fully-Decoupled Nuclear Plants with Thermal Energy Storage - Technoeconomic Optimization

New nuclear power plants may be one of the technologies for future zero carbon electricity production. These future systems will however also need significant flexibility to cope with fluctuating demand and large share of intermittent renewable supply, rather than running in conventional baseload generation. The present work explores the use of thermal energy storage (TES) as a buffer between the reactor heat and its conversion to electricity, enabling flexible operation of nuclear plants. The focus is on maximizing flexibility, ideally as full decoupling of the nuclear and power cycle islands, as well as on system efficiency in various modes. A system design presented for a high temperature gas cooled reactor (HTGR) presents a slightly complex solution, as separate high- and low-temperature TES systems are required in order to cover the extended temperature range. Although this configuration imposes certain limitations on the discharge system configuration, it also presents the opportunity to design a more efficient system. For this case in particular, a steam reheat cycle is advantageous. Dynamic models were developed for the decoupled system in order to generate insights into aspects of off design operation and system control. A technoeconomic analysis, furthermore, provides sizing and costing of the component, followed by size and dispatch economic optimization considering energy arbitrage. This optimization shows that in all explored markets, the addition of TES system with the proposed configuration results in positive impact on project net present value. Further sensitivity analyses show impact of multiple inputs and possible technical limitations.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗
DOE OSTI2014

Centrifugally decoupling touchdown bearings

Centrifugally decoupling mechanical bearing systems provide thin tensioned metallic ribbons contained in a support structure. This assembly rotates around a stationary shaft being centered at low speeds by the action of the metal ribbons. Tension springs are connected on one end to the ribbons and on the other end to the support structure. The ribbons pass through slots in the inner ring of the support structure. The spring preloading thus insures contact (or near-contact) between the ribbons and the shaft at rotation speeds below the transition speed. Above this speed, however, the centrifugal force on the ribbons produces a tensile force on them that exceeds the spring tensile force so that the ribbons curve outward, effectively decoupling them from mechanical contact with the shaft. They still remain, however, in position to act as a touchdown bearing in case of abnormally high transverse accelerations.

42 ENGINEERING↗
DOE OSTI2021

Systems and methods of decoupled hydrogen generation using energy-bearing redox pairs

Described herein are systems and methods of hydrogen generation and electrolyte regeneration as independent operations in separate redox flow cells. The operations can be decoupled by using an energy-bearing redox pair that electrochemically bears energy facilitating flexible, efficient hydrogen generation. In one example, the hydrogen generation redox flow cell can include a liquid, energy-bearing electrolyte solution in which at least one species of an energy-bearing redox pair is dissolved, to decouple the hydrogen evolution reaction from the reaction at the opposite electrode (e.g., the oxygen evolution reaction of conventional direct water electrolysis). Each species of the energy-bearing redox pair is associated with a standard electrode potential within the water electrolysis window.

Wang, Wei↗
DOE OSTI2021

Load-decoupling attachment system

A load-decoupling attachment system is configured to secure a component to a primary structure. The load-decoupling system includes a fore end coupling bracket that is configured to attach to a fore end of the component. A first tie rod is coupled to the fore end coupling bracket. The first tie rod is configured to couple to a first portion of the primary structure. A second tie rod is coupled to the fore end coupling bracket. The second tie rod configured to couple to a second portion of the primary structure. A universal joint mount assembly is configured to couple to an aft end of the component and a third portion of the primary structure.

Weathers, Jeffrey W.↗
DOE OSTI2026

Dissipation Enables Strongly Detuning-Dependent Interference in Pulsed Dynamical Decoupling

One of the defining features of pulsed dynamical decoupling is its suppression of a driven qubit's sensitivity to static detuning errors between the drive field and qubit resonance. In this paper, we show that dissipation, in the form of excited-state decay, can change this behavior entirely, producing an interference signal with a strong detuning dependence. This signal arises from decay during driven evolution and relies on coherence retained by the qubit after such a decay event. We develop analytical and numerical models that capture the underlying mechanism and observe this same dissipation-induced detuning dependence experimentally in both a free-space strontium atom interferometer and a superconducting transmon qubit system. We also use this dissipation-induced detuning dependence as the basis for a new spectroscopic technique called Dissipative Carr-Purcell Spectroscopy (DCPS) and compare it with a traditional Ramsey sequence. Our results establish a regime of pulsed dynamical decoupling in which dissipation reshapes, rather than merely degrades, coherent control, and we expect these dynamics to be relevant to a wide range of quantum systems.

DeRose, Kenneth [Northwestern U.; Fermilab] (ORCID↗
DOE OSTI2012

Apparent Decoupling of the Dynamics of a Protein from the Dynamics of its Aqueous Solvent

Studies of the low-temperature dynamics of proteins in aqueous solutions are limited by the crystallization of water. In this work, we use a solution of LiCl in D{sub 2}O as a solvent for a protein to prevent crystallization and study the dynamics of both the protein and its aqueous solvent by quasielastic neutron scattering (QENS) in the temperature range of 210 to 290 K. Our results reveal that, while the dynamics of the aqueous solvent undergoes a crossover at about 220 K, the dynamics of the protein itself shows no transition at this temperature. The prevailing view is that the {beta}-fluctuations of the protein are governed by the {alpha}-fluctuations of the solvent; therefore, observation of the apparent decoupling between the dynamics of the protein and its solvent below the crossover temperature is remarkable.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2011

Electron spin decoherence in nuclear spin baths and dynamical decoupling

We introduce the quantum theory of the electron spin decoherence in a nuclear spin bath and the dynamical decoupling approach for protecting the electron spin coherence. These theories are applied to various solid-state systems, such as radical spins in molecular crystals and NV centers in diamond.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2014

Decoherence suppression combining quantum uncollapsing and dynamical decoupling

We demonstrate a protocol, that combines quantum uncollapsing and dynamical decoupling, to protect the quantum state stored in a qubit against decoherence errors. The protocol can simultaneously suppress the two kinds of decoherence processes: the energy relaxation and the low-frequency noise induced dephasing. We present the analytical derivation and numerical simulations in detail. We also provide a preliminary experimental test in superconducting phase qubits, using the process fidelity to calibrate the performance of the protocol. Our results suggest that the protocol can be effective against errors due to both energy relaxation and the low-frequency dephasing noise, except at a reduced probability of success.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2014

Novel type of chimera spiral waves arising from decoupling of a diffusible component

Spiral waves composed of coherent traveling waves surrounding a core containing stochastically distributed stationary areas are found in numerical simulations of a three-variable reaction-diffusion system with one diffusible species. In the spiral core, diffusion of this component (w) mediates transitions between dynamic states of the subsystem formed by the other two components, whose dynamics is more rapid than that of w. Diffusive coupling between adjacent sites can be “on” or “off” depending on the subsystem state. The incoherent structures in the spiral core are produced by this decoupling of the slow diffusive component from the fast non-diffusing subsystem. The phase diagram reveals that the region of incoherent behavior in chimera spirals grows drastically, leading to modulation and breakup of the spirals, in the transition zones between 1{sup n-1} and 1{sup n} local mixed-mode oscillations.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2014

Universal construction of controlled-unitary gates using dynamical decoupling and the quantum Zeno effect

We present two new algorithms that universally construct a quantum circuit approximating a controlled-U(t) up to a global phase factor of U(t), denoted by Λ{sub θ}U(t), where U(t) = e{sup −iHt} is the unitary evolution operator of an unknown Hamiltonian H of the system, and is given as a black box with tunable parameter t. We show that it is possible to approximately construct Λ{sub θ}U(t) with arbitrarily high accuracy. This algorithm is based on the dynamical decoupling effect [1]. If another black box consisting of a time-inverted version of U(t), namely U(−t), is also available we can implement Λ{sub θ}U(t) exactly with arbitrarily high success probability. This algorithm is based on the quantum Zeno effect.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2015

Decoupling of epitaxial graphene via gold intercalation probed by dispersive Raman spectroscopy

Signatures of a superlattice structure composed of a quasi periodic arrangement of atomic gold clusters below an epitaxied graphene (EG) layer are examined using dispersive Raman spectroscopy. The gold-graphene system exhibits a laser excitation energy dependant red shift of the 2D mode as compared to pristine epitaxial graphene. The phonon dispersions in both the systems are mapped using the experimentally observed Raman signatures and a third-nearest neighbour tight binding electronic band structure model. Our results reveal that the observed excitation dependent Raman red shift in gold EG primarily arise from the modifications of the phonon dispersion in gold-graphene and shows that the extent of decoupling of graphene from the underlying SiC substrate can be monitored from the dispersive nature of the Raman 2D modes. The intercalated gold atoms restore the phonon band structure of epitaxial graphene towards free standing graphene.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2016

Decoupling ion conductivity and fluid permeation through optimizing hydrophilic channel morphology

Approaches to improve membrane ion conductivity usually leads to higher degree of swelling, more serious fuel cross-over and often sacrificed membrane mechanical strength. Preserving all three main membrane properties is a tough challenge in searching high ion conducting fuel cell membrane. The long standing dilemma is resolved by decoupling ion conduction and fluid permeation property by creating optimized channel morphology using external electric field poling. Success of this approach is demonstrated in the proton conducting membrane composed of poly(ether sulfones) (PES) and sulfonated poly(ether ether ketone) (sPEEK, degree of sulfonation=50%) composites prepared under electric field poling condition. The external field enhanced the aromatic chain ordering from both sPEEK and PES and improved the miscibility. This induced interaction is conducive to the formation of more densely packed amorphous domains that eventually leads to preferentially ordered hydrophilic proton conducting channels having a average dimension (3 nm) smaller than that in generic sPEEK or Nafion. The narrower but more ordered channel displayed much lower methanol permeability (3.17×10{sup −7} cm{sup 2}/s), and lower swelling ratio (31.20%), while the conductivity (~10{sup −1} S/cm) is higher than that of Nafion, or sPEEK at higher (64%) degree of sulfonation. The composite is chemically stable and highly durable with improved membrane mechanical strength. Nearly 50% increase of DMFC power output is observed using this membrane, and the best power density is recorded at 155 mA/cm{sup 2} (80 °C, 1M Methanol).

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2013

DECOUPLING PHASE VARIATIONS IN MULTI-PLANET SYSTEMS

Due to the exquisite photometric precision, transiting exoplanet discoveries from the Kepler mission are enabling several new techniques of confirmation and characterization. One of these newly accessible techniques analyzes the phase variations of planets as they orbit their stars. The predicted phase variation for multi-planet systems can become rapidly complicated and depends upon the period, radius, and albedo distributions for planets in the system. Here we describe the confusion that may occur due to short-period terrestrial planets and/or non-transiting planets in a system, which can add high-frequency correlated noise or low-frequency trends to the data stream. We describe these sources of ambiguity with several examples, including that of our solar system. We further show how decoupling of these signals may be achieved with application to the Kepler-20 and Kepler-33 multi-planet systems.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2014

The effective gravitational decoupling between dark matter and the CMB

e present a detailed and self-contained analytical derivation of the evolution of sub-horizon cosmological perturbations before decoupling, based on previous work by S. Weinberg. These solutions are valid in the minimal ΛCDM scenario, to first order in perturbation theory, in the tight-coupling limit and neglecting neutrino shear stress. We compare them to exact numerical solutions computed by a Boltzmann code, and we find the two to be in very good agreement. The analytic solutions show explicitly that CDM and the baryon-photon fluid effectively behave as separate self-gravitating fluids until the epoch of baryon drag. This in turn leads to the surprising conclusion that the CMB is much less sensitive to the clustering properties of minimally coupled Dark Matter models than what would be naively expected.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2016

Relic neutrino decoupling with flavour oscillations revisited

We study the decoupling process of neutrinos in the early universe in the presence of three-flavour oscillations. The evolution of the neutrino spectra is found by solving the corresponding momentum-dependent kinetic equations for the neutrino density matrix, including for the first time the proper collision integrals for both diagonal and off-diagonal elements. This improved calculation modifies the evolution of the off-diagonal elements of the neutrino density matrix and changes the deviation from equilibrium of the frozen neutrino spectra. However, it does not vary the contribution of neutrinos to the cosmological energy density in the form of radiation, usually expressed in terms of the effective number of neutrinos, N{sub eff}. We find a value of N{sub eff}=3.045, in agreement with previous theoretical calculations and consistent with the latest analysis of Planck data. This result does not depend on the ordering of neutrino masses. We also consider the effect of non-standard neutrino-electron interactions (NSI), predicted in many theoretical models where neutrinos acquire mass. For two sets of NSI parameters allowed by present data, we find that N{sub eff} can be reduced down to 3.040 or enhanced up to 3.059.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2011

Symmetry-enhanced performance of dynamical decoupling

We consider a system with general decoherence and a quadratic dynamical decoupling sequence (QDD) for the coherence control of a qubit coupled to a bath of spins. We investigate the influence of the geometry and of the initial conditions of the bath on the performance of the sequence. The overall performance is quantified by a distance norm d. It is expected that d scales with {tau}, the total duration of the sequence, as {tau}{sup min{l_brace}N{sub x},N{sub z}{r_brace}+1}, where N{sub x} and N{sub z} are the number of pulses of the outer and of the inner sequence, respectively. We show both numerically and analytically that the state of the bath can boost the performance of QDD under certain conditions: The scaling of QDD for a given number of pulses can be enhanced by a factor of 2 if the bath is prepared in a highly symmetric state and if the system Hamiltonian is SU(2) invariant.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗